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LA BASE DE DONNEES SPECTROSCOPIQUES GEISA : version actuelle et mise à jour 2007 N. Jacquinet-Husson, R. Armante, N.A. Scott, A. Chédin Laboratoire de Météorologie Dynamique Atmospheric Radiation Analysis Group Ecole Polytechnique 91128, Palaiseau, France http://ara.lmd.polytechnique.fr
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LA BASE DE DONNEES SPECTROSCOPIQUES N. Jacquinet …ara.abct.lmd.polytechnique.fr/htdocs-public/oral_pub/2007/icsa07... · GEISA-03 Associated Institutions and Co-Authors BIRA/IASB

Nov 09, 2018

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Page 1: LA BASE DE DONNEES SPECTROSCOPIQUES N. Jacquinet …ara.abct.lmd.polytechnique.fr/htdocs-public/oral_pub/2007/icsa07... · GEISA-03 Associated Institutions and Co-Authors BIRA/IASB

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LA BASE DE DONNEES SPECTROSCOPIQUES GEISA : version actuelle et mise à jour 2007

N. Jacquinet-Husson,R. Armante, N.A. Scott,

A. Chédin

Laboratoire de Météorologie DynamiqueAtmospheric Radiation Analysis Group

Ecole Polytechnique91128, Palaiseau, France

http://ara.lmd.polytechnique.fr

Page 2: LA BASE DE DONNEES SPECTROSCOPIQUES N. Jacquinet …ara.abct.lmd.polytechnique.fr/htdocs-public/oral_pub/2007/icsa07... · GEISA-03 Associated Institutions and Co-Authors BIRA/IASB

� �� �� �� �� �� �� �� ���� �� �� � ��� � ��� � ��� � � �� �� � � �� �� � � �� �� � � �� �� � � �� �� �� � �� �� � ��� � �� �� � ��� � �� �� � ��� � �� �� � �

GEISA-03 Associated Institutions and Co-Authors

BIRA/IASB Belgian Institute for Space Aeronomy A. C. VandaeleDLR, Deutsches Zentrum für Luft und raumfahrt (Germany) M. Birk, F. Schreier, G. WagnerFord Motor Company M. D. HurleyGSMA, Groupe de Spectrométrie Moléculaire et Atmosphérique (France) A. Barbe, L. Daumont, M.R.

Debacker-Barilly, A. Hamdouni, L. Régalia-Jarlot, V.G. TyuterevHarvard Smithonian Center for Astrophysics (USA) K. ChanceIAO, Institute of Atmospheric Optics (Russia) A. A. Chursin, S. N. Mikhailenko, S. A. TashkunJPL, Jet Propulsion Laboratory (USA) L.R. Brown, R.A. TothLITMS, Laboratory for Information Technologies and Mathematical Simulation (Russia) A. RublevLPMAA, Laboratoire de Physique Moléculaire pour l’Atmosphère et l’Astrophysique (France) V. Dana,

J.Y. Mandin, J.L. Teffo, C. Claveau, D. JacquemartLISA, Laboratoire Inter-Universitaire des Systèmes Atmosphériques (France) J.M. Flaud, I. Kleiner, J.

Orphal, A. PerrinMax Plank Institut für Meteorologie, Hamburg (Germany) L. SchultMeteorologisches Institut der Universität München (Germany) M. Hess, K. KöpkeNASA Langley Research Center C. P. RinslandNCAR, National Center for Atmospheric Research (USA) S. MassieRAL, Rutherfford Appleton Laboratory (UK) D. Newham, K.M. SmithState University of New-York at Stony Brook (USA) V. Nemtchinov, P. VaranasiULB, Université Libre de Bruxelles (Belgique) C. Clerbaux, P.F. Coheur, J. Vander – Auwera, S. FallyUniversity of Bologna (ITALY) G. Di LonardoUniversity of Denver (USA) A. Goldman

19 institutions41 co-authors

Page 3: LA BASE DE DONNEES SPECTROSCOPIQUES N. Jacquinet …ara.abct.lmd.polytechnique.fr/htdocs-public/oral_pub/2007/icsa07... · GEISA-03 Associated Institutions and Co-Authors BIRA/IASB

