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Lecture 6. Laminar Non-premixed Flames part 2
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Lecture 6. Laminar Non-premixed Flames part 2. Bai Laminar Non-premixed Flames Where is the reaction zone? Zst Burnable mixture A F O 2 O 2 F F Fuel-rich mixing zone Reaction zone

May 25, 2018

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Page 1: Lecture 6. Laminar Non-premixed Flames part 2. Bai Laminar Non-premixed Flames Where is the reaction zone? Zst Burnable mixture A F O 2 O 2 F F Fuel-rich mixing zone Reaction zone

Lecture 6. Laminar Non-premixed Flames

part 2

Page 2: Lecture 6. Laminar Non-premixed Flames part 2. Bai Laminar Non-premixed Flames Where is the reaction zone? Zst Burnable mixture A F O 2 O 2 F F Fuel-rich mixing zone Reaction zone

X.S. Bai Laminar Non-premixed Flames

Content

•  Structures of laminar non-premixed flames •  Mixture fraction •  Burke-Schumann flame-sheet model •  Jet diffusion flames •  Laminar diffusion flame at high mixing rate

Page 3: Lecture 6. Laminar Non-premixed Flames part 2. Bai Laminar Non-premixed Flames Where is the reaction zone? Zst Burnable mixture A F O 2 O 2 F F Fuel-rich mixing zone Reaction zone

X.S. Bai Laminar Non-premixed Flames

Where is the reaction zone?

Zst

Burnable mixture

A F

Diffusion velocity: Fick’s Law

YiVi = Di!Yi, Vi = Di / Yi!Yi "Di / !

!Mixing length

Page 4: Lecture 6. Laminar Non-premixed Flames part 2. Bai Laminar Non-premixed Flames Where is the reaction zone? Zst Burnable mixture A F O 2 O 2 F F Fuel-rich mixing zone Reaction zone

X.S. Bai Laminar Non-premixed Flames

Where is the reaction zone?

Zst

Burnable mixture

A F

O2

O2

F

F

Preheat zone Post flame zone

Page 5: Lecture 6. Laminar Non-premixed Flames part 2. Bai Laminar Non-premixed Flames Where is the reaction zone? Zst Burnable mixture A F O 2 O 2 F F Fuel-rich mixing zone Reaction zone

X.S. Bai Laminar Non-premixed Flames

Where is the reaction zone?

Zst

Burnable mixture

A F

O2

O2

F

F

Preheat zone Post flame zone

Page 6: Lecture 6. Laminar Non-premixed Flames part 2. Bai Laminar Non-premixed Flames Where is the reaction zone? Zst Burnable mixture A F O 2 O 2 F F Fuel-rich mixing zone Reaction zone

X.S. Bai Laminar Non-premixed Flames

Where is the reaction zone?

Zst

Burnable mixture

A F

O2

O2

F

F

Preheat zone Post flame zone

Page 7: Lecture 6. Laminar Non-premixed Flames part 2. Bai Laminar Non-premixed Flames Where is the reaction zone? Zst Burnable mixture A F O 2 O 2 F F Fuel-rich mixing zone Reaction zone

X.S. Bai Laminar Non-premixed Flames

Where is the reaction zone?

Zst

Burnable mixture

A F

O2

O2

F

F

Preheat zone Post flame zone

Page 8: Lecture 6. Laminar Non-premixed Flames part 2. Bai Laminar Non-premixed Flames Where is the reaction zone? Zst Burnable mixture A F O 2 O 2 F F Fuel-rich mixing zone Reaction zone

X.S. Bai Laminar Non-premixed Flames

Where is the reaction zone?

Zst

Burnable mixture

A F

O2

O2

F

F

Preheat zone Post flame zone

Page 9: Lecture 6. Laminar Non-premixed Flames part 2. Bai Laminar Non-premixed Flames Where is the reaction zone? Zst Burnable mixture A F O 2 O 2 F F Fuel-rich mixing zone Reaction zone

X.S. Bai Laminar Non-premixed Flames

Where is the reaction zone?

Zst

Burnable mixture

A F

O2

O2

F

F

Preheat zone Post flame zone

Page 10: Lecture 6. Laminar Non-premixed Flames part 2. Bai Laminar Non-premixed Flames Where is the reaction zone? Zst Burnable mixture A F O 2 O 2 F F Fuel-rich mixing zone Reaction zone

X.S. Bai Laminar Non-premixed Flames

Where is the reaction zone?

