I 5 i r Proceedings ?f CONF- 700401 a GAS-COOLED REACTOR INFORMATION MEETING at the OAK RIDGE NATIONAL LABORATORY April 27-30, 1970 Oak Ridge Playhouse Oak Ridge, Tennessee li i f i 1 7 'A- .; ~ A .-- . United States Atomic Energy Commission. . 4 /' Division of Technical Information - _I_. - ,
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I
5
i r
Proceedings ?f
CONF- 700401
a
GAS-COOLED REACTOR INFORMATION MEETING
at the OAK RIDGE NATIONAL LABORATORY
April 27-30, 1970 Oak Ridge Playhouse Oak Ridge, Tennessee
li
i f i
1 7
' A - .; ~ A
.-- . United States Atomic Energy Commission.
. 4 /' Division of Technical Information -
_I_. - ,
DISCLAIMER
This report was prepared as an account of work sponsored by an agency of the United States Government. Neither the United States Government nor any agency Thereof, nor any of their employees, makes any warranty, express or implied, or assumes any legal liability or responsibility for the accuracy, completeness, or usefulness of any information, apparatus, product, or process disclosed, or represents that its use would not infringe privately owned rights. Reference herein to any specific commercial product, process, or service by trade name, trademark, manufacturer, or otherwise does not necessarily constitute or imply its endorsement, recommendation, or favoring by the United States Government or any agency thereof. The views and opinions of authors expressed herein do not necessarily state or reflect those of the United States Government or any agency thereof.
DISCLAIMER Portions of this document may be illegible in electronic image products. Images are produced from the best available original document.
I
L E G ’ A L N O T I C E This report was prepared a s an account of Government sponsored work. Neither the United States, nor the,Commission. nor any person acting on behalf of the Commission:
A. Makes any warranty or representation, expressed or implied, with respect to the accu- racy, completeness. or usefulness of the information contained in this report. or that the use of any information, apparatus. method, or process disclosed in this report may not infringe privately owned righte; or
B. Assumes any liabilities with respect to the use of, or for damages resulting from the use of any information, apparatus. method, or process disclosed in this report.
A s used in the above, “person acting on behalf of the Commission” includes any em- ployee or contractor of the Commission, or employee of such contractor, to the extent that such employee or contractor of the Commission, or employee of such contractor prepares, disseminates, o r provides access to. any information pursuant to his employment or contract with the Commission. or his employment with such contractor.
This report has been reproduced directly from the best available copy.
Printed in USA. P r i c e $10.00. Available f rom the Clearing- house for Federal Scientific and Technical Information, Na- tional Bureau of Standards, U. S. Department of Commerce, Springfield, Virginia 22151.
- --- CONF-700401
REACTOR TECHNOLOGY (TID -45 00)
.-
GAS-COOLED REACTOR INFORMATION MEETING
Proceedings of Meeting at the
OAK RIDGE PLAYHOUSE
Oak Ridge, Tennessee
April 27 - April 30, 1970
Sponsored by
Oak Ridge National Laboratory
Oak Ridge, Tennessee
L E G A L NOTICE This report was prepared as an account of work sponsored by the United States Government. Neither the United States nor the United States Atomic Energy Commission, nor any of their employees, nor any of their contractors, subcontractors, or their employees, makes any warranty, express or implied, or assumes any legal liability or responsibility for the accuracy, com- pleteness or usefulness of any information, apparatus, product or process disclosed, or represents that its use would not infringe privately owned rights.
-. .* .
iv
General Chairman:
Assoc ia te Chairman:
MEETING OFFICERS
D. B. Trauger, Oak Ridge Nat iona l Laboratory
J . H. Coobs, Oak Ridge Nat iona l Laboratory
Coordinator f o r Proceedings: E. R. Taylor , Oak Ridge Nat iona l Laboratory
Adminis tr a t i v e S e c r e t a r y : June L. Zachary, Oak Ridge Nat iona l Laboratory
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EDITORIAL NOTE
The papers and d i scuss ions incorpora ted i n t h e proceedings a r e
e d i t e d only t o t h e e x t e n t considered necessary f o r t h e r e a d e r ' s a s s i s t a n c e .
The views expressed and t h e gene ra l s t y l e - a d o p t e d remain, however, t h e
r e s p o n s i b i l i t y of t h e named au tho r s or p a r t i c i p a n t s .
The a f f i l i a t i o n s of au thors and p a r t i c i p a n t s a r e those given a t
t h e t i m e of t h e meeting.
The mention of s p e c i f i c companies or of t h e i r products o r brand-
names does no t imply any endorsement o r recommendation on t h e p a r t of
t h e Oak Ridge Nat iona l Laboratory.
vii
FOREWORD
Hel ium-cooled n u c l e a r r e a c t o r s o f f e r p o t e n t i a l f o r meet ing t h e major long- te rm requ i rements f o r e l e c t r i c power genera t i on . i n t o two c a t e g o r i e s : f i r s t , t h e High-Temperature Gas-Cooled Conver te r Reactor (HTGR o r HTR) t h a t uses g r a p h i t e f o r t h e f u e l s t r u c t u r e and moderator ; and second, t h e Gas-Cooled Fas t Breeder Reactor ( G C B R o r GCFBR) which has a c o r e composed o f m e t a l l i c - c l a d p i n s o f mixed uran ium-p lu ton ium o x i d e f u e l . o r a modern steam c y c l e f o r energy recove ry t o d r i v e t h e e l e c t r i c genera to r .
The r e a c t o r s f a l l
Both r e a c t o r s can be used w i t h e i t h e r a d i r e c t t u r b i n e c y c l e
Ma jor i n c e n t i v e s f o r a p p l i c a t i o n o f t h e HTGR a r e t h e p rospec ts f o r economica l l y c o m p e t i t i v e power p r o d u c t i o n w h i l e u t i l i z i n g more e f f e c t i v e l y t h e uranium o r e reserves. formance make p o s s i b l e h i g h burnup th rough which low f u e l - c y c l e c o s t s can be o b t a i n e d and ma in ta ined as uranium o r e c o s t s r i s e . tempera ture c a p a b i l i t y o f t h e g r a p h i t e co re s t r u c t u r e f a c i l i t a t e s o p e r a t i o n a t h i g h thermodynamic e f f i c i e n c i e s , and thus requ i rements f o r heat d i s s i p a t i o n t o t h e env i ronment a r e l o w . E x c e l l e n t r e t e n t i o n o f f i s s i o n p roduc ts and o t h e r r a d i o a c t i v e m a t e r i a l s appears t o be a c h i e v a b l e by t h e c o o l a n t c i r c u i t s housed i n c o n c r e t e p ressu re vesse ls ,
The e x c e l l e n t neu t ron economy and f u e l pe r -
The h i g h -
The he l ium-coo led GCBR o f f e r s a h i g h b reed ing r a t i o w i t h a f u e l d o u b l i n g t ime o f l e s s than 10 years , a c o r e convers ion r a t i o o f a p p r o x i - ma te l y 1.0, a smal l r e a c t i v i t y change f rom l o s s o f c o o l a n t , a p o t e n t i a l l y n o n r a d i o a c t i v e c i r c u i t , and h i g h thermal e f f i c i e n c y . The p r i n c i p a l ques t i ons concern ing t h e concept c e n t e r around t h e h igh -p ressu re c o o l a n t , p a r t i c u l a r l y f o r a f t e r h e a t removal f o l l o w i n g l o s s - o f - c o o l i n g a c c i d e n t s , and t h e performance o f m e t a l - c l a d ceramic f u e l e lements f o r r e l a t i v e l y h i g h tempera ture o p e r a t i o n , app rox ima te l y 700°C.
Development of gas-cooled r e a c t o r s for e l e c t r i c g e n e r a t i n g power s t a t i o n s has been under way i n t h e U n i t e d S ta tes s i n c e 1956 and f o r a l onger p e r i o d i n seve ra l European c o u n t r i e s . Four he l ium-coo led r e a c t o r s have opera ted - Peach Bottom, i n Pennsylvania, t h e AVR a t J U l i c h , Germany, t h e Dragon Reactor i n t h e South o f England, and UHTREX a t Los Alamos. Three o f t h e r e a c t o r s rep resen t e a r l y concepts f o r he l ium-coo led nuc lea r e l e c t r i c power s t a t i o n s . The f o u r t h , UHTREX, was modeled for d i r e c t use o f heat . The o p e r a t i n g exper ience w i t h these r e a c t o r s p r o v i d e s a broad b a s i s f o r new des igns and c o n t r i b u t e s g r e a t l y t o t h e p r o j e c t i o n o f HTGR pe r f o rma nce .
The Oak Ridge N a t i o n a l L a b o r a t o r y ho lds p e r i o d i c meet ings f o r t h e r e p o r t i n g o f i t s work i n gas-cooled r e a c t o r development. T h i s meet ing c o n s t i t u t e d an e x t e n s i o n t o p r o v i d e g r e a t l y inc reased p a r t i c i p a t i o n by o t h e r s . I n e f f e c t , t h e meet ing was conducted as an i n t e r n a t i o n a l symposium a t which comprehensive papers were presented on a l l aspec ts of gas-cooled r e a c t o r technology. The papers and d i s c u s s i o n a t t h e meet ing p r o v i d e d an o p p o r t u n i t y t o rev iew the t o t a l development program, t h e des ign concepts, and t h e o p e r a t i n g exper ience f rom gas-cooled r e a c t o r s w i t h emphasis on t h e HTGR which i s now e n t e r i n g t h e commercial f i e l d , An @
viii
important session at the meeting, however, was that on the gas-cooled fast breeder reactor held in conjunction with the Molten-Salt Breeder Reactor meeting. Here considerable advances in the study and analysis of safety problems for the GCBR indicated more clearly its feasibility and practicality. as having longer-term potential for reducing capital costs.
Direct helium turbine cycle systems were described
In the presentation o f these proceedings the Oak Ridge National Laboratory wishes to thank all o f those who participated in the meeting. Particular appreciation is expressed to the authors, the session chair- men, and panelists who were m o s t cooperative in providing abstracts, texts of papers, and discussion comments so that the timely preparation o f these proceedings would be possible.
D. B. Trauger
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I
CON TENTS
In t roductory Remarks . . . . . . . . . H. G . MacPherson, Deputy D i r e c t o r Oak Ridge Nat iona l Laboratory
SESSION I : WACTORS I N OPERATION
Chairman - J. S. Kemper, PE Co-Chairman - S. I . Kaplan, ORNL
B. G . Chapman, Dragon P r o j e c t . . . . . . . . . . . . . . . . . . . . . . . . . . . Operating Experience with t h e AVR Experimental Power S t a t i o n
Objec t ives and Plans f o r Fuel T e s t i n g i n t h e Peach Bottom HTGR (3/138) . . . . . . . . . . . . . . . . . . . . . . . . . . 60 K. P. Steward, GGA Discussion . . . . . . . . . . . . . . . . . . . . . . . . . . . . 89
SESSION I1 : PLANT CONSTRUCTION EXPERIENCE
Chairman - G . E . Locket t , Dragon P r o j e c t Co-Chairman - M. Bender, ORNL
F o r t S t . Vrain Construct ion Progress (1/105) 93 H. N . Wellhouser, GGA Discussion . . . . . . . . . . . . . . . . . . . . . . . . . . . 111
The Rela t ionship of t h e HTR with E a r l i e r Gas-Cooled Reactors
B. N . Furber, TNPG; C. S. Lowthian, TNPG
SESSION 111: H E R NEW AND ADVANCED DESIGNS
Chairman - J . D. Thorn, R i s l e y Co-Chairman - G. D. Whitman, ORNL
The High Temperature Reactor Development i n Germany (Present S i t u a t i o n , Program and Future Role) (1/101) . . . . . . . . . . . 145
Discussion . . . . . . . . . . . . . . . . . . . . . . . . . . . 160 H. K r ' a m e r , KFA
Design Fea tures and Engineer ing S t a t u s of t h e THTR 300 Mwe Prototype Power S t a t i o n (2/113) . . . . . . . . . . . . . . . . . 161 H. Oehme, BBK; J . Schgning, BBK Discuss ion . . . . . . . . . . . . . . . . . . . . . . . . . . . 179
X
The Layout of t h e Core and Fuel Elements of t h e TYTK (3/112) . . . . . . . . . . . . . . . . . . . . . . . . . . . . .
Large HTGR Design S t a t u s (Ul.21) . . . . . . . . . . . . . . . . . . K. Ehlers , BBK; H . Harder, BBK; E. Schrb'der, BBK Discussion . . . . . . . . . . . . . . . . . . . . . . . . . . . A . J. Goodjohn, GGA Discussion . . . . . . . . . . . . . . . . . . . . . . . . . . . Temperature Reactor and Helium Turbine (5/115) . . . . . . . . . -4. Yodzic, BBK; K. W . Marx W. TYvardziok, GHH; S. Fb'rster, KFA Discussion . . . . . . . . . . . . . . . . . . . . . . . . . . .
Conceptual Design f o r a 600 Mwe Xuclear Power P lan t with High
GHH; W . StrGmer, BBK;
Development Work f o r Large-Scale Helium Turbine P l a n t s with High Temperature Reactors .(6/117) . . . . . . . . . . . . . . . . . . E. Bbhm, GHH; W . Twardziok, GHH; H. Oehme, BBK; H. Weiskopf, BBC Discussion . . . . . . . . . . . . . . . . . . . . . . . . . . .
The Program of Plate-out I n v e s t i g a t i o n s i n t h e Gas Turbine P r o j e c t (7/127) . . . . . . . . . . . . . . . . . . . . . . . . . C. B. von d e r Decken, KFA Discussion . . . . . . . . . . . . . . . . . . . . . . . . . . .
The HTR Direct Cycle: Engineer ing P o s s i b i l i t i e s and Mater ia l Requirements (8/102) . . . . . . . . . . . . . . . . . . . . . . G. E. Locket t , Dragon P r o j e c t ; R . A. U. Huddle, Dragon P r o j e c t ; Discussion . . . . . . . . . . . . . . . . . . . . . . . . . . .
180
192 195
21 2
214
228
231
SESSION I V : PRESSURE VESSEL TECHNOLOGY AND SAFETY TOPICS
Chairman - T. A. Jaeger , BFM Co-Chairman - H. J . deNordwall, ORNL
S a f e t y Aspects of High Temperature Reactors (1/125) . . . . . . . . 293
of a Large HTR S t a t i o n (2/118) . . . . . . . . . . . . . . . . . 31-1
Discussion . . . . . . . . . . . . . . . . . . . . . . . . . . . 359 F i s s i o n Product Transport i n HTGR Systems - A Summary (3/104) . . . 361
F. P. 0. Ashworth, Dragon P r o j e c t The Rela t ion of F i s s i o n Product Release Limi ta t ions t o t h e Design
R . H. Flowers, AERE, Harwell
F. E . Vanslager, GGA; W. E . B e l l , GGA; 0. Sisman, ORNL; M. T. Morgan, ORNL
Shear F a i l u r e s i n End S l a b s of P r e s t r e s s e d Concrete Pressure
M. A . Sozen, U. of Ill.; W . C . Schnobrich, U. of 111.; S. L. Paul, U. of I l l .
I n v e s t i g a t i o n s of Time-Dependent Behavior of P r e s t r e s s e d Concrete Pressure Vessels (5/108) . . . . . . . . . . . . . . . . . . . . 403 J . P. Cal lahan, ORNL; J . M. Corum, ORNL; G. D. Whitman, ORNL Discussion . . . . . . . . . . . . . . . . . . . . . . . . . . . 431
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By T i t l e - Concrete Pressure Vessels - 1969 Assessment (6/-) . . . . . . . . . . . . . . . . . . . . . . . . H. Benzler, Euratom; J. Terps t ra , Euratom Oral s ta tement by D. D. Tytgat , Euratom
SESSION V : H E R FUEL ELFIvENT DESIGN, PERFORMANCE AND MANUFACTURE
Chairman - R. F. Turner, GGA Co-Chairman - , J. H. Coobs, ORNL
HTGR Fuel I r r a d i a t i o n Performance and Impl ica t ions on Fuel Design (1/131) . . . . . . . . . . . . . . . . . . . . . . . W . V . Goeddel, GGA; E. 0. Winkler, GGA; C. 2;. Luby, GGA Discussion . . . . . . . . . . . . . . . . . . . . . . . . .
Development of Bonded Beds of Coated P a r t i c l e s for HTGR Fuel Elements (2/107) . . . . . . . . . . . . . . . . . . . . . . J . L. Scott,,ORNL; J . A. Conlin, ORNL; J . H.. Coobs, ORNL; D. M. H e w e t t e 11, ORNL; J. M. Robbins, ORNL; R. L. Senn, ORNL D i s cus s i on . . . . . . . . . . . . . . . . . . . . . . . . . (3/132) . . . . . . . . . . . . . . . . . . . . . . . . . . . E. Smith, Dragon P r o j e c t Discussion . . . . . . . . . . . . . . . . . . . . . . . . .
The Development and Performance of HTR Core M a t e r i a l s (4/106) . L. W . Graham, Dragon P r o j e c t Discussion . . . . . . . . . . . . . . . . . . . . . . . . .
Choice of Fuel Design f o r Homogeneous Low Enriched HTR (5/126) . D. J . Merrett, TNFG; M. Gaube, Belgonucleaire D i scu s s i on
H. B a i r i o t , Belgonucleaire; L. Aerts, Belgonucleaire; R. A . Skinner, TNFG; J . Vangeel, CEN Discussion ; . . . . . . . . . . . . . . . . . . . . . . . .
HTR Fuel and M a t e r i a l s Development i n Germany, Present S i t u a t i o n and Program (7/128) . . . . . . . . . . . . . . . . . . . . . B. Liebmann, KFA; J . Bugl, GHH; K . Ehlers , BBK; K . G. Hackstein, NUKEM Discussion . . . . . . . . . . . . . . . . . . . . . . . . .
Behavior of Coated P a r t i c l e Fuel i n DFR I r r a d i a t i o n Experiments (8/133) . . . . . . . . . . . . . . . . . . . . . . . . . . . J. Baier , KFA; W. i n d e r Schmitten, NUKEM; P. Walger, BBK Discussion . . . . . . . . . . . . . . . . . . . . . . . . .
Experiments with t h e Production of AVR-Fuel Elements (9/116) . . K. G. Hackstein, NUKEM Discussion . . . . . . . . . . . . . . . . . . . . . . . . .
The Design of Pr i smat ic High Temperature Reactor Fuel Elements
SESSION V I : ECONOMICS OF HTGR FUEL RECYCLE AND POWER GENERATION
Chairman - H . B. S tewar t , GGA Co-Chairman - R . S . Carlsmith, ORNL
Thorium-Fuel-Reprocessing Research and Development work a t t h e KFA J z l i c h (1/136) . . . . . . . . . . . . . . . . . . . . . . . 62 1 J . Bohnenstingl, KFA; B. G. Brodda, KFA; 0 . Coenegracht, KFA; E . F i scher , KFA; G. K a i s e r , KFA; H . Kirchner, KFA; M. L a s e r , KFA; W . Litzow, KFA; E . Merz, KFA; H. J. Riedel, KFA; D. Thie le , KFA; U. Wenzel, KFA; H . W i e m e r , KFA; H. W i t t e , KFA; E . Z i m m e r , KFA
D. E . Ferguson, ORNL By T i t l e - Review of USAEC-ORNL HTGR Fuel Recycle Program (2/-) . . 647
Designs (3/135), P a r t I, P a r t I1 67 1 Some Fea tu res of t h e Low Enriched HTR f o r Various Fuel Element . . . . . . . . . . . . . . . .
G. Graz ian i , CCR Euratom - I s p r a ; C . R i n a l d i n i , CCR Euratom- I s p r a ; C. Zanantoni, CCR Euratom - I s p r a ; H . B a i r i o t , Belgonucleaire; P. Haubert, Belgonucleaire; G. G h i l a r d o t t i , AGIP Nucleare; M. Baur, GHH . . . . . . . . . . . . . . . . . . . . . . . . . . . Discussion 69 2
Comparison of HTGR Fuel Cycles f o r Large Reactors (4/130) . . . . . 694 R. C . Dahlberg, GGA D i s c u s s i o n 708
Po in t of V i e w (5/129) . . . . . . . . . . . . . . . . . . . . . 710
. . . . . . . . . . . . . . . . . . . . . . . . . . . Economics of Recycle i n LWR's and HTGR's i n t h e U.S.--A Consul tants
W . V . Macnabb, NUS; J . C. Scarborough, NUS . . . . . . . . . . . . . . . . . . . . . . . . . . . Parametr ic Survey on Fuel Cycles and To ta l Generating C o s t s f o r
HTR's w i th H o l l o w Rod, Te led ia l , and Tubular I n t e r a c t i n g Fuel
H . Gutmann, Dragon P r o j e c t ; J . Daub, Dragon P r o j e c t ; H . Schnober, Dragon P r o j e c t ; C. R ina ld in i , Euratom-Ispra; G. Graz ian i , Euratom-Ispra; J . J o u r n e t , CEA; J . Malherbe, CEA Discussion . . . . . . . . . . . . . . . . . . . . . . . . . . . 7 52
. . . . . . . . . . . . . Evening Program - HTGR's and Greenhouses 7 55 S . E . B e a l l , OFDL
. . . . . . . . Panel Discussion - Prospects f o r t h e Next Ten Years 765
J. A. Lane, ORNL; C. L. Rickard, GGA; R . D. Vaughan, TNPG; K. Wirtz, KFK
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SESSION V I I : GAS-COOLED FAST REACTOR DESIGN, SAFETY STUDIES AND FUEL DEVELOPMENT
Chairman - C. A . Rennie, P. Co-Chairman - P. P a t r i a r c a , ORNL
The GCFR Demonstration P l a n t Design (1/119) . . . . . . . . . . . . G a s Turbine Power Conversion Systems f o r Helium Cooled Breeder
P. Fortescue, GGA; W . I . Thompson, GGA
Reactors (2/114) . . . . . . . . . . . . . . . . . . . . . . . . L. A . Lys, EIR; G. Ciszewski, SGI; H . F ru t sch i , BST
(3/139) . . . . . . . . . . . . . . . . . . . . . . . . . . . . H. B a i r i o t , Belgonucleaire ; J . M. Tiromson, Belgonucleaire; L. A e r t s , Be3gonucleaire D i s c u s s i o n . . . . . . . . . . . . . . . . . . . . . . . . . . . (4/123) . . . . . . . . . . . . . . . . . . . . . . . . . . . . M. D a l l e Donne, Gfk; E . Eisemann, GfK; K. Wirtz, Gfk
Development ‘of Coated P a r t i c l e Fuel f o r a Gas E%reeder Reactor
La te s t Ca lcu la t ions f o r a GCFR wi th a Vanadium Clad Pin C o r e
R . B. F i t t s , OWL; J . R . Lindgren, GGA; E . I,. Long, ORNL; D. R . Cuneo, ORNL Discussion . . . . . . . . . . . . . . . . . . . . . . . . . . . J . M. Waage, GGA; J . A . Larrimore, GGA
S a f e t y S tud ie s f o r t h e Gas-Cooled Fas t Reactor (6/109) . . . . . . Discussion . . . . . . . . . . . . . . . . . . . . . . . . . . .
S a f e t y And Af terhea t Removal S tud ie s of t h e Gas-Cooled Fas t Reactor (7/110) . . . . . . . . . . . . . . . . . . . . . . . . C. S . Walker, ORNL D i s c u s s i o n . . . . . . . . . . . . . . . . . . . . ; . . . . . .
Aspects of Gas-Cooled Fas t Reactor Development a t ENEA . . . . . . W. F. Haussermann
79 5
81 2
833
852
8 54
861 864
878 879
890
90 3 904
. . . . . . . . . 907 Fas t Breeder Reactors, N o t LMFBR o r GCFR--but FBR Compton A . Rennie, P
Welcome t o Tennessee and t o t h e Oak Ridge Nat ional Laboratory.
a r e deeply honored and pleased t o p l ay h o s t t o such a d i s t ingu i shed
ga the r ing of expe r t s on h igh temperature gas-cooled r e a c t o r s . If t h e r e
i s anything we can do t o make your s t a y he re more p l easan t , p l ease l e t us know.
We
Since t h i s i n t e r n a t i o n a l meeting on gas-cooled r e a c t o r s i s be ing
he ld i n Oak Ridge, I t h i n k it i s appropr i a t e t o pay t r i b u t e t o t h e e a r l y
e f f o r t s of Fa r r ing ton Daniels . P ro fes so r Daniels had a l l t h e r i g h t s e n t i -
ments and motives t o win approval of t h i s audience - t h e only t r o u b l e was
t h a t he was a c t i v e about 10 years t oo e a r l y .
t h e Meta l lu rg ica l Laboratory, now t h e Argonne Nati-onal Laboratory, he
proposed a pebble bed r e a c t o r t o use a mixture of g ranh i t e and uranium
ca rb ide pebbles or b a l l s .
t o p re sen t day s tandards . H e suggested such th ings a s ope ra t ion a t
2000 OC, a r e a c t o r diameter of 35 f e e t t o ope ra t e on n a t u r a l uranium,
cool ing with e i t h e r H e or b o i l i n g bismuth, and d i s t i l l i n g Pu and f i s s i o n
products for t h e r e a c t o r dur ing ope ra t ion .
I n 1944, i n what was then
This was a r a t h e r advanced proposa l according
These ideas l e d t o t h e a u t h o r i z a t i o n of t h e Power P i l e P r o j e c t i n
1946. T h i s was a helium-cooled BeO-moderated r e a c t o r , c a l l e d the Daniels
P i l e , which was t o be b u i l t i n Oak Ridge. Although t h i s r e a c t o r p r o j e c t
was canceled be fo re it was two yea r s o ld , t h e group of engineers t h a t was
assembled f o r t h i s purpose went on t o b u i l d t h e U. S. submarine r e a c t o r .
Fa r r ing ton Daniels d id not g ive up, d e s p i t e t h e o f f i c i a l discourage-
ment. H e modified h i s ideas , and made a s p e c i f i c proposa l of a more
simple graphite-moderated gas-cooled r e a c t o r i n 1950. This r e a c t o r pro-
posa l was very s p e c i f i c f o r t h e ope ra t ion of a gas t u r b i n e using N2 a s a
coolan t , and he even went t o t h e t r o u b l e of l o c a t i n g a v a i l a b l e gas t u r -
b ines and g e t t i n g quota t ions on t h e i r d e l i v e r y . This proposal f e l l on
deaf e a r s , b u t back a t t h e Un ive r s i ty of Wisconsin Daniels continued h i s
r e sea rch a c t i v i t i e s .
xvi
I n 1955 w e had some correspondence a t a t ime when he was seeking a
method of s e a l i n g uranium f u e l t i g h t l y i n smal l p ieces of g raph i t e .
was then wi th t h e Carbon Products Div is ion of Union Carbide Corporation,
and we provided him wi th our t hen b e s t e f f o r t a t a small sealed g raph i t e
capsule .
i n 1956 proposing a helium-cooled r e a c t o r based on t h i s f u e l .
h i s major i n t e r e s t tu rned t o s o l a r energy a s a h e a t source f o r backward
coun t r i e s .
I
This was no t q u i t e good enough, b u t Daniels d id publ i sh a paper
Af t e r t h a t
It i s too bad t h a t Danie ls ' enthusiasm and e f f o r t had t o come 10
yea r s t o o soon, both from a p o l i t i c a l and a t e c h n i c a l p o i n t of view.
The world was no t ready f o r commercial nuc lea r power when he s t a r t e d , and
he was not ab le 60 p e r s i s t long enough t o be rescued by t h e development
of p y r o l y t i c a l l y carbon-coated f u e l p a r t i c l e s , a s t h e r e s t of you have
been.
u c t r e t e n t i o n by p y r o l y t i c coa t ings i s t h e most important s i n g l e advance
i n gas-cooled r e a c t o r technology s i n c e Fa r r ing ton Daniels s t a r t e d i n 1944, i n t h a t it makes gas-cooled r e a c t o r s c r e d i b l e from a commercial p o i n t of
view.
It i s my per sona l op in ion t h a t t h e d iscovery of t r u e f i s s i o n prod-
1
mACTORS I N OPERATION
(Sess ion I)
2
Chairman : J . S. Kemper, ’
Phi l ade lph ia Electr ic Company
Co-Chairman: S . I . Kaplan, Oak Ridge National Laboratory
Paper 1/137 2' 0
DRAGON OPERATING EXPERIENCE .ur
--ly
B. G. Chapman I -'1 0 j' ;? 0 OECD Dragon P r o j e c t
' I
ABSTRACT
The u s e of Dragon as a f u e l i r r a d i a t i o n f a c i l i t y has generated a g r e a t d e a l of experience i n ope ra t iona l areas svch as helium u t i l i s a - t i o n and engineer ing , maintenance of helium c i r c u i t s , a c t i v i t y behaviour i n HTR c i r c u i t s , and t h e d e t e c t i o n and clean-up of chemical impur i t i e s . yea r s a t Dragon.
The paper desc r ibes t h i s experience over t h e l a s t f i v e
It i s f r equen t ly d i f f i c u l t t o p r e d i c t t h e ope ra t iona l performance of l a r g e p l a n t s from t h e drawing board and t h e ch ie f va lue of exper ience i s t o e s t a b l i s h t h e p r a c t i c a l l i m i t s which can be achieved. I n t h i s r e s p e c t Dragon has demonstrated t h e e s s e n t i a l v i a b i l i t y of t h e HTR concept and has enabled r e a l i s t i c design c r i te r ia t o be l a i d down.
3
4
A
INTRODUCTION
Dragon was b u i l t t o prove an i d e a and t h e h e a r t of t h a t i d e a was a
r e a c t o r core cons t ruc ted e n t i r e l y of g r a p h i t e and ceramic nuclear
f u e l s , and cooled with helium.
of t h e r e a c t o r experiment w e r e secondary t o t h a t of c r e a t i n g t h e
c o r r e c t environment f o r t h e ope ra t ion of such a core.
many des ign f e a t u r e s w e r e int roduced which are not t y p i c a l of a
commercial HTR plant . Nevertheless , i n a d d i t i o n t o f u e l t e s t i n g , a
g r e a t d e a l of experience and informat ion has accrued from t h e P r o j e c t
t o guide des igne r s of f u t u r e systems.
A l l o t h e r cons ide ra t ions i n t h e design
For t h i s reason
Since t h e r e a c t o r f i r s t achieved f u l l power i n A p r i l , 1966, f o u r
y e a r s of development have gone i n t o t h e ope ra t ion and maintenance
techniques app l i cab le t o the HTR.
15 d i f f e r e n t core l ayou t s have been i r r a d i a t e d and some major
d i f f i c u l t i e s overcome. I n p a r t i c u l a r , s i n c e t h e first b o i l e r tube
f a i l u r e i n February, 1967, t h e r e a c t o r has been dogged by water-side
cor ros ion t r o u b l e s - of almost no re levance t o t h e concept of t he HTR.
Dozens of t ubes have been plugged and 13 b o i l e r changes c a r r i e d out .
This has had a s e r i o u s e f f e c t on u t i l i s a t i o n . During Charge I1
u t i l i s a t i o n w a s 52.5% (about 60% of t h e t a r g e t set by cons ide ra t ions
of f u e l changing). For Charge I11 t he corresponding figures are 50%
and 68% (Fig. 1) ” *. There can be l i t t l e doubt t h a t , wi thout t h e
b o i l e r problem, over 90% of t h e des i r ed i r r a d i a t i o n would have been
achieved. The t i m e t h a t has been l o s t i n i r r a d i a t i o n , however, has
provided va luable experience i n maintenance and ope ra t ing techniques
and it i s p r imar i ly with t h i s a spec t t h a t t h i s paper i s concerned.
F ive main areas w i l l be considered.
Three f u e l charges cons is t ing of
The Performance of Large Sca le H e l i u m C i r c u i t s and Associated Components
The use of an expensive coolan t such as helium p laces c i r c u i t
leakage uppermost i n t h e des igne r s ’ mind. The t a r g e t leakage ra te of
O.l%/day, t o which Dragon w a s designed, has become almost t r a d i t i o n a l - y e t it i s impossible t o r e l a t e t o des ign d a t a f o r components.
5
The d i f f u s i o n of helium through metals can be below t h e l i m i t s of
d e t e c t i o n provided t h a t c a r e f u l s e l e c t i o n and c o n t r o l a r e exerc ised .
For i n s t a n c e , some leakage may be expected along a r o l l e d b a r and
small diameter cover p l a t e s must be made from r o l l e d p l a t e ( i n which
imperfec t ions are l a t e r a l ) and no t from b a r ( i n which imperfec t ions are
l o n g t i t u d i n a l ) . S imi la r ly , welds of good s tandard may be expected t o
show n e g l i g i b l e leakage.
f o r imperfec t ions r a t h e r than conformity with a des ign predic t ion .
Since, i n t h e absence of imperfec t ions , t h e leakage should be
vanish ingly small, t h e tes t s p e c i f i c a t i o n becomes r e l a t e d t o t h e
s e n s i t i v i t y of t h e test procedure.
developed by Wade
e i t h e r i n t h e vacuum mode (component evacuated i n a helium atmosphere)
o r a s " s n i f f e r s " (component p re s su r i sed wi th helium o r hel ium/ni t rogen
mixture). S e n s i t i v i t y can be increased and t h e o v e r a l l t e s t i n g of
l a r g e components s impl i f i ed by "bagging" i n polythene and al lowing
helium build-up i n t h e bag f o r a s p e c i f i e d period.
leakage rates a t least two o r d e r s of magnitude less than O.l%/day can
be measured.
Thus most components are t e s t e d pr imar i ly
The Dragon l eak t e s t i n g r o u t i n e s 3 are based upon s p e c i f i e d mass-spectrometers used
By these means,
Turning t o j o i n t s and seals, it i s poss ib l e t o l a y down average
performance d a t a from l abora to ry tests.
used on Dragon have a t y p i c a l leak ra te of 1 x 10 a ta cm /s/ft a t
25 a t m . ra te of 3 x 10-7%/day4' 5.
an e x c e l l e n t poss ib l e performance b u t are mostly very s e n s i t i v e t o
f l e x i n g and thermal cycl ing.
leakage from each coupl ing may be very s m a l l , they are used i n l a r g e
numbers widely d i s t r i b u t e d i n space.
The s i l v e r gaske t j o i n t s -8 3
There are 600 f t of such gaske t s i n Dragon leading t o a leak
Small p ipe coupl ings and "Conoseals" have
The problem he re i s t h a t a l though t h e
From t h i s i t can be seen t h a t a t a r g e t figure of O.l%/day makes a
It a l s o sets a problem f o r generous allowance f o r t h e f r a i l t y of man. o p e r a t o r s i n t h a t l eak rates of t h i s o rde r can be very d i f f i c u l t t o
d e t e c t , l e t a lone measure.
i s t o carry ou t r e g u l a r coolan t balances.
v e s s e l s , p ipes , etc., be provided with p re s su re and temperature
The usua l r o u t i n e i n gas cooled r e a c t o r s
This r e q u i r e s t h a t a l l
6
monitoring so t h a t gas con ten t s can be ca l cu la t ed .
ba lances are c a r r i e d out weekly and al though g r e a t care i s taken with
instrument c a l i b r a t i o n and Van de Waals d e v i a t i o n s from t h e p e r f e c t gas
l a w s are taken i n t o account, experience shows t h a t an accuracy of 23%
i s typ ica l .
temperatures ranging from 150 C t o 830 C, i s d i f f i c u l t t o assess. Thus
helium ba lances w i l l no t show a O.l%/day l e a k ra te i n under f o u r weeks.
A t Dragon such
I n p a r t i c u l a r t h e con ten t of t h e primary c i r c u i t , wi th 0 0
It has been poss ib l e , a t Dragon, t o measure t h e t o t a l unaccountable
leakage by use of t h e containment bui ld ing .
cont inuously v e n t i l a t e d by an open c i r c u i t system with a complete a i r
in te rchange every 22 hours.
by a mass-spectrometer which has been c a l i b r a t e d by making measured r e l e a s e s of helium i n t o t h e bui ld ing . By t h i s means w e f i n d t h a t a
l eak ra te of 0.045%/day g ives 100 vpm of helium i n air. Fig. 2 shows
a t y p i c a l h i s t o r y from which it can be seen that normal leak rates l i e
between 0.025 and 0.05%/day. The assessment of human f r a i l t y seems
s u r p r i s i n g l y co r rec t .
Fig. 3 shows t h e t o t a l usage of helium over t h e same period,
This bu i ld ing i s
The helium i n a i r concent ra t ion i s measured
computed from helium balances.
l o s s e s are h igh compared with those c a l c u l a t e d from Fig. 2.
are three reasons f o r t h i s :
It i s apparent t h a t t h e unaccountable
There
( a ) Losses occur dur ing shutdown when t h e mass-spectrometer i s no t
used because t h e containment bu i ld ing doors are open.
( b ) Large l e a k s (shown by peaks on Fig. 2 ) are usua l ly co r rec t ed
be fo re t h e helium-in-air measurement h a s equ i l ib ra t ed .
(c ) Usage of helium f o r chemical a n a l y s i s i s not metered accu ra t e ly
and a no t iona l figure i s used i n t h e balances. It would not be
economically j u s t i f i e d t o improve t h i s s i t u a t i o n .
The most important conclusion from our experience i s t h a t t h e
t o t a l usage of helium f a r outweighs t h e loss by leakage. I n a
commercial HTR t h i s w i l l be even more t rue . Usage i n purging on-load
r e f u e l l i n g machines and mul t ip l e s tand pipe c l o s u r e s w i l l be h igher
than t h a t r equ i r ed f o r t h e Dragon machinery and leakage should be less
A
A
7
(expressed as a d a i l y percentage) .
complex areas such as instrument and a n a l y s i s small bore l i n e s and no t
from t h e l a r g e vesse ls . Since Dragon i s very h ighly instrumented,
leakage experience i s probably pess imis t i c .
W e f i n d most leaks arise from
What l e s sons can des igne r s l e a r n from t h i s ?
A l eak r a t e of O.l%/day should be comfortably achievable.
Helium-in-air monitoring i s by f a r t h e quickes t and most s e n s i t i v e
technique f o r c o n t r o l l i n g leakage. If poss ib l e , r e a c t o r b u i l d i n g s
and v e n t i l a t i o n p l a n t should be designed t o f a c i l i t a t e t h i s .
Wherever poss ib l e , components should be s p e c i f i e d on a Itno
d e t e c t a b l e leak" basis. Although t h i s cannot be defended i n
terms of t o t a l leakage it g r e a t l y f a c i l i t a t e s t h e maintenance of
l o w backgrounds and s i m p l i f i e s l eak d e t e c t i o n and loca t ion . If
t h e component manufacturing i n d u s t r i e s are encouraged t o th ink i n
t h e s e terms, t h e economic penal ty need not be s i g n i f i c a n t .
A l o w p re s su re c o l l e c t i o n system and recovery compressors are
essent ia l . A s much a s poss ib l e of t h e p l a n t should be designed f o r evacuat ion
t o m i n i m i s e purging l o s s e s p r i o r t o major maintenance.
A computing data logger capable of producing r o u t i n e helium
balances would h e l p i n l o c a t i n g major leaks.
Ear ly r ecogn i t ion of p o s s i b l e l u b r i c a t i o n problems i n oxygen-free
helium l e d t o ex tens ive t e s t i n g i n t h i s area. The design and construc-
t i o n of Dragon however, preceded much of t h i s work and t h e fact t h a t no
bear ing s e i z u r e has occurred i n t h e primary circuit must be a t t r i b u t e d
t o des ign r a t h e r t han any s t a r t l i n g new materials. Wherever poss ib l e ,
bear ings (always r o l l i n g surfaces) are pos i t ioned i n low temperatures
and f l u x e s , mechanisms are designed t o accept h igh c learances , speeds
and t o t a l d u t i e s are low, and grease packing i s used. Experience has
shown t h a t sea led greased bea r ings do no t produce s i g n i f i c a n t
contamination. Greases are se l ec t ed f o r m i n i m u m tendency t o genera te
ttgummytl r e s i d u e s and later developments i nc lude oxygen r e l e a s i n g
8
add i t ives . Where condi t ions preclude t h e use of grease , s tandard
bear ings ( 3 dot-pressed cage) a r e used a f t e r N i t a l e tch ing and MoS
treatment .
d e t a i l s can be found i n . A u s e f u l summary of design
d e s i d e r a t a i s contained i n .
2 Bearings have been designed f o r more arduous duty and
6, 7, 8, 9 , 10
11
A des ign of p a r t i c u l a r i n t e r e s t i s t h e use of o i l ba th l u b r i c a t i o n
These boxes are loca ted i n cool r eg ions i n the c o n t r o l rod gear-boxes.
and are connected t o t h e main v e s s e l by p res su re tubes which ca r ry t h e
d r i v e sha f t s . Normal nuc lear grade o i l s , a f t e r degassing, perform
w e l l , and no foaming has been encountered on depressur i sa t ion . This
technique would appear i d e a l l y s u i t e d f o r PCRV app l i ca t ion .
The bear ing types r e f e r r e d t o are s u i t a b l e only €or l i g h t loads ,
moderate speeds and occas iona l use. The main c i r c u l a t o r s c l e a r l y
r e q u i r e a more r a d i c a l approach and gas bea r ings were se l ec t ed f o r
Dragon, t hus avoiding t h e r o t a t i n g s h a f t seal problem. During t h e
100,000 t o t a l machine hours t o d a t e , no machine has f a i l e d i n normal
se rv ice . Four f a i l u r e s have occurred, a l l a t m i n i m u m i d l e speed
(1,500 rpm) i n n i t rogen a t 1 a ta . Two of t h e s e w e r e considered t o be
due t o d e f i c i e n t jacking gas f low a t s t a r t -up , one t o l o s s of dynamic
balance due t o a loose nose f a i r i n g and t h e o the r t o water i n g r e s s
fol lowing a h e a t exchanger tube f a i l u r e . I n a l l cases i n t e r m i t t e n t
bear ing temperature rises preceded t h e f a i l u r e by seve ra l hours and
t h e machines r a n normally u n t i l they w e r e d e l i b e r a t e l y stopped. They
then re fused t o restart. I n a d d i t i o n t o t h e above f o u r machines, two
have been s t r i p p e d f o r r o u t i n e examination a f t e r about 16,000 hours
and found t o be i n e x c e l l e n t condi t ion. The only se rv ic ing requi red
has been minor reba lanc ing t o the s p e c i f i c a t i o n of 0.5 g cm.
C i r c u l a t o r r e l i a b i l i t y i s usua l ly a central po in t i n t h e sa fe ty
O u r experience would i n d i c a t e t h a t a n a l y s i s of gas cooled r e a c t o r s .
gas bea r ings have p a r t i c u l a r l y favourable c h a r a c t e r i s t i c s i n t h i s
respec t .
speed, t h e machine experiences i t s most d i f f i c u l t tes t a t s t a r t -up and
i d l e speed opera t ion . Thus, i f a machine starts s a t i s f a c t o r i l y , we
Since t h e bear ing sepa ra t ing f o r c e s r ise so r a p i d l y with
9
0 have confidence i n i t s i n t e g r i t y f o r normal high speed duty. To tes t
the machine's a b i l i t y t o withstand a primary c i r c u i t f a i l u r e , one
c i r c u l a t o r w a s depressur i sed a t 50 p s i / s , on a test r i g . N o bear ing
touch occurred, indeed, t h e bear ing capac i ty measurement ind ica t ed a
n e g l i g i b l e change i n c learance.
F i n a l l y , some mention must be made of diaphragm compressors.
These machines have been t h e cause of cons iderable d i f f i c u l t y on a l l
c u r r e n t HTR p lan ts . Fig. 4 shows t h e genera l improvement i n diaphragm
l i f e from about 100 hours , 5 y e a r s ago, t o i n excess of 1 ,000 hours
cu r ren t ly . This improvement has been achieved p a r t l y by modi f ica t ions
and p a r t l y by improved ope ra t iona l technique. A s suppl ied , t he
machines had t r i p l e diaphragms, two mild steel on t h e o i l s i d e and one
s t a i n l e s s s t e e l on t h e gas s ide . These were assembled dry. It has
been found p re fe rab le t o f i t t he s t a i n l e s s diaphragm between the mild
s t e e l ones and t o smear them with o i l be fo re assembly. Changes have
been made t o t h e i n t e r s t a g e pressure c o n t r o l l e r , t h e o i l and water
coo le r s , and an o i l catch-pot with o i l d e t e c t o r f i t t e d t o t h e d ischarge
l i n e . A sump o i l l e v e l gauge t o d e t e c t o i l loss has a l s o been
i n s t a l l e d . Operat ional r o u t i n e s have been devised t o avoid excess ive
hammering and s t r e s s i n g of t h e diaphragms. These inc lude unloaded
s t a r t i n g , minimised running a g a i n s t low d ischarge p res su res , p ressure
relief on shutdown and the avoidance of sub-atmospheric pressures at
i n l e t . As a r e s u l t of t h e s e changes, t h e performance of t h e
compressors i s acceptab le although w e cont inue t o be i n t e r e s t e d i n
more r e c e n t developments such as the "roll-sock" machines.
Summarising, our experience with t h e Dragon helium c i r cu i t s , I
consider t h a t , a s t he r e s u l t of conserva t ive design, c a r e f u l
maintenance and monitoring and t h e s teady improvement t o components
and opera t ing r o u t i n e s , w e have now reached t h e s t a g e of a f f i rming
t h a t helium cool ing i s e n t i r e l y p rac t i cab le . I am convinced t h a t t h e
m e r i t s of helium cool ing can be r e a l i s e d without excess ive economic o r
ope ra t iona l demands.
10
The Behaviour of F i s s i o n Products ii? the Primary C i r c u i t
T h e primary c i r c u i t a c t i v i t y l e v e l s i n Dragon are low by aln?osk
any power r e a c t o r s tandards. OY course, experimental and explora tory
f u e l s a r e d e l i b e r a t e l y p ro tec t ed by t h e purge system b u t i n r e c e n t
cores the f r a c t i o n of f u e l purged i s small (Charge I1 -35% Charge 111
Core 8 -24%)).
indicat . ion of cond i t ions app l i cdb le t o power r e a c t o r design.
Nevertheless , r e l a t i v e l y small d i f f e r e n c e s i n f u e l p a r t i c l e design,
f u e l p i n geometry and opera t ing cond i t ions can a f f e c t a c t i v i t y r e l e a s e
s t rong ly - p a r t i c u l a r l y i n r e s p e c t of those i s o t o p e s of low v o l a t i l i t y
and high tendency t o p la te -out on g raph i t e o r metal sur faces . Thus i n
Dragon P r o j e c t work, p r e d i c t i o n s of a c t i v i t y l e v e l s i n power H T R ' s a r e
be ing based on two foundat ions.
i s being assessed us ing t h e o r e t i c a l models.
c a l c u l a t i o n s i s no t being taken from d i rec t measurements of Dragon
primary c i r c u i t a c t i v i t i e s . This would be too crude and l i a b l e t o
e r r o r . In s t ead , the d e t a i l e d informat ion coming from purge gas
measurements and s t u d i e s of f i s s i o n product d i s t r i b u t i o n s i n the
p a r t i c l e s , compacts and f u e l tubes of i r r a d i a t e d elements, i s used a s
t h e b a s i c data . The need f o r t h i s i s f u r t h e r r e in fo rced by the s h o r t
i r r a d i a t i o n t i m e s i n Dragon as compared with t h e power r e a c t o r .
Thus the primary c i r c u i t a c t i v i t i e s g ive a v a l i d
Release from power r e a c t o r f u e l p ins
The d a t a f o r these
The o t h e r foundat ion i s t h e use of t h e Dragon Reactor t o study t h e
behaviour of r e l eased f i s s i o n products a s they move around t h e primary
c i r c u i t . It i s t h i s a spec t which w i l l be discussed here.
It i s p o s s i b l e t o a f f i r m now t h a t gas-born a c t i v i t y per se i n a
HTR w i l l no t c o n s t i t u t e a problem. That i s t o say, d i r e c t r a d i a t i o n
from coolant duc t s and p ipes w i l l be small. Equally, l eaks from t h e
c i r c u i t should not p re sen t a hazard. There are f o u r v i t a l ques t ions
which must be answered (and upon which f u e l des ign c r i t e r i a w i l l r e s t ) .
( a ) What w i l l be t h e long-term a c t i v i t y build-up on components which
need maintenance o r i n spec t ion?
11
( b ) How much deposi ted a c t i v i t y w i l l exist i n t h e c i r c u i t which could
be r e l eased under s e r i o u s acc ident condi t ions?
(c ) What a r e t h e problems of decontamination?
( d ) HOW can f a i l i n g f u e l be b e s t loca ted be fo re s e r i o u s r e l e a s e
r e s u l t s ?
The s t a r t - p o i n t f o r t hese s t u d i e s i s t h e de te rmina t ion of a f u l l
a c t i v i t y burden s p e c i f i c a t i o n f o r t h e coolant .
For a number of yea r s , f i s s i o n product a c t i v i t y l e v e l s i n the
primary c i r c u i t w e r e measured e i t h e r by an i n s t a l l e d continuous f low
P chamber o r by the counting of d i s c r e t e gas samples on a Y-spectro-
meter. The p c6unter was c a l i b r a t e d with Xe-133 and f o r t h i s reason
gas a c t i v i t i e s a r e usua l ly expressed a s "Xe-133 equiva len ts" . There
i s no doubt t h a t t h i s method y i e l d s a reasonable e s t ima te of bulk gas
a c t i v i t y which i s v a l i d f o r e s t ima t ing r a d i a t i o n l e v e l s from duc t s ,
e t c . Typical va lues i n Dragon a r e low, e.g., 1,000 pCi/cm3 o r 0.4 C i
t o t a l c i r c u l a t i n g a c t i v i t y . y-spectrometry of {gas samples r a r e l y
showed any d e t e c t a b l e a c t i v i t y o the r than rare (gases and f o r t h i s
reason the presence of 1-131, Sr-90, Cs-137, etc., i n the gas was not
suspected. Fu r the r confirmation of t h i s view w a s suggested by the lack
of 1-131 i n b o i l e r water which had been subjected t o a f low of primary
c i r c u i t gas through leaking tubes.
Deta i led s t u d i e s of a l l b o i l e r s and blowers removed from t h e
r e a c t o r however, revealed measurable q u a n t i t i e s of Iodine , Caesium and
Strontium.
c i r c u l a t i n g i n t h e coolan t b u t t h e o r i g i n a l sampling techniques f a i l e d
t o d e t e c t them - probably because those a c t i v i t i e s w e r e deposi ted on
t h e l i n e s lead ing t o the chambers o r sample b o t t l e s . A new sampling
system known a s a "Dracule" (Fig. 5 ) has t h e r e f o r e been i n s t a l l e d
which draws a sample of primary c i r cu i t gas as c lose a s p o s s i b l e t o
the core exit.
removable tube with a con t ro l l ed temperature g rad ien t . A f t e r
removal, depos i ted a c t i v i t y can be assayed with a y-spectrometer. A
There was thus no doubt t h a t s o l i d f i s s i o n products w e r e
The gas sample i s then cooled by passing it through a 15
12
number of v a r i a t i o n s are poss ib le . The tube may be f i t t e d with f i l t e r s
o r i s o - k i n e t i c heads f o r dus t sampling and may have s p e c i a l l y prepared
ac t iva t ed su r faces , e t c . A t y p i c a l p r o f i l e f o r 1-131 i s shown i n
Fig. 6 taken from . One unexpected discovery i s t h a t Xe-133 i s q u i t e
s t rongly absorbed on the tube surface.
15
By use of t h e Dracule and t h e gas sampling systems a t o t a l gas
impuri ty s p e c i f i c a t i o n can be der ived. Short-term measurements be fo re
a shut down can then be r e l a t e d t o t h e deposi ted short- l ived
a c t i v i t i e s found on t h e su r faces of r e a c t o r components removed during
the shu t down. T h i s i s of p a r t i c u l a r i n t e r e s t f o r 1-131. T h e
assessment of accumulation of long-lived i so topes such a s Cs-137
r e q u i r e s a t i m e i n t e g r a t i o n of c i r c u i t l e v e l s and the i n s t a l l a t i o n of
new b o i l e r s and c i r c u l a t o r s with known a c t i v i t y l e v e l s w i l l provide a
s u i t a b l e base l i n e f o r t h i s purpose.
Shor t ly be fo re t h e shut down f o r t h e i n s t a l l a t i o n of new b o i l e r s ,
t h e primary c i r c u i t a c t i v i t y was unusual ly high having a t o t a l
s p e c i f i c a t i o n a s i n Table 1.
A s soon a s components w e r e removed from t h e primary c i r c u i t they
were assayed f o r depos i ted a c t i v i t y . The fo l lowing r e s u l t s f o r 1-131
t y p i c a l :
From the su r face of t he s t a i n l e s s steel nose cone of t h e b o i l e r s
which r u n s a t about 735OC, 5 t o 10 x pCi/cm2 was removed by
methanol s t r y g i 1.
From t h e su r face of b o i l e r t ubes (Fig. 7 ) - mild s t e e l a t about
205-235 C - 10-20 pCi/cm . The l e v e l s of i od ine do not appear
t o vary much with t h e angle of inc idence of t h e gas.
suppor ts t h e view t h a t t h e i o d i n e i s i n gaseous r a t h e r than
p a r t i c u l a t e form; Deposi t ion of i s o t o p e s such a s Cs-137 i s
s t rong ly dependent on t h e gas f low d i r e c t i o n .
0 2
This
From t h e blower i m p e l l e r s - a l l o y steel a t about 330°C - on t h e
t r a i l i n g faces of t h e vanes 20 pCi/cm2 and on t h e lead ing f a c e s
2 p C i / c m . 2 This d i f f e r e n c e i s probably accounted f o r by the
13
s i g n i f i c a n t l y g r e a t e r d u s t deposi t i -on on the t r a i l i n g f aces .
0 ( d ) Cn the Nimonic-75 coolan t duc t runnir,g a t about 740 C no 1-131
2 could be de tec ted . The main a c t i v i t - 1 was Cs-137 a t 0.14 p C i / c m . This value i s of i n t e re s t since it r e p r e s e n t s a s i t u a t i o n s i m i l a r
t o t h a t cf a d i r e c t cyc le gas t u r b i n e blade.
The methods used t o remove a c t i v i t y f o r assay provide some c l u e s
t o t h e problems of a c t i v i t y r e l e a s e under acc ident cond i t ions and t h e
d i f f i c u l t i e s of maintenance and decontamination.
r e s u l t s obtained with methanol and phosphoric ac id s t r y g i l s and t h e
"electroleech". I n add i t ion p l a s t i c (BEX) f i l m has been used. Perhaps
t h e most s i g n i f i c a n t f a c t i s t h a t removal of a c t i v i t y from s t a i n l e s s
steel i s d i f f i c u l t compared with mild steel presumably because the
oxide f i l m i n t o which t h e a c t i v i t y d i f f u s e d i s much more adherent.
l6 de scribe s t h e
The Chemistry of H e l i u m C i r c u i t s
The choice of an i n e r t coolan t f o r t h e HTR would a t f i r s t s i g h t
seem t o e l imina te t h e normal concern regard ing cor ros ion of t h e core
assembly. Unfortunately, ( f o r two r e a s o n s ) , chemical e f f e c t s cannot
be neglected. F i r s t l y , a t i n i t i a l commissioning and a f t e r t h e loading
of new f u e l , some absorbed gases w i l l be introduced. Secondly, i f t h e
HTR i s employed with a steam cyc le , some in leakage of steam must be
expected and, i f o i l i s used as a l u b r i c a n t i n the c i r c u i t , some
hydrocarbon contamination w i l l arise.
of des ign and opt imis ing ope ra t iona l procedures, a clear under-
s tanding of t h e chemical r e a c t i o n s of t r a c e i m p u r i t i e s i n helium i s
requi red . I n CO cooled r e a c t o r s , t h e moderate temperatures lead t o a
s i t u a t i o n i n which r a d i o l y t i c r e a c t i o n s assume precedence over those
with thermally con t ro l l ed k i n e t i c s and i n - p i l e experiments are
e s s e n t i a l t o d e f i n e t h e des ign cri teria. This s i t u a t i o n needed
i n v e s t i g a t i o n f o r t he HTR.
Thus both f o r t h e purposes
2
Dragon provides an i d e a l environment f o r conducting experiments
The normal on t h e i n j e c t i o n of i m p u r i t i e s i n t o t h e primary c i r cu i t .
impuri ty l e v e l s are extremely low a s shown i n Table 2.
14
The achievement of t h e s e l e v e l s has been aided by a number of
des ign f e a t u r e s (such a s a steam pres su re below t h a t of t he primary
c i r c u i t ) some of which are no t poss ib l e i n a commercial p l a n t where
l e v e l s would be expected t o be higher . The only s e r i o u s pe r tu rba t ion
on t h e above p i c t u r e , arises from waters ide cor ros ion on t h e b o i l e r s .
When se r ious b o i l e r cor ros ion was occurr ing , t h e primary c i r c u i t
hydrogen l e v e l s rose , a t t i m e s up t o 40 vpm, b u t it i s hoped t h a t
t h e new b o i l e r s and water t rea tment methods w i l l s t a b i l i s e t h e
hydrogen below 0.5 vpm.
A l a r g e number of experiments have been c a r r i e d out12 us ing both
" s ing le shot" and continuous i n j e c t i o n s . A t y p i c a l r e s u l t from a slow
water i n j e c t i o n i s shown i n Fig. 8. Space does not permit a d e t a i l e d
analysis here , b u t the fo l lowing genera l conclusions can be drawn.
( a ) For Water I n j e c t i o n s
(i) The r e a c t i o n s a r e s imple f irst order with r e s p e c t t o water
i n agreement with l abora to ry experiments.
A (t i) The "water s h i f t " r e a c t i o n H 0 + CO - H 0 + CO can be 2 2 2 neglected under Dragon condi t ions.
(iii) Carbon depos i t i on r e a c t i o n s can be neglected (even though
'H / H 0 >lo) because of t h e long induc t ion per iod before
metal su r f aces become c a t a l y t i c a l l y a c t i v e (-lo4 hours a t
100 vpm CO) .
C 2 2
( i v ) No oxygen pick-up i s observed i n t h e gaseous cons t i t uen t s .
( v ) Mass ba lances show t h a t only about 65% of the water reacts
quickly. The rest i s absorbed and presumably r e l eased
slowly over a long period.
( b ) For Gaseous I n j e c t i o n s (H CO, C 0 2 , CH4) 2'
(i) Oxygen pick-up i s observed. The source of oxygen i s
unconfirmed b u t assumed t o be metal oxides. This e f f e c t i s
more marked with CO than H 2-
15
Table 1. Primary C i r c u i t A c t i v i t y Concent ra t ions (end of Core 7 Charge 111)
Isotope Method of Measurement Act . ivi ty Concent ra t ion 3 g i / m
~ ~~
A l l g a s e s Ion chamber 13,500
Xe-133 Y-spec. sample 9 50
Xe-135 Y-spec. sample 4,700
Kr-8 5m Y-spec. sample 2 , 900
Kr-87 y-spec. sample 4,200
1-131 "Dracule 'I 19
CS-137
Ag-111
"Dracule"
"Dracule"
Data c o l l e c t e d n o t y e t analysed
Table 2. Typica l Primary C i r c u i t Impur i ty Levels
Impuri ty P.C. Level L i m i t of Detec t ion
VPm VPm
H2°
H2
co
CH4
2 0
~
< 0.05
0.3
0.16
<0.04
<0.02
0.05
0.05
0.08
0.04
0.02
~~
Table 3 . Core Water/Graphite React ion Rate Cons tan ts
Charge Core Power
Mw
Rc h- l
I 4 20 0.35
I1 1 20 1.02
I1 2 18 0.90
I11 4 ( a ) 15 5.3
111 4 ( a ) 20 10.3
I11 6 20 4.0
I11 7 20 2.2
16
( c ) Hydrocarbon I n j e c t i o n s
(i) Cracking proceeds r a p i d l y through decreas ing molecular weight
hydrocarbons t o hydrogen and methane. The longer term
r e a c t i o n s a r e those a s soc ia t ed with these two gases. Oxygen
pick-idp occurs.
A t t h i s s t age i n t h e development of t he HTR, t he most important
conclusion i s ( a ) (i) because it confirms t h a t out-of-pile experiments
can give v a l i d des ign data .
The r a t e cons t an t f o r t he f i r s t order r e a c t i o n with water i s of
g r e a t s ign i f i cance not only because of i t s impl i ca t ions on core
cor ros ion b u t because it i s t h e v i t a l parameter i n sa fe ty s t u d i e s on
the e f f e c t s of b o i l e r f a i l u r e s producing explosive water gas. The
r e a c t i o n r a t e r ises so sharply with temperature that a f e w small a r e a s
of high su r face temperature g raph i t e can completely outweigh t h e rest
of the core. Th i s i s shown dramat ica l ly i n Table 3.
It can be seen t h a t t h e r e has been a genera l t r end towards
i n c r e a s i n g r a t e cons t an t s b u t Charge I1 Core 4 ( a ) had an outs tandingly
h igh value. This was due t o the i n t r o d u c t i o n of some c e n t r a l l y cooled
elements which had a small a r ea of g r a p h i t e su r face a t about 1200°C.
When small a r e a s of t h e core can e x e r t such a c o n t r o l l i n g in f luence
it w i l l be apprec ia ted t h a t t h e o r e t i c a l p r e d i c t i o n s of r a t e cons tan t
a r e d i f f i c u l t b u t some success i s being achieved. The ca l cu la t ed
value f o r Charge I11 Core 4 ( a ) i s 10.5 h - l ( c f . 10.3 experimental)
b u t such agreement i s admit tedly f o r t u i t o u s .
A r e g u l a r s e r i e s of i n j e c t i o n experiments i s c a r r i e d ou t f o r
success ive co res i n Dragon. These, as can be seen, from t h e above,
y i e l d o v e r a l l core f i g u r e s d i f f i c u l t t o i n t e r p r e t e i n t e r m s of b a s i c
d a t a b u t of d i r e c t re levance i n confirming t h e continued a p p l i c a b i l i t y
of t h e r e a c t o r s a f e t y c learance . They a r e b e s t descr ibed a s
" e f f e c t i v e temperature" measurements (weighted by sur f ace a rea and an
Arrhenius temperature r e l a t i o n s h i p ) .
A new series of experiments i s about t o commence us ing special
f u e l elements i n core p o s i t i o n O/O. Arrangements have been made t o
17
r eve r se t h e normal purge flow on t h i s element, so t h a t wet helium can
be passed over t h e f u e l boxes. These boxes can then be removed f o r
d e t a i l e d examination t o determine weight loss, depth of pene t r a t ion
of cor ros ion , t h e e f f e c t of i r r a d i a t i o n on r a t e cons tan t by modifica-
t i o n of t h e g raph i t e s t r u c t u r e , etc.
Spec ia l Instruments f o r HTR's
The r a p i d impuri ty r e a c t i o n s and t h e i r s e l e c t i v e a t t a c k upon
l imi t ed core a reas requires t h e maintenance of except iona l ly low l e v e l s
of impuri ty . The f i r s t ope ra t iona l requirement i s a r e l i a b l e set of
a n a l y t i c a l ins t ruments capable of ope ra t ing down to l e v e l s a t l e a s t an
order of magnitude less than those normally of i n t e r e s t .
The instrument s e l ec t ed f o r water measurement a t Dragon was the
Goldsmith-Cox e l e c t r o l y t i c hygrometer developed €o r use a t high
pressures , This instrument i s simple and r e l i a b l e , i s capable of being
made absolu te and improves i n s e n s i t i v i t y a s t h e pressure i s increased
( i n terms of vpm l e v e l s s ince it b a s i c a l l y measures absolu te water
p re s su res and c o l l e c t s more e f f i c i e n c l y a t low gas v e l o ~ i t i e s ) ' ~ .
u l t i m a t e s e n s i t i v i t y i s determined by leakage c u r r e n t s a r i s i n g from
contaminants and imperfec t ions i n t h e phosphoric ac id /g lycer ine f i lm.
Although capable of d e t e c t i n g 0.003 vpm H 0 i n 20 a t a helium i n t h e
l abora to ry , p l a n t experience suggests t h a t 0.05 vpm i s a p r a c t i c a l
f i g u r e f o r ope ra t iona l use.
explore t h e pulsed use of t hese instruments . Higher c u r r e n t s w i l l be
obtained by us ing in t e r ruped e l e c t r o l y s i s and i t i s hoped t h a t a
f u r t h e r decade of s e n s i t i v i t y w i l l be obta ined; t h a t i s a u s e f u l l i m i t
of 0.002 vpm a t a c i r c u i t p re s su re of 60 a ta . The development of a
process-type i n d i c a t i n g and supply system should not p re sen t any
d i f f i c u l t y .