� �� �� �� �� �� �� �� ���� �� �� � ��� � ��� � ��� � � �� �� � � �� �� � � �� �� � � �� �� � � �� �� �� � �� �� � ��� � �� �� � ��� � �� �� � ��� � �� �� � �

OUTLINE

GEISA and GEISA/IASI System Overview- GEISA-03 line transition parameters sub-database- GEISA-03 IR cross-sections sub-database- GEISA-03 UV/VIS cross-sections sub-database

- GEISA-03 and GEISA/IASI common aerosols sub-database

GEISA and GEISA/IASI Interactive UseImplementation of the databases on the Ether Products and Data Center

(CNES/CNRS)

GEISA and Planetary Atmosphere Studies

GEISA 2007 Archive in Preparation:line transition parameter sub-database

Concluding Comments

Page 4: LA BASE DE DONNEES SPECTROSCOPIQUES N. Jacquinet …ara.abct.lmd.polytechnique.fr/htdocs-public/oral_pub/2007/icsa07... · GEISA-03 Associated Institutions and Co-Authors BIRA/IASB

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MORE RECENT REFERENCES

Jacquinet-Husson N. et al. The GEISA spectroscopic database system revisited for IASI direct radiative transfer modelling. Atmospheric and Oceanic Optics. 16, No.3, 256-82, 2003.

Jacquinet-Husson N. et al. A spectroscopic database system for the second generation vertical sounders radiance simulation. Proceedings of the 13th International TOVS Study Conference, Sainte-Ad�le, Canada ; 28 October � 4 November 2003.

Jacquinet-Husson N. et al. The 2003 edition of the GEISA/IASI spectroscopic database.JQSRT, 95, 429-67, 2005.

Page 5: LA BASE DE DONNEES SPECTROSCOPIQUES N. Jacquinet …ara.abct.lmd.polytechnique.fr/htdocs-public/oral_pub/2007/icsa07... · GEISA-03 Associated Institutions and Co-Authors BIRA/IASB

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Extraction of GEISA-03 between 599 & 3001 cm-1

Individual spectral lines spectroscopic parameters sub-database14 molecules (53 isotopic species): H2O, CO2, O3, N2O, CO, CH4, O2, NO, SO2, NO2, HNO3, OCS, C2H2, N2

IR absorption cross-sections sub-database (mainly CFC’s)6 molecular species: CFC-11, CFC-12, CFC-14, CCl4, N2O5, HCFC-22

Microphysical and optical properties of Basic Atmospheric aerosol components sub-database (similar with the GEISA-03 one)

GEISA/IASI database general context

IASI : Infrared Atmospheric Sounder Interferometer AIRS : Advanced InfraRed SounderISSWG : IASI Sounding Science Working Group CNES : Centre National d’Etudes Spatiales, FranceEUMETSAT : EUropean organization for the exploitation of METeorological SATellites

Continuous update

Related with:CNES/EUMETSAT EPS missionIASI measurement capabilities assessmentISSWG

Associated interest for AIRS

Total # entries:

702,550

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GEISA-03 line transition parameters sub-database

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����� � � �� � � � � � � � � �� � � � � � � � � � � � � � � �� �7777"""" ' 8' 8' 8' 8 """"7' 0 77' 0 77' 0 77' 0 7""""9999

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�� �� � � �� � � � � � � � � �� � � � � � � � � � � � � � � � � �� �7777#### ' 0 8' 0 8' 0 8' 0 8 ���� ' :' :' :' : """"7' 0 7�7' 0 7�7' 0 7�7' 0 7� 9999

