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Magnetothermopower in high-mobility 2D electron gas: effect of microwave irradiation Oleg Raichev Department of Theoretical Physics Institute of Semiconductor Physics, Kiev, Ukraine [email protected]
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Magnetothermopower in high-mobility 2D electron gas: effect of microwave irradiation Oleg Raichev Department of Theoretical Physics Institute of Semiconductor.

Jan 17, 2016

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Page 1: Magnetothermopower in high-mobility 2D electron gas: effect of microwave irradiation Oleg Raichev Department of Theoretical Physics Institute of Semiconductor.

Magnetothermopower in high-mobility 2D electron gas:

effect of microwave irradiation

Oleg Raichev

Department of Theoretical PhysicsInstitute of Semiconductor Physics, Kiev, Ukraine

[email protected]

Page 2: Magnetothermopower in high-mobility 2D electron gas: effect of microwave irradiation Oleg Raichev Department of Theoretical Physics Institute of Semiconductor.

displacement inelastic

MIRO in high-mobility 2D electron gas in magnetic field. Photon-assisted electron scattering in the regime of Landau quantization.

Page 3: Magnetothermopower in high-mobility 2D electron gas: effect of microwave irradiation Oleg Raichev Department of Theoretical Physics Institute of Semiconductor.

MIRO in high-mobility 2D electron gas in magnetic field. Photon-assisted electron scattering in the regime of Landau quantization.

What about transport coefficients other than resistance? The same mechanisms are involved.

Motivation: 1. Search for new effects 2. Verification of theoretical conceptsLet us study the magnetothermoelectric phenomena!

displacement inelastic

Page 4: Magnetothermopower in high-mobility 2D electron gas: effect of microwave irradiation Oleg Raichev Department of Theoretical Physics Institute of Semiconductor.

OutlineOutline

Brief review of thermoelectric physics and experimental studies of thermopower in 2D systems.

What is expected under microwave irradiation?Theoretical approach to the problem of thermoelectric

current and thermopower in the presence of microwaves.Presentation of results, discussion, conclusions.

Page 5: Magnetothermopower in high-mobility 2D electron gas: effect of microwave irradiation Oleg Raichev Department of Theoretical Physics Institute of Semiconductor.

Seebeck (1821)Longitudinal thermovoltage

Nernst, EttingshausenTransverse thermovoltage

TT j

T ˆˆEj

1ˆˆ,ˆˆˆ,ˆ0 TEj

(V/K) er tensor thermopow theis

xxtrcxyyxxxyy )(~, symmetrysimilar have ˆ andˆ

V

Page 6: Magnetothermopower in high-mobility 2D electron gas: effect of microwave irradiation Oleg Raichev Department of Theoretical Physics Institute of Semiconductor.

Two mechanisms

F

Te

ˆ

||3ˆ

2 Mott relation Degenerate electron gasQuasi-equilibrium

TTems

phtrph

,||E Effective “electric field”

Diffusive

Phonon drag

xxtrcxyyxxxyy )(, (diagonal) 1~ˆˆˆ 1

Quantum magnetotransport: Shubnikov-de Haas oscillations.

phim JJf

ce

eTT

fpp

pp

pp p

BvEv

][

For 2D electrons phonon drag dominates at T> 0.5 K (experiments in GaAs QWs)

Page 7: Magnetothermopower in high-mobility 2D electron gas: effect of microwave irradiation Oleg Raichev Department of Theoretical Physics Institute of Semiconductor.

J. Zhang, et al. PRL 92, 156802 (2004)GaAs,x 106 cm2/Vs

Longitudinal thermopower

SdH oscillations at B>0.5 T

cFph nspqs 2

Magnetophonon oscillations (similar to PIRO in resistance).Mechanism: resonant phonon-assisted backscattering of electrons.

MIRO are observed in samples of similar mobility in the same region of magnetic fields

Page 8: Magnetothermopower in high-mobility 2D electron gas: effect of microwave irradiation Oleg Raichev Department of Theoretical Physics Institute of Semiconductor.

Under MW irradiation

1. 2DEG is far away from equilibrium: distribution function is strongly modified near Fermi energy.Violation of Mott relation for diffusive mechanism.Additional terms in thermopower appear in the quantum transport regime.

Page 9: Magnetothermopower in high-mobility 2D electron gas: effect of microwave irradiation Oleg Raichev Department of Theoretical Physics Institute of Semiconductor.

Under MW irradiation

1. 2DEG is far away from equilibrium: distribution function is strongly modified near Fermi energy.Violation of Mott relation for diffusive mechanism.Additional terms in thermopower appear in the quantum transport regime.

2. Influence of MWs on electron-phonon interaction: combined phonon- and photon-assisted scattering.Contribution of phonon drag mechanism is modified. Picture of quantum oscillations is changed (combined resonances).

Page 10: Magnetothermopower in high-mobility 2D electron gas: effect of microwave irradiation Oleg Raichev Department of Theoretical Physics Institute of Semiconductor.

Under MW irradiation

1. 2DEG is far away from equilibrium: distribution function is strongly modified near Fermi energy.Violation of Mott relation for diffusive mechanism.Additional terms in thermopower appear in the quantum transport regime.

2. Influence of MWs on electron-phonon interaction: combined phonon- and photon-assisted scattering.Contribution of phonon drag mechanism is modified. Picture of quantum oscillations is changed (combined resonances).

3. Polarization of MW field is a source of transport anisotropy. Symmetry of thermopower tensor is changed. Sensitivity to polarization.

Page 11: Magnetothermopower in high-mobility 2D electron gas: effect of microwave irradiation Oleg Raichev Department of Theoretical Physics Institute of Semiconductor.