The
2
Experiments a r e a t p resent i n progress t o
The above instrument has also been success fu l ly proved a s a
hydrogen monitor by preceding t h e hygrometer with a small copper oxide
furnace a t 400°C. S e n s i t i v i t i e s a r e i d e n t i c a l with those f o r water.
18
The o t h e r irnpuni.ties of i n t e r e s t (CO, CO,], 0 CH4, PJ and - 2’ 2
hydrocarbons) are measured Gsing a d i f f e r e n t i a l concen t r a t ion gas
chromatograph . I n t h i s ins t rument i m p u r i t i e s a r e absorbed on l i q u i d
n i t rogen cooled t r a p s and then r e l e a s e d thnoujn a inolecular s i e v e t o a
katharometer. This c o n s t r u c t i o n a t 0nc.e achieves concen t r a t ion f a c t o r s
of m 0 r . e thar! 100 and elirninatee t h e l e a k s and s t agnan t pockets
a s s o c i a t e d with sampling va lves (F igs . 9 and 10). Three types of
chromatograph have been b u i l t . One uses a n i t rogen c a r r i e r f o r
de t e rn in ing hydrogen and helium i n steam c i r c u i t padding gas , t h e
second a helium c a r r i e r f o r i:se i n any helium c i r c u i t app l i ca t ion .
The t h i r d type i s a p o r t a b l e multipurpose ins t rument designed f o r
d i r e c t attachment t o t h e p l a n t where t h i s was p r e f e r a b l e to t ak ing
samples t o t h e l a b o r a t o r y ins t ruments . The minimum l e v e l s d e t e c t a b l e
wi th confidence by these machines are shown i n Tahle 4.
14
rdblt. 4. ivlinim,m Impurity Levels De tec t ab le oy D i f f e r e n t i a l Concent ra t ion Chromatograplis (with Katharometer De tec to r )
Impur i ty L i m i t of Detec t ion
A 0.02 vpm i n 20 a t a heliam
O 2
2 N
0.02 vpm i n 20 a t a he l i lm
0.04 vpm i n 20 a t a helium
0.04 vpm. i n 20 a t a helium
CO 0.08 vpm i n 20 a t a helium
CH4
0.02 vpm i n 20 a t a helium c02
Such s e n s i t i v i t y i s remarkable cons ider ing t h e use of a katharo-
meter and experiments are now s t a r t i n g wi th t h e u s e of a helium
i o n i s a t i o n d e t e c t o r . This system has been used mainly with an argon
carr ier bu t should have g r e a t e r s e n s i t i v i t y wi th h igh p u r i t y helium
a s i t e x p l o i t s t h e h igh i o n i s a t i o n and e x c i t a t i o n p o t e n t i a l s of t h e
r a r e gases. Improvements of one and p o s s i b l y two decades of
s e n s i t i v i t y are hoped f o r .
19
THE MAINTENANCE OF HELIUM CIRCUITS
It i s n a t u r a l f o r o p e r a t o r s cons ider ing t h e maintenance of an HTR
primary c i r c u i t t o be concerned by t h e absence of m e t a l l i c c ladding of
t h e f u e l and p o s s i b l e consequent a c t i v i t y hazards. Fuel loaded i n t o an
HTR w i l l b e suppl ied t o a release s p e c i f i c a t i o n which i s n o t zero a s
wi th o t h e r r e a c t o r s a t p re sen t i n use. The hard l e s s o n of exper ience
i n p r e s e n t power r e a c t o r s i s , however, t h a t even i n t h e absence of some
f a i l e d f u e l (and some f a i l e d f u e l i s t h e usua l s i t u a t i o n ) , very s ign i -
f i c a n t r a d i a t i o n hazards develop from a c t i v a t e d crud o r co r ros ion
products , The minimal co r ros ion i n t h e ETR e l imina te s t h i s problem and
one i s concerned only with t h e f u e l i n t e g r i t y . Many u t i l i t i e s a r e
r i g h t l y f i r m i n t h e i r demands t h a t b o i l e r and blower i n s p e c t i o n should
be p o s s i b l e throughout t h e l i f e of t h e s t a t i o n . T h i s requirement
r e so lves i tsel f i n t o two main a reas .
c e n t r e around 1-131 and h e r e Dragon exper ience j.s very r e l evan t . On
t h e o t h e r hand long-lived i s o t o p e s such a s Cs-137 g ive r ise t o a direct
r a d i a t i o n hazard bu t Dragon exper ience cannot be taken d i r e c t l y because
of t h e r e l a t i v e l y s h o r t h i s t o r y .
The problems of i nges t ed a c t i v i t y
Between November, 1969 and March, 1970, Dragon Lias shutdown f o r a
complete replacement of t h e b o i l e r s and steam loops, A s a test case,
very c a r e f u l measurements were taken of r a d i a t i o n l e v e l s , body burdens,
and Contamination levels around the p lan t . Shortly before shutdoLm,
t h e primary c i r c u i t a c t i v i t y l e v e l was unusual ly h igh and e s t ima tes
i n d i c a t e about 1 2 C i of 1-131 e x t e r n a l t o t h e f u e l p a r t i c l e s . A t t h e
t i m e of opening t h e c i r c u i t t h i s would have decayed t o about 1.5 C i .
A s a matter of i n t e r e s t t h i s amount of 1-131 i s s u f f i c i e n t t o produce
one maximum pe rmis s ib l e concen t r a t ion f o r i n h a l a t i o n (mpc) i n about
2 x 1 0 rn of a i r o r 2.5 x 10 containment bu i ld ing volumes. Sirice
under maintenance cond i t ions wi th open a i r - locks , one a i r chdnge occurs
i n about 10 hours i t can be seen t h a t a f r a c t i o n a l release r a t e of
about 4.5 x p e r hour of t h e " f r ee" i o d i n e would g ive r i se t o
1 mpc i n t h e containment bui ld ing . The h i g h e s t genera l a i rbo rne l e v e l
was about 1 mpc - an a s ton i sh ing ly small r e l ease .
8 3 4
20
P r i o r t o opening t h e c i r c u i t , t h e helium atmcsphere was exchanged
with dry n i t rogen t o minimise convection e f f e c t s a t t h e open f l anges
(about 80 c m i n d iameter ) .
containment during removal of t h e b o i l e r s and c i r c u l d t o r s . A f t e r
removal each f l a n g e was c losed with a simple l i g h t a l l o y cover with an
i n f 1 a t a b l e seal.
Apart from t h i s no attempt was made a t
1 7 The c i r c u l a t o r s were drawn back on r a i l t r o l l e y s and sheeted
wi th PVC a s soon as c l ea rance w a s a v a i l a b l e (Fig. 11). The r a d i a t i o n
l e v e l s on t h e impe l lo r s w e r e gene ra l ly about 200 mr/h a t 1 ft.
masks were worn a s a p recau t ion dur ing t h i s phase although n o t e s s e n t i a l .
The h i g h e s t a i r b o r n e 1-131 l e v e l i n t h e a c t u a l opening was 45 mpc.
man who worked f o r about an hour around t h e open h o l e without an a i r
mask was found subsequently t o have a thy ro id burden of 170 pCi compared wi th t h e ICRP permi t ted l e v e l of 700 pCi f o r continuous working.
A i r
One
The b o i l e r s w e r e withdrawn v e r t i c a l l y i n t o PVC s l e e v e s (Fig. 32)
and gave r a d i a t i o n l e v e l s of about 50 m r / h P/y on c o n t a c t wi th t h e
p l a s t i c shee t .
a i r masks w e r e n o t worn. I n o r d e r t o minimise r e l e a s e a t t h e openings
a s m d l l s u c t i o n w a s maintained on t h e thermocouple branches lower clown
t h e duc ts . This i s a u s e f u l technique worthy of a p p l i c a t i o n elsewhere
although i t probably i n c r e a s e s t h e oxygen contamination of t h e n i t rogen
b l anke t gas.
c i r c u l a t o r s , which l a s t e d about 4 weeks, no person was exposed t o
i n t e r n a l o r e x t e r n a l r a d i a t i o n t o a l e v e l imposing any i n d i v i d u d
r e s t r i c t i o n s .
Airborne release dur ing t h i s phase was n e g l i g i b l e and
During t h e whole process of changing 6 b o i l e r s and
Contamination c o n t r o l proved excep t iona l ly s t r a igh t fo rward . A
l o c a l c o n t r o l a r e a was set up immediately ad jacen t t o t h e primary
c i r c u i t openings and a c o v e r a l l and overshoe r c u t i n e e s t ab l i shed .
t h i s means t h e spread of contamination t o t h e main containment bu i ld ing
w a s l i m i t e d t o an e x t e n t t h a t "blue" a r e a cond i t ions appl ied
By
2 pCi/cm and no p r o t e c t i v e c l o t h i n g w a s requi red . I n t h e g r e a t
ma jo r i ty of t h e containment bu i ld ing p u b l i c access would have been
permiss ib le .
2 1
Summarising, a major maintenance opera t ion has been c a r r i e d o u t on
Dragon with primary c i r c u i t condi t ions a t l e a s t a s severe a s t hose
expected on a power HTR.
e i t h e r i n r e s p e c t of t h e mechanical ope ra t ions o r t h e con t ro l of
r ad ia t ion . The c o r e remained f u l l o f i r r a d i a t e d f u e l throughout t h i s
process and t h e experience sugges ts t h a t maintenance may w e l l be
quicker and e a s i e r than on o t h e r r e a c t o r types.
During t h e per iod fol lowing shutdown, a b o i l e r tube f a i l u r e
N o s i g n i f i c a n t d i f f i c u l t i e s were encountered,
r e l eased some water i n t o the primary c i r c u i t and t h e w a t e r l e v e l reached
5.5%. I n add i t ion t o t h i s when t h e c i r c u i t was n i t rogen blanketed
wi th open f l a n g e s , some a i r in leakage occurred and a t one s t a g e t h e
oxygen concent ra t ion reached 1%. A f t e r r ec los ing , t h e c i r c u i t w a s
evacuated and f i l l e d w i t h c l ean helium. By t h i s means, t h e "free"
contaminants w e r e reduced t o a low l e v e l which was f u r t h e r improved by
t h e ope ra t ion of t h e clean-up p l a n t s during t h e l a t t e r s t a g e s of t h e
s h u t down. However, it was expected t h a t cons iderable absorp t ion of
impuri ty on t h e co re and r e f l e c t o r g r a p h i t e would t a k e place. These
i m p u r i t i e s would no t be removable u n t i l d r iven o f f by t h e c i r c u i t heat-
i n g as t h e approach t o power took place.
seen i n Fig. 13.
rises i n impuri ty l eve l . I n o rde r t o minimise co re cor ros ion each rise i s reduced by t h e clean-up p l a n t s before t h e next s t e p i s applied.
T h i s process can be c l e a r l y
Large temperature s t e p s are accompanied by sharp
A fu r the r complicat ing f a c t o r w a s t he i n j e c t i o n of hydrogen
produced from forming t h e magnet i te f i l m on t h e new bo i l e r s .
experience has shown t h a t hydrogen d i f f u s e s r a p i d l y through t h e tubes
from i t s p o i n t of formation.
above t h e equi l ibr ium H /H 0 = 8 /1 which would be expected a t f u l l
power. This equi l ibr ium i s shown as a do t t ed l i n e i n Fig. 1 3 from
which it appears t h a t t h e hydrogen no t produced from water i s f a l l i n g
slowly, e.g., from 3.0 vpm on 28th March t o 0.8 vpm on 1st April . The
carbon monoxide l e v e l i s seen t o fo l low the hydrogen l e v e l q u i t e
c l o s e l y and again t o fo l low about an 8/1 r e l a t i o n with water.
P a s t
For t h i s reason t h e hydrogen l e v e l s t a y s
2 2
22
The most s i g n i f i c a n t demonstrat ion f r c m this process i s t h e small
uptake of w a t e r and oxygen by t h e c o r e durinq open-c i rcc i t maintenance
i n s p i t e of very high contarninan’i l eve l s .
ACKNOWLEDGMENTS
The experience descr ibed i n t h i s review i s c u l l e d from 5 years
e f f o r t s by Dragon Operat ions and P r o j e c t S t a f f t oo numerous t o mention
by name.
t h e p r i v i l e g e of r epor t ing such a convincing demonstration of t h e
v i a b i l i t y of t h e HTR concept.
I thank both them and t h e Chief Execut ive, Dragon P r o j e c t f o r
REFERENCES
1.
2.
3.
4.
5.
6.
7.
8.
9.
10 .
C. Hunt and M. D. Joyce, Opera t iona l Data f o r Charge I, D.P. Report 561, (1967).
C. Hunt and L. J. Poston, Operat ional Data f o r Charge 11, D.P. Report 614, (1969).
F. Wade, Dragon P r o j e c t Helium Leak Tes t ing , D.P. Report 2 2 5 , (1963 1 . H. J. Woodley, Development Work on S e a l s - Experimental Work c a r r i e d o u t by t h e Component Development Group t o Determine t h e Ef fec t iveness of Various Sea l ing Systems Proposed f o r U s e on t h e Draqon P r o j e c t , D.P. Report 251, (1963).
W. E. Simmons, Flanqed Joints f o r Draqon Primary C i r c u i t - Pre l iminary Report , D.P. Report 197, (1963).
H. F r i c k e r , Pre l iminary Report on D r y Bearings f o r t h e Dragon Reactor Experiment, D.P. Report 24 , (1961).
G. W. Horsley and H. F r i c k e r , The S e l e c t i o n of Greases f o r t h e Lubr ica t ion of Bearinqs i n t h e Draqon Reactor , D.P. Report 51 , (1961).
G. Coast , Some Enqineerinq Problems Associated with t h e Draqon Reactor Experiment, D.P. Report 129 (1962).
H. F r i c k e r , Bearings and Gears f o r Operation i n I n e r t Gases, D.P. Report 163, (1963).
H. F r i c k e r , Bearing T e s t s - A Summary of Work Done up t o December, 1964, D.P. Report 386, (1965).
n
23
11. J. R. Dean, Control Rod System and Mechanisms f o r Hiqh-Temperature Gas-Cooled Power Reactor with Feed and Breed Fuel , P a r t 2 , D.P. Report 457, (1967).
1 2 . M. C a r l y l e and D. V. Kinsey, Resu l t s of t h e I n j e c t i o n of Impur i t i e s i n t o t h e Dragon Reactor P r i m a r y Coolant , D.P. Report 544, (June, 1969).
13. P. S. Gray and I. Gordon, J. Sci . Instrum Vol. 44, (1967).
14. P. S. Gray, D. R. O w e n s and L. 0. Green, A D i f f e r e n t i a l Con- c e n t r a t i o n G a s Chromatograph €or t h e Analysis of Low Levels of Impur i t i e s i n H e l i u m , D.P. Report 443, (1966).
15. P. R. Rowland, M. C a r l y l e and G. C. Soubel-et , The D i s t r i b u t i o n of F i s s i o n Products i n a High Temperature G a s Cooled Reactor , D.P. ReDort 702. (1970).
16. P. R. Rowland, N e w Methods f o r t h e I n v e s t i g a t i o n of Radioisotope Transport i n a G a s Cooled Reactor , D.P. Report 639, (1969).
17. P. S. Gray, J. D. Hamilton, R. L e w i s and F:. Sage, Improved Primary C i r c u i t Maintenance Techniques - The Removal of E Primary H e a t Exchanger, D.P. Report 635, (1969).
1 1 2 1 3 1 I I I 1 2 1 3 1 1 1 1 2 I 3 1414~ 1 5 1 6 .I 7 1 COR i! CORES CORES
1. Dragon Operating History.
25
800.
700-
MASS SPECTROMETER READINGS DURING CHARGE COR'ES .5 -7
CORE 5 -1 600-
500-
1 400- IC 5 3
300-
6004
500-
1 400- IC 5 3
300-
160 -
140 -
120.
100-
$ - I
TOTAL USAGE
// UNACCOUNTABLE /
'00°1
k C O R E 6 -L(
a 2. Inner Containment Helium Concentrations.
HELIUM USAGE
SEPT OCT MAY JUN JUL AUG
3. Helium Usage.
2000
1800
I bOC
1400
I 2 0 C
IOOC
8 oc
6 0 C - 400-
26
COMPRESSOR DIAPHRAGM LIFE
- - I 1 I I
I I I I r I 1
- 1
- HIGH PRESSURE
LOW PRESSURE ---
I I I I 200-
I N I I T
T I I I I I I I I I I I I I I I I I
I 1 I 1
I I 1 I I I I I
I T
I 1 I #
1 I
t GI
/DIAPHRAGMS STILL IN USE
DATE OF REPLACEMENT OF DIAPHRAGMS
4. Compressor Diaphragm L i f e .
,HOT D U C T
/ . - O U , T C R D U C ?
T U E R M O C O U C L E I A L L V A L V E O-RING SEAL TRANSFLR TUDE O-RING S E A L
LXTlNSlOl l ROD
4 C O N T R O L V A L V E
5. Schematic Diagram of Dracule.
6. 1-131 P r o f i l e i n Dracule.
7. Sectioning a Primary Heat Exchanger.
28
co
8. Resu l t s of a Water I n j e c t i o n Experiment.
29
KATH AROM ETER
- \ -
FLOW SAMPLgARRIER CONTROLLER - - -
Cog CONCENTRATION[ CONCEIJTRATION
STAINLESS STEEL u TRAP TRAP I
- SILICA GEL
MOL E CULA R SIEVE
LIQUID N I T R O G E N
9. Flow Sheet of D i f f e r e n t i a l Concentrat ion Gas Chromatograph.
10. Process Model Chromatograph.
11. Circulator on Removal Trolley. 12 . Primary Heat Exchanger (Boiler) a f t e r Removal.
c
I
DRAGON STARTUP IMPURITIES (CHARGE a CORE8)
too vpm
IO vpm
I vpm
- - HYDROGEN LEVEL IN EQUILIBRIUM WITH WATER
(AT FULL POWER)
0.1 vpm
- - - - - - -
W c.
13. Impurity Levels dur ing Restart of the Reactor.
32
DISCUSSION
J. Kemper: What f u t u r e p lans have been made f o r Dragon?
B. G. Chapman: A s you can see, w e have l o s t considerable t ime as a
r e s u l t of b o i l e r tube failures, b u t w e b e l i e v e t h i s problem i s now behind
us. What w e want now i s two or t h r e e years of s t eady opera t ion t o con-
c e n t r a t e on t e s t i n g power r e a c t o r f u e l p ins , on f u r t h e r chemical corro-
s i o n work, and f i s s i o n product t r a n s p o r t and depos i t i on s t u d i e s .
Bender: H e l i u m leakage dur ing e a r l y per iod of ope ra t ion -was i t a problem?
B. G. Chapman: We had no s e r i o u s problem. A l l c i r c u i t components
were s t r i n g e n t l y t e s t e d a t t h e Con t rac to r ' s works by ou r own s p e c i a l i s t
teams. The r e s i d u a l problems of t e s t i n g s i t e work are not d i f f i c u l t i f
one v i t a l p recau t ion i s observed. The helium background i n the p l a n t
a r e a must be kep t very low s o t h a t l e a k l o c a t i o n i s f a c i l i t a t e d . Be-
cause concre te has a long "memory" f o r helium, a l l gas ( e i t h e r helium o r
lO$ helium i n n i t r o g e n ) used f o r p re s su re and l e a k t e s t i n g , must be
vented a f t e r t e s t ou t s ide the p l a n t bu i ld ings .
used l o c a l e x t r a c t systems should be provided.
I f " h e l i a r c " welding i s
It i s i n t e r e s t i n g t o note t h a t dur ing a r e c e n t shutdown a t Dragon
a small q u a n t i t y of helium was r e l eased (from welding) and our conta in-
ment b u i l d i n g l e v e l s are s t i l l w e l l above normal and w i l l t ake s e v e r a l
months t o c l e a r .
A . P. Fraas : To what degree would your maintenance a c t i v i t i e s have
been handicapped i f the l e v e l of r a d i o a c t i v i t y i n t h e gas c i r c u i t had
been increased by a f a c t o r of loo?
B. G. Chapman: A c t i v i t i e s would have been hampered bu t not rendered
impossible . The a i r b o r n e a c t i v i t y would have requi red airhood p r o t e c t i o n
around open holes , b u t t h e containment bu i ld ing l e v e l s would not have
been unacceptable. More urgency would have e x i s t e d f o r f i t t i n g temporary
seals on openings. Radioact ive Contamination was fo-Trd t o be very f i rmly
adherent and c o n t r o l would be not s e r i o u s l y more d i f f i c u l t . Di rec t r a d i a -
t i o n would r e q u i r e some s m a l l amount of temporary s h i e l d i n g or f a i r l y
t i g h t working t ime l i m i t a t i o n .
33
R. Huddle: I would l i k e t o comment on W. Chapman's remark regard ing
f a i l e d f u e l .
which i s designed t o f a i l - t o o b t a i n f a i l u r e da t a . The f a i l e d f u e l
which Chapman r e f e r r e d t o was when t h e purge on one o f t h e s e elements
ceased t o be e f f e c t i v e . The important po in t i s t h a t it shows t h a t w e do
not n e c e s s a r i l y need p e r f e c t f u e l f o r H T R ' s .
We have a very l a r g e amount of experimental f u e l i n Dragon
~
Paper 2/103
QPERATIKG' -EXPERIENCE-WZ"E, VR - EXPERIMENTAL POWER STATION
H. J. Hantke, Brown Boveri/Krupp Reaktorbau GmbH G.,,Ivens , Arbeitsgemeins c h a f t Versuchsreaktor GmbH E. A. Nephew, Oak Ridge Nat iona l Laboratory
ABSTRACT
This r e p o r t desc r ibes t h e ope ra t ing performance of t h e AVR experimental power s t a t i o n dur ing i t s commissioning pro- gram as w e l l as power ope ra t ions fo l lowing customer accep- t ance of t he p l a n t i n May 1969. The p l a n t outages, which have occurred s i n c e t h e power commissioning program began on December,18, 1967, a r e enumerated and eva lua ted accord- i n g t o t h e i r na tu re and dura t ion . The o v e r a l l p l a n t a v a i l - a b i l i t y , t o March 31, 1970, has been g r a t i o i n g l y h igh and amply demonstrates the feasibility of the pebble bed reac- t o r concept.
INTRO DUCT1 ON
The AVR experimental s t a t i o n employs a h igh temperature , helium-
cooled r e a c t o r and i s t h e f i r s t power p l a n t t o use s p h e r i c a l f u e l e le-
ments, The core c o n s i s t s of a randomly packed pebble bed conta in ing
approximately 100,000 spheres , each having a diameter of 6 cm. The con-
t r a c t f o r t he cons t ruc t ion of t h i s demonstrat ion power p l a n t was s igned
on August 13, 1959 by t h e Arbei tsgemeinschaft Versuchs-Reaktor GmbH (Am) and t h e Brown Boveri/Krupp Reaktorbau GmbH (BBK).
o f t h e p l a n t began n e a r l y two years l a t e r , having been delayed by d i f f e r -
ences of opinion concerning t h e t e c h n i c a l des ign of t h e r e a c t o r founda-
t i o n and by t h e l a c k of r e g u l a t o r y l a w s i n t h e Federa l Republic of
Germany governing t h e cons t ruc t ion and ope ra t ion of nuc lea r power s ta - t i o n s . The AVR s t a t i o n i s shown i n F ig . 1.
Actual cons t ruc t ion
F i r s t c r i t i c a l i t y was achieved on August 26, 1966 and t h e f i r s t
product ion of e l e c t r i c i t y began on December 18, 1967 fol lowing a compre-
hensive program o f zero power experiments. The t o t a l e l e c t r i c a l energy
63 generated by March 31, 1970 i s 138.1 X l o6 kWh. The f u e l elements have
34
35
a t t a i n e d a n average burnup of 43.3% f i f a , corresponding t o 7.0% fima.
The p l a n t a v a i l a b i l i t y f a c t o r , t aken as t h e r a t i o of gene ra to r ope ra t ion
t i m e t o t o t a l ca lendar t ime, has been q u i t e good. The o v e r a l l p l a n t
a v a i l a b i l i t y f a c t o r f o r t h e 27 month per iod of p l a n t ope ra t ion i s 64.6%.
The p l a n t a v a i l a b i l i t y achieved f o r s e l e c t e d per iods of ope ra t ion are:
51.4% during t h e y e a r 1968,
92.0% during t h e win te r months from October 1968 t o March 1969,
71.6% dur ing t h e yea r 1969, and
95.45 during t h e win te r months from October 1969 t o March 19'70.
Because of t h e good ope ra t ing experience obtained, t h e power s t a t i o n
was turned over t o t h e AVR organ iza t ion by BBK i n May 1969. P r i o r t o t h e
acceptance of t h e p l a n t by t h e customer, a f i n a l thorough i n s p e c t i o n of
t h e va r ious p l a n t components w a s made by t h e cons t ruc to r f i rm. The i n -
s p e c t i o n and maintenance program, conducted from March 1, 1969 t o A p r i l 15,
1969, revea led t h a t t h e degree of r a d i o a c t i v e contamination of primary
c i r c u i t components was smal le r t han had been expected, f o r example, d i s -
assembly of t h e f u e l handl ing f a c i l i t y was poss ib l e without s p e c i a l
s h i e l d i n g precaut ions . The a c t i v i t y l e v e l of t he primary coolan t gas
has been c o n s i s t e n t l y low, about 300 c u r i e s , throughout r e a c t o r opera-
t i o n s t o da t e . This i n d i c a t e s good f u e l element performance wi th no
d e t e r i o r a t i o n of t h e i r f i s s i o n product r e t e n t i o n c a p a b i l i t y occurr ing
due t o fas t neutron exposure and burnup.
The operational experience acquired w i t h the AVR Experimental Sta-
t i o n over t h e p a s t two years v e r i f i e s t h e v a l i d i t y of i t s b a s i c des ign
and e s t a b l i s h e s t h e pebble bed concept as a v i a b l e a l t e r n a t i v e wi th in
t h e HTR r e a c t o r l i n e . There has been no evidence of f u e l spheres be ing
unduly damaged by t h e severe environmental condi t ions of t h e core or by
t h e mechanical l oads imposed upon them dur ing normal f u e l handl ing opera-
t i o n s . The b a s i c f e a s i b i l i t y of t h e pebble bed r e a c t o r concept has been
amply demonstrated and t h e o v e r a l l performance of t h e power s t a t i o n has
been such as t o j u s t i f y t h e cons t ruc t ion of a l a r g e r , p ro to type pebble
bed power s t a t i o n . Present p lans c a l l for t h e cons t ruc t ion of a 300 Mwe
high temperature , pebble bed power s t a t i o n t o begin l a t e t h i s year .
A
'ig .
Fig. 1.
2. View
The AVR Power Station in Julich.
of Reactor Building.
Stbra- chonnel Ibr Spent Fuei Elements
37
DESCRIPTION OF THE AVR POWER STATION
A b r i e f d e s c r i p t i o n of t h e AVR power s t a t i o n i s provided here t o
c l a r i f y t h e d i scuss ion which fo l lows .
r e a d i l y a v a i l a b l e i n t h e open l i t e r a t u r e .
of t h e r e a c t o r bu i ld ing . The core i s f i l l e d wi th approximately 100,000
s p h e r i c a l f u e l , g raph i t e and boron elements. The AVR f u e l element con-
s i s t s of an unfueled g r a p h i t e s h e l l f i l l e d w i t h coated uranium-thorium
d ica rb ide p a r t i c l e s which a r e uniformly d ispersed i n an inne r g r a p h i t e
mat r ix .
of thorium. The core i s doubly contained i n two s t e e l p re s su re v e s s e l s ,
with pure helium maintained a t a s l i g h t overpressure i n t h e volume
between t h e two vessels t o prevent p o s s i b l e outward leakage of t h e
contaminated coolant gas .
More d e t a i l e d information i s
F igure 2 shows a s e c t i o n view
Each f u e l element con ta ins 1 g of 92% enr iched uranium and 5 g
The coolan t gas e n t e r s t h e core through r a d i a l s l o t s i n t h e bottom
r e f l e c t o r and streams upward through t h e core . Two helium blowers c i r -
c u l a t e t h e coolan t gas through a carbon b r i c k b r idge , l o c a t e d above t h e
su r face of t h e pebble bed, t o t h e steam genera tor . The carbon b r i c k
b r idge se rves t o s h i e l d t h e steam genera tor from f a s t neutrons. T h i s i s
important because t h e steam genera tor i s not r ep laceab le due t o t h e
i n t e g r a t e d cons t ruc t ion which has been used. The steam genera tor i s a
forced-flow Benson system wi th four p a r a l l e l s e c t i o n s , each having i t s own r e g u l a t o r y and c o n t r o l devices .
The f u e l handl ing system i s comprised of gas l o c k s , mechanical
swi tches , and t r a n s p o r t t ubes through which t h e f u e l spheres are charged
i n t o the core by means of helium p res su re . During r e a c t o r ope ra t ion , t h e
f u e l spheres are recyc led cont inuously from t h e bottom of t h e core back
i n t o t h e t o p i n order t o provide f u e l mixing and a t t a i n uniform burnup
and a f l a t power d i s t r i b u t i o n .
f o r c e of g r a v i t y and t h e pneumatic energy r equ i r ed t o e l e v a t e t h e spheres
i s provided by t h e p re s su re d i f f e r e n t i a l genera ted by t h e main helium
blowers. Thus, t h e f u e l handl ing system i s simple and rugged and posses-
s e s a minimum number of components wi th moving mechanical p a r t s .
Spheres a r e removed from t h e core by t h e
38
AVR PLANT OPERATING EXPERIENCE
Power Program
A summary of AVR power g e n w a t i o n achievements s i n c e December 1967
i s presented i n Tables L &nd 2. A s of March 31, 1970, a t o t a l o f 12,912
hours of genera tor a i l - l ine t i m e had been achieved and t h e t o t a l e l e c t r i -
cal- energy produced amounted to 138,075 Mwh. The f u e l elements have a t - t a ined a n average hurnup of 43.328 f i f a , corresponding t o 7.08 f i m a . A t
t h e p re sen t time, t h e core and f u e l handl ing c i r c u i t s con ta in 47,729 f u e l
spheres . This number i s g radua l ly inc reas ing as f r e s h f u e l elements a r e
loaded and dummy g raph i t e spheres a r e discharged. The maximum power l e v e l
reached thus fa r i s 50 Mwth, or 15.6 Mwe. This was achieved by inc reas -
i n g t h e helium blower speed from 4000 t o 4400 rpm and r a i s i n g t h e coolan t
gas p re s su re from 1 0 t o 11 a t m . The i n s u f f i c i e n t shutdown worth of t h e
rods had p rev ious ly prevented ope ra t ion a t t h e nominal des ign l e v e l ,
15 Mwe.
The power h i s t o r y of t h e AVR s t a t i o n i s depic ted i n Fig. 3 . During
t h i s 27 month per iod, some 60 i n t e r r u p t i o n s i n power gene ra t ion occurred
due t o r e a c t o r scrams and scheduled p l a n t shutdowns. I n Fig. 3 , t h e
scheduled p l a n t shutdowns are i d e n t i f i e d by t h e c a p i t a l l e t t e r s A through
Q, and t h e unscheduled shutdowns i n i t i a t e d by t h e automatic s a f e t y c i r - c u i t s are i d e n t i f i e d by numbers. I n t h e case of a n a c t u a l commercial
power s t a t i o n , t h e scheduled p l a n t shutdowns would have allowed s u f f i -
c i e n t t i m e t o b r i n g r e se rve s t a t i o n s on l i n e whereas t h e automatic scrams
would have r e s u l t e d i n a temporary r educ t ion i n t h e t o t a l power a v a i l -
a b l e t o t h e g r i d . This d i s t i n c t i o n , however, i s not app l i cab le t o a n
experimental power s t a t i o n , p a r t i c u l a r l y one such as t h e AVR undergoing
i t s commissioning t e s t s . Here, it se rves merely t o d i f f e r e n t i a t e between
outages occurr ing unexpectedly dur ing r o u t i n e r e a c t o r ope ra t ion and those
which were c l e a r l y fo re seeab le .
Scheduled P l a n t Shutdowns.--The scheduled p l a n t shutdowns shown i n
Fig. 3 are grouped according t o t h e i r causes and l o c a t i o n i n t h e p l a n t
system and l i s t e d i n Table 3 . Por t ions of t h e t o t a l outage per iods a re
somewhat a r b i t r a r i l y ass igned t o s p e c i f i c components and systems even
c
Table 1. Summary of AVR Operations During the Year 1968
C
Jan Feb Mar APT h Y June J u l y Aug Sept Oct Nov D e C
The a v a i l a b i l i t y of t h e AVR power s t a t i o n , c a l c u l a t e d as t h e r a t i o
of genera tor on-line t ime t o t o t a l ca lendar t ime, has been except iona l
f o r an experimental power s t a t i o n undergoing i t s commissioning tes t s .
can be seen i n Fig. 4, t h e p l a n t performance has improved s t e a d i l y s i n c e
power ope ra t ion began i n l a t e 1967. a b i l i t y w a s 51.4%, i n s p i t e of extended p l a n t shutdowns f o r f u e l loading
and maintenance of t h e gas p u r i f i c a t i o n and f u e l handl ing f a c i l i t i e s .
The a v a i l a b i l i t y f a c t o r f o r t h e year 1969 w a s 71.6%. months from October 1968 t o March 1969, t h e o v e r a l l p l a n t a v a i l a b i l i t y
w a s 92%, inc reas ing t o 95.4% f o r t h e same t ime per iod i n 1969-70. t a k e s i n t o account a l l power ope ra t ions t o d a t e , inc luding both t h e com-
missioning and run-in phases of operation prior to customer acceptance of
t h e p l a n t , t h e o v e r a l l a v a i l a b i l i t y amounts t o 64.6%.
As
I n 1968, t h e o v e r a l l p l a n t avail-
During t h e win ter
If one
AVR Reactor Core
Fuel Behavior.--Although t h e average f u e l burnup has reached 7% fima,
t h e f i s s i o n product r e t e n t i o n of t h e f u e l has remained l a r g e l y unchanged
and good.
of t h e coolan t gas has remained e s s e n t i a l l y cons tan t a t 300 c u r i e s .
a c t i v i t y a r i s e s mainly from uncoated uranium p resen t - i n t h e f u e l elements.
The R / B r a t i o f o r 1 3 3 X e i s one t e n t h of t h e s p e c i f i e d va lue of 5 x lo?
A p o r t i o n of t h e f i r s t charge f u e l has a l r eady experienced a burnup of 1 2 %
f i m a , cons iderably more than t h e f u e l s p e c i f i c a t i o n va lue of 9% f i m a .
Never the less , it i s planned t o r e t a i n t h e s e h igh ly burned f u e l elements i n
t h e core f o r some t i m e longer and t o d e l i b e r a t e l y recharge them t o t h e
h ighes t f l u x zone during r ecyc l ing ope ra t ions . The purpose of t h i s a c t i o n ,
which w i l l probably l e a d t o a p a r t i a l d e s t r u c t i o n of t h e f u e l p a r t i c l e
coa t ings , i s t o demonstrate t h e o p e r a b i l i t y of a pebble bed r e a c t o r even
when some of t h e f u e l elements become d e f e c t i v e .
Throughout t h e two yea r s of power ope ra t ion , t h e a c t i v i t y l e v e l
This
Primary C i r c u i t Impurities.--The concent ra t ions of gaseous impuri-
t i e s i n t h e primary c i r c u i t , a r i s i n g from t h e outgass ing of core s t r u c -
t u r a l material dur ing power ope ra t ion , have dec l ined s t e a d i l y due t o t h e
c l eans ing a c t i o n of t h e gas p u r i f i c a t i o n p l a n t .
t h e s e chemical contaminants a r e : CO - 30 vpm, H2 - 9 vpm, CH4 - 2 vpm,
The present l e v e l s of
45
C 0 2 - 5 vpm, and H 2 0 - 0.1 vpm. The presence of t hese i m p u r i t i e s i n t h e
primary c i r c u i t has not r e s u l t e d i n any apprec iab le co r ros ive damage t o
t h e f u e l elements.
Refuel ing Program. --Fuel loading and r ecyc l ing i s c a r r i e d out dur ing
power ope ra t ion a t a ra te s e t mainly by core r e a c t i v i t y cons idera t ions .
The German l i c e n s i n g a u t h o r i t i e s r e q u i r e t h a t t h e core must no t be loaded
t o a r e a c t i v i t y which exceeds t h e worth of t h e f o u r shutdown rods l e s s
1/2 Ni le , as measured wi th r e s p e c t t o t h e r e fe rence shutdown temperature
of 105°C. The complete AVR f u e l element c i r c u i t p r e s e n t l y conta ins
107,381 f u e l , boron, and g r a p h i t e spheres . O f t hese , 13,200 spheres a r e
l o c a t e d i n t h e sphere d ischarge tube a t the base of t h e core . Table 5
l i s t s t h e p re sen t composition of t h e r e a c t o r core and a s s o c i a t e d f u e l
c i r c u i t s . O f t h e 47,729 f u e l spheres i n the AVR c i r c u i t , some 30,000 are t h e f irst charge U. S. -manufactured, machined f u e l spheres , 4390 are t h e
"wallpaper" type, and t h e res t a r e spheres manufactured by new molding
techniques developed by t h e German f i rm N u k e m .
Table 5. AVR Core Composition, March 31, 1970
Complete Fuel Discharge C i r c u i t Tub e Sphere Type Core
Fuel 47729 42840 4889
Graphi te 57354 49363 7991
Boron 2298 1978 3 20
T o t a l 107381 94181 13200 .-
The f u e l loading ra te i s chosen 'on t h e b a s i s of t h e o r e t i c a l p red ic-
t i o n s obtained from two-dimensional, mult iple-zone burnup c a l c u l a t i o n s
which inco rpora t e t h e known load ing and r e c y c l i n g program as we l l as t h e
flow behavior of t h e spheres w i t h i n t h e pebble bed. Deviations from t h e I pred ic t ed behavior are manifested i n t h e form of changing gas e x i t t e m -
pe ra tu re s from t h e core. When t h i s occurs , t h e r e f u e l i n g program i s a l -
t e r e d t o r e - a t t a i n t h e des i r ed ope ra t ing condi t ions . However, a time
AVR 70.13-1
Fig. 5. Sphere Flow Characteristics in the AVR Pebble Bed Core.
AVR 70.13-2
I BBC/KRUPP
A
Fig. 6. Example f o r a Representation of AVR Core in 2-D Erebus Burnup Calculation.
47
delay of 4 t o 6 weeks e x i s t s be fo re t h e a l t e r e d r e f u e l i n g and r ecyc l ing
program t a k e s e f f e c t , There i s t h e r e f o r e a h igh i n c e n t i v e t o o b t a i n
q u a n t i t a t i v e accuracy i n t h e burnup c a l c u l a t i o n s so t h a t t h e opt imal f u e l
loading program can be s e l e c t e d .
Burnup c a l c u l a t i o n s f o r a pebble bed r e a c t o r are complicated by t h e
f a c t t h a t t h e zonal nuc l ide concent ra t ions i n the core va ry bo th wi th
f u e l burnup and f u e l movement. Figure 5 shows t h e flow p a t t e r n of spheres
as they t r a v e r s e t h e core .
sphere v e l o c i t y depends s t r o n g l y upon i t s r a d i a l p o s i t i o n i n t h e core .
The power d i s t r i b u t i o n c a l c u l a t i o n s must adequate ly account f o r t h e con-
t i nuous ly changing core conf igu ra t ion as w e l l as t h e long term f i s s i o n
product accumulation. Figure 6 shows how t h e movement of f u e l spheres
through t h e core i s s imulated i n t h e EREBUS burnup program by mul t ip l e
zone core c a l c u l a t i o n s a t d i s c r e t e t i m e s t e p s .
The sur face p r o f i l e l i n e s c l e a r l y show t h a t t h e
Core Physics Measurements
Rod Drop Experiment.--Several rod drop experiments have been per-
formed t o determine t h e r e a c t i v i t y worth of t h e f o u r rod bank. The fou r
rods are scrammed during r e a c t o r power ope ra t ion and t h e r e s u l t i n g f l u x -
t ime t r a c e i s recorded. An a c o u s t i c a l record of t h e no i ses generated by
t h e rack and p in ion gears of each rod i s used t o determine t h e depth of
rod i n s e r t i o n as a func t ion of t ime. The f lux- t ime t r a c e i s analysed by an inve r se k i n e t i c s program developed by M r . K. J. K a l k e r o f the KFA
Nuclear Research Center a t J ' a i c h . Although t h e t h e o r e t i c a l b a s i s of t h e
experiment i s not f u l l y understood, t h e experimental results ag ree w e l l
wi th estimates o f t h e t o t a l rod worth obta ined by o t h e r methods. The
rod drop experiment has been adopted as a s tandard means f o r p e r i o d i c a l l y
i n v e s t i g a t i n g changes i n rod worth due t o f u e l burnup and a l t e r e d core
conf igura t ion .
Simulated Rod Fai lure . - -The marginal shutdown worth of t h e AVR rod
bank makes it important t o know t h e consequences of a poss ib l e s i n g l e
rod fa i lure . For t h i s reason, experiments have been performed t o measure
t h e nuc lear behavior of t h e ho t core when he ld s u b c r i t i c a l by only t h r e e
of t h e f o u r rods. I n t h e s e experiments, t h e r e a c t o r core was allowed t o
48
cool by n a t u r a l convect ion f o r a per iod s u f f i c i e n t l y long t o e s t a b l i s h
t h e cool ing down ra te . The blowers were then used t o f o r c e f u l l y cool
t h e core u n t i l it aga in reached c r i t i c a l i t y by v i r t u e of t h e negat ive
temperature c o e f f i c i e n t of r e a c t i v i t y . This was done t o expedi te t h e
cool ing process which would otherwise r e q u i r e s e v e r a l weeks. It was
found t h a t t h e r e a c t o r power l e v e l s ou t t o about 30 kw, a f t e r undergoing
o s c i l l a t i o n s t o 50 kw, fo l lowing i t s r e t u r n t o c r i t i c a l . The experiment
demonstrates t h a t a t l ea s t s e v e r a l weeks would be a v a i l a b l e t o provide
a d d i t i o n a l shutdown r e a c t i v i t y i f one rod f a i l s t o opera te during a
scram a t f u l l r e a c t o r power.
Temperature Coef f i c i en t . --The temperature c o e f f i c i e n t of r e a c t i v i t y
has been determined by means o f per iod measurements of a given core con-
f i g u r a t i o n made a t two d i f f e r e n t temperatures . A t t h e r e fe rence shutdown
temperature of 105"C, t h e temperature c o e f f i c i e n t of r e a c t i v i t y was found
t o be -18.9 mN/"C.
10% due t o e r r o r s i n measuring t h e temperature , i s t h e average of t h r e e
s e p a r a t e measurements and ag rees f a i r l y w e l l wi th ca l cu la t ed r e s u l t s .
The experimental procedure employed was t o e s t a b l i s h a s l i g h t l y super-
c r i t i c a l rod p o s i t i o n a t a core temperature of 103°C and t o then measure
t h e r e a c t o r per iods of t h i s core conf igu ra t ion f o r core temperatures of
103"C, llO"C, and 114°C. The core temperature was va r i ed by a d j u s t i n g
t h e temperature of t h e feedwater t o t h e steam genera tor .
This . va lue , conta in ing a n es t imated unce r t a in ty of
T r i t i u m Measurements i n t h e AVR Reactor.--The AVR coolant gas con-
t a i n s ve ry l i t t l e tritium dur ing normal power opera t ion , on t h e o r d e r of
about 0 .5 c u r i e s .
r e a c t i o n wi th Li-6, which i s p resen t as a n impur i ty i n the g raph i t e and
carbon b r i c k s t r u c t u r a l r a t e r i a l , and d i r e c t l y as a f i s s i o n product.
T r i t i u m has a l s o been de tec t ed i n t h e AVR secondary c i r c u i t i n concen-
t r a t i o n s of about 2 . 5 microcur ies p e r l i t e r o f feedwater, corresponding
t o a n o v e r a l l a c t i v i t y of about 0.14 c u r i e s i n t h e steam c i r c u i t , The
o r i g i n of t h e tritium found i n t h e secondary c i r c u i t i s not y e t c l e a r .
It i s suspected t h a t a t l eas t a p o r t i o n of t h e secondary c i r c u i t tritium
i s produced by neutron a c t i v a t i o n of nitrogen-14, a n i so tope present i n
The primary sources of tritium i n t h e AVR a r e t h e ( n , a )
t h e feedwater from t h e ammonia and hydrazine used t o prepare and process
t h e feedwater.
49
The main po r t ion of the t r i t i i m found i n the secondary c i r c u i t ,
however, must a r i s e e i t h e r from ano the r more product ive ac t iva tLon proc-
ess or frorn f i i f fus ion of t h e primary c i r c u i t tritium through t h e s t ee l
tu-bing o f t h e steam genei-ator. Seve ra l e x p r i m e n t s have been performed
t o a s c e r t a i n which of t h e s e r ep resen t s t h e primary mechanism. These ex-
pe r inen t s a r e based on t h e de te rmina t ion of t h e ra te of tritium bui ldup
i n t h e steam c i r c u i t . I f t h e tritium i n t h e feedwater a r i s e s from neu-
t r o n a c t i v a t i o n of some impuri ty , t h e time requi red f o r i t s bui ldup t o
equ i l ib r ium concent ra t ion should be r e l a t i v e l y long. If, on t h e o t h e r
hand, t h e tritium d i f f u s e s from t h e primary c i r c u i t i n t o the secondary
c i r c u i t , i t s concent ra t ion i n t h e steam c i r c u i t should b u i l d up i n a manner similar t o t h a t i n t h e helium c i r c u i t .
During a r e a c t o r shutdown per iod , i n which one would expect n e i t h e r
a c t i v a t i o n or d i f f u s i o n t o occur , t h e e n t i r e feedwater was rep laced wi th
f r e s h water conta in ing no tritium. Following t h e r e a c t o r s t a r t u p , t h e
tritium concent ra t ions i n t h e helium and steam c i r c u i t s were c a r e f u l l y
monitored. It was found t h a t tritium b u i l t up i n bo th c i r c u i t s propor-
t i o n a l l y , i n d i c a t i n g t h a t a d i f f u s i o n process wi th a de lay t i m e of only
a few minutes w a s t ak ing p lace . However, i n another experiment, some
5 c u r i e s of tritium toge the r wi th s e v e r a l hundred l i t e r s of hydrogen were
i n j e c t e d i n t o t h e primary c i r c u i t . The tritium and hydrogen concentra-
t i o n s i n t h e steam c i r c u i t were then monitored. As tonish ingly , no i n -
c rease i n t h e i r l e v e l s could be de t ec t ed .
The reason f o r t h e nega t ive result of t h e tritium i n j e c t i o n expe r i -
ment i s not c l e a r l y understood a t t h e p re sen t t i m e . I t i s t h e r e f o r e
planned t o r epea t t h i s experiment, under more c a r e f u l l y c o n t r o l l e d condi-
t i o n s and using more s e n s i t i v e measuring procedures, sometime i n t h e near
f u t u r e . It i s p r e s e n t l y be l i eved t h a t on ly d i r e c t d i f f u s i o n of tritium
through t h e steam gene ra to r t ub ing can account f o r t h e concent ra t ion ob-
served i n t h e secondary c i r c u i t . The y i e l d s of o t h e r poss ib l e r e a c t i o n s
a r e considered t o be too s m a l l t o s u f f i c i e n t l y e x p l a i n t h e e f f e c t .
50
Amnionia Injection Experiment.--In laboratory tests, ammonia when
admixed to the helium coolant gas has been shown to act as a gaseous
lubricant, reducing the coefficient of friction between graphite spheres
in a pebble bed reactor. In anticipation of possible future requirements
in large pebble bed reactors, ammonia was injected into the AVR primary
circuit in an experiment conducted on January 23, 1969. The purpose of
the experiment was to determine the stability or decomposition rate of
NH3 in a realistic reactor environment of radiation and temperature. decomposition rate of the ammonia in the primary circuit was determined
by observing the growth of the decomposition products, hydrogen and nitro-
gen. The concentrations of these impurities were measured by gas chroma-
tography at regular intervals following the injection of the ammonia.
The decomposition half-life for ammonia was measured to be from 8 to 12 minutes in the AVR core environment.
The
Dynamics Experiments.--Reactor operating parameters such as the
feedwater flow rate, the coolant gas blower speed, and the position of
the shutdown rods have been varied stepwise to determine the dynamic
response characteristics of the plant. Further tests have been conducted
to determine the consequences of the loss of sensitive components such
as the main feedwater pump and the helium circulators. In the case of
loss of connection to the electrical grid, it was demonstrated that the
generator can supply the plants own needs without difficulty. In all the
simulated incidents, the automatic safety circuits operated according to
plan and functioned reliably to prevent any unsafe reactor condition from
arising .
SUMMARY AND CONCLUSIONS
The successful operation of the AVR experimental power station over
the past 27 months verifies the validity of its basic design and estab-
lishes the pebble bed concept as a viable alternative within the HTGR
reactor line.
tion, which includes the power commissioning program, has been excep-
tionally good for an experimental power station.
and significant is the fact that the plant availability record has
The availability of the plant during this period of opera-
Even more gratifying
improved s t e a d i l y as f a m i l i a r i t y and experience wi th complicated p l a n t
systems, such as t h e gas p u r i f i c a t i o n p l a n t and t h e f u e l handl ing f a c i l -
i t y , were acqui red .
down phase of power opera t ions have e l imina ted many weak s p o t s and g r e a t l y
improved t h e o v e r a l l r e l i a b i l i t y of t h e power s t a t i o n .
Improvements and r e v i s i o n s made dur ing t h e shake-
I n our opinion, t h e promising p o t e n t i a l i t y of pebble bed r e a c t o r s
and t h e good performance of t h e AVR power s t a t i o n j u s t i f i e s t he planned
cons t ruc t ion of a 300 h e pro to type power s t a t i o n based on the pebble
bed concept. The prospec ts f o r f u l l y automating t h e f u e l element pro-
duc t ion process , using sphere molding techniques developed by N u k e m could
g r e a t l y reduce f u e l element manufacturing cos t s , a key i t e m i n a s s e s s i n g
t h e economic p o t e n t i a l of pebble bed r e a c t o r s . It should be kep t i n mind
t h a t a l though good performance has been obtained i n a c c e l e r a t e d capsule
t e s t s , adequate f u e l element behavior a t t h e requi red burnup and f a s t
neut ron exposure must be demonstrated i n r e a c t o r experiments. The ex-
c e l l e n t s a f e t y c h a r a c t e r i s t i c s , good f u e l cycle economy and h igh e f f i -
c iency of pebble bed power s t a t i o n s combine t o make t h e prospec ts q u i t e
promising t h a t t h i s type of power s t a t i o n w i l l emerge as a s e r i o u s com-
p e t i t o r i n t h e f u t u r e energy market.
52
APPENDIX
This appendix provides a d e t a i l e d d e s c r i p t i o n of t h e scheduled p l a n t
shutdowns depic ted i n Fig. 3 , i nc lud ing t h e da t e , na tu re and dura t ion of
t he va r ious outage per iods .
Scheduled P l a n t Shutdowns
A. December 19 t o 22, 1967 - A p re sc r ibed i n s p e c t i o n of t h e t u r b i n e
bear ings was performed as p a r t of t h e commissioning program. P l a n t
down t i m e , 72 hours.
B. January 15 t o February 15, 1968 - This shutdown period served as p a r t
o f t h e commissioning program f o r the f u e l handl ing f a c i l i t y . During
t h e shutdown period, some 2450 a d d i t i o n a l f u e l elements and 6370
g raph i t e elements were loaded i n t o t h e core thereby inc reas ing t h e
core r e a c t i v i t y from 8 .68 t o 10.61 Ni l e s . A s i s t h e case f o r a l l
prolonged p l a n t shutdowns, t h e outage per iod w a s a l s o u t i l i z e d t o
c a r r y o u t r e p a i r s , r ev i s ions , and improvements on va r ious components.
P l an t down time, 740 hours.
A p r i l 16 t o June 19, 1968 - The p l a n t was shut down f o r a comprehen-
s i v e i n s p e c t i o n and maintenance of p l a n t components and t o concur-
r e n t l y c a r r y out a major r e c y c l i n g of t h e in-core f u e l elements under
cold r e a c t o r condi t ions . During t h e r e a c t o r shutdown, acceptance
t e s t s were performed on secondary c i r c u i t components and experiments
t o s imula te t h e loss of e l e c t r i c a l l oad and l o s s of t h e main feed-
water pump were conducted. The dynamic response of t h e p l a n t t o
t h e s e s imulated i n c i d e n t s w a s determined and the automatic s a f e t y
system was found t o perform according t o design.
C.
The sphere r ecyc l ing program was delayed by d i f f i c u l t i e s which
a r o s e wi th t h e f u e l handl ing f a c i l i t y . Mechanical components such as
t h e s e v e r a l i z e r , s i n g u l i z e r , and sphere locks l o c a t e d i n t h e f u e l
t r a n s p o r t tubes jammed f r equen t ly because of t h e higher c o e f f i c i e n t
of f r i c t i o n i n a d r y helium atmosphere.
reso lved and by June 12, 1968 some 6120 spheres had been recyc led ,
r e s u l t i n g i n a r e a c t i v i t y loss of 560 mN as t h e c e n t r a l boron zone
was pu l l ed deeper i n t o t h e core . Malfunctioning of t h e f u e l handl ing
The problems were g radua l ly
53
f a c i l i t y became less f r equen t as f a m i l i a r i t y and experience wi th
t h e system were acquired.
By June 14, 1968, thermal power ope ra t ion could be resumed and
f i v e days l a t e r t h e coolant gas impur i t i e s dropped t o a l e v e l per-
m i t t i n g h igher gas o u t l e t temperatures from the core. On June 19,
1968, steam condi t ions a l lowing t u r b i n e ope ra t ion were a t t a i n e d and
e l e c t r i c a l power product ion resumed. P lan t down time, 1537 hours.
J u l y 15 t o J u l y 27, 1968 - The r e a c t o r was shu t down i n o rde r t o i n -
s p e c t t h e low temperature s t ages of t h e W-4 gas p u r i f i c a t i o n p l a n t .
Four days e a r l i e r l a r g e helium l o s s e s had been noted a f t e r t hese
u n i t s had been charged wi th helium a t ope ra t ing pressure . The i n -
s p e c t i o n revea led t h a t t h e helium tub ing i n t h e low temperature u n i t s
had ruptured because it had been mounted too r i g i d l y t o accommodate
t h e f o r c e s of con t r ac t ion . The low temperature s e c t i o n s of t h e gas
p u r i f i c a t i o n p l a n t were dismantled and removed f o r r e p a i r ou t s ide t h e
r e a c t o r b u i l d i n g and t h e p l a n t resumed ope ra t ion a t 8 Mwe. The
forced shutdown period was u t i l i z e d t o i n s t a l l a d d i t i o n a l thermo-
couples on t h e o u t e r p re s su re v e s s e l l i d and t o perform acceptance
t e s t s on t h e f u e l burnup and i d e n t i f i c a t i o n device. Other small re-
p a i r s and improvements, such as t h e i n s t a l l a t i o n of microphones
a long t h e t r a n s p o r t tubes of t h e f u e l handl ing f a c i l i t y t o provide
a c o u s t i c monitoring, were e f f e c t e d . P l an t down t i m e , 302 hours. E. August 9 t o October 6, 1968 - This p l a n t shutdown, of n e a r l y two
D.
months d w a t i o n , was i n i t i a t e d by a diaphragm rup tu re i n t h e helium
compressor of t he gas p u r i f i c a t i o n p l a n t . The d e c i s i o n w a s t aken
t o extend t h e outage per iod f o r two weeks t o i n s t a l l t h e RA-4 gas
p u r i f i c a t i o n u n i t s which had been r epa i r ed i n t h e meantime. I n
p a r a l l e l wi th t h e M-4 i n s t a l l a t i o n , core dry ing ope ra t ions were
undertaken t o remove moisture from t h e primary c i r c u i t which had
been admit ted as a result of t h e diaphragm rup tu re of t h e water d r iven compressor MK-2. This was done by c i r c u l a t i n g t h e primary
gas through a B a O f i l t e r f o r f ive days and subsequent ly ope ra t ing
t h e r e a c t o r a t a low thermal power l e v e l of 1 M w .
t h e core dry ing opera t ions and t h e RA-4 i n s t a l l a t i o n work we, r e com-
p l e t ed , b u t resumption of power ope ra t ion was delayed by a new series
By August 25, 1968,
F.
G.
54
of d i f f i c u l t i e s wi th t h e f u e l handl ing f a c i l i t y . n
The r ecyc l ing of i n -co re spheres , which had cont,nued d r i n g t h e
i n i t i a l phase of t h e shutdown per iod , was h a l t e d on August 17, 1968
by weak e l e c t r o n i c s i g n a l s f r o n t h e sphere d e t e c t i o n c o i l s l oca t ed
along t h e pneumatic t r a n s p o r t tubes . These c o i l s d e t e c t t h e passage
of a sphere through t h e t r a n s p o r t tubes and provide con t ro l s i g n a l s
t o t h e Z u s e 32 computer used t o d i r e c t and record f u e l handl ing op-
e r a t i o n s . I n v e s t i g a t i o n revea led t h a t t h e weakened s i g n a l s a r o s e
from t h e a l t e r e d phys ica l p r o p e r t i e s of g raph i t e caused by neutron
i r r a d i a t i o n . The a m p l i f i c a t i o n of t h e s e s i g n a l s was improved and t h e
sphere r ecyc l ing program resumed on September 14, 1968.
FYequent mechanical d i f f i c u l t i e s wi th components of t h e f u e l
handl ing f a c i l i t y , however, s eve re ly hindered t h e r ecyc l ing ope ra t ions .
The p o r t s e l e c t o r wheel f a i l e d t o p o s i t i o n proper ly t o t h e t r a n s p o r t
tube p o r t s and on September 19, 1968, t h e Dosierrad jammed completely.
The removal and disassembly of t h e s e u n i t s i s t ime consuming because
they a re loca ted i n s i d e t h e barr ier gas envelope surrounding t h e p r i -
mary system.
wheel and a s t ronge r motor-clutch d r i v e u n i t was provided f o r t h e
Dosierrad. Thermal power ope ra t ion of t h e AVR s t a t i o n began aga in
on October 4 , 1968 and e l e c t r i c a l genera t ion resumed on October 6,
1968. P l a n t down time, 1401 hours .
October 24, 1968 - This scheduled shutdown w a s made t o in spec t poss i -
b le damage t o t h e steam t u r b i n e dur ing a t o o r ap id res tar t i n c i d e n t
which occurred s i x days e a r l i e r . The i n s p e c t i o n revea led only minor
damage t o t h e t u r b i n e and r e p a i r was de fe r r ed t o t h e next shutdown
per iod scheduled f o r March 1, 1969. P l a n t down time, 1 hour and 6
minutes.
February 28 t o A p r i l 18, 1969 - This major p l a n t shutdown f o r r e v i -
s i o n and maintenance was scheduled t o provide a f i n a l thorough i n -
spec t ion of t h e p l a n t f a c i l i t i e s p r i o r t o customer acceptance of t h e
experimental nuc lea r s t a t i o n . The i n s p e c t i o n and maintenance a c t i v i -
t i e s were c a r e f u l l y organized i n advance t o minimize t h e l eng th of
t h e outage per iod . The shutdown period was ushered i n a day prema-
t u r e l y by a d e f e c t i v e s i g n a l a m p l i f i e r i n the s a f e t y c i r c u i t s which
New end-switches were i n s t a l l e d on t h e p o r t s e l e c t o r
55
t r i g g e r e d a r e a c t o r scram. During t h e ensuing outage per iod , t h e
d e f e c t i v e a m p l i f i e r w a s r epa i r ed and a h o s t of o the r maintenance and
r e v i s i o n a c t i v i t i e s were c a r r i e d out on the steam t u r b i n e , t h e f u e l
handl ing system and numerous components of t h e primary and secondary
c i r c u i t s .
Thermal power ope ra t ion of t h e p l a n t resumed on A p r i l 18, 1969
a f t e r t h e major r e v i s i o n and i n s p e c t i o n program was completed on
schedule .
while t h e gas p u r i f i c a t i o n system cleansed t h e primary c i r c u i t o f gas-
eous impur i t i e s admit ted during t h e r e p a i r and i n s p e c t i o n a c t i v i t i e s .
A f t e r t h r e e days, t h e impur i ty concent ra t ions dec l ined t o a l e v e l
where h igher coolant gas temperatures could be accepted. The r e a c t o r
power l e v e l w a s t hen r a i s e d t o 20 Mwth g iv ing a h o t gas temperature
o f 600°C and pe rmi t t i ng t h e t r a n s i t i o n t o steam product ion and turbo-
a l t e r n a t o r opera t ion . P l a n t down t i m e , 1245 hours.
I n i t i a l l y , t h e thermal power l e v e l w a s r e s t r i c t e d t o 10 Mw
H. A p r i l 21, 1969 - Following t h e r e p a i r of t h e steam t u r b i n e , t h e ro-
t a t i o n of t h e t u r b i n e s h a f t was c a r e f u l l y checked and found t o be
f ree of imbalances. On A p r i l 21, 1969, t h e t u r b i n e was shu t down
f o r a s h o r t t i m e so t h a t t h e in s t rumen ta t ion f o r checking i t s b a l -
ance could be removed. Following t h i s , t h e r e a c t o r power l e v e l was
g radua l ly r a i s e d t o 39 Mwth and ope ra t ion o f t h e e l e c t r i c a l genera-
t o r resumed l a t e t h e same day. P l a n t down time, 10 hours .
May 10 t o May 13, 1969 - The r e a c t o r was shu t down t o r e p a i r t he main
coolant water pump which had been damaged by i n s u f f i c i e n t bea r ing
l u b r i c a t i o n . P l a n t down t i m e , 72 hours .
May 1 5 t o May 16, 1969 - This shutdown w a s made t o r ep lace a defec-
t i v e steam pressure r e g u l a t o r f o r t h e t u r b i n e . P l an t down t i m e ,
26 hours and 31 minutes.
I.
J.
K. June 9 t o June 13, 1969 - This shutdown was r equ i r ed t o r e p a i r t h e
p o r t s e l e c t o r wheel o f t h e f u e l handl ing f a c i l i t y .
79 hours.
June 18, 1969 - Power ope ra t ion was i n t e r r u p t e d t o conduct a rod drop
experiment t o measure t h e r e a c t i v i t y worth of t h e four shutdown rods.
P l a n t down time, 1 5 hours and 8 minutes.
P l a n t down time,
L.
56
M. J u l y 30 t o August 6, 1969 - This p l a n t shutdown was made t o c a r r y
out dynamics experiments and t o provide t i m e f o r needed maintenance
work. The dynamics experiments cons is ted of a rod drop experiment
t o measure t h e worth of t h e f o u r shutdown rods. Following t h i s , one
of t h e rods w a s f u l l y withdrawn from t h e core t o s imula te a "jammed
rod" i n c i d e n t and t o a s c e r t a i n how long t h e r e a c t o r would remain sub-
c r i t i c a l i f on ly t h r e e rods were a v i l a b l e f o r i n s e r t i o n during f u l l
power opera t ion . This information, t oge the r wi th knowledge of t h e
power l e v e l t o which t h e r e a c t o r w i l l s t a b i l i z e a f t e r r e t u r n t o c r i t i -
ca l , i s important i n a s s e s s i n g t h e se r iousness of an a c t u a l acc iden t
of t h i s type. It was concluded t h a t a t l eas t s e v e r a l weeks would be
a v a i l a b l e t o provide supplementary shutdown r e a c t i v i t y i n t h e event
of a n a c t u a l s i n g l e rod fa i lure . P l a n t down t i m e , 177 hours.
N. August 9 t o September 3, 1969 - A gas flow blockage developed i n t h e
low temperature s e c t i o n s of t h e RA-4a and RA-4b p u r i f i c a t i o n s t ages
on August ET, 1969 due t o f rozen moisture . The u n i t s were taken out
of ope ra t ion when t h e p re s su re drop ac ross them reached t h r e e atmos-
pheres and r e a c t o r power ope ra t ion continued f o r a s h o r t time wi th-
ou t t h e s e s t ages of t h e p u r i f i c a t i o n f a c i l i t y . The r i s i n g concen-
t r a t i o n of water vapor i n t h e primary c i r c u i t , however, made it nec-
e s s a r y t o s h u t down t h e r e a c t o r on August 9, 1969. The source of
t he water i s be l ieved t o have been from t h e b a r r i e r gas system which
enc loses t h e primary r e a c t o r p re s su re v e s s e l . Shor t ly be fo re t h e
flow blockage developed, a po r t ion of t h i s gas had been routed t o
t h e RA-4 u n i t f o r p u r i f i c a t i o n .
