Sergey Kravchenko Approaching an (unknown) phase transition in two dimensions A. Mokashi (Northeastern) S. Li (City College of New York) A. A. Shashkin (ISSP Chernogolovka) V. T. Dolgopolov (ISSP Chernogolovka) T. M. Klapwijk (TU Delft) M. P. Sarachik (City College of New York in collaboration with:
Approaching an (unknown) phase transition in two dimensions. Sergey Kravchenko. in collaboration with:. A. Mokashi (Northeastern) S. Li (City College of New York) A. A. Shashkin (ISSP Chernogolovka) V . T. Dolgopolov (ISSP Chernogolovka) T . M. Klapwijk (TU Delft) - PowerPoint PPT Presentation
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Sergey Kravchenko
Approaching an (unknown) phase transition in two dimensions
A. Mokashi (Northeastern)
S. Li (City College of New York)
A. A. Shashkin (ISSP Chernogolovka)
V. T. Dolgopolov (ISSP Chernogolovka)
T. M. Klapwijk (TU Delft)
M. P. Sarachik (City College of New York
in collaboration with:
• Low disorder: weak (logarithmic) insulator
Non-interacting electron gas in two dimensions (boring):
• High disorder: strong (exponential) insulator
~35 ~1 rs
Wigner crystal Strongly correlated liquid Gas
strength of interactions increases
Coulomb energy Fermi energyrs =
Terra incognita
Suggested phase diagrams for strongly interacting electrons in two dimensions
Magnetic field, by aligning spins, changes metallic R(T) to insulating:
Such a dramatic reaction on parallel magnetic field suggests unusual spin properties!
Spin susceptibility near nc
103
104
105
0 2 4 6 8 10 12
r (O
hm)
B (Tesla)
1.01x1015 m-2
1.20x1015
3.18x1015
2.40x1015
1.68x1015
T = 30 mK
Spins become fully polarized (Okamoto et al., PRL 1999; Vitkalov et al., PRL 2000)
Magnetoresistance in a parallel magnetic field
Shashkin, Kravchenko, Dolgopolov, and
Klapwijk, PRL 2001
Bc
Bc
Bc
0
1
2
3
4
5
0 2 4 6 8 10
BB c (meV
)
ns (1015 m-2)
nc
0
0.2
0.4
0.8 1.2 1.6 2
BB c (meV
)
ns (1015 m-2)
Extrapolated polarization field, Bc, vanishes at a finite electron density, n
Shashkin, Kravchenko, Dolgopolov, and
Klapwijk, PRL 2001
Spontaneous spin polarization at n?
n
gm as a function of electron densitycalculated using g*m* = ћ2ns / BcB
1
2
3
4
5
0 2 4 6 8 10
gm/g
0mb
ns (1015 m-2)
ns= n
c
(Shashkin et al., PRL 2001)
n
2D electron gas Ohmic contact
SiO2
Si
Gate
Modulated magnetic fieldB + B
Current amplifierVg
+
-
Magnetic measurements without magnetometer
suggested by B. I. Halperin (1998); first implemented by O. Prus, M. Reznikov, U. Sivan et al. (2002)
i ~ d/dB = - dM/dns
1010 Ohm
M
ns
dM
ns
dns
B
Magnetization of non-interacting electrons
spin-down spin-up
gBB
Magnetic field of the full spin polarization vs. ns
Bc
ns0
Bc = h2ns/2Bmb
ns
0
dMdns
M = Bns =Bns B/Bc for B < Bc
Bns for B > Bc
B > Bc
B < Bc
B
Bc = h2ns/B g*m*
n
non-interacting systemspontaneous spin polarization at n
-2
-1
0
1
2
0 1 2 3 4 5 6 7
-1
-0.5
0
0.5
1
d/d
B (
B)
i (10
-15 A
)
ns (1011 cm-2)
1 fA!!
Raw magnetization data: induced current vs. gate voltaged/dB = - dM/dn
B|| = 5 tesla
Bar-Ilan University
Raw magnetization data: induced current vs. gate voltageIntegral of the previous slide gives M (ns):complete spin polarization
ns (1011 cm-2)
M (1
011 B
/cm
2 )
met
al
insu
lato
r
0
0.5
1
1.5
0 2 4 6
B|| = 5 tesla
at ns=1.5x1011 cm-2
Spin susceptibility exhibits critical behavior near the sample-independent critical density n : ~ ns/(ns – n)
1
2
3
4
5
6
7
0.5 1 1.5 2 2.5 3 3.5
magnetization datamagnetocapacitance dataintegral of the master curvetransport data
/ 0
ns (1011 cm-2)
nc
insulator
T-dependent regime
g-factor or effective mass?