Zst

Burnable mixture

A F

O2

O2

F

F

Fuel-rich mixing zone Reaction zone Oxidizer-rich mixing zone

Page 11: Lecture 6. Laminar Non-premixed Flames part 2. Bai Laminar Non-premixed Flames Where is the reaction zone? Zst Burnable mixture A F O 2 O 2 F F Fuel-rich mixing zone Reaction zone

X.S. Bai Laminar Non-premixed Flames

Where is the reaction zone?

Zst

Burnable mixture

Fuel-rich Fuel-lean

T

Z Zst

Tst

T1 T2

0 1

Tcr

A F

Page 12: Lecture 6. Laminar Non-premixed Flames part 2. Bai Laminar Non-premixed Flames Where is the reaction zone? Zst Burnable mixture A F O 2 O 2 F F Fuel-rich mixing zone Reaction zone

X.S. Bai Laminar Non-premixed Flames

Burke-Schumann flame-sheet structure

A P P F

Zst

1

Yi

Z

Reaction zone

Fuel-rich Fuel-lean

Reactions occur in a zero thickness sheet at Z=Zst

Soot problem

Page 13: Lecture 6. Laminar Non-premixed Flames part 2. Bai Laminar Non-premixed Flames Where is the reaction zone? Zst Burnable mixture A F O 2 O 2 F F Fuel-rich mixing zone Reaction zone

X.S. Bai Laminar Non-premixed Flames

Burke-Schumann flame-sheet structure

Reaction zone

Reactions occur in a zero thickness sheet at Z=Zst

Fuel-rich Fuel-lean

T

Z Zst

Tst

T1

T2

0 1

NOx problem

Page 14: Lecture 6. Laminar Non-premixed Flames part 2. Bai Laminar Non-premixed Flames Where is the reaction zone? Zst Burnable mixture A F O 2 O 2 F F Fuel-rich mixing zone Reaction zone

X.S. Bai Laminar Non-premixed Flames

Content

•  Structures of laminar non-premixed flames •  Mixture fraction •  Burke-Schumann flame-sheet model •  Jet diffusion flames •  Laminar diffusion flame at high mixing rate

Page 15: Lecture 6. Laminar Non-premixed Flames part 2. Bai Laminar Non-premixed Flames Where is the reaction zone? Zst Burnable mixture A F O 2 O 2 F F Fuel-rich mixing zone Reaction zone

X.S. Bai Laminar Non-premixed Flames

Laminar jet diffusion flames

Zst

Mixing layer

A non-reactive fuel jet

Fuel

Air

Zst

Burnable mixture

Page 16: Lecture 6. Laminar Non-premixed Flames part 2. Bai Laminar Non-premixed Flames Where is the reaction zone? Zst Burnable mixture A F O 2 O 2 F F Fuel-rich mixing zone Reaction zone

X.S. Bai Laminar Non-premixed Flames

Laminar jet diffusion flames

Air

A+P

Air F+P

A jet diffusion flame Fuel

Fuel rich

Air rich

Reaction zone

a-b

c-d c-d

O2 F P

a-b

O2 F

1, 0, 1 1

stF A P

st st

Z Z ZY Y YZ Z− −

= = =− −

0, 1 , F A Pst st

Z ZY Y YZ Z

= = − =

soot NOx

Fuel rich zone

Fuel lean zone

Page 17: Lecture 6. Laminar Non-premixed Flames part 2. Bai Laminar Non-premixed Flames Where is the reaction zone? Zst Burnable mixture A F O 2 O 2 F F Fuel-rich mixing zone Reaction zone

X.S. Bai Laminar Non-premixed Flames

Jet diffusion flame: mathematical description

Zst

Mixing layer

A non-reactive fuel jet

Fuel

Air

11F P F P st

A

Z Y Y Y Y Zγ

= + = ++

FZ Y=

Combustion

No combustion (pure mixing)

!!Z!t

+"# (!!vZ) ="# (!D"Z)

!!Yi!t

+"#!Yiv!="#!Di"Yi +"i

!!YF!t

+"#!YFv!="#!DF"YF +"F

!!YP!t

+"#!YPv!="#!DP"YP +"P

DF = DP = D, !F +!PZst = 0

Page 18: Lecture 6. Laminar Non-premixed Flames part 2. Bai Laminar Non-premixed Flames Where is the reaction zone? Zst Burnable mixture A F O 2 O 2 F F Fuel-rich mixing zone Reaction zone

X.S. Bai Laminar Non-premixed Flames

Height of laminar jet flame

R

The image cannot be displayed. Your computer may not have enough memory to open the image, or the image may have been corrupted. Restart your computer, and then open the file again. If the red x still appears, you may have to delete the image and then insert it again.