The gas i n t a k e l i n e s t o t h e RA-4 u n i t were d r i e d by a u x i l l i a r y
hea t ing and on August 19, 1969 t h e r e a c t o r was brought t o a power
l e v e l of Mwth t o f a c i l i t a t e dry ing of t h e primary c i r c u i t . On
August 26, 1969, dur ing t h e removal of t h e auxi l l ia ry hea t ing equip-
ment, t r a c e s of hydrau l i c o i l were found on some gas va lves . The
r e a c t o r was s h u t down and t h e source of t h e o i l w a s found t o be rup-
tu red diaphragms i n compressors MK-6a/b.
carbon t e t r a c h l o r i d e and a n i t rogen drying s t ream began a t once, This
work was completed on September 3, 1969 and e l e c t r i c a l power genera-
t i o n resumed a t t h a t t i m e . P l a n t down t i m e , 611 hours.
Cleansing opera t ions wi th
57
0 . January 19, 1970 - A rod drop experiment was performed t o measure t h e
r e a c t i v i t y worth of t h e fou r shutdown rods. P l a n t down t i m e , 2 hours
and 23 minutes.
P. January 20 t o January 25 , 1970 - The p l a n t was shu t down f o r r o u t i n e
maintenance work, no tab ly t h e replacement of e l e c t r i c a l c o i l s on t h e
magnetic valves of gas c i r c u i t s i n s i d e t h e containment v e s s e l . I n
add i t ion , t h e s u b c r i t i c a l i t y of t h e r e a c t o r , wi th a l l f o u r shutdown
rods i n s e r t e d and t h e core a t a temperature of 105OC, was measured.
The s c r a p s e p a r a t o r u n i t of t h e f u e l handl ing f a c i l i t y w a s inspec ted
and found t o be not func t ion ing properly. It was then disassembled
and 350 undamaged spheres were found t o have accumulated i n t h e hopper
arrangement loca t ed beneath t h e r o t a t i n g drum of t h e u n i t .
The spheres were removed from t h e hopper b p means of a provisory
s u c t i o n device , The malfunct ion w a s found t o have a r i s e n from t h e
increased c o e f f i c i e n t of f r i c t i o n between t h e g r a p h i t e spheres and
s t e e l caused by t h e d r y helium atmosphere and excess ive a x i a l p l ay
i n t h e r o t a t i n g drum. When it became apparent t h a t ex tens ive r e -
p a i r s were requi red , i nc lud ing t h e cons t ruc t ion and i n s t a l l a t i o n of
a completely new and improved r o t a t i n g drum u n i t , t h e r e a c t o r was
brought back t o power t o avoid a prolonged shutdown per iod .
work on t h e sc rap s e p a r a t o r u n i t proceeded concurren t ly wi th r e a c t o r
power opera t ion . P l a n t down t i m e , 139 hours and 20 minutes. March 6 t o March 13, 1970 - The r e a c t o r power g radua l ly dec l ined from
14.5 Mwe i n January t o 9 Mwe i n e a r l y March because of f u e l burnup.
Since t h e f u e l handl ing f a c i l i t y w a s ou t o f commission, it was i m -
poss ib l e t o c a r r y ou t normal f u e l loading and r ecyc l ing and on March 6, 1970 t h e power s t a t i o n had t o be s h u t down.
Repair
Q.
The r e p a i r s t o t h e s c r a p s e p a r a t o r were completed and completely
s a t i s f a c t o r y ope ra t ion of t h e f u e l handl ing f a c i l i t y has s i n c e been
obtained. The outage pe r iod was prolonged by t h e n e c e s s i t y of pump-
i n g t h e r e a c t o r coolant gas inventory i n t o s t o r a g e so t h a t a d e f e c t i v e
va lve i s o l a t i n g t h e s c r a p s e p a r a t o r from t h e primary c i r c u i t could be
rep laced . P l an t down t ime, 177 hours and 48 minutes.
58
DISCUSSION
R. C . Ihh lberg : P lease comment on t h e type of opera tor e r r o r s which
cause unscheduled shutdowns.
H. Knt fer : F a i l u r e s are not only caused by opera tors t h a t use s h i f t
people, b u t about 2/3 by maintenance people and 1/3 by s h i f t people.
Example by maintenance people: a n e l e c t r i c i a n drew t h e e l e c t r o n i c card
f o r t h e main blowers i n s t e a d of a n a u x i l i a r y blower. Example by s h i f t
people: a n ope ra to r opened a wrong va lve f o r dep res su r i s ing a small room
of t h e blocking-gas-system. This caused a pressure drop f o r t h e helium
pressure c o n t r o l system and dropped a rod. Some poss ib l e ways t o mini-
mize human f a i l u r e s ( t o a b o l i s h them i s imposs ib le ) : 1) Minimizing
maintenance work t h a t could in f luence opera t ion , 2 ) i n s t a l l a t i o n o f more
warning s i g n a l s , and 3 ) i n t r o d u c t i o n of more check lists.
John Kemper: W y t h e sea rch f o r t r i t i u m ? I thought t h a t HTGR's were
e s p e c i a l l y f o r t u n a t e i n t h i s r e s p e c t .
G. Ivens : Y e s , you are q u i t e c o r r e c t i n say ing t h a t tritium produc-
t i o n i s e s p e c i a l l y low i n HTGR's . The tritium presen t i n t h e primary
c i r c u i t can be e a s i l y handled by t h e gas p u r i f i c a t i o n p l a n t . O u r i n t e r -
e s t was t o f i n d out t he o r i g i n of t h e s m a l l amount of tritium which has
been de tec t ed i n t h e steam c i r c u i t .
P. Cohen: I n f u t u r e experiments on tritium it might be u s e f u l t o
add tritium as HTO.
E. Hoinkis : What i s t h e iod ine concent ra t ion i n t h e primary coolan t
c i r c u i t ?
G. Ivens : There i s no d e t e c t a b l e l e v e l of i od ine i n t h e AVR primary
coolan t gas. Furthermore, no iod ine could be de t ec t ed e i t h e r on g raph i t e
spheres which are removed from t h e core or on s t e e l su r faces of components
i n d i r e c t contac t w i th t h e coolant gas. Unfortunately, t h e most in te res t - i n g su r faces , which are i n con tac t wi th t h e h o t primary gas, a r e not ac-
c e s s i b l e f o r i n spec t ion .
P. S. Weltevreden: Comparing t h e impur i ty l e v e l s of AVR an?. Dragon
it appears t h a t t h e AVR l e v e l a r e o r d e r s of magnitude h ighe r t han those of
Dragon.
59
G. Ivens: The gaseous impurities in the AVR primary circuit were
initially high because of the presence of more than 1QCJ trjns of carbon
brick structural material. This ungraphitized carbonaceous material
emits large quantities of E20 and C 0 2 when heated,
the ear ly AVR operations was restricted because of the presence of these
oxidizing impurities. In the meantime, outgassing has proceeded to the
point that the AVR power level is no longell limited by these impurities.
It should be noted, however, that in a pebble bed reactor corrosion is
distributed evenly amongst the fuel elements because they are in contin-
uous motion.
The povzr level of
Paper 3/138
OBJECTIVES AND PLANS FOR FEXESJTN?
IN THE PEACH- B-OTTOM HTGR* --"-w.-4 ___ --..
K . P . Steward
Gulf General Atomic Incorporated
San Diego, C a l i f o r n i a
ABSTRACT
The Peach Bottom r e a c t o r o f f e r s unique c a p a b i l i t i e s as a t es t f a c i l i t y f o r HTGR f u e l s . It i s t h e only r e a c t o r i n t h e United States t h a t can i r r a d i a t e HTGR f u e l i n a proper neutron spectrum, i n a pressur ized helium environ- ment, and i n an HTGR temperature regime. I n a d d i t i o n , t h e Peach Bottom r e a c t o r can accommodate kilogram q u a n t i t i e s of t es t f u e l s f o r long p e r i o d s , and complete f u e l element assemblies can be t e s t e d t o e v a l u a t e t h e i n t e r a c t i o n s of f u e l p a r t i c l e s , f u e l beds, and g r a p h i t e s t r u c t u r e s . One of t h e fundamental o b j e c t i v e s of Peach Bottom Core 2 , t h e r e f o r e , i s t o e x p l o i t t h e unique c a p a b i l i t i e s of t h i s r e a c t o r as a test f a c i l i t y f o r i r r a d i a t i o n of HTGR f u e l concepts .
Gulf General Atomic p lans i n i t i a l l y t o des ign and f a b r i c a t e f o u r types of tes t elements f o r i n s e r t i o n wi th Core 2 . Up t o 40 tes t elements may be i r r a d i a t e d w i t h i n t h e c o r e a t any one t i m e . The major objec- t ives of each element type a r e as fol lows:
1. Fuel T e s t Elements (FTEs). To e v a l u a t e t h e performance of HTGR f u e l s over a wide range of o p e r a t i n g condi t ions
2 . Recycle Fuel Test Elements (RTEs). To provide i r r a d i a t e d HTGR f u e l i n s u f f i c i e n t q u a n t i t i e s t o develop r e c y c l e processing technology, and t o tes t r e c y c l e p a r t i c l e s
3 . Fuel Bed Test Elements (FBTEs). To provide l a rge - scale tes ts of 1100-MW(e) HTGR f u e l
4 . Proof Test Elements (PTEs). To demonstrate i r r a d i a t i o n performance of F o r t S t . Vrain f u e l
*Work supported i n p a r t by t h e U.S. Atomic Energy Commission under Contracts AT(04-3)-633 and AT(04-3)-167, P r o j e c t Agreement No. 1 7 .
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Emphasis i s being placed on t h e f i r s t t h r e e element types s i n c e t h e s e have t h e g r e a t e s t re levance t o 1100-MW(e) HTGR technology. I n p a r t i c u l a r , t h e FTEs w i l l be used (1) t o determine t h e time-at-temperature l i f e t i m e s of v a r i o u s types of f u e l , (2) t o o b t a i n d a t a t o i d e n t i f y mechanisms of p a r t i c l e f a i l u r e and thereby t o improve f u e l performance and l i f e t i m e s , (3) t o t es t l o o s e p a r t i c l e g r a p h i t e i n t e r - a c t i v e f o r c e s i n blended beds, and (4) t o conduct c o n t r o l l e d i r r a d i a t i o n experiments on f u e l p a r t i c l e thermal s t a b i l i t y , meta l l ic d i f f u s i o n rates, f i s s i o n product release, and g r a p h i t e mechanical p r o p e r t i e s .
Experiments w i l l be conducted as func t ions of temperature and f l u e n c e up t o 4.2 x 1021 n/cm2; burnups w i l l b e Q20% FIMA i n t h e mixed f i s s i l e and Q60% FIMA i n t h e UC2 f i s s i l e p a r t i c l e s a t end of l i f e . s t a b i l i t y samples w i l l b e i r r a d i a t e d a t temperatures from 1000° t o 16OOOC i n thermal g r a d i e n t s up t o 1000"C/in. i n order t o determine time-temperature l i m i t s f o r coated p a r t i c l e s under i r r a d i a t i o n . Extensive p o s t i r r a d i a t i o n examination of t h e FTEs w i l l be performed. One of t h e FTEs t o b e i r r a d i a t e d f o r 3 y r i s being sponsored by t h e USAEC.
Some thermal
Object ives of t h e FBTEs, i n a d d i t i o n t o la rge-sca le t e s t i n g of 1100-MW(e) f u e l , are (1) t o eva lua te v a r i o u s 1100-MW(e) bonded bed concepts , and ( 2 ) t o determine t h e dimensional changes of blended beds of r e f e r e n c e 1100-MW(e) f u e l by p e r i o d i c gamma scanning. A l l of t h e s e elements w i l l be i r r a d i a t e d f o r 3 y r and w i l l r e c e i v e a dose of approximately 4 x 1 O 2 I n/cm2 dur ing t h i s t i m e . Most of t h e FBTEs w i l l c o n t a i n only one f u e l combination and may be monitored c o n t i n u a l l y during i r r a d i a t i o n by sampling t h e i n d i v i d u a l purge g a s streams.
The RTEs are sponsored by t h e USAEC as an i n t e g r a l p a r t of t h e Nat iona l HTGR Recycle Program. They inc lude both r e f e r e n c e and advanced concepts f o r 1100-MW(e) r e c y c l e f u e l , p r i m a r i l y as bonded r o d s , a l though some blended beds w i l l a l s o be included, tests of oxide f u e l produced by t h e sol-gel process and w i l l c o n s t i t u t e proof tests of t h e r e c y c l e 4:2(Th,U)02 B I S O p a r t i c l e s . I n a d d i t i o n , 2:O(Th,U)02 B I S O p a r t i c l e s w i l l b e i r r a d i a t e d , a t t a i n i n g t h e burnup a f t e r 3 y r i n t h e Peach Bottom r e a c t o r t h a t t h e o t h e r p a r t i c l e s would receive a f t e r 4 y r i n t h e 1100-MW(e) HTGR. The RTEs w i l l provide i r r a d i a t e d material f o r head end reprocess ing s t u d i e s a t ORNL a f t e r 1-, 2-, and 3-yr i r r a d i a t i o n s i n Core 2.
These elements w i l l provide la rge-sca le
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1. I N T R O D U C T I O N
The Peach Bottom r e a c t o r , operated by Phi lade lphia E l e c t r i c Company,
o f f e r s unique c a p a b i l i t i e s as a tes t f a c i l i t y f o r high-temperature gas-
cooled r e a c t o r (HTGR) f u e l s . It i s t h e only r e a c t o r i n t h e United States
t h a t can i r r a d i a t e HTGR f u e l i n a r e p r e s e n t a t i v e HTGR neutron spectrum
and helium coolant environment. I n a d d i t i o n , t h e Peach Bottom r e a c t o r
can accommodate kilogram q u a n t i t i e s of tes t f u e l s f o r long i r r a d i a t i o n
p e r i o d s , and f u l l - s c a l e f u e l element assemblies can be t e s t e d t o e v a l u a t e
t h e i n t e r a c t i o n s of f u e l p a r t i c l e s , f u e l beds , and g r a p h i t e s t r u c t u r e s . One
of t h e fundamental o b j e c t i v e s of Peach Bottom Core 2 ( t h e second co re t o
b e loaded i n t o Peach Bottom), t h e r e f o r e , i s t o u t i l i z e t h e unique capabi-
l i t i e s of t h i s r e a c t o r as a tes t f a c i l i t y f o r i r r a d i a t i o n of HTGR f u e l
concepts . Table 1 compares l i g h t water r e a c t o r and HTGR environments
and i n d i c a t e s t h e s u i t a b i l i t y of t h e Peach Bottom r e a c t o r f o r i r r a d i a t i n g
HTGR f u e l s .
Gulf General Atomic (GGA) has designed and i s f a b r i c a t i n g fou r types
of t es t elements f o r i n s e r t i o n wi th Core 2. Up t o 40 t es t elements may be
i r r a d i a t e d w i t h i n t h e c o r e a t any one t i m e . The element t ypes are l i s t e d
below, and t h e ch ief o b j e c t i v e s of each are given i n Table 2 .
Fuel test elements (FTEs)
Recycle f u e l tes t elements (RTES)
Fuel bed tes t elements (FBTEs)
Proof t e s t elements (PTES)
The f i r s t t h r e e element types have b a s i c a l l y t h e same des ign , w i t h
t h e f u e l being contained i n c y l i n d r i c a l g r a p h i t e bodies w i t h i n r e g u l a r
Peach Bottom f u e l element sleeves. I n c o n t r a s t , t h e PTE des ign s imula tes
a s e c t i o n of a large-HTGR f u e l block and i s hexagonal i n shape. Emphasis
i s being placed on t h e FTEs, R T E s , and FBTEs, s i n c e t h e s e elements have
g r e a t e r f l e x i b i l i t y f o r t e s t i n g f u e l under s p e c i a l l y c o n t r o l l e d condi t ions .
These elements are sponsored both p r i v a t e l y by GGA and by t h e Atomic
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Table 1. Comparison of Reactor Operating Conditions
H20 Test Reactor (ETR) Peach Bottom HTGR 1100-MW(e) HTGR
Environment
Neutron spectrum
Thermal flux (n/cmz-sec)
Fast flux (n/cm2-sec)
Core Th:U ratio
Peak fuel temp. ("C)
Thermal gradient
Burnup rate
Low-pressure static helium
Light-water reactor (Lm)
14 2x10
14 4x10
2 : l
>1300
High
Hieh
High-pressure flowing helium
HTGR
4xio13
4~10'~
8:l
>1300
Moderate
Moderate
High-pressure flowing helium
HTGR
13 4x10
13 4x10
4:l
1340
Moderat e
Moderat e I
Table 2. Chief Objectives of Various Test Elements
Fuel test elements (FTES)
1. Evaluate the performance of HTGR fuels over a wide range of operating conditions and lifetimes
a. Determine the time-at-temperature lifetimes of various types of fuel
b. Obtain data to identify mechanisms of particle deteriora- tion under extreme conditions and thereby to improve fuel performance and lifetimes
C. Evaluate various production processes
2. Conduct controlled irradiation experiments on:
a. Fuel particle thermal stability
b. Metallic diffusion rates in an HTGR environment
c. Fission product release of various types of fuel particles
d. Graphite mechanical and creep properties
e. Various fuel rod fabrication concepts
and bonded rods under HTGR conditions 3. Evaluate the long-term, in-pile performance of blended beds
1. Demonstrate performance of recycle type fuel and beds unaer actual RTLK operating conaitions
2 . Produce significant quantities of irradiated APGR fuel for reprocessing scudies at UKNL, and subsequently to:
a. Demonstrate separability of particles
b. Prove out reprocessing equipment
1. Demonstrate performance of large-HTGR fuel beds i b. Periodic gamma scanning for dimensional changes
under actual reactor operating conditions
fuel combinations for:
a. Periodic monitoring for fission gas release
Recycle fuel test elements (RTEs)
Fuel bed tes 2. Provide bonded and blended bed elements containing single elements (FBTEsJ
Proof test elements (PTEs)
1. Demonstrate irradiation performance of reference Fort St. Vrain fuel
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Energy Commission. I n a d d i t i o n , t e s t i n g of PTE-2, which has received 150
equiva len t full-power days (EFPD) of i r r a d i a t i o n i n Core 1, w i l l cont inue
i n Core 2 . Another proof t es t element (PTE-3) i s scheduled f o r i n s e r t i o n
a f t e r 300 EFPD. Both of t h e s e PTEs a re designed t o f u l f i l l t h e proof test
requirements f o r F o r t . S t . Vrain (FSV) f u e l , and are being funded under
t h e P u b l i c Serv ice of Colorado (PSC) development c o n t r a c t .
2 . D E S I G N OF TEST ELEMENTS
Fuel Test Elements
The FTEs are designed t o r e p l a c e instrumented and non-instrumented
Peach Bottom Core 2 f u e l elements. E x t e r n a l l y , t h e s e elements have t h e same appearance as s tandard C o r e 2 f u e l elements, and their b a s i c arrange-
ment and des ign are a l s o s imilar (F igs . 1 and 2 ) .
The top r e f l e c t o r , sleeve, and bottom connector components, which
form t h e o u t e r containment envelope of each tes t element, are s tandard
Core 2 f u e l element components. The lower r e f l e c t o r and i n t e r n a l t r a p are very s i m i l a r t o t h e s tandard f u e l element components. The act ive f u e l
p o r t i o n i s made up of l ong , c y l i n d r i c a l H-327;k g r a p h i t e f u e l bodies which
r e p l a c e t h e f u e l compacts i n t h e Core 2 f u e l element. Each tes t element
comprises e i t h e r t h r e e 31-in.-long f u e l bodies o r s i x 15.5-in.-long f u e l
bodies , depending on t h e s p e c i f i c t e s t o b j e c t i v e s . Eight a x i a l purge
grooves a r e p r e s e n t on t h e o u t s i d e diameter of each f u e l body. The f u e l
bodies conta in e i g h t l /Z-in.-diameter f u e l h o l e s equal ly spaced on a
c i r c u l a r p a t t e r n and are f i l l e d wi th coated f u e l p a r t i c l e s , e i t h e r i n t h e form
of f u e l rods o r blended beds (F ig . 1). The sleeve, t o p r e f l e c t o r , and
bottom connector assembly c o n s t i t u t e a completely closed containment around
t h e f u e l bodies .
A c e n t r a l (spine), 1.1-in.-diameter h o l e i s provided f o r c o n t r o l l e d
i r r a d i a t i o n t e s t i n g of v a r i o u s sample types. These c e n t e r (spine) samples
a r e enclosed w i t h i n t h e i r own c o n t a i n e r s and inc lude f u e l p a r t i c l e s and
When samples are not included, the center irradiation
Each test element is cooled by the flow of helium in the tricusp
channels between fuel elements in the same manner as the Core 2 elements,
and is purged in the same basic manner as the Core 2 fuel elements.
the purge gas flows in the purge grooves and the annular clearance gap between
the fuel body outside diameter and sleeve inside diameter. Seven test
elements will be located in special positions within.the core at which
the purge gas stream can be sampled periodically for release of fission
products.
A l l
Approximately 12 of the test elements occupy instrumented locations
within the core. Each of these elements has a tungsten-rhenium and a Chromel-
Alumel thermocouple located at the plane of maximum temperature of the
element. The core locations of the remaining uninstrumented test elements
have been selected to meetthe objective of maintaining relatively constant
power de ty within these elements during their irradition lifetime. Axial
and radial temperature profiles in a representative element are shown in
Figs. 3 and 4 .
Proof Test Elements
The PTEs are designed to replace standard instrumented Core 2 fuel
elements. Externally, they are different from Core 2 elements, having a
hexagonal shape over the fueled region (Fig. 1). Also , these elements are
cooled both internally and externally, and there is no purge stream to remove
released fission products.
Each element consists of seven sections joined together. From
bottom to top,these sections consist of a bottom connector, a bottom
reflector, four fuel zones, and a top reflector. The bottom portion of the
element is cylindrical with a transition to a hexagonal shape in the
bottom reflector section. The active fuel zones are hexagonal, with the 6d
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width a c r o s s t h e f l a t s equal t o t h e diamerer of t h e in te rmedia te spacers
of t h e r e g u l a r elements. The tes t element l e n g t h i s t h e same as f o r a
s tandard Peach Bottom element. A s shown i n p lan view i n Fig. 1, t h e element
has seven in te rna l - coolan t channels and 1 2 f u e l rod holes d i s t r i b u t e d
w i t h i n t h e hexagonal g r a p h i t e body.
seven i n t e r n a l coolant channels and t h e s i x modified t r i c u s p channels
ad jacent t o t h e element. The elements are n o t purged, but a r e instrumented
w i t h two thermocouples whose j u n c t i o n s are loca ted 53 i n . above t h e bottom
of t h e act ive core. A Chromel-Alumel thermocouple i s loca ted i n t h e
g r a p h i t e body, and a tungsten-rhenium thermocouple i s loca ted i n t h e i n n e r
r i n g of ho les w i t h i n an annular f u e l rod.
Cooling i s provided both by t h e
The a c t i v e p o r t i o n of t h e f u e l element i s composed of fou r f u e l zones
j o i n e d t o g e t h e r a x i a l l y by cemented threaded j o i n t s . Each fuel zone
conta ins 1 2 b l i n d f u e l h o l e s d r i l l e d from t h e top of t h e zone t o w i t h i n
about 0.4 i n . of t h e bottom. The diameter of t h e r e g u l a r f u e l ho les i s
0.470 i n . The f u e l h o l e s conta in ing t h e annular f u e l r o d s wi th t h e
thermocouples have a diameter of 0’.517 i n . The seven coolan t channels are
continuous from t h e top t o t h e bottom of t h e zone, and they are a l igned with
t h e channels i n a d j a c e n t zones t o form continuous i n t e r n a l coolan t
channels over t h e f u l l l e n g t h of t h e f u e l element.
PTE-2, o r i g i n a l l y i r r a d i a t e d i n Core 1, w a s n o t removed from t h e
c o r e and w i l l cont inue i r r a d i a t i o n i n Core 2 .
p r o f i l e s dur ing o p e r a t i o n are shown i n F igs . 5 and 6 . Axia l and r a d i a l temperature
3 . HTGR FUEL LOADING COMBINATIONS
Present HTGRs employ carbon-coated uranium and thorium carb ide spheres
as t h e i r f u e l .
i n diameter , are bonded i n t o f u e l rods o r compacts and a re subsequently
loaded i n t o g r a p h i t e elements o r blocks. A p o s s i b l e a l t e r n a t i v e f o r
f u t u r e HTGRs i s t o load t h e b locks wi th blended beds of l o o s e p a r t i c l e s .
I n genera l , i t i s d e s i r e d t o g a i n a b e t t e r understanding of HTGR
f u e l des ign technology i n t h e s e areas and assess t h e p r o p e r t i e s and
These f u e l p a r t i c l e s , which can vary from 250 t o 1000 pm
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performance of v a r i o u s types of coated p a r t i c l e s , f u e l r o d s , and
blended beds under i r r a d i a t i o n . The loadings of t h e test elements are
t h e r e f o r e d i c t a t e d by t h e f u e l loadings proposed f o r c u r r e n t and f u t u r e
HTGRs .
@
The f u e l p a r t i c l e s considered a re of t h e same genera l t y p e , having
s p h e r i c a l c a r b i d e o r oxide k e r n e l s , a porous "buffer" l a y e r of p y r o l y t i c
carbon (PyC) t o absorb f i s s i o n gases , a t t e n u a t e f i s s i o n r e c o i l s , and
al low f o r k e r n e l swel l ing , and an o u t e r l a y e r of r e l a t i v e l y dense
i s o t r o p i c PyC t o r e t a i n f i s s i o n gases . Such p a r t i c l e s a re termed B I S O
by GGA; T R I S O p a r t i c l e s a re s imilar b u t inc lude an e x t r a l a y e r of dense
p y r o l y t i c s i l i c o n c a r b i d e sandwiched between two l a y e r s of i s o t r o p i c PyC
t o r e t a i n meta l l ic f i s s i o n products . Cross s e c t i o n s of B I S O and T R I S O
p a r t i c l e s are shown i n Fig. 7 . P a r t i c l e s may be e i t h e r f i s s i l e (conta in ing 2 3 2 ) U235) o r f e r t i l e (conta in ing only Th
k e r n e l type and p a r t i c u l a r r e a c t o r a p p l i c a t i o n .
, and t h e i r s i z e depends on t h e
The s tandard elements i n Peach Bottom Core 2 w i l l be loaded wi th B I S O
f i s s i l e p a r t i c l e s i n t h e form of compacts. The F o r t S t . Vrain co re w i l l
b e loaded wi th TRISO f i s s i l e and TRISO f e r t i l e p a r t i c l e s i n t h e form of
f u e l rods.
and B I S O f i s s i l e p a r t i c l e s and BISO f e r t i l e p a r t i c l e s i n t h e form of
The 1100-MW(e) HTGR w i l l i n i t i a l l y be loaded wi th both TRISO
rods (see F i g . . 8 ) . T h e test element program i s aimed p r i m a r i l y toward
f u r t h e r i n g 1100-MW(e) HTGR technology, a l though advanced knowledge of t h e
performance of F o r t S t . Vrain f u e l s w i l l be obtained from t h e bonded
TRISO/TRISO f u e l included i n t h e program.
r e s t r i c t e d t o t h e 1100-MW(e) HTGR s t a r t u p and r e c y c l e modes of opera t ion .
The d i s c u s s i o n below i s
I n t h e 1100-MW(e) HTGR, two types of g r a p h i t e block loadings w i l l
b e used ( see Fig. 8 ) . The p a r t i c l e s i n t h e A-type block can be processed
t o g e t h e r a f t e r i r r a d i a t i o n , bu t t h e p a r t i c l e s i n t h e B-type block r e q u i r e
s e p a r a t i o n . This s e p a r a t i o n i s necessary because f i s s i o n a b l e U i s
bred i n t o t h e f e r t i l e p a r t i c l e s and i s recycled i n t h e (Th,U233)02 B I S O
r e c y c l e p a r t i c l e s .
233
However, l a r g e q u a n t i t i e s of U236 are produced i n t h e
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U235C2 T R I S O p a r t i c l e s , and continuous r e c y c l e of t h i s m a t e r i a l i s no t
d e s i r e d . The amount of U236 bred i n t o t h e U235C2 B I S O p a r t i c l e s i n t h e
s t a r t u p A block i s r e l a t i v e l y s m a l l and i s progress ive ly d i l u t e d wi th
every r e c y c l e ; t h e s e p a r t i c l e s t h e r e f o r e do not need separa t ing . I n t h e
FTEs and FBTEs, emphasis i s placed upon t h e performance of t h e s t a r t u p A
and B block combinations, both as rods and loose p a r t i c l e s . The RTEs
emphasize only t h e v a r i o u s r e c y c l e block loadings and p o s s i b l e a l t e r n a t i v e s
t o t h e r e f e r e n c e loadings shown i n Fig. 8. The loading combinations being
i n v e s t i g a t e d i n t h e v a r i o u s elements and t h e j u s t i f i c a t i o n s f o r t h e i r
i n c l u s i o n are given i n Table 3.
4 . RECYCLE FUEL TEST ELEMENTS
Eight RTEs a re being f a b r i c a t e d f o r i n s e r t i o n i n Peach Bottom Core 2.
These elements are funded by t h e USAEC a s an i n t e g r a l p a r t of t h e Nat ional
HTGR Recycle Program, and are being f a b r i c a t e d j o i n t l y by GGA and Oak
Ridge Nat iona l Laboratory (ORNL). The main o b j e c t i v e s of t h e elements
are l i s t e d i n Table 2 . Two of t h e RTEs are t o be i r r a d i a t e d f o r 1 y r ,
two f o r 2 y r , and fou r f o r 3 y r ( s e e F ig . 9 ) . A l -yr i r r a d i a t i o n i n t h e
Peach Bottom HTGR i s roughly 300 EFPD. P e r i o d i c v i s u a l and gamma scanning
w i l l be conducted on t h e elements , bu t they w i l l n o t be instrumented. The
elements w i l l be shipped t o ORNL f o r p o s t i r r a d i a t i o n examination and subsequent
s t u d i e s a f t e r d i scharge from t h e Peach Bottom r e a c t o r .
Each element c o n s i s t s of s i x 15.5-in. g r a p h i t e bodies i n which t h e
uranium loading is determined by t h e p o s i t i o n i n t h e r e a c t o r . The f u e l
p a r t i c l e combinations and l o c a t i o n s i n t h e elements have been s e l e c t e d t o
produce i r r a d i a t e d f u e l bed materials which w i l l have been exposed t o a
wide range of r e a c t o r environmental condi t ions . These f u e l bed m a t e r i a l s
w i l l be used segment by segment t o t e s t and develop f u e l reprocess ing
equipment and processes . The u n i t o p e r a t i o n a l processes which w i l l be
i n v e s t i g a t e d inc lude s i z e r e d u c t i o n , s i z e s e p a r a t i o n , burning, chemical
d i s s o l u t i o n , leaching , and s o l i d s t r a n s p o r t . I n a d d i t i o n , t h e elements
w i l l provide proof tes ts of so l -ge l oxide f u e l p a r t i c l e s and, i n p a r t i c u l a r ,
t h e r e f e r e n c e r e c y c l e (Th,U)02 f u e l p a r t i c l e s .
69
Tab le 3 . F u e l Loading Combina t ions i n Advanced T e s t E lements
J u s t i f i c a t i o n D e s i g n a t i o n Comb i n a t i o n Type of Loading
RTE s
(4 .2 Th,U)02 B I S O
U02 BISO + ThC2 BISO
(2 .0 Th,U)02 B I S O + Tho2 B I S O
(2 .0 Th,U)C2 B I S O + ThC2 BISO
UC2 B I S O + ThC2 BISO
U C 2 TRISO + ThC2 B I S O
U02 BISO + Tho2 BISO
UC2 B I S O + Tho2 BISO
UC2 TRISO + ThC2 TRISO
Loose & bonded
Bonded
Bonded
Bonded
Loose & bonded
Loose & bonded
Bonded
Bonded
Bonded
Refe rence r e c y c l e p a r t i c l e ; w i l l check o u t bed s t i c k i n g , chemica l s e p a r a t i o n , e t c .
Backup r e c y c l e A b l o c k l o a d i n g i f Th i s e l i m i n a t e d from (Th,U)O p a r t i c l e s
A l t e r n a t e r e c y c l e A b l o c k l o a d i n g ; 2:l r a t i o t o o b t a i n e n d - o f - l i f e burnup (20%) i n 3 y r . Tho2 proposed i f o x i d e p r o c e s s adop ted .
Recyc le A b l o c k l o a d i n g ; 2:l r a t i o t o o b t a i n 20% burnup i n 3 y r
S t a r t u p A b l o c k l o a d i n g
S t a r t u p and r e c y c l e B b l o c k l o a d i n g
Backup B b l o c k l o a d i n g i f Th is e l i m i n a t e d and i f s o l - g e l Tho2 i s used
Backup A o r B b l o c k l o a d i n g ; s e p a r a b l e chemica l ly o r by s e l e c t i v e b u r n i n g
A l t e r n a t e B b l o c k l o a d i n g i f c l e a n e r pr imary c i r c u i t s r e q u i r e d
2
~
FTEs and FBTEs
e UC2 BISO + ThC2 BISO Loose & bonded S t a r t u p A b l o c k l o a d i n g
f UC2 TRISO + ThC2 BISO Loose & bonded S t a r t u p and r e c y c l e B b l o c k l o a d i n g
k (2 .0 Th,U)C2 BISO + ThC2 B I S O Loose & bonded Recycle A b l o c k l o a d i n g w i t h (Th,U)C2 s u b s t i t u t i n g f o r (Th,U)02
1 (2 .0 Th,U)C2 TRISO + ThC2 TRISO Loose & bonded Refe rence F o r t S t . V r a i n l o a d i n g
Tab le 4 . RTE Loading Combinationsa
F i r s t D i scha rge Second Discha rge F i n a l D i scha rge Cen te r L i n e
P o s i t i o n of Temp RTE 1, RTE 3 , RTE 5 , RTE 7 , Fuel Body Range A l l Bonded A l l Bonded A l l Bonded RTE 6 , A l l Bonded i n Element (OF) (Quar t e red ) RTE 2 (Quar t e red ) RTE 4 (Quar t e red ) A l l Bonded (Quar t e red ) RTE 8
6 2050- b d e i f b d e i b d e i g a c f g f b
( t o p of 1950 r e a c t o r )
5 2250- bdeh bdeh d bdeh f ac f g i b
2050
4 2250- a c f g e a c f g f a c f g f bdeh d
3 2050- a c f g f b a c f g a c f g d b d h i e
(max. f l u x ) 2300
b
(max. f l u x ) 2250
2 1650- ac f g d ac f g f b a c f g 2050
f b d h i i
1 1050- ac f g ac f g e a c f g e b d h i f b b
(bot tom of 1650 r e a c t o r )
aLoadings are i n d i c a t e d by letters a , b , c , d , e , f , g, h , and i, and are d e f i n e d i n T a b l e 3 . bBlended beds .
70
A
The proposed loadings of t h e RTEs a re shown i n Table 4 . I n R T E s 1,
3 , 5 , and 7 , a l l s i x bodies are "quartered," and c o n t a i n a d i f f e r e n t f u e l
combination i n every two h o l e s of a given body. These elements w i l l be
used f o r small-scale reprocess ing i n t h e ORNL h o t c e l l . RTEs 2 , 4 , 6 , and
8 , which conta in only s i n g l e loadings i n a given body, w i l l provide l a r g e r
amounts of t h e ch ie f combinations of i n t e r e s t f o r h o t c e l l work and a l s o
w i l l provide t h e i n i t i a l i r r a d i a t e d material requi red f o r reprocess ing i n
t h e Thorium-Uranium Recycle F a c i l i t y (TURF). A d d i t i o n a l l y , some blended
beds w i l l be i r r a d i a t e d i n RTEs 2 , 4 , and 8 , s i n c e t h e s e elements c o n s t i t u t e
a backup des ign f o r f u e l rods i n t h e HTGR.
Fuel f o r t h e RTEs i s being f a b r i c a t e d by both ORNL and GGA. ORNL has
produced and coated a l l t h e so l -ge l oxide k e r n e l s , and GGA has produced
and coated t h e v a r i o u s c a r b i d e k e r n e l s . The p a r t i c l e s have been made t o
t e n t a t i v e 1100-MW(e) HTGR s p e c i f i c a t i o n s . Fuel rods wi th d i f f e r e n t matrices
are be ing f a b r i c a t e d f o r t h e RTEs both a t GGA and ORNL by means of t h e
h o t i n j e c t i o n molding process . Blended beds are being loaded a t GGA. A l l
element assembly w i l l t a k e p l a c e a t GGA, and i t i s planned t o s h i p t h e
elements t o Peach Bottom by May 15.
5 . FUEL BED TEST ELEMENTS
S i x FBTEs being f a b r i c a t e d f o r i n s e r t i o n i n Peach Bottom Core 2.
The main o b j e c t i v e s of t h e s e elements , which are funded p r i v a t e l y by
GGA, are given i n Table 2. It i s planned t o i r r a d i a t e a l l of t h e s e elements
f o r 3 y r (900 EFPD), and t o conduct p e r i o d i c v i s u a l and gamma scanning.
Gamma scanning w i l l reveal dimensional changes of t h e beds, p a r t i c u l a r l y i n
t h e case of FBTEs 5 and 6 , which are l o o s e bed elements. A l l s i x FBTEs
w i l l be instrumented and w i l l be i n s t a l l e d on stand-off p i n s where t h e
purge gas stream can b e monitored p e r i o d i c a l l y dur ing i r r a d i a t i o n . In-p i le
f i s s i o n produce release d a t a can t h u s b e obtained from t h e s e elements. The
mixed element (FBTE-5), which i s complementary t o FTEs 1 and 2 (see Sec t ion 6 ) , w i l l c o n t a i n g r a p h i t e s p i n e samples and w i l l receive p o s t i r r a d i a t i o n
examination; t h e o t h e r elements w i l l conta in no s p i n e samples and may b e used f o r reprocess ing s t u d i e s a t ORNL a f t e r d i scharge .
71
Each element c o n s i s t s 'of t h r e e 31-in. bodies r a t h e r than s i x 15.5-in.
bodies as i n . t h e R T E s . The proposed f u e l p a r t i c l e loading combinations a r e
shown i n Table 5 , and i n each case t h e s e are r e l e v a n t t o t h e 1100-MW(e) HTGR
loadings.
b i n a t i o n s r e p r e s e n t t h e s t a r t u p mode f o r t h e 1100-MW(e) HTGR (F ig . 8 > , and
(Th,U)C B I S O + ThC B I S O r e p r e s e n t s t h e r e c y c l e A block loading w i t h
carb ide r a t h e r than oxide f i s s i l e k e r n e l s .
T R I S O p a r t i c l e s are t o be used i n F o r t S t . Vrain,and t h i s p a r t i c u l a r
element w i l l t h e r e f o r e provide advanced knowledge of t h e performance of such
bonded f u e l . I n a d d i t i o n , t h e f i s s i o n gas release d a t a obtained by purge
stream sampling w i l l provide cont inuing s u r v e i l l a n c e of F o r t S t . Vrain
opera t ing condi t ions . Only a s i n g l e f u e l combination i s t o be used throughout
FBTEs 1, 2, 3 , 4 , and 6 i n order t h a t t h e f i s s i o n gas release d a t a can be
d i r e c t l y r e l a t e d t o t h e performance of a p a r t i c u l a r type of f u e l .
The U C 2 B I S O + ThC2 B I S O and UC TRISO + ThC2 B I S O bonded com- 2
2 2 Bonded (Th,U)C2 TRISO + ThC2
The o u t e r bed loadings of t h e mixed element FBTE-5, which are t h e
s a m e as i n FTEs 1 and 2, are shown i n F ig . 10. This i s a blended bed element
i n which t h e p a r t i c l e s are mixed w i t h c a l c i n e d petroleum coke ('L0.15 g/cm
of f u e l h o l e ) . Body 1 conta ins p a r t i c l e s wi th propylene-derived coa t ings
which are r e l e v a n t t o t h e F o r t S t . Vrain and 1100-MW(e) HTGRs. These
p a r t i c l e s have r e l a t i v e l y high PyC coa t ing d e n s i t i e s (1.70 t o 1 .80 g/cm
f o r TRISO and 1.80 t o 1 .90 g/cm3 f o r BISO). I n bodies 2 and 3 , t h e e f f e c t of PyC d e n s i f i c a t i o n r a t e on t h e r h e o l o g i c a l problems of blended beds w i l l
be i n v e s t i g a t e d . The high-densi ty PyC i n t h i s case is 1.80 t o 1 . 9 0 g/cm
and t h e low-density PyC i s 1.55 t o 1 .65 g/c:m , The ra te a t which
stresses i n blended beds b u i l d up may v a r y wi th t h e PyC d e n s i f i c a t i o n r a t e
on t h e p a r t i c l e s , t h e l a t te r rate being h i g h e r , t h e lower t h e PyC d e n s i t y 21 2 f o r doses up t o about 4 x 10 n/cm . Owing t o such u n c e r t a i n t y of
blended bed behavior , t h e 3-yr i r r a d i a t i o n s p i n e samples i n FTE-3 w i l l
b e contained i n a bonded element, and FBTE-5 w i l l demonstrate t h e 3-yr
i r r a d i a t i o n behavior of such beds.
i n t e r a c t i o n stresses w i l l n o t b u i l d up s i g n i f i c a n t l y u n t i l a t least t h e
t h i r d year of i r r a d i a t i o n ,
from t h e r e a c t o r f o r p o s t i r r a d i a t i o n examination a t any s u i t a b l e t i m e ,
s i n c e i t w i l l c o n t a i n no c r i t i c a l s p i n e samples.
3
3
3
It i s a n t i c i p a t e d t h a t p a r t i c l e / g r a p h i t e
I f necessary , however, FBTE-5 could be removed
72
6. FUEL TEST ELEMENTS
S i x FTEs are being f a b r i c a t e d f o r i n s e r t i o n with Peach Bottom Core 2 .
The o v e r a l l o b j e c t i v e s of t h e s e elements a r e given i n Table 2 ; more s p e c i f i c
o b j e c t i v e s of t h e v a r i o u s s p i n e samples a r e d iscussed i n t h e following
s e c t i o n s . The elements w i l l c o n t a i n both bonded rods and blended beds as
t h e d r i v e r f u e l , and c o n t r o l l e d experiments w i l l be conducted i n t h e s p i n e s
Two of t h e FTEs w i l l be i r r a d i a t e d f o r 1 y r , two f o r 2 y r , and two f o r 3 y r
( s e e F ig . 9 ) . This schedule was chosen p r i m a r i l y t o a s s e s s t h e e f f e c t s
of i r r a d i a t i o n dose on t h e performance of t h e blended beds, bonded r o d s ,
and s p i n e samples. A l l t h e elements w i l l b e instrumented, and FTE-6 w i l l be a t a purge sampling p o s i t i o n . P o s t i r r a d i a t i o n examinations of a l l t h e
elements w i l l be conducted a t GGA.
Outer Bed Loadings
Each element c o n s i s t s of t h r e e 31-in. bodies . The loadings of FTEs
3 , 4 , 5 , and 6 are shown i n F ig . 11; and t h e o u t e r bed loadings of FTEs
1 and 2 are shown i n Fig. 1 0 . FTEs 1 and 2 use blended beds as descr ibed i n Sec t ion 5, whi le FTE-3 uses bonded rods conta in ing t h e same
p a r t i c l e s , The loadings of FTEs 4 , 5, and 6 a r e i d e n t i c a l , and
t h e p a r t i c l e s are t h e same as those i r r a d i a t e d i n FBTEs 1-4. f u e l rods i n a given body w i l l be bonded wi th an i s o t r o p i c coke + p i t c h ,
and t h e remainder w i l l be bonded wi th a n a t u r a l f l a k e g r a p h i t e + p i t c h .
Since any p a r t i c u l a r combination and mat r ix runs t h e complete l e n g t h of
any given element, i t w i l l be p o s s i b l e t o determine t h e e f f e c t s of
temperature , f l u x , and f l u e n c e up t o 4 . 2 x 1021 n/cm
performance of t h e s e rods. Likewise, t h e e f f e c t s of t h e same v a r i a b l e s
on blended bed performance can be checked i n FTEs 1 and 2 and FBTE-5.
Half of t h e
2 on t h e i r r a d i a t i o n
73
diameter s p i n e ho le .
i n t o f i v e c a t e g o r i e s according t o t h e samples i n s e r t e d and t h e tes t o b j e c t i v e s :
I n g e n e r a l , t h e s p i n e sample program can be divided
1. Thermal s t a b i l i t y of f u e l p a r t i c l e s
2 . F i s s i o n product release from f u e l p a r t i c l e s
3 . Metallic f i s s i o n product d i f f u s i o n through g r a p h i t e
4 . Isothermal proof t e s t i n g of f u e l rods
5. Phys ica l p roper ty changes of g r a p h i t e s
The specimens d i f f e r i n d e s i g n , bu t they a re a l l contained w i t h i n 1-in.-
diameter c y l i n d r i c a l c r u c i b l e s having s u f f i c i e n t c l e a r a n c e w i t h i n t h e f u e l
body c e n t e r h o l e t o prevent i n t e r f e r e n c e w i t h t h e g r a p h i t e body a t any
t i m e dur ing i r r a d i a t i o n . By us ing t h e s e c r u c i b l e s , a l l t h e c e n t e r samples
are i n e f f e c t t r i p l y contained, and t h e experiments r e q u i r i n g more p r e c i s e
p o s t t e s t i n g a n a l y s i s ( thermal s t a b i l i t y and f i s s i o n product r e l e a s e ) employ
smaller c o n t a i n e r s i n s i d e t h e s e c r u c i b l e s . The purpose and d e s c r i p t i o n of
each type of experimental sample are presented below, and t h e p r i n c i p a l
experimental v a r i a b l e s being i n v e s t i g a t e d w i t h each type of sample are
d iscussed . I n a l l cases, t h e experiments are repeated i n 1-, 2- , and 3-yr
i r r a d i a t i o n elements , o f t e n a t d i f f e r e n t temperatures s o t h a t t h e e f f e c t s
of i r r a d i a t i o n dose and temperature can be assessed .
Fuel P a r t i c l e Thermal S t a b i l i t y Samples
The purposes of t h e s e experiments are:
1. To expose f u e l p a r t i c l e s t o a w i d e range of o p e r a t i n g v e r i a b l e s ,
p a r t i c u l a r l y high temperatures and temperature g r a d i e n t s
2 . To determine t h e time-at-temperature l i f e t i m e s of v a r i o u s types of
f u e l
3 . To o b t a i n d a t a which can, when i n t e g r a t e d with o t h e r work, lead t o
a b e t t e r understanding of p a r t i c l e d e t e r i o r a t i o n and f a i l u r e under
extreme condi t ions
I n g e n e r a l , u s e f u l data concerning p a r t i c l e performance and des ign l i m i t s
can be obtained o n l y by exposing v a r i o u s p a r t i c l e types t o condi t ions severe
74
enough t o cause f a i l u r e of some of t h e p a r t i c l e s . This can be achieved by
combining abnormally high i r r a d i a t i o n temperatures and thermal g r a d i e n t s *
which can cause k e r n e l migra t ion , kernel-coat ing i n t e r a c t i o n , and subsequent
p a r t i c l e coa t ing f a i l u r e .
The most s a t i s f a c t o r y way t o achieve high temperatures and high thermal
g r a d i e n t s i n t h e tes t elements i s t o use t h e sample des ign shown i n F ig . 1 2 .
P a r t i c l e s are loaded i n d i v i d u a l l y i n t o s e p a r a t e holes of t h e inne r g r a p h i t e
c r u c i b l e s . These c r u c i b l e s s l i d e i n t o t h e c y l i n d r i c a l s p i n e c r u c i b l e , which
i s then loaded wi th l o o s e p a r t i c l e s , and a l i d i s screwed i n t o p l ace . The
amount of uranium i n t h e p a r t i c l e s and t h e a x i a l p o s i t i o n of t h e c r u c i b l e
i n t h e element determine t h e maximum temperature and temperature g r a d i e n t
experienced by t h e p a r t i c l e s i n t h e i n n e r c r u c i b l e s . Several of t h e i n n e r
crucibles are assembled within each 1-in.-diameter crucible. The maximum
temperature of t h e s e c r u c i b l e s w i l l b e about 1 5 O O 0 C , and temperature g r a d i e n t s
w i l l be up t o 1000"C/in.
o t h e r s are bonded i n p l ace . The experiment i s designed t o provide condi t ions
under which k e r n e l migra t ion can occur and p o s s i b l y r e s u l t i n t h e f a i l u r e of
some of t h e p a r t i c l e coa t ings i n t h e i n n e r c r u c i b l e s , c e r t a i n of which have
been e s p e c i a l l y s e l e c t e d because of high migra t ion ra tes observed i n out-of-
p i l e tests. Some o t h e r , s impler c r u c i b l e s a r e a l s o being used t o i r r a d i a t e
p a r t i c l e s from t h e same ba tches under almost i so thermal condi t ions .
Some p a r t i c l e s i n t h e s e c r u c i b l e s are l o o s e and
Var iab les o t h e r than f l u e n c e and temperature t h a t are being i n v e s t i g a t e d
can b e convenient ly divided i n t o two c a t e g o r i e s :
v a r i a b l e s . Kernel v a r i a b l e s inc lude :
k e r n e l v a r i a b l e s and coa t ing
Kernel type . . . . . . U C 2 , (Th,U)C2, ThC2, U02,(Th,U)02, Tho2
Th:U r a t i o . . . . . . Zero, 2:1, 4 : 1 , 18:l
Impurity con ten t . . . . Various amounts
Hydrogen content . . . . Kernels d e l i b e r a t e l y hydrolyzed before coa t ing
Coating v a r i a b l e s inc lude :
B I S O and TRISO type coa t ings
D i f f e r e n t c o a t i n g gases
High and low c o a t i n g d e n s i t i e s
75
The c r u c i b l e s were radiographed before and w i l l be radiographed a f t e r
. i r r a d i a t i o n i n hopes of r e v e a l i n g k e r n e l and coa t ing dimensional changes,
k e r n e l - m i g r a t i o n , and p a r t i c l e f a i l u r e . Other p o s t i r r a d i a t i o n examination
tests w i l l i n c l u d e photomacrography, gamma scanning, autoradiography,
metal lography, and e l e c t r o n microprobe a n a l y s i s .
Fuel P a r t i c l e F i s s i o n Product Release Samples
The purpose of t h e s e experiments i s t o o b t a i n t h e fol lowing information:
1. I n - p i l e and out-of-pi le f i s s i o n product r e l e a s e d a t a f o r B I S O and
TRISO f u e l p a r t i c l e s as a func t ion of burnup and temperature
2 . D i s t r i b u t i o n c o e f f i c i e n t s of f i s s i o n products between k e r n e l s and
coated p a r t i c l e s
3 . Kernel release d a t a a s a func t ion of burnup and temperature
4 . The e f f e c t of d i f f e r e n t types of k e r n e l s ( f i s s i l e , f e r t i l e , ox ides ,
carb ides) on f i s s i o n product r e l e a s e
5 . Thorium and uranium migrat ion i n k e r n e l and coa t ing as a f u n c t i o n
of temperature 6 . The e f f e c t of m e t a l doping of t h e coa t ings on t h e f i s s i o n
product r e l e a s e
T h e des ign of g r a p h i t e c r u c i b l e s f o r f i s s i o n product release samples i s
shown schemat ica l ly i n F ig . 1 3 . A few hundred l o o s e p a r t i c l e s are loaded i n t o
each c r u c i b l e a long w i t h g r a p h i t e f l o u r t o absorb f i s s i o n products .
c r u c i b l e i s i n t u r n contained w i t h i n an o u t e r g r a p h i t e c r u c i b l e approximately
1 i n . i n diameter by 1 . 2 5 i n . long. Some of t h e small c r u c i b l e s a re contained
w i t h i n thick-walled niobium cans ( % 1 / 4 i n . t h i c k ) , as shown i n Fig. 1 4 . The o b j e c t of t h e niobium cans i s t o r e t a i n a l l t h e f i s s i o n products r e l e a s e d
during i r r a d i a t i o n w i t h i n t h e c r u c i b l e , and t h i s can be achieved only w i t h
a s e a l e d can. However, r e a c t o r phys ics c o n s i d e r a t i o n s l i m i t t h e amount
of metal which can be placed i n t h e c o r e , and t h e r e f o r e g r a p h i t e o u t e r
c r u c i b l e s have been used f o r most of t h e s e samples. The v a r i a b l e s being
i n v e s t i g a t e d w i t h t h e f i s s i o n product release samples are:
The
76
BISO versus TRISO coatings
uc2, (Th,U)C2, ThC2, U 0 2 , (Th,U)02, Tho2 kernels
Effect of doping of fissile particle coatings
Postirradiation examination of the fission product release samples,
which will be carried out in the Chemistry Department facilities at GGA
rather than the Hot Cell, will include:
1. Fission gas release and fission product release measurements
2. Determinations of fission product concentrations between kernels,
coatings, graphite, and charcoal, leading to in-pile release data
3 . Postirradiation anneals to confirm release data 91 4 . Postactivation analyses for Sr release
5. Bare kernel release measurements
6. Fission product release measurements on doped particles
Metallic Diffusion Samples
The purpose of the metal diffusion studies is to obtain:
1. Migration rates for strontium, cesium, barium, samarium, etc., in
graphite under reactor conditions as a function of metal concentra-
tion and temperature
2 . Data on the effects of the presence of other fission product metals
on the migration rate of individual metals (especially strontium)
3 . Data on the ability of getter materials to reduce metal migration.
(Getter materials combine with fission products such as strontium
to inhibit their diffusion into the reactor system.)
4 . Data on the integrity of getter materials
A typical graphite crucible for the diffusion samples is shown in
Fig. 15. The graphite crucibles are about 1.25 in. long and 1.0 in.
in outside diameter. The annular hole contains various metals (such as
strontium, cesium, and barium) in the form of carbides, mixed in known
proportions in a graphite matrix material.
77
Variables to be investigated include different fission product elements
and element concentrations, combinations of various elements, and getters. crs
I Postirradiation examination will include:
1. Sectioning of crucibles and determination of metal concentrations
across the crucible walls
2. Analyses of the source materials to determine total metal l o s s
3 . Calculations of migration rates for each metal
4 . Determination of the effects of getters 5. Investigations of getter integrity
Bonded Rod Samples
Bonded rod samples are included to evaluate the performance of various
types of bonded fuel rod concepts as functions of temperature and irradiation
dose, and thereby to determine the best overall fuel rod concept for use
in future HTGRs.
Bonded rods are approximately 1 1 2 in. in diameter and from 314 in.
to 2 in. long.
with a screw-on top.
type, production method, and packing fraction.
Each rod is inserted in a 1-in.-diameter graphite crucible
The variables being investigated include filler
Postirradiation examination of the samples will include visual
_ _ _ _ _ _ _ _ _ _ - _ - B O O V I-_- _ _ _ _ - _ - - - - _ - -_- -_-
LOW DENSITY = 1.55-1.65 G/CM3 HIGH DENSITY = 1.80-1 -90 G/CM3
Fig . 10. Outer Bed Loadings of FBTE 5 ( a l s o FBTEs 1 and 2 ) .
86
FTE 3 I I
UC2 + ThC2 (HIGH DENSITY)
I I I
ACETYLENE BUFFERS: MIXED GAS ISOTROPIC COATINGS
FTE 4,5,6 I I
(Th,U)C2 + ThC2 (HIGH DENSITY)
(Th,U)C2 TRISO + ThC2 TRISO
I I I
PROPYLENE BUFFERS: PROPYLENE ISOTROPIC COATINGS
Fig . 11. Outer Bed Loadings of Fuel Test Elements. For FTEs 1 and 2 see F ig . 8 ; loading of a l l three bodies i n each element i s i d e n t i - c a l ; a l l bonded rods.
-1
P A R T I C L E S
INNER CRUCIBLE (MINUS L I D )
r 3" T O 6"
";I
L I D (SCREWS I N ) /
,OUTER C R U C I B L E - 1 " O . D . MAX
/CRUCIBLE AS SHOWN AT LEFT
/ U N BO ND E D P A R T I C L E S
F i g . 12.
OUTER CRUCIBLE
Design of Thermal S t a b i l i t y Spine Samples.
C I NNER GRAPH I T E CRUC I B L E
COKE \ F I L L E R
GRAPH I T E CRUC I B L E
1 .
0"
Fig. 13. Design of Fission Product Release Spine Samples.
N I O B I U M N I O B I U M F O I L S H I M SPACER W I R E AND GRAP-HO I L ( P y C )
FOIL S H I M
GRAPH I T E CRUC I B L E
WELD F U E L PART I C L E S
rig. 14. Design of Alternative Fission Product Release Spine Samples.
88
/
\J
a, d a
co c d
$ w
w
w c M
d
rn
d
89
DISCUS SI ON
S. I. Kaplan: P lease desc r ibe t h e removal of t h e broken f u e l e l e -
ment t h i s p a s t month.
John Kemper: During t h e removal of t h e Peach Bottom Core I f u e l
elements t h a t had developed cracked g raph i t e s l eeves , one of t h e f u e l
elements f e l l back i n t o t h e core . When a second a t tempt w a s made t o
remove t h e f a l l e n element only t h e upper s e c t i o n could be removed. A
s p e c i a l removal t o o l and jacking device weredeveloped and t e s t e d . The
bottom s e c t i o n was jammed on t h e s t andof f p in , b u t with t h e new t o o l i t
w a s s u c c e s s f u l l y removed without d i f f i c u l t y . A s of t h i s d a t e , a l l o f
t h e f u e l elements t h a t had experienced cracked s l eeves have been success-
f u l l y removed, and over 200 new Core I1 type elements have been loaded.
It i s planned TO have Core I1 loaded and the p l a n t r e tu rned t o power by
e a r l y t h i s summer. It i s a c r e d i t t o t h e r e f u e l i n g t e a m and t h e HTGR
concept t h a t wi th cons iderable unforeseen f u e l element removal problems,
t h e elements were a l l removed from t h e core i n a r e l a t i v e l y s h o r t per iod
of e lapsed t ime,
G. Meijer : Refer r ing t o your i r r a d i a t i o n experiments of 1100 Mwe
H E R f u e l , what are t h e des ign burnup, f luence and temperature condi t ions
f o r t he 1100 Mwe HTGR f u e l ?
K. P. Steward: M a x i m u m burnup i n m i x e d f i s s i l e particles i s 20%.
Maximum burnup i n UC2 b u f f e r d i l u t e d f i s s i l e p a r t i c l e s i s approximately
75% maximum; fast f luence expected i s approximately 8 x lo2' nvt .
mem temperatures experienced by t h e f u e l w i l l be 1350°C.
Maxi-
D. Tytga t : 1. What w i l l be t h e d i f f e r e n t pyrocarbon d e n s i t i e s
adopted f o r t h e coated p a r t i c l e s ? 2. The f u e l element experiments i n
Peach Bottom a r e supposed t o s t a y 1, 2, and 3 yea r s . Are these years
f u l l power ope ra t ing years or ca lendar y e a r s ?
K. P. Steward: 1. On BISO p a r t i c l e s t h e "high" d e n s i t y PyC w i l l be
Outer PyC 1.80-1.90 g/cm3 and the "low" d e n s i t y w i l l be 1 .55-1.65 g/cm3.
d e n s i t i e s on TRISO p a r t i c l e s w i l l be 1.70-1.80 g/cm3.
per iods r e f e r r e d t o are increments of 300 e f f e c t i v e f u l l power days. Each
2. The ope ra t ing
90
such increment w i l l t a k e up approximately one ca lendar year of Peach
Bottom i r r a d i a t i o n .
Hugh B. Stewart : John KemRer has pointed out t h e e f f e c t i v e way i n
which t h e cracked Core No. I f u e l elements have been removed. It i s
worth not ing t h a t the cracked s l eeves i n Core No. I occurred as a result of compact expansion due t o t h e very p r imi t ive coated p a r t i c l e s t h a t were,
used i n t h a t core. I n f a c t , Roy Huddle has pointed out t ha t t h e s e p a r t i -
c l e s were not coated p a r t i c l e s ; they were "covered" p a r t i c l e s . Core No. I1 w i l l use t h e h igh ly developed coated p a r t i c l e s now a v a i l a b l e t o us and t h e phenomenon tha t was observed i n Core No. I w i l l not occur i n
Core No. 11.
91
PLANT CONSTRUCTION EXPERIENCE
(Session 11)
92
Chairman : G. E. Locket t , OECD High Temperature Reactor P ro jec t
Co-Chairman: M. Bender, Oak Ridge Nat iona l Laboratory
Paper 1/105
FORT ST. V R A I N CONSTRUCTION PROGRESS -* - -' ~ ~ _. ."..--.=f*-"-h.
"-II_._ -_._-.- .-- .- * *- - H . N . Wellhouser
A s s i s t a n t P r o j e c t Manager For t S t . Vrain
San Diego, C a l i f o r n i a Gulf General Atomic
ABS TRACT
The 330-Mw(e) F o r t S t . Vrain Nuclear Generating S t a t i o n i s being b u i l t by Gulf General Atomic Incorporated a s prime c o n t r a c t o r f o r t h e P u b l i c Serv ice Company of Colorado as p a r t o f t h e USAEC Power Reactor Demonstration Program. Among t h e s i g n i f i c a n t design f e a t u r e s incorporated i n t h e p l a n t are t h e p r e s t r e s s e d concre te r e a c t o r v e s s e l , once-through modular steam g e n e r a t o r s with i n t e g r a l superhea ters and r e h e a t e r s , steam- d r i v e n axial-f low helium c i r c u l a t o r s , and hexagonal g r a p h i t e f u e l elements incorpora t ing improved coated f u e l p a r t i c l e s . Construct ion of t h e p l a n t f e a t u r e d t h e u s e of ground f r e e z i n g t o provide a cofferdam t o keep ground water from t h e excava- t i o n and preplaced aggregate concre te f o r t h e bottom head of t h e p r e s t r e s s e d concre te r e a c t o r vsse l . A s of March 31, 1970 , c o n s t r u c t i o n i s est imated t o be over 62% complete and on schedule f o r a completion d a t e of June 1 9 7 1 .
I N T R O D U C T I O N
The 330-Mw(e) For t S t . Vrain Nuclear Generating S t a t i o n , now under con-
s t r u c t i o n , i s being b u i l t by Gulf General Atomic Incorporated f o r t h e Publ ic
Service Company of Colorado and i n cooperat ion with t h e USAEC as p a r t of t h e
Power Reactor Demonstration Program. The s t a t i o n i s loca ted approximately
35 m i l e s n o r t h of Denver, Colorado, and i s scheduled t o go i n t o commercial
o p e r a t i o n i n 1 9 7 2 . Gulf General Atomic h a s r e t a i n e d Sargent & Lundy as
Architect-Engineer and EBASCO Services as c o n s t r u c t o r .
The F o r t S t . Vrain p l a n t i n c o r p o r a t e s a number of s i g n i f i c a n t des ign
f e a t u r e s new t o power r e a c t o r systems. The most prominent are t h e p r e s t r e s s e d
concre te r e a c t o r vessel (PCRV), once-through modular steam genera tors wi th
0 i n t e g r a l superhea ters and r e h e a t e r s , steam-driven ax ia l - f l o w helium c i r c u l a t o r s ,
93
94
and hexagonal g r a p h i t e f u e l e lements i nco rpora t ing improved pyrocarbon-si l i -
con ca rb ide coated f u e l p a r t i c l e s .
The flow diagram shown i n F ig . 1 p o i n t s ou t t h e major opera t ing parameters .
