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Topological states of matter in correlated electron systems Qiang-Hua Wang National Lab of Solid State Microstructures, Nanjing University, Nanjing 210093, China Seminar @ Tsinghua, Dec.5/2012 CollaboratorsDunghai Lee (Berkely), F Wang (MIT), F Yang (Beijing) Students: Wan-Sheng Wang and Yuan-Yuan Xiang Wang WS, et al, PRB 2012; Xiang YY, et al, PRB 2012
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Topological states of matter in correlated electron · PDF file · 2012-12-10Topological states of matter in correlated electron systems ... • Seek point group with odd parity...

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Page 1: Topological states of matter in correlated electron · PDF file · 2012-12-10Topological states of matter in correlated electron systems ... • Seek point group with odd parity degenerate

Topological states of matter in correlated electron systems

Qiang-Hua Wang National Lab of Solid State Microstructures, Nanjing

University, Nanjing 210093, China

Seminar @ Tsinghua, Dec.5/2012

Collaborators:Dunghai Lee (Berkely), F Wang (MIT), F Yang (Beijing) Students: Wan-Sheng Wang and Yuan-Yuan Xiang

Wang WS, et al, PRB 2012; Xiang YY, et al, PRB 2012

Page 2: Topological states of matter in correlated electron · PDF file · 2012-12-10Topological states of matter in correlated electron systems ... • Seek point group with odd parity degenerate

Outline

•  Introduction and motivation •  T-breaking topological phases in doped

Graphene and kagome lattices •  T-invariant topological superconductors •  Conclusions

Page 3: Topological states of matter in correlated electron · PDF file · 2012-12-10Topological states of matter in correlated electron systems ... • Seek point group with odd parity degenerate

Topology in daily life

Zero handle

One handle

Page 4: Topological states of matter in correlated electron · PDF file · 2012-12-10Topological states of matter in correlated electron systems ... • Seek point group with odd parity degenerate

Topological states in 1D: kink and soliton

∫ −+∂= ]cos1)([ 2 φφxKdxH

0

2*pi

Page 5: Topological states of matter in correlated electron · PDF file · 2012-12-10Topological states of matter in correlated electron systems ... • Seek point group with odd parity degenerate

Topological states in 2D: vortex

W=1

Page 6: Topological states of matter in correlated electron · PDF file · 2012-12-10Topological states of matter in correlated electron systems ... • Seek point group with odd parity degenerate

Topological states in 2D: vortex

W=0

Page 7: Topological states of matter in correlated electron · PDF file · 2012-12-10Topological states of matter in correlated electron systems ... • Seek point group with odd parity degenerate

Topology and topological states of matter Hasan and Kane, RMP 2010

Page 8: Topological states of matter in correlated electron · PDF file · 2012-12-10Topological states of matter in correlated electron systems ... • Seek point group with odd parity degenerate

Topology and mapping k à H(k)

.2},{

,])([

ββα δ

ψεψ

a

kkk

k IkBH

=ΓΓ

+Γ⋅=∑ +

Page 9: Topological states of matter in correlated electron · PDF file · 2012-12-10Topological states of matter in correlated electron systems ... • Seek point group with odd parity degenerate

TKNN invariant, Chern number and edge states Thouless, Kohmoto, Nightingale, and den Nijs 1982

Topological number can not change smoothly. Topologically distinct phases are connected by a) gap closing in the quantum phase transition point in parameter space, or b) gapless edge states in real space. There is a 1 to 1 correspondence between the change of Z across the boundary and the number of edge states.

Page 10: Topological states of matter in correlated electron · PDF file · 2012-12-10Topological states of matter in correlated electron systems ... • Seek point group with odd parity degenerate

TKNN invariant, Chern number and edge states

Skippy cyclotron orbits Edge state in the Haldane model

Page 11: Topological states of matter in correlated electron · PDF file · 2012-12-10Topological states of matter in correlated electron systems ... • Seek point group with odd parity degenerate

Spin polarized p+ip superconductor, Z=1

Read and Green 2000

The effective field B(k) cover the Bloch sphere once.