� ��� � � � �� � � � � � � � � � � � � � � � � � � � � � � �� �: 7' � �7: 7' � �7: 7' � �7: 7' � �7"""" ' : 7' : 7' : 7' : 7"""" ' : 8' : 8' : 8' : 8 #### ' � 8 : 7' � 8 : 7' � 8 : 7' � 8 : 7#### ' � 78 ' 8 1 ' �' � 78 ' 8 1 ' �' � 78 ' 8 1 ' �' � 78 ' 8 1 ' � 8 0 !8 0 !8 0 !8 0 ! ' �' �' �' � 8 ; �8 ; �8 ; �8 ; � ' � 8 �' �' � 8 �' �' � 8 �' �' � 8 �' � 0 ! 70 ! 70 ! 70 ! 7' � 70 �' � 8' � 70 �' � 8' � 70 �' � 8' � 70 �' � 8 """" 0 7' � < 80 7' � < 80 7' � < 80 7' � < 8 ####9999��� � � � � � � �� � � � � � � � � � � � �� �� � � � � � � � � � � � � � � � � � � � � � � � � � � � �

� � � � � � � ! � �0 8 $ ' � 0 8 ) = ' � 0 8 ' � 0 8 � ' � �� 8 � ' � 8 0 : ' � 0 ) 8 ( ' � 0 ) 8 � �0 8 $ ' � 0 8 ) = ' � 0 8 ' � 0 8 � ' � �� 8 � ' � 8 0 : ' � 0 ) 8 ( ' � 0 ) 8 � �0 8 $ ' � 0 8 ) = ' � 0 8 ' � 0 8 � ' � �� 8 � ' � 8 0 : ' � 0 ) 8 ( ' � 0 ) 8 � �0 8 $ ' � 0 8 ) = ' � 0 8 ' � 0 8 � ' � �� 8 � ' � 8 0 : ' � 0 ) 8 ( ' � 0 ) 8 � � 9999

Spectral range: 0 35,877 cm-1

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GEISA-03 line transition parameters sub-databasecontent summary

C2H6 14981CH3D 5518C2H2 3115C2H4 12978GeH4 824HCN 2550C3H8 8983C2N2 2577C4H2 1405HC3N 2027HOCl 17862N2 120CH3Cl 18344H2O2 100781H2S 20788HCOOH 3388COF2 83750SF6 11520C3H4 3390HO2 38804ClONO2 32199

H2O 58726CO2 76826O3 319248N2O 26681CO 13515CH4 216196O2 6290NO 99123SO2 38853NO2 104224NH3 29082PH3 11740HNO3 171504OH 42866HF 107HCl 533HBr 1294HI 806ClO 7230OCS 24922H2CO 2701

Molecule # TransitionsMolecule # Transitions

42 molecules

96 isotopic species

Spectral range:0 35,877 cm-1

Total # transitions :1,668,371

GEISA specific moléculesof planetaryatmosphere interest

Mol8888culesGEISA/IASI

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Spectral range

230 – 1333 nm

11 molecular species

164 T,P sets

12,958,953 entries

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"�� � � ��� � � ��� � � ��� � � �" ? � � � � � � � �? � � � � � � � �? � � � � � � � �? � � � � � � � �" ? � � � � � � � � ! � � �? � � � � � � � � ! � � �? � � � � � � � � ! � � �? � � � � � � � � ! � � �" ? � � � � � � ! � ! � � � � � � � �? � � � � � � ! � ! � � � � � � � �? � � � � � � ! � ! � � � � � � � �? � � � � � � ! � ! � � � � � � � �"�� � � � � ! � � ��� � � � � ! � � ��� � � � � ! � � ��� � � � � ! � � �"� ! � � � � � � � � � � �� ! � � � � � � � � � � �� ! � � � � � � � � � � �� ! � � � � � � � � � � �

A Database on atmospheric aerosols from LITMS (Rublev, 1994)

The software package and database OPAC (Optical Properties of Aerosols and Clouds) (Hess et al., 1998)

The Global Aerosol Data Set: GADS (Koepke et al., 1997)

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� �� �� �� �� �� �� �� ���� �� �� � ��� � ��� � ��� � � �� �� � � �� �� � � �� �� � � �� �� � � �� �� �� � �� �� � ��� � �� �� � ��� � �� �� � ��� � �� �� � �

� �� ' � ( ) � � � * * ' � ( ' � � �� ' + � � ' % + � � ' � � �� �� ' � ( ) � � � * * ' � ( ' � � �� ' + � � ' % + � � ' � � �� �� ' � ( ) � � � * * ' � ( ' � � �� ' + � � ' % + � � ' � � �� �� ' � ( ) � � � * * ' � ( ' � � �� ' + � � ' % + � � ' � � �� , � �� � ' - . � * �� � , � �� � ' - . � * �� � , � �� � ' - . � * �� � , � �� � ' - . � * ��

CLASSES OF SOLAR SYSTEM MAIN COMPONENTS ATMOSPHERES ATMOSPHERES OBJECT (non exhaustive lists)

H2-He atmospheres JUPITER H2, He, CH4, C2H2, C2H6, C2H4, H2O, C4H2, C6H6of the giant planets C3H4, NH3, PH3, GeH4, CO, AsH3, CO2, �� ��

SATURN H2, He, CH4, C2H2, C2H6, C3H4,CH3,H2S,CH3,H2O, C3H8, NH3, PH3, GeH4, H2O, AsH3,C2H6,C2H4, CO, CO2,CH3C2H, �� ��

URANUS H2, He, CH4, .......NEPTUNE H2, He, CH4, C2H4, C2H2, H2S(?),

NH3 (?), CH3, � � � � � �� � � � � �� � � � � �� � � � � �

Terrestrial CO2 VENUS CO2, N2, SO2, H2SO4, CO, O, N2, O3,atmospheres HCl, HF, Ne, H2S , OCS, H, H2, He

FeCl3(?), H2O, O2, Cl, ClO, ClO2, COCl, ..

MARS CO2, N2, Ar, O2, H2O, CO, H2O,O3, OH, HO2, H, D, HDO, Ar, Ne, Kr, Xe, …

N2 atmospheres TITAN N2, CH4, O2, Ar, CO, C2H6, C3H8, H2O, CO, CO2,C2H4, NH3, HCN, C2N2, HC3N, CH3CN, C4H2, CH2CCH2, C6H2,C3H4, HC5N, C4N2,…..

EARTH N2, O2, Ar, H2O, CO2, O3, N2O, CH4, NO, SO2, NO2, HNO3, OCS, NH3, HCN,H2CO, …

PLUTO N2, CO, CH4, …..TRITON N2, CO, CH4,

--------------------------------------------------------------------------------------------------------------------------------------------------Volcanic IO SO2, ….--------------------------------------------------------------------------------------------------------------------------------------------------Exospheres MOON Na, K, …..

MERCURY Na, K, …….

--------------------------------------------------------------------------------------------------------------------------------------------------Comae COMETS H2O, CH4, CO, CO2, CH3OH, …..

MoleculesNot inGEISA

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� �� �� �� �� �� �� �� ���� �� �� � ��� � ��� � ��� � � �� �� � � �� �� � � �� �� � � �� �� � � �� �� �� � �� �� � ��� � �� �� � ��� � �� �� � ��� � �� �� � �

������(001����%�������������� ���2

����� ����� ���������� ����3,� �3���

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� �� �� �� �� �� �� �� ���� �� �� � ��� � ��� � ��� � � �� �� � � �� �� � � �� �� � � �� �� � � �� �� �� � �� �� � ��� � �� �� � ��� � �� �� � ��� � �� �� � �

Updates for 2007 Edition of GEISA line transition parameterssub-database

+(� 400, 5000���,6���������������������������������������������7�8��"�� %9 �������� #

*�( ((00,1000���,6������������������������������������������ 7�8��"�� %9 �������� #

.000,:000���,6 7�8�"�������;�)����#

'(��� 6:00,<500���,6��������������������������������������������7�8��"�� %9 �������� #

*+. 140,6&40���,6���������������������������������������� 8����8�*� �8�/)���$��8������������������

(540,&640���,6 "������ ���=#

.500,:(00���,6 '����������� ����������� ����� �7�8�"�)����#

�+& 110,&<06���,6�������������������������������������������7�8�8����")������)� �����$������#

+'�& ��3������� �� 7�8�">������ ���=#

����4,����:�����".(6���,6#��������������������? ��!% �� � ������ %����3�����%��� � �(����:,����:���".&5���,6#�����������������������/������� �����7�8������"�� @��� ���=�#66=(�A��"����4����(����:#�������������������8�����"B�������������� ���=#

5=&�A��"����5-����:#����"����<-����1#�

+(*� 6=41&�A������������������������������������������%����� � � ��� ��� ����"*%���#

4,60A��"����(�����&�����.�����<#��������������� �

Molecule Spectral Range/ OriginBand Id.