The helium coolant a t a p re s su re of about 700 p s i a flows downward through t h e
r e a c t o r core where i t i s hea ted t o 1430°F. The coolan t flow can be trimmed
by t h e use of o r i f i c e va lves loca t ed a t t h e top of t h e core t h a t are i n t e g r a l
wi th t h e c o n t r o l rod d r i v e mechanisms. From t h e r e a c t o r c o r e , t h e coolan t
f lows through t h e steam gene ra to r s . A f t e r pass ing through t h e steam gene ra to r s ,
t h e helium i s r e tu rned t o t h e co re a t a temperature of about 760°F by fou r
steam-turbine-driven helium c i r c u l a t o r s . Two i d e n t i c a l loops are used , each
inc luding a six-module steam gene ra to r and two helium c i r c u l a t o r s . Each loop
c o n t r i b u t e s h a l f t h e t o t a l ou tput of t h e nuc lear steam supply system, which produces s t e a m a t 2400 p s i g and 1000°F wi th s i n g l e r ehea t t o 1000°F. The
helium c i r c u l a t o r s are d r iven by t h e exhaust steam from t h e high-pressure
tu rb ine . This steam i s then rehea ted and r e tu rned t o t h e intermediate-pres-
s u r e t u r b i n e . The c i r c u l a t o r s are a l s o equipped with a Pe l ton water wheel
d r i v e so t h a t they may be d r iven us ing t h e b o i l e r feed pumps f o r emergency
cond i t ions .
The gene ra l r e a c t o r arrangement can be seen i n F ig . 2 . The p res t r e s sed
concre te r e a c t o r v e s s e l (PCRV) i s 31 f t i n i n t e r n a l diameter with a 75-ft
i n t e r n a l h e i g h t . The upper and lower heads a re nominally 15 f t t h i c k , and
t h e w a l l s have a nominal t h i ckness of 9 f t . Thus t h e PCRV provides t h e dua l
func t ion of conta in ing t h e coolan t a t ope ra t ing p res su re and a l s o providing
r a d i o l o g i c a l s h i e l d i n g . The e x t e r i o r v e r t i c a l s u r f a c e of t h e v e s s e l may be
descr ibed as an hexagonal prism wi th v e r t i c a l p i l a s t e r s a t each co rne r . I t
i s 61 f t ac ross p i l a s l t e r s , 49 f t ac ross f l a t s , and 106 f t h igh .
The conc re t e w a l l s and heads of t h e PCRV are cons t ruc ted around a carbon-
s t e e l l i n e r which i s nominally 314 i n . t h i c k . The l i n e r i s anchored t o t h e
concre te and provides a hel ium-t ight membrane. A s y s t e m of water-cooled tubes
welded t o t h e concre te s i d e of t h e l i n e r provides a heat-removal s y s t e m t o
c o n t r o l concre te temperature . I n a d d i t i o n t o t h e coolan t t ubes , a thermal
b a r r i e r i s provided on t h e i n s i d e su r face of t h e l i n e r t o l i m i t t he flow of
hea t t o t h e l i n e r w a l l s .
95
The top head has r e f u e l i n g p e n e t r a t i o n s t h a t a l s o house t h e c o n t r o l rod
d r i v e s . It a l s o inco rpora t e s p e n e t r a t i o n s and w e l l s t o house t h e helium
p u r i f i c a t i o n system and neut ron d e t e c t i o n chambers. The bottom head has
pene t r a t ions f o r each of t h e steam-generator modules and helium c i r c u l a t o r s
p lus a l a r g e c e n t r a l opening f o r access t o t h e main c a v i t y .
All of t h e p e n e t r a t i o n s through t h e PCRV are provided wi th two indepen-
dent c l o s u r e s . The PCRV i n n e r c a v i t y and t h e primary c losu res serve as primary
containment f o r t h e r e a c t o r ; t h e massive PCRV and t h e secondary c losu res a c t
as t h e secondary containment.
The v e s s e l i s p r e s t r e s s e d t o p l ace t h e conc re t e s t r u c t u r e i n compression
p r i o r t o s e r v i c e . The p r e s t r e s s i n g system used is known as a l i n e a r tendon
pos t t ens ion ing system. During cons t ruc t ion , s teel tubes are embedded i n t h e
v e s s e l conc re t e f o r later i n s e r t i o n of t h e tendons, each of which c o n s i s t s of
up t o 170 1/4-in.-diameter "thermalized" w i r e s .
means of cold-deformed bu t ton heads t o a washer assembly t h a t t r a n s f e r s and
d i s t r i b u t e s t h e loads over s p l i t shims and a s teel bear ing p l a t e i n t o the
concre te . Three tendon arrangements are used: 90 l o n g i t u d i n a l ( v e r t i c a l )
tendons, 310 c i r cumfe ren t i a l tendons , and 48 crosshead tendons.
The w i r e s are anchored by
I n s i d e t h e PCRV i s t h e core suppor t f l o o r , a water-cooled s t r u c t u r e of s teel and r e in fo rced conc re t e 5 f t t h i c k . It is supported from t h e bottom
of t h e PCRV c a v i t y by 1 2 water-cooled s tee l columns. Twelve duc t s conduct
r e a c t o r - o u t l e t helium through t h e co re support f l o o r t o t h e 1 2 steam gene ra to r
modules loca t ed below.
CONSTRUCT I ON
One of t h e f i r s t t h ings done a f t e r moving onto t h e cons t ruc t ion s i t e
i n Apr i l of 1968 w a s t o pour a conc re t e pad ad jacen t t o t h e area where t h e
r e a c t o r bu i ld ing would be loca ted .
e r e c t i o n of t h e PCRV l i n e r bottom head and o t h e r l i n e r components, thus allow-
ing work t o be c a r r i e d ou t concurren t ly wi th t h e cons t ruc t ion of t h e r e a c t o r
This provided a working area f o r t h e
@
36
b u i l d i n g foundat ion and t h e support r i n g f o r t h e r e a c t o r v e s s e l . Figure 3
shows t h e l i n e r assembly area and t h e r e a c t o r bu i ld ing excavat ion. By
car ry ing ou t t h e PCRV l i n e r f a b r i c a t i o n concurren t ly with t h e c o n s t r u c t i o n
of t h e r e a c t o r b u i l d i n g foundat ion, t h e schedule w a s shortened s i g n i f i c a n t l y .
Concurrently w i t h t h e s e two o p e r a t i o n s a plywood mockup of a s e c t i o n of t h e
PCRV bottom head w a s cons t ruc ted f o r use i n t r a i n i n g t h e c o n s t r u c t i o n f o r c e
and t o h e l p i n planning f u t u r e opera t ions .
Construct ion of t h e r e a c t o r b u i l d i n g r e q u i r e d an excavation t o bedrock,
which w a s l o c a t e d some 50 t o 55 f t below ground leve l . The excavat ion w a s
t o be roughly 100 f t x 150 f t x 50 f t deep w i t h a d d i t i o n a l p e n e t r a t i o n i n t o
bedrock of 25 f t i n some areas. This excavat ion requi red t h e removal of about
30,000 cu yd of sand and g r a v e l t o expose t h e P i e r r e s h a l e bedrock and some-
what over 3,200 cu yd of s h a l e . Excavation work w a s complicated by the f a c t
t h a t t h e w a t e r t a b l e w a s a t a depth of 20 t o 25 f t i n sands having a high
t r a n s m i s s a b i l i t y and w a s f u r t h e r complicated by t h e c h a r a c t e r i s t i c of t h e
P i e r r e s h a l e t o decompose upon exposure t o a i r . For normal excavat ion of
t h i s type of sandy s o i l , s i d e s l o p e s would have had t o be a t l eas t 2-112 t o
1. This would have increased t h e yardage t o be excavated and would a l s o have
caused a l a r g e p o r t i o n of t h e area f o r t h e t u r b i n e b u i l d i n g t o be u n a v a i l a b l e
f o r work as long as t h e excavat ion w a s open.
Although s h e e t p i l i n g and convent ional w e l l p o i n t dewatering w a s considered,
t h e underground water flow w a s s o s t r o n g t h a t i t w a s ques t ionable whether t h i s
method could have s u c c e s s f u l l y kept t h e excavat ion dry. The ground f r e e z i n g
technique w a s s e l e c t e d as a b e t t e r method and because i t enabled n e a r l y ve r t i -
cal s i d e excavat ion and provided a w a l l capable of support ing heavy loads ,
t hus permi t t ing c l o s e access t o t h e work.
The freeze-wal l method of providing a cofferdam, shown i n Fig. 4 , i s
r e l a t i v e l y new i n t h i s country. For an oblong excavat ion such as For t S t .
Vrain, t h e w a l l , i n p lan view, is roughly an e l l i p s e . The th ickness of t h e
f rozen w a l l averaged about 6 f t a t t h e t o p , and a t rock e l e v a t i o n , about 8
f t . (Four l o c a t i o n s were d e l i b e r a t e l y thickened t o serve as crane p la t forms . )
97
To c o n s t r u c t t h i s w a l l , 180 U-tube p i p e assemblies c o n s i s t i n g of two
55-ft s e c t i o n s of 1-1/2-in. p ipe connected by a r e t u r n bend a t t h e bottom,
w e r e sunk i n t o t h e ground on t h e per imeter i n p r e d r i l l e d 4-in. h o l e s f i l l e d
wi th a b e n t o n i t e s l u r r y as a d r i l l i n g a i d . Ninety more assemblies were sunk
on t h e i n n e r pe r ime te r , and an a d d i t i o n a l 90 assemblies were used f o r c rane
pads and gan t ry t r a c k pads. All of t h e U-tubes were connected t o common
b r i n e supply and r e t u r n headers , which r a n from t h e r e f r i g e r a t i o n compressor
house near t h e n o r t h e a s t norner of t h e excavat ion . Af t e r t h e w a l l w a s f rozen ,
t h e b r i n e (wi th a f r e e z i n g po in t of -45°F) w a s cont inuous ly c i r c u l a t e d through
a l l of t h e p i p e s a t a supply temperature of -11°F and a r e t u r n temperature
of -6°F.
s ing le -cyc le ammonia compressors. Each r e f r i g e r a t i o n u n i t had i t s own cool ing
tower. I n t h e event of a power f a i l u r e , a standby d i e s e l gene ra to r of 625
kVA capac i ty w a s connected t o t h e system.
The r e f r i g e r a t i o n system cons i s t ed of two 85-ton and one 66-ton
Wall f r e e z i n g w a s s t a r t e d on May 6 , 1968, and by June 3 , 1968, most of
t h e w a l l w a s f rozen . I n o rde r t o exped i t e c l o s u r e i n some areas, a d d i t i o n a l
U-tubes w e r e i n s t a l l e d , and l i q u i d n i t r o g e n w a s in t roduced . I n o t h e r areas
t h a t proved d i f f i c u l t t o c l o s e , a d d i t i o n a l ho le s w e r e d r i l l e d and a c l ay
s l u r r y w a s in t roduced t o impede t h e flow and permit f r e e z i n g t o occur.
To p r o t e c t t h e sha le- type bedrock from d e t e r i o r a t i o n by exposure t o a i r , the shale had t o be covered w i t h conc re t e o r g u n i t e w i t h i n e i g h t hour s . It
w a s imposs ib le t o p r o t e c t t h e s h a l e and t o l i n e d r i l l and b l a s t s imul taneous ly .
A s a r e s u l t t h e s h a l e w a s excavated only t o rough l i m i t s , l e av ing about 9 t o
1 2 i n . of s h a l e i n p l ace . The s h a l e w a s t hen c u t back t o f i n i s h l i m i t s and
p ro tec t ed wi th g u n i t e on t h e v e r t i c a l s u r f a c e s and conc re t e on t h e h o r i z o n t a l
s u r f a c e s .
The excavat ion w a s completed i n t i m e t o permit t h e f i r s t permanent con-
crete t o be poured on September 18, 1968, fo l lowing t h e award of t h e cons t ruc-
t i o n permit on September 17 , 1968. The f reeze-wal l system remained i n ope ra t ion
u n t i l t h e r e a c t o r b u i l d i n g basement w a l l s were completed and b a c k f i l l e d t o
grade i n February 1969.
98
The suppor t r i n g f o r t h e PCRV, which i s a c y l i n d e r 50 f t i n o u t s i d e
diameter , 3 f t 6 i n . t h i c k , and 33 f t h igh , requi red 575 cu yd of concre te .
When a l l t h e s tee l w a s complete, t h e concre te w a s placed i n a continuous pour
over a per iod of 18 hours us ing Pumpcrete machines. The f i n a l seismic
des ign f o r t h e r i n g requi red a much l a r g e r q u a n t i t y of r e i n f o r c i n g s teel
( s e e F ig . 5) than w a s o r i g i n a l l y a n t i c i p a t e d . Because of t h i s , a 14-week
de lay occurred i n t h e completion of t h e r i n g , which took p lace on February
13, 1969.
Meanwhile, work on t h e bottom head assembly c o n s i s t i n g of t h e s teel
l i n e r , p e n e t r a t i o n s , and t h e co re suppor t f l o o r columns, which w a s s t a r t e d
i n June 1968, w a s completed, and t h e assembly w a s moved t o i t s permanent posi-
t i o n over t h e PCRV support r i n g i n February 1969. This assembly, which weighed
s o m e 400 tons inc lud ing a temporary e r e c t i o n j i g , s t ee l f o r m s f o r t h e b o t t o m
head, and some of t h e r e i n f o r c i n g s teel , w a s moved on r a i l s by a modified
t u r b i n e g e n e r a t o r s t a t o r l i f t i n g r i g and w a s lowered i n t o p l a c e on temporary
support s tee l e r e c t e d w i t h i n t h e support r i n g . F igure 6 shows t h e assembly
during t h e move.
The c o n s t r u c t i o n sequence r e q u i r e d t h a t t h e bottom head l i n e r p l a t e be
i n p l a c e p r i o r t o c o n c r e t e placement, i n o r d e r t o a s s u r e i n t i m a t e c o n t a c t
between t h e concre te and t h e unders ide of t h e bottom head l i n e r and penetra-
t i o n s . It w a s t h e r e f o r e decided t o u s e t h e Preplaced Aggregate Concrete
(PAC) technique i n t h e bottom head t o ensure s a t i s f a c t o r y q u a l i t y . A s t h e
name i m p l i e s , t h e PAC technique c o n s i s t s of p lac ing c l e a n coarse aggregate
i n t o t h e forms. The aggrega te i s placed i n l a y e r s t o avoid formation of
l a r g e v o i d s i n t h e aggrega te mass, and t o achieve i n t i m a t e contac t wi th a l l
embedments. Grout i s pumped under p r e s s u r e i n a continuous opera t ion through
previous ly embedded p i p e s t o f i l l t h e v o i d s e x i s t i n g i n t h e aggregate m a s s .
For t h e F o r t S t . Vrain PAC, t h e v o i d s amounted t o about 48 per cen t of t h e
aggregate volume.
A f u l l - s c a l e mockup of a s e c t i o n of t h e bottom head w a s made us ing PAC
t o i n v e s t i g a t e t h e concre te s t r e n g t h p r o p e r t i e s as w e l l as o t h e r v a r i a b l e s
of PAC and t o t es t t h e c a p a b i l i t y of PAC g r o u t pumping equipment, t h e capabi
99
of t h e b a t c h p l a n t t o mix t h e grout w i t h i n t h e s t r l n g e n t l imi - t a t ions of t h e
s p e c i f i c a t i o n s , and t h e c a p a b i l i t y of monitoring equipment t o be used f o r
grout l eve l i n d i c a t i o n , and t h e a b i l l t y t o p l a c e t h e PAC without v o i d s . The
r e s u l t s of t h e mockup were h i g h l y encouraging a r d provided information t h a t
w a s v a l u a b l e i n o p e r a t i o n a l planning f o r t h e PAC f o r t h e bottom head.
A f t e r a l l t h e bottom head embedments, inc luding tendon tubes and r e i n -
f c r c i n g s t ee l w e r e i n s t a l l e d (Fig. 7 ) , 1400 cu yd of 1-1/2-in. aggregate
w e r e p laced i n t o t h e bottom head forms. The aggregate w a s screened and washed
before being loaded on t r u c k s f o r d e l i v e r y t o t h e PCRV. A t t h e d e l i v e r y p o i n t ,
i t w a s aga in passed through a r o t a r y washer and discharged i n t o a holding
hopper. From t h e holding hopper t h e aggregate w a s placed i n t o p o s i t i o n by
hand (Fig. 8) .
Before t h e grout ing opera t ion w a s s t a r t e d , t h e aggrega te w a s cooled by
f l u s h i n g and p a r t l y f i l l i n g t h e forms with cold water and i c e .
i n g r e d i e n t s , sand, f l y a s h , cement, i n t r u s i o n a i d ( a combination of f l u i d i f i e r
and expansion a g e n t ) , w a t e r , and i ce w e r e batched and measured by weight 21%
by a Gulf General Atomic automatic concre te batching p l a n t , which i s loca ted
on t h e s i t e and provides a l l of t h e j o b concre te . The p l a n t i s r a t e d a t
100 cu y d l h r (with provis ions f o r h e a t i n g o r cool ing t h e concent r ic mix) and
i s capable of handl ing a l l requi red des ign mixes.
l a b o r a t o r y , which inc ludes a 600,000-lb Forney t e s t i n g machine, permits t e s t i n g
of a l l concre te and r e i n f o r c i n g s t ee l and inc ludes t h e c a p a b i l i t y of t e s t i n g
t o f a i l u r e a s i z e 18s b a r .
The grout
A well-equipped t e s t i n g
The ba tches w e r e loaded i n t o concre te t r a n s i t mixing t r u c k s t h a t premixed
t h e g r o u t .
a g i t a t o r u n i t s and 12 pumps, w a s e r e c t e d a t t h e PCRV s i t e . The mixer-agi ta tor
discharged t h e grout i n t o a common manifold t o which t h e 1 2 h o r i z o n t a l p i s t o n
pumps were connected.
a c t u a l l y i n u s e during t h e bottom head grout ing opera t ion , t h e remaining equip-
ment being on s tandby.
wi th cool ing c o i l s and i n s u l a t i o n t o maintain t h e grout a t 45" t 3°F.
A mixing and pumping p l a n t , c o n s i s t i n g of t h r e e s t a t i o n a r y mixer-
Only two of t h e mixer -ag i ta tors and e i g h t pumps w e r e
The mixer -ag i ta tors and t h e manifold were provided
P r i o r
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t o release of t h e g rou t from t h e mixe r -ag i t a to r s i n t o t h e manifold, t h e t e m -
p e r a t u r e and f l u i d i t y of t h e g r o u t were t e s t e d . Each pump served one i n s e r -
t i o n p o i n t a t a t i m e . The i n s e r t i o n p o i n t s were changed as t h e g rou t ing
ope ra t ion proceeded.
Grout flowed under pump p r e s s u r e through t h e g rou t p ipes i n t o t h e
aggrega te .
h o r i z o n t a l l a y e r s . The number and l o c a t i o n of t h e h o r i z o n t a l g rou t p i p e s
w e r e s u f f i c i e n t l y redundant t o provide f u l l and uniform grout coverage of
t h e PCRV bottom head.
Hor i zon ta l l-in.-diameter g r o u t p ipes w e r e placed i n several
Grout i n j e c t i o n s t a r t e d from t h e lowest p o i n t i n t h e form a t t h e cen te r
of t h e aggrega te mass. A s t h e g rou t ing o p e r a t i o n proceeded t h e g rou t t ubes
w e r e s lowly r e t r a c t e d t o produce an upward and outward g rou t f l o w from the
c e n t e r to t h e per iphery . The s l o p e of t h e advancing g rou t w a s such t h a t
entrapment of a i r w a s prevented, and displacement of l a i t a n c e and water
toward t h e ven t ing areas w a s achieved.
Shor t v e r t i c a l g rou t p i p e s w e r e employed f o r topping o f f a t t h e construc-
t i o n j o i n t . A s u r p l u s of g rou t w a s i n j e c t e d t o more than f i l l t h e aggregate
m a s s u n t i l overf low of und i lu t ed g rou t w a s observed a t t h e s u r f a c e of t h e
aggrega te . D i lu t ed g rou t w a s c o n t i n u a l l y broomed o f f t h e s u r f a c e . The grout-
i ng o p e r a t i o n took 5 4 hours and w a s completed on June 2 1 , 1969.
The u s e of sounding o r obse rva t ion w e l l s , which are u s u a l l y employed
f o r g rou t - l eve l d e t e c t i o n and c o n t r o l i n preplaced aggregate conc re t e work,
w a s n o t f e a s i b l e f o r t h e PAC i n t h e PCRV because of t h e requirement t h a t no
openings were allowed through t h e bottom l i n e r p l a t e .
f o r determining g rou t levels w a s t h e r e f o r e developed, u s ing t h e p r i n c i p l e of
t i m e domain r e f l ec tomet ry . The p r i n c i p l e i s based upon sending a f a s t - r i s e
p u l s e down a c a b l e and observing t h e amplitude c h a r a c t e r i s t i c s of t h e r e f l e c t e d
pu l se . A s t h e t r ansmi t t ed p u l s e encounters d i s c o n t i n u i t i e s i n t h e c a b l e ,
marked changes i n amplitude are d e t e c t e d . One of t h e cab le d i s c o n t i n u i t i e s
t h a t can be d e t e c t e d i s t h e p o i n t i n t h e cab le where t h e surrounding medium
changes from a i r t o water o r g r o u t .
An e l e c t r o n i c method
The s i g n a l w a s d isplayed on an o s c i l l o s c
101
There were 94 p a i r s of sensor w i r e s , each w i r e running t h e f u l l depth of
t h e aggrega te m a s s . The complete p r o f i l e of t h e g rou t a t any t i m e dur ing t h e
g rou t ing ope ra t ion could thus be observed and displayed i n a three-dimensional
p l a s t i c model. The continuous v i s u a l d i s p l a y i n t h e model of t h e g rou t l e v e l s
allowed a c o n t r o l l e d grout ing ope ra t ion . A f t e r completion of t h e g rou t ing
ope ra t ion , j u s t below where t h e i n i t i a l s e t of t h e g rou t w a s expected, t h e
w i r e mesh on t h e c o n s t r u c t i o n j o i n t s u r f a c e w a s removed i n p repa ra t ion f o r t h e
"green cu t t i ng ' ' o p e r a t i o n , which w a s s t a r t e d a f t e r t h e i n i t i a l s e t b u t p r i o r
t o a f u l l hardening of t h e g rou t . Green c u t t i n g removed t h e s u r f a c e g rou t
and exposed t h e aggregate without loosening o r breaking t h e aggregate p a r t i c l e s .
The c o n s t r u c t i o n j o i n t s u r f a c e w a s wet-cured t h e r e a f t e r .
The l a r g e mass of t h e bottom head PAC, approximately 1600 cu yd, r equ i r ed
c a r e f u l temperature c o n t r o l dur ing t h e hydra t ion phase. One hundred and f o r t y
thermocouples measured t h e conc re t e tempera tures . The cool ing system w a s de-
s igned t o ma in ta in conc re t e cu r ing temperatures below 130°F. The a c t u a l mea-
sured maximum temperature w a s 117°F. Cooling w a s provided by (1) c i r c u l a t i n g
r e f r i g e r a t e d water through 70 s e l e c t e d v e r t i c a l tendon tubes and through
supplemental p ipes ( 2 i n . d iameter ) embedded i n t h e c o n c r e t e , ( 2 ) c i r c u l a t i n g
r e f r i g e r a t e d water i n t o t h e bottom head l i n e r p e n e t r a t i o n s , and (3) maintaining
t h e ambient temperature of t h e s u r f a c e s t o about 60°F by a system of coo l water
sp rays and w e t bu r l ap . A 190-ton cool ing system provided t h e necessary r e f r i g - e r a t e d water . Postcool ing w a s commenced a t t h e completion of g rou t ing and w a s
terminated when t h e average conc re t e temperature w a s down t o 70" & 1 0 ° F .
The remainder of t h e conc re t e f o r t h e PCRV w a s convent ional ly mixed and
p laced . The conc re t e , which i s designed f o r a s t r e n g t h of 6000 p s i , con ta ins
aggregate t h a t i s c a r e f u l l y c o n t r o l l e d f o r g r a d a t i o n , f r i a b l e p a r t i c l e s , and
o rgan ic con ten t . The conc re t e temperature i s l i m i t e d t o 130°F dur ing cu r ing
t o minimize shr inkage and high-temperature-gradient c racks . An ex tens ive
i n s p e c t i o n and t e s t i n g program w a s developed f o r t h e vessel conc re t e t o ensure
compliance w i t h t h e s p e c i f i c a t i o n .
I n p r e p a r a t i o n f o r pouring t h e s i d e w a l l conc re t e l i f t s , t h e l i n e r b a r r e l
s e c t i o n s were completed i n t h e assembly area, moved i n t o t h e r e a c t o r b u i l d i n g
102
(F ig . 9 ) , and welded i n p l ace . Rebar, tendon tubes , and forms w e r e placed
f o r t h e 1 4 success ive l i f t s of about 5 f t each making up t h e PCRV s idewal l .
The f i r s t l i f t w a s poured on J u l y 17 , 1969, with t h e four teenth on January 7 ,
1970. I n t h e meantime, t h e top head l i n e r has been completed and i n s t a l l e d
(Fig. lo), and prepara t ions w e r e under way f o r t h e t h r e e l i f t s of t h e top head.
The f i r s t of t h e s e l i f t s w a s poured on January 30, and t h e f i n a l pour t o com-
p l e t e t h e PCRV w a s made on February 1 3 , one week ahead of schedule (F ig . 11 ) .
This i s p a r t i c u l a r l y impressive because i t inc ludes 1 4 weeks l o s t on t h e
schedule during t h e c o n s t r u c t i o n of t h e support r i n g . The t o t a l concrete
placed i n t h e PCRV i s about 6500 cu yd, inc luding t h e 1600-cu yd PAC i n t h e
bottom head.
The i n s t a l l a t i o n of t h e tendons w a s s t a r t e d i n October 1969. The tendons
are p a r t i a l l y f a b r i c a t e d when they a r e rece ived a t t h e s i t e . Af te r they are
pul led through t h e in-place tendon tubes , they are buttonheaded and then pre-
s t r e s s e d wi th 1000-ton j a c k s from both ends of curved tendons and one end of
t h e s t r a i g h t tendons (F ig . 1 2 ) . The f i r s t tendon w a s s t r e s s e d on January 16 ,
1970. A s of March 31, a l l 4 4 8 tendons i n t h e PCRV have been i n s t a l l e d , and
1 4 2 have been s t r e s s e d .
A s t h e concre te was being placed f o r t h e PCRV s i d e w a l l s and top head,
workers continued wi th t h e PCRV i n t e r n a l s . The i n t e r n a l s inc lude t h e l i n e r
i n s u l a t i o n , support columns f o r t h e co re support f l o o r , t h e co re support
f l o o r , and c o r e b a r r e l . S team g e n e r a t o r i n s t a l l a t i o n w a s s t a r t e d i n January
1970. This o p e r a t i o n w a s begun by i n s t a l l i n g t h e secondary modules, which
r e s i d e w i t h i n t h e p e n e t r a t i o n s i n t h e PCRV bottom head (F ig . 1 3 ) .
I n s t a l l a t i o n of t h e helium c i r c u l a t o r s and t h e f u e l t r a n s f e r machine
i s scheduled t o begin i n J u l y - August of t h i s yea r . The convent ional p a r t
of t h e p l a n t i s progress ing a t an e q u a l l y r a p i d pace and i s on schedule .
S ince moving onto t h e c o n s t r u c t i o n s i t e i n A p r i l 1968, over 50,000 cu yd
of e a r t h have been excavated, n e a r l y 38,000 cu yd of concre te have been poured,
and over 3,700 tons of s t ee l have been e r e c t e d o r i n s t a l l e d . A s of March 31,
1970, t h e c o n s t r u c t i o n i s es t imated t o be over 62% complete and on schedule .
F igure 1 4 i s a r e c e n t o v e r - a l l view of t h e c o n s t r u c t i o n s i t e .
Cons t ruc t ion i s on schedule f o r a completion d a t e of June 1971.
Fig. 1. Simplified flow diagram.
104
Fig . 2 . General arrangement of the primary reactor components.
F i g . 3 . V i e w of construct ion s i te showing l i n e r assembly area t o the l e f t of reactor bui ld ing excavat ion.
I 105
NOTE: Tvpical Only. A l l Fraaze Points Ara
Nat Shown
0 E X C A V A T I O N , ’ L I M I T S
c
Fig. 4 . Plan view of freeze-wall cofferdam.
Fig. 5. Top of support r i ng rebar s t r u c t u r e showing PCRV support hinge mounting corbels.
106
Fig. 6. PCRV bottom head assembly (approximately 400 tons) being moved to pos i t ion on temporary support s t e e l i n s ide the support r i ng (covered with p l a s t i c ) .
F ig . 7 . PCRV bottom head re inforc ing s t e e l and tendon tubes.
Fig . 8. S p e c i a l aggrega te be ing p rep laced i n t h e bottom head p r i o r t o t h e pumping of t h e g r o u t .
F ig . 9 . L i n e r s e c t i o n s two and t h r e e be ing lowered i n t o p o s i t i o n on t o p of t h e f i r s t l i n e r s e c t i o n . This double s e c t i o n is 34 f t h igh .
108
Fig. 10. PCRV l i n e r top head i n its permanent loca t ion p r i o r t o t h e pouring of the 14th and f i n a l s idewal l l i f t .
Fig. 11. Fina l concrete placement i n the PCRV top head
109
Fig. 12. 1000-ton jack in place for stressing a circumferential tendon
Fig. 13. One of the secondary steam generator modules being moved into position for installation in a bottom head penetration.
i?
Fig. 14 . Over-all view of c o n s t r u c t i o n s i t e showing switch-yard ( r i g h t foreground) , r e a c t o r b u i l d i n g - t u r b i n e bui ld ing ( c e n t e r ) , and main cool ing tower ( l e f t r e a r ) .
111
0 DISCUSS I ON
D. B. Trauger: Futuhe r e a c t o r s a r e of t he pod design which i s a
more complex conf igura t ion .
t i o n experience e x t r a p o l a t e t o t h e f u t u r e v e s s e l s , p a r t i c u l a r l y w i t h
placement of concrete and p r e s t r e s s i n g sequence?
c u l t o r e a s i e r ?
How does t h e For t S t . Vrain v e s s e l construc-
W i l l t hey be more d i f f i -
H. N. Wellhouser: We b e l i e v e t h e pod design i s s impler t o cons t ruc t .
The concrete placement experience
The concrete placement
There a r e many fewer tendons t o stress. gained w i t h F o r t S t . Vrain i s d i r e c t l y r e l a t e a b l e .
requirements f o r t h e 1100 Mwe v e s s e l should be cons iderably e a s i e r than
For t S t . Vrain because of t h e absence of c ross head and c i r cumfe ren t i a l
tendons.
G. Mei je r : Can you give the cons t ruc t ion time being es t imated f o r
t h e 1100 Mwe HTGR?
H. N. Wellhouser: Actual cons t ruc t ion t i m e for t h e nuc lear steam
supply system i s est imated t o be 37 months.
G. E. Locket t : I understood you t o say t h a t t h e maximum l i f t was about 190 tons and th i s was done by a 160 t o n crane.
e s t e d t o know how t h i s was achieved.
I should be i n t e r -
H. N. Wellhouser: I n t h e U.S . , crane manufacturers a l l o w f o r a 25%
overload provided t h e overload l i f t s a r e done inf’requently. I n t h i s case
w e worked c l o s e l y wi th t h e manufacturer so as not t o void t h e warranty.
M. Bender: I n t h e pas t , t h e r e have been claims t h a t concrete ves-
s e l s would shor t en the cons t ruc t ion schedule f o r a r e a c t o r p l a n t over
t h a t requi red wi th s teel v e s s e l s because of t h e d e l i v e r y per iod needed
f o r steel vesse l s . Could you comment on the v a l i d i t y of t h a t claim on
t h e b a s i s of Fo r t S t . Vrain exper ience? Could a concrete v e s s e l be con-
s t r u c t e d i n t h e equiva len t per iod of t i m e needed f o r a concrete contain-
ment v e s s e l ?
H. N. Wellhouser: It seems t h e cons t ruc t ion t ime f o r t h e PCRV i s
somewhat s h o r t e r than f o r v e s s e l s common t o water r e a c t o r s . With the
112
except ion of t he r e a c t o r i n t e r n a l s , the For t St . Vrain PCRV could be
completed and s t r e s s e d i n about 24 months.
B. G. Chapman: What techniques have been used f o r providing the
l e a k t i g h t n e s s o f t h e PCRV l i n e r ?
H. N. Wellhouser: A l l welds on the PCRV l i n e r a r e 106 radiographed
and helium l eak checked.
G. D. Whitman: What i s the s t a t u s of t h e p r e s t r e s s i n g ope ra t ion?
H. N. Wellhomer: A l l 448 tendons have been i n s t a l l e d and s t r e s s e d .
The las t tendons were stressed on A p r i l 24, 1970.
T. A. J aege r : H a s the des ign of t h e p re s t r e s sed concrete r e a c t o r
pressure v e s s e l been developed on the b a s i s of t h e convehtional s tandard
s p e c i f i c a t i o n s f o r p r e s t r e s s e d concrete o r d id you apply s p e c i f i c a l l y
developed des ign c r i t e r i a ?
Concerning the u t i l i z a t i o n of the ground breathing technique, I
would l i k e t o know whether a d e t a i l e d d e s c r i p t i o n of t h e experiences, es-
p e c i a l l y of t h e t roub le s experienced, i s a v a i l a b l e .
H. N. Wellhomer: Concrete s tandards were used where a p p l i c a b l e as
w a s ASME Sec t ion I11 nuclear code.
I don ' t know of any publ ished r e p o r t tha t covers t h i s work i n t h e
d e t a i l I th ink you a r e looking f o r .
Paper 2/120
THE RELATIONSHIP OF THE HTR WITH EARLIER GAS-COOLFD RFACTORS
C.S. Lowthian
ABSTRACT
Many of t h e p o t e n t i a l advantages of t h e HTR stem from t h e concept of p a r t i c l e f u e l and t h e use of helium as a cool- an t . It is t h e r e f o r e s i g n i f i c a n t l y d i f f e r e n t i n seve ra l a spec t s from t h e type of r e a c t o r a l ready developed i n t h e UK, but it is s t i l l b a s i c a l l y a gas-cooled r e a c t o r system. The design and opera t ing experience gained with t h e magnox r e a c t o r s and t h e AGR, even i f not immediately app l i cab le , i s d i r e c t l y re levant t o determining t h e type of problems l i k e l y t o be encountered and t o f i n d i n g t h e economic so lu t ions . This paper reviews t h e design, experimental and cons t ruc t ion- a1 experience of e a r l y gas-cooled r e a c t o r s which is app l i c - a b l e t o t h e HTR.
INTRODUC T I ON
A nuc lear power s t a t i o n i s a l a r g e and t e c h n i c a l l y complicated in-
vestment made wi th t h e s i n g l e objec t of producing e l e c t r i c i t y economically.
Innovations a r e requi red t o reduce both t h e c a p i t a l cos t and t h e running
cos t o f new power s t a t i o n s , but must not be introduced at t h e expense of
reliability. An investment will only pay for itself if a high l o a d fac-
t o r can be achieved.
continued r e l i a b i l i t y i s t o develop a family o f r e a c t o r s , each drawing
on t h e experience of i t s forbears .
One way of achieving successfu l innovat ion with
I n t h e UK t h e gas-cooled r e a c t o r has been developed over 20 years .
The i n i t i a l dec is ion t o adopt gas cool ing and g raph i t e moderation w a s taken f o r economic reasons r e l a t i n g t o t h e a v a i l a b i l i t y of d i f f u s i o n
p lan t and heavy water. The e a r l y magnox r e a c t o r s have now been operat-
i ng success fu l ly f o r a number of y e a r s with high load f a c t o r s and, des-
p i t e t h e i r high i n i t i a l c a p i t a l c o s t , have met t h e i r t a r g e t genera t ion
cos ts .
113
114
The High Temperature Reactor (HTR) i s t h e l a t e s t development i n
t h e design of gas-cooled r eac to r s .
ment and power s t a t i o n cons t ruc t ion a r e going ahead rap id ly .
UK t h e ex tens ive experience of t h e design and cons t ruc t ion of gas-
cooled r e a c t o r s is a v a i l a b l e t o t ake maximum advantage of t h e p o t e n t i a l
of t h e HTR. This paper reviews some of t h e r e l evan t experience and
i n d i c a t e s how t h e des ign i s be ing evolved.
I n t h e US and i n Germaqy develop-
In t h e
COOLANT GAS
General P r o p e r t i e s
The coolant gas is t h e heat t r a n s f e r and heat t r a n s p a t medium
wi th in t h e r e a c t o r system. The o v e r a l l p r o p e r t i e s of helium a r e l i t t l e
d i f f e r e n t from those of carbon dioxide i n t h i s r e spec t . The low dens i ty
is o f f s e t by t h e high s p e c i f i c heat so t h a t f l o w v e l o c i t i e s a r e not
g r e a t l y d i s s i m i l a r , while dynamic f o r c e s a r e decreased. I n l o c a l a r e a s
t h e p a r t i c u l a r p r o p e r t i e s of helium l e a d t o no t i ceab le d i f f e rences . For
example, t h e high thermal conduct iv i ty o f helium r e q u i r e s a th i ckness
of i n s u l a t i o n pack up t o t h r e e t imes t h a t i n carbon dioxide. I n gene ra l ,
however, because che p r o p e r t i e s a r e s o wel l known, t h e e f f e c t s can be
c a l c u l a t e d and t h e experience wi th carbon d ioxide can be r e a d i l y u t i l i s e d .
The chemical p r o p e r t i e s of helium a r e markedly d i f f e r e n t from those
of carbon d ioxide , t h e oxygen content of which has l e d t o cor ros ion
problems wi th l o w grade m i l d s t e e l s . Helium i s chemically i n e r t , f o r
p r a c t i c a l purposes, i n a r e a c t o r c i r c u i t , but t h e i n i t i a l experiences
at Dragon and Peach Bottom have suggested t h e increased importance of
t r a c e impur i t ies . The c i r c u i t gas w i l l have a hydrogen l e v e l o f t h e
order of 10 ppm, because of t h e chemical r educ t ion of water f rom minute
l e a k s from t h e b o i l e r s and from d i f f u s i o n of hydrogen through t h e b o i l e r
tubes.
I n t h e r e s u l t a n t reducing atmosphere t h e metal components o f t h e
c i r c u i t may l o s e t h e i r normal p r o t e c t i v e oxide l a y e r , l eav ing them open
t o a t t a c k from f u r t h e r impur i t i e s . I n p a r a l l e l , t h e su r face p r o p e r t i e s
of t h e m a t e r i a l s w i l l be d i f f e r e n t t o those i n an ox id i s ing atmosphere,
and f r i c t i o n and wear phenomena must be c a r e f u l l y inves t iga t ed .
115
Chemical Tropert i e s
A nuc lea r power s t a t i o n has t o be b u i l t n e c e s s a r i l y f o r at l e a s t a 20 y e a r l i f e . The s t r eng th , and p a r t i c u l a r l y t h e c reep performance, of
most common engineer ing m a t e r i a l s a r e known f o r such long opera t ing
per iods , o r can at l e a s t be conf ident ly predicted. The e f f e c t of t h e
environment wi th in a nuc lea r r e a c t o r is u n c e r t a i n however, so du r ing the.
e a r l y design per iod of t h e magnox r e a c t o r s ex tens ive experimental pro-
grammes were i n i t i a t e d . of p a r t i c u l a r i n t e r e s t w a s t h e chemical r e a c t i o n
between t h e coolant , carbon dioxide, and t h e ma te r i a l s of those compon-
e n t s i n t h e r eac to r , which because of r a d i a t i o n e f f e c t s could only be
r ep laced with g rea t d i f f i c u l t y .
0
There w a s a h o w n r e a c t i o n between t h e gas and t h e g raph i t e modera-
t o r , t h e r e a c t i o n r a t e be ing dependent on bo th t h e temperature and t h e
neutron f lux . This r e a c t i o n w a s i n v e s t i g a t e d u s i n g complex in-p i le rigs
and t h e design information produced has beery e n t i r e l y s a t i s f a c t o r y , as
shown by t h e successfu l opera t ion of t h e Calder r e a c t o r s f o r I 5 years .
The r e a c t i o n s wi th o the r m a t e r i a l s were a l s o i n v e s t i g a t e d and similar design information w a s produced. Unfortunately t h e e f f e c t o f break-away
cor ros ion i n low s i l i c o n semi-kil led s t e e l s was not f u l l y appreciated.
O f l i t t l e concern on open su r faces , it can produce s t r a i n s i n mechanically
r e s t r a i n e d assemblies and t h i s was not n o t i c e d u n t i l inspec t ion of t h e
Bradwell r e a c t o r s after they had been running success fu l ly f o r 6 years .
It has been found necessary f o r t h e t ime be ing t o reduce gas temperatures
at Bradwell, and a l l succeeding magnox s t a t i o n s , t o con t ro l t h e r a t e of ox ida t ion , and inev i t ab ly t h e output has been reduced. Nevertheless a load f a c t o r (based on guaranteed output ) of 82.3% w a s achieved at
Bradwell during 1969 d e s p i t e t h e r e s t r i c t i o n .
The research programme on s t e e l s has been increased s ince t h e d is -
covery of t h e s t r a i n phenomena, p a r t i c u l a r l y t o cover t h e higher pressure
and temperature condi t ions of t h e AGR.
much more use of s t a i n l e s s s t e e l s , which have a higher r e s i s t a n c e t o
oxidat ion and no d i f f i c u l t i e s a r e expected. Research i s cont inuing,
however, t o confirm e x i s t i n g r e s u l t s .
I n general t hese r e a c t o r s make
116
The chemical p r o p e r t i e s of helium a r e e n t i r e l y d i f f e r e n t t o those of
carbon dioxide, but similar research is i n v e s t i g a t i n g any cor ros ion
e f f e c t s of impur i t i e s c a r r i e d by t h e gas. A new phenomenon is t h e e f f e c t
of t h e r e a c t o r gas on t h e su r face p r o p e r t i e s o f ma te r i a l s , p a r t i c u l a r l y
t h e c o e f f i c i e n t o f f r i c t i o n . Table 1 g ives some t y p i c a l r e s u l t s of
dynamic f r i c t i o n c o e f f i c i e n t s measured i n pure helium.
Table 1. Dynamic F r i c t i o n Fac tors
Mater ia l C ornb i n a t ion
C r Carbide on s e l f
Graphit e on s e l f
316 Stain- l e s s s t e e l on s e l f
Helium Pressure
Atmospheres
1 50
1 50
1 50
Temperature C 0
800 800 800 800
6 50 6 50
Contact Pressure kg/cm2
65 65 65 65 21 21
F r i c t i o n f a c t o r min max mean
0.62 1.29 1.17 0.37 0.56 0.47
0.24 0.41 0.34
1.85 2.83 2.65 0.22 0.34 0.30
1.08 2.92 1.6
These r e s u l t s a r e very d i f f e r e n t f r o m t h e corresponding p r o p e r t i e s
i n a i r and show an i n t e r e s t i n g tendency f o r t h e c o e f f i c i e n t t o decrease
wi th i n c r e a s i n g gas pressure. The abso lu te l e v e l s a r e high however, and
emphasise t h e ca re which w i l l have t o be t aken i n ma te r i a l s e l ec t ion .
Vibra t ions and Noise
O f t h e order of 5% of t h e gross e l e c t r i c a l power produced i n a gas-
cooled nuc lear r e a c t o r s t a t i o n is used t o c i r c u l a t e t h e gas around t h e
system. There is t h e r e f o r e a cons iderable amount of energy i n t h e gas
stream which, i n t h e event of a v o r t e x shedding frequency co inc id ing with
a n a t u r a l frequency w i t h i n a contained volume, could cause s i g n i f i c a n t
mechanical damage. Several e f f e c t s such as t h i s have been r e p o r t e d
du r ing t h e h i s t o r y of gas-cooled r eac to r s ' and i l l u s t r a t e t h e growing
s o p h i s t i c a t i o n i n commissioning experimentat ion r e q u i r e d as gas pressures
and f l o w dynamic heads increased wi th r e a c t o r development.
A t Dungeness 'A' e a r l y d i f f i c u l t i e s were experienced during t h e
prel iminary commissioning t e s t s of a bypass c i r c u i t . This c i r c u i t , which
117
i s 60 f t long and 4 f t :diameter bypasses t h e c i r c u l a t o r o u t l e t gas back
t o a point mid-way along t h e l eng th of t h e b o i l e r s adjacent t o t h e evap-
o r a t o r bank of tubes and enables t h e c i r c u l a t o r s t o be run independently
of t h e main r e a c t o r gas c i r c u i t . During t h e c i r c u l a t o r commissioning it w a s found t h a t at speeds above a c r i t i c a l value t h e noise l e v e l and duct
v i b r a t i o n became i n t o l e r a b l e . The c i r c u i t w a s ins t rumentated w i t h s t r a i n
gauges, accelerometers and pressure t ransducers and t e s t s showed t h a t t h e
f requencies at which t h e duct w a s v i b r a t i n g were 133 Hz and 158 Hz. The
maximum s t r e s s l e v e l i n t h e duc t ing w a s measured at 780 lb/ in .2 peak-to-
peak; at 133 Hz t h e maximum a c c e l e r a t i o n recorded w a s 9 g and t h e maximum 2 gas pressure pu l sa t ion w a s 0.7 lb/ in . peak-t o-peak.
Af t e r cons5derable inves t iga t ion , which included measuring t h e pre-
dominant response f requencies of t h e duct , t h e phenomenon w a s t r a c e d t o resonance between an aerial v i b r a t i o n i n t h e duct and a vor t ex shedding
frequency from t h e t r a i l i n g edges of two cruciforms suppor t ing t h e tongue
of a duct bellows unit. The severe v i b r a t i o n s were e l imina ted by modify-
i n g t h e cruciform t r a i l i n g edges, when t h e maximum duct a c c e l e r a t i o n l e v e l
w a s reduced t o 0.64 g.
A similar and p o t e n t i a l l y more s e r i o u s resonance w a s found during
b o i l e r commissioning between an a e r i a l v i b r a t i o n i n t h e b o i l e r s h e l l and
pa r t of t h e a c t u a l tube assembly, i . e . t h e t o p rows of t h e superhea ter
and t h e support beam system. I n t h i s case it w a s not poss ib le t o modify
t h e i n i t i a t i n g member, s o an attempt w a s made t o f i t b a f f l e s wi th in t h e
b o i l e r s h e l l t o change t h e frequency of t h e a e r i a l v ib ra t ion .
Tests at s i t e became s o time-consuming and expensive t h a t it w a s decided t o adopt wind tunnel techniques t o f i n d t h e form of a s u i t a b l e
b a f f l e , wi th in t h e confines of t h e e x i s t i n g tube banks.
amount of modelling work w a s necessary before condi t ions i n t h e b o i l e r
could be reproduced, but eventua l ly seve ra l forms of s o l u t i o n were
evolved which, i n t h e wind tunnel , suppressed t h e resonance. Not a l l
of t hese s o l u t i o n s were successfu l i n t h e a c t u a l b o i l e r however, f o r
reasons which a r e n o t f u l l y understood, a l though it may have been e i t h e r
an over s i m p l i f i c a t i o n i n t h e modelling technique o r a d i f f e rence i n
A considerable
118
some unappreciated c r i t i c a l dimension between t h e model and t h e f i n a l
app l i ca t ion .
behind some of t h e tube banks w a s success fu l , however, i n reducing t h e
The f i n a l s o l u t i o n of f i t t i n g t r a n s v e r s e b a f f l e s immediately
maximum a l t e r n a t i n g s t r e s s measured on a tube t o -0.4 + t / i n . 2 , which i s s i g n i f i c a n t l y l e s s t h a n t h e f a t i g u e s t r e n g t h a s ses sed on t h e l i f e o f t h e
p l an t .
During t h e design s t a g e f o r Oldbury an a n a l y s i s w a s made of t h e
poss ib l e v i b r a t i o n s of t h e many components. Ca lcu la t ions showed t h a t t h e
b o i l e r s could be s u s c e p t i b l e t o e f f e c t s similar t o those found at Dungeness ' A ' , s o t h a t des ign w a s changed t o incorpora te a continuous
v e r t i c a l b a f f l e through t h e tube banks. As a precaut ion , commissioning
tes t s were c a r r i e d out first wi th co ld air at atmospheric pressure and
then wi th hot p r e s s u r i s e d air at a range of cond i t ions chosen t o g ive
t h e r equ i r ed son ic v e l o c i t i e s and gas dens i ty .
l e v e l w i th in t h e b o i l e r s was found t o be i n s i g n i f i c a n t , a l though a d i s c r e t e p re s su re pu l se w a s p resent throughout t h e e n t i r e c i r c u l a t o r
speed range at a frequency o f w i t h i n 5% of t h a t p red ic ted .
I n t h e event , t h e s t r e s s
Oldbury w a s indeed a very ' q u i e t ' r e a c t o r i n terms of v i b r a t i o n s
but dur ing t h e commissioning a new phenomenon r e l a t e d t o t h e n o i s e pro-
duced by t h e c i r c u l a t o r w a s found. This w a s a cons iderable amount of
sound energy appear ing at very l o w f r equenc ie s ( o f t h e order o f 50 Hz)
i n a r e a s very c l o s e t o t h e c i r c u l a t o r o u t l e t and r ep resen t ing , t h e r e f o r e ,
a p o t e n t i a l hazard t o t h e i n s u l a t i o n cover p l a t e s .
For t h e AGR design at Hinkley 'B' t h e design o f t h e cover p l a t e s
has been modified i n case similar e f f e c t s occur. The c i r c u l a t o r d r i v e
i s a cons tan t speed e l e c t r i c motor, and t h e impel lor and d i f f u s e r have
been d e s i d e d t o avoid a l l s i g n i f i c a n t t r a c e o f blade-passing frequency.
The pre l iminary t e s t s at atmospheric p re s su re have ind ica t ed low over-all
no i se l e v e l s , but a f u l l t e s t programme i s planned t o i n v e s t i g a t e t h e
f i n a l l e v e l s i n t h e r e a c t o r .
To complement t h e AGR commissioning t e s t s , ex t ens ive experimental
f a c i l i t i e s a r e be ing developed by TNPG.
check t h e p r e d i c t i o n s on no i se performance wi th helium c i r c u l a t o r s . No
These w i l l be used a l s o t o
119
@ immediate problems are apparent, for although the velocity of sound is
very much higher the acoustic impedance (sound velocity x density) is
little different to that of carton dioxide. Noise, as a general subject,
has only a limited theoretical basis however, especially in enclosures
where the dimensions are less than the wave-length of the sound waves,
and a considerable amourit of experimental work will be necessary.
CIRCUIT ENGINEERING
Def ini t ion
The term circuit engineering in a gas cooled reactor includes all
the plant which is necessary to translate the heat generated in the
reactor into steam to drive the turbo-generators, i.e. the reactor pres-
sure vessel and its associated liner, insulation and cooling equipment,
the boilers, and the gas circulators.
The pre-stressed IconcrGte pressure vessel is the basis of the cir-
cuit engineering of an integrated concept giving the designer freedom
in specifying vessel shape and gas pressure and yet always guaranteeing
reactor safety because of the massive redundancy in the number of stres-
sing cables. The cloncrete must be isolated from the high reactor gas
temperatures, however, and one of the major problems which has arisen is
the design and erection of the liner insulation.
Insulat ion
Metallic foil and wire mesh insulation and fibre insulation are the
two main types which have been used in the concrete pressure vessels
built in the UK.
for both types.
T"G have'been heavily involved in the development work
Metallic Foil and Wire Mesh Insulation
Feasibility studies to prove the integral concrete pressure vessel
concept for the Magnox reactors were completed by TNPG in 1960 and the
insulation of the vessel liner was then realised to be a major problem.
There was virtually no published information relevant to the thermal per-
formance of insulants in a high pressure gas environment and most conven-
tional insulants were excluded because of the compati bility requirements. @
120
Development work was therefore started by TNPG. Subsequently it
was learned that Darchem Ehgineering Ltd were working on lqwrallel lines
and from 1962 with the Oldbury tender awarded to TNPG, the two research and design teams worked together to develop what is now called metallic
foil and wire mesh insulation.
Oldbury reactor were insulated with 30 layers of 0.004 in. stain- less steel foil separated by a wire mesh (0.048 in. dia x 2 in. pitch), the whole pack being compressed by a mild steel cover plate in. thick
to a pack thickness of 2.00 in.
A s an example of this material the
Similar insulation has since been used for the Wylfa (Magnox) and
for Dungeness *B* (AGR) reactors. Considerable commissioning and opera-
tional experience has therefore been obtained in carbon dioxide at temp-
eratures up to 400 C and pressures up to 400 psia. The major problems
associated with surface pressure gradient effects have been fully
reported .
0
2 , 3
Fibre Insulation
With the completion of the Oldbury insulation, work on all aspects
of the AGR insulation was accelerated.
of the AGR were less severe than for Magnox reactors and a much wider
range of materials could therefore be used. Higher temperatures and
pressures (650 psia and 650°C for Hinkley *B*) had to be considered. TNPG decided to review the whole field in an attempt to develop an insul-
ant to meet the following specification:
The compat ibility requirements
(a) The required thermal performance under natural convect ion over
the full range of pressures and temperatures likely to be used
in AGRs and HTRs.
(b) A high resistance to surface pressure gradients.
(c) A low installed cost. This involves both low initial cost and a
relatively small site cost. Installation time was to be kept to
a minimum.
(d) The insulant must be capable of accommodating local irregularities
of the cold fade (reactor liner). A
121
(e) Isotropic properties. Insulants with highly anisotropic properties
cannot readily be used for penetrations and regions with complex
boundaries . A s a result of the review it was clear that a fibrous insulation had
many of the required properties and this type of insulation was eventually
chosen for Hinkley 'B' and Hunterston 'B'. The development work for both
these stations is being carried out in conjunction with the insulation
contractors, Delaney Gallay Ltd. A s an example, the insulation for the liner walls consists of layers of Triton Kaowool fibre compressed by a
7 in. thick stainless steel cover plate to 2 in. thickness overall. The
cover plate is mounted on a single bimetallic stud welded to the liner.
1
Thermal Performance
4,59697 In the last ten years work in England, France and elsewhere
has enabled an adequate understanding of the thermal performance of
insulants in a high pressure gas environment to be established. The bulk
of the experimental work has been carried out in high pressure carbon
dioxide but the limited work in helium is in fair agreement with the
correlations developed.
879
Metallic Foil and Wire Mesh - Natural Convection. - In any analysis of experimental data the convective contribution is first obtained by
deducting the metal conduction and radiation terms" from the measured
conductivity of the insulant. The convective contribution, which in
most realistic assemblies in carbon dioxide is the dominant contribution,
can then be correlated for a given insulant assembly against the pack
Rayleigh number (Fig 1 ). where
N = Nusselt number U
- heat out of cold face when gas movement occurs
N-- = Mean Nusselt number over cold face
- heat out of cold race under static gas conditions -
U C P fm 2 d 3 9 A T
4 R = Rayleigh number = a
P, k3 h lw\ For values of Ra above 100 convection within the insulation becomes
122
significant. Two lines are shown on Fig 1 which indicate the improvements
that are possible as a result of internal sealing features. The lower
line can be considered typical of the performance of well designed insula-
tion incorporating back lap seals2' 39 plane of the foils.
to reduce the permeability in the
A s a guide to thermal performance, complex flow pressure drop measure-
ments are carried out on representative insulation details. These measure-
ments have shown that foil and wire mesh is highly anisotropic; the perm- eability measured in the plane of the foils being between I O 4 and 10 5
times that measured normal to the foils.
The most successful theoretical model, developed by kvidson 4 , treats the whole pack as an anisotropic permeable solid.
Fibres and Granular Materials - Natural Convection. - For isotropic materials the Davidson theory is equally applicable6 and a comparison
between predicted and measured mean Nusselt number is given in Fig 2.
Data from are also included.
p y = Permeability in the vertical (y) direction
D = Pack thickness
H = Pack height
K = Thermal conductivity of a porous body with no overall gas movement through the body.
Otherwise the same notation has been used as defined on Fig 1.
The importance of one parameter which is normally overlooked,namely
the sealing characteristics of the hot face, is clearly demonstrated.
This correlation is equally applicable to HTR conditions where it should be possible to reduce the value of R a D/H to below the value for which
convection and hot face sealing effects are important.
Surface Pressure Gradient Wfects. - In gas cooled reactors it is
inevitable that the hot face of the insulation is exposed to surface
pressure gradients. The insulation must be capable of satisfactory
123
opera t ion when r a p i d pressure changes (due f o r example t o a change i n
r e a c t o r power) t ake place and t o achieve acceptab le pressure d i f f e r e n t i a l s
a c r o s s t h e hot f a c e it must be permeable. Surface pressure g r a d i e n t s can
t h e r e f o r e inf luence t h e pressure d i s t r i b u t i o n wi th in t h e in su lan t .
Davidson's theory has been extended t o cover t h i s case6 and t h e
inf luence of a uniform pressure grad ien t on t h e mean and l o c a l pack
Nusselt numbers is given on Fig 3 f o r t h e case of an open face. where
&)eo CP PA-. o2
F = = j t m 4 H = t h e constant p r e s s u r e > g r a d i e n t over t h e hot f a c e = v e r t i c a l d i s t ance measured from t h e high pressure region
( ' p 4 ) , , y
Otherwise t h e same n o t a t i o n has been used as def ined on F ig 1.
The theory has now been extended s o t h a t t h e inf luence of t h e hot face
s e a l i n g c h a r a c t e r i s t i c s can be inves t iga t ed . A considerable programme of
b a s i c experimental work is i n progress at " P G t o provide s u b s t a n t i a t i o n of t h i s theory. I n i t i a l r e s u l t s obtained on r e a c t o r prototype i n s u l a t i o n f o r
t h e f l o o r of Hinkley 'B' t e s t e d i n high pressure carbon dioxide a r e
encouraging.
Mechanical Design Aspects
I n both t h e f o i l and wire mesh and t h e f i b r e i n s u l a n t s developed f o r
t h e Oldbury and Hinkley 'B' r e a c t o r s t h e i n s u l a t i o n pack w a s he ld i n posi-
t i o n and p ro tec t ed by cover p l a t e s . D i f f e r e n t i a l expansion problems a r e severe and i n order t o rninimise s l i d i n g at supports s i n g l e s tud supports
a r e used i n both designs. Adequate space between t h e cover p l a t e when co ld
ensured t h a t t h e r e w a s no i n t e r a c t i o n between hot cover p l a t e s . However, s l i d i n g problems cannot be e l imina ted as t h e gaps between cover p l a t e s
must be br idged t o conta in o r p ro tec t t h e in su lan t . The cover p l a t e s pro-
v ide t h e in su lan t compressive loads and t h e f r i c t i o n a l f o r c e s between t h e s l i d i n g components a r e r e a c t e d by t h e s tud.
Liner Studs. - Studs a r e e i t h e r gun welded o r hand welded t o t h e l i ne r . The number, s i z e and ma te r i a l s a r e subjec t t o t h e fol lowing cons t r a in t s :
(a) Thermal
( i) Stud dens i ty as expressed by t h e t o t a l s t u d c ross -sec t iona l a r e a per
u n i t a r e a of l i n e r is r e s t r i c t e d by heat loading. I n t h e "I%
124
t h i s r e s t r i c t i o n is l e s s severe because of t h e r e l a t i v e l y high
conduct iv i ty of t h e b a s i c i n su lan t .
(ii) Single s t u d s i z e in f luences t h e maximum l i n e r temperature and
temperature grad ien ts . The in su lan t t h i c k n e s s is g r e a t e r i n t h e
HTR and l a r g e r s t u d diameters a r e t h e r e f o r e acceptable .
( i i i ) W e l d i n g problems a r e eased if a mild s t e e l s t u d is used. However,
thermal conduction and t h e hot f a c e temperature condi t ions r equ i r e
t h e use of s t a i n l e s s ma te r i a l s . Bi-metall ic s tuds have t h e r e f o r e
been used extensively.
( b ) Mechanical
( i v ) Pack compression f o r c e s r e s u l t i n t e n s i l e s tud loads. Also due
t o t h e non-uniformity of t h e pack t h e e f f e c t i v e cen t r e of t h e
pack loading is unlikely to coincide with t h e stud c e n t r e l i n e
and bending loads a r e t h e r e f o r e introduced.
( v ) Bending loads on t h e s tuds r e s u l t from t h e f r i c t i o n f o r c e s between
t h e s l i d i n g su r faces and a l s o from t h e weight of t h e cover p l a t e s
on v e r t i c a l sur faces .
( v i ) Qnamic loads a r i s e because t h e sound pressure l e v e l w i th in t h e
r e a c t o r can be high enough t o in t roduce v i b r a t i o n i n t h e i n s u l a t i o n
component s
Cover P la tes . - The dimensions o f t h e cover p l a t e s a r e inf luenced
by d e f l e c t i o n , s t u d loading and d i f f e r e n t i a l expansion problems. Edge
d e f l e c t i o n must be r e s t r i c t e d as t h e s e a l i n g e f f e c t i v e n e s s of t h e ma te r i a l
b r i d g i n g t h e cover p l a t e gaps is a f f ec t ed .
The acous t i c response of t h e cover p l a t e s can in t roduce random c y c l i c
p l a t e s t r e s s e s which w i l l e x i s t throughout r e a c t o r l i f e and cover p l a t e
s i z e , t h i c k n e s s and m a t e r i a l must c a t e r f o r t h e problem of f a t i g u e and
creep.
Fibre. - It is very important t h a t t h e f i b r e used t o r e s t r i c t t h e
gas movement should have adequate long term compression c h a r a c t e r i s t i c s
over t h e f u l l range of r e a c t o r temperatures. Compatibi l i ty and dust
content a r e a l s o important c o n s i d e r a t i o n s i n t h e choice of f i b r e .
i
125
Insulation for HTRs crs Theoretical and experimental work have enabled correlations to be
produced for both the natural and forced convection situations. Because
of the relatively low pack Rayleigh number, the thermal problems of the
insulants in a helium environment are eased and height effects and hot
face sealing characteristics are not so important.
Analytical procedures of the kvidson type may not be necessary for
HTR insulants. It is not difficult to design the insulation so that the
effects of convection are negligible but this does not necessarily result
in the most economic design. Consideration of the F parameter indicates
that the lower density and lower pressure gradients in the HTR (due to the
reduced gas circulation) are likely to reduce the effect of surface pres-
sure gradients relative to the AGR.
However, if after an overall cost assessment of the cooling system
and insulation designs the same conductance as used in the AGR is re-
quired then, because of the high thermal conductivity of the gas, packs
of two to three times the thichess of those used in the AGR are likely.
For higher temperature applications, fibres with a higher resilience
than Triton are required and a dust free fibre would be an advantage.
However, permeability requirements can be relaxed as a value of Ra D/H
(Fig 2) less than 2 can be easily achieved and a wide range of fibres
and fibre sizes can be considered for use in the HTR. A considerable programme of physical property measurements on fibrous materials has
therefore been initiated by TNPG.
Many of the mechanical problems investigated during the development
of the AGR insulation have direct relevance to the HTR insulation. Acous-
tic effects and stud heat loading are likely to be less severe but stic-
tion and sliding problems demand sophisticated studies. Ideally thermal
cycling and similar proving tests should be carried out in a helium
environment of the reactor purity.
Elsewhere special solutions are proposed (Fig 4), as some of the materials used to date would not be suitable. These problems are dis-
cussed in detail later under Basic HTR Design. 6d
126
PENETRATIONS
The i n t e g r a l b o i l e r concre te pressure v e s s e l must be pene t ra ted at v a r i o u s po in t s t o a l l o w t h e loading and discharge of f u e l , t h e i n s e r t i o n
of con t ro l rods, ins t rumenta t ion e t c .
arrangement i s proposed and t h i s g r e a t l y s i m p l i f i e s t h e water and
steam p e n e t r a t i o n problems.
For t h e HTR a podded b o i l e r
The major i n s u l a t i o n p e n e t r a t i o n problem involves t h e s tandpipes
( F i g 4) through which f u e l and con t ro l rods a r e passed.
t i o n s a r e very numerous and from t h e l i n e r coo l ing and thermal i n s u l a t i o n
a r e a Etignificant pa r t of t h e t o t a l problem.
These penetra-
Under normal opera t ion t h e s tandpipes conta in a plug and t h e l i n e r
However, t h e plug i s re- coo l ing and i n s u l a t i o n problem i s then s m a l l . moved p r i o r t o r e f u e l l i n g on load and each s tandpipe can t h e n be consid-
e r e d t o be a h igh aspect r a t i o i n s u l a t e d v e r t i c a l pipe z l w e d at t h e t o p
and open at t h e bottom t o an i n f i n i t e high pressure , high temperature
environment. It is t h e empty s t a t e which d i c t a t e s t h e design of t h e
i n s u l a t i o n and cool ing system.