F + P

A + P air

Lf

R

vf

x

Lf !vFR

2

D

!!Z!t

+"# (!!vZ) ="# (!D"Z)

!vF / Lf

!D / R20 Mixing layer analysis

Page 19: Lecture 6. Laminar Non-premixed Flames part 2. Bai Laminar Non-premixed Flames Where is the reaction zone? Zst Burnable mixture A F O 2 O 2 F F Fuel-rich mixing zone Reaction zone

X.S. Bai Laminar Non-premixed Flames

Height of laminar jet flame

R

The image cannot be displayed. Your computer may not have enough memory to open the image, or the image may have been corrupted. Restart your computer, and then open the file again. If the red x still appears, you may have to delete the image and then insert it again.

F + P

A + P

air Lf

R

vf

x

Lf !vFR"D!vFR

2

D

X = vFt,

Y = R !VO2t = R !1!DO2t

Mixing layer analysis

YiVi = Di!Yi, Vi = Di / Yi!Yi "Di / !

X = Lf = vFtf ,

Y = 0 = R ! 1!DO2tf

Page 20: Lecture 6. Laminar Non-premixed Flames part 2. Bai Laminar Non-premixed Flames Where is the reaction zone? Zst Burnable mixture A F O 2 O 2 F F Fuel-rich mixing zone Reaction zone

X.S. Bai Laminar Non-premixed Flames

Jet diffusion flame: experimental obervation

O

F

O

U x

Pe 50 Pe 50 Pe 200 Pe 1

Lf !vFR

2

D=vFRD

!

"#

$

%&R = Pe 'R

Page 21: Lecture 6. Laminar Non-premixed Flames part 2. Bai Laminar Non-premixed Flames Where is the reaction zone? Zst Burnable mixture A F O 2 O 2 F F Fuel-rich mixing zone Reaction zone

X.S. Bai Laminar Non-premixed Flames

Propagation of laminar diffusion flame

N+5 PDE equations

!!!t+"#!v

!= 0

!!!v

!t+"!

!v!v ="# pI+!( )

!DhDt

!DpDt

="# !""h ! !" 1! 1Lei

$

%&&

'

())hi"Yi

i=1

N

*$

%&&

'

())+!Qr +# :"

"v

!!Yi!t

+"#!Yiv!="#!Di"Yi +"i

Page 22: Lecture 6. Laminar Non-premixed Flames part 2. Bai Laminar Non-premixed Flames Where is the reaction zone? Zst Burnable mixture A F O 2 O 2 F F Fuel-rich mixing zone Reaction zone

X.S. Bai Laminar Non-premixed Flames

Burke-Schumann flame-sheet model

!!!t+"#!v

!= 0

!!Z!t

+"# (!!vZ) ="# (!""Z)

Yi = a + bZT = c+dZ

6 PDE equations

!!!v

!t+"!

!v!v ="# pI+!( )

!DhDt

!DpDt

="# !""h ! !" 1! 1Lei

$

%&&

'

())hi"Yi

i=1

N

*$

%&&

'

())+!Qr +# :"

"v

Burke-Schumann flame sheet relation

Page 23: Lecture 6. Laminar Non-premixed Flames part 2. Bai Laminar Non-premixed Flames Where is the reaction zone? Zst Burnable mixture A F O 2 O 2 F F Fuel-rich mixing zone Reaction zone

X.S. Bai Laminar Non-premixed Flames

Content

•  Structures of laminar non-premixed flames •  Mixture fraction •  Burke-Schumann flame-sheet model •  Jet diffusion flames •  Laminar diffusion flame at high mixing rate

Page 24: Lecture 6. Laminar Non-premixed Flames part 2. Bai Laminar Non-premixed Flames Where is the reaction zone? Zst Burnable mixture A F O 2 O 2 F F Fuel-rich mixing zone Reaction zone

X.S. Bai Laminar Non-premixed Flames

Finite-rate chemistry effect

•  Burke-Schumann flame-sheet model is not always true; it is true only when the chemical reactions are much faster than the mixing of fuel and the oxidizer

•  If the mixing is very fast, what is going to happen?

