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Igor Aleiner (Columbia) Theory of Quantum Dots as Zero-dimensional Metallic Systems Physics of the Microworld Conference, Oct. 16 (2004) Collaborators: B.L.Altshuler (Princeton) P.W.Brouwer (Cornell) V.I.Falko (Lancaster, UK) L.I. Glazman (Minnesota) I.L. Kurland (Princeton)
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Igor Aleiner (Columbia) Theory of Quantum Dots as Zero-dimensional Metallic Systems Physics of the Microworld Conference, Oct. 16 (2004) Collaborators:

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Page 1: Igor Aleiner (Columbia) Theory of Quantum Dots as Zero-dimensional Metallic Systems Physics of the Microworld Conference, Oct. 16 (2004) Collaborators:

Igor Aleiner (Columbia)

Theory of Quantum Dots as Zero-dimensional Metallic Systems

Physics of the Microworld Conference, Oct. 16 (2004)

Collaborators:B.L.Altshuler (Princeton)P.W.Brouwer (Cornell)V.I.Falko (Lancaster, UK)L.I. Glazman (Minnesota)I.L. Kurland (Princeton)

Page 2: Igor Aleiner (Columbia) Theory of Quantum Dots as Zero-dimensional Metallic Systems Physics of the Microworld Conference, Oct. 16 (2004) Collaborators:

Outline:• Quantum dot (QD) as zero dimensional metal• Random Matrix theory for transport in quantum dotsa) Non-interacting “standard models”.b) Peculiar spin-orbit effects in QD based on 2D electron gas.

• Interaction effects:a) Universal interaction Hamiltonian;b) Mesoscopic Stoner instability; c) Coulomb blockade (strong, weak, mesoscopic);

d) Kondo effect.

Page 3: Igor Aleiner (Columbia) Theory of Quantum Dots as Zero-dimensional Metallic Systems Physics of the Microworld Conference, Oct. 16 (2004) Collaborators:

“Quantum dot” used in two different contents:

“Artificial atom”

Description requires exact diagonalization.

“Artificial nucleus”

Statistical description is allowed !!!

(Kouwnehoven group (Delft))

Number of electrons:1)

(Marcus group (Harvard))

2)

For the rest of the talk:

Page 4: Igor Aleiner (Columbia) Theory of Quantum Dots as Zero-dimensional Metallic Systems Physics of the Microworld Conference, Oct. 16 (2004) Collaborators:

Random Matrix Theory for Transport in Quantum Dots

2DEGQD

L

Energy scales

2DEG Level spacing

Thouless Energy

ConductanceAssume:

Page 5: Igor Aleiner (Columbia) Theory of Quantum Dots as Zero-dimensional Metallic Systems Physics of the Microworld Conference, Oct. 16 (2004) Collaborators:

Statistics of transport is determinedonly by fundamental symmetries !!!

Reviews: Beenakker, Rev. Mod. Phys. 69, 731 (1997) Alhassid, Rev. Mod. Phys. 72, 895 (2000) Aleiner, Brouwer, Glazman, Phys. Rep., 309 (2002)

Original Hamiltonian: Confinement, disorder, etc

RMT

Page 6: Igor Aleiner (Columbia) Theory of Quantum Dots as Zero-dimensional Metallic Systems Physics of the Microworld Conference, Oct. 16 (2004) Collaborators:

No magnetic field, no SO

Magnetic field, no SO

No magnetic field, strong SO

Magnetic field + SO

Page 7: Igor Aleiner (Columbia) Theory of Quantum Dots as Zero-dimensional Metallic Systems Physics of the Microworld Conference, Oct. 16 (2004) Collaborators:

IV

Conductance of chaotic dotclassical Mesoscopic

fluctuations

Weak localization

Jalabert, Pichard, Beenakker (1994)Baranger, Mello (1994)

Page 8: Igor Aleiner (Columbia) Theory of Quantum Dots as Zero-dimensional Metallic Systems Physics of the Microworld Conference, Oct. 16 (2004) Collaborators:

IV

Conductance of chaotic dotclassical Mesoscopic

fluctuations

Weak localization

[Altshuler, Shklovskii (1986)]

Universal quantum corrections

Page 9: Igor Aleiner (Columbia) Theory of Quantum Dots as Zero-dimensional Metallic Systems Physics of the Microworld Conference, Oct. 16 (2004) Collaborators:

Peculiar effect of the spin-orbit interaction

Naively:SO

But the spin-orbit interaction in 2D is not generic.