TNPG have c a r r i e d out very ex tens ive i n v e s t i g a t i o n s of t h i s problem
and t h e inf luence of gas, gas pressure , gas temperature and e x t e r n a l
thermal r e s i s t a n c e has been measured f o r a range of pipe s i z e s inc luding
prototype Hinkley 'B' s tandpipes .
s tandpipe i n t e r n a l d e t a i l s on heat loading and temperature d i s t r i b u t i o n
has been covered. Tests on t h e Hinkley 'Bv s tandpipes us ing helium a r e
now i n progress and t e s t s on t h e much l a r g e r diameter s tandpipes pro-
posed f o r t h e HTR a r e be ing planned.
I n t h e l a t t e r case t h e inf luence of
Only r e s u l t s f o r t h e empty s tandpipe case with a high thermal re -
s i s t a n c e t o t h e heat s i n k w i l l be given i n k h i s paper.
Standpipe Tests
On F i g 5 t e s t r e s u l t s a r e given f o r two s tandpipes , one of which
was t e s t e d i n helium and carbon dioxide, t h e o the r i n carbon dioxide
only. 0 The maximum pressures and temperatures were 400 p s i g and 500 C.
The heat t r a n s f e r c o e f f i c i e n t i n t h e Nusselt number is obtained
127
@ from l o c a l gas and s tandpipe temperatures and heat f l u x e s and t h e mean
va lue over t h e height of t h e s tandpipe i s used. The v a r i a t i o n of l o c a l
Nusselt number with height w a s not large. - ' y- D = Nusselt number
R; = Rayleigh number L Cp pm2D39 A7
u k T = heat t r a n s f e r c o e f f i c i e n t between gas
and s tandpipe
b = standpipe bore
AT = temperature drop between gas and s tandpipe
T = mean abso lu te gas temperature
Otherwise t,he same n o t a t i o n as f o r F i g 1 w a s used.
Basic s t u d i e s have a l s o been conducted i n which f l o w v i sua l i&\ ion
techniques were used t o i n d i c a t e t h e n a t u r a l convection flows f o r t h i s
s i t u a t i o n .
work and a l s o by gas temperature measurements i n t h e high pressure gas
t e s t s suggest t h a t a complete unders tanding of t h e problem i s u n l i k e l y
at t h e present t ime.
The complexity and i n s t a b i l i t y of t h e f l o w ind ica t ed by t h i s
HTR Standpipes
Designs o f HTR s tandpipes d i f f e r i n two important and opposi te
F i r s t l y , i n order t o a l l o w t h e core f u e l r e s p e c t s from t h e AGR designs.
b r i c k s t o be removed a much l a r g e r diameter of s tandpipe is proposed.
Secondly, t h e use o f a downward flow core exposes t h e s tandpipe t o t h e
low temperature gas. Under present design condi t ions t h e n e t t e f f e c t of
t h e s e d i f f e rences i s t o reduce t h e Rayleigh number i n t h e HTR by at l e a s t
one order of magnitude r e l a t i v e t o t h e AGR.
The thermal loading problem of t h e HTR s tandpipe is t h e r e f o r e of
t h e same order as t h e AGR and it i s p a r t l y f o r t h i s reason that f u l l
s c a l e t e s t s a r e planned. An even more important reason, however, is that it i s e s s e n t i a 1 , t o know t h e temperatures of a l l t h e charge chute compon-
eats and t h i s can bes t be done by t e s t i n g prototgpes.
component temperatures due t o t h e downward f l o w core is very s i g n i f i c a n t .
The reduct ion of
C i r c u l a t o r s
I n t h e e a r l y magnox r e a c t o r s , which were housed i n s t e e l p ressure
128
v e s s e l s with ex te rna l duc ts t o t h e b o i l e r s , t h e gas c i r c u l a t o r s were
housed wi th in t h e ducts. They were dr iven by s h a f t s p e n e t r a t i n g t h e
pressure c i r c u i t through a gas s e a l . Many forms o f d r ive were used,
from steam tu rb ine t o e l e c t r i c motor with f l u i d coupling.
t h e first of t h e i n t e g r a t e d designs with t h e whole of t h e pressure c i r -
c u i t w i th in a s i n g l e v e s s e l , t h e concept w a s r e t a ined , with t h e c i r c u l a t o r
be ing dr iven by an extension s h a f t l o c a t e d i n a tunnel through t h e ves se l
w a l l . For Hinkley 'B' however, a new concept of encapsulated motor d r ive
was introduced, based on t h e success fu l ful ly-enclosed design pioneered
by Howdens at Winscale AGR, wi th t h e motor l o c a t e d wi th in t h e ves se l w a l l and opera t ing under f u l l r e a c t o r gas pressure, s o e l i m i n a t i n g t h e need f o r
a s h a f t s ea l .
A t Oldbury,
The design incorpora tes many of t h e d e s i r a b l e f e a t u r e s which have
been proved on e a r l i e r designs. F i r s t l y , t h e d r ive is a constant speed
e l e c t r i c motor, which has cons iderable advantages i n f l e x i b l e commission-
ing and i n providing emergency suppl ies . Var i a t ion of r e a c t o r mass f l o w
at Hinkley 'B' i s achieved us ing v a r i a b l e i n l e t guide vanes, an arrange-
ment which i s wel l proven i n conventional c i r c u l a t o r design, but which
of course remains t o be t e s t e d under r e a c t o r condi t ions.
motor and t h e impel lor form a s i n g l e compact u n i t which can be removed
r e l a t i v e l y quickly from se rv ice , and be r ep laced equal ly quickly a f t e r
maintenance and r epa i r .
Secondly, t h e
Although t h e r o t a t i n g s h a f t gas s e a l has been el iminated, t h e whole
of t h e s h a f t b e a r i n g assembly i s i n t h e gas c i r c u i t , and ex tens ive dev-
elopment work has been necessary t o design s e a l i n g arrangements f o r t h e
l u b r i c a t i o n o i l system. I n p a r a l l e l , much of t h e a n c i l l a r y equipment
i n t h e motor compartment, such as t h e water coolers f o r c o n t r o l l i n g t h e
l o c a l gas temperatures , have had t o be designed and manufactured t o a
very high s tandard t o ensure minimum contamination o f t h e r e a c t o r gas.
The f i r s t Hinkley 'B' c i r c u l a t o r i s now ready f o r prototype t e s t i n g
under s imulated r e a c t o r condi t ions before f i n a l i n s t a l l a t i o n . The form
o f design has been adopted f o r t h e o the r AGR s t a t i o n s now on order , and
r ep resen t s a s o l i d b a s i s f o r f u t u r e HTR designs.
129
Boilers c.$ The boilers in gas-cooled reactor stations are much more like gas to
water cross-flow heat exchangers in conventional coal or oil-fired boilers.
Throughout, there has been a compromise between the desire for large face
area, and so small gas-side pressure drops and dynamic forces, and the re-
quirements for fitting them into expensive pressure shells. Manufacturing
costs have influenced the compromise to a considerable extent.
Early designs were assemblies of straight tubes, tightly packed in
staggered or in-line banks, connected at each end by forged bends. Welding
costs were inevitably high, so methods have been developed for manipulation
of continuous lengths of tube to achieve the same low horizontal and vert-
ical pitching which is necessary in producing compact boilers.
In principle the inter-connections between tubes are relatively
straightforward because of the regular pitching and both welded and clamp-
ing designs have been used. Clamps have the particular advantage of pro-
viding damping of any tube vibration and worked well with low alloy steel
boilers;
tures have risen, galling problems have been encountered and T " G now
use welded connections. The lack of damping is allowed for in the ex-
tensive vibration survey now carried out during the design stage.
Relatively little trouble has been experienced by TNPG w i t h
as higher alloy material has been introduced as gas tempera-
nuclear boilers, but occasional tube failures have, of course, been
experienced. In general, they have become apparent early in the life
of the station, and can often be traced to individual defective welds.
The tubes are blanked-off external to the reactor vessel and, while
this means a small loss of heat transfer surface, no measurable opera-
tional penalty has been experienced. The siting of the boilers within
the reactor pressure vessel, as at Oldbury or Hinkley 'B', inevitably
raises the question of what can be done in the event of massive tube
failure because of a systematic design fault.
occurring is extremely small as gas temperatures are rigorously con-
trolled at a low level (relative to those in fossil-fired boilers) and
it is now general practice to install full-flow treatment plant for the
The probability of this
130
b o i l e r feedwater.
however, so t h e b o i l e r s a r e p r o t e c t e d from d i r e c t r a d i a t i o n from t h e
core by a shield-wall. The c a l c u l a t e d a c t i v a t i o n is such t h a t access
f o r inspec t ion w i l l be a v a i l a b l e throughout t h e l i f e of t h e p lan t . If
massive f a i l u r e i s d e t e c t e d t h e n t h e b o i l e r s could be r ep laced under an
extreme emergency procedure which would involve a major breach of t h e
vesse l . This would t ake a cons iderable t ime, but not longer than t h a t
r e q u i r e d t o d e s i g n and manufacture new b o i l e r s .
Experience wi th once-through b o i l e r s is l imi t ed ,
The ex ten t of t h e opera t ion is such t h a t it would only be t a c k l e d
under extreme condi t ions. The main emphasis i n t h e design i s placed
not on removeabi l i ty but on i n v e s t i g a t i n g and t e s t i n g e x i s t i n g fo rms of
b o i l e r t o redrice t h e r i s k of a major systematic f a i l u r e t o an absolu te
minimum.
FUEL HANDLING
One of t h e e a r l i e s t dec i s ions i n t h e evolu t ion of gas-cooled
r e a c t o r s w a s t o design f o r on-load f u e l handling.
achieve a p lan t which could be operated at t h e h ighes t poss ib l e a v a i l a -
b i l i t y wi th planned outage f o r t h e r e a c t o r be ing wi th in t h a t necessary
f o r t h e turb ine .
t h e wish t o use t h e b e n e f i c i a l e f f e c t s on r e a c t i v i t y of t h e build-up of
plutonium and t h e r e l a t i v e l y low f u e l l i f e .
The objec t w a s t o
With magnox r e a c t o r s t h e d e c i s i o n w a s r e i n f o r c e d by
The r e s t r i c t i o n of n a t u r a l uranium as a f u e l p l aces a high premium
on core r e a c t i v i t y .
plutonium i n f u e l of low i r r a d i a t i o n can be used t o o f f s e t t h e low re-
a c t i v i t y of highly i r r a d i a t e d f u e l .
With a continuous r e - f u e l l i n g cycle t h e build-up of
There a r e over 3000 f u e l channels per r e a c t o r i n t h e first two s t a t i o n s at Berkeley and Bradwell and with an average f u e l dwell time
of f o u r yea r s , corresponding t o an i r r a d i a t i o n l i f e of 3000 MWD/te, t h e
annual r a t e of channel replacement approached 800. a v a i l a b i l i t y of off-load f u e l handl ing w a s , t he re fo re , considerable and
extremely expensive because of t h e very high cos t of f u e l i n t h e a l t e r -
n a t i v e f o s s i l - f u e l l e d s t a t i o n s .
The e f f e c t on r e a c t o r
With t h e i n t r o d u c t i o n of enr iched f u e l i n t o t h e AGR design t h e
131
benefits of on-load refuelling on fuel life were reduced, but equivalent
advantages soon became apparent. Because the reactivity of the reactor
is an average of the reactivities of the individual channels, the irra-
diations of which are uniformly distributed over the range new to fully
irradiated fuel, the overall reactivity is almost independent with time.
There is no need therefore to include an excess number of control rods
to control the inevitable high reactivity of the new fuel in a reactor
which is re-fuelled on a yearly off-load basis.
is the fact that all the replacement fuel is of an enrichment which is
known well in advance of it being required on site. If a station, for
any reason, runs only at a poor load factor, then the refuelling is ad-
justed by reducing the rate at which channels are changed. The level
of enrichment is also reduced compared to a fuel cycle with yearly re-
fuelling which reduces the fuel costs by $4/kW to $5/kW.
Of pmticular importance
The decision to adopt on-load refuelling was taken in full reali-
sation of the mechanical problem involved and the successful achievement
has not been without substantial difficulty. The basic problem on a
magnox reactor is to penetrate the reactor pressure vessel, locate a
channel some 50 feet away, and grab and remove a fully irradiated, deli- cately designed, fuel element. The handling mechanisms must operate in
high pressure carbon dioxide at a temperature of 400 C, replace the new
fuel precisely in the right position without damaging the fuel beneath
with any impact loads, then retract from the vessel leaving the pressure
vessel closure secure.
0
During the early fuel-handling trials difficulties were experien-
ced with the operation of some of the mechanisms because of distortions
due to the uneven rates of heating, while the fuel element grabs had a
very limited life. None of the reactor stations designed by TNPQ has ever suffered a loss of availability because of deviatioh from the
planned fuel cycle and the final success of the operations can be seen
from the history of the Berkeley and Bradwell stations during 1967 (lhbles 2 and 3).
132
Total number of channels refuelled in 1967 Total number of channels refuelled to 31/12/67 Deviation from programme on 31/12/67( channels) Maximum channel average fuel irradiation - MwD
Te
Table 2 Fuelling Performance at Berkeley during 1967
Reactor 1 Reactor 2
8 20 799 3518 3517 - 3 + 4 3555 3530
T o t a l number of channels refuelled in 1967
Total number of channels refuelled to 31/12/67
Maximum channel average fuel irradiation - MwD
Deviation from programme on 31 /I 2/67 ( channels)
Te
Table 3 Fuelling Performance at Bradwell during 1967
The performance during 1967 has been chosen to illustrate the re- fuelling rates which can be achieved after the initial difficulties have
been overcome. The very high rate on Reactor 1 at Bradwell is indeed
due to the final clearing up of a residual back-log from earlier years.
During these early years there were considerable difficulties at both
stations, but without detriment to the overall load factors (based on
guaranteed output) which are given in Table 4.
Table 4 Annual Percentage Load Factors
~~~ ~
The advantages of on-load refuelling will be as important for the
HTR as for the earlier gas-cooled reactors, The reactor is being spec-
ifically designed to achieve these advantages, for example by adopting
133
downward gas flow such that the refuelling equipment will operate at the
relatively low temperature of 300 C.
earlier designs in that the mechanisms must work in helium, and the fuel
element is heavier and must be loaded into free-standing columns. With the
experience already gained, however, there is every chance that the early
operational difficulties will be significantly less than those experienced
at Berkeley and Bradwell.
0 There are major differences from
THE BASIC "IT DESIGN
A sketch of the reactor section is given on Fig 4 and illustrates the main features of the design. The object of the design is to exploit
the natural advantages of the HTR - high ratings and gas temperatures - while taking full account of existing experience on gas-cooled reactors
in order to reduce risks and produce a reliable station.
The basis of the pressure circuit design is the pre-stressed concrete
pressure vessel, but in a new departure for TNPG the boilers are located in vertical pods in the vessel wall. The main reason for this is economy,
for the high gas temperatures have so reduced the boiler heat transfer
surface that we nu longer have to arrange the units in an annulus round
the core in order to get sufficient frontal area. The boilers are very
compact and fit into four of the eight available pods, the other four
being used for helium storage.
Many detail .designs of boiler are being investigated but the prefer-
red arrangement at the moment is very similar to that used for the AGR.
Alternative boiler designs are being investigated based on the principle
of helically coiled elements, which give a more compact overall unit.
They represent a marked change in manufacturing procedure, however, and
until much more experimental work has been done there are several tech-
nical unknowns. These are concerned with the variable pitch between the
tubes and thus the uncertainty of predicting heat transfer and vibration
characteristics, as well as the erection of the preferred welded tube-to-
tube connect ions.
The coolant gas flow is downwards through the reactor to avoid 0 0 having hot gas (750 C) anywhere near the standpipes in the top of the
134
A
v e s s e l , and t 6 enable on-load r e f u e l l i n g i n an ambient temperature of
30OoC. The s tandpipes a r e d i f f i c u l t t o i n s u l a t e i n themselves, and they
conta in t h e v i t a l con t ro l rod mechanisms which must at a l l t imes be pre-
vented f rom over-heat ing.
The o v e r a l l i n s u l a t i o n wi th in t h e ves se l has been divided i n t o two
Cooling f l o w s at 3OO0C have been designed s o q u i t e d i s t i n c t d iv is ions .
t h a t a l l t h e i n s u l a t i o n p r o t e c t i n g t h e v e s s e l l i n e r s e e s gas of a maximum temperature of 4OO0C.
similar t o t h a t used at Hinkley 'B' AGR, t a k i n g due allowance f o r t h e
helium atmosphere.
r e a c t o r i n l e t gas temperature constant during a l l normal running
sequences, t h i s i n s u l a t i o n w i l l experience a minimum of thermal cyc l ing
and can t h e r e f o r e be guaranteed f o r long l i f e .
This i n s u l a t i o n w i l l be designed i n a manner
A s t h e r e a c t o r con t ro l system tends t o keep t h e
The f u n c t i o n of t h e high temperature i n s u l a t i o n , which covers a
r e s t r i c t e d Pegion from t h e core o u t l e t t o t h e b o i l e r i n l e t , w i l l be
l i m i t e d as f a r as poss ib l e t o r e s t r i c t i n g t h e passage of heat from t h e
hot t o t h e c o l d gas streams r a t h e r t h a n t o maintain component tempera-
t u r e s .
and t h e r e f o r e s t a t i o n e f f i c i e n c y , and represent no hazard t o t h e s a f e t y
of t h e p l an t . It is hoped t o use s o l i d in su lan t s , because of doubts
about t h e r e s i l i e n c e o f f i b r e ma te r i a l s , at high temperatures. The
r e a c t o r core , f o r example, w i l l s t and on a f i r e b r i c k hear th .
Any breakdown w i l l r e s u l t only i n a l o s s of temperature p o t e n t i a l ,
The c i r c u l a t o r s a r e l o c a t e d i n p e n e t r a t i o n s through t h e t o p s l a b of
t h e ves se l above t h e b o i l e r pads.
l a r g e t o a l l o w t h e passage of a b o i l e r , during e r e c t i o n , and as a remote
p o s s i b i l i t y du r ing removal f o r replacement, t h e r e is s u f f i c i e n t space t o accommodate a l l t h e c i r c u l a t o r a u x i l i a r y se rv ices . The design of t h e
c i r c u l a t o r w i l l most probably f o l l o w t h a t be ing developed f o r t h e AGR,
but a l l of t h e assumptions i m p l i c i t i n t h a t design a r e be ing re-examined.
For example, it may prove p r e f e r a b l e t o go back t o a v a r i a b l e speed
e l e c t r i c d r ive if f r i c t i o n and wear experiments i n helium show any pot-
e n t i a l d i f f i c u l t i e s with an i n l e t guide-vane mechanism.
A s t h e s e p e n e t r a t i o n s a r e s u f f i c i e n t l y
The HTR i s s i g n i f i c a n t l y d i f f e r e n t from e a r l i e r gas-cooled r e a c t o r s
135
63 i n t h e use of p a r t i c l e f u e l and t h e helium coolant . Outside t h e
immediate environment o f t h e core , however, much of t h e engineer ing is
l i t t l e d i f f e r e n t i n cha rac t e r t o t h a t o f previous gas-cooled r eac to r s .
The experience gained on t h e s e r e a c t o r s is be ing used t o evolve an HTR
design with t h e same r e l i a b l e high load f a c t o r opera t ion t h a t has a l ready
been achieved at Berkeley and Bradwell. By t h e end of 1970 TNPG w i l l have
completed such a design f o r a 600 W(E) power s t a t i o n t o be i n opera t ion
i n 1975.
ACKNOWLJ3EEMENTS
The work descr ibed i n t h i s paper has been c a r r i e d out by many
people wi th in The Nuclear Power Group Ltd. The au thors acknowledge
t h e advice and a s s i s t a n c e given by t h e i r co l leagues and would a l s o thank t h e i r Di rec tors f o r permission t o publ i sh t h e information.
136
REFERENC E S
1. J. Derbyshire and R. Stead, Vibration problems in Nuclear Power Plant, Paper No 2, Symposium or$ High Pressure Gas as a Heat Transport Medium, I. Mech. E., Vol. 181, March 1?67. -
2. J.W. Hughes et al, Insulation design and development for the Oldbury vessels, Conference on Prestressed Concrete Pressure Vessels, 1.C .E. Paper No.60, March 1967
3. J. W. Hughes and C. O'Tallamhain, Metallic foil insulation, Research Report RI, p. 235, Symposium of High Pressure Gas as a Heat Transport Medium, I. Mech.E., Vo1.181, - March I967
4. J. Davidson, Heat transfer behaviour of metallic foil insulation in high pressure gas, Paper No 13, Symposium on High Pressure Gas as a Heat Transport Medium, I. Mech.E., Vo1.181, - March 1967
5. R. Grossin et al, Heat transfer by natural convection in a porous medium, Paper No - 27 Second Conference - November 1969
6. B.N. Furber and J. Davidson, The thermal performance of porous insulants in a high pressure gas environment, Paper No 28, Second Conference on Prestressed Concrete Reactor Vessels and their Thermal Insulation, Brussels 18-20th November 1969
7. G. Mordchelles Regnier et al, Quelques Recherches Rgcentes Effectuees en France sur 1'Isolation Thermique des RBacteurs Nucleaires, Paper SM 1-11/76, Proceedings of a Symposium on Advanced and High Temperature Gas Cooled Reactors, I.A.E.A., Julich, October 1968
8. P.G. Cowap and B.N. Furber, The performance of Stainless Steel Foil insulation in a helium atmosphere, D.P. Report $2, 1967
9. B.N. firber, Contribution to discussion, p. 744, Conference on Prestressed concrete pressure vessels, I.C.E. March 1967
IO. B.N. Furber and R. Broderick, The development of an apparatus to measure the normal emissivity of small plane samples in a controlled atmosphere, Paper l2,Bristol 'Convention, I.Mech.E., 1968
11. J.C. Grebetz, Compression and Permanent deformation characteristics of Fibrous insulation, Materials Research and Standards, Jan. 1970, p. 26-31 and 61-63
12. W. J. Green, Temperature distributions along thermally insulated enclosed vertical pipes containing a pressurised gas - to be pub1 is hed
. . . - . . -
137
NOT*IIOH
CI i S f E C l F l C HEAT OF G A S ( C 0 N S T . PRESSURE)
P m - G A S D E N S 1 1 1 A T 1.
p.= G A S V I S C O S I T Y A T 1.
L , - C A S C o N n u c r i v i r i AT r. 4 - M E A N GAS C A f T H I C K N E S S . i N U L I N E I O f GAS G A P S
1. - M E A N GAS T E Y I E I A T U R E A T - T E M P E R A T U R E D I F I E R E N C E A C R O S S P A C K
S P E C I M E N DETLlLS ND O F FOILS 1 0 10 I I P A C K T H I C K N E S S I . 4 0 T O 1 . 2 1 I N . X 0 A W I T H I H T E R N A L S E A L I N G F E A T U R E S 0 V W I T H N O I N T E R N A L S E A L I N G F E A T U R E S
M A X PRESSURE 5 1 0 . t i .
M A X T E M P E R A T U R E b I O ‘C
rfsr CONDITIONS ( C A R N O N DIOXIDE)
t P A C K V T E S T E D I N H E L l U I l
1 I I 1 I I l l 1 I 1 3 4 5
I 0’ lol 2 3 4 5 ,ol 2 3 4 5
1. Foi l and Wire Insulat ion - Variation of i”, with Ra - Natural Convection.
2. I so t ropic Insulat ion - Variation of with R D,” - Natural Convection.
138
F H/y 10
2 3 I O I O I . -
I S H O W E V E R SMALL
I I O I OL F
IO '
I s o t r o p i c I n s u l a t i o n - Local and Mean Nusse l t Number - Forced Convect ion.
I CORE 5 CHARGE MACHINE 1 CORE SUPPORT 6 CHARGE MACHINE C H U T f 3 CIRCULATOR 7 CONCRETE PRESSURE VESSEL 4 BOILER 8 STANDPIPE
4. . Reactor E l e v a t i o n - HTR.
n
MEAN RAYLEICH NUMBER R o
5. S t a n d p i p e s - V a r i a t i o n of N w i t h R . u a
140
DISCUSSION
G. Meijer : Is your evapora t ion i n t h e steam genera tor downhill or
u p h i l l ?
Do you p lan t o do any tes t f o r downhill evapora t ion?
B. N. Furber: The flow i n the b o i l i n g s e c t i o n i n t h e TNPG design i s
u p h i l l .
Tests are i n progress t o i n v e s t i g a t e t h e heat t r a n s f e r and s t a b i l i t y
a spec t s . It may a l s o be of i n t e r e s t t o r e p o r t that Professor W. B. Hall (Manchester Un ive r s i ty ) is i n v e s t i g a t i n g s u p e r c r i t i c a l bo i l i ng . Resul t s
t o da t e sugges t t h a t downhill s u p e r c r i t i c a l b o i l i n g i s more c o n s i s t e n t t han
u p h i l l s u p e r c r i t i c a l b o i l i n g .
M. Dal le Donne: You mentioned t h a t t h e Nusselt number a t t h e i n s u l a -
t i o n and a t the s tandpipe i s about 10 t i m e s lower w i t h helium than w i t h
C 0 2 .
tha t of C 0 2 , s o t h a t t h e hea t t r a n s f e r c o e f f i c i e n t i s about t h e same and
t h e h e a t l o s s e s through t h e i n s u l a t i o n a r e about t h e same.
I n r e a l i t y t h e thermal conduc t iv i ty of helium i s 7 times h igher than
B. N. Furber: The r educ t ion of Raleigh number by a f a c t o r of 10
I n t h i s des ign a a p p l i e s approximately t o t h e TNPG s tandpipe design.
l a r g e s tandpipe diameter i s requi red t o enable f u e l b r i c k s t o be changed.
Assuming t h i s f a c t o r of 10, then t h e Nussel t number i s reduced by approxi-
mately 2.5. This does not compensate f o r t h e increased thermal conduc-
t i v i t y of helium. Nevertheless , t he main po in t i s that t h e increased hea t
t r a n s f e r c o e f f i c i e n t i n t h e TNFG s tandpipe des ign can be accommodated.
R. Huddle: What m a t e r i a l s do you in tend t o use f o r t h e hot f ac ings
of duc ts and l i n e r s ? Do you th ink t h e r e i s a material problem?
B. N. Furber: I n t h e low temperature regions t h e ho t f ace materials w i l l be similar t o those used i n the HTR. I n t h e high temperature reg ions
ceramic materials ( f o r example, s i l i c o n n i t r i d e ) a r e be ing s e r i o u s l y con-
s ide red .
M. Bender: The HTGR r e a c t o r s of t h e Dragon type opera te a t tempera-
t u r e s t h a t may be s e v e r a l hundred degrees above those of t h e AGR type.
141
0 Could you i n d i c a t e w h a t e f f e c t t h e s e e l eva ted temperatures would have on
t h e i n s u l a t i o n requirements and c h a r a c t e r i s t i c s .
Many people do not r e a l i z e t h a t concrete v e s s e l s are usua l ly designed s o
that coolant gas ad jacen t t o t h e concre te i s a t r e a c t o r i n l e t temperatures
and t h e i n s u l a t i o n performance i s t h e r e f o r e not very s e n s i t i v e t o core
o u t l e t temperature condi t ions . Nevertheless , t h e r e i s some inc rease i n
coolan t temperatures over t hose i n t h e AGR systems, and my impression i s
that t h e s e do t a x t h e c a p a b i l i t y o f r e f l e c t i v e i n s u l a t i o n s because the
seals between i n s u l a t i o n panels are d i f f i c u l t t o hold t o low leakage
l e v e l s . This i s t h e main reason why f i b e r i n s u l a t i o n s have become a t t r a c -
t i v e . The speaker ev iden t ly d i d no t understand t h e ques t ion and it d i d
not seem worthwhile t o -be labor t h e po in t .
(Supplementary note :
M.B. )
B. N. Furber: There i s no b a s i c thermal problem r e s u l t i n g from t he
h igher gas temperatures of t h e inc rease of thermal conduct iv i ty i f tempera-
t u r e i s not l i n e a r . The des ign conductance results from a s tudy and it i s probable tha t i n s u l a t i o n th i ckness could be 4 t o 6 i n . o r 2 t o 3 t i m e s
A. G. R.
143
HTGR N E W AND ADVANCED DESIGNS
(Session 111)
Chairman : J. D. Thorn, U n i t e d Kingdom Atomic E n e r g y A u t h o r i t y R i s l e y , W a r r i n g t o n , LanCS.
Co-Chairman: G. D. Whitman, Oak Ridge N a t i o n a l L a b o r a t o r y
144
Paper 1/101
THE H I CH,,TE~-EE-VJTURE REACT-OR.,DE-S?E LOP.EEuT . I N .&E RMANX- (PRESENT SITUATION, PROCRAM AND FUTURE ROLE)
ABSTRACT
Although HTR-development i n t h e German F e d e r a l Repub l i c i s b e i n g s u p p o r t e d by t h e government t o abou t t h e same e x t e n t as f a s t - b r e e d e r deve lopment , ana about one thousand m i l l i o n DM w i l l be s p e n t by 1 9 7 5 a c c o r d i n g t o t h e p r e s e n t p l a n s , t h e u t i l i t i e s c o n t i n u e t o show r e l a t i v e l y l i t t l e i n t e r e s t i n t h e HTR system.
N e w developments , however, e s p e c i a l l y i n t h e f i e l d o f r e a c t o r s a f e t y and p o l l u t i o n i n d i c a t e a poten- t i a l l y broad f u t u r e marke t f o r t h e HTR a l o n g s i d e LWR’s, as w e l l as f o r o t h e r r e a c t o r t y p e s n o t d i r e c t - l y i n v o l v e d i n t h i s development program. These market chances are coupled w i t h t h e s p e c i f i c c h a r a c t e r i s t i c s of t h e HTR-system, namely; f a v o u r a b l e economy, h i g h i n h e r e n t s a f e t y , a v e r y much b e t t e r f u e l u t i l i z a t i o n , and less c o o l a n t water demand t h a n f o r t h e LWR’s. Some o f t h e s e c h a r a c t e r i s t i c s w i l l become g r e a t l y i m p o r t a n t i n t h e F e d e r a l Repub l i c of Germany because of t h e r e s t r i c t e d number o f s i t e s w i t h s u f f i c i e n t f r e s h water c o o l i n g and because t h e h i g h p o p u l a t i o n d e n s i t y means t h a t s i tes v e r y n e a r t o c i t i e s must be t a k e n i n t o c b n s i d e r a t i o n more and m o r e .
I
With t h e r e a l i z a t i o n of t h e f i r s t l a r g e HTR-plant i n t h e F e d e r a l Repub l i c o f Germany, t h e HTR development w i l l e n t e r t h e d e c i s i v e phase i n t h i s c o u n t r y . T h e f i n a l d e c i s i o n f o r t h i s p l a n t , t h e 300 MWe THTR, i s e x p e c t e d by t h e midd le o f May 1 9 7 0 . Of g r e a t impor t ance a l s o i s t h e fo r thcoming a s s o c i a t i o n of t h e f i r m s GHH, KRUPP, and BBC.
The work on t h e HTR i s p r o c e e d i n g i n t h r e e s t e p s . During t h e f i r s t s t e p , work w a s c o n c e n t r a t e d on two c y c l e s p l a n t s . T h i s i n i t i a l development work, now e s s e n t i a l l y comple ted , was d i r e c t e d towards t h e con- s t r u c t i o n of t h e AVR-reactor and t h e d e s i g n o f t h e THTR. During t h e c o n s t r u c t i o n phase f o r t h e THTR, f u r t h e r component and f u e l e lement t es t s w i l l be made w i t h i n t h e framework of a s p e c i f i c i n d u s t r i a l d e v e l - opment program.
145
146
I n t h e second s t e p , t h e c o u p l i n g o f t h e HTR i n c l o s e d c y c l e d i r e c t l y t o a he l ium t u r b i n e w i l l be i n v e s t i - g a t e d . Such a development program h a s a l r e a d y s t a r t e d and w i l l be f i n i s h e d i n 1 9 7 4 w i t h t h e p r e p a r a t i o n o f t h e c o n s t r u c t i o n documents f o r a 600 MWe p l a n t . Some v e r y i m p o r t a n t p r o j e c t s w i t h i n t h i s program are:
1.
2 .
3 .
C o n s t r u c t i o n and o p e r a t i o n of t h e 2 2 MWe KWSH-plant. The commissioning of t h i s power p l a n t i s schedu led f o r 1 9 7 4 .
C o n s t r u c t i o n and o p e r a t i o n o f a f o s s i l f i r e d 5 0 MWe power p l a n t employing a he l ium t u r b i n e .
E s t a b l i s h i n g a m u l t i p u r p o s e t e s t f a c i l i t y which p a r t i c u l a r l y i n c l u d e s a t e s t s e c t i o n w i t h a he l ium t u r b i n e r e p r e s e n t a t i v e o f a 300 M W e p l a n t , w i t h which f u l l scale components of t h e pr imary c i r c u i t can be t e s t e d u n d e r r e a l i s t i c o p e r a t i n g c o n d i t i o n s .
T h i s development p r o g r a n i s e x p e c t e d t o r e a c h t h e s t a g e of commercial a p p l i c a t i o n by 1 9 8 0 .
During t h e t h i r d development s t e p , t h e d i r e c t u s e o f t h e r m a l e n e r g y from H T R ’ s f o r chemica l p r o c e s s e s w i l l be i n v e s t i g a t e d . Such p r o c e s s e s are t h e p r o d u c t i o n of hydrogen for u s e i n s t e e l manufac tu re by c r a c k i n g methane, heavy o i l or c o a l . Another a p p l i c a t i o n i s t h e p r o d u c t i o n o f r a w materials f o r t h e chemica l i n d u s t r y . T h i s work i s p r e s e n t l y i n t h e p r o j e c t d e f i n i t i o n phase . We assume t h a t i n 1 9 7 1 t h e development work can be s t a r t e d on f u l l scale.
The above mentioned a c t i v i t i e s w i l l b e s u p p o r t e d by a broad materials development program.
The p a p e r g i v e s a s h o r t r e p o r t on t h e p r e s e n t s t a t u s o f HTR development i n Germany. The main problems which are s t i l l open are p o i n t e d o u t and t h e p lanned a c t i v i - t i e s are mentioned.
147
I N T R O D U C T I O N
The p r imary and s t i l l most i m p o r t a n t g o a l of t h e p r e s e n t HTR development i s t o p r o v i d e t h e u t i l i t i e s w i t h an economic and safe n u c l e a r h e a t s o u r c e , which a l l o w s t o r e a l i z e a modern steam t u r b i n e p r o c e s s . We know t h a t t h e s a t u r a t e d steam t u r b i n e does n o t r e p r e s e n t a f i n a l s o l u t i o n , i n s p i t e o f t h e f ac t t h a t t h e y have been improved v e r y much i n t h e frame of t h e LWR development . On t h e o t h e r hand t h e i n v e s t i g a t i o n s of t h e l a s t f e w y e a r s have shown t h a t HTR h a s f u r t h e r development p o t e n t i a l beyond t h e r e a l i z a T i o n o f a modern steam c y c l e . T h i s p o t e n t i a l con- s i s l s f i r s t i n t h e u s e of t h e more p r o g r e s s i v e and i n p r i n c i p l e , more s i m p l e gas t u r b i n e p r o c e s s for e l e c t r i c i t y p r o d u c t i o n . Another p o t e n t i a l development i s t h e d i r e c t conve r s ion of n u c l e a r h e a t i n t o chemica l ene rgy i n form of a steam r e f o r m i n g p r o c e s s .
Th i s means, t h a t t o d a y w e have t o c o n s i d e r t h e HTR as a r e a c t o r f a m i l y more as a s i n g l e p l a n t t y p . The d i f f e r e n t v a r i a t i o n s o f f e r due t o t h e i r s p e c i f i c p r o p e r t i e s broad p o s s i b i l i t i e s o f a p p l i c a t i o n n o t o n l y on t h e e l e c t r i c a l ene rgy marke t b u t a l s o on t h e p r imary ene rgy marke t . T h i s p o t e n t i a l i s of g r e a t i m - p o r t a n c e because of t h e f ac t t h a t t h e p r imary ene rgy market t o d a y i s n e a r l y 4 t i m e s l a r g e r t h a n t h e marke t f o r e l e c t r i c a l e n e r g y t o which n u c l e a r ene rgy h a s t h u s f a r been l i m i t e d ex- c l u s i v e l y , and t h a t i n 30 y e a r s as F ig . 1 shows, it w i l l s t i l l be as l a r g e as t h e marke t f o r e l e c t r i c a l energy .
CHARACTERISTIC ITEMS OF THE GERMAN HTR-PROGRAM
Without any change i n t h e most u r g e n t t a s k , namely t o push t h e f i r s t HTR-concept ( w i t h steam t u r b i n e ) from t h e e x p e r i m e n t a l i n t o t h e commercial phase .
crs
148
I n West Germany development work f o r t h e more advanced con- c e p t w i t h d i r e c t c y c l e and f o r t h e i n d u s t r i a l p l a n t h a s a l - r e a d y been s t a r t ed of c o u r s e w i t h d i f f e r e n t p r i o r i t i e s and d i f f e r e n t ra tes .
The i n i t i a t i v e f o r t h i s r e s u l t s f rom t h e f o l l o w i n g r e a s o n s : I n West Germany t h e l i g h t water r e a c t o r h a s meanwhile e s t a b - l i s h e d v e r y s t r o n g i n d u s t r i a l s u p p o r t and h a s r e a c h e d a n as- t o n i s h i n g p o s i t i o n i n t h e e n e r g y marke t . I t has been e s t i - mated , f o r example , t h a t f o r t h i s y e a r a p p r o x i m a t e l y h a l f o f t h e new power p l a n t i n s t a l l a t i o n s w i l l b e s h a r e d by PWR and BWRs. Thus new economic c r i t e r i a have been e s t a b l i s h e d a g a i n s t which e a c h f u r t h e r n u c l e a r deve lopment i n West Germany must be matched. A g e n e r a l s u c c e s s f o r r e a c t o r companies s u p p o r t i n g t h e HTR for t h a t r e a s o n w i l l o n l y be a c h i e v e d i f extreme e f f o r t s are u n d e r t a k e n and i f t h e y are f o c u s s e d as soon as p o s s i b l e t o HTR c o n c e p t s w i t h t h e h i g h e s t economic p o t e n t i a l .
I may r e c a l l t h a t t h e H T R c o n c e p t h a s had i n West Germany r a t h e r modest s u p p o r t by t h e u t i l i t i e s u n t i l 1 r e c e n t l y . T h i s s i t u a t i o n i s c h a n g i n g s l o w l y now. One of t h e r e a s o n s are t h e growing s a f e t y r e q u i r e m e n t s f o r n u c l e a r p l a n t s i n h i g h dea- s i t y p o p u l a t e d areas s u c h as West Germany.
A f u r t h e r i m p o r t a n t r e a s o n i s g i v e n by t h e s i t u a t i o n f o r c o o l i n g water p r o v i s i o n i n West Germany. S e v e r a l a n a l y s e s i n d i c a t e a t e r m i n a t i o n of f r e s h water c o o l i n g i n f o r e s e e a b l e t i m e . I n LWRs t h e u s e of c o o l i n g towers l e a d s t o e s s e n t i a l l y h i g h e r c o s t p e n a l t i e s t h a n i n o t h e r c o n c e p t s and would c lear- l y a f f ec t t h e p o s i t i o n o f t h i s p l a n t t y p e i n i n d u s t r i a l c o m p e t i t i o n .
As f a r as w e know t o d a y H T R s w i t h h e l i u m t u r b i n e s h o u l d have t h e l a r g e s t p o t e n t i a l o f a l l n u c l e a r c o n c e p t s w i t h res-
-
149
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600
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23% / portion tor elcctrual energ- production
1 1 . 1950 1960 I970 )980 1990 m
F i g . 1 P r i m a r y Energy Demand i n West Germany u n t i l 2000
-I -- I hydrocraainrl_ r---------- I I I I H,S I I I I I
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1 react or 2 steam turbine cycle 3 heat exchanger 4 convertion CO+H.O+CXh + HI 5 C a -wash 6 methan separation 7 direct reduction 8 condensation: Ha0 9 H2 - compressor 10 hydrocracker 11 tube cracking furnace
CH, + HI 0 -CO+3H2 -49Kcallmol
u\ pldtr stctl
F i g . 2 Schemes for I n d u s t r i a l HTR-Plants
150
p e c t t o r e q u i r e m e n t s f o r c o o l i n g water. Even a i r c o o l i n g cou ld come i n t o c o n s i d e r a t i o n . A q u i c k l y and comple t e ly
e x h a u s t i n g t h e d i r e c t c y c l e sys tem a l r e a d y t o d a y shou ld t h e r e f o r e make t h e marke t ing of t h e HTR e s s e n t i a l l y easier .
t h e p o t e n t i a l o f t h e HTR concep t by developinR
The i n t e r e s t i n development work f o r t h e t h i r d g e n e r a t i o n o f H T R p l a n t s , i . e . i n d u s t r i a l complexes comes from i n d u s t r i a l groups o u t s i d e of t h e e l e c t r i c i t y i n d u s t r y whose economic and p o l i t i c a l i n f l u e n c e can have a s t r o n g impact on t h e whole HTR development . The r e a s o n f o r t h i s i n t e r e s t l i e s p a r t l y i n t h e hope o f m a i n t a i n i n n t h e b a s i s for t h e i r i n d u s t r i - a l e x i s t e n c e ( coa l ) p a r t l y i n t h e p r o s p e c t of b r o a d e n i n g t h e
market for t h e i r p r o d u c t s (brown c o a l , n a t u r a l g a s ) , and a l s o i n t h e p o s s i b i l i t y of u s i n g more new economic i n d u s t r i a l p r o c e s s e s ( s t e e l making, p r o d u c t i o n of chemical r a w materials e tc . 1.
I n F i g , 2 as examples two p r o c e s s e s are ahown which cou ld be
r e a l i z e d w i t h an HTR i n d u s t r i a l complex. The lower drawing shows a scheme for s t ee l manufac tu re : n a t u r a l g a s is c racked i n t o hydrcgen and carbon d i o x i d e i n a t u b e c r a c k i n g t u r n a c e a t 900'- 95OoC u s i n g n u c l e a r h e a t . The hydrogen i s p i p e d t h e n t o a p l a n t for d i r e c t r e d u c t i o n of i r o n o x i d e i n t o i r o n sponge t h a t w i l l be f u r t h e r c o n v e r t e d t o s t e e l i n a n e l e c t r i c arc. The n e c e s s a r y e l e c t r i c ene rgy for t h e a rc i s produced i n t h e same H T R p l a n t by a steam t u r b i n e d y c l e . The steam gene- r a t o r f o l l o w i n g t h e t u b e c r a c k i n g f u r n a c e i n t h e p r imary he l ium c i r c u i t .
S i m i l a r i n d u s t r i a l complexes are p o s s i b l e f o r making a c e t y l e n e , e t h y l e n e o r o t h e r r a w materials from n a t u r a l gas . I n s t e a d of n a t u r a l gas a l s o o i l or p o s s i b l e g o a l cou ld be used i n t h e s e p r o c e s s e s .
151
6d The upper drawing i n F ig . 2 shows a p o s s i b l e scheme f o r h y d r o c r a c k i n g of o i l t o g a s o l i n e .
HTR WITH STEAM T U R B I N E
F ig . 3 shows a s u r v e y of t h e t o t a l program of West Germany s u b d i v i d e d a l o n g t h e l i n e s of development a l r e a d y mentioned. The most i m p o r t a n t s o u r c e o f c o n s t r u c t i o n - and o p e r a t i o n e x p e r i e n c e f o r t h e t w o - c i r c u i t l i n e and s i m u l t a n e o u s l y t h e s t a r t i n g p o i n t f o r t h e o t h e r development l i n e s i s t h e 1 5 M W e e x p e r i m e n t a l power s t a t i o n AVR, t h a t a t t h e end o f 1 9 6 7 s t a r t e d power o p e r a t i o n and s i n c e t h e n h a s o p e r a t e d w i t h s a t i s f a c t o r y , r e s u l t s as d e s c r i b e d i n p a p e r 2/103.
On t h e b a s i s o f t h e main d e s i g n p r i n c f i p l e s of t h i s p l a n t d u r i n g t h e y e a r s 1 9 6 4 - 6 8 , t h e 300 MW THTR p l a n t h a s been developed by BBK and KFA i n a s s o c i a t i o n w i t h EURATOM.
More t h a n a y e a r ago BBK made a b i d t o H K G , a c o n s o r t i a of s e v e r a l u t i l i t i e s f o r t h i s THTR power p l a n t . The c o n t r a c t n e g o t i a t i o n s f o r t h e c o n s t r u c t i o n o f t h e p l a n t , i n t h e c o u r s e of which n o t i n c o n s i d e r a b l e d i f f i c u l t i e s a r o s e are i n t h e v e r y f i n a l s t a g e n o w . The l i c e n s i n g p r o c e d u r e h a s been r a n n i n g s i n c e
t h e b e g i n n i n g of t h i s y e a r and h a s p r e s e n t e d no a p p a r e n t d i f f i - c u l t i e s t h u s fa r .
I n t h e THTR p r o j e c t s p h e r i c a l f u e l e l e m e n t s c o n t a i n i n g uranium/ thor ium o x i d e w i l l be used i n an o n - l i n e r e f u e l l i n g scheme. The e l e m e n t s have become so w e l l deve loped i n t h e l as t y e a r s t h a t t h e s u p p l y i n g company, NUKEM, i s i n t h e p o s i t i o n t o d a y o f g i v i n g f a r - r e a c h i n g g u a r a n t e e s on t h e a c h i e v a b l e burn-up . I n p a r a l l e l t o t h e c o n s t r u c t i o n of t h e p l a n t a R and D-pro- gram w i l l be carried o u t , i n which a l l t h e main components
I . Generation H T R-ST
Construct +
152
E. Generation HTR-HT
Commercial p lonb
I//////' H T R - marerid and fue l development
1. Generation HTR-PH
+J definition
1
Fig. 3 Main a c t i v i t i e s Wi th in The HTR-Development Program
Tab le 1. T y p i c a l Datas of F i r s t - G e n e r a t i o n HTR P l a n t s
Electrical output (Generctor net power)
Gas temperature core in let core outlet
Gas-pressure (maximum
Power density in the core
Specific Burn-up
Type of Fuel
Diameter o f fuel kernel
Direction of gas flow in the core
Core-diameter
Core-heigh t
Prestressed Concrete PV
inner diameter inner height
Live-steam pressure temperature
MW
OC
OC
kg/cm 2
MW/m3
MWd/t U
CL
m
m
m m
2 k d c m OC
THTR
FR-Germany
307,5
250 750
40
6
115.000
uo2-Tho2
400
d o w n w a r d s
5,6
6
cylindrical
15,9 15,3
181 530
~
Fort St.Vrain
USA
330
404 776
49,l
6,3
100.000
uc2-Thc2
400
l o w n w a r d
4,7
6
cylindrical
9,45 22,8
169 538 I
Mark Ill
;reat Britain
640
300 800
56,25
6 3
6o.Ooo
uc2-Thc2
800
d o w n w a r d s
8,79
6 8
cy1 .with pods
9,5(core-part) 16 (core-part)
1 74 565 -_
n
153
w i l l b e t e s t e d i n d e t a i l . Among t h e s e components are t h e f u e l c h a r g i n g d e v i c e , t h e r e g u l a t i n g and shut-down r o d s , p a r t s of t h e g r a p h i t e s t r u c t u r e , the h o t g a s c a n a l between core and t h e steam b o i l e r s , t h e burn-up measurement p l a n t , t h e b o i l e r s and blowers.
G
A p a r t f rom t h e f u e l e l e m e n t s and t h e p e r t i n e n t f u e l c h a r g i n g d e v i c e t h e THTR shows as i s descr ibed i n more d e t a i l i n t h e
n e x t p a p e r (2/113) a wide - sp read agreement i n t h e d e s i g n w i t h c o r r e s p o n d i n g c o n c e p t s of t h e GCA and €hose o f t h e B r i t i s h companies ( see t a b l e 1). The t i m e s c h e d u l e f o r t h e f i r s t commerc ia l HTR p l a n t i n West Germany w i l l be f i x e d e x c l u s i v e l y by t h e r e s p o n s i b l e f i r m s B B C , BBK and GHH. Up t o now no b f f i c i a l s t a t e m e n t s have been d i v u l g e d . Q u i t e con- s i d e r a b l e e f f o r t s f o r f u r t h e r deve lopment on an p u r e l y i n - d u s t r i a l scale has y e t t o be done and i t i s c e r t a i n t h a t an order for t h e f i r s t commercial p l e n t i s n o t t o be e x p e c t e d before a t r u s t w o r t h y a p p r a i s a l on t h e v a l i d i t y of t h e c o s t c a l c u l a t i o n s f o r THTR have been made. The e a r l i e s t d a t e for t h i s seems t o be t w o y e a r s a f t e r t h e b e g i n n i n g o f the con- s t r u c t i o n p h a s e f o r t h e THTR, b u t p r o b a b l y an even l o n g e r p e r i o d w i l l b e n e c e s s a r y ,
I t i s a p p a r e n t t h a t t h e main e f f o r t s w i t h i n t h e s t e a m c y c l e l i n e t o r e a c h t h e commercial s t a g e i n West Germany are con- c e r n e d w i t h t h e c o n c e p t of s p h e r i c a l f u e l e l e m e n t s . However i n v e s t i g a t i o n s are b e i n g made a lso f o r reactor c o r e s w i t h b l o c k t y p e f u e l e l e m e n t s . The q u e s t i o n , which f u e l c o n c e p t w i l l have t h e l a r g e r l o n g t e r m p o t e n t i a l i n Germany i s q u i t e open , i t also depends on t h e f u r t h e r r e s u l t s o f t h e deve lop - ment f o r an HTK d i r e c t c y c l e p l a n t ( H H T ) which i s b e i n g p e r - formed f o r t h e t i m e b e i n g i n t w o p a r a l l e l l i n e s one f o r t h e b a l l and one f o r t h e b l o c k t y p e f u e l c o n c e p t .
I
I
154
A
HTR WITH HELIUM T U R B I N E ( H H T )
HT development work i s b a s e d on t h e f o l l o w i n g main p r o j e c t s .
1.) The e x p e r i m e n t a l p l a n t KWSH, a 2 2 MW n u c l e a r p l a n t w i t h h e l i u m t u r b i n e u s i n g a n o n - i n t e g r a t e d a r r angemen t and rod - shaped f u e l e l e m e n t s .
2 . ) A 50 M W e h e l i u m t u r b i n e p l a n t i n Oberhausen w i t h a f o s s i l f u e l f i r e d heater.
3 . ) A t es t s i t e w i t h 4 i n s t a l l a t i o n s which have been p l a n n e d i n s u c h a way t h a t t h e y supp lemen t e a c h o t h e r w i t h r e s p e c t t o magni tude and a v a i l a b i l i t y . A l though t h e e x p e r i m e n t a l p l a n t KWSH which h a s been o r d e r e d one y e a r ago s h o u l d f u r n i s h i m - p o r t a n t datas on t h e o p e r a t i o n a l b e h a v i o r o f a t y p i c a l d i r e c t c y c l e H T R p l a n t , i n p a r t i c u l a r on i t s r e g u l a t i n g and f a u l t b e h a v i o r , and a l t h o u g h it s h o u l d i n a d d i t i o n o f f e r t h e p o s s i - b i l i t y of t e s t i n g p r i s m a t i c f u e l e l e m e n t s , KWSH h a s come u n d e r d i s c u s s i o n a g a i n . T h i s d i s c u s s i o n i s s t i l l i n f u l l swing. F i n a l d e c i s i . o n s w i l l b e made o n l y i n c lose c o o r d i n a t i o n w i t h t h e s p e c i a l o b j e c t i v e s of t h e g e n e r a l HHT development .
I n t h e 5 0 MW p l a n t i n Oberhausen t h a t w i l l b e o r d e r e d by RWE and t h e c i t y o f Oberhausen w i t h i n t h i s y e a r w i l l o v e r t a k e t h e
f u n c t i o n of a d e m o n s t r a t i o n p l a n t . Q u e s t i o n s of t h e long- t ime b e h a v i o r , a v a i l a b i l i t y and m a i n t e n a n c e o f h e l i u m t u r b i n e s w i l l i n v e s t i g a t e d t h e r e . S i m u l t a n e o u s l y t h i s p l a n t o f f e r s t h e p o s s i - b i l i t y o f e v a l u a t i n g t h e t r a n s i e n t b e h a v i o r of t h e main compo- n e n t s i n t h e h e l i u m t u r b i n e c i r c u i t e x p e r i m e n t a l l y .
The d e s i g n of t h e d i f f e r e n t machines of t h e HHT t e s t s i t e and t h e i r s p e c i f i c t a s k s are d e s c r i b e d i n p a p e r 6/117. I s h o u l d s a y h e r e t h a t t h i s t e s t s i t e w i l l be t h e c e n t r a l p o i n t f o r e x t e n s i v e component work.
155
The main a c t i v i t i e s are d e a l i n g w i t h problems o f t h e t u r b i n e , ( t h e b e a r i n g , s e a l i n g and t h e r o t o r and b lade c o o l i n g : ) , and problems of t h e h o t g a s d u c t s between t h e r e a c t o r c o r e ou t - l e t and t h e t u r b i n e e n t r y ( i n s o l a t i o n , expans ion d e v i c e s , v a l v e s and f i t t i n g s ) .
crs
The mass f low for t h e d i f f e r e n t p l a n t s of t h e t e s t s i t e c o v e r s t h e r a n g e from 3 t o 250 k g / s e c . The t empepa tu res v a r y i n t h e r e g i o n from 400 t o 85OoC p r o b a b l y even 1000°C. T h e a v a i l a b l e diameter of t h e t e s t s e c t i o n s l i e s between 0 . 2 and 2 meters. I t i s b e i n g e s t a b l i s h e d a t KFA by t h e i n d u s t r i a l f i r m s BBC and GHH. These companies w i l l o p e r a t e a l s o t h e p l a n t t o g e t h e r w i t h KFA. F i r s t expe r imen t s can be s t a r t ed w i t h i n t h e n e x t f e w months, t h e comple t ion o f t h e whole t e s t s i t e w i l l n o t be ach ieved b e f o r e end of 1 9 7 2 .
Pa ra l l e l t o t h e c o n s t r u c t i o n and o p e r a t i o n o f t h e above men- t i o n e d i n s t a l l a t i o n s , t h e o r e t i c a l and e x p e r i m e n t a l i n v e s t i - g a t i o n s have been s t a r t ed i n meantime. These w i l l f o r t h e most p a r t be concerned w i t h two problem zreas , 1. d e f i n i n g t h e l ay -ou t o f t h e p l a n t and 2 . t h e p l a t e - o u t of f i s s i o n pro- d u c t s i n t h e t u r b i n e c i r c u i t , a knowledge which i s of d e c i - s i v e s i g n i f i c a n c e f o r t he e v a l u a t i o n of H T R d i r e c t cyc le power
p l a n t s .
The p o s s i b l e l a y - o u t s are s t i l l judged i n a r a t h e r d i f f e r e n t way from c o u n t r y t o c o u n t r y , as t h e mee t ing of t h e BNES i n London a g a i n showed j u s t r e c e n t l y , and are unde r much d i s - c u s s i o n . The q u e s t i o n o f t h e bes t d e s i g n i s n o t y e t d e c i d e d even i n s i d e i n d i v i d u a l working groups . Under d i s c u s s i o n are non-, h a l f - , and f u l l y i n t e g r a t e d c o n c e p t s . I n s i d e o u r working groups p r e s e n t l y a c i r c u i t o u s and d e t a i l e d e v a l u a t i o n scheme i s b e i n g set up t h a t can be a p p l i e d s y s t e m a t i c a l l y t o t h e d i f f e r e n t c o n c e p t s . F i n a l r e s u l t s can n o t be expec ted u n t i l
156
t h e end o f t h i s y e a r . P a r t i c u l a r d e t a i l s on it w i l l be p r e s e n t e d i n pape r No, 5 / 1 1 5 .
A s u r v e y o f t h e work p lanned f o r s t u d y i n g t h e b e h a v i o r o f f i s s i o n p r o d u c t s i n t h e c o o l i n g c i r c u i t i s g iven i n pape r No. 7 / 1 2 7 .
At. t h e c e n t r a l p o i n t of t h i s work i s an i n - p i l e expe r imen t t h a t w i l l be s t a r t e d i n t h e r e a c t o r PEGASE (Cadarache) i n t h e middle of t h i s y e a r and t h a t w i l l s i m u l a t e as w e l l as p o s s i b l e t h e o p e r a t i n g c o n d i t i o n s o f a o n e - c i r c u i t power p l a n t .
The knowledge from these i n v e s t i g a t i o n s as w e l l as t h a t worked o u t i n o t h e r a f o r e mentioned p r o j e c t s w i l l be u t i - l i z e d f o r t h e d e s i g n work o f a 600 M W e p l a n t whose uppe r he l ium gas t e m p e r a t u r e h a s a l r e a d y been e s t a b l i s h e d a t 85OoC. The comple t ion of t h e s e d e s i g n s i s expec ted by 1 9 7 4 . T h i s means t h a t t h e commissioning of t h e f i r s t l a r g e HHT p l a n t i n West Germany can n o t be e x p e c t e d b e f o r e t h e end of t h i s decade .
THE I N D U S T R I A L HTR - PLANTS
The development work f o r an i n d u s t r i a l p l a n t , t h e t h i r d g e n e r a t i o n o f H T R s , was s t a r t e d more t h a n one y e a r ago and h a s now reached t h e s t a t u s o f a p r o j e c t d e f i n i t i o n phase . We assume t h a t t h e p r o p e r development program can s t a r t a f t e r a p o s i t i v e c o n c l u s i o n of t h i s phase i n t h e c o u r s e of n e x t y e a r . T h i s program w i l l encompass t h e f o l l o w i n g a c t i v i t i e s : 1.) Exper imen ta l and t h e o r e t i c a l thermodynamic s t u d i e s i n c o n t e x t w i t h t h e d e s i g n work f o r a t u b e c r a c k i n g f u r n a c e , b e g i n n i n g a t a s i n g l e t u b e (10 m l o n g , 0 , l m d i a m e t e r ) Later a t a whole t u b e bundle .
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157
2.) Coal g a s i f i c a t i o n expe r imen t s u s i n g hydrogen a t 100 b a r s i n s e v e r a l i n s t a l l a t i o n s o f d i f f e r e n t s i z e . ( L a b o r a t o r y scale - 1 kg c o a l / h , - h a l f t e c h n i c a l scale - 50 kg c o a l / h , and f i n a l l y i n a p i l o t p l a n t o f 1 t o 2 t c o a l / h )
0
3. Expe r imen ta l i n v e s t i g a t i o n s t o t h e k i n e t i c s of r e a c t i o n s between coal and steam (steam r e f o r m i n g ) and a b o u t t h e r e a c t i v i t y of c o a l s hav ing d i f f e r e n t q u a l i t i e s .
4 . ) F u r t h e r development work for r e a c t o r components w i t h r e s p e c t t o r e a c h h i g h e r gas t e m p e r a t u r e s ( 9 5 O o C ) .
I n a d d i t i o n t o KFA, t h e companies Rhe in i sche Braunkohlewerke, Cologne, and Bergbauforschung Essen are i n v o l v e d i n t h e de-
velopment work d u r i n g t h e f i r s t phase.
HTR MATER I AL- AND FUEL ELEMENT DEVELOPMENT
The development work mentioned so f a r i s , as shown i n F ig . 3 , accompanied by a broad H T R - m a t e r i a l and f u e l e lement development program. T h i s program i n c l u d e s bas ic work on t h e u n d e r s t a n d i n g of t h e i r r a d i a t i o n b e h a v i o r o f a l l f u e l e lement components - ( p a r t l y i n c l o s e c o o p e r a t i o n w i t h DRAGON) , the
c o l l e c t i o n of material d a t a s t h a t are r e q u i r e d f o r t h e f u e l e l e m e n t s d e s i g n work, and t h e development o f manufac tu r ing t e c h n i q u e s f o r s p e c i f i c f u e l e lement components. A f u r t h e r i m p o r t a n t p o i n t o f t h i s program, which i s s u p p o r t e d by NUKEM and KFA, i s r e l a t e d t o t h e p r e p a r a t i o n , per formance and e v a l u a t i o n o f s p e c i f i c a t i o n t es t s f o r t h e THTR-, KWSH- and t h e HHT-project. S i n c e d e t a i l s o f t h i s program w i l l be r e p o r t e d i n p a p e r No. 7/128, t h e p a r t i c u l a r p o i n t s and t h e s p e c i a l problems can be d i s p e n s e d w i t h h e r e .
158
RE PRO CE S S IN G
I n orPder t o g i v e a comple t e p i c t u r e of HTR development i n West Germany, one must s t i l l t o u c h upon t h e i m p o r t a n t work i n t h e area o f r e p r o c e s s i n g ( g i v e n i n d e t a i l by Dr. Merz i n p a p e r No. 1 / 1 3 6 ) . T h i s work i n c l u d e s t h e head-end and t h e r e c o v e r y of f i s s i o n materials, t h e l a t t e r b e i n g r e l a t e d o n l y t o t h e uran ium-thor ium-cycle . Out of a g r e a t number o f d i f f e r e n t t e c h n i q u e s t h a t were worked t h r o u g h i n t h e f i r s t p h a s e o f t h i s p r o j e c t t h e b u r n - l e a c h method as head end and t h e t h o r e x p r o c e s s f o r t h e uranium s e p a r a t i o n have been f i n a l l y s e l e c t e d as t h e most f a v o r a b l e ones f o r d e t a i l e d i n v e s . t i g a t i o n s . Dry t e c h n i q u e s are recommended t o l a t e r de- ve lopment work. The i n v e s t i g a t i o n s t o d a t e have s t i l l t h e s t a t u s of l a b o r a t o r y e x p e r i m e n t s , however t h e y are b e i n g p e r - formed a l r e a d y w i t h h o t mater ia l and w i t h i n a comple t e scheme. The r e s u l t s o b t a i n e d have been t h u s f a r s a t i s f a c t o r y , s o t h a t d e s i g n work f o r a p i l o t p l a n t c o u l d be s t a r t e d meanwhile. T h i s p l a n t s h o u l d r e a c h a t h r o u g h p u t of 2 - 3 k g / d a y i n 1973 which i s enough t o p r o c e s s t h e bu rned f u e l of t h e AVR.
The re i s n o t y e t a d e f i n i t e c o n c e p t i o n on t h e c o n s t r u c t i o n of a b i g p r o t o t y p e p l a n t f o r r e p r o c e s s i n g t h o r i u m c o n t a i n i n g HTR f u e l e l e m e n t s . S e v e r a l v a r i a t i o n s are p o s s i b l e and are b e i n g a n a l y s e d p r e s e n t l y . The t o t a l deve lopment o f n u c l e a r e n e r g y i n West Germany w i l l i n f l u e n c e t h e d e c i s i o n b u t a l s o t h e q u e s t i o n of how q u i c k l y t h e uran ium-thor ium c y c l e c a n s u b s t i t u t e t h e l o w e n r i c h e d uranium c y c l e s w i l l p l a y a r o l e a t l ea s t i n Europe .
PROS PE CT S
Only a small p a r t of t h e a c t i v i t i e s men t ioned are a l r e a d y comple t ed , namely , t h e AVR-project and t h e deve lopment o f t h e THTR. The o t h e r s are s t i l l i n p r o g r e s s and a p a r t of
‘I
159
6d them h a s j u s t been s ta r ted .
Because of t h e r e l a t i v e l y f a r - r e a c h i n g g o a l s v e r y much and u n f o r t u n a t e l y t h e most d e c i s i v e work i s s t i l l i n f r o n t of u s . The f o r e s e e n f u n d s which are q u i t e c o n s i d e r a b l e f o r Germany are, a t l eas t i n p r i n c i p l e , ag reed t o by t h e p e r t i n e n t federal m i n i s t r y . I n fac t t h e HTR-development i n West Germany has
meanwhile r eached t h e same p r i o r i t y as t h e development o f t h e l i q u i d coo led f a s t breeder.