Zst

Burnable mixture

Page 25: Lecture 6. Laminar Non-premixed Flames part 2. Bai Laminar Non-premixed Flames Where is the reaction zone? Zst Burnable mixture A F O 2 O 2 F F Fuel-rich mixing zone Reaction zone

X.S. Bai Laminar Non-premixed Flames

Flamelet equation

!!Yi!t

+"#!Yiv!="#!Di"Yi +"i

Yi(x,y,z, t) =Yi(Z(x,y,z, t)),

!(x,y,z, t) =!(Z(x,y,z, t)),T(x,y,z, t) = T(Z(x,y,z, t))

Flamelet assumption:

!!Z!t

+"# (!!vZ) ="# (!D"Z)

Species transport

Mixture fraction

Page 26: Lecture 6. Laminar Non-premixed Flames part 2. Bai Laminar Non-premixed Flames Where is the reaction zone? Zst Burnable mixture A F O 2 O 2 F F Fuel-rich mixing zone Reaction zone

X.S. Bai Laminar Non-premixed Flames

Flamelet equation

!12!"d2YidZ2

=#i

d2YidZ2

= !2!i

"#

! = 2D(!Z "!Z) Scalar dissipation rate: mixing rate

Damköhler number Da = (mixing time)/(chemical reaction time) Da ! 2!i"#

Page 27: Lecture 6. Laminar Non-premixed Flames part 2. Bai Laminar Non-premixed Flames Where is the reaction zone? Zst Burnable mixture A F O 2 O 2 F F Fuel-rich mixing zone Reaction zone

X.S. Bai Laminar Non-premixed Flames

Finite rate chemistry effect

F O2

F O2

2

2id Y

dZ→∞

2

2 finiteid YdZ

=

Damköhler number infinity Damköhler not very high

iY iY

Z ZstZ

stZ

stZ

Page 28: Lecture 6. Laminar Non-premixed Flames part 2. Bai Laminar Non-premixed Flames Where is the reaction zone? Zst Burnable mixture A F O 2 O 2 F F Fuel-rich mixing zone Reaction zone

X.S. Bai Laminar Non-premixed Flames

Effect of mixing rate

F O2

iYiY

Z Z

χ ↑

χ ↑

χ ↑

stZ stZ

Increase of scalar dissipation rate leads to •  the leakage of fuel to the oxygen rich side increases •  the leakage of oxygen to the fuel rich side increases •  the flame temperature decreases, as a result of insufficient oxidation of

the fuel

Page 29: Lecture 6. Laminar Non-premixed Flames part 2. Bai Laminar Non-premixed Flames Where is the reaction zone? Zst Burnable mixture A F O 2 O 2 F F Fuel-rich mixing zone Reaction zone

X.S. Bai Laminar Non-premixed Flames

Flame quenching at high scalar dissipation rate

Adiabatic flame

With preheating

With radiation heat loss

Flame sheet Flamelet Quenched

PT

[ ]1P sχ −

qT

1qχ−

Page 30: Lecture 6. Laminar Non-premixed Flames part 2. Bai Laminar Non-premixed Flames Where is the reaction zone? Zst Burnable mixture A F O 2 O 2 F F Fuel-rich mixing zone Reaction zone

X.S. Bai Laminar Non-premixed Flames

Laminar jet diffusion flame

Air

A+P F+P

Lift-off hight

Diffusion flame

Lean premixed flame Rich premixed

flame

Fuel inlet

c

Zst

Burnable mixture

Page 31: Lecture 6. Laminar Non-premixed Flames part 2. Bai Laminar Non-premixed Flames Where is the reaction zone? Zst Burnable mixture A F O 2 O 2 F F Fuel-rich mixing zone Reaction zone

X.S. Bai Laminar Non-premixed Flames

Effect of mixng rate

•  For very small scalar dissipation rate the flame temperature is high; changing the scalar dissipation a little would not affect the flame temperature. This regime can be described by the simple Burke-Schumann flame sheet model.

•  For intermediate scalar dissipation rate, the flame temperature is lower than the Burke-Schumann flame temperature. Increasing the scalar dissipation rate leads to a decrease of the flame temperature until to a critical condition, at which the flame temperature changes rapidly. This regime may be called flamelet

•  For scalar dissipation rate higher than the quenching scalar dissipation rate, no flame exists. The flame is quenched.