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Sub-hourly Variation of Tropospheric Ozone Profiles Measured by the Huntsville DIAL Shi Kuang 1* , John Burris 2 , M. J. Newchurch 1* , Steve Johnson 3 , and Stephanie Long 4 1 Atmospheric Science Department, University of Alabama in Huntsville, 320 Sparkman Dr., Huntsville, Alabama 35805, USA 2 NASA-Goddard Space Flight Center, Code 694, Greenbelt, Maryland 20771, USA 3 NASA-Marshall Space Flight Center, Office Code VP61, Huntsville, Alabama 35812, USA 4 Department of Physics, University of Alabama in Huntsville, Huntsville, Alabama 35805, USA
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Sub-hourly Variation of Tropospheric Ozone Profiles Measured by the Huntsville DIAL Shi Kuang 1*, John Burris 2, M. J. Newchurch 1*, Steve Johnson 3, and.

Jan 29, 2016

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Page 1: Sub-hourly Variation of Tropospheric Ozone Profiles Measured by the Huntsville DIAL Shi Kuang 1*, John Burris 2, M. J. Newchurch 1*, Steve Johnson 3, and.

Sub-hourly Variation of Tropospheric Ozone Profiles Measured by the Huntsville DIAL

Shi Kuang1*, John Burris2, M. J. Newchurch1*, Steve Johnson3, and Stephanie Long4

1 Atmospheric Science Department, University of Alabama in Huntsville, 320 Sparkman Dr., Huntsville, Alabama 35805, USA

2NASA-Goddard Space Flight Center, Code 694, Greenbelt, Maryland 20771, USA

3NASA-Marshall Space Flight Center, Office Code VP61, Huntsville, Alabama 35812, USA

4Department of Physics, University of Alabama in Huntsville, Huntsville, Alabama 35805, USA

Page 2: Sub-hourly Variation of Tropospheric Ozone Profiles Measured by the Huntsville DIAL Shi Kuang 1*, John Burris 2, M. J. Newchurch 1*, Steve Johnson 3, and.

The Team

Photo: Front: (left to right) Whitney Guerin, Stephanie Long, Shi Kuang. Back: (left to right) John Burris, Mike Newchurch, Steve Johnson

Page 3: Sub-hourly Variation of Tropospheric Ozone Profiles Measured by the Huntsville DIAL Shi Kuang 1*, John Burris 2, M. J. Newchurch 1*, Steve Johnson 3, and.

Outline

• Instrument description.• Aerosol corrections.• Validation against balloon sondes.• Data• Conclusions.

Page 4: Sub-hourly Variation of Tropospheric Ozone Profiles Measured by the Huntsville DIAL Shi Kuang 1*, John Burris 2, M. J. Newchurch 1*, Steve Johnson 3, and.

Dye Laser

Page 5: Sub-hourly Variation of Tropospheric Ozone Profiles Measured by the Huntsville DIAL Shi Kuang 1*, John Burris 2, M. J. Newchurch 1*, Steve Johnson 3, and.

The Instrument

Page 6: Sub-hourly Variation of Tropospheric Ozone Profiles Measured by the Huntsville DIAL Shi Kuang 1*, John Burris 2, M. J. Newchurch 1*, Steve Johnson 3, and.

Instrument Characterization

• Telescope’s performance validated.• PMT response function and SIN correction

determined. • LED test - quantified electronic system

response. Established system reliability.• Mini receiver installed.

• LICEL (analog/photon counting) units replaced MCS boards (photon counting).

Page 7: Sub-hourly Variation of Tropospheric Ozone Profiles Measured by the Huntsville DIAL Shi Kuang 1*, John Burris 2, M. J. Newchurch 1*, Steve Johnson 3, and.

Model

Glued signal with SIB correction

Glued signal w/o SIB correction

SIB fit

Page 8: Sub-hourly Variation of Tropospheric Ozone Profiles Measured by the Huntsville DIAL Shi Kuang 1*, John Burris 2, M. J. Newchurch 1*, Steve Johnson 3, and.