Page 10: Igor Aleiner (Columbia) Theory of Quantum Dots as Zero-dimensional Metallic Systems Physics of the Microworld Conference, Oct. 16 (2004) Collaborators:

Spin-orbit interaction in GaAs/AlGaAs (001) 2DEG

- spin-orbit lengths

[001]

Rashba term

Dresselhaus term

Dyakonov-Perel spin relaxation

Page 11: Igor Aleiner (Columbia) Theory of Quantum Dots as Zero-dimensional Metallic Systems Physics of the Microworld Conference, Oct. 16 (2004) Collaborators:

Approximate symmetries of SO in QDAleiner, Fal’ko (2001)

T - invariance

But

Spin dependent flux Spin relaxation rate

Mathur, Stone (1992)

Khaetskii, Nazarov (2000)

Meir, Gefen, Entin-Wohlman (1989)

Lyanda-Geller, Mirlin (1994)

Page 12: Igor Aleiner (Columbia) Theory of Quantum Dots as Zero-dimensional Metallic Systems Physics of the Microworld Conference, Oct. 16 (2004) Collaborators:

Energy scales:

Brouwer, Cremers,Halperin (2002) May be violated for

Page 13: Igor Aleiner (Columbia) Theory of Quantum Dots as Zero-dimensional Metallic Systems Physics of the Microworld Conference, Oct. 16 (2004) Collaborators:

Effect of Zeeman splitting

Orthogonal, !!!

But no spin degeneracy; spins mixed:

New energy scale:

Page 14: Igor Aleiner (Columbia) Theory of Quantum Dots as Zero-dimensional Metallic Systems Physics of the Microworld Conference, Oct. 16 (2004) Collaborators:

6 possible symmetry classes:

Page 15: Igor Aleiner (Columbia) Theory of Quantum Dots as Zero-dimensional Metallic Systems Physics of the Microworld Conference, Oct. 16 (2004) Collaborators:

6 possible symmetry classes:

Page 16: Igor Aleiner (Columbia) Theory of Quantum Dots as Zero-dimensional Metallic Systems Physics of the Microworld Conference, Oct. 16 (2004) Collaborators:

Orbital effect of the magnetic field

Page 17: Igor Aleiner (Columbia) Theory of Quantum Dots as Zero-dimensional Metallic Systems Physics of the Microworld Conference, Oct. 16 (2004) Collaborators:

Orbital effect of the magnetic fieldObserved inFolk, Patel, Birnbaum, Marcus, Duruoz, Harris, Jr. (2001)

Page 18: Igor Aleiner (Columbia) Theory of Quantum Dots as Zero-dimensional Metallic Systems Physics of the Microworld Conference, Oct. 16 (2004) Collaborators:

Interaction HamiltonianEnergies smaller than Thouless energy:

Random matrix ????

In nuclear physics:

from shell model

random

Page 19: Igor Aleiner (Columbia) Theory of Quantum Dots as Zero-dimensional Metallic Systems Physics of the Microworld Conference, Oct. 16 (2004) Collaborators:

Universal Interaction HamiltonianEnergies smaller than Thouless energy:

are NOT random !!!

Kurland, Aleiner, Altshuler (2000)

Only invariants compatible with the circular symmetry

Page 20: Igor Aleiner (Columbia) Theory of Quantum Dots as Zero-dimensional Metallic Systems Physics of the Microworld Conference, Oct. 16 (2004) Collaborators:

Universal Interaction HamiltonianEnergies smaller than Thouless energy:

Valid if:

1)2) Fundamental symmetries

are NOT broken at larger energies

Random matrixNot random

Page 21: Igor Aleiner (Columbia) Theory of Quantum Dots as Zero-dimensional Metallic Systems Physics of the Microworld Conference, Oct. 16 (2004) Collaborators:

Universal Interaction HamiltonianEnergies smaller than Thouless energy:

Valid if:

1)2) Fundamental symmetries

are NOT broken at larger energies

One-particle levels determined by Wigner – Dyson statistics

Interaction with additional conservations

Zero dimensional Fermi liquid

Page 22: Igor Aleiner (Columbia) Theory of Quantum Dots as Zero-dimensional Metallic Systems Physics of the Microworld Conference, Oct. 16 (2004) Collaborators:

Universal Interaction Hamiltonian

Analogy with soft modes in metals

Singlet electron-holechannel.

Triplet electron-holechannel. Particle-particle

(Cooper) channel.

Page 23: Igor Aleiner (Columbia) Theory of Quantum Dots as Zero-dimensional Metallic Systems Physics of the Microworld Conference, Oct. 16 (2004) Collaborators:

Universal Interaction Hamiltonian

Cooper Channel:Renormalization:

Normal

Superconducting(e.g. Al grains)

Page 24: Igor Aleiner (Columbia) Theory of Quantum Dots as Zero-dimensional Metallic Systems Physics of the Microworld Conference, Oct. 16 (2004) Collaborators:

Universal Interaction Hamiltonian

Triplet Channel:is NOT renormalized

But may lead to the spin ofThe ground state S > ½.