Page 12: Topological states of matter in correlated electron · PDF file · 2012-12-10Topological states of matter in correlated electron systems ... • Seek point group with odd parity degenerate

Majorana fermions in 1d and 2d cases

+E and –E forms a canonical fermion, not protected E=0 comes in pair and sit on opposite edges, protected

Page 13: Topological states of matter in correlated electron · PDF file · 2012-12-10Topological states of matter in correlated electron systems ... • Seek point group with odd parity degenerate

Majorana fermion and non-Abelian statistics

Page 14: Topological states of matter in correlated electron · PDF file · 2012-12-10Topological states of matter in correlated electron systems ... • Seek point group with odd parity degenerate

Topological quantum computing

April 2006 www.sciam.com

Page 15: Topological states of matter in correlated electron · PDF file · 2012-12-10Topological states of matter in correlated electron systems ... • Seek point group with odd parity degenerate

Spin singlet d+id superconductor

)2exp(~)(,),(

,),(

,)()()()(

0*0

k

Tkkk

Tkkk

kk

k

ikdcc

cc

kHkdkdkH

H

θ

ψ

ψ

ψµ

µψ

+

+↓−↑

↓−+↑

+

++

=

=

⎟⎟⎠

⎞⎜⎜⎝

−Δ

Δ−=∑

The effective field B(k) cover the Bloch sphere twice, thus Z=2

Page 16: Topological states of matter in correlated electron · PDF file · 2012-12-10Topological states of matter in correlated electron systems ... • Seek point group with odd parity degenerate

Edge states for d+id pairing (Z=2)

−1 0 1

−6

−4

−2

0

2

4

6

q//

Energy

Page 17: Topological states of matter in correlated electron · PDF file · 2012-12-10Topological states of matter in correlated electron systems ... • Seek point group with odd parity degenerate

Z2 number in T-invariant insulators

Enen crossings:Z2=0 Odd crossings: Z2=1

Kramers degeneracy on T-invariant momenta Г

In-gap edge states In-gap edge states

Page 18: Topological states of matter in correlated electron · PDF file · 2012-12-10Topological states of matter in correlated electron systems ... • Seek point group with odd parity degenerate

Quantum spin Hall system

Konig et al, 2007

Page 19: Topological states of matter in correlated electron · PDF file · 2012-12-10Topological states of matter in correlated electron systems ... • Seek point group with odd parity degenerate

T-invariant topological insulator/superconductor

Roy et al 2008; Schnyder et al 2008 Kitaev 2009; Qi et al 2009; Qi et al, RMP 2011

For a topological insulator,ψk

+ = (ak↑+ ,bk↑

+ ,ak↓+ ,bk↓

+ )

ψk = (ak↑,bk↑,ak↓,bk↓)T .

For a superconductor,ψk

+ = (ak↑+ ,a−k↑,ak↓

+ ,a−k↓)

ψk = (ak↑,a−k↑+ ,ak↓,a−k↓

+ )T .

)( yx ippip +=±

Page 20: Topological states of matter in correlated electron · PDF file · 2012-12-10Topological states of matter in correlated electron systems ... • Seek point group with odd parity degenerate

Edge state in a T-invariant topological superconductor

Page 21: Topological states of matter in correlated electron · PDF file · 2012-12-10Topological states of matter in correlated electron systems ... • Seek point group with odd parity degenerate

A convenient criterion for T-invariant topological superconductor

Roy et al 2008; Schnyder et al 2008 Kitaev 2009; Qi et al 2009; Qi et al, RMP 2011

Page 22: Topological states of matter in correlated electron · PDF file · 2012-12-10Topological states of matter in correlated electron systems ... • Seek point group with odd parity degenerate

3d topological insulators

Fang et al Xue et al

Page 23: Topological states of matter in correlated electron · PDF file · 2012-12-10Topological states of matter in correlated electron systems ... • Seek point group with odd parity degenerate

3d topological superconductors

Page 24: Topological states of matter in correlated electron · PDF file · 2012-12-10Topological states of matter in correlated electron systems ... • Seek point group with odd parity degenerate

Ando et al, PRL 2010

Page 25: Topological states of matter in correlated electron · PDF file · 2012-12-10Topological states of matter in correlated electron systems ... • Seek point group with odd parity degenerate

Fu and Berg, PRL 2010

Page 26: Topological states of matter in correlated electron · PDF file · 2012-12-10Topological states of matter in correlated electron systems ... • Seek point group with odd parity degenerate

Periodic table of topology

Page 27: Topological states of matter in correlated electron · PDF file · 2012-12-10Topological states of matter in correlated electron systems ... • Seek point group with odd parity degenerate

Challenges in the search of (intrinsic) topological superconductors

•  Energy scale of topological insulators: eV

•  Finding a BdG hamiltonian finishes only a half of the job

•  Proximity effect generated topological superconductor depends solely on the edge (surface) states of topological insulator (many literatures in this direction)

•  Intrinsic topological superconductor relies on the system itself, such as Sr2RuO4 and He-III B-phase.