Aerosol model

Calculated aerosol

O3 model

O3 w/o aerosol correction

O3 with aerosol correction

Page 9: Sub-hourly Variation of Tropospheric Ozone Profiles Measured by the Huntsville DIAL Shi Kuang 1*, John Burris 2, M. J. Newchurch 1*, Steve Johnson 3, and.

ModelS=40, η=0.5S=40, η=0S=40, η=1S=20, η=0.5S=60, η=0.5

Page 10: Sub-hourly Variation of Tropospheric Ozone Profiles Measured by the Huntsville DIAL Shi Kuang 1*, John Burris 2, M. J. Newchurch 1*, Steve Johnson 3, and.

Typical statistical errors for day and nighttime ozone retrievals on the high and low altitude channels

Page 11: Sub-hourly Variation of Tropospheric Ozone Profiles Measured by the Huntsville DIAL Shi Kuang 1*, John Burris 2, M. J. Newchurch 1*, Steve Johnson 3, and.

Validation of DIAL ozone using balloon sondes

(8AM)

All sondes are launched at 1pm except one at 8am.

Low channel works a little better than high channel. High channel has a oscillation above 6. 285 laser doesn’t have power. High statistical error and SIB error at 7-8 km relatively.

Page 12: Sub-hourly Variation of Tropospheric Ozone Profiles Measured by the Huntsville DIAL Shi Kuang 1*, John Burris 2, M. J. Newchurch 1*, Steve Johnson 3, and.

The mean and standard deviation of the ozone retrieval in last slide.

Page 13: Sub-hourly Variation of Tropospheric Ozone Profiles Measured by the Huntsville DIAL Shi Kuang 1*, John Burris 2, M. J. Newchurch 1*, Steve Johnson 3, and.

August 9-10, 2008

Page 14: Sub-hourly Variation of Tropospheric Ozone Profiles Measured by the Huntsville DIAL Shi Kuang 1*, John Burris 2, M. J. Newchurch 1*, Steve Johnson 3, and.

August 17-18, 2008

Page 15: Sub-hourly Variation of Tropospheric Ozone Profiles Measured by the Huntsville DIAL Shi Kuang 1*, John Burris 2, M. J. Newchurch 1*, Steve Johnson 3, and.

Oct. 5, 2008 Nighttime Ozone Enhancement

Similar aerosol and O3 time-height structures suggest a same pollutant source.

Page 16: Sub-hourly Variation of Tropospheric Ozone Profiles Measured by the Huntsville DIAL Shi Kuang 1*, John Burris 2, M. J. Newchurch 1*, Steve Johnson 3, and.

8-hour peak Air Quality Index for ozone at Mississippi/Alabama region in October 2008

This was Sat.!

Page 17: Sub-hourly Variation of Tropospheric Ozone Profiles Measured by the Huntsville DIAL Shi Kuang 1*, John Burris 2, M. J. Newchurch 1*, Steve Johnson 3, and.

Horizontal Transport

24-hr Backtrajectories at 500, 1500 and 4000m for the nighttime ozone enhancement event observed in Huntsville on Oct. 5, 2008.

Page 18: Sub-hourly Variation of Tropospheric Ozone Profiles Measured by the Huntsville DIAL Shi Kuang 1*, John Burris 2, M. J. Newchurch 1*, Steve Johnson 3, and.

October 18, 2008

Page 19: Sub-hourly Variation of Tropospheric Ozone Profiles Measured by the Huntsville DIAL Shi Kuang 1*, John Burris 2, M. J. Newchurch 1*, Steve Johnson 3, and.
Page 20: Sub-hourly Variation of Tropospheric Ozone Profiles Measured by the Huntsville DIAL Shi Kuang 1*, John Burris 2, M. J. Newchurch 1*, Steve Johnson 3, and.

Conclusions

• RAPCD DIAL instrument is retrieving excellent lower tropospheric data.

• Retrievals with aerosol correction have a verified accurate of 5-20% between 1-8 km.

• 24-hr 10-min curtain plots shows many interesting trop O3 features in time and space.