These facts o b l i g e u s t o a n a l y s e r e g u l a r i l y and v e r y s e r i o u s - l y t h e whole program t h a t means t o p u t up t h e q u e s t i o n : Whether t h e e x i s t i n g f i n a n c i a l and p e r s o n e l b a s e i s s u f f i - c i e n t f o r a s u c e s s f u l comple t ion of t h e mentioned a c t i v i t i e s and whether these a c t i v i t i e s are i n a r e a s o n a b l e r e l a t i o n t o t h e a i m s . During t h e n e x t weeks w e w i l l u n d e r t a k e such a n a n a l y s i s once more.
A s t h e HTR l i n e can n o t r e l y on e x t e n s i v e m i l i t a r y deve lop- ments , which w a s t h e case f o r t h e commercial e x p l o i t a t i o n of t he LWR-systems, i n Germany w e are wor ry ing abou t a p o s s i b l e o v e r c h a r g e o f t h e d i s p o s a b l e f o r c e s a l r e a d y i n t he c o u r s e of i n t r o d u c i n g t h e f i r s t HTR g e n e r a t i o n i n t o t h e f r e e e n e r g y marke t as it e x i s t s i n our c o u n t r y . The f u s i o n of a l l german i n d u s t r i a l companies s u p p o r t i n g t h e HTR which i s b e i n g com- p l e t e d w i t h i n t h e n e x t months, g i v e s g r e a t hopes i n t h i s r e s p e c t b u t i t i s p o s s i b l e t h a t o n l y an even g r e a t e r , t h a t means i n t e r n a t i o n a l i n d u s t r i a l base can g a r a n t e e a good chance f o r t h e commercial e x p l o i t a t i o n o f t h e HTR. An effec- t i v e i n t e r n a t i o n a l c o o p e r a t i o n between t h e competent c o u n t r i e s shou ld t h e r e f o r e be p u t i n t o c o n s i d e r a t i o n much more i n t h e f u t u r e .
180
DISCUSSION
F. L. Culler: 1. Is 1600°F (approximately 850°C) high enougk tem-
perat .De todri .ve t h e water gas r e a c t i o n ? W i l l t h e h e l l m i not have t o be
a t cons iderably h ighe r temperature to o b t a i n good y i e l d s of w e t f u e l gas
wi th t h e steam carbon r e a c t i o n ? 2. Have i r r a d i a t e d g raph i t e f u e l element
saniples been burned and leached ?
H. Kr'kner: 1. 850°C i s not a s u f f i c i e n t l y h igh temperature for a steam-reforming process , 900-950°C w i l l be necessary. We are hopeful t h a t
such gas temperatures can be reached w i t h i n t h e next 5-7 years . 2. Y e s ,
i n ho t c e l l experiments, d e t a i l e d d e s c r i p t i o n s of t h e experiment w i l l be
DESIGN, FEATURES AND ENGINEERING STATUS OF THE THTR 300 MWe -I- . -d - * I io
PROTOTYPZ POWER STATION - -nmw-=w,- -A
H. Oehme J. Schoning -3
Brown Boveri/Krupp Reaktorbau Ltd. is developing a line of high-temperature helium-cooled pebble-bed reactors, with completely integrated primary sys- tem. The feasibility of the concept has been dem- onstrated by the AVR experimental reactor, which has been supplying electricity to the grid since December 1967. The next stage in the development is the 300 MWe THTR, which has the same design characteristics as the AVR. However, various com- ponents were modified because of the increased dimensions of the THTR, such as the prestressed concrete pressure vessel, The design of the THTR, its safety concept, and supporting development tests are described, as well as the status of engineering and construction arrangements.
GENERAL CHARACTERISTICS OF THE 300 MWe THTR
The main activity of the Brown Boveri/Krupp Reaktorbau L t d .
is concentrated on a thorium high temperature reactor line based on spherical fuel elements. iTh e main characteristics o f this reactor line are the following:
- spherical fuel elements - helium as coolant - high primary gas temperatures up to 800 C - primary system completely integrated
0
The spherical fuel element permits continuous fuel loading
during operation. Each individual fuel element has a negligible
amount of reactivity.
161
162
The feasibility and advantages of this reactor concept have
been demonstrated by the construction and operation of the AVR
experimental reactor ( 15 NWe) which was brought to criticality
for the first time in August 1966. Since December 1967 AVR has supplied electricity to the grid, and during 1969 the plant achieved an availability of 72 5. The thorium high temperature reactor (THTR) possesses essentially the same construction characteristics
as the AVR (Slide 1). However, based on the experience gained with
A V R , and in view of the higher power of THTR the following compo-
nents were introduced or changed:
- the prestressed concrete pressure vessel - the core structure - the shut-down system - the fuel element circulating system
The 300 MWe THTR prototype reactor is designed and optimized
as a direct predecessor of a reactor of commercial size (Slide 2).
THE INTEGRATED PRIMARY SYSTm
The reactor core and all main components of the primary system - blowers, steam generators, shut-down system -, excluding the fuel circulating system and gas purification plant, are completely inte-
grated in a prestressed concrete pressure vessel. Access to these
components is not foreseen although they can be removed in case of
failure or of inspection or maintenance work. All other components
and facilities are located outside the prestressed concrete pressure
vessel and are accessible during reactoa operation (Slide 3) .
The reactor core consists of approximately TOO 000 spherical fuel elements of 6 cm diameter. The cylindrical core of 5,6 m diameter and 6 m height is formed by a graphite wall which acts as reflector and surrounds the core on all sides. The bottom re-
flector is conically shaped with an inclination of 30° and opens
into a central discharge tube of 800 mm dia.
163
Graphite is a well-known material proven in many reactors. The
THTR reflector is exposed to a higher radiation dose (maximum total
dose 2 nvt) and to a considerably higher temperature. Apart
from that and in addition to its usual function as a reflector, and
as nuclear and thermal shielding, it must perform the mechanical
function of a supporting and containing structure for the pebble bed.
By an appropriate choice of the graphite (considering the important
influence of the cementing resin) it is possible to remain within
controllable dimension changes of the structure since the determining
fast neutron flux decreases very rapidly in the reflector so that
a noticeable shrinkage can occur only up to a depth of 10 - 20 cm of the inner graphite layer. With the selected graphite type and
the total maximum dose to be expected a maximum shrinkage of 2 $ and an corresponding growth to the initial dimensions was taken as
a design basis. Because of all these requirements, special measures
for the core structure are necessary, to provide the necessary
flexibility of the graphite structure for temperature- and radiation-
induced dimensional changes, thus avoiding possible compressive
forces while insuring the stability of the total structure. These
requirements were met by relatively small blocks specially shaped
and arranged in columns and by connecting and fixing the blocks
with wedges and dowels (Slide 4 and 5).
The prestressed concrete pressure vessel acting at the same time as pressure vessel and as gas- and pressure tight safety
containment, includes all main components of the primary circuit.
It is a cylindrical vessel of- 16 m diameter and 15 m height with
a wall thickness of approximately 5 m. Prestressing is achieved
with annular and vertical stressing cables having a guaranteed rupture
sheaths embedded in the concrete and are grouted after prestressing
to insure sufficient protection against corrosion.
load of 890 Mp. The prestressing cables are inserted in
164
For the pressure vessel a relatively conservative design was
selected, which has been proven in numerous large-scale constructions
and has been and will be tested in a number of model tests ( l :5 , 1:45, 1:20 ). The test result will be incorporated in the large- scale construction. For further Frojects, while retaining the same
vessel shape, various technical and cost-saving improvements are
foreseen, such as transition to a horizontal wire winding pre-
s+,ressing system and reduction of the inner dimensions by an optimum
arrangement of components. It is possible that further economic
advantages may result from the podded design; the pressure vessel
cost and the technical safety requirements are approximately equal
for both vessel types.
For the introduction of blowers, steam generators, absorber r o d s ,
pipes, etc. the prestressed concrete pressure vessel is equipped
with penetrations. These penetrations are reenforced by ,shutter-
tubes designed t o absorb the forces in the area near the penetrations.
The largest openings of 2,25 m diameter for the steam generators
are located in the top slab of the vessel.
Gas-tightness is achieved by application of a metal liner of
20 - 30 mm thickness serving at the same time as the inner shutter-
ing for the prestressed concrete pressure vessel during construction.
For the liner material special properties are required, such as
high elasticity, good weldability, and high yield strength.
An insulation on the inner wall and a water cooling system
welded on the outside of the liner protect the steel liner and the
concrete against excessive temperature effects. A s insulation a
metal foil insulation (stainless steel) proved to be the optimum
solution since with this insulation purity requirements can be
easily met, irradiation behaviour of the materials is sufficiently
known, mechanical properties are satisfactory, and aging and
corrosion are not to be expected. The thickness of the heat
insulation of the liner is approximately 70 mm.
165
Six parallel single-stage radial blowers each supplying one
steam generator, circulate the coolant gas. The blower is designed
as an insertable unit. The impeller is mounted in an overhung po-
sition and is oil-lubricated. A baffer-gas system avoids the pene- tration of oil into the primary gas. Each blower is equipped with
a combined bypass and shut-off valve system to allow connection of a single blower while other blowers are operating, trimming of
coolant gas flow through one steam generator under constant blower
speed, and shut-off of one line in the event of failure of one steam
generator. A s drive a bipolar ?-phase squirrel cage motor was se- lected which is characterized by simple design and high operational
safety. Blower power is controlled by variable frequency. Three
blowers are supplied by one turbine generator set. In the event of
failure of the two turbine sets, operation can be maintained with
constant speed by the mains power supply. In addition, transformer
sets are provided, permitting start up and emergency operation of
individual blowers (Table 1 and Slide 6).
0
Table 1. Blower Data
ITumber of units 6 Delivery per circulator 49,25 kp/sec
Pressure at suction duct 38,9 ata
14 m 3 /sec Delivery in volume
Pressure increase 1 , l ata
Temperature at suction duct 25OoC
Circulator power 1780 kW
Six steam generators connected in parallel transfer the heat
generated in the core to the secondary water-steam-circuit. The
main steam generator date are listed in the table (Table 2).
166
Table 2. Steam Generator Data
Number of units
Diameter of tube bundle
Height of bundle
Gasflow through the generator
Total length
Output per unit
Hot gas temperature Cold gas temperature
Gas pressure
Pressure drop at gas side Gas m a s s flow
Live steam conditions
Feed water conditions
Rehe at ing
at entry at exit
Steamflow
6 2 000 + 55 mm max. 12 500 mm upwards
17 800 mm 128 MW
750°c
39,35 ata max. 0,45 ata
49,25 Kr/sec 335OC / 190 ata 18OoC / max. 240 ata
250°C
The helium flows through the steam generators in an upward direction.
The tube bundles of superheater, reheater, evaporator, economizer
are arranged in gas flow direction. The steam generator operates
in a once-through-system. The water steam-flow through economizer,
evaporator, and reheater is in counter-flow direction, the super-
heater in uniflow direction. Three steam generators are connected
in one main group, which is equipped with a common feed-water line,
a start up flush-tank, and a common cold reheater line. To insure safe emergency cooling and removal of decay heat from the core
each steam generator can be operated independently of the other
steam generators, i.e. each is equipped with separate shut off and
control valves. Each tube bundle of the steam generator is sub-
divided into forty independent systems which are individually led
through the top slab of the prestressed concrete pressure vessel
16’7
0 and connected outside of the vessel. Hence, in the event of a tube
failure each system can be isolated from outside. The steam generator
is so designed that it can be replaced.
The control and shut-down system is designed so that the reactor load can be varied between 40 and 100 $ and the shut-down reactivity required to keep the reactor in the cold critical state is available.
Fine control is carried out by 36 rods which are freely moved in bore holes in the reflector. Shut-down of the reactor under both
normal and fault conditions is effected by 42 core rods which are
directly inserted into the pebble bed. This procedure was verified
by exterrsive tests on a complete model 1:6, 1:lO and on sectional
models in 1:1, 1:2, 1:3. This proved that the rods can be directly
inserted into the pebble bed under all operating conditions of the
reactor and neither the fuel elements nor the absorber rods them-
selves are exposed to excessive stresses. Each core rod is driven
by a pneumatic step drive, achieving safe insertion at a step size of 2 cm and a step frequency of 0,3 sec. For rapid shut-down a
long-stroke pneumatic system is provided, with an insertion speed
of 30 cm/sec. Each drive has a separate supply system with re-
dundancy (Slide 7).
The THTR fuel element circulating system is of special interest. It is not integrated in the primary circuit and in contrast to
reactors with rod type fuel elements, requires no machinery inside
the core for charging, exchanging, and discharging fuel elements.
For the downward motion of the fuel elements from the core (fuel
element discharge) gravity is used and upward movement (fuel element charge) is achieved with pneumatic energy by helium from the primary
circuit. For the construction of the fuel element circulating system
a building block system, composed of conventional units was used
(Slide 8 and 9 ) .
168
Because of their special requirements, the components involved
in the helium system required the development of a new technology
which can be roughly divided into three problem areas:
- helium purification and purity - helium leak-tightness - lubrication and friction in an extremely pure and dry helium atmosphere
According to the present state of technology, these problems
can be considered essentially solved. For selection and application
of components, however, a number of aspects must be taken into
account, which have proven to be advisable, on the basis of know- ledge and experience gained up to now, especially through con-
struction and operation of the AVR. The following aspects are of importance:
- good accessibility to the components needing maintenance (location outside of radiation area)
- good maintenance facilities for systems with flanged and screwed joints (plastic material)
- protection of the sensitive instruments against dust and dirt caused by assembly, through use of suitable filters
components (oil, air, etc.)
- protection of the helium against pollution from the operating
- simple and conservative design of systems - well-defined and separated tasks for individual systems, thus allowing uncomplicated design
- use of conventional proven components These fundamental aspects partly result from special newly
developed designs which were carried out to achieve an optimum
solution of the reactor concept of the gas cooled high temperature
line
169
The mechanical impurities which are mainly produced by the gas
circulation plant the fuel element abrasion in the core and the
assembly protection and which impair the leak tightness and the
control exactness of a number of valves, can be controlled by
mechanical filters but even more effectively by restricting or re-
moving the impurity sources. The impurities from the gas circulation
facilities can be largely avoided by barrier gas systems or oil free
blowers and compressors (gas-bearings blowers, membrane compressors
and dry operation compressors). The impurities produced by assembly work are reduced to a minimum by careful assembly (freedom of
grease, scale, and corrosion of all helium-carrying systems) in
appropriate clean conditions standards. For this purpose pre-assembly
in the workshops of the suppliers must be demanded. The dust which
is unavoidable due to fuel element abrasion is eliminated by appro-
priate mechanical filters in the gas purification plant.
0
The wear problems occuring under these specific reactor condi-
tions are solved by special constructions (cageless ball bearings,
special bearing clearances, dry lubricated structures) with appro-
priate auxiliary measures such as barrier gas systems.
For safety and economy reasons, the problem of leak tightness
is of special importance for the HTR. Although welding is the most simple, most economic and safest solution, it is only appl icable
for static seals and this applies for operational reasons only in
some cases. The solution adopted for dynamic seals is to be de-
monstrated for two especially critical cases, that is gas tightness by valves and gas tightness in the event of rotary motion (momentum
of rotation). In both cases a satisfactory solution could be achieved only by redesigning the components in parallel with sealing material
and lubricant developments for these components. Because of the
favourable development results of plastics materials such as Viton,
Kel-F, Vespel, RCH 1000 all now available, which in addition to sufficient radiation and temperature resistance, have satisfactory
mechanical properties; the same applies for lubricants.
c3
170
The first example concerns a simple, safe, and economic gas shut-off bellows valve (leak tightness in the valve cap is achieved
by a specially mounted plastic material). (Slide 10)
The second example concerns a gas-tight rotary drive. Also in
this case, special importance was attached to safety and economy.
In this type of solution, the gas tightness is achieved by using grease which forms a considerably less complicated fluid seal.
Higher pressure relative to system pressure, grease expansion due
to temperature changes, and re-lubrication are effected by pressure
reservoirs (Slide 11 ) .
SAFETY CONCEPT
In this connection only those facts will be mentioned, in which the safety concept of THTR differs from those of other reactors. The decisive safety aims are:
Complete integration of the primary coolant circuits in the pre-
stressed concrete pressure vessel
- hence limited l o s s of coolant in the event of credible accidents - release of activity via ventilation stack in the maximum credible accident
- no sudden depressurization of core - integrity of core structure The penetrations in the concrete vessel are designed to prevent
activity release by either
- two pressure-tight covers or - an outer pressure-tight cover, and an inner flow limiting cover
(about 33 cm2 corresponding to a coolant pipe diameter of 65 mm) which, in the case of the outer cover being damaged, restricts
the escaping coolant flow to a precise value.
A
171
Those primary coolant pipes which lead from the concrete pressu-
re vessel to the auxiliary circuits are 6 6 5 mm diameter. These pipes are double walled as far as the fast action safety release
valves. The safety container has no safety valves and is designed
for the pressure of the maximum credible accident. The total primary
building is divided into three categories of rooms, according to
their different activity levels (Slide 12).
- Rooms continuously accessible during operation - Rooms accessible only for a short time during operation,
0
for inspection purposes
- Rooms no% accessible during operation, access possible only after partial or total shut-down of plant
The third category includes primarily the room for the installation
of the fuel circulating plant and part of the room for the gas purification plant as well as the space between air duct and pre-
stressed concrete pressure vessel. According to their room catego-
ries, these rooms are separately ventilated and are connected to the ventilation stack via the normal exhaust air system and in
addition, by a pressure safety system.
The safety analysis of this concept showed that, the maximum
credible accident, with reference to endangering the surroundings, requires two independent faults to occur, namely
- a break in a primary coolant pipe ( 6 65 mm f8) outside the concrete pressure vessel
- the simultaneous malfunctioning of the safety release valve in that pipeline
In this case the escape of coolant gas is relatively slow, without
a noticeable pressure rise in those rooms and can easely be vented.
men in the case of this maximum credible accident, the allowable
contamination of the surroundings is not reached.
The largest realistic reactivity excursion through
- the accidental withraval of the two most effective control rods from the core
the largest realistic coolant disturbance by 6id
- the simultaneous breakdown of three blowers, and the largest realistic pressure change through
- the burst of a steam generator pipe and causing water ingress into the core
have such a limited effect on the reactor, that the surroundings
are not endangered.
THE STATUS OF THE 300 Mlrle THTR-PROTOTYPE
Construction documents for this prototype plant have been
completed and an offer has been submitted. The licensing procedure
has been initiated early 1970 ( l 5 / l ) . A utility group for the operation of this reactor plant has been founded and construction
work is to be started in the beginning of 1971. The construction
period is 5 years, including a test run of the plant of three month.
R l ROOYCATEGORY - NOT ACCESSIBLE DURING REACTOR OPERATION
R t RWUCAIEGORI - ACCESSIBLE TEMPORARILY
R 3 RMYCATEURV- ACCESSIBLE PERMANENTLY
I CORE
2 STEAM GENERATOR
3 CIRCULATOR
4 PRESTRESS0 PRESSURE VESSEL
5 FUEL ELEMENT OUTLET
6 CONTROL RW
BBC / KRUPP
12 Safe ty Concept
179
DISCUSSION
B. N. Furber: I would l i k e t o have fur ther d e t a i l s of the meta l l ic
insulat ion. I n the experience of TNPG t h i s insu la t ion suf fers from a t least two weaknesses: c u l t t o design t o accept in te r face pressure gradients. I n the c i r c u l a t o r
o u t l e t these two weaknesses a r e l i k e l y t o ser iously a f f e c t the insu la t ion
performance.
(1) It is highly anisotropic , ( 2 ) it i s very d i f f i -
What t e s t work has been carr ied out i n t h i s a r e a ?
J. Schzning: We are aware of the problems raised by you and our
people have a concept t o overcome them, the detai ls of which we are not
ab le t o present. work going on t o confirm the concept t h a t has been selected.
There are extensive experiments and de ta i led design
R. D. Vaughan: The THTR reac tor sec t ion shows the b o i l e r s t o be of
cy l indr ica l plan form, but located i n the pressure vesse l vaul t along w i t h
the reac tor core. May I conclude t h a t the designers have looked a t the a l t e r n a t i v e with pods i n t h e w a l l of the pressure vessel and found it would be more expensive?
J. Sch'dning: The\design of the THTR pressure vesse l and t h e arrange- ment of the b o i l e r s within the vesse l was already decided upon i n 1965.
A t t h a t time the pod-type vesse l did not ye t seem t o be evaluated.
t h i s time a change of the concept i s not possible due t o the advanced state of development and design. It is important, however, that the THTR-
vesse l allows the removal of the b o i l e r s i n t h e same way as the pod-type vesse l does. s t a t i o n a de ta i led comparison of the two vessels and t h e i r influence upon the p lan t i s under way.
At
Within the development work f o r a l a r g e commercial power
M. Dalle Donne: Coming back t o t h e question of Dr. Furber, I think
he answered h i s question himself with h i s paper. With helium one i s i n the region of Raleigh number where the Nusselt number i s constant, so t ha t
a var ia t ion of helium v e l o c i t y does not change the heat t r a n s f e r coeff i -
c ien t of the insu la t ion ; although t h i s may be the case w i t h C 0 2 , where
the heat i s mainly t ransfer red by convection, while with helium it i s
t ransfer red by conduction.
Paper 3/112
TRE LAYOUT OF T m CORE AND FUEL ELEMENTS OF THl3 THTR -”-%.
- -------- - - -- - - - - w l L - - r . - S - - ~ - ~ ~ , ~ * r W - c ” c l l r r r - -._. __ K. Ehbers (Brown Boveri/Krupp Reaktorbau GmbH,
Cologne, Federal Republic of Germany)
H. Harder (Brown Boveri/Krupp Reaktorbau GmbH, Cologne, Federal Republic of Germany)
E. Schroder (Brown Boveri/Krupp Reaktorbau GmbH, Cologne, Federal Republic of Germany)
\A‘ ABSTRACT
The continuous loading and circulation of the fuel elements in pebble bed reactors results in a number of performance differen- ces from reactors with prismatic fuel elements. Their influence on the layout of the core and fuel elements of the THTR is de- scribed.
Introduction
The THTR is a high-temperature gas cooled pebble bed reactor, the construction of which is expected to be licensed within 1970. The THTR is operated on an uranium/thorium cycle, with fissile and fertile material mixed within each fuel element in a ratio of 1 : l O . The first batches of fuel elements discharged from the reactor will not undergo immediate reprocessing but will be stored for an unspecified period. Although an uranium/ plutonium cycle operating at a lower enrichment would, under these conditions, result in equal or slightly lower fuel cycle costs, the uranium/thorium cycle has been selected because of its greater potential when reprocessing facilities w i l l be available. Optimization calculations have resulted in the fol- lowing design of fuel elements:
180
181
Content of fissile material ( ~ 2 3 5 Content of thorium
Enrichment
6d 0.96 g/sphere
9.62 g/sphere
0.93 Mean residence time in reactor 3.0 years
Mean fast neutron dose (E 2 0. I MeV) 4.8-102’ nvt
Maximum power per sphere
Mean burn-up [fima]
Mean burn-up [fifa)
3.5 kW
0.12
1.34 Mean number of circulations through core 6
The spherical fuel element has a diameter of 6 cm and con- sists of an exterior fuel-free graphite shell with a minimum thickness of 5 mm. Inside of this shell the coated particles are embedded in a graphite matrix of the same composition as the exterim shell.
Core Design
The initial core of the THTR consists of a mixture of approxi- mately 350 000 of such fuel elements and an approximately equal number of graphite spheres, of the same diameter, containing no fuel. The same fuel element type is used for the initial core and the running-in period as well as for the equilibrium core, which allows a considerable reduction in the fuel element fabri- cation cost. The total uranium inventory of 359 kg U235 in the initial core is approximately equivalent to the sum of the con- tents of U235 and U233 in the equilibrium core. Because in the initial core, the thorium to uranium ratio is only h a l f that of the equilibrium core and fission products have not yet been generated, approx. 40 000 absorber spheres must be added to the initial core, each containing 4 g of natural hafnium. Hence no trim rods are required for the initial core and the running-in period.
The core is subdivided in two radial zones. The central zone of 4 m dia is surrounded by an outer zone of 0.80 m width. In order to flatten the power and to obtain a sufficient reactivity worth of control rods inserted into the radial reflector, the ratio of fissile isotope density between the.outer and inner zone is 1.5 and the burnable poison density ratio 0.66. This is achieved by mixing fuel, absorber, and graphite spheres in the two zones accordingly.
182
In this way a reasonable power flattening and a reactivity worth of 4.5-Nile of 36 control rods in the radial reflector is obtained. Such a worth of the reflector rods -is needed to com- pensate for reactivity changes during load-changing between :OO and 40 $ (Xe-override) and for other adjustments.
The neutron flux increase in the outer zone of the reactor core required for this purpose is close to the economically optimal neutron flux distribution. Neutron leakage is increased only slightly. During steady load operation, a major number of these rods are inserted in the reflector to compensate for 1.7 to 2.6 Nile excess reactivity which must be available for con- trolling partial load operation and fine adjustment. If a daily load curve is to be followed, a few additional rods must be in- serted or withdrawn for a few hours. The periods during which all reflector rods are either extracted or inserted are both very short.
When power operation starts the pebble bed is circulated. The spheres pass through the core in the downward direction within average transit time of six months. By the conical shape of the core bottom, the spheres are directed towards the central dis- charge tube, through which they are extracted from the core. Each sphere subsequently passes through a measuring equipment, by which the type of sphere - fuel element, graphite or absorber sphere -, and the burn-up state of the fuel elements can be de- t ermine d .
Initially, some of the graphite and absorber spheres entering into the measuring equipment but no fuel elements are discharged from the system. An equal number of new fuel elements are added to the core to compensate fuel burn-up. The new fuel elements, together with the other spheres not discharged from the system, are lifted pneumatically through guiding tubes and drop on the pebble bed from a low height, thus closing the circulation loop.
The flow lines on which the spheres pass through the core* and the time required for passing through the core on different core radii have been experimentally determined in models of similar geometry. Specifically, it has been verified that the separation of the initial core into an inner and outer zone is maintained sufficiently distinct in spite of the circulation process. A mixing of the two zones which occurs in a region of two or three sphere diameters at the zone boundary is desirable, since steep gradients of power at the boundary are avoided.
A
183
In order to maintain the subdivision of the core into zones, three refuelling tubes point at the core center, and twelve at the outer zone. By an appropriate distribution of fresh and re- circulated spheres to both of these tube systems any desired width of the core-zones can be established, but cones of diffe- rent heights over both core-zones must be accepted.
crs
With increasing burn-up the recirculated fuel elements, graphite and absorber spheres are distributed to the inner and outer zone of the core such as to maintain the power distribu- tion of the initial core. After approximately one and a half years of full power operation - i.e., at a mean fima value of approximately 4.5 $ - all graphite spheres will have been re- placed by new fuel elements. At this time the overall thorium: uranium ratio has largely been shifted towards the equilibrium value, and fission products have accumulated to a considerable degree
As power operation is continued, the first burnt fuel ele- ments must be discharged from the core and replaced by new fuel elements. The burn-up measuring facility insures the discharge of fuel elements with highest burn-up; during the running-in phase these are the fuel elements of the initial core.
After a total of 3 years of full power operation the equi- librium phase in reactor fuelling is almost achieved. From then on the core composition and hence also the power distribution remains constant. Every day 621 new fuel elements must be added to compensate fuel burn-up.
To maintain the desired different fuel concentrations in both core zones during the equilibrium phase the fuel elements are divided into 3 classes, as determined by the measuring facility. Fuel elements having remained in the reactor more than 2 . 9 years of full power are discharged. Because of the different times for passing through the core at different radii this value corresponds to a mean residence time of the fuel elements of 3.0 years at full power. Fuel elements with a burn-up corresponding to a residence time between 1.6 and '2.9 years are subsequently added to the inner zone of the core. Fuel elements with a re- sidence time of less than 1.6 years and all fresh elements are added at a ratio of 79 % to the outer zone and 21 % to the inner zone.
184
Figure 1 shows the residence time spectrum of the discharged fuel elements. Since it is required that only a negligibly small share of the burnt fuel elements (approx. 10-4) remains in the reactor longer than 4.2 years of full power (corresponding to 14 $ fima), the burn-up measuring facility must determine the uranium content of these elements to an accuracy of approx. f 15 mg U235 equivalent. The fissile material content at dis- charge amounts to approx. 50 mg U235 and 250 mg U233. It has been confirmed by experiments that this condition can be met by measuring and evaluating the reactivity increase caused by the fuel elements passing through a measuring reactor of some hun- dred Watts of power. When the operation of the TRPR or further irradiation tests permit an increase of the maximum residence time, the accuracy of burn-up measurement can be reduced.
The distribution of the fuel residence time round the mean value of three years is of small influence on the reactivity and hence on fuel cycle costs.
By recirculating the fuel elements with higher bum-up into the inner zone and by adding the new and the fuel elements of low burn-up preferably to the outer zone, the reactivity worth of the reflector rods of 4.5 Nile can be maintained also in the equilibrium core. Figure 2 shows the radial power distribution taken from a two-dimensional calculation at the core height of maximum power for completely withdrawn, completely inserted re- flector rods, and for a rod position corresponding to full load operation. At full power operation leakage losses are 8.5 $. The maximum fluctuation of the local gas temperature caused by the shifting of the reflector rods are 200 - 250 OC, however with a gradient of less than 10 OC/min. The maximum fuel and gas tem- peratures have been calculated at 1250 OC, and 935 OC respec- tively.
The fuel temperatures in the THTR are favourably influenced by the mode of fuelling the reactor. Since the fuel elements are added from the top and part of their fissile material is burnt during their transit through the core, the power maximum is shifted towards the upper half of the core, that is towards the cold gas side.
Because of the continuous flow of the fuel elements the maxi- mum temperatures in the fuel elements occur only during a short period, compared to their life time. The maximum temperatures occur at the gas stagnation area between the main coolant gas flow and the bypass which cools the element discharge tube. This area occupies approx. 10-4 of the core volume.
185
The fuel elements pass through this region within approx. 20 days. The maximum temperatures are generated in the fuel ele- ments only during this time and only if all margins left for calculation errors on the reflector rod effectiveness sum up to
0
I I During later transits through the core the fuel elements have
the pessimistic side, which then requires insertion of all rods.
already reached a partial burn-up so that lower fuel temperatures result after the first transit.
During operation no reactivities must be compensated other then the reactivity fluctuations resulting essentially from partial load operation, which are to be compensated by the re- flector rods. Thus the 42 absorber rods located above the core are required for reactor shut-down exclusively, and can remain in withdrawn position during almost the entire power operation. Only for stdrt-up after an extended shut-down, several absorber rods must remain inserted to compensate the positive reactivity due to the reduced xenon concentrations and to the decay of pro- tactinium into uranium-233 during the shut-down period.
The requirement of the reactivity worth of these 42 rods must be calculated for the end of a shut-down period of several months. Then the protactinium has completely decayed into U233. A balance at that time is shown in Table 1.
Calculation Procedures
The calculation methods applied for the design of pebble bed reactors largely coincide with the procedures for other high temperature reactors. In addition to these standard methods com- puter programs were developed by which the unique method of charging pebble bed reactors can be taken into account.
The isotope distribution within the core, essential for cal- culating criticallity, power distribution and control rod worth results only if the burn-up state and the local position of the individual fuel elements are known, which however depend on the neutron flux distribution, the flow behaviour of the spheres, and the charging strategy. Therefore, for calculating the equi- librium isotope distribution, a flux distribution must be assessed, and a charging strategy assumed.
186
For several fictive concentric flow channels, the increase of the fuel element burn-up is determined f o r each transit. By averaaing the nuclide concentrations over appropriate volume fractions, an impoved qeutron flux distribution is calculated. If after several steps of itsration this distribution differs too much from the desire6 distrihtion, the charging strategy is varied.
The computer program which calculates this position-dependent core composition for a given charging strategy, takes into account the different transit times of the fuel elements in different flow channels, the influence of the burn-up moasuring accuracy on the distribution of the recirculated fuel elements to the inner and outer core, and their final discharge from the reactor circuit . The 2-dimensional f lux calculations in r,z- geometry must be carriec! out with a rather fine subdivision of the core volume into material zones, i n order to represent the flow paths of the elements suffjciently.
1
During the running-in period the core composition and the power distribution are time dependent. Therefore, burn-up cal- culations are carried out starting with the power distribution of the initial core. The core is subdivided into a number of sphere packages. Using the neutron flux averaged over such a sphere package, the burn-up in the fuel elements of this package is calculated f o r a time increment with the assumption that the circulation movement can be neclected. Subsequently %he indivi- dual sDhere packages are shifted according to the paths ahancet! due to their movement during this time increment. The calcula- tion of' tbe further increase in burn-up is then performed with the neutron flux at the new position of each sphere package. After a number of time increments, Cukie flux distribution must be recalculated. A difficult data storaqe problem within this pro- cedure is the follow-up of the nuclide concentration in those sphere packages which are recirculated after a transit through the core and where individual spheres are either assigned to different core zones o r partly discharTed. The nuclide concen- trations must be distributed accordincly.
The temperature distribution is also calculated in r,z- 'Zeometq. The eeometry is described by a mesh layout. The mass flow distribution is determined by similar aethods as developed in electrical network theory. The mass flow and temperature de- pendence of the flow resistance is taken in$o account.
A
187
For determinirig the release of fission products the tem- perature and burn-up history of one representative fuel slement during its residence time is calculated. As transport mechanism of solid fission products, temperature-activated solid-state diffusion and evaporation from the eiirface of the fuel element into the coolant gas are considered. The time-dependent diffu- sion equation is solved numerically under variable temperature and power conditions for the fuel particles, the fuel coating, the graphite matrix, and the fuel-free shell of the fuel ele- ment. The contamination of the coating and the matrix by fission material during fabrication and the diffusion of inert gas pre- decessors for various radioactive decay chains are taken into account .
The results are time-dependent release rates of one repre- sentative element and - by integration over the core volume and time - the total release of the core.
With similar procedures corrosion rates and atresses are calculated, the latter program makes use of an existing com- puter code "STRETCH", adapted to the requirements of a moving fuel bed.
Consequences for the Fuel Elements Layout
The major part of activity in the primary circuit is due to gasous fission products caused by the contamination of the fuel elements with fissile material, either directly or indirectly by decay of a gaseous predecessor.
The favourable influence of the moving fuel on the total re- lease from the core can be demonstrated by comparing a static core with a continuously flowing core of identical temperature distribution and residence times.
The release rates of long-lived fission products from the moving fuel elements are far below those of the static core; for strontium 90 e.g. they are lower by approx. 3 orders of magnitude. Therefore, even without having a secondary contain- ment around the primary circuit no layer of Sic is required in the coating of particles. This is important for improving the neutron economy, and lowering both fabrication and reprocessing costs.
188
Since the fuel elements will remain within the region of high temperatures for relatively short periods only, no stringent re- quirements are needed for the irradiation resistance of the gra- phite. The graphite selected for the fuel elements (see Figure 3 ) starts expanding at temperatures of approx. 900 OC and doses of 8 x 102l nvt (E t 0.1 MeV). This has to be compared with the maximum dose of 6 . 3 x 1021 nvt in the reactor, which is only reached by a fraction of 10-4 of all elements discharged.
The results of stress analysis for the fuel elements in reactor operation are shown in Figure 4. The maximum tensile stresses occur after the first transit through the core, since then the temperature gradient disappears because of the sharp reduction of power production. In the core the temperature ea- dient partially compensates the stresses caused by dimensional changes due to irradiation. The sudden change of tension de- creases with increasing burn-up. A compariscjn with calculated stresses of irradiation experiments shows (see Figure 5) that the maximum stresses occuring in these experiments are much higher than those to be expected in the THTR. Therefore, there will be no damage of the fuel elements by irradiation-induced and thermal stresses.
REFERENCES
1. L. Massimo, Nukleonik 11, 72 (1968)
189
Table 1. Reactivity Balance
Reqiiirement
1.7 Nile le-everride between full and 40 $ load (normally compensated by reflector rods)
2.0 Nile Temperature
3.8 Nile Xe-equilibrium
3.6 Nile Pa-233 decay and U233 build up
0.5 Bile Margin to compensate fluctuations due t o deviations from refuelling plan
11.6 + 1.1 Total
Rod efficiency
17.3 Nile Calculated worth of 42 rods
1.3 Nile Worth of the two most efficient rods
16.0 + 2
+ 4:;4,;=2:?: Shut-down margin
Table 2. Fission Product Release into Primary Circuit
moving core 1 ~~
Isotope 1. from. I from impurities kernel
Xe 133 Xe 135 Kr 88 Kr 85m J 131 J 132
J 133 Sr 90
Cs 137
1300 Ci
150 Ci
1350 Ci 750 Ci
ci
ci
ci -
260 Ci
static core
from impurities
1300 Ci
150 Ci
1350 Ci
750 Ci 50 Ci
ci
0.1 Ci -
1500 Ci
from kernel
- - - - - - - 5 ca.10 Ci
E-10000 Ci
190
\
rei. units 1
P (T
10
10'
1 0 - ~
io-' 2.0 3.0 L .O 5.0
T [years]
Fig. 1. THTR Fuel Element Residence Time Bistribution
F'unc t ion.
region boundory
Fig. 2. Radial Power Distribution in THTR Equilibrium Core.
1 2 3 4 5 6 7 e 10"""t I 1 1 1 I I I 1 )
E 70,l MeV
( '!. 1 I
Fig. 5. Dimensional Changes of THIrR Fuel Element Graphite.
191
IRRADIATION TIME (DAYS I
Fig. 4. Reference Fuel Element: TangenCial Stresses and
Power in THTR.
ANGENTIAL ;TRESS kp lcm2)
x)
0
- 10 - 2 0
-a
-40
-50 II II I I J IRRADIATION TIME [DAYS I
POWER I k W I
Fig. 5 . Reference Fuel Element: Tangential Stresses and
Power in Irradiation Experiment.
192
DISCUSSION
J. D. Thorn:
H. Harder: 1 X
What i s the design value of R/B?
L. W. Graham: I n looking a t t h e s t r e s s e s i n the b a l l , have you con-
s idered t h e e f f e c t s of the d i f f e r e n t i a l dimensional changes between the
f u e l and un:fueled p a r t s ?
H. Harder: No. The s t r e s s e s shown i n t h e s l i d e concern a sphere of homogeneous graphi te matrix.
J. D. Thorn: What changes i n hea t t r a n s f e r a r e expected around the
f u e l element b a l l ?
H. Harder: Not s i g n i f i c a n t .
F. P. 0. Ashworth: There i s a complex vec tor f i e l d of b a l l ve loc i - t i es and swel l times i n the core. Is the re a p robab i l i t y of a b a l l s tay- i n g i n the core long enough for t he r e l ease t o exceed the t o l e r a b l e core t o t a l f o r a p a r t i c u l a r f i s s i o n product?
H. Harder: There i s only an extremely sma,ll p robab i l i t y t h a t spheres remain i n the core f o r such a long time. Even then t h i s would r e s u l t i n a neg l ig ib l e e f f e c t on t o t a l a c t i v i t y of t h e primary coolant.
T. A. Jaeger: This ques t ion concerns the diagram showing t h e r e s u l t s of a thermoviscoelastic ana lys i s of the sphe r i ca l f u e l element. Could you
give some d e t a i l s on the underlying assumptions and the method of ana lys i s u t i l i z e d , e .g . , d i d you include considerations on the a f f e c t s of contact pressures and l o c a l hea t t r a n s f e r disturbances ?
H. Harder: The temperature d i s t r i b u t i o n due t o the power produced i n a f u e l element during i t s seve ra l t r a n s i t s through t h e core and the
s t r e s s e s r e s u l t i n g from the time-dependent temperature gradients i n the sphere have been calculated. The stresses due t o i r r a d i a t i o n a f f e c t s Lave been determined by piecewise eva lua t ion of t he curves representing
shrinkage of graphi te versus neutron dose as measured i n i r r a d i a t i o n ex- periments a t t h e corresponding temperatures. l l i s includes some approxi- mation because the temperature i n each of t hese experiments has been
193
@ confined during t h e whole i r r a d i a t i o n times. For creep, p r o p o r t i o n a l i t y
The e f f e c t s o f contac t between d/dt (fill) and stress has been assumed.
p re s su res and l o c a l heat t r a n s f e r d i s turbances have not been considered
i n t h i s ca l cu la t ion .
W. R. Martin: What i s t h e absorber m a t e r i a l t o be used i n t h e 42
con t ro l r o d s ?
H. Harder: B4C.
W. R. Martin: How i s t h e H f and B being incorpora ted i n t o t h e f u e l
elements as a burnable poison?
H. Harder,: The burnable poisons w i l l not be incorpora ted i n t o t h e
f u e l elements, bu t will be contained i n absorber spheres , which a r e f r e e
of f u e l .
W. P. Ear thold : How we l l do you measure the burnup and what i s the
peak-to-average burnup r a t i o ?
H. Harder: The burnup can be measured wi th an accuracy of 10-12 mg
U235 equiva len t .
i n g r e a c t o r .
mean burnup 12% fima.
This has been demonstrated i n a prototype of t h e measur- The maximum burnup i n t h e equi l ibr ium core i s 145 f i m a , t h e
B. G. Chapman: Was the f i g u r e of 2.0 n i l e s r e a c t i v i t y change f o r
temperature, t h e ful l value from f u l l power t o a cold core, o r t o a warm core wi th decay h e a t after shutdown?
H. Harder: 2 .0 n i l e s i s t h e r e a c t i v i t y change from f u l l power t o a cold core. This f i g u r e concerns t h e equi l ibr ium core. I n the i n i t i a l
core , t he corresponding va lue i s about 4.0 n i l e s .
L. A. Lys: Could you desc r ibe t h e des ign p r i n c i p a l of t he c o n t r o l
rod, i n p a r t i c u l a r t h e i r mode of o p e r a t i o n . f o r r e a c t o r scram.
H. Harder: The con t ro l rods a r e i n s e r t e d i n t o the pebble bed w i t h -
ou t guiding tubes.
has been demonstrated by a s e r i e s of experiments i n models of similar geometry that such a procedure i s poss ib l e without having too high loads
It has been descr ibed by Sch'dning i n h i s paper. It
194
J. D. Hart: What i s the design l i m t t f o r corrosion of the f u e l
spheres?
t h a t t h i s would cause dust t o be generated?
Should t h i s l e v e l of corrosion occur i n pract ice , i s i t expected
H. Harder: The exact spec i f ica t ion of the corrosion r a t e w i l l be
given by Dr. Hackstein i n h i s paper. Concerning dust, we can r e l y on
the AVR experience, where only negl igible amounts of dust have been found
up t o now.
G. Ivens: Because of the la rge amounts of chemical impurit ies i n
the AVR primary c i r c u i t , we should have expected considerable corrosion
and dimensional changes. I n f a c t , we have found no evidence of such
changes i n f u e l spheres taken from the AVR core.
A. Chamberlain: I n paper 1/101 De. Kr'ber referred t o extensive guarant,ees on THTR f u e l from the f u e l manufacturer. T h i s presmbly i m -
p l i e s t h a t the i r r a d i a t e d f u e l elements a r e monitored f o r f i s s i o n product
re lease before being fed back i n t o the reactor . I n t h i s context what con-
s t i t u t e s a f u e l element which has not m e t the guarantees?
H. Krgmer: The THTR has divided f o r measuring the burnup of each
b a l l leaving the core; and it a l s o has a device f o r measuring the f i s s i o n
gas re lease of each b a l l .
f i s s i o n gas re lease of more than 5 X
guarantee given gy Nukem.
Balls having a burnup l e s s than 8$ fima and a
R/B w i l l be replaced under the
Paper 4/121
LARGE HTGR D E B
A . J . Goodjohn Gulf General Atomic I n c o r p o r a t e d 40
San Diego, C a l i f o r n i a
A ABSTRACT -5i
The d e s i g n s t a t u s of a n u c l e a r steam supply system employing a h igh- tempera ture gas-cooled r e a c t o r and c a p a b l e of producing s u f f i c i e n t h i g h - q u a l i t y steam t o g e n e r a t e approximate ly 1100 m ( e ) i n a c o n v e n t i o n a l r e h e a t steam c y c l e i s d i s c u s s e d . T h i s design--the r e s u l t of more t h a n two y e a r s of e n g i n e e r i n g e f f o r t by a l a r g e f r a c t i o n of t h e d e s i g n e n g i n e e r i n g s t a f f of Gulf Genera l Atomic Incorpora ted- - i s based on t h e s a m e technology and development work as t h e 330-MW(e) F o r t S t . V r a i n Nuclear Genera t ing S t a t i o n which Gulf Genera l Atomic i s p r e s e n t l y c o n s t r u c t i n g f o r t h e P u b l i c Service Company of Colorado under t h e United States Atomic Energy Commission Power Reac tor Demonstrat ion Program. S e v e r a l d e s i g n improvements have been i n c o r p o r a t e d which e i t h e r improve t h e s a f e t y o r economics o r f a c i l - i t a t e t h e o p e r a t i o n and maintenance of t h e p l a n t . The r e a s o n s f o r some of t h e s e improvements are sum- marized.
INTRODUCTION
The l a r g e h igh- tempera ture gas-cooled r e a c t o r (HTGR) p r e s e n t l y b e i n g
o f f e r e d commercially by Gulf Genera l Atomic I n c o r p o r a t e d i s t h e r e s u l t
of o v e r a decade of development i n t h e b a s i c technology of gas-cooled
r e a c t o r s and i n t h e d e s i g n and p r o o f - t e s t i n g of t h e components which w i l l
b e used i n t h e p l a n t t o g e n e r a t e h i g h - q u a l i t y steam f o r e lec t r ica l power
g e n e r a t i o n .
(40-MW(e)) p l a n t and from t h e d e s i g n , l i c e n s i n g , and c o n s t r u c t i o n of t h e
The e x p e r i e n c e ga ined from t h e o p e r a t i o n of t h e Peach Bottom
195
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F o r t S t . V r a i n (330-MW(e)) p l a n t h a s provided t h e guidance f o r systen; and
component d e s i g n f o r t h e l a r g e HTGR n u c l e a r steam supply system.
p r e l i m i n a r y d i s c u s s i o n s have been h e i d w i t h t h e Uni ted States l i c e n s i n g
a u t h o r i t i e s on t h e d e s i g n of t h e p l a n t . T h e i r review h a s been h e l p f u l
i n e s t a b l i s h i n g t h e d e s i g n b a s e s f o r t h e engineered s a f e t y f e a t u r e s and
i n p r o v i d i n g a s s u r a n c e t h a t t h e d e s i g n can b e s u c c e s s f u l l y engineered
and l i c e n s e d and s a f e l y o p e r a t e d .
containment b u i l d i n g and a u x i l i a r y c o o l i n g loops, as a r e s u l t of t h e
d i s c u s s i o n s w i t h t h e l i c e n s i n g a u t h o r i t i e s , i s expected t o b e a major
f a c t o r i n e a s i n g l i c e n s i n g d i f f i c u l t i e s .
Moreover,
The u s e of a c o n v e n t i o n a l secondary
NUCLEAR STEAM SUPPLY DESCRIPTION
The HTGR nuclear s t e a m supply system (NSS) i s p r e s e n t l y des igned t o
produce main s u p e r h e a t e d steam a t 955°F and 2400 p s i g and r e h e a t steam a t
1001°F and 575 p s i g i n s u f f i c i e n t q u a n t i t i e s t o g e n e r a t e 1100 MW(e) i n a
c o n v e n t i o n a l r e h e a t steam t u r b i n e - g e n e r a t o r u n i t . F i g u r e 1 i s a schemat ic
f low diagram f o r t h e p l a n t . Helium a t a p r e s s u r e of 685 p s i g i s c i r c u l a t e d
by means of s team-turb ine-dr iven a x i a l compressors downward through t h e
r e a c t o r c o r e and upward through t h e once-through steam g e n e r a t o r s . S i x
loops are u s e d , each loop having a s i n g l e hel ium c i r c u l a t o r u n i t and a
s i n g l e steam g e n e r a t o r u n i t . The main s u p e r h e a t e d steam p a s s e s t o t h e
h i g h - p r e s s u r e element of t h e t u r b i n e . The h igh-pressure t u r b i n e exhaus t
i s used t o d r i v e t h e hel ium c i r c u l a t o r s b e f o r e p a s s i n g f i r s t t o t h e r e h e a t
s e c t i o n s of t h e steam g e n e r a t o r s and t h e n t o t h e i n t e r m e d i a t e - p r e s s u r e and
low-pressure s e c t i o n s of t h e main t u r b i n e .
The pr imary c o o l a n t he l ium i s h e a t e d from 630" t o 1377°F mixed mean
i n p a s s i n g through t h e r e a c t o r c o r e . The p r e s s u r e drop i n t h e e n t i r e pr imary
c o o l a n t c i r c u i t i s approximate ly 15.25 p s i , about h a l f of which t a k e s p l a c e
through t h e r e a c t o r c o r e .
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F i g u r e 2 shows t h e g e n e r a l arrangement of t h e major components of t h e
NSS w i t h i n t h e p r e s t r e s s e d c o n c r e t e r e a c t o r vessel (PCRV). The r e a c t o r
c o r e , r e f l e c t o r , c o n t r o l r o d s , and i n t e r n a l s t r u c t u r e s occupy t h e c e n t r a l
c a v i t y , which i s about 37 f t i n d i a m e t e r by 44 f t h i g h . The s i x s e p a r a t e
main c o o l i n g loops occupy 13-f t -diameter cav i t ies which are spaced
symmetr ica l ly around t h e c e n t r a l c a v i t y and connected t o i t by i n s u l a t e d
r a d i a l d u c t s . The PCRV i s a r i g h t c y l i n d e r , 81 f t h igh by 96 f t 6 i n . i n
d i a m e t e r . P r o c e s s and service c o n n e c t i o n s t o t h e steam g e n e r a t o r u n i t s
are made through p e n e t r a t i o n s a t t h e bottom of t h e PCRV, and c o n n e c t i o n s
t o t h e c i r c u l a t o r s a re made a t t h e top . C o n t r o l rod d r i v e a s s e m b l i e s are
mounted i n t h e 73 r e f u e l i n g p e n e t r a t i o n s i n t h e t o p head, where a d d i t i o n a l
p e n e t r a t i o n s a re a l s o provided f o r he l ium p u r i f i c a t i o n system components
and n u c l e a r i n s t r u m e n t s . Three a d d i t i o n a l cav i t ies approximate ly 7 f t
i n d iameter w i t h p e n e t r a t i o n s i n t h e t o p head a re provided f o r t h e a u x i l i a r y
c i r c u l a t o r s and h e a t exchangers which are used t o s a t i s f y t h e emergency
c o o l i n g requi rements f o r t h e r e a c t o r .
0
-
P r e s t r e s s e d Concre te Reac tor Vessel
The PCRV f u n c t i o n s as t h e pr imary c o o l a n t sys-tem boundary. The complete
PCRV c o n s i s t s of (1) a n i n t e r n a l s t e e l l i n e r which acts as a s e a l i n g
membrane, ( 2 ) a thermal b a r r i e r mounted on t h e i n s i d e of t h e l i n e r and a c o o l i n g c o i l system a t t a c h e d t o t h e o u t s i d e of t h e l i n e r whose j o i n t
f u n c t i o n i s t o l i m i t t h e tempera ture of t h e c o n c r e t e , ( 3 ) p e n e t r a t i o n s and
c l o s u r e s which p r o v i d e access t o t h e vessel cav i t i e s , and ( 4 ) h i g h - s t r e n g t h
c o n c r e t e w i t h bonded r e i n f o r c e m e n t s t e e l and a p r e s t r e s s i n g system t o
p r o v i d e s t r e n g t h .
anchored t o t h e f o u n d a t i o n pad.
The e n t i r e assembly i s mounted on a s u p p o r t s t r u c t u r e
The PCRV f o r t h e l a r g e HTGR h a s a d i f f e r e n t c o n f i g u r a t i o n t h a n t h e F o r t
S t . V r a i n vessel . The m u l t i c a v i t y d e s i g n and t h e r a d i a l l o c a t i o n of t h e
steam g e n e r a t o r s and c i r c u l a t o r s are d e s i g n improvements which r e s u l t i n
b e t t e r loop s e p a r a t i o n and a n improved c a p a b i l i t y f o r t h e removal, i f
n e c e s s a r y , of t h e steam g e n e r a t o r s and c i r c u l a t o r s f o r maintenance and
r e p a i r . 0 The m u l t i c a v i t y d e s i g n a l s o r e s u l t s i n a s h o r t e r PCRV, which y i e l d s
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a n improved c a p a b i l i t y t o w i t h s t a n d a c c e l e r a t i o n s due t o ear thquakes .
The l a r g e HTGR i n c o r p o r a t e s s i n g l e c l o s u r e s on t h e PCRV p e n e t r a t i o n s
w i t h f low r e s t r i c t i o n d e v i c e s i n o r d e r t o l i m i t t h e r a t e of d e p r e s s u r i z a t i o n
of t h e PCRV f o r t h e h y p o t h e t i c a l c l o s u r e f a i l u r e a c c i d e n t . The s t r u c t u r a l l y
s e p a r a t e containment b u i l d i n g p r o v i d e s t h e secondary containment f o r t h e l a r g e
HTGR, whereas t h e containment f o r t h e F o r t S t . V r a i n p l a n t i s provided by
secondary c l o s u r e s on every p e n e t r a t i o n . This p a r t i c u l a r d e s i g n change
r e s u l t e d from d i s c u s s i o n s w i t h t h e l i c e n s i n g a u t h o r i t i e s which l e d t o
i n t h e requi rement t o c o n s i d e r t h e double c l o s u r e f a i l u r e as a d e s i g n b a s i s
a c c i d e n t . It t h u s became a p p a r e n t t h a t t h e c o n t r o l of r a d i o a c t i v i t y
releases t o t h e s i t e boundary under t h e assumed a c c i d e n t c o n d i t i o n s could
b e accomplished more economical ly i f a secondary containment s t r u c t u r e
w a s added.
'
The PCRV i t s e l f i s v e r y s i m i l a r t o t h e H a r t l e p o o l vessel b e i n g c o n s t r u c t e d
by T a y l o r Woodrow C o n s t r u c t i o n i n Great B r i t a i n . L i n e a r tendons are used
f o r v e r t i c a l p r e s t r e s s and wire winding i s used f o r t h e c i r c u m f e r e n t i a l
p r e s t r e s s . Work sponsored by Gulf Genera l Atomic i s under way t o deve lop
and p r o o f - t e s t t h e machinery r e q u i r e d t o perform t h e w i r e winding o p e r a t i o n .
The u s e of w i r e winding r e p r e s e n t s a s i g n i f i c a n t improvement over t h e
l i n e a r c i r c u m f e r e n t i a l p r e s t r e s s i n t h a t c o n s i d e r a b l e r e l i e f i s o b t a i n e d
i n embedment c o n g e s t i o n and i n t h e c o m p l e x i t i e s a s s o c i a t e d w i t h p i l a s t e r s
f o r t h e c i r c u m f e r e n t i a l p r e s t r e s s anchors . Moreover, t h e p r e s e n t d e s i g n
does n o t i n c o r p o r a t e head tendons, s i n c e s u f f i c i e n t p r e s t r e s s t o t h e top
and bottom heads of t h e vessel can b e a p p l i e d by t h e c i r c u m f e r e n t i a l
p r e s t r e s s i n g o p e r a t i o n .
S i n c e b o t h t h e steam g e n e r a t o r and t h e c i r c u l a t o r a re i n s t a l l e d through
t h e same p e n e t r a t i o n , a c o n c r e t e p l u g i s used i n t h e upper end of each
steam g e n e r a t o r c a v i t y as a means of reducing t h e p e n e t r a t i o n d iameter
t o t h a t r e q u i r e d f o r t h e c i r c u l a t o r a f t e r t h e steam g e n e r a t o r h a s been
i n s t a l l e d . These p l u g s are b o l t e d t o t h e top of t h e steam g e n e r a t o r
p e n e t r a t i o n l i n e r s and have a c e n t r a l h o l e through which t h e c i r c u l a t o r
assembly i s i n s t a l l e d . A
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Steam Generators
The once-through steam gene ra to r s f o r t h e l a r g e HTGR are gene ra l ly
l a r g e r ve r s ions of the For t S t . Vrain modules. Each of t h e s i x u n i t s i s
approximately a f a c t o r of s i x l a r g e r i n weight and hea t ou tput per module.
F igure 3 i s a schematic diagram of an i n s t a l l e d u n i t . Helium e n t e r s t h e
u n i t a t t h e bottom and flows upward through a U-tube r e h e a t e r l oca t ed i n
t h e c e n t e r duc t . The flow i s reversed a t t h e top of t h e u n i t , and t h e
helium then flows downward over t h e h e l i c a l l y c o i l e d superheater-evaporator-
economizer bundles. A t t he bottom of t h e u n i t , t h e flow i s aga in reversed ,
and t h e helium flows upward i n t h e annular reg ion between t h e steam generator
shroud and t h e cover p l a t e s on t h e i n s u l a t i o n f o r t h e steam genera tor c a v i t y
l i n e r . Uphi l l -bo i l ing i n t h e main steam s e c t i o n has been r e t a i n e d i n t h e
design, and t h e d i f f e r e n c e between t h e l a r g e HTGR steam genera tor and t h e
smaller F o r t S t . Vrain module conf igu ra t ions is t h e d i r e c t r e s u l t of t h i s
des ign dec i s ion . Downhill-boiling w a s considered i n earlier conceptual
des igns bu t w a s no t used owing t o concern over flow s t a b i l i t y a t low power.
A s i g n i f i c a n t design s i m p l i f i c a t i o n w a s made i n t h e method of headering
t h e feedwater and steam tubes a t t h e steam genera tor pene t r a t ion . The F o r t
S t . Vrain steam gene ra to r s have a domed primary c losu re .
h e a t e r subheaders pass through t h i s c l o s u r e , a re co i l ed through the i n t e r s p a c e , and then p a s s through t h e secondary c l o s u r e t o r ingheaders mounted outside
of the pene t r a t ion .
p ipe arrangement i n t h e c e n t e r of each c l o s u r e . The l a r g e HTGR uses
tubeshee ts f o r headering t h e feedwater and a l l of t h e steam tubes.
tubeshee ts form p a r t of t h e c:Losure f o r t h e steam genera tor pene t r a t ion .
I n a d d i t i o n t o t h e helium flow r e s t r i c t o r s i n each p e n e t r a t i o n which provide
t h e flow r e s t r i c t i o n necessary t o l i m i t t h e hypo the t i ca l PCRV depressur iza-
t i o n acc iden t , f low r e s t r i c t o r s are a l s o provided t o l i m i t t h e i n g r e s s of
steamlwater i n t o t h e r e a c t o r :€or a h y p o t h e t i c a l tubeshee t f a i l u r e .
Feedwater and super-
Reheat steam i n l e t and o u t l e t are through a concen t r i c
These
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Direct access f o r t u b e p lugging o p e r a t i o n s is provided by t h i s d e s i g n
s i m p l i f i c a t i o n .
shutdown by removing s e c t i o n s of t h e p i p i n g below t h e t u b e s h e e t s , manually
p lugging t h e l e a k i n g c i r c u i t s , and t h e n r e p l a c i n g t h e p i p e s e c t i o n s .
These o p e r a t i o n s would b e accomplished d u r i n g a p l a n t
The materials used i n t h e steam g e n e r a t o r s range from carbon s t e e l
t o n i c k e l - b a s e a l l o y .
items such as t h e feedwater t u b e s h e e t and t h e feedwater t u b e s . Var ious
grades of low-al loy s t e e l a re used f o r t h e c l o s u r e , t h e co ld r e h e a t t u b e s h e e t ,
p o r t i o n s of t h e shroud, and t h e economizer-evaporator t u b e s and t h e i r s u p p o r t
s t r u c t u r e . N i c k e l iron-chrome a l l o y ( Incoloy 800 o r e q u i v a l e n t ) i s used
f o r t h e s u p e r h e a t e r t u b e s , t h e r e h e a t e r t u b e s , and p o r t i o n s of t h e shroud,
and a h i g h - s t r e n g t h n icke l -base a l l o y ( I n c o n e l 625 o r e q u i v a l e n t ) i s
used f o r the supe rhea te r tubeshee t , t h e h o t reheat tubeshee t , and the s u p p o r t
Carbon s t e e l i s used i n t h e low-design-temperature
s t r u c t u r e s f o r t h e s u p e r h e a t e r and r e h e a t e r .
Main Helium C i r c u l a t o r s
The main hel ium c i r c u l a t o r s (shown i n F i g . 4 ) are g e n e r a l l y l a r g e r
v e r s i o n s of t h e F o r t S t . V r a i n s e r i e s - s t e a m - t u r b i n e d r i v e n a x i a l f l o w
u n i t s , w i t h f l o w and power r e q u i r e m e n t s approximate ly double t h o s e of each
of t h e F o r t S t . Vrain c i r c u l a t o r s . The t h r u s t and j o u r n a l b e a r i n g s a r e
w a t e r - l u b r i c a t e d h y d r o s t a t i c b e a r i n g s w i t h hydrodynamic c a p a b i l i t y a t h i g h
speed , similar t o t h o s e i n t h e F o r t S t . V r a i n u n i t s , Owing t o t h e r e a c t o r
arrangement , t h e u n i t s are i n v e r t e d re la t ive t o t h e F o r t S t . V r a i n c i r c u l a t o r s
and t h e he l ium f l o w through t h e compressor i s r e v e r s e d , b u t t h e s e are minor
d e s i g n m o d i f i c a t i o n s . A s h u t o f f valve i s l o c a t e d a t t h e d i s c h a r g e of each
c i r c u l a t o r t o p r e v e n t backflow of hel ium through a shutdown c i r c u l a t o r .
C o n t r o l Rod Drives
F i g u r e 5 shows a c o n t r o l rod d r i v e u n i t i n s t a l l e d i n a r e f u e l i n g
p e n e t r a t i o n . These u n i t s , which a re v e r y similar t o t h e F o r t S t . V r a i n
u n i t s , are e s s e n t i a l l y e l e c t r i c a l l y powered winches, each of which raises
and lowers a p a i r of c o n t r o l r o d s by means of f ’ l e x i b l e s t e e l c a b l e s . The
201
c o n t r o l r o d s are guided i n t o t h e c o r e by a g u i d e t u b e assembly l o c a t e d
i n t h e upper plenum above t h e r e a c t o r c o r e . Scram o c c u r s by g r a v i t y a c t i o n ,
w i t h t h e v e l o c i t y b e i n g c o n t r o l l e d by r e g e n e r a t i v e b r a k i n g a c t i o n of t h e
motor.
Fuel. Handling Equipment
R e f u e l i n g o p e r a t i o n s w i l l . b e c a r r i e d o u t w i t h t h e p l a n t o f f - l i n e and
w i t h t h e r e a c t o r he l ium i n l e t t empera ture and p r e s s u r e lower t h a n 250°F
and a tmospher ic , r e s p e c t i v e l y . The p r i n c i p a l equipment (shown i n F i g . 6 ) c o n s i s t s of a f u e l h a n d l i n g machine f o r a c t u a l l y removing and r e p l a c i n g f u e l
and r e f l e c t o r e lements i n t h e r e a c t o r ; f u e l t r a n s f e r c a s k s f o r t r a n s f e r r i n g
canned e lements between t h e f u e l h a n d l i n g machine and s t o r a g e ; a n a u x i l i a r y
service c a s k f o r removing and i n s t a l l i n g c o n t r o l rod d r i v e a s s e m b l i e s b e f o r e
and a f t e r r e f u e l i n g ; r e a c t o r i s o l a t i o n valves t o p r o v i d e s h i e l d i n g and s e a l i n g
f o r t h e r e f u e l i n g p e n e t r a t i o n s d u r i n g t h e r e f u e l i n g o p e r a t i o n ; and motorized
v e h i c l e s f o r t r a n s p o r t i n g t h e f u e l t r a n s f e r c a s k s between t h e f u e l h a n d l i n g
machine and s t o r a g e .
The i n - c o r e o p e r a t i o n s are i d e n t i c a l t o t h o s e f o r t h e F o r t S t . Vrain
r e a c t o r ; i . e . , a complete s e v e n column r e f u e l i n g r e g i o n i s r e f u e l e d a t any
one t i m e . However, t h e F o r t S t . V r a i n r e f u e l i n g machine i t s e l f t e m p o r a r i l y
s t o r e s t h e f u e l and r e f l e c t o r e lements and i s moved to the location of the
f u e l s t o r a g e t o d e p o s i t t h e s p e n t f u e l and r e l o a d w i t h new f u e l . This t y p e
of o p e r a t i o n w a s p r o h i b i t e d i n t h e c o n v e n t i o n a l l y c o n t a i n e d p l a n t u n l e s s a
v e r y l a r g e access door w a s provided between t h e containment and t h e r e a c t o r
service b u i l d i n g . Moreover, it was found t h a t t h e r e f u e l i n g t i m e could b e
s h o r t e n e d c o n s i d e r a b l y i f t h e r e f u e l i n g machine w a s n o t moved and f u e l w a s
t r a n s p o r t e d by t h e t r a n s f e r c a s k s and motor ized v e h i c l e s .