•  In repulsive systems, the energy scale involved in superconducting transition: 1 ~ 40meV. Energy hierarchy requires RG treatment.

Page 28: Topological states of matter in correlated electron · PDF file · 2012-12-10Topological states of matter in correlated electron systems ... • Seek point group with odd parity degenerate

Ideas of RG and FRG Wilson RG Wetterich FRG

Energy S

cale

Page 29: Topological states of matter in correlated electron · PDF file · 2012-12-10Topological states of matter in correlated electron systems ... • Seek point group with odd parity degenerate

Ideas of RG and FRG Wilson RG Wetterich FRG

Energy S

cale

Page 30: Topological states of matter in correlated electron · PDF file · 2012-12-10Topological states of matter in correlated electron systems ... • Seek point group with odd parity degenerate

Ideas of RG and FRG Wilson RG Wetterich FRG

Energy S

cale

Page 31: Topological states of matter in correlated electron · PDF file · 2012-12-10Topological states of matter in correlated electron systems ... • Seek point group with odd parity degenerate

Ideas of RG and FRG Wilson RG Wetterich FRG

Energy S

cale

Page 32: Topological states of matter in correlated electron · PDF file · 2012-12-10Topological states of matter in correlated electron systems ... • Seek point group with odd parity degenerate

Singular-mode FRG

: orthonormal form factors

P

C D

Cf: Husemann and Salmhofer

Page 33: Topological states of matter in correlated electron · PDF file · 2012-12-10Topological states of matter in correlated electron systems ... • Seek point group with odd parity degenerate

FRG flow

Page 34: Topological states of matter in correlated electron · PDF file · 2012-12-10Topological states of matter in correlated electron systems ... • Seek point group with odd parity degenerate

FRG flow

Page 35: Topological states of matter in correlated electron · PDF file · 2012-12-10Topological states of matter in correlated electron systems ... • Seek point group with odd parity degenerate

FRG flow

Page 36: Topological states of matter in correlated electron · PDF file · 2012-12-10Topological states of matter in correlated electron systems ... • Seek point group with odd parity degenerate

A simple view of mode-mode coupling

±ciσ+ ciσcjτ

+ cjτ ⇔ ± ciσ+ cjτ

+ cjτciσ

Si ⋅Sj ⇔ −12(ci↑

+cj↓+ − ci↓

+cj↑+ )(cj↓ci↑ − cj↑ci↓)+ ... ⇒ ↑↓−↓↑

−Si ⋅Sj ⇔ −14ci↑+cj↑

+ cj↑ci↑+ ... ⇒ ↑↑, ↓↓, ↑↓+↓↑

Singlet pair

Triplet pair

+ more general bond-type density wave interactions

Page 37: Topological states of matter in correlated electron · PDF file · 2012-12-10Topological states of matter in correlated electron systems ... • Seek point group with odd parity degenerate

Instabilities

•  Q=0 p-p susceptibility always logarithmically divergent à universal Cooper instability wrt infinitesimal attraction

•  p-h susecptibility usually finite (unless in case of perfect nesting or van Hove singularity) àStoner instability wrt finite interaction

Page 38: Topological states of matter in correlated electron · PDF file · 2012-12-10Topological states of matter in correlated electron systems ... • Seek point group with odd parity degenerate

•  Introduction and motivation •  T-breaking topological phases in doped

Graphene and kagome lattices •  T-invariant topological superconductors •  Conclusions

Page 39: Topological states of matter in correlated electron · PDF file · 2012-12-10Topological states of matter in correlated electron systems ... • Seek point group with odd parity degenerate

Band structure of graphene

The band structure of graphene with t1=2.8ev, t2=0.1ev , t3=0.07ev at ¼ doping

Physics near van Hove singularity?

Physics near the Dirac point

Page 40: Topological states of matter in correlated electron · PDF file · 2012-12-10Topological states of matter in correlated electron systems ... • Seek point group with odd parity degenerate

Semenoff, PRL53,2449,1984

Zhang et al., Nature 438,201(2005)

Relativistic quantum mechanics near the Dirac point

Page 41: Topological states of matter in correlated electron · PDF file · 2012-12-10Topological states of matter in correlated electron systems ... • Seek point group with odd parity degenerate

C. L. Kane and E.J. Mele , QSHE in Graphene , PRL95,226801(2005)

C. L. Kane and E. J. Mele, Z2 topological Order and the QSHE, PRL95, 146802 (2005)

Spin quantum Hall effect?