Page 25: Igor Aleiner (Columbia) Theory of Quantum Dots as Zero-dimensional Metallic Systems Physics of the Microworld Conference, Oct. 16 (2004) Collaborators:

Mesoscopic Stoner Instability Kurland, Aleiner, Altshuler (2000)

Also Brouwer, Oreg, Halperin (2000)

vs.

Energy of the ground state:

NO randomness

NO interactions

FM instabilityStoner (1935)

random with known from RMTcorrelation functions

Spin is finite even for

Typical S:

Does not scale with the size of the system

Page 26: Igor Aleiner (Columbia) Theory of Quantum Dots as Zero-dimensional Metallic Systems Physics of the Microworld Conference, Oct. 16 (2004) Collaborators:

Universal Interaction Hamiltonian

Singlet Channel:is NOT renormalized

gate voltage

But

Q: What is charge degeneracy of the ground state

Page 27: Igor Aleiner (Columbia) Theory of Quantum Dots as Zero-dimensional Metallic Systems Physics of the Microworld Conference, Oct. 16 (2004) Collaborators:

- half-integer Otherwise

degeneracygap

(isolated dot)

Page 28: Igor Aleiner (Columbia) Theory of Quantum Dots as Zero-dimensional Metallic Systems Physics of the Microworld Conference, Oct. 16 (2004) Collaborators:

Coulomb blockade of electron transport

Term introduced by Averin and Likharev (1986);Effect first discussed by C.J. Gorter (1951).

For tunneling contacts:

Chargedegeneracy

Charge gap

Page 29: Igor Aleiner (Columbia) Theory of Quantum Dots as Zero-dimensional Metallic Systems Physics of the Microworld Conference, Oct. 16 (2004) Collaborators:

Small quantum dots Small quantum dots (~ (~ 500 nm500 nm))

M. Kastner, Physics Today (1993)E.B. Foxman et al., PRB (1993)

cond

ucta

nce

(e2 /

h)

gate voltage (mV)

In metals first observed in Fulton, Dolan, PRL, 59, 109, (1987)

Page 30: Igor Aleiner (Columbia) Theory of Quantum Dots as Zero-dimensional Metallic Systems Physics of the Microworld Conference, Oct. 16 (2004) Collaborators:

Coulomb blockade (CB) (II)

Strong CB

Weak CB

Mesoscopic CB

(reflectionlesscontacts) Random phase but

not period.

Page 31: Igor Aleiner (Columbia) Theory of Quantum Dots as Zero-dimensional Metallic Systems Physics of the Microworld Conference, Oct. 16 (2004) Collaborators:

Courtesy of C.Marcus

Statistical description of strong CB:

Theory:Peaks: Jalabert, Stone, Alhassid (1992);Valleys: Aleiner, Glazman (1996);Reasonable agreement,But problems with values of the correlationfields

Page 32: Igor Aleiner (Columbia) Theory of Quantum Dots as Zero-dimensional Metallic Systems Physics of the Microworld Conference, Oct. 16 (2004) Collaborators:

Mesoscopic Coulomb Blockade

Based on technique suggested by: Matveev (1995); Furusaki, Matveev (1995);Flensberg (1993).

Aleiner, Glazman (1998)

Page 33: Igor Aleiner (Columbia) Theory of Quantum Dots as Zero-dimensional Metallic Systems Physics of the Microworld Conference, Oct. 16 (2004) Collaborators:

Experiment:Cronenwett et. al. (1998)

SuppressionBy a factor of 5.3

Th: Predicted 4.

Page 34: Igor Aleiner (Columbia) Theory of Quantum Dots as Zero-dimensional Metallic Systems Physics of the Microworld Conference, Oct. 16 (2004) Collaborators:

Even-Odd effect due to Kondo effect

Spin degeneracy in odd valleys:

Effective Hamiltonian:

magnetic impuritylocal spin density of conduction electrons

Predicted:Glazman, Raikh (1988)Ng, Lee (1988)

Page 35: Igor Aleiner (Columbia) Theory of Quantum Dots as Zero-dimensional Metallic Systems Physics of the Microworld Conference, Oct. 16 (2004) Collaborators:

Observation:D. Goldhaber-Gordon et al. (MIT-Weizmann) S.M. Cronenwett et al. (TU Delft)J. Schmid et al. (MPI @ Stuttgart)

1998

van der Wiel et al. (2000)

200 nm

15 mK 800 mK

Page 36: Igor Aleiner (Columbia) Theory of Quantum Dots as Zero-dimensional Metallic Systems Physics of the Microworld Conference, Oct. 16 (2004) Collaborators:

Conclusions

1)Random matrix is an adequate description for the transport in quantum dots if underlying additional symmetries are properly identified.

2) Interaction effects are described by the Universal Hamiltonian (“0D Fermi Liquid”)