The r e f u e l i n g c y c l e i s based on a 4-yr l i f e ; i . e . , one-quar te r of t h e
c o r e i s r e p l a c e d each y e a r by new o r r e c y c l e d f u e l .
time r e q u i r e d f o r t h e r e f u e l i n g o p e r a t i o n i s e s t i m a t e d t o b e a b o u t 1 4 d a y s ,
i n c l u d i n g t h e t i m e r e q u i r e d f o r pump-down and cool-down of t h e r e a c t o r
The r e a c t o r shutdown
0 and t h e t i m e r e q u i r e d f o r pump-up and r e a c t o r s t a r t u p .
202
R e a c t o r Core
The r e a c t o r c o r e (shown i n F i g . 7 ) c o n s i s t s of approximate ly 3800
hexagonal g r a p h i t e b l o c k f u e l elements of t h e same b a s i c t y p e as w i l l b e
used i n t h e F o r t S t . V r a i n p l a n t ; i . e . , e lement o v e r a l l dimensions are
approximate ly 31 i n . l o n g and 1 4 i n . a c r o s s t h e f l a t s . The g r a p h i t e f u e l
e lements are a r r a n g e d i n columns e i g h t b l o c k s h i g h and are surrounded by a
g r a p h i t e r e f l e c t o r approximate ly 4 f t t h i c k . The c o r e i t s e l f i s d i v i d e d
i n t o 73 r e g i o n s , each c o n s i s t i n g of a c e n t r a l f u e l element column surrounded
by up t o s i x columns. Edch c e n t r a l f u e l e lement column c o n t a i n s t h e ve r t i ca l
h o l e s f o r t h e a s s o c i a t e d c o n t r o l r o d p a i r and a h o l e f o r t h e i n s e r t i o n of
t h e reserve shutdown material .
Convent iona l nuc lear -grade g r a p h i t e w i l l b e used throughout t h e c o r e .
The f u e l materials i n t h e i n i t i a l c o r e w i l l b e 93% e n r i c h e d uranium and
f e r t i l e thorium i n c a r b i d e form. I n t h e l a te r r e c y c l e mode, U-233 w i l l b e
i n c l u d e d as a f e e d material , r e p l a c i n g much of t h e U-235. The uranium and
thorium c a r b i d e p a r t i c l e s a re c o a t e d w i t h l a y e r s of p y r o l y t i c carbon and
bonded i n t o r o d s b e f o r e b e i n g loaded i n t o t h e g r a p h i t e e lements .
Apar t from d i f f e r e n c e s i n l o a d i n g s , t h e major d i f f e r e n c e between t h e
l a r g e HTGR f u e l and F o r t S t . V r a i n f u e l i s i n t h e c o a t i n g s . I n o r d e r t o
minimize t h e accumulat ion of Sr-90 as p l a t e o u t i n t h e c i r c u i t , which
would o t h e r w i s e b e p o t e n t i a l l y r e l e a s a b l e i n t h e h y p o t h e t i c a l depres-
s u r i z a t i o n a c c i d e n t , a l l t h e F o r t S t . Vra in f u e l p a r t i c l e s have an
added l a y e r of s i l i c o n c a r b i d e . The a d d i t i o n of c o n v e n t i o n a l containment
on the l a r g e HTGR p l a n t h a s r e l i e v e d t h i s release problem. However, i n t h e
l a r g e HTGR c e r t a i n U-235 f u e l p a r t i c l e s a l s o have a s i l i c o n c a r b i d e c o a t i n g
t o f a c i l i t a t e s e p a r a t i o n d u r i n g r e p r o c e s s i n g o p e r a t i o n s .
A u x i l i a r y Cooling Loops
Three a u x i l i a r y c o o l i n g l o o p s have been provided i n t h e NSS f o r t h e
l a r g e HTGR. Each loop c o n s i s t s of a hel ium c i r c u l a t o r , a water-cooled
203
o p e r a t i n g c o n d i t i o n s , i n c l u d i n g a
f u l l i n v e n t o r y p r e s s u r e and
h e a t exchanger , and t h e i r a s s o c i a t e d service equipment. F i g u r e 8 shows one
of t h e l o o p s i n s t a l l e d i n t h e PCRV c a v i t y .
i s t o p r o v i d e emergency c o r e c o o l i n g and decay h e a t removal i n case of
f a i l u r e of t h e main loops . Any two loops can c o o l t h e c o r e .
The pr imary f u n c t i o n of t h e loops
c o r e c a v i t y p r e s s u r e anywhere between t h e
a tmospher ic . O i l - l u b r i c a t e d b a l l b e a r i n g s are
The requi rement f o r t h e s e a u x i l i a r y c o o l i n g l o o p s was a consequence of
d i s c u s s i o n s w i t h t h e l i c e n s i n g a u t h o r i t i e s and t e c h n i c a l d i f f i c u l t i e s i n
p r o v i d i n g a d e q u a t e s t a t i c c o o l i n g f o r t h e l a r g e HTGR c o r e i n a manner s i m i l a r
t o t h a t p rovided f o r t h e F o r t S t . V r a i n c o r e . F a i l u r e of b o t h t h e steam
d r i v e s and t h e water t u r b i n e d r i v e s on a l l t h e F o r t S t . V r a i n c i r c u l a t o r s
r e s u l t s i n t h e h y p o t h e t i c a l l o s s of f o r c e d c i r c u l a t i o n a c c i d e n t w i t h t h e
decay h e a t b e i n g removed by r a d i a t i o n and conduct ion t o t h e l i n e r c o o l i n g
system. Although h i g h tempera tures are reached i n t h e c o r e of t h e F o r t S t .
V r a i n r e a c t o r d u r i n g t h e c o u r s e of t h i s h y p o t h e t i c a l e v e n t , t h e r e a c t o r can
r i d e through t h e long term h e a t u p and cooldown w i t h o u t v i o l a t i n g t h e containment
provided by t h e PCRV.
system of t h e l a r g e HTGR i s more d i f f i c u l t s imply because of t h e l o n g e r
r a d i a t i o n and conduct ion p a t h s . Higher tempera tures would b e a t t a i n e d i f a
s imilar l o s s of a l l f o r c e d c i r c u l a t i o n a c c i d e n t i s h y p o t h e s i z e d . Attempts
t o a s s u r e s a f e t y by some means of s t a t i c c o r e c o o l i n g d i d n o t prove sa t i s -
f a c t o r y , and as a r e s u l t a n a d d i t i o n a l method of p r o v i d i n g f o r c e d c o o l i n g
w a s adopted.
However, removal of a f t e r h e a t by t h e l i n e r c o o l i n g
c i r c u l a t o r s are o p e r a t i n g .
204
ENGINEERED SAFEGUARDS AND SAFETY PHILOSOPHY
The e v o l u t i o n of t h e l a r g e HTGR d e s i g n h a s r e s u l t e d i n two major changes
i n t h e engineered s a f e g u a r d s systems:
1. The a d d i t i o n of a s e p a r a t e c o n v e n t i o n a l containment b u i l d i n g t o
p r o v i d e g r e a t e r p h y s i c a l s e p a r a t i o n between t h e pr imary and
secondary conta inments .
2. The i n c o r p o r a t i o n of a u x i l i a r y c o o l i n g loops t o p r o v i d e emergency
c o r e c o o l i n g i n case of f a i l u r e of t h e main c i r c u l a t o r / h e a t removal
system.
A s noted p r e v i o u s l y , t h e acceptance of a hypo the t i ca l d e p r e s s u r i z a t i o n
of t h e PCRV as a d e s i g n b a s i s was t h e pr imary r e a s o n f o r t h e a d d i t i o n of t h e s e p a r a t e containment b u i l d i n g .
l i m i t f o r t h e r a t e of d e p r e s s u r i z a t i o n , t h e h y p o t h e t i c a l a c c i d e n t i s assumed
t o occur through a p e n e t r a t i o n i n t h e PCRV a f t e r f a i l u r e of t h e c l o s u r e ,
w i t h t h e subsequent d e p r e s s u r i z a t i o n r a t e b e i n g determined by t h e f r e e - f l o w
area around a f l o w r e s t r i c t o r i n t h e p e n e t r a t i o n .
r e s t r i c t o r s are engineered s a f e t y f e a t u r e s and have t h e c a p a b i l i t y of
I n o r d e r t o p r o v i d e a n a c c e p t a b l e upper
The p e n e t r a t i o n f low
L l i m i t i n g t h e e f f e c t i v e f ree- f low area t o a maximum of 100 i n . F i g u r e 9 shows t h e tempera ture and p r e s s u r e p u l s e i n t h e containment which would occur
d u r i n g t h i s e v e n t . Since t h e energy c o n t e n t of t h e s ing le-phase hel ium
c o o l a n t i s s o s m a l l , a s e p a r a t e h e a t removal sys tem i n t h e containment i s
n o t n e c e s s a r y ; t h e h e a t c o n t e n t of t h e hel ium i s removed by t r a n s f e r t o
t h e c o o l e r s u r f a c e s of t h e containment and i t s c o n t e n t s .
The f u n c t i o n of t h e a u x i l i a r y c o o l i n g l o o p s , which a re a l s o engineered
s a f e t y f e a t u r e s , i s t o p r o v i d e a d e q u a t e removal of t h e decay h e a t from t h e
c o r e f o l l o w i n g t h e d e s i g n b a s i s d e p r e s s u r i z a t i o n a c c i d e n t . The main c o o l i n g
loops are n o t c o n s i d e r e d t o b e engineered s a f e t y f e a t u r e s ; however, t h e y a l s o
have t h e c a p a b i l i t y of removing t h e decay h e a t and a d e q u a t e l y c o o l i n g t h e
r e a c t o r c o r e .
205
The e v o l u t i o n of t h e s a f e t y phi losophy f o r t h e NSS h a s a l s o l e d t o
c o n s i d e r a t i o n of t h e p o s s i b i l i t y of some a d d i t i o n a l i n p u t t o t h e d e s i g n
b a s i s a c c i d e n t from small l e a k s i n t h e secondary c o o l a n t system. It i s
becoming common p r a c t i c e t o c o n s i d e r s u i t a b l e d e s i g n margins f o r such a n
e v e n t i n t h e l i c e n s i n g of power r e a c t o r s . For t h e HTGR, t h e p o s s i b i l i t y of
steam/water i n g r e s s i n t o t h e r e a c t o r c o i n c i d e n t w i t h o r subsequent t o t h e
d e p r e s s u r i z a t i o n a c c i d e n t does r e q u i r e t h e a d d i t i o n a l engineered s a f e t y
f e a t u r e s . U n t i l a l l s e c t i o n s of t h e r e a c t o r c o r e are cooled t o below t h e
t h r e s h o l d f o r t h e s team-graphi te chemica l r e a c t i o n , some hydrogen and carbon
monoxide w i l l b e g e n e r a t e d . I t i s n e c e s s a r y t o p r o v i d e a d e q u a t e moni tor ing
f o r m o i s t u r e i n t h e system and s u i t a b l e i s o l a t i o n d e v i c e s t o l i m i t t h e amount
of steam/water i n g r e s s t o less t h a n t h a t which could l e a d t o p o t e n t i a l l y
flammable m i x t u r e s of hydrogen and carbon monoxide i n t h e a i r - f i l l e d c o n t a i n -
ment. The m o i s t u r e moni tor ing d e v i c e s and t h e i s o l a t i o n systems f o r s o u r c e s
of l a r g e steam/water l e a k s have t h e r e f o r e a l s o been c l a s s e d as engineered
s a f e t y f e a t u r e s f o r t h e l a r g e HTGR.
SUMMARY
T h i s paper h a s covered only t h e h i g h l i g h t s of t h e NSS f o r t h e l a r g e HTGR.
S u f f i c i e n t d e s i g n and development work h a s been done on t h e d e s i g n f o r Gulf
General Atomic t o now o f f e r t h e n u c l e a r steam supply f o r t h e g e n e r a t i o n of
base load electrical power in 1100-MW(e) units on a commercial basis. The
HTGR's p o t e n t i a l f o r improved performance i n terms of h i g h e r p l a n t e f f i c i e n c y ,
reduced r a d i o a c t i v e and thermal e f f l u e n t , and less s t r i n g e n t f u e l r e q u i r e -
ments i s r a p i d l y approaching r e a l i z a t i o n i n t h e 1100-MW(e) d e s i g n .
F i g u r e 10 shows a n o v e r a l l view of t h e 1100-MW(e) HTGR power p l a n t .
Design c r i t e r i a have been e s t a b l i s h e d f o r t h e major sys tems and components
i n t h e p l a n t , and work on t h e d e t a i l e d d e s i g n i s proceeding .
containment s t r u c t u r e s u r r o u n d i n g t h e PCRV i s a c a r b o n - s t e e l - l i n e d conven-
t i o n a l l y r e i n f o r c e d c o n c r e t e s t r u c t u r e w i t h c y l i n d r i c a l walls, a f l a t b a s e ,
and a h e m i s p h e r i c a l dome.
d i a m e t e r about 126 f t .
The secondary
Its o v e r a l l h e i g h t i s about 230 f t and i t s i n s i d e
A minimum c l e a r a n c e of approximate ly 8 f t i s main ta ined
206
around t h e PCRV t o permi t p o s t - t e n s i o n i n g of t h e c i r c u m f e r e n t i a l w i r e wrappi@
Access t o t h e containment b u i l d i n g i s provided by a 7-f t -diameter p e r s o n n e l
h a t c h and a 22-f t -diameter equipment h a t c h .
The r e a c t o r service b u i l d i n g c o n t a i n s t h e new and used f u e l s t o r a g e
f a c i l i t i e s and t h e r e a c t o r a u x i l i a r y systems and i s approximate ly 90 f t
wide, 130 f t long , and 172 f t h i g h . The t h r e e - s t o r y t u r b i n e b u i l d i n g i s
approximate ly 136 f t wide, 300 f t l o n g , and 102 f t h i g h .
207
CIRCUMFERENTIAL PRESTRESS CHANNELS-
Fig. 1. Schemat ic Flow Diagram of NSS for Large HTGR.
-REFUELING PENETRATION nous CONTROL I NG ROO
MECHANISM
-CIRCULATOR
N J X l L IARY CIRCULATOR'
CORE AUYIL I ARY HEAT EXCHANGERc
PRESTRESSED' CONCRETE PRESSURE VESSEL-
\
F i g . 2 . General Arrangement of Large HTGR.
- V E R T I C A L PRESTRESS 1 END 0 N S
* S T E M GENERATOR
COLD H E L l
E C O N O M I Z E R - EVAPORATOR SUPERHEATER BUNDLE
HOT H E L l
' FEEDWATER
COLD REHEAT S T E A M
M A I N S T E A M
REHEATER B U N D L E
, PCRV
PR l MARY CLOSURE
Fig. 4. Helium Circulator Installation Assembly.
Fig' Q Steam Generator Installation. ' HOT R E H E A T S T E A M
Fig. 5. Cont ro l Rod Drive and Reserve Shutdown Assembly.
Fig. 6. Fuel Handling Equipment.
A U X I L I A R Y C I R C U L A T O R SHUTOFF V A L V E
PCRV\
C O R E + /ue COOLANT FLOW REMOVABLE P E R M A N E N T REFLECTOR REFLECTOR. - -- --- 1 . - - - - "%a-*t- -_-- -.- ..-"-- *___- --- "
Fig. 7 . Core Arrangement.
. A U X I L I A R Y C I R C U L A T O R
.D
. I UM
CORE A U X l L l ARY H E A T EXCHANGER
I UM
Lng Lo p s .
211
-
PHERE PRESSURE E I E N T S FROM A PCRV
- BLOWDOWN AREA OF 100 SQ. I N . POST-SCRAM C O O L I N G BY TWO A U X I L I A R Y LOOPS
h
U - a 30
CONTAINMENT VOLUME OF 1 . 7 X I O 6 CU F T - ln -.
v
-
-
I I 1
500
400 0 v
W CT 3
300 5 cc W a E k
200 U U cc W >
100
0
Fig . 9. Containment Pressure and Temperature Tran- sients during Design Basis PCRV Accident in 1100-MW(e) H E R with Concurrent Steam Leak.
212
DISCUSSION
D. Tytgat: What l e d you t o t h e choice of a secondary containment v e s s e l ? Was it t h e u n r e l i a b i l i t y of the secondary closures of the l a r g e penetrations o r t h e general s a f e t y philosophy adopted i n the USA f o r l a r g e water reac tors ?
A. J. Goodjohn: After severa l discussions with l icensing authori- ties, it became apparent that a rapid depressurization of the PCRV could be considered as a design bas is accident f o r the concept. Moreover, it a l s o became apparent t h a t the general public would r a i s e several concerns over a plant without the secondary containment independent of any safe ty arguments on the very low probabi l i ty of PCRV failure. adopted secondary containment by means of a conventional containment bui lding i n order t o satisfy the general s a f e t y philosophy adopted i n the
United S ta tes and not because o f any concern over the r e l i a b i l i t y of the
secondary closures on the l a r g e penetrations,
Therefore, GGA
G. Meijer: One of the major differences between the GGA design f o r a 1100 Mwe HTGR and t h e "PG HTGR design i s t h a t you a r e designing f o r off-load re fue l ing and TNPG f o r on-load refuel ing. Therefore, there ap-
pears t o be no p a r t i c u l a r reason f o r having a downflow i n the GGA reac- t o r . It appears t h a t w i t h an upflow i n the core the steam generator de-
s ign would have been simplified, i .e . , cheaper - and a l s o the core sup- port would have been cheaper. Therefore, I am in te res ted t o l e a r n what
made you decide on a downward cooled core; i s t h i s because of pressure drop or because of o ther reasons?
A. J. Goodjohn: We decided t o s t a y w i t h downflow through the core f o r the following reasons: A. The p o s s i b i l i t y of going t o on-line re- fuel ing on a fu ture p lan t improvement, B. Fort St . Vrain has downflow and t h e developnent of t h e control rod dr ives and the thermal insu la t ion have been based on t h i s arrangement. We would have t o develop a control rod dr ive f o r ho t hel iun (cable problem) and redo much of our insu la t ion
work.
213
D. Pa t te rson: You assume a 100 sq in . opening f o r t he design b a s i c
acc ident . What determined t h e s i z e of t h i s assumed fai lure?
A. J. Goodjohn: The 100 sq in . opening i n a pene t r a t ion as a design
b a s i s f o r t h e hypoteht ica l dep res su r i za t ion acc ident i s g r e a t e r than t h e
s i ze of opening which one obta ins by design of flow r e s t r i c t o r devices
(approximately 30 t o 50 sq i n . f o r l a r g e pene t r a t ions ) and smaller than
t h e s i z e of t h e opening which could result i n secondary e f f e c t s i n the
primary c i r c u i t ; i . e . , fa i lure of i n t e r n a l seals or duct work. The li- censing a u t h o r i t i e s agreed with t h i s design b a s i s f o r For t S t . Vrain.
T. A. Jaeger : My ques t ion refers t o the design of t h e concrete pres-
sure vesse l . You s t a t e d t h a t t h e c i rcumferent ia l w i r e winding p r e s t r e s s -
i n g provides adequate p r e s t r e s s i n g of t h e v e s s e l cap. I n t h i s way t h e
cap i s t ak ing t h e load e n t i r e l y by a rch ing a c t i o n which may imply a sudden
mode of fa i lure . f o r t h e design of t he cap a s compared with t h e c y l i n d r i c a l wall?
What i s your philosophy with regard t o s a f e t y margins
A. J. Goodjohn: By applying s u f f i c i e n t c i rcumferent ia l p r e s t r e s s t o
t h e head one can a s su re s u f f i c i e n t s t r e n g t h i n the h e a d , t o y i e l d as g r e a t
a s a f e t y margin a g a i n s t overpressure blowout of t h e head as aga ins t f l e x -
ural fa i lure of t he s i d e w a l l . One, i n f a c t , designs t h e p r e s t r e s s s o t h a t ultimate failure mode a t very high pressures i s p red ic t ab le and i s
not head fa i lure or s i d e w a l l fa i lure but fa i lure a t t h e haunch between the head and the s ide w a l l . The model tes ts have proven t h i s concept.
R. E. Helms: Most large f o s s i l p l a n t s i n t h e U.S. use t h e super-
c r i t i c a l steam cycle 3500 psia/1000"F/1000"F.
s e l e c t i n g the s u b c r i t i c a l steam cycle 2400 psia/1000"F/1000"F?
o f f were made, i f any?
What was GGA's basis f o r
What t r ade -
A. J. Goodjohn: GGA d id eva lua te the s u p e r c r i t i c a l steam cycle f o r
t h e l a r g e HTGR and decided on an economic b a s i s p r imar i ly t o remain wi th
t h e s u b c r i t i c a l s 2400 psia/1000 "F/1000"F cycle.
Paper 5/115
CONCEPTUAL DESIGN FOR A 600 MW, NUCLEAR POWER P U N T ’ WITH H I G H TEMPERATURE REACTOX AND HELIiiM
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I n t h e F e d e r a l R e p u b l i c of Germany a development program f o r a 6 0 0 MWe High Tempera tu re Reactor Power P l a n t w i t h c l o s e d g a s t u r b i n e c y c l e h a s been i n i t i a t e d . The p a p e r describes t h e p r e s e n t s t a t e of the c o n c e p t u a l d e s i g n s t u d i e s .
The a c t i v i t i e s are c o n c e n t r a t e d on t h e l a y o u t of t h e c o m p l e t e p l a n t , deve lopment of f u e l e l e m e n t s f o r h i g h t e m p e r a t u r e s w i t h l o w f i s s i o n p r o d u c t release ra tes , problems of d e p o s i t i o n of f i s s i o n p r o d u c t s , a n d development and t e s t i n g of s p e c i a l components .
The d e c i s i o n c o n c e r n i n g t h e l a y o u t of t h e main components w i l l be made i n 1 9 7 0 , a p r e l i m i n a r y d e c i s i o n o n t h e f u e l e l e m e n t t y p e i n 1 9 7 2 . By 1975 c o m p l e t e c o n s t r u c t i o n documents w i l l be a v a i l a b l e .
.-
+ ) The work h a s been c a r r i e d o u t w i t h i n a c o o p e r a t i o n c o n t r a c t between t h e c o r p o r a t i o n s Brown Bover i / Krupp R e a k t o r b a u G m b H , Brown,Boveri & C i e A G , F r i e d . Krupp GmbH, G u t e h o f f n u n g s h t i t t e S t e r k r a d e A G , M a s c h i n e n f a b r i k Augsburg-Ntirnberg A G , N U K E M , Nuklear-Chemie und -Metallurgic Gmbh and Kern fo r - s c h u n g s a n l a g e J u l i c h GmbH , r e g a r d i n g t h e p r e p a r a t i o n of t h e c o m p l e t e c o n s t r u c t i o n documents f o r a 600 M W e power p l a n t w i t h HTR and h e l i u m t u r b i n e , u n d e r t h e s p o n s o r s h i p of t h e F e d e r a l M i n i s t r y f o r S c i e n t i f i c R e s e a r c h ( I n v . Reactor 6 5 1 .
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I N T R O D U C T I O N
The r a p i d p r o g r e s s i n t h e development o f f u e l e l e m e n t s for h i g h t e m p e r a t u r e r e a c t o r s i n r e c e n t y e a r s h a s p rov ided t h e t e c h n i c a l basis f o r t h e e x p l o i t a t i o n o f t h e h i g h e f f i c i e n c y of t h i s r e a c t o r t y p e , by c o u p l i n g it d i r e c t l y w i t h a he l ium t u r b i n e . Other a d v a n t a g e s a s s o c i a t e d w i t h d i r e c t c o u p l i n g , such as lower s p e c i f i c c a p i t a l c o s t , lower consumption of c o o l a n t water and h i g h e f f i c i e n c y even i n p a r t i a l load o p e r a t i o n , h e l p t o e n s u r e t h a t t h e h i g h t e m p e r a t u r e r e a c t o r w i t h he l ium t u r b i n e w i l l , i n t h e l o n g r u n , t a k e up a f a v o u r a b l e p o s i t i o n a l o n g s i d e fas t b r e e d e r s i n t h e ene rgy p r o d u c t i o n i n d u s t r y .
I n t h e F e d e r a l Repub l i c o f Germany a program has been i n i t i a t e d for t h e development o f a 600 M W e p l a n t . The program is b e i n g c a r r i e d o u t by s e v e r a l companies i n co- o p e r a t i o n w i t h t h e Kernforschungsanlage J u l i c h Gmbh ( K F A ) . For e x p e r i m e n t a t i o n and development up t o t h e s t a g e a t which a n of fe r c a n be p r e s e n t e d , a p p r o x i m a t e l y 1 3 0 Mio DM are a v a i l a b l e . The a c t i v i t i e s a re c o n c e n t r a t e d on t h e l a y o u t of t h e comple te p l a n t , development of f u e l e l e m e n t s f o r h i g h t e m p e r a t u r e s with l o w f i s s i o n p r o d u c t release rates, problems of d e p o s i t i o n o f f i s s i o n p r o d u c t s , and development and t e s t i n g of s p e c i a l components. U s e o f s p h e r i c a l and rod- t y p e f u e l e l e m e n t s are c u r r e n t l y b e i n g i n v e s t i g a t e d i n p a r a l l e l ; however, f i n a l d e s i g n f o r c o n s t r u c t i o n i s ' t o be carried o u t f o r one f u e l e l emen t t y p e o n l y .
D E S I G N A S P E C T S
The a i m of t h e d e s i g n work is t o e s t a b l i s h a n optimum between h i g h e f f i c i e n c y and low c a p i t a l c o s t , fo r a p l a n t t o be b u i l t w i t h i n a few y e a r s .
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I n F i g . 1 l i s t e d , showing a se t of d a t a A f o r t h e minimum o p e r a t i n g cost and a set B f o r t h e minimum c o s t .
t h e b a s i c data f o r t h e p l a n t d e s i g n a re
- The maximum p r o c e s s t e m p e r a t u r e ( g a s t u r b i n e i n l e t ) o f 85OoC w a s selected as a r ea l i s t i c v a l u e w i t h r e g a r d t o t h e p e r m i s s i b l e f u e l e l emen t l o a d , release of f i s s i o n p r o d u c t s and u s e of a v a i l a b l e materials. A t e m p e r a t u r e i n c r e a s e c a n be env i saged r e s u l t i n g i n a h i g h development p o t e n t i a l s i n c e it c a n be d i r e c t l y e x p l o i t e d w i t h t h e a p p l i c a t i o n of g a s t u r b i n e s . A t e m p e r a t u r e i n c r e a s e by 5OoC r e s u l t s for i n s t a n c e i n a n i n c r e a s e of t o t a l e f f i c i e n c y by a p p r o x i m a t e l y 2 p o i n t s and w i l l p robab ly a l l o w a n e s t i m a t e d r e d u c t i o n i n cap i ta l cos t by 2 0 DM/kW i n s t a l l e d power.
- To a c h i e v e a maximum p o s s i b l e s i t e independence a i r c o o l i n g h a s been s e l e c t e d . Under t h e a s sumpt ion t h a t a n i n t e r m e d i a t e c o o l i n g c i r c u i t i s r e q u i r e d for s a f e t y r e a s o n s t h e minimum p r o c e s s t e m p e r a t u r e h a s been chosen t o 35OC. A p o s s i b l e l o w e r i n g of t h i s t e m p e r a t u r e down t o a p p r o x i m a t e l y 2 2 O C by u s i n g r i v e r water f o r r e c o o l i n g would r e s u l t i n a n i n c r e a s e o f t o t a l e f f i c i e n c y by a p p r o x i m a t e l y 2 p o i n t s , which c o r r e s p o n d s t o a n i n c r e a s e of t u r b i n e i n l e t t e m p e r a t u r e by 5OoC.
- A s i m p l e i n t e r c o o l i n g w a s f avoured t o r e d u c e t h e b u i l d i n g volume, and machinery costs . Although doub le i n t e r m e d i a t e c o o l i n g r e s u l t s i n a n i n c r e a s e i n e f f i c i e n c y by a p p r o x i - ma te ly 1 1 / 2 p o i n t s , t h e o v e r a l l economics of t h e power p l a n t however, becomes less f a v o u r a b l e because of t h e h i g h e r c a p i t a l cos t .
- F o r t h e c h o i c e of maximum p r e s s u r e l e v e l - i n t h i s case a p p r o x i m a t e l y 6 0 bar - a compromise had t o be r eached between p l a n t s i z e and costs on t h e one hand and e f f i c i e n c y of t h e t u r b o machinery on t h e o t h e r hand.
0 - The i n v e s t i g a t i o n s of t h i s p r o j e c t are based on t h e u s e of a s i n g l e - s h a f t h o r i z o n t a l l y - a r r a n g e d g a s t u r b i n e p l a n t . A m u l t i - s h a f t a r r angemen t has been exc luded due t o t h e f a c t t h a t it r e s u l t s i n h i g h e r c a p i t a l c o s t s , h a s a more c o m p l i c a t e d l a y o u t and r e q u i r e s a l a r g e r c o n t r o l sys tem. Thus fo r example t u r b i n e compressor u n i t s w i t h v e r t i c a l sha f t c o u l d be deve loped o n l y a t c o n s i d e r a b l e a d d i t i o n a l e x p e n s e s .
- The n e t e f f i c i e n c y of t h e power p l a n t o f 4 2 % w a s de t e rmined on the basLs of these basic d a t a by o p t i m i z a t i o n of t h e t u r b i n e expans ion r a t i o o v e r t h e r e a c t o r i n l e t t e m p e r a t u r e , t h e p r e s s u r e l o s s e s , and t h e h e a t exchanger t e m p e r a t u r e d i f f e r e n t i a l . With d o u b l e i n t e r c o o l i n g and r e c o o l i n g by r i v e r water, p l a n t e f f i c i e n c y i s i n c r e a s e d t o 45,s %. The o v e r a l l economics, however remain a p p r o x i m a t e l y unchanged because o f t h e i n c r e a s e of c a p i t a l c o s t .
SAFETY ASPECTS
The e s s e n t i a l s a f e t y r e q u i r e m e n t s have been de te rmined unde r t h e f o l l o w i n g c o n s i d e r a t i o n s :
- possibility to s h u t down t h e reactor
- removal of decay h e a t - r a d i a t i o n dose i n normal o p e r a t i o n and i n
f a u l t c o n d i t i o n s .
The most s e r i o u s problem r e g a r d i n g shut-down of t h e reactor i s t h e " lo s s of c o o l a n t " a c c i d e n t , caused by r u p t u r e of a p i p e i n t h e main c i r c u i t . Due t o t h e r e l a t i v e l y l a r g e p i p e d i a m e t e r s i n t h e main g a s c i r c u i t and t h e h i g h v e l o c i t y of sound i n he l ium t h e r u p t u r e of a p i e e r e s u l t s i n a v e r y r a p i d d e p r e s s u r i z a t i o n of t h e c i r c u i t and t h e c o r e . The same a p p l i e s , though t o a lesser e x t e n t , t o a n e q u a l i z a t i o n o f p r e s s u r e w i t h i n t h e sys t em, caused by a n a c c i d e n t , w i t h o u t release of c o o l a n t g a s t o t h e envi ronment . Because of t h e
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p o s s i b i l i t y t h a t a r a p i d d e p r e s s u r i z a t i o n may o c c u r , s p e c i a l d e s i g n and l a y o u t a re n e c e s s a r y for t h e c o r e s t r u c t u r e t o p r e v e n t damage t o t h e c o r e and t h e re la ted s t r u c t u r e so t h a t r e a c t o r shut-down i s n o t i m p a i r e d . The same a p p l i e s t o t h e removal o f decay h e a t .
The decay hea t removal sys t em must o p e r a t e under v a r i o u s p r e s s u r e c o n d i t i o n s , between f u l l d e s i g n p r e s s u r e and approximate ambient p r e s s u r e . T h e r e f o r e s t r i n g e n t r e q u i r e - ments r e s u l t f o r t h e d e s i g n c F t h i s sys t em and f o r t h e c o n t r o l of t h e b lower power. S p e c i a l a t t e n t i o n must be a t t a c h e d t o t h e problem o f t he rma l shocks .
The r a d i a t i o n I exg_osure -- of t h e environment and w i t h i n t h e power p l a n t d u r i n g normal o p e r a t i o n and under f a u l t c o n d i t i o n s d o e s n o t create any in su rmoun tab le problems for t h e e q u i l i b r i u m c o o l a n t g a s a c t i v i t y e x p e c t e d .
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Based on e x p e r i e n c e , t h e p e r m i s s i b l e normal l e a k a g e w i l l n o t be exceeded , even w i t h a s h a f t p e n e t r a t i o n th rough t h e PCPV and a g r e a t number of f l a n g e s t o be sealed.
- The release of t h e t o t a l c o o l a n t i s h a n d l e d , f rom t h e s a f e t y s t a n d p o i n t , by a c o n t r o l l e d re lease t h r o u g h a v e n t i l a t i o n s t a c k .
- There are some u n c e r t a i n t i e s i n m a i n t a i n i n g s u f f i c i e n t l y low r a d i a t i o n d o s e s d u r i n g i n s p e c t i o n and r e p a i r work w i t h i n t h e area o f t h e main c i r c u i t , s i n c e a t t h e p r e s e n t d a t e i n s u f f i c i e n t i n f o r m a t i o n on c o n t a m i n a t i o n mechanisms i s a v a i l a b l e . Favourab le e x p e r i e n c e w i t h t h e DRAGON and t h e AVR r e a c t o r i n d i c a t e , however, t h a t a l s o f o r t h i s problem a c c e p t a b l e s o l u t i o n s c a n be e x p e c t e d .
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The c i r c u i t components a r r a n g e d c o n c r e t e p r e s s u r e v e s s e l : compressors
LAYOUTS
o u t s i d e of t h e p r e s t r e s s e d and t u r b o s e t , h e a t
I n the development phase a g r e a t number of d i f f e r e n t d - s i g n s and l a y o u t s are p o s s i b l e which a p p e a r e q u i v a l e n t , T h e r e f o r e a s y s t e m a t i c e v a l u a t i o n i s r e q u i r e d . According t o r e c e n t c o n s i d e r a t i o n , t h i s e v a l u a t i o n c a n be reduced t o a f e w p r i n c i p l e f e a t u r e s . It becomes e v i d e n t t h a t t h e d i f f e r e n t p o s s i b i l i t i e s of l a y o u t are c h a r a c t e r i z e d by t h e a r rangement of t h e main c i r c u i t components i n s i d e or o u t s i d e t h e p r e s t r e s s e d c o n c r e t e p r e s s u r e v e s s e l , by t h e i r i n t e r c o n n e c t i o n s and by t h e d e s i g n o f t h e t u r b o s e t . These e s s e n t i a l l a y o u t s are c a t e g o r i z e d as n o n - i n t e g r a t e d (N), f u l l y - i n t e g r a t e d (J) and p a r t l y - i n t e g r a t e d ( T I sys tems and t h e i r d i f f e r e n t t y p e s of l a y o u t are compared i n t h e d i f f e r e n t columns of F i g . 2 ,
Going from l e f t t o r i g h t t h e p o s s i b i l i t i e s o f l o c a t i o n of components are compared, s t a r t i n g f rom i n s t a l l a t i o n of t h e heat exchange r s i n a n a n n u l a r s p a c e around t h e core and end ing w i t h t h e pod t y p e l a y o u t .
Based on t h e a n a l y s i s o f t h e p o s s i b l e p l a n t l a y o u t s , t h o s e o f f e r i n g good p r o s p e c t s were i n v e s t i g a t e d r e g a r d i n g t h e i r t e c h n i c a l f e a s i b i l i t y , c a p a b i l i t y of s a f e t y r e q u i r e m e n t s , a v a i l a b i l i t y , and economics,
I n t h e n o n - i n t e g r a t e d sys t em, o n l y t h e r e a c t o r i s l o c a t e d i n t h e p r e s t r e s s e d c o n c r e t e p r e s s u r e v e s s e l ; t h e p r e s s u r e v e s s e l and t h e o t h e r corn\ponents of t h e c i r c u i t are connected t o t h e r e a c t o r v i a ductis ( c f . F i g . 3 ) .
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The g a s , coming from 4 v e r t i c a l l y a r r a n g e d r e c u p e r a t i v e h e a t exchange r s , e n t e r s t h e upper p a r t o f t h e r e a c t o r by 4 r a d i a l openings i n t h e p r e s t r e s s e d c o n c r e t e p r e s s u r e v e s s e l , and e x i t s t o t h e t u r b i n e by a c e n t r a l p i p e i n t h e bottom of t h e p r e s t r e s s e d c o n c r e t e p r e s s u r e v e s s e l . The g a s e x i t f rom t h e r e a c t o r c o n t a i n s a s h i e l d i n g body t o p r o t e c t t h e t u r b i n e a g a i n s t e x c e s s i v e r a d i a t i o n . T h i s body s i m u l t a n e o u s l y s e r v e s a s a c r o s s s e c t i o n l i m i t a t i o n .
All h i g h p r e s s u r e g a s l i n e s ending i n t h e r e a c t o r are manufactured as doub le w a l l p i p e s . For s a f e t y c o n s i d e r a t i o n s even t h e i n n e r p i p e is des igned f o r t h e f u l l p r e s s u r e d i f f e r e n c e a g a i n s t ambient p r e s s u r e .
Two of t h e f o u r decay heat c o o l e r s l o c a t e d above t h e
p r e s t r e s s e d c o n c r e t e p r e s s u r e v e s s e l , s e r v e as r e s e r v e u n i t s . The decay h e a t c o o l e r s a re connec ted t o t h e r e a c t o r by a doub le w a l l p i p e and are l o c a t e d i n a s a f e t y c o n t a i n e r .
A l l g a s l i n e s t o and from t h e t u r b o s e t a re connec ted t o t h e upper p a r t of t h e c a s i n g , Apar t f rom t h e t u r b i n e i n l e t , f o r a l l g a s l i n e s t w o p a r a l l e l l i n e s are provj-ded. For assembly , i n s p e c t i o n and r e p a i r pu rposes t h e lower p a r t of t h e c a s i n g of t h e t u r b o s e t w i t h t h e r o t o r can be lowered by a s p e c i a l h y d r a u l i c or mechanic d e v i c e ; t h e uppe r p a r t of t h e t u r b o - se t c a s i n g and t h e g e n e r a t o r remain on t h e f o u n d a t i o n .
I n t h i s l a y o u t f o u r p r e c o o l e r s and f o u r i n t e r c o o l e r s a re p rov ided . The p r e c o o l e r s a r e d i r e c t l y connec ted t o t h e r e c u p e r a t i v e hea t exchange r s . A l l h e a t exchange r s o p e r a t e i n coun te r f low and are manufactured as p i p e h e a t exchangers .
I n t h e p a r t l y i n t e g r a t e d sys t em, t h e reactor i s l o c a t e d i n t h e p r e s t r e s s e d c o n c r e t e p r e s s u r e v e s s e l , t h e t u r b i n e i s i n s t a l l e d i n a machine c a v i t y , and t h e h e a t exchange r s and
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@ p r e c o o l e r s are l o c a t e d i n pods ( F i g . 4 ) .A second p r e s t r e s s e d c o n c r e t e p r e s s u r e v e s s e l c o n t a i n s t h e compresso r s , i n t e r - c o o l e r s , and t h e he l ium p u r i f i c a t i o n sys t ems . T h i s v e s s e l i s des igned f o r a p r e s s u r e of 8 b a r which r e p r e s e n t s t h e e q u i l i b r i u m p r e s s u r e a f t e r t h e maximum loss o f c o o l a n t a c c i d e n t . Both p r e s s u r e v e s s e l s are connected by a common f o u n d a t i o n p l a t f o r m . T h i s l a y o u t shows e s s e n t i a l c h a r a c t e r i s t i c s o f t h e i n t e g r a t e d sys tem.
The he l ium f low from t h e r e a c t o r e n t e r s t h e t u r b i n e v i a a s h u t t e r t u b e i n t h e h i g h p r e s s u r e p r e s t r e s s e d c o n c r e t e v e s s e l . (The t u r b i n e i s f l a n g e d d i r e c t l y t o t h e s h u t t e r t u b e and i s p r o t e c t e d by s h i e l d i n g s t r u c t u r e s a g a i n s t e x c e s s i v e r a d i a t i o n . ) From t h e t u r b i n e t h e he l ium f l o w s th rough t h e f r ee p a r t of t h e machine c a v i t y i n t o t h e h e a t exchangers and i n t o t h e p r e c o o l e r s i n s t a l l e d above . Then t h e coo led g a s f l o w s downwards th rough t h e c h a n n e l s i n t h e c o n c r e t e and i n h o r i z o n t a l d i r e c t i o n th rough t h e f o u n d a t i o n p l a t e t o t h e compressors w i t h a n i n t e r m e d i a t e c o o l i n g s t a g e . The h i g h p r e s s u r e g a s i s a l s o d i r e c t e d th rough t h e f o u n d a t i o n p l a t e t o t h e h e a t exchange r s . I t f l o w s a l o n g t h e t u b e bund les of the h e a t exchangers i n cross c o u n t e r flow and e n t e r s t h e
reactor l a t e r a l l y a t t h e h e i g h t of t h e lower r e f l e c t o r , c o o l i n g t h e metal s t r u c t u r e s b e f o r e b e i n g r e h e a t e d i n t h e c o r e . Thus, all h a n d l i n g and measuring equipment f o r f u e l e l emen t s are l o c a t e d i n t h e r e g i o n of low g a s t e m p e r a t u r e s . Otherwise t h e r e a c t o r c o r r e s p o n d s t o t h o s e used w i t h steam t u r b i n e p l a n t s .
The main c i r c u i t i s i n t e g r a t e d up t o t h e p r e c o o l e r o u t l e t . T h i s e n s u r e s s u f f i c i e n t l y l o w p r e s s u r e change ra tes i n t h e i n t e g r a t e d p o r t i o n of t h e main c i r c u i t , i n t h e e v e n t of r u p t u r e of a g a s p i p e , because of t h e t h r o t t l i n g e f f e c t of t h e t u r b i n e , t h e l a r g e g a s volumes o f t h e heat exchange r s
@
222
and p r e c o o l e r s , and t h e p a r a l l e l p i p e s l e a v i n g t h e pre- Q s t r e s s e d c o n c r e t e p r e s s u r e v e s s e l . The O 2 c o n t e n t of t h e g a s r e s u l t i n g from t h e m i x t u r e of a i r and he l ium does n o t c o n s t i t u t e a danger t o t h e reactor.
Removal of decay h e a t i s e f f e c t e d by a r edundan t sys tem c o n s i s t i n g of a p r e c o o l e r , a b lower , and a h e a t exchange r , l o c a t e d i n t w o a d d i t i o n a l c a v i t i e s i n t h e p r e s t r e s s e d c o n c r e t e p r e s s u r e v e s s e l .
I n t h e i n t e g r a t e d sys tem a l l components are l o c a t e d i n s i d e t h e p r e s t r e s s e d c o n c r e t e p r e s s u r e v e s s e l ( F i g . 5). P e n e t r a t i o n s th rough t h e p r e s s u r e v e s s e l are r e q u i r e d only f o r t h e s h a f t c o n n e c t i n g t h e t u r b i n e w i t h t h e a l t e r n a t o r , and f o r assembly and d i sa s sembly of t h e components l o c a t e d w i t h i n t h e v e s s e l .
A two-room p r e s t r e s s e d c o n c r e t e p r e s s u r e v e s s e l i s env i saged ( w i t h o u t p r e s s u r e s e p a r a t i o n ) . Heat exchange r s and coolers are a r r a n g e d i n t h e a n n u a l s p a c e around t h e r e a c t o r and t h e compressor t u r b i n e u n i t , r e s p e c t i v e l y . Compressors and t u r b i n e are l o c a t e d i n a s e p a r a t e room below t h e r e a c t o r and are p r o t e c t e d by s h i e l d i n g s t r u c t u r e s . I n t h i s room also t h e c o o l e r s are l o c a t e d which o p e r a t e i n a pu re he l ium envi ronment , a s t h e compressor t u r b i n e u n i t .
The c o o l a n t gas flows from t h e core th rough t h e s h i e l d i n g and th rough a s h o r t l i n e , c o n t a i n i n g a s h u t - o f f v a l v e , i n t o t h e t u r b i n e . From t h e t u r b i n e i t f l o w s upwards t o t h e h e a t exchangers and downwards t o t h e c o o l e r s and compressors .
T h i s d e s i g n i s c h a r a c t e r i z e d by t h e f e a t u r e s t h a t a l l components are i n t e r c o n n e c t e d by d u c t s , no d u c t of t h e main c i r c u i t , however, l e a v e s t h e p r e s t r e s s e d c o n c r e t e v e s s e l , and t h a t t h e room c o n t a i n i n g t h e compressor t u r b i n e u n i t
6d and t h e c o o l e r s must be k e p t a t t h e maximum he l ium p r e s s u r e a n d , u s i n g i n v e n t o r y c o n t r o l , t h e p r e s s u r e l e v e l w i t h i n t h i s room w i l l v a r y w i t h t h e p r e s s u r e l e v e l of t he whole sys t em.
For emergency c o o l i n g t w o emergency c o o l i n g b lowers w i t h v a r i a b l e speed and emergency c o o l e r s are p r o v i d e d .
T h i s sys t em is a l s o c h a r a c t e r i z e d by a two-room p r e s t r e s s e d c o n c r e t e p r e s s u r e v e s s e l w i t h o u t p r e s s u r e s e p a r a t i o n , t h e heat t r a n s f e r u n i t s a r e , l o c a t e d i n pods ( F i g . 6). The o t h e r c h a r a c t e r i s t i c s c o r r e s p o n d t o t h o s e o f t h e l a y o u t shown i n F i g . 5 .
I n t h e i n t e g r a t e d sys t em i n F i g . 7 t h e compressor t u r b i n e is l o c a t e d i n a machine c a v i t y . The i n t e r c o o l e r s a re a r r a n g e d i n h o r i z o n t a l open ings i n t h e lower p a r t of t h e p r e s t r e s s e d c o n c r e t e p r e s s u r e v e s s e l . I n a d d i t i o n , t h i s l a y o u t is c h a r a c t e r i z e d by t h e f e a t u r e t h a t a l l g a s d u c t s are formed by c h a n n e l s i n t h e c o n c r e t e of t h e p r e s t r e s s e d c o n c r e t e p r e s s u r e v e s s e l and i n t h e s l a b s e p a r a t i n g c o r e and machine c a v i t y .
u n i t
T h e v a r i o u s l a y o u t c o n c e p t s d e s c r i b e d show a g r e a t number o f common and s p e c i f i c problems. The i n v e s t i g a t i o n of t h e s e problems i s b e i n g c a r r i e d o u t w i t h i n a l a r g e sys t ems a n a l y s i s . To d e c i d e which d e s i g n c o n c e p t w i l l be f u r t h e r deve loped a n e v a l u a t i o n of t h e i n d i v i d u a l c o n c e p t s is b e i n g carried o u t w i t h i n 1 9 7 0 . Applying common s a f e t y s t a n d a r d s t h e
e v a l u a t i o n i s c a r r i e d o u t a c c o r d i n g t o t h e f o l l o w i n g c r i t e r i a :
- f e a s i b i l i t y - a v a i l a b i l i t y and - c o s t s .
224
The main i t e m s which a re be ing i n v e s t i g a t e d , a r e :
- assembly , d i s a s s e m b l y , p i p e c o n n e c t i o n s , a c c e s s i b i l i t y , f o u n d a t i o n l a y o u t o f t h e t u r b o s e t
- l a y o u t o f t h e g a s p i p e s o f t h e main c i r c u i t
- f l o w behav iour a f t e r p i p e r u p t u r e s and t h e i r effects
- d e s i g n and l o c a t i o n of s h u t - o f f v a l v e s o f t h e main c i r c u i t
- h a n d l i n g he l ium volume d u r i n g c o n t r o l procedures and r e p a i r
- open ings and p e n e t r a t i o n s of t h e
p r e s t r e s s e d c o n c r e t e p r e s s u r e v e s s e l .
The c o n c e p t s d e s c r i b e d are t h e r e s u l t of t h e f i r s t d e s i g n phase ( sys t ems a n a l y s i s ) . The d e s i g n w i l l be deve loped i n s u f f i c i e n t d e t a i l so t h a t i n 1970 a d e c i s i o n c a n b e made on t h e g e n e r a l l a y o u t . The d e c i s i o n r e g a r d i n g t h e t y p e o f f u e l e l e m e n t s i s e x p e c t e d i n 1 9 7 2 . Complete c o n s t r u c t i o n documents w i l l be a v a i l a b l e i n 1 9 7 5 .
Components w i l l be t e s t e d i n t h r e e he l ium t e s t l o o p s which are under c o n s t r u c t i o n . By e x t e n s i v e f u e l e l emen t development work, i n c l u d i n g a n i n v e s t i g a t i o n of t h e d e p o s i t i o n mechanisms of f i s s i o n p r o d u c t s , a c c o u n t w i l l be t a k e n of t h e s p e c i a l c o n d i t i o n s of t h e s i n g l e - c y c l e p l a n t . The e x p e r i e n c e g a i n e d w i t h t h e o p e r a t i n g h i g h t e m p e r a t u r e t e s t r e a c t o r s and t h e p r o t o t y p e power p l a n t s unde r con- s t r u c t i o n o r t o be c o n s t r u c t e d i n t h e n e a r f u t u r e , w i l l c o n s i d e r a b l y c o n t r i b u t e t o t h e s u c c e s s f u l e x e c u t i o n of t h e pro j ec t .
225
max. processtemperat ure min. processtemperature number of intercoolers max. processpressure thermal reactor power electrical output net efficiency
F i g . 1.
PARTLY INTEGRATED(
MACHINERY ROOM I
mffi 515EI i INTEGRATED LAYOUT
P, = e
A 850 O C
22 O C
2 60 bar 1333MW 600 MW 45%
B 850 O C
35 O C
1 60 bar
1428MW 600 MW
42 Yo
i iominal 3 e s i g n Data
I I
F i g . 2 ., V a r i o u s l a y o u t s c h e m a t i c s 63
Teilintegrierte Anlage
Fig. 4. Partly integrated layout
. . . , .. ----- Fig. 3. Non-integrated layout
F i g . 6 . I n t e g r a t e d l a y o u t 2
l a y o u t
228
DISCUSSION
S. I. Kaplan: How would you provide emergency c o o l i n g ?
H. Oehme: A l l designs descr ibed have two a u x i l i a r y loops for emer-
gency cool ing which can ope ra t e a t a l l pressures from fu l l pressure t o
atmospheric . J. D. Thorn: To what e x t e n t i s your s e l e c t i o n of p l a n t layout i n -
f luenced by a preference f o r a h o r i z o n t a l s h a f t and a s i n g l e machine?
H. Oehme: I n the beginning of OUT a n a l y s i s our t u r b i n e des igners
looked for t h e most d e s i r a b l e s o l u t i o n s f o r t h e i r po in t of view. They
proposed t h e s i n g l e s h a f t h o r i z o n t a l machine, s o we made it a b a s i s of
our l ayou t a n a l y s i s . The reasons f o r t h a t a r e descr ibed i n t h e paper. I may mention one po in t - having a s i n g l e s h a f t h o r i z o n t a l machine o r v e r -
t i c a l l y arranged compressor t u r b i n e units wi th a h o r i z o n t a l power t u r b i n e
as i n some B r i t i s h proposals , one needs i n both cases approximately t h e
same lower p a r t of diameters i n t h e lower p a r t of t h e PCRV f o r p l ac ing or
r e p l a c i n g t h e power tu rb ine .
L. J. Connery: W i l l your helium t u r b i n e [discharge i t s waste h e a t t o
a i r r a t h e r than a cool ing water s o u r c e ?
H. Oehme: All t h e l ayou t s d i scussed i n t h e paper i nco rpora t e a n i n -
te rmedia te water cool ing c i r c u i t f o r s a f e t y reasons and a f i n a l d i s p o s i -
t i o n of h e a t t o t h e a i r t o acqu i r e s i t e independence. Because of t h e
r e l a t i v e l y h igh of f -gas temperature i n t h e HHT t h i s s o l u t i o n i s t echn i -
c a l l y f e a s i b l e and burdened wi th a reasonable decrease i n e f f i c i e n c y only.
G. Meijer: Regarding t h e problem of fast c l o s i n g i s o l a t i o n va lves
i n connection wi th nonin tegra ted and p a r t i a l l y i n t e g r a t e d layout , I wodd
l i k e t o make t h e fol lowing remarks: I n s p i t e of decay h e a t removal loops
be ing capable t o remove the decay h e a t a f t e r a fas t dep res su r i za t ion , I am a f r a i d t h a t one s t i l l w i l l need fas t operati-ng i s o l a t i o n va lves f o r
nonin tegra ted designs. Based on the present knowledge, I must emphasize
t h i s , t h e reasons are:
even wi th a v e n t u r i i n t h e duc ts , ( 2 ) h igh temperatures of t h e a i r -he l ium
mixture i n t h e secondary containment dur ing and a f t e r dep res su r i za t ion
(1) D i f f i c u l t core l e v a t i o n problems poss ib ly
229
0 through a main coolant duc t .
have t o opera te i n a high temperature environment f o r t he nonin tegra ted
des igns .
development per iod and cons iderable cos t w i l l be involved and even i f
t e c h n i c a l l y f e a s i b l e a :Licensing problem must be a n t i c i p a t e d . I n a par-
t i a l l y i n t e g r a t e d design, one may or may not need fas t c los ing i s o l a t i o n
va lves . This has not been determined y e t . However, i f w e would need them
i n t h i s type of layout , t h e va lves would be loca ted i n t h e cold duc ts .
They, t h e r e f o r e , a r e more f e a s i b l e from a t e c h n i c a l s tandpoin t and e a s i e r
t o l i c e n s e . Because of t h e above reasons, I a m of t h e opinion t h a t non-
i n t e g r a t e d designs do not seem t o be as f e a s i b l e and t h a t one should con-
c e n t r a t e on p a r t i a l l y i n t e g r a t e d and f u l l y i n t e g r a t e d des igns .
t h i s t h e requirements f o r nonin tegra ted des igns w i l l au tomat i ca l ly emerge.
I f one needs fas t c los ing va lves , t hey w i l l
Although fas t c l o s i n g va lves may be t e c h n i c a l l y f e a s i b l e , a long
I n doing
H. Oehme: I f u l l y agree . I n f a c t , I may add two remarks wi th r e -
s p e c t t o t h e nonin tegra ted des igns .
t h a t even i f t h e f e a s i b i l i t y of a n emergency c los ing va lve i s a problem
it may not be accepted by t h e l i c e n s i n g committee, even i f you have two
va lves i n ser ies . For t h e reasons mentioned by you and for o t h e r reasons,
w e , i n f a c t , t end t o f avor one of t h e i n t e g r a t e d des igns .
We have a l r e a d y had t h e experience,
L. A. Lys: You ha-ve a d d i t i o n a l emergency cool ing loops i n your de-
Does it mean tha- t you must r e l y upon a fast c los ing va lve t o i s o - s ign . l a t e the main loop in order t o avoid bypassing of the core in the case of
emergencies ?
W. Twardziok: We (don’t need quick c l o s i n g va lves t o ope ra t e t h e
emergency cool ing system, because w e have t i m e enough before s t a r t i n g t h e
emergency cool ing. We ag ree t h a t w e have t o i s o l a t e t h e main loop t o de-
c rease t h e mass flow f o r t h e emergency cooling, b u t t h a t can be done
slowly.
L. A. Lys: I n your i n t e g r a t e d des ign I have not no t i ced space f o r
helium which m u s t be removed from t h e loop i n t h e case when t h e p re s su re
l e v e l c o n t r o l system i s used,
p re s su re v e s s e l pipes , pene t r a t ing t h e w a l l of t h e v e s s e l i s , of course,
If the helium i s s t o r e d ou t s ide of t h e
necessary. This , however, w i l l c o n f l i c t wi th t h e p r i n c i p l e s of t h e i n -
@ t e g r a t e d design.
230
W. Twardziok: For a l l HTR gas tu rb ine designs ( in t eg ra t ed or non- i n t e g r a t e d ) w e proposed t o have a combination of bypass and pressure l e v e l cont ro l . Quick changes w i l l be done w i t h the bypass cont ro l . For t he
pressure l e v e l c o n t r o l there w i l l be more time, t h a t means only small d i -
ameter pipes for the connection of the primary c i r c u i t and the helium
s to rage system, arranged outs ide of the pressure ves se l . Loss of coolant
m u s t be taken i n t o account a l s o for t h e in t eg ra t ed systems, b u t it means only small dep res su r i za t ion rates which leaves enough t i m e for valve ac- t i o n .
Paper 6/li7
D EV EL 0 PME N T WO R K F 0 R L _ ~ E ; = b S $ J d J f 3 ~ ~ C , L - ~ A_R_._HFL-IJJM T U R B I N E PLANTS \\'ITH WIG1I-TEMPERATURE REACTORS -**-Emu--
% E. B6hm and W . Twardziok - GHN-Oberhausen 3? 2- H. Oehme - BBC/Krupp Mannheirn iq/ 0 !-z H. Ke i skopf - BBC Mannheim
ABSTFtACT
The main p a r t o f t h e deve lopmen t programme f o r h i g h - t e m p e r a t u r e r e a c t o r s w i t h h e l i u m t u r b i n e i s p roposed t o be s p e n t on t e s t f a c i l i t i e s and t e s t work. Three t e s t r i g s f o r t h e n o n - n u c l e a r t e s t s on h e l i u m components and s y s t e m s a r e d e s c r i b e d . The r i g s a r e p r o p o s e d t o be e r e c t e d j o i n t l y w i t h t h e a u x i l i a r y i n s t a l l a t i o n s i n a common t e s t f i e l d on t h e p r e m i s e o f KFA i n J u l i c h . The pro- b lems o f t e s t work a re b r i e f l y d e s c r i b e d by t h e two examples , h o t g a s v a l v e s and i n s u l a t i o n .
231
232
1. Introduction
Within the framework of the development programme for high-temperature reactors with helium turbine of high
output (HHT-programme), an extensive test programme will be performed parallel to the projecting work. The importance of this part o f the programme can be seen from a cost comparison, which shows that about 80 $ of the total cost is proposed to be spent on test work and 10 % each on the projecting work and on an accom- panying programme for basic research.
The nuclear test programme requires about 25 $I o f the total cost, it comprises mainly the development and testing of fuel elements and materials. For the non-
nuclear test programme about 55 % of the total c o s t
is envisaged; here the task is to develop and test reactor and helium turbine Components and systems. The overall idea is to prove, with the aid of the test programme, the technical feasibility, the safety and the economy of components and systems for large HTR- plants with a direct cycle.
The following is dealing only with the non-nuclear test programme, which can be divided into two phases. The first phase comprises non-concept-bound tests on
smaller test rigs and the erection o f rigs for testing full-scale components of the 600 MWe-plant. The second phase covers the concept-bound tests and the testing
of prototypes.
2. Test rigs
For carrying out the test and development work, exis- ting helium test rigs will be concentrated in one
place and completed by loops in which the parameters
o f the coolant are to be realized which are envisaged
233
for the nuclear power plant being projected. I n all installations helium is circulated at high temperature
and pressure, with reactor impurity levels being aimed
at.
The arrangement and main data of the three helium test
rigs are shown in Fig. 1. The helium test loop (HVK)
consists o f the circulator ( a ) , the heat exchanger (b), the test section (b'), the heater (c), the mixer (d),
the cooler (e) and the motor (f). At a mass flow of
1 kg/sec in the test section a temperature o f 8 0 0 ° C
and a pressure o f 20 bar is achieved. The main com- ponents of the helium test turbine rig (HVT) are the LP compressor (a), the intercooler (b), the HP com- pressor (c), the heat exchanger (d), the natural-gas-
fired heater (e), the turbine (f), the pre-cooler (g),
the by-pass cooler (h), the test section (i), the
gearbox ( k ) and the starting motor (1). The mass-flow
in the test section is about 6 kg/sec at a tempera-
ture of approximately 700 C and a pressure of 22 bar.
The high-temperature helium test plant (HHV), with a mass flow of about 220 kg/sec at a maximum temperature of 1 0 0 0 ° C and a maximum pressure of 50 bar, is pro- posed to be used for prototype testing. Its main components are the hot-gas compressor (a), the test section ( b ) , the turbine ( c ) , the mixer (d), the by-
pass cooler (e), the gas circulator (f) and the
driving motor for the turbo set. The thermal energy
for the loop is supplied by the motor driver of the
turbo set.
0
._
The helium test loop (HVK) is proposed to go into operation in the autumn of 1970. A view o f the HVK model is shown in Fig. 2. In the foreground is the vertical test section, on the right is the heater
234
and i n t h e background i s t h e v e r t i c a l l y a r r a n g e d h e a t e x c h a n g e r .
The h e l i u m t u r b o s e t o f t h e h e l i u m t e s t t u r b i n e r i g i s shown i n F i g . ? d u r i n g a s s e m b l i n g . From l e f t t o r i g h t one c a n s e e t h e LP c o m p r e s s o r , t h e IIP compresso r and t h e h e l i u m t u r b i n e w i t h a x i a l o u t l e t , s t i l l e q u i p p e d w i t h n o z z l e r i n g s . T h i s f i r s t h e l i u m t u r b i n e s e t o f t h e
w o r l d w a s o r i g i n a l l y u s e d u n d e r t h e name o f L a F l e u r i n Phoen ix , A r i z o n a ( U S A ) , i n a n i t r o g e n l i q u e f y i n g p r o c e s s . The machine s e t w a s b u i l t by E s c h e r Wyss, Z u r i c h . I t i s u n d e r m o d i f i c a t i o n by GHH t o become a t e s t i n g i n s t a l l a t i o n . F i g . 4 , wh ich shows t h e h e l i u m h e a t e r of a b o u t 15 m h e i g h t , g i v e s a n i m p r e s s i o n o f t h e s i z e of t h i s t e s t r i g . The h e a t e r i s f i r e d w i t h
n a t u r a l g a s ; t h e t h e r m a l o u t p u t i s a b o u t 7 M W t h and t h e g a s consumpt ion about 1300 Nm 3 /h . Between t h e
h e a t e r and t h e t u r b i n e t h e r e i s a n a u s t e n i t i c p i p e l i n e o n t o wh ich t h e t e s t s e c t i o n i s t o be c o n n e c t e d .
A c r o s s s e c t i o n o f t h e t u r b o s e t o f t h e BBC-planned h i g h - t e m p e r a t u r e h e l i u m t e s t p l a n t i s shown i n F i g . 5 , w i t h 1 b e i n g the machine c a s i n g , 2 t h e h o t - g a s i n l e t , 3 t h e h o t - g a s o u t l e t , 4 t h e by-pass i n l e t , 5 t h e by- p a s s o u t l e t , 6 t h e t u r b i n e b l a d i n g , 7 t h e r o t o r , 8 t h e c o m p r e s s o r b l a d i n g and 9 t h e o i l - l u b r i c a t e d r a d i a l b e a r i n g . The two-s tage t u r b i n e has an o u t p u t o f a b o u t 50 MW, w h i l e t h e IO-s tage c o m p r e s s o r h a s a power r e - q u i r e m e n t o f a b o u t 90 MW. The a d d i t i o n a l power r e - q u i r e d i s s u p p l i e d by a s y n c h r o n o u s moto r w i t h s t a r t i n g equ ipmen t . F o r c o o l i n g t h e f e r r i t i c - d i s c r o t o r and f o r s e a l i n g t h e r e i s a s e p a r a t e b lower c i r c u i t . The r o t o r o f t h e t u r b o s e t h a s a b o u t t h e same d i m e n s i o n s as t h a t o f a 300 MWe-helium t u r b i n e s e t .