Page 42: Topological states of matter in correlated electron · PDF file · 2012-12-10Topological states of matter in correlated electron systems ... • Seek point group with odd parity degenerate

X.Du et al., Nature 462,192; Bolotin et al., Nature 462,196

Correlations revealed by fractional QH

Page 43: Topological states of matter in correlated electron · PDF file · 2012-12-10Topological states of matter in correlated electron systems ... • Seek point group with odd parity degenerate

Doping graphene…

Eli Rotenberg

Extended van Hove singularity

Page 44: Topological states of matter in correlated electron · PDF file · 2012-12-10Topological states of matter in correlated electron systems ... • Seek point group with odd parity degenerate

What’s so special of graphene •  van Hove singularity and correlation effect

•  Under C6v point group,( ,xy) and (x,y) are doublets. Candidates for the gap function.

•  T-breaking mixing of degenerate pairing gaps very likely, leading to a full gap

•  Possible pairing symmetries: s, d+id, p+ip, f

22 yx −

Page 45: Topological states of matter in correlated electron · PDF file · 2012-12-10Topological states of matter in correlated electron systems ... • Seek point group with odd parity degenerate

x=1/4, U=3.6t, V=0 Van Hove singularity and perfect nesting

V_sdw V_sc

Page 46: Topological states of matter in correlated electron · PDF file · 2012-12-10Topological states of matter in correlated electron systems ... • Seek point group with odd parity degenerate

Chiral SDW

LiTao, arxiv 1103.2420, honeycomb lattice Martin and Batista, PRL101,156402, triangle lattice

Page 47: Topological states of matter in correlated electron · PDF file · 2012-12-10Topological states of matter in correlated electron systems ... • Seek point group with odd parity degenerate

Chern number and quantized anomalous Hall conductivity

1

Page 48: Topological states of matter in correlated electron · PDF file · 2012-12-10Topological states of matter in correlated electron systems ... • Seek point group with odd parity degenerate

Non-perturbative quantum Monte Carlo

Page 49: Topological states of matter in correlated electron · PDF file · 2012-12-10Topological states of matter in correlated electron systems ... • Seek point group with odd parity degenerate

x=0.211, U=3.6t, V=0

V_sdw V_sc

Page 50: Topological states of matter in correlated electron · PDF file · 2012-12-10Topological states of matter in correlated electron systems ... • Seek point group with odd parity degenerate

T-breaking d+id Two degenerate d-wave pairing:

d+id

MF or GL theory predict that the d+id pairing is energetically more favorable

R Nandkishore et al, Nature Physics 8, 158 (2012)

Full gap

Nodal gap

Page 51: Topological states of matter in correlated electron · PDF file · 2012-12-10Topological states of matter in correlated electron systems ... • Seek point group with odd parity degenerate

Edge states for d+id pairing (Z=2)

−1 0 1

−6

−4

−2

0

2

4

6

q//

Energy

Page 52: Topological states of matter in correlated electron · PDF file · 2012-12-10Topological states of matter in correlated electron systems ... • Seek point group with odd parity degenerate

Phase diagram

Both chiral SDW and chiral d+id are topological.

Cf: Keisel et al, arxiv 1109.2953

Page 53: Topological states of matter in correlated electron · PDF file · 2012-12-10Topological states of matter in correlated electron systems ... • Seek point group with odd parity degenerate

Kagome lattice

Upper van Hove filling Lower van Hove filling

Page 54: Topological states of matter in correlated electron · PDF file · 2012-12-10Topological states of matter in correlated electron systems ... • Seek point group with odd parity degenerate

Upper van Hove filling

D-wave Permoranchuk

FM

Intra-cell AFM

sSC

Page 55: Topological states of matter in correlated electron · PDF file · 2012-12-10Topological states of matter in correlated electron systems ... • Seek point group with odd parity degenerate

Lower van Hove filling

Page 56: Topological states of matter in correlated electron · PDF file · 2012-12-10Topological states of matter in correlated electron systems ... • Seek point group with odd parity degenerate

•  Topological states of matter and challenges of the search of intrinsic topological superconductors