Preliminary non exhaustive list

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� �� �� �� �� �� �� �� ���� �� �� � ��� � ��� � ��� � � �� �� � � �� �� � � �� �� � � �� �� � � �� �� �� � �� �� � ��� � �� �� � ��� � �� �� � ��� � �� �� � �

Updates for 2007 Edition of GEISA line transition parameterssub-database (Following)

C2H6 12 µm region ULB, Calgary Univ., LISA (Auwera)

CH3D 3250-3700 cm-1 LTS,LPUB, JPL ( in preparation by Brown)

C2H2 2.5 µm and 3.8 µm New line list prepared by Jacquemart1.5 µm region New line list prepared by Auwera0.83 µm region New line list (ULB required)

Molecule Spectral Range/ OriginBand Id.

Preliminary non exhaustive list

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� �� �� �� �� �� �� �� ���� �� �� � ��� � ��� � ��� � � �� �� � � �� �� � � �� �� � � �� �� � � �� �� �� � �� �� � ��� � �� �� � ��� � �� �� � ��� � �� �� � �

Updates for 2007 Edition of GEISA line transition parameters sub-database (Following)

MIPAS (Michelson Interferometer for Passive Atmospheric Sounding) experiment operating on board the ENVISAT satellite since March 2002, recording emission limb sounding spectra at 0.025 cm-1 (unapodized) in the spectral range 685-2410 cm-1

Starting from HITRAN-96 and GEISA-97, and updated in 2001 and 2003 with specific spectroscopic studies or from spectroscopic studies prior to their publications. Validation through ATMOS and MIPAS recorded spectra 31 molecules retained from the HITRAN list (O, NO+, HOBr, C2H4, CH3OH, H2CO,

H2CO, SF6 discarded)

The MIPAS data base in the spectral range597.046462 – 2502.957500 cm-1

(Flaud, Piccolo, Carli, Perrin, Coudert,Teffo, and Brown, Atmos. Oceanic Opt., 16, 172-182, 2003)

New PF 3.2 Version (courtesy of J.M. Flaud)

Comparison with GEISA contentAssessment of updates to be made in GEISA

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� �� �� �� �� �� �� �� ���� �� �� � ��� � ��� � ��� � � �� �� � � �� �� � � �� �� � � �� �� � � �� �� �� � �� �� � ��� � �� �� � ��� � �� �� � ��� � �� �� � �

Updates for 2007 Edition of GEISA line transition parameterssub-database (Following)

C2H4 850- 1500 cm-1 LPUB,ULB, UNIV.LOUVAIN New line list in preparation by Rotger

HCN 14 µm (����2 and 2����2��������2) Line lists under evaluation

C2N2 203.872 - 266.320 cm-1 Coustenis Private communication(LISA/GPCOS; Jolly, Benilan, et al.)

C4H2 199.1 - 244.0 cm-1 Coustenis Private communication605.5 - 651.4 cm-1 (LISA/GPCOS; Jolly, Benilan, et al.)

C3H4 290.3 – 360.0 cm-1 Coustenis Private communication592.8 – 673.5 cm-1 (Graner line list)

HC3N 16 µm (����5) LISA (Jolly et al.)20µm (����6 � �� �� �� �

Molecule Spectral Range/ OriginBand Id.

Laboratory for Space Research, Observatoire de Paris-Meudon, FranceCooperation (Athena Coustenis; Bruno Bezard)

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� �� �� �� �� �� �� �� ���� �� �� � ��� � ��� � ��� � � �� �� � � �� �� � � �� �� � � �� �� � � �� �� �� � �� �� � ��� � �� �� � ��� � �� �� � ��� � �� �� � �

New Molecular Species for GEISA 2007 Edition

CH3Br 16 µm spectral region Lab. De dynamique, Interactions et Réactivité, LISA (Jacquemart et al. )

CH3CN 305 - 415 cm-1 JPL, LISA, PNNL (Brown et al.)