Under MW irradiation

1. 2DEG is far away from equilibrium: distribution function is strongly modified near Fermi energy.Violation of Mott relation for diffusive mechanism.Additional terms in thermopower appear in the quantum transport regime.

2. Influence of MWs on electron-phonon interaction: combined phonon- and photon-assisted scattering.Contribution of phonon drag mechanism is modified. Picture of quantum oscillations is changed (combined resonances).

3. Polarization of MW field is a source of transport anisotropy. Symmetry of thermopower tensor is changed. Sensitivity to polarization.

4. Since the drift current compensates thermoelectric current, longitudinalresistivity, which is strongly modified by MWs, enters the thermopower. MIRO can be seen in transverse thermopower.

)0()0()0(

2

)(

]1)[(

xyxxxxxyxyxxxxxyxy

trcyxxyxxxxyxxyxx

Page 12: Magnetothermopower in high-mobility 2D electron gas: effect of microwave irradiation Oleg Raichev Department of Theoretical Physics Institute of Semiconductor.

Theoretical approach

Quantum Boltzmann equation

approximations: overlapping Landau levels, neglect of SdH oscillations

ˆˆˆ TT j

Page 13: Magnetothermopower in high-mobility 2D electron gas: effect of microwave irradiation Oleg Raichev Department of Theoretical Physics Institute of Semiconductor.

Dark thermopower results (phonon drag only):

scattering anglepolar angle of phonon wave vector (in 2D plane)inclination angle of phonon wave vector

B-independent (classical TP)

c1: oscillating with B (quantum TP)

Page 14: Magnetothermopower in high-mobility 2D electron gas: effect of microwave irradiation Oleg Raichev Department of Theoretical Physics Institute of Semiconductor.

Calculated dark thermopower (both mechanisms included)

Magnetophonon oscillations both in longitudinal and transverse TP

Amplitude increases until Bloch-Gruneisen temperature is reached

Page 15: Magnetothermopower in high-mobility 2D electron gas: effect of microwave irradiation Oleg Raichev Department of Theoretical Physics Institute of Semiconductor.

MW-induced longitudinal thermopower

inelastic and displacement mechanisms (the same as in resistance)

b describes MW polarization effect

polarization anglep – radiative decay rate

Page 16: Magnetothermopower in high-mobility 2D electron gas: effect of microwave irradiation Oleg Raichev Department of Theoretical Physics Institute of Semiconductor.

Calculated MW-induced longitudinal thermopowerinelastic mechanism displacement mechanism

Page 17: Magnetothermopower in high-mobility 2D electron gas: effect of microwave irradiation Oleg Raichev Department of Theoretical Physics Institute of Semiconductor.

Calculated MW-induced longitudinal thermopowerinelastic mechanism displacement mechanism

Effect of MW on TP is small compared to effect on resistance

impurity-assisted (resistance) phonon-assisted (TP)fixed transition energy average over phonon energies

Page 18: Magnetothermopower in high-mobility 2D electron gas: effect of microwave irradiation Oleg Raichev Department of Theoretical Physics Institute of Semiconductor.

MW-induced transverse thermopower

T

Ej

T

j

xV

E T T

E

xV

yV

Polarization-dependent term in transverse TP is of dissipationless nature. MW-induced anisotropy Dissipationless thermoinduced current is not perpendicular to

no MW with MW

T

Page 19: Magnetothermopower in high-mobility 2D electron gas: effect of microwave irradiation Oleg Raichev Department of Theoretical Physics Institute of Semiconductor.

Calculated MW-induced transverse thermopower

Small T and B : mostly MIRO in transverse TPHigher T and B: polarization dependent transverse TP

For higher mobility the polarization dependent part is more important

dash: dark thermopower

Page 20: Magnetothermopower in high-mobility 2D electron gas: effect of microwave irradiation Oleg Raichev Department of Theoretical Physics Institute of Semiconductor.

Amplitude of polarization dependent term in transverse thermopower

Page 21: Magnetothermopower in high-mobility 2D electron gas: effect of microwave irradiation Oleg Raichev Department of Theoretical Physics Institute of Semiconductor.

Conclusions Conclusions

Magnetophonon oscillations due to phonon drag are present

both in longitudinal and transverse TP.

Microwave irradiation adds quantum corrections to TP tensor. Relative changes are small for longitudinal TP and large for transverse TP.

MIRO can be observed in the transverse TP. Transverse TP, unlike the resistance, is strongly sensitive to

linear polarization of microwaves.

Experimental studies are desirable

A theory is developed to describe effects of Landau quantization in thermopower (TP) both without and with MW irradiation

Page 22: Magnetothermopower in high-mobility 2D electron gas: effect of microwave irradiation Oleg Raichev Department of Theoretical Physics Institute of Semiconductor.

Thank you for the attention Thank you for the attention

Page 23: Magnetothermopower in high-mobility 2D electron gas: effect of microwave irradiation Oleg Raichev Department of Theoretical Physics Institute of Semiconductor.

incident Et(i) : linear polarization in plane Et : elliptical polarization

MWEt(i)

Et

2D plane

Description of microwave field

polarization anglep – radiative decay rate

Page 24: Magnetothermopower in high-mobility 2D electron gas: effect of microwave irradiation Oleg Raichev Department of Theoretical Physics Institute of Semiconductor.

3D phonon model

spatially anisotropic phonon distribution

Expressions for collision integrals

Page 25: Magnetothermopower in high-mobility 2D electron gas: effect of microwave irradiation Oleg Raichev Department of Theoretical Physics Institute of Semiconductor.

Thermoelectric tensor (phonon-drag)

Thermoelectric tensor (diffusive)

Page 26: Magnetothermopower in high-mobility 2D electron gas: effect of microwave irradiation Oleg Raichev Department of Theoretical Physics Institute of Semiconductor.