•  T-breaking topological phases in doped Graphene

•  T-invariant topological superconductors, a road map

•  Conclusions

Page 57: Topological states of matter in correlated electron · PDF file · 2012-12-10Topological states of matter in correlated electron systems ... • Seek point group with odd parity degenerate

Gap function of a T-invariant superconductor

Qi et al, Kitaev et al: 1) Even number of spin-split pockets, each encircles an odd number of T-invariant momenta. 2) Number of pockets with + and - signs: Even = Odd + Odd

singlet triplet

Page 58: Topological states of matter in correlated electron · PDF file · 2012-12-10Topological states of matter in correlated electron systems ... • Seek point group with odd parity degenerate

Gap-function of a T-invariant superconductor

H0 =Ψ k+(εkσ 0 +λγ k ⋅σ )Ψ k → ψk

+(εk ±λ |γ k |)ψk,

−k,a = iσ 2K k,a

If dk ~ γ k, T − invar iant, and

HP =Ψ k+(φkσ 0 + dk ⋅σ )iσ 2 (Ψ−k

+ )T

→−ψk,a+ ( φk ± | dk | )(ψ−k,b

+ )Tδa,b

γ k = (−sinky, sinkx, 0)

Page 59: Topological states of matter in correlated electron · PDF file · 2012-12-10Topological states of matter in correlated electron systems ... • Seek point group with odd parity degenerate

i(px + ipy )↓↓+i(px − ipy )↑↑

Page 60: Topological states of matter in correlated electron · PDF file · 2012-12-10Topological states of matter in correlated electron systems ... • Seek point group with odd parity degenerate

Our road map

•  Seek ferromagnetic spin fluctuations to favor triplet pairing

•  Seek point group with odd parity degenerate irreducible representation (such as C4v and C6v)

•  Seek a system with 2(2n+1) spin-split pockets

•  Rashba coupling causes degenerate triplets to recombine into a T-invariant gap, plus small induced singlet component.

Page 61: Topological states of matter in correlated electron · PDF file · 2012-12-10Topological states of matter in correlated electron systems ... • Seek point group with odd parity degenerate

Non-centrosymmetric systems

Page 62: Topological states of matter in correlated electron · PDF file · 2012-12-10Topological states of matter in correlated electron systems ... • Seek point group with odd parity degenerate

Spin-resolved fully anti-symmetrized SM-FRG

Page 63: Topological states of matter in correlated electron · PDF file · 2012-12-10Topological states of matter in correlated electron systems ... • Seek point group with odd parity degenerate

Topological pairing near van Hove singularity

Page 64: Topological states of matter in correlated electron · PDF file · 2012-12-10Topological states of matter in correlated electron systems ... • Seek point group with odd parity degenerate

Topological pairing triggered by small-q inter-pocket scattering

Page 65: Topological states of matter in correlated electron · PDF file · 2012-12-10Topological states of matter in correlated electron systems ... • Seek point group with odd parity degenerate
Page 66: Topological states of matter in correlated electron · PDF file · 2012-12-10Topological states of matter in correlated electron systems ... • Seek point group with odd parity degenerate

Possible candidates with ferromagnetic spin fluctuations

Aoki and Flouquet, JPSJ 81, 011003 (2012).

Shimizu et al, NATURE 412, 316 (2001).

Reyren, etal, Science 317, 1196 (2007).

Iron under high pressure

Page 67: Topological states of matter in correlated electron · PDF file · 2012-12-10Topological states of matter in correlated electron systems ... • Seek point group with odd parity degenerate

•  Motivation •  T-breaking topological phases in doped

Graphene •  T-invariant topological superconductors, a

road map •  Conclusions

Page 68: Topological states of matter in correlated electron · PDF file · 2012-12-10Topological states of matter in correlated electron systems ... • Seek point group with odd parity degenerate

Conclusions •  Graphene near ¼ doping is either a Chern

insulator or a chiral d+id superconductor.

•  Ferromagnetic instability is the key to T-invariant topological insulator, plus Rashba coupling and 2(2n+1) spin split fermi pockets (encircling T-invarint momenta).

•  T-invariant topo-SC can be triggered by 1) proximity to van Hove singularity and 2) by small-q inter-pocket scattering

Page 69: Topological states of matter in correlated electron · PDF file · 2012-12-10Topological states of matter in correlated electron systems ... • Seek point group with odd parity degenerate

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