CH3OH 0.02 - 33.27 cm-1 JPL, Univ. of New Brunswick10 µm region (Brown, Li Hong Xu)

C2HD 451.5 - 580.2 cm-1 (LISA/GPCOS; Jolly, Benilan, et al.)600.1 - 760.0 cm-1

C6H6 642.4 –705.3 cm-1 Coustenis Private communication(Dang line list)

Molecule Spectral Range/ OriginBand Id.

Laboratory for Space Research, Observatoire de Paris-Meudon, FranceCooperation (Athena Coustenis; Bruno Bezard)

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� �� �� �� �� �� �� �� ���� �� �� � ��� � ��� � ��� � � �� �� � � �� �� � � �� �� � � �� �� � � �� �� �� � �� �� � ��� � �� �� � ��� � �� �� � ��� � �� �� � �

*�������!�*����� �

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����� � �� � �� � �� � � ���� � � � � � � � �� � � �� � � �� � � � ���� � � � �� � �� � �� � �� � �

����� � � � � � � � � � � � � � � � � � � � � � �� � � � � � � � � � � � � � � � � � � � � � �� � � � � � � � � � � � � � � � � � � � � � �� � � � � � � � � � � � � � � � � � � � � � �� � � � � � �� � � � � � �� � � � � � �� � � � � � �

���� ����� � � �� � � �� � � �� � � �

��������� �� �� �� �

������������� �� �� �� �

�������� � � � � � � � �

������������� �� �� �� ����� ��������� � � � � � � �

����������������� �� �� �� �

� ! � " "� ! � " "� ! � " "� ! � " " ����" # � $ % � � "" # � $ % � � "" # � $ % � � "" # � $ % � � "

� � � $ % � & & '� � � $ % � & & '� � � $ % � & & '� � � $ % � & & '( % � # �( % � # �( % � # �( % � # �' % ) % � *' % ) % � *' % ) % � *' % ) % � *

( % � # �( % � # �( % � # �( % � # �+ ! � , - # � % � *+ ! � , - # � % � *+ ! � , - # � % � *+ ! � , - # � % � *

( % � # �( % � # �( % � # �( % � # �% � $ # � " % $ % # "% � $ # � " % $ % # "% � $ # � " % $ % # "% � $ # � " % $ % # "

( % � # �( % � # �( % � # �( % � # �. � " % $ % � �. � " % $ % � �. � " % $ % � �. � " % $ % � �

' � ( # � & ( #' � ( # � & ( #' � ( # � & ( #' � ( # � & ( #

From ISSWG-14 (March 24-26 /2001) Conclusions

STATUS OF MOLECULES FOR IASI RADIATIVE TRANSFER MODELLING

Prepared by A. Perrin (GIDSC chairman)GIDSC: GEISA/IASI Database Scientifiv Commitee

1: Parameters that need to be improved; 2 rd priority; 3 rd priorityY no problem clearly identified; ? The databases have to be checked

WHERE ARE WE NOW ?

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& @& @& @& @ �� � � + � � � � � 6 � � � � � � � � � � � � � � � � � � � � � � � � � � /�� � � + � � � � � 6 � � � � � � � � � � � � � � � � � � � � � � � � � � /�� � � + � � � � � 6 � � � � � � � � � � � � � � � � � � � � � � � � � � /�� � � + � � � � � 6 � � � � � � � � � � � � � � � � � � � � � � � � � � / � � � ! ! � � � � � � �� � � ! ! � � � � � � �� � � ! ! � � � � � � �� � � ! ! � � � � � � �� � � 6 � ! � � � � � � A� � � 6 � ! � � � � � � A� � � 6 � ! � � � � � � A� � � 6 � ! � � � � � � A

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Some conclusions of validation exercises, using e.g. : the 4A-00/LMD Model, in the case of IASI radiative transfer

modelling

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Laboratoire Inter-Universitaire des

Systèmes Atmosphériques

Groupe de Physico-Chimie Organique

Spatiale

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ACKNOWLEDGMENTS

to

CNES, CNRS/INSU and EUMETSAT

for their Encouragements and Supports