Shashkin, Kravchenko, Dolgopolov, and Klapwijk, PRB (2002)
0
1
2
3
4
0 2 4 6 8 10
m/m
b , g
/g0
ns (1011 cm-2)
g/g0
m/mb
Effective mass vs. g-factor (from the analysis of the transport data in spirit of
Zala, Narozhny, and Aleiner, PRB 2001) :
Another way to measure m*: amplitude of the weak-field Shubnikov-de Haas oscillations
vs. temperature
(Rahimi, Anissimova, Sakr, Kravchenko, and Klapwijk, PRL 2003)
250
300
350
400
0.2 0.25 0.3 0.35 0.4 0.45 0.5
r (W
/squ
are)
B_|_ (tesla)
430 mK
230 mK
42 mK
1000
2000
3000
4000
0 0.2 0.4 0.6 0.8 1r
(W/s
quar
e)B
_|_ (tesla)
T = 42 mK
2800
2900
3000
3100
0.3 0.4 0.5 0.6
132 mK
42 mK82 mK
=14
=10
= 6
high density low density
Comparison of the effective masses determined by two independent experimental methods:
0
1
2
3
4
0 1 2 3 4
m/m
b
ns (1011 cm-2)
50 30 20 15 12r
s
(Shashkin, Rahimi, Anissimova, Kravchenko, Dolgopolov, and
Klapwijk, PRL 2003)
15 11 8 rs
Thermopower
Thermopower : S = - V / (T) S = Sd + Sg = T + Ts
V : heat either end of the sample, measure the induced voltage difference in the shaded region
T : use two thermometers to determine the temperature gradient
Divergence of thermopower
1/S tends to vanish at nt
Critical behavior of thermopower
(-T/S) (ns- nt)x
x=1.0+/-0.1
nt=7.8+/-0.1*1010 cm-2
and is independent of the level of the disorder
∝
In the low-temperature metallic regime, the diffusion thermopower of strongly interacting 2D electrons is given by the relation
T/S ∝ ns /m
Therefore, divergence of the thermopower indicates a divergenceof the effective mass:
m ∝ ns /(ns − nt)
Divergence of the effective electron mass
Dolgopolov and Gold, JETP Lett. 2011
We observe the increase of the effective mass up to m 25mb 5me!!
i. using Gutzwiller's theory (Dolgopolov, JETP Lett. 2002)
ii. using an analogy with He3 near the onset of Wigner crystallization (Spivak, PRB 2003; Spivak and Kivelson, PRB 2004)
iii. extending the Fermi liquid concept to the strongly-interacting limit (Khodel et al., PRB 2008)
iv. solving an extended Hubbard model using dynamical mean-field theory (Pankov and Dobrosavljevic, PRB 2008)
v. from a renormalization group analysis for multi-valley 2D systems (Punnoose and Finkelstein, Science 2005)
vi. by Monte-Carlo simulations (Marchi et al., PRB 2009; Fleury and Waintal, PRB 2010)
A divergence of the effective mass has been predicted…
Transport properties of the insulating phase
If the insulating state were due to a single-partical localization, a severalorders of magnitude higher electric field would be needed to delocalize an electron:
eEc l > Wb ~ 0.1 – 1 meV
But if this is a pinned Wigner solid,the electric field “pulls” many electrons while only one is pinned – hence, much weaker electric fields are required to depin it and break localization.
SUMMARY:
• In the clean regime, spin susceptibility critically grows upon approaching to some sample-independent critical point, n, pointing to the existence of a phase transition. Unfortunately, residual disorder does not allow to see this transition in currently available samples
• The dramatic increase of the spin susceptibility is due to the divergence of the effective mass rather than that of the g-factor and, therefore, is not related to the Stoner instability. It may be a precursor phase or a direct transition to the long sought-after Wigner solid. However, the existing data, although consistent with the formation of the Wigner solid, are not enough to reliably confirm its existence.