T h e t e s t r i g s d e a l t w i t h i n t h e f o r e g o i n g a re p roposed
235
t o be e r e c t e d j o i n t l y w i t h t h e a u x i l i a r y i n s t a l l a t i o n s i n a common t e s t f i e l d o n t h e p r e m i s e s o f K F A , t h e
n u c l e a r research c e n t r e i n J i i l i c h . The ground p l a n on t h e h e l i u m t e s t f i e l d a t p r e s e n t i n t h e p l a n n i n g s t a g e i s shown i n F i g . 6. The s m a l l e r i n s t a l l a t i o n s , t h e h e l i u m t e s t l o o p ( W K ) and t h e h e l i u m t e s t t u r b i n e r i g (I-IVT) a r e accommodated i n t h e h a l l of a b o u t 1 2 m h e i g h t on t h e r i g h t and t h e h i g h - t e m p e r a t u r e h e l i u m t e s t p l a n t (HIIV) i n t h e h a l l o f a b o u t 20 m h e i g h t on t h e l e f t . I n a l o w e r c o n n e c t i n g bay a r e t h e common h e l i u m s u p p l y s y s t e m w i t h t h e s t o r a g e t a n k s and t h e common h e l i u m p u r i f i c a t i o n p l a n t . Above t h e s e t h e c o n t r o l s t a t i o n s f o r t h e r i g s and t h e data c o l l e c t i o n s y s t e m a r e a r r a n g e d . The t e s t h a l l s a r e p r e c e d e d by t h e shop , l a b o r a t o r y and o f f i c e b u i l d i n g . On t h e l e f t and r i g h t b e s i d e t h e h a l l s a r e t h e power f e e d i n g and d i s t r i b u t i n g s t a t i o n s s o t h a t t h e r e i s o n l y a s h o r t way t o t h e consumers . The e r e c t i o n of t h i s b u i l d i n g i s s c h e d u l e d t o be comple t ed by t h e m i d d l e o f 1971 t o t h e e x t e n t t h a t o p e r a t i o n s c a n be s t a r t e d . The t e s t o p e r a t i o n s are p roposed t o be ca r r i ed o u t by t h e g r o u p of BBC, GHH and F K i n c o o p e r a t i o n w i t h KFA.
A p a r t f rom t h e a f o r e - d e s c r i b e d i n s t a l l a t i o n s , a con- v e n t i o n a l l y f i r e d 50 MWe-helium t u r b i n e power s t a t i o n i s p roposed t o be e r e c t e d u n d e r t h e HHT programme, i n o r d e r t h a t a l l components o f a h e l i u m t u r b i n e i n s t a l l a t i o n c a n be combined and t e s t e d i n c o n t i n u o u s o p e r a t i o n i n a r e a l power s t a t i o n c i r c u i t . The main data o f t h e p roposed p l a n t a r e shown i n F i g . 7 . The t u r b i n e i n l e t t e m p e r a t u r e o f 7 3 O o C a p p l i e s t o con- t i n u o u s o p e r a t i o n . F o r t e s t i n g p u r p o s e s i t i s p o s s i b l e t o a c h i e v e h i g h e r t e m p e r a t u r e s f o r a s h o r t t ime . With a maximum p r e s s u r e o f 40 bar, a n e x p a n s i o n r a t i o o f 2 .5 , c o m p r e s s o r i n l e t t e m p e r a t u r e s o f 25 C , s i n g l e - 0
236
s t a g e i n t e r m e d i a t e c o o l i n g and a t e m p e r a t u r e a p p r o a c h i n t h e h e a t e x c h a n g e r o f 3 O o C , a mass f l o w o f 86 k g / s e c i s a c h i e v e d . The n e t o u t p u t i s 50 MWe and r e s u l t s , t o g e t h e r w i t h t h e t h e r m a l o u t p u t o f t h e h e a t e r o f 156 MWth, a t a n e t e f f i c i e n c y o f a b o u t 32 9. I n t h e 50 MWe-plant, i t i s i n t e n d e d t o t e s t s y s t e m s and components o f l a r g e d i m e n s i o n s f o r r e l i a b i l i t y and s a f e t y i n c o n t i n u o u s o p e r a t i o n and t o a s c e r t a i n t h e dynamic b e h a v i o u r and t h e j o i n t o p e r a t i o n o f t h e components o f t h e h e l i u m t u r b i n e p l a n t .
3. T e s t programme
During the f i r s t p r o j e c t phase, i n which the des ign
c o n c e p t o f t h e 600 MWe-plant i s t o be f o u n d , o n l y s u c h t e s t s c a n be c a r r i e d o u t which a re o f a bas i c , i , e . non-concept-bound c h a r a c t e r . F o r t h e s e t e s t s , which s e r v e t o s u p p o r t t h e judgemen t and c h o i c e o f t h e f i r s t p l a n t c o n c e p t , t h e two small t e s t r i g s HVK and HVT a r e s u i t a b l e . F o r c o s t r e a s o n s t h e com- p o n e n t s o f o r i g i n a l d i m e n s i o n s can o n l y be b u i l t and t e s t e d a f t e r c o m p l e t i o n o f t h e r e f e r e n c e d e s i g n o f t h e 600 MWe-plant. They a re i n t e n d e d t o s e r v e as p r o t o t y p e s f o r d i r e c t p r e p a r a t i o n o f f i n a l d r a w i n g s a n d data f o r t h e 600 W e - p l a n t .
3 . 1 S u r v e y
The t i m e s c h e d u l e f o r t h e most i m p o r t a n t t e s t s i s shown i n F i g . 8. A t t h e t o p t h e t h r e e t e s t r i g s a re g i v e n , s t a r t i n g f rom commencement o f t h e t e s t o p e r a t i o n s . The g a s d u c t s w i t h t h e h o t - g a s i n s u - l a t i o n s and e x p a n s i o n b e l l o w s a re f i r s t t o be examined by p r e l i m i n a r y t e s t s on t h e HVK, t h e r e - a f t e r , w i t h more c o m p l i c a t e d g e o m e t r i e s , on t h e IIVT
237
and finally, with the dimensions resulting from the
reference design, on the HHV rig. The same proce- dure will be adopted for the hot-gas valves, which,
depending on the concept, may be equipped with or
without trip gear. The flow distribution, thermal-
shock behaviour, tightness and dynamic behaviour
of the heat-exchanging units will also b e investi-
gated step by step on the three test rigs. The hot testing of the reactor internals i s proposed to be carried out on the HVT and IIHV rigs. While the tests aiming at design solutions t o safety problems are carried out on all of the three rigs, the dy-
namic behaviour o f a helium turbo set and the other components can only be studied on the HVT. However,
the main results will have to come from the 50 MWe- plant.
Finally the shaft seals are shown, which will be
developed at a separate test installation and tested during operation o f the plants. The HHV rig is pro- posed to be equipped with a shaft seal whose di-
mensions correspond to those o f a 600 MWe-turbine seal.
The specifications for the various tests are under
preparation. The problems are briefly described
in the following by two examples.
3.2 Hot-gas valves
HTR plants with helium turbine require shut-off and control valves o f large diameters for operation in helium of high purity at high temperature and
pressure. Especially in plants which are not fully
integrated, these valves must have a high inner and outer tightness and a short closing time. Fig. 9 shows a design of a non-conventional hot-gas valve
238
with small dimensions. Such a valve with small di-
mensions i s proposed to be examined by preliminary tests before a large unit is tested.
The pneumatic control principle i s briefly described in the following (see Fig. 9 ) . O n normal opening and closing operations the valves V 5 and V 6 are actuated. On trip-closing the servo valve 1 is operated, with
a sufficient quantity o f gas being caused, by actua- tion o f control valve V I , t o flow into the lower cylinder space from the pressure accumulator 5 through the charging line 6. Before reaching its upper end position, the valve plate is braked by the damping
pin 4. The blocking p i n 7 fixes the plate in its upper end position; it is operated via the valves
V 3 and V 4 . During every velve motion the load on the two sealing plates 8 i s removed to the LP tank through
the pipes 2 . The control system is fed from the auxi-
liary supply system 9. The entirc valve casing and
the valve plate have to be kept at a lower tempera- ture by means of the cooling gas 3.
The most essential difference as compared to con-
ventional designs is that the valve plate, which is
guided in needle bearings, has also the function of
the control slide. This design avoids penetrations
and is particularly compact, which is advantageous
especially for installation in the prestressed- concrete vessel. The most important problems to be
examined are :
cold welding o f parts i n motion and at rest, material abrasion,
wear o f needle-bearing guide, tightness at seats,
control-gas requirement and closing forces,
239
cooling-gas supply and requirement, and efficiency o f damping.
The purpose of the investigations is to prove the functional reliability and safe availability with respect to application o f such valves in the safety concept of large HTR-plants with helium turbine.
3.3 Hot-gas insulations
The special problems o f hot-gas insulation in HTR- plants with helium turbine result from
the system-inherent high-pressure-chan- ging rates during control operations and
accidents,
the high gas flow velocities in the gas ducts due to the large volumes and the
correspondingly high-pressure drops and dynamic forces , and the high gas temperature and pressure with helium of reactor impurity.
Fig. 10 shows the most important insulation geo- metries to be examined. These are the straight
insulation section (a), the bend ( b ) , the T- branching (c) and the straight vessel wall (d). In addition to these geometries there is the insu- lation at the turbine inlet, which may have par- ticularly complicated geometries.
With regard to the nuclear purity conditions, the insulations used in reactor building are either all-metallic foil or mat insulations or ceramic
fiber insulations with tight metallic liners.
Fig. 10 shows as an example the connection o f two sections of a foil insulation (e) and a pipe branching ( f ) having a fibrous insulation with a
2 40
liner. In designing these insulations it is necessary to provide the clearances or openings required for thermal
expansion and depressurization in such a way as to en- sure that the dynamic behaviour is not badly affected
and hot spots are avoided.
The problems t o be investigated can be divided into three main groups :
(a) the thermodynamic behaviour with regard
to heat conductivity,
jb) the mechanical behaviour with regard to
thermal txpansion and depressurization,
and
( c ) the vibration behaviour with regard to
alternating stress from gas and sound
forces and mechanical vibrations.
The testing is proposed to be performed step by step. At the beginning there will be preliminary tests on
the helium test loop concerning the thermodynamic
behaviour of a pipe insulation in helium at high
temperature, pressure and flow velocities.
For these tests a special test section has been de-
signed and built, which is shown in Fig. ll. The
inner pipe (a) is provided with a metal foil insu- lation (b) which carries the displacement body (c).
At the displacement body the static pressure
tappings (d) are fixed. A joint of the insulation
sections (e) is shown in the lower part and the
bellows to absorb thermal expansion in the upper
part (f). The hot gas enters at OOO°C at point 1
and leaves at point 2, the cooling gas at 350°C flows in counter-current from 3 t o 4. The test sec- tion is being provided with the instrumentation and
241
the tests are proposed to start at the end o f this year.
With the displacement body it is possible to achieve
gas flow velocities of up to about 100 m/sec, so that
pressure drops per insulation section can be achieved
and even exceeded as will occur in the future large
unit. Fig. 12 shows a comparison of the test sec- tion data of the three loops with the data of the
600 We-plant. A s can be seen, it is necessary to provide the insulation test sections o f both the HVK and HVT with a displacement body to achieve the gas flow velocities required for ascertaining the
thermodynamic behaviour. The integral behaviour of
the insulation can only be examined with the origi- nal dimensions o f the pipe on the HHV rig as in this installation comparable dynamic gas forces
are expected.
Parallel to the thermodynamic tests described, the
insulations, especially with helium turbine plants,
have to be tested with regard to their behaviour
on rapid pressure changes. Other than in HTR two-
operation, to master pressure changing rates which amount to about 10 bar/sec and are thus higher by about the factor 10 to 20. Depending on the arrange- ment of the plant as a whole (integrated or non-
integrated), rates o f up to 100 bar/sec may occur
in an accident such as pipe rupture.
cycle plants, it is necessary even i n normal control
A depressurization vessel in which these high changing rates are achieved is shown in Fig. 13. In the tank (a) a pipe section with a test insulation (b) is fitted. At the outlet nozzle in the upper
head it is possible t o set different cross sections
242
by means o f an orifice, which before conmencement of a test is covered by two bursting discs. These discs are caused to burst during the test by admitting
pressure gas to the space between them. The pressule
djfferentials between the pipe interior and the interior of the insulation or behind the insulation
are measured during depressurization as well as the
i deformation o f the inner liner at the joints.
The first preliminary tests on a foil insulation with cold gas have been started at EURATOM in Ispra.
At present a larger test vessel is designed by GHH, in which insulation geometries o f original dimen- sions can be tested also at high temperatures. The
flow tests and depressurization tests will be
carried out on insulations with the same design and
geometry.
243
Helium Test Loop
HVK
Ressure : 20 bar
Temperature : 800 OC
Mass Flow : 1 kg/s
Helium Test Turbine
HVT
u
2 2 bar
700 "C
6 kg/s
High Temperature Helium Test Plant
H HV
5 0 bar
1000 O C
220 kg/s
F i g . 1 Arrangement and Main Data o f t h e Hel ium T e s t R i g s
- HVK ( h e l i u m t e s t l o o p ) - HVT ( h e l i u m t e s t t u r b i n e )
a c i r c u l a t o r a b h e a t e x c h a n g e r b b' t e s t s e c t i o n C
c h e a t e r d d m i x e r e e c o o l e r f f mo to r g
h HHV ( h i g h - p r e s s u r e i
h e l i u m t e s t r i g ) k 1 a c o m p r e s s o r
b t e s t s e c t i o n c t u r b i n e d mixer e by-pass c o o l e r f c i r c u l a t o r g d r i v i n g moto r
-
LP compresso r i n t e r c o o l e r €IP compressor h e a t e x c h a n g e r h e a t e r t u r b i n e p r e - c o o l e r by-pass c o o l e r t e s t s e c t i o n g e a r b o x s t a r t i n g motor
244
F i g . 2 Model of a H e l i u m T e s t Loop (HVK)
F i g . 3 Turbo S e t o f the H e l i u m T e s t Turbine ( H V T )
24 5
F i g . 4 Gas-Fired Heater o f the Helium Test Turbine(HVT)
F i g . 5 Turbo S e t of the High-Temperature Helium Test Plant (HHV)
1 machine c a s i n g 6 turbine b lading 2 ho t-gas i n l e t 7 r o t o r 3 hot-gas o u t l e t 8 compressor b lading 4 by-pass i n l e t 9 o i l - l u b r i c a t e d r a d i a l bearings 5 by-pass o u t l e t
246
Fig. 6 Helium Test Field for HEIT Development
in Julich
Turbine inlet temperature Turbine inlet pressure Pressure ratio Compressor inlet temperature Number of intercooling Hea t exchanger temp era t ur e difference Mass flow Net power Heater thermal power Net efficiency
C bar
0
C 0
deg C
MWe k d s
MW th %
730 40
2 9 5 25 1
Fig. 7 Preliminary Layout Data of the Conventionally
Fired 50 MWe-Helium Turbine Power Station
247
'est Facilities
Helium Test Loop (HVK)
1 Helium Test Turbine (HVT)
I Hlgh Temperature Helium Test Plant (HHV)
1 Ducts, Compensation. Insulation
2 Valves
3 Heat Exchangers
L Reactor lnternals
5 Safety Aspects
6 Dynamic Behaviour
7 Shaft Seals
1970
1
Fig. 8 HHT Test Programme
vz
. ~~
Fig. 9 Hot-Gas Valve for Helium Turbine Plants
1 servo valve 6 charging line 2 to LP tank 7 blocking pin 3 cooling gas 8 sealing plate 4 damping pin 9 auxiliary supply system 5 pressure accumulator VI to V 6 control valves
248
b
f
Fig. 10 Problems with Hot-Gas Insulations
a str~ight insulation section b 180 bend c pipe branching d vessel wall e foil insulation f fibrous insulation at a pipe branching
C
‘ 3 Fig. 11 Test Section for Hot-Gas Insulations
a inner pipe f bellows b foil insulation 1 ho t-gas inlet c displacement body 2 hot-gas outlet d static pressure tappings 3 cooling-gas inlet e joint of insulation packs 4 cooling-gas outlet
249
4elium Test Loop
HVK
lelium Turbine Test Loop
HVT
lelium High Temperature
e s t Plant HHV
600 MWe-HHT-Plant
with displacement bod
ressure Temperature Mass- Diameter of Velocity of Gas Frow Hot Gas Duct
bar O C kg/s mm m/s
20 800 1 216l’ 100
22 7 00 6 400 76
50 1000 220 1020 142
60 850 700 1570 140
Fig. 12 Main Data of the Helium Test Rigs
I: 25 bar Pressure Temperature 5 5OOOC
Depressurisation S 1OOborA
Fig. I3 Depressurization Vessel a vessel
b test insulation
250
DISCUSSION
B. N. Furber: I would be i n t e r e s t e d i n f u r t h e r d e t a i l s of the metal-
l i c i n s u l a t i o n proposed f o r t h e duc t i n s u l a t i o n , p a r t i c u l a r l y f o r t h e 180"
bend.
s t a t i c pressure f i e l d make t h e i n s u l a t i o n problems ( p a r t i c u l a r l y l e a k i n g )
very severe .
Here t h e d i f f i c u l t i e s of i n s u l a t i o n combined wi th a very complex
W. Twardziok: I f u l l y ag ree t h a t t h e r e a r e s p e c i a l problems concern- i ng t h e duc t i n s u l a t i o n f o r bends.
t h e s e geometries wi th f o i l i n s u l a t i o n as w e l l as wi th f i b e r i n s u l a t i o n .
I n both cases w e have t o t ake ca re f o r t h e s e a l i n g wi th r e spec t t o t h e
forced convect ion on t h e one s i d e and for t h e openings wi th r e spec t t o
t h e dep res su r i za t ion ra te on t h e o t h e r s i d e .
t i o n w e propose to take a m e t a l l i c foil i n s u l a t i o n w h i c h i s d iv ided i n t o
s e v e r a l s e c t i o n s and weld i t t o t h e p ipe circumference on one end.
Therefore , we propose t o do tes ts on
For our f i r s t bend t e s t sec-
Paper 7/127
THE PROGRAM OF PLATE-OUT I INVESTIGATIONS IN THE G A S TURBINE PROJECT
3 I . , ~ - . o p 1 c r r ; r ; l ~ ~ ~ ~ ~ ~ ~ - ---4-M--
0 C.B. von der Decken &/$-3*3e
The HHT-project, the project for the development of a HTR- system with direct cycle gas turbine has been described extensively in the foregoing papers. In this paper I want to speak about a special subject from this project, the plate-out of fission products.
Due to the development of the coated particles the fission products are retained very well inside the fuel elements. One need not speak at present of a contaminated cooling gas system in HTR's. The level of activity in the primary system of HTR's is comparable to the level in the primary system of reactors with metallic cladded fuel elements, at least in practical reactor operation taking into account problems of the production failures, etc. This has been demonstrated by a large number of in-pile experiments, but especially by the operation experience in three reactors, -Dragon, Peach Bottom and AVR.
Nevertheless, the low-level contamination of the cooling gas and the components is still large enough to play an important role in the safety philosophy and possible accidents. The lack of detailed knowledge of the behavior of fission products leads to a pessimistic view in the safety philosophy and with this to an over-emphasis of the safety provisions in the lay- out of the plant which could be an important factor in the economics of the HTR's.
This is a problem f o r all HTR-systems but specially for a system with a direct cycle gas turbine because of the relative- ly large conduit cross-section which could be opened by a practical or hypothetical accident. In such a case the depressurisation of the plant would be much quicker and higher gas velocities would occur in many parts of the system. In a large loss of coolant accident therefore the release of fission products out of the primary system could be much higher compared to steam cycle systems. Furthermore the distribution of fission products over the surface of the system is important for maintenance and repair because the gas turbine itself represents a large piece of equipment and the necessary precautions of shielding and safety for the maintenance operations will have an important influence on the design, the costs and the availability. For these reasons in the frame work of bhe HHT-project an extensive program has been developed to study the problems of the plate- out of fission products. I will try to give an overview of this program. 6i3
251
252
The discussion of such a program shoulq start with a summary of what is known up to now. Over the previous years important and good work has been done specially at Batelle, Oak Ridge and Gulf General Atomic. But I believe I can avoid giving such a summary today because this will be the subject of a special paper later in this conference,
@
The plate-out program in the HHT-project consists of the following main items.
1) Calculation models and computer programs 2) Measurement of the adsorption and desorption rates 3 ) In-pile experiment "Saphir" 4) Out-of-pile experiment "Smoc" (Saphir - model - out-of-pile 5) Adsorption of fission products on graphite dust 6) Investigations in the Am-reactor
- c ircui tT
Due to limited time I will be able only to discuss the main ideas of the different items and to give a short description of the experiment "Saphir" ,
253
6lJ CALCULATION MODELS AND COMPUTER PROGRAMS
To understand the behavior of fission products in complex system like primary circuits in HTR's a number of calculation models have to be worked out. The ultimate hope is that it might be possible to describe the complete process in the cooling system with a large computer program.
The mass transport in the gaseous phase can be described by the known laws of mass transport and heat transfer under flow conditions. Immediately near the wall there exists a boundary layer out of which the adsorption or desorption takes place. To work out a calculation model one can assume as a first step that the adsorption equilibrium with a boundary layer takes place spontaneously. With this assumption we are now preparing a computer program "fish-trade No. 1" (fission - product transport and deposition) which describes the tem- poral and local behavior of the fission products in any given complex tube system. Tube sections in parallel and in series, different temperatures, tube proflles, Reynolds numbers and adsorption constants can be taken into account. The program is based on the description of the adsorption by the of Henry and Langmuir. It will be ready soon.
The second step will be the program "fish-trade X" which corresponds to the program "fish-trade No. l", but experi- mentally determined adsorption isotopes will be used which will have been measured for a number of fission products and materials. The next step will be the program "fish-trade Y" which corresponds to the Predep-program from Kress not using the assumption of spontaneous equilibrium in the boundary layer. In this program also, experimentally determined ad- sorption and desorption rates will be used. O n e m i g h t better use in this case the expression, reaction rates, because in addition to the adsorption effects, chemical reactions of the fission products with structural materials will play an important role.
laws
MEASUREPENT OF THE ADSORPTION AND DESORPTION RATES
To use the computer programs alarge number of characteristic basic data have to be measured; for example, the adsorption and desorption rates for the most important fission products on the structural reactor materials. These basic data depend on a large number of parameters.
The fission products of main interest are Sr, I and Cs. Bay Ce, Ru and Te are of minor importance. The adsorption materials are all materials which are in contact with the primary cooling gas. This means ferritic and austenitic steels with different surface properties and graphites with @
2 54
different structure and surface areas and other ceramic materials . For the fission products Sr, I and Cs the already known measurements of the adsorption isotherms under static or laminar conditions will be repeated and extended. In the literature a large number cf such measurements have been described. Specially the publications of Zumwalt and co- workers and those from ORNL have to be mentioned. These measurements are already giving a rough picture of the circumstances, but many of the detailed results are still contradictiony and they cannot be extrapolated to other materials and conditions. During these experiments in our program the following view points will be taken into account particularly.
3) We will select only materials as an adsorber which will be important for the technical lay-out of a plant. The surface properties and conditions of these materials will be defined as clearly as possible. The surface conditions of some of the materials will change during reactor opera- tion and we will specially look in this problem. The influence of oxidic layers on steel surfaces is an example.
b) In the work already published the adsorption of the diffe- rent isotopes has been measured f o r single isotopes only. The influence of any co-adsorption has been neglected. Probably the influence of the co-adsorption is only important near the saturation. Adsorption isotherms had to be measured up to saturation and repeated in the presence of other fission products, for example: Cs/Sr.
Furthermore, an important parameter will be the level of impurities in the cooling gas. This influences the condi- tion of the adsorption surfaces and the fission products themselves. Concentrations of only a few Natm of water vapor or carbon-dioxide in the cooling gas represents some orders of magnitude more atoms per cm3 compared with the concentrations of' fission products. This means that, f o r example, Cs, which might be created in the atomic form would have a good chance to react with the impurities of the cooling gas before reaction with any surface takes place .
Furthermore, the measurements of the adsorptioc isotherms will be extended to turbulent flow conditions. Up to the present such measurements have been done only up to 20 m/sec max. gas velocity.
Since there will be much higher gas velocities in the reactor system we want to measure up to 100 m/sec gas velocity in maximum. This is because it has not been clearly establiehed today whether the velocity of turbulent motion immediately next to the wall is comparable to the mean velocity of the molecules. It might be sufficient to make experiments for a few typical cases only.
A next group of important data are the desorption rates especially for safety predictions in case of reactor accident with loss of coolant. The measurements of desorption rates have to be done under static or laminar and under turbulent flow conditions.
In addition to adsorption, chemical reaction of the fission products with the structure materials will be important. In some cases the mass transport coefficient must be considered, while in other cases the velocity cnnstant of the surface reactions will be the more essential. The problem has not been examinated systematicly up to now. As the mass transport coefficient for the most common flow conditions and geometries is well known we will measure in the next series of experi- ments the velocity constants for a number of important reactions and the time dependence. If the methods prove to work well, we will also study the temperature dependence. Based on the results of these experiments it should be possible to determine whether the quantity of adsorbed fission products for various materials and conditions depends mainly upon chemical kinetics of surface reactions or upon the convective mass transfer coefficient.
The experiments to measure the adsorption and desorption rates under static or laminar conditions will be done in an apparatus which is shown schematicly in Fig. 1. A quartz tube contains the adsorption material and the source fission product. Independent heating provides for temperature regula- tion and for establishing given partial pressure. For de- sorption measurements the system can be evacuated.
Part of the experiments with iodine will be done with inactive iodine. We hope to develope the detection technique for iodine to a high level of sensitivity. The advantage of using an inactive apparatus is, of course, a simpler technique, and greater flexibility. We hope also for better accuracy to define the different parameters such as partial pressure, etc. A schematic drawing of the apparatus is shown in Fig. 2. The experiment will be done in standard atmospheric conditions. Clean air will be mixed with iodine vapor. The partial pressure of the iodine can be regulated by the temperature of the iodine source. The apparatus will be started by by-passing the test section until the partial pressure is constant. Then the gas
256
stream will be switched over to the test section. By this method conditions during the start-up of the experiment will be avoided. The same apparatus can be used for desorption measurements.
The experiment Smoc which will be described later will be used for all the other experiments under turbulent flow conditions.
IN-PILE EXPERImNT "SAPHIR"
In the reactor Phgase in Cadarache we are preparing an irra- diation experiment in the Loop Saphir, which we consider as an integral test with respect to the several out-of-pile experiments mentioned above. This experiment will last about two years. We will measure the deposition of solid fission products released from spherical elements under operation conditions of a gas cooled high temperature reactor. We will find out the dependence on Reynolds number, temperature, different materials and surface conditions of the materials. The gaseous impurities of the helium coolant will be moni- tored and controlled continuously.
Description of the Loop "Saphir"
The loop consists of the main circuit with the test assembly in an in-pile position of the reactor and an auxiliary circuit for purification and analysis of the coolant. The auxiliary circuit is connected to a bypass of the main circuit in an out-of-pile position.
The main circuit
Fig. 3 shows the scheme of the main circuit. The helium coolant flows from the blower through an electrical pre- heater (110 kW) and a Venturi nozzle measuring the total helium-flow to the test assembly. Here the helium divides into two streams. About 90 $ of the helium flows through an outer annulus of the test assembly back to the blower. Depending on the test conditions one can lead a part of the helium through a heat exchanger, which is placed in a bypass in front of the blower. The other part of the helium flows through the test assembly to the auxiliary circuit and then back to the main circuit.
The main circuit is mounted in a frame which is lowered to the bottom of the reactor tank. It then is moved to the core on rails.
257
Fig. 4 shows the test assembly. In a graphite sleeve 14 sphere elements each with a diameter of 60 mm are arranged in line. The sleeve is surrounded with Silicagel-wool in- sulation. Between the insulation and the outer tube of the test assembly is the annulus for the external helium-flow.
bove the fuel elements the interchangeable test tube is mounted. It is 2 m in length with a diameter of 30 mm, followed by a tube with a length of about 1 m and an inner diameter of 20 mm. The last one fits through the upper plug of the main circuit. A 180 - bend connects this tube with an absolute filter for solid fission products, both mounted out of the pressure tube of the main circuit in the reactor tank.
The absolute filter has a volume of 2 ltr. It contains some layers of a special glass fibre, and silver plated molecular sieve, type 13 X.
The inner mass flow of the helium (10 $ of the total flow) flows inside of the insulation over the fuel elements. Depending on the test conditions it is heated up from 250 - 400 OC entrance temperature to 800 - 850 OC at the exit of the sphere arrangement. Then the helium passes the test tube. The helium stream which flows outside along the insulation and the test tube cools the hot helium in the inner side of the tube to 500 - 650 OC. The inner helium flows through the bend and the absolute filter which is cooled by water of' the reactor tank. It the1 flows through a control filter filled with charcoal and a mass flow meter to the auxiliary circuit.
A part of the released solid fission products deposits on the inner side of the test tube and the bend depending on temperature and flow conditions. The rest will be adsorbed quantitatively in the filter,
The main circuit is laid out for an operation pressure of 60 ata and a maximum temperature of 550 OC. In a preliminary test the mean neutron flux in the fuel has been determined to be 6 1013 cm'* s-1.
The auxiliary circuit
Fig. 5 shows a scheme of the auxiliary circuit. Its operatio pressure is 60 at, the gas temperature is about 40 OC. The helium coming from the main circuit is driven through the aux'liary circuit by a compressor with a maximum output of
second one it will be purified. In addition it is possible 9 m 3 /h at 40 at. In a bypass the gas will be analysed; in a
0
258
to inject defined amounts of impurities into the helium.
The gaseous impurities in the helium are measured with a hygrometer and a gas chromatograph. The H2 will be determined with a Cu 0 - filter followed by a hygrometer. To measure the gaseous fission products a part of the inner mass flow (about 50 mg/sec) will be bypassed before the absolute filter and led through a mass flow meter into a filter f o r short-lived or another filter for long-lived fission products. The short-lived isotopes are determined by their solid daughter products.
The total activity in the auxiliary circuit is controlled by a monitor.
The purification facility consists of three elements. A filter with BTS-catalysator oxidizes H 2 and CO. The operation temperature is 200 OC. Behind the filter the helium is cooled to 10 oc.
Then the helium passes two molecular sieve filters working at room temperabure. In the first one H20 is adsorbed in the second one C02.
Then a part of the helium flows through a charcoal trap cooled by liquid air. Its volume is 2,5 ltr. In this filter N2, 02, Kr and Xe is adsorbed.
To control the effectivity of the purification system it is possible to connect a gas chromatograph or a hygrometer behind the filters.
The purification system is laid out in duplicate to avoid interruptions in operation due t o defects o r the regeneration of the filters.
Experimental procedure
The test tubes together with the bends and the absolute filter are changed five times a year and analysed quanti- tatively with respect to solid fission products. O f special interest are the isotopes I 131, S r 89, Sr 90, Cs 137, Te 132 and Ba 140. The concentration profile of the deposited solid fission products is measured in both longitudinal and radial directions of the test tube.
In case the activation by neutrons of the test tube is neglegible a scan is performed in longitudinal direction in the hot cells. Then the tube is cut into equal segments each of which is leached and analysed cy -spectrornetrically,
2 59
6$ As test material several kinds of steel and graphite tubes such as may be used in a HT-reactor with different diameters are provided. The gas inlet and outlet temperature and thereby the surface temperature of the test tube is varied by changing the inner mass flow. The power output of the fuel elements is kept constant. Between two changes the experimental conditions are not varied.
Table 1 shows the operation data which are attained in the
Spherical fuel elements of the HTR type are to be used. To get a sufficient output of solid fission products the coated particles are fabricated with a thinner coating than usual. The thickness of the sealing and outer coating is about 6 0 , ~ . The kernal consists of U02 and Th 02 with a ratio of 1 : 5. The lay-out of the elements allows a constant power generation of 3 kW per sphere for one year. To compensate for the fuel consumption the loop is moved nearer to the core during the test time. The reference temperatures are those of the fuel elements and the inlet gas temperature of the test tube.
loop.
In case the released rate of solid fission products is too small to produce measurable effects at the test tube the fuel elements are exchanged by a second charge. This charge containes coated particles with a buffer coating of 60 - 7 0 , ~ but no sealing and outer coating.
In a preliminary test which will probably start at the beginning of July this year the commissioning tests of the loops are to be carried out with normal THTR fuel spheres. If this test is satisfactory the first radiations will start at the beginning of August this year.
260
Table 1 Data of operation
$as temperature [OC]
entrance fuel outlet fuel entrance test tube outlet test tube
250 - 400 800 - 850 800 - 850 500 - 650
gas pressure [at) 40 - 60
pas flow [ g / SI total flow main circuit test tube auxiliary circuit
purification system
mean Reynolds number fuel
Reynolds number test tube
fuel element mean power / sphere number of spheres maximum surface temperature loading of U 235 / sphere
mean thermal neutron flux
100 - 250
15 - 24 15 - 24
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c3 OUT-OF-PILE EXPERIMENT "SMOC"
A large reactor experiment like "Saphir" is very costly in operation and not very flexible. Therefore the possibilities of varying the different parameters such as material, surface conditions, geometries and temperatures etc. are very limited. Each experiment with a given set of parameters wosld require two to four months for completion. F o r this reason we are planing an out-of-pile experiment "Smoc" (Saphir model out- of-pile circuit) in which we can vary all Eecessa'Fy para- meters. An important consideration for the lay-out of Smoc is to simulate the operating conditions of Saphir as closely as possible in order to correlate both experiments. It is hoped that the results which c a n be achieved with Smoc can be translated easily to in-pile conditions.
In addition to this important comparison of the two experi- ments, Saphir and Smoc, the main purpose of the Smoc experi- ment is to measure the adsorption and desorption rates under turbulent flow conditions. Different steel and graphite test samples up to 50 mm in diameter and 4 m in length can be used and may be examined at temperatures up to 800 OC. Gas pressures up to 80 at, gas temperatures up to 800 O C , gas velocities up to 50 m/sec and Reynolds numbers up to lo5 can be achieved. The gaseous impurities will be monitored and controlled. More complex test sections will also be used to test different computer programs.
The experiment Smoc is still under design and I am not able to give you more detailed information today.
ADSORPTION OF FISSION PRODUCTS ON GRAPHITE DUST
In HTR's with prismatic fuel elements only minor quantities of graphite dust are present in the primary system. The quantity of graphite dust in pebble-bed reactors is somewhat larger. We are trying to determine the total amount graphite dust present in the AVR reactor.
Estimates have shown that the quantity of graphite dust in the AVR reactor is much less than had been assumed for the lay-out of the reactor. Nevertheless, even small quantities of graphite dust could be important in case of a large accident with loss of coolant if a large amount of fission products would be adsorbed on the dust. In such a case the dust could be blown out immediately during loss of coolant without any desorption process. Besides the adsorption rates the quantity of fission products on the dust depends on the surface area and this depends on the particle size distri- bution of the dust. @
2 62
Experiments at Brown Boverie / Krupp which had been done in connection with the problems of errosion have shown that the graphite dust at high gas velocities in the cooling system is broken into small pieces very quickly. The dust particles under operation conditions are very small and have a large specific surface area. A typical particle size distribution of graphite dust which had been blown around. in a circuit with a velocity of l r ) m/sec is shown in Fig. 6. Curve 1 represents a particle size spectrum of the graphite dust which had been inserted before the start oi' the experiment.
Curve 2 shows the particle size distribution after 30 minutes of operation of the circuit. If the graphite dust is blown around in the circuits for a longer time the particle size distribution does not change very much. As one can see from the diagram the particle size is about a few ,u.
In the investigation program we will make experiments which should define the graphite dust and will show how to handle this very fine dust. Later on we will insert dust in the experiments Saphir and Smoc to measure the amount of fission products which will be adsorbed on this dust. In addition we will try to find out how the dust will plate-out on surfaces and will be removed by a gas stream from the surface.
IWVESTIGATIONS I N THE AVR-REACTOR
In model experiments it is very difficult to simulate the conditions of particle reactor operation well enough to extrapolate the results of these model experiments with sufficient certainty to actual reactor conditions. 'This is because in case of plate-out of fission products a larger number of' parameters are involved and the corresponding data f'or the reactor conditions are not known. Measurements of' fission product distribution in reactors in operation now could in principal give important results. Unfortunately it turns out to De impossible to test the calculation models on reactor systems in operation at present because of the lack of knowledge or' all necessary data. In addition the number of possible investigations on reactor systems under operation is very limited due to time and design reasons.
in the first place tne main of objection of' the AVR operation, for example, is to the testing of' the whoie system, the fuel elements and the components. Major interference in the system to measure the plate-out fission products on surfaces of the system would interrupt the reactor operation too much. In addition the AVR reactor is designed as a power station and this means that the possibilities for making detailled experiments are very limited. 63
Besides the routine measurement of the rare gas isotopes, the moderator spheres which contain only graphite are being investigated to measure the fission products on the surface of these spheres, Furthermore the surface of the primary system which has to be dismantled for maintenance and repair will be investigated for plate-out of fission products. Up to now, fortunately for the reactor, but unfortunately for these experiments, only components out of the secondary circuits had to be dismantled, for example, the components of the fuel handling system. In principle only the blowers and the butterfly valves for the bypass can be dismantled from the primary system. These components worked without failures up to now and dismantling is for inspection purposes later on. Also the access to the dust filter is very difficult. For this we plant to design a small bypass with a dust filter which can be changed easily. We hope that it might be possible to measure the quantity of dust which is present in the primary circuit under operation and measure the particle size and the contamination of this dust.
In closing, I would very much like to emphasize that this program is a co-operative one that has been worked out by all the partners of the HHT-project. The theoretical and experimental work is being done and will be done by the different partners. I would like to thank all the people who have contributed to this program,
264
A Vakuum pump Ouartz t u b Heater lup lo 1000°C) Thermostat Source Shielding
7 Test specimen 8 p-measurement
Fig . 1. M e a s u r e m e n t of a d s o r p t i o n - i s o t h e r m s ( C s , I)
sorptions-and desorptions- test -section
circulotor /
I analytical Y I U
Fig . 2. A p p a r a t u s f o r s o r p t i o n s - and deso rp t ions e x p e r i m e n t s
265
f-
auxiliary circuit
r - - I I I I I I I I I core
I I I
n n nozzle \ I 1 1 1 1 1 I
1 1 - 0 0 I -
Fig . 3 . Main c i r c u i t of Loop Saph i r
f&40*c absolute filter
_-ca 500'C
1
W
Fig . 4 . T e s t a s s e m b l y of Loop S a p h i r
filter
- 7
I I
I I I I I I I I I I
I I
266
compressor
Fig . 5 . A u x i l i a r y c i r c u i t of L o o p Saph i r
fraction of particles up to diameter D co/o]
'tides diam.
Fig . 6 . P a r t i c l e s i z e d i s t r ibu t ion of g raph i t e d u s t
267
DISCUSSION
L. R. Z m w a l t : 1. Do you a t p re sen t have d a t a on t h e f i s s i o n prod-
uc t conten t of g raph i t e d u s t from t h e AVR? 2.
l a b o r a t o r y experiments f o r determining t h e abso rp t ion isotherms of mixed
f i s s i o n products on g raph i t e d u s t t y p i c a l of HHT ( A V R ) ?
Have you contemplated
C . B. von de r Decken: 1. Unfortunately w e do not have access t o
t h e d u s t f i l t e r i n t h e AVR. Dismantling t h i s f i l t e r would i n t e r f e r e wi th
t h e r e a c t o r ope ra t ion g r e a t l y and it i s not contemplated i n t h e near fu-
t u r e . We have designed a s m a l l bypass wi th an e a s i l y removable f i l t e r t o
do s t u d i e s on t h i s problem i n t h i s d i r e c t i o n . 2. We w i l l t r y t o do t h i s
f i r s t s i n c e one has t o de f ine what w i l l be p re sen t i n t h e HTR.
F. H. N e i l l : What i s t h e source of f i s s i o n products i n your out-of-
p i l e l o o p ?
C. B. von de r Decken: The des ign of t h e ou t -o f -p i l e loop has not y e t
been completed.
We w i l l des ign t h e loop f o r us ing d i f f e r e n t sources .
s i o n a t a l a t e r da t e and hope t h a t w e can p r o f i t from t h e experience of
o t h e r groups.
We have not decided on t h e kind of source w e w i l l use.
We w i l l make a dec i -
A. P. Fraas : Could you do d i r e c t con tac t maintenance on AVR compo-
nents ?
G. Ivens : I an sorry t h a t I cannot g ive you exac t f i g u r e s concern-
i n g the a c t i v i t y l eve l on t h e AVR components. I can s ta te , however, t h a t
maintenance work on components of t h e f u e l handl ing f a c i l i t y which were
i n con tac t w i th f u e l elements and t h e primary c i r c u i t gas could be c a r r i e d
out without any s p e c i a l s h i e l d i n g precaut ions .
C . B. von der Decken: An examination of t h e g raph i t e spheres (gra-
p h i t e on ly ) i nd ica t ed t h a t t h e h ighes t level of a c t i v i t y r e s u l t e d from
impur i t i e s i n t h e g raph i t e .
found i n t h e spheres . I a m s o r r y t h a t I do not have any d a t a wi th m e on t h i s sub jec t .
A very low l e v e l of f i s s i o n products was
Paper 8/102
THE HT8.- _DIREC.T-GY.C.U2 : ENGINEERING PO~SIBILITIES AND MATERIAL REQUIREYENTS
G. E. Lockett R. A. U. Huddle OECD Dragon P ro jec t
ABSTRACT
I n t e r e s t i n direct cyc le Gas Turbine Power P lan t s l inked t o High Temperature Gas Cooled Reactors, stems from the p o t e n t i a l savings i n e l e c t r i c i t y generat ing cos ts . An expected reduct ion i n c a p i t a l c o s t s toge ther with a somewhat higher thermal e f f i c i ency appears s u f f i c i e n t t o j u s t i f y se r ious study; wh i l s t , i n the longer t e r m , t he gradual r a i s i n g of temperature and e f f i c i ency can provide a cont inuing opportuni ty f o r improvement.
A s a f i r s t s t e p towards eva lua t ing t h e p r a c t i c a l p o s s i b i l i t i e s , r ecen t Dragon Project w o r k has selected a plant layout arrangement and produced a re ference design. It has been used a s a b a s i s f o r s i z i n g components, i d e n t i f y i n g problem a reas and assess ing the effects of hea t exchanger performance, pressure drops, design conf igura t ions and gas temperature l i m i t s .
When opera t ing with helium a t high core o u t l e t temperatures and a t t h e low and r ep resen ta t ive impurity levels , expected i n a c losed cyc le system, the re i s a need t o show t h a t t he behaviour of any chosen high temperature ma te r i a l i s completely sa t i s f ac to ry . regarding the choice of ma te r i a l s and an i n d i c a t i o n from exploratory test r e s u l t s i s given.
A philosophy
The paper g ives a view on some of t h e problems foreseen and some of t h e proposed general so lu t ions . b e no insuperable problem b u t f u r t h e r study could lead t o u s e f u l improvements.
It concludes t h a t t h e r e appears t o
INTRODUCTION
The growing i n t e r e s t i n a d i r e c t cycle gas turb ine power p l an t
l inked with a high temperature helium cooled r e a c t o r stems from t h e
p o t e n t i a l savings i n e l e c t r i c i t y generat ing costs .
t h e i n d i r e c t steam cycle system the savings appear s u f f i c i e n t t o
j u s t i f y se r ious study.
When compared with
The expected savings r e s u l t from the o v e r a l l
268
2 69
p l a n t and bui ld ing s i ze , coupled with t h e somewhat higher thermal
e f f i c i ency of power generat ion which can be achieved with present ly
acceptable operat ing temperatures. Furthermore, i n the longer term,
the gradual r a i s i n g of temperature and e f f i c i ency can b e seen a s
providing a continuing opportuni ty f o r improvement.
The l i m i t i n g temperatures are d i c t a t e d on t h e one hand by the
turbo-machinery design which must opera te continuously and r e l i a b l y ;
and on t h e o ther hand by t h e r e a c t o r core i n which f u e l and moderator
must opera te with a high degree of i n t e g r i t y and with a low f i s s i o n
product emission.
c o n t r o l l i n g t h e gas f low between them i s not without i t s problems,
b u t i n a l l a r eas the re appears t o be a so lu t ion ava i l ab le and no
immediately r e s t r i c t i v e b a r r i e r t o achieving very adequate working
temperatures i s evident.
The supplementary requirements of duct ing and
FUEL AND GAS TEMPERATURES
For a f i r s t s tage exploratory study, a peak nominal f u e l tempera- 0 ture of 1300 C i s regarded a s a s u i t a b l e l i m i t and i n present s t u d i e s
corresponding o u t l e t gas temperatures from peak channels can reach
lloooc.
The mixed gas temperature from a l l core channels, toge ther with
con t ro l rod and r e f l e c t o r cooling streams, l e a d s t o a t u r b i n e i n l e t
temperature of about 967'C (124O0K) and t h i s i s t h e o r e t i c a l l y capable
of producing a thermal e f f i c i ency of power generat ion of over 47%.
Although the above mixed o u t l e t gas temperature i s between 100°C 0 and 200 C higher than cu r ren t ly conceived steam cycle designs t h e core
i tself appears v i r t u a l l y i d e n t i c a l .
more than 50 C higher and t h i s i s l a rge ly achieved by l i m i t i n g core
power dens i ty t o about 5.8 MW/m . even before taking i n t o account t h e expected improvements i n f u e l
spec i f i ca t ions and performance which could occur during t h e next
4-5 years.
Peak f u e l temperatures a r e no 0
3 These are predic tab ly safe values
270
Regarding the r e a c t o r core , down-flow cool ing i s now usual i n
H T R ' s and it i s even more appropr ia te f o r the direct cycle system
because acc identa l pressure t r a n s i e n t s i n the d i r e c t i o n of flow must
not l e v i t a t e t he core (e.g., loss of tu rb ine b lad ing) . A coarse
f l a t t e n i n g of channel gas o u t l e t temperatures by s h i f t i n g gagged top
r e f l e c t o r blocks a t r e f u e l l i n g i n t e r v a l s corresponds t o a devia t ion
of approximately 240 C, about a mean value when c a r r i e d out a t l i f e
i n t e r v a l s .
considered necessary i n HTR cores where t h e f u e l can t o l e r a t e t he
temper a t u r e swing s occurring.
0
The complication of continuously va r i ab le gagging i s not
The core i n l e t temperature i n t h e d i r e c t cycle system b r ings i t s own p a r t i c u l a r problems. With good recupera t ive hea t exchangers, core
i n l e t gas temperatures will be l i k e l y t o exceed 500 C, thus , on-load
f u e l changing must be designed t o s u i t t h i s temperature i n t h e upper
plenum and a l s o around the core support framework, which, toge ther with
t h e thermal neutron sh ie ld ing , must e i ther opera te a t t h i s temperature
o r be cooled by co lder by-pass streams. The l a t t e r so lu t ion has been
adopted i n t h e present study and the cool ing streams are used
subsequently t o remove r a d i a l r e f l e c t o r hea t before en te r ing t h e under
core plenum a t a temperature which does not degrade t h e core o u t l e t
gas temperature unduly.
0
The main penal ty arises from the f a c t t h a t cool by-pass streams
do no t pass through the recupera tor and hence the h e a t exchanger
e f f i c i ency i s lowered.
I n the d i r e c t cyc le system considered here , f u e l element surface 0 temperatures can reach about 1170 C compared with values of about
1000uC i n t he steam cycle case, b u t s ince the re i s no steam inleakage
problem i n t h e direct cyc le , g raph i t e corrosion effects can be
discounted and the change i n dimensional s t a b i l i t y of t he graphi te due
t o shrinkage behaviour, although worse, i s not seen a s r e s t r i c t i v e .
271
Control rod cooling streams which pass khhrough the core i n
p a r a l l e l with the f u e l channels w i l l be l a rge ly heated by t h e
swrounding core graphi te , thus con t ro l rods must be designed to
opera te a t a re la t i .vely high temperature, kypical ly 700-800 C. 0
CHOICE OF LAYOUT
Whilst previous cornments o u t l i n e a general view of t he d i r e c t
cyc le which can be backed by thermodynamic eva lua t ion over a range of
cases, i t becomes necessary t o a s ses s the p r a c t i c a b i l i t y of the
concept.
design which i s followed through i n t o p r a c t i c a l d e t a i l t o expose the
s p e c i f i c a reas where design and ma te r i a l problems exist. This s tage
i s preceded by some eva:luation of major components and explora t ion of
layout p o s s i b i l i t i e s . As a r e s u l t of such work a s u i t a b l e design
philosophy tends t o emerge.
It i s the re fo re necessary t o choose and develop a re ference
A nwnber of b a s i c opt ions a r e ava i l ab le t o t h e designer; he can
choose f u l l y in t eg ra t ed , semi-integrated o r non-integrated p l a n t
arrangements, and may s e l e c t e i t h e r a f ixed speed turbo-machinery
design with a l l compressors and tu rb ines on a s ing le s h a f t , o r a s p l i t
s h a f t design i n which the power tu rb ine opera tes a t f i xed speed while
t he turbo-compressor set may run a t va r i ab le speed. A f u r t h e r freedom
of choice app l i e s i n r e spec t of s i n g l e o r mul t ip le turbo-compressor loop arrangements.
I n the re ference design a s p l i t s h a f t turbo-machinery design was
selected f o r severa l reasons. F i r s t l y i t lends i tself t o a va r i e ty of
p l an t part-load con t ro l methods, un l ike t h e s i n g l e s h a f t arrangement,
which, by v i r t u e of t he r e l a t i v e l y narrow range of flow v a r i a t i o n
achievable with f ixed speed compressors, i s made l a rge ly dependent on
helium inventory control . Secondly the turbo-compressor u n i t can
r e a d i l y be mounted v e r t i c a l l y t o occupy a reac tor -vesse l w a l l cavi ty .
Thirdly a separa te turbo-compressor u n i t can be designed t o r u n a t
speeds s u b s t a n t i a l l y higher than t h e generator synchronous speed.
This r e s u l t s i n more compact machines and smaller w a l l c a v i t i e s .
272
With regard t o p l a n t i n t e g r a t i o n , t h e r e can be no doubt t h a t from
sa fe ty cons idera t ions preference must l i e w i t h a f u l l y in t eg ra t ed
layout , i.e., one i n which t h e r e a c t o r and gas turb ine p lan t a r e
housed within a s ing le , enclosing pres t ressed concrete vessel . On
the o the r hand, t he complexity of t he gas c i r c u i t tends t o pose
d i f f i c u l t problems f o r t h e ves se l designer which make it d i f f i c u l t ,
i f not impossible, t o achieve a x i a l symmetry i n a f u l l y in t eg ra t ed
design. The tendency i s f o r ves se l conf igura t ions t o emerge where
the tendon arrangements f o r p re s t r e s s ing are unsa t i s f ac to ry and the
ana lys i s w i l l r equ i r e t h e de r iva t ion of very complex programmes.
The so lu t ion adopted f o r t he re ference design houses the r e a c t o r ,
turbo-compressor u n i t s and a11 hea t exchangers and coolers i n an
e s s e n t i a l l y axi-symmetric concrete vesse l , very similar i n design to
t h e pod-vessel developed f o r t h e steam cycle HTR. The depar ture from
complete i n t e g r a t i o n concerns t h e power tu rb ines which are located i n
separa te ho r i zon ta l p res t ressed concrete ves se l s posi t ioned underneath
t h e main vessel . By ensuring t h a t t h e in te rconnec t ions a r e arranged
t o s a t i s f y t h e same i n t e g r i t y r u l e s a s would apply t o a s i n g l e vesse l ,
t he arrangement o f f e r s t h e advantage of a fu:lly in t eg ra t ed design.
The arrangement i s i l l u s t r a t e d i n Figs. 1 and 2 where it can be
seen tha t four turbo-compressor loops a r e used.
each loop forms one half of a back-to-back p a i r so t h a t only two
genera tors are required.
The power turb ine i n
FEATURES
Whilst the safe ty aspec ts of a pres t ressed concrete ves se l are
wel l known, some add i t iona l po in t s are worthy of mention s ince they
con t r ibu te t o easy maintenance and s impl i f i ca t ion of the enclosed
components . F i r s t l y t h e water cooled l i n e r can be called upon i n many areas
t o apply a use fu l temperature control .
elastomer s e a l s may be used a t pene t ra t ion plugs giving both
f l e x i b i l i t y and easy removal.
One obvious example i s t h a t
. ~ _ - . - ............... . .....
273
Secondly t h e ves se l l i n e r r e q u i r e s no expansion f e a t u r e s and many
of t h e interconnect ing duc ts r e q u i r e no in su la t ion . Where higher
temperature duc t s are requi red separa te in su la t ed l i n e r s can be
arranged.
removable assemblies.
I n the reference design these have been designed a s
Penet ra t ion diameters need only be l a r g e enough t o pass t h e
contained assemblies, gas plenums and flow pa ths may be made much
l a r g e r by i n t e r n a l l i n e r design.
I n t h e re ference design pre-coolers and i n t e r c o o l e r s are each
b u i l t a s one of t h e pene t ra t ion plugs and no demountable water j o i n t s
are i n s i d e the vessel .
assemblies, mounting may be arranged so t h a t p re s t r e s s ing d i s t o r t i o n s
do not react on machine un i t s .
By arranging machine u n i t s i n self-complete
T h e general philosophy on maintenance i s t o withdraw and r ep lace
Such an exe rc i se should be much f a s t e r than the a u n i t i f necessary,
t a s k of opening up the sealed pressure envelope of a non-integrated
set.
Regarding the machine frames, they only have t o be designed t o
s u i t t he l o c a l p r e s s u r e d i f f e rences and s ince t h e gas plenums
genera l ly l i e outs ide the frame diameters i n t h e ves se l w a l l s , t h e
s i z e and handling weight of each assembly i s s u b s t a n t i a l l y reduced.
The foregoing remarks cover some of the main advantages b u t most i n t e re s t w i l l be centred on t h e problems and one of t h e most important
of these i s t h e achievement of adequate sea l ing between c i r c u i t zones
of s i g n i f i c a n t pressure d i f fe rence . P i s ton r i n g type s e a l s have been
used i n t h e re ference design study b u t it i s not y e t known i f sonic
ve loc i ty leakages may a r i s e and cause e ros ion; some R. & D. work here
i s c l e a r l y necessary.
I n the case of p o t e n t i a l l y hof seals such as those around t h e
H.P. Turbine She l l an Iexcess pressure co ld feed i s appl ied between
mul t ip le r i n g s after bl?ing used t o cool t h e s h e l l and s h e l l hangars.
Leaks towards the tu rb ine i n l e t w i l l degrade the temperature s l i g h t l y
274
and can be made good by a small i nc rease i n r e a c t o r o u t l e t temperature,
b u t leakages downstream towards t h e L.P. tu rb ine involve an e f f i c i ency
loss.
space between ho t face duct i n s u l a t i o n and cold ves se l l i n e r i n su la t ion ,
thus permit t ing a higher h e a t f l u x through t h e h o t f a c e i n s u l a t i o n than
t h a t l o s t t o hea t r e j e c t i o n v i a the vesse l l i n e r .
Where poss ib le , use i s made of t hese flows t o sweep an i n t e r -
S i m i l a r p r i n c i p l e s a r e used f o r the L.P. t u rb ines bu t i f e f f i c i ency
lo s ses a r e t o be minimised any cool ing stream must be l imi ted t o j u s t
s a t i s f y i t s required hea t load and unwanted leakages must a l s o be
m i nimi sed . T h e Table , in Fig. 3 l i s t s t h e effect of an eva lua t ion between a
t h e o r e t i c a l case and t h e p r a c t i c a l case of t h e re ference design where
the lower e f f i c i ency of t h e l a t t e r i s almost en t . i re ly due t o by-pass
cool ing streams and Leakages.
The use of higher gas temperatures has necess i ta ted a new look a t
t h e problem of high temperature i n s u l a t i o n , and i n p a r t i c u l a r f o r t he
under-core plenum which w i l l experience t h e h ighes t temperatures i n t h e
c i r c u i t and which, furthermore, must support -the core load. A s u i t a b l e
so lu t ion which depends on t h e use of s i l i c o n n i t r i d e ( S i N 1 i s
i l l u s t r a t e d i n Fig. 4. Each column of f u e l l e d blocks i n the core r e s t s
on i t s own g raph i t e support column which i s headed by end r e f l e c t o r
blocks and a l l of these members can be removed i f required.
columns a r e seated on slabs of foamed s i l i c o n n i t r i d e which are
mounted i n t u r n on a series of thermal neutron sh ie ld p l a t e s .
reasonably good conductive path f o r hea t f low i s f i n a l l y made by a
l aye r of lead and steel shot compressed t o give a s u f f i c i e n t l y f l a t
upper face f o r near contac t with t h e lowest sh i e ld p la te . If
necessary the s i l i c o n n i t r i d e can a l s o be removed after a graphi te top
l aye r has been cleared.
3 4
The
A
Although t h e thermal conduct ivi ty o f S i N i s not a s low a s one
would l i k e and a knowledge of i t s conduct ivi ty i n the foamed form i s
s t i l l lacking, it appears t o have very a t t r a c t i v e design p rope r t i e s
such a s a very low expansion c o e f f i c i e n t (about ha l f t h a t of g raph i t e ) ,
3 4
275
c.$ a s t r eng th much higher than graphi te and a high thermal shock
r e s i s t ance , I t s behaviour under i r r a d i a t i o n from the l i m i t e d da t a
ava i l ab le t o da t e , looks q u i t e s a t i s f a c t o r y f o r t h i s appl ica t ion . I t s
s t a b i l i t y i n the r eac to r coolant i s t h e o r e t i c a l l y good up t o a t l e a s t
1000°C, b u t f u r t h e r work must be undertaken t o prove i t s s u i t a b i l i t y
on a l l counts.
If t h e r e a r e no problems with the use of s i l i c o n n i t r i d e it will be very s u i t a b l e f o r use a s a high temperature i n s u l a t i o n i n s i d e metal
duct l i n e r s . Should i t be f e l t necessary t o provide a metal covering
t o t h e sur face then methods of a t t ach ing a sheet layer , such a s
molybdenum, can be arranged.
CONTROL
Three b a s i c methods are ava i l ab le f o r load cont ro l :
1.
2.
3 ,
Inventory Control: Where t h e system pressure i s var ied t o s u i t
the load required. T h i s i s the most e f f i c i e n t method b u t t he
speed of response i s dependent on the t i m e required t o change
p res sure.
By-pass Control:
where a by-pass can be used f o r con t ro l purposes.
can be r ap id b u t t he thermal e f f i c i ency of the p l a n t a t lower loads i s poor.
There are var ious pos i t i ons i n t h e c i r c u i t
The response
Temperature Control: By moving r e a c t o r con t ro l rods t h i s
method can be r e l a t i v e l y f a s t i f high r a t e s of r e a c t i v i t y change
are accepted.
previous cases.
The e f f i c i ency a t part-load l i e s between the two
For m a x i m u m f l e x i b i l i t y some combination w i l l very l i k e l y be
used. I f , f o r example, p ressure l e v e l i s set f o r t h e peak load
expected then l imi ted v a r i a t i o n s i n demand can be handled by tempera-
ture con t ro l with l i t t l e loss of e f f ic iency . If quicker response i s
required than can be (achieved by con t ro l rod speed then by-pass
con t ro l i s needed, bu t t h e e f f i c i e n c y loss w i l l be grea te r .
276
Loss of generator load i s a more exac t ing problem and i n t h i s
event a quick ac t ing tu rb ine by-pzss, toge ther with a blocking of the
normal f low path through t h e tu rb ine i s Reeded. A t y p i c a l overspeed
r a t e i s lG% per second so t h a t f u l l d ive r s ion of f low i n about ha l f
a second i s required. A so lu t ion t o t h i s problem can be achieved by
t h e use of mul t ip le poppet valves each held shut by an overpressure
Sellows-sealed ac tua tor through an appropr ia te linkage.
ac tua to r pressure t h e l inkage co l l apses and system pressure blows each
valve open. Twenty-four 10 c m diameter va lves b u i l t i n t o each L.P.
t u rb ine s t a t o r casing provide t h e d ive r s ion i n t h e re ference design
case. The c los ing of t h e path through t h e turb ine i s achieved by
f l a p s which are l inked t o the r e spec t ive ac tua tor and which f o l d i n
from t h e s h e l l t o expose t h e gas path through each corresponding
poppet valve. The gas temperature a t L.P. tu rb ine en t ry i s about
760 C and t o l i m i t t h e temperature of t h e d ive r t ed gas, a g raph i t e
hea t s ink i s interposed which a l s o provides a s u i t a b l e pressure drop
t o r n i n i m i s e pressure t r a n s i e n t s and t h e consequent tendency t o speed
up the H.P. turbine.
By r e l e a s i n g
0
Other by-pass valves do no t seem t o involve any real d i f f i c u l t y .
A clear s p e c i f i c a t i o n f o r t h e i r duty i s dependent on the completion of
con t ro l s t u d i e s b u t they may be t y p i c a l l y as fol lows:
(i) Small by-pass con t ro l valves between H.P. compressors and
H.P. t u rb ine t o give temperature con t ro l of H.P. t u rb ine i n l e t .
One need f o r t h i s valve would b e i n an e a r l y shut down condi t ion
when H.P. tu rb ine load would be small and a low tu rb ine i n l e t
temperature would be needed t o prevent t h e o u t l e t temperature
from being too high.
It can a l s o be used f o r quick load reduct ion.
(ii) A by-pass valve from t h e cold H.P. s i de of t he recupera tor
(13OoC) t o the h o t L.P. s i d e t o produce a l imi ted flow d ive r s ion
w i l l e f f e c t i v e l y cool t h e gas en te r ing t h e recupera tor from t h e
L.P. t u rb ine exhaust.
tend t o co l lapse t h e pressure d i f f e rences between H.P. and L.P.
The use of a thermodynamically s t a b l e a l loy would of course
e l imina te t h i s phenomenon completely. However, t he r e l a t i v e l y poor
mechanical p rope r t i e s of such a l l o y s i n h i b i t s t he designer t o such an
ex ten t t h a t some degree of me ta l lu rg ica l i n s t a b i l i t y must be accepted
i n order t o ob ta in adequate s t r eng th a t opera t ing temperatures.
At ten t ion must also be directed t o t h e choice of a l loy ing add i t ions
and t o t h e na ture of t he p r e c i p i t a t e s t h a t are formed. Very long
per iods a t temperatures approaching the use fu l l i m i t of the a l loy
(from t h e mechanical p rope r t i e s po in t of view) can lead t o continuous
g r a i n boundary p rec ip i t a t ion .
e n t i r e l y d i f f e r e n t corrosion c h a r a c t e r i s t i c s t o t h a t of the parent
metal, and i f f o r example t h e p r e c i p i t a t e i s a t tacked premature
f a i l u r e w i l l occur.
These p r e c i p i t a t e s may w e l l have
A cons idera t ion of t h e above f a c t o r s suggests t h a t t he s t a b i l i s e d
a u s t e n i t i c s ta inless steels (provided they a r e completely f r e e from
sigma phase formation) t h e Inconels , t he Incoloys, I N 102, and f o r
temperatures i n excess of 800 C, molybdenum should b e appropriate . 0
The use of helium avoids any gross cor ros ion problem. However,
t he effect of t he r e s i d u a l impur i t i e s are such tha t they must no t be
overlooked.
t h a t , under opera t ing condi t ions impurity concentrat ions i n the range 1/10 t o 1 vpm t o t a l impur i t i e s can be expected i n a direct cyc le
plant . Although these o r i g i n a t e pr imar i ly from air and moisture
adsorbed on t o the core and t h e r e f l e c t o r g raph i t e - only a small
f r a c t i o n desorbes from metals - they soon e q u i l i b r a t e with t h e l a rge
volume of ho t carbon and graphi te i n t h e core.
r e s u l t s i n a mixture comprising hydrogen, water vapour, carbon
monoxide, carbon dioxide, methane and ni t rogen, t he f i n a l product
having an oxida t ion p o t e n t i a l equiva len t t o a hydrogen - water
mixture of H :H 0 10:l. With the higher temperatures involved i n
the d i r e c t cyc le system t h e r a t i o i s l i k e l y t o be somewhat higher ,
probably approaching 100 : 1.
Experience i n the Dragon Reactor Experiment has shown
This equi l ibr ium
2 2
280
W e have the re fo re a s coolan t , a gas, predominantly helium, a t 0
50-100 atmospheres pressure, a t temperatures up t o 1050 C containing
t r a c e s of impur i t i e s which from the chemico-thermodynamic poin t of
view are reducing t o t h e elements n i cke l , coba l t , i r o n , copper, t i n ,
molybdenum, tungsten, etc., b u t ox id i s ing t o chromium, aluminium,
t i tanium, niobium, etc. The same thermodynamic p r inc ip l e s apply t o
ca rbur i sa t ion due t o t h e presence of methane and carbon monoxide.
The conventional high temperature nickel/chromium a l l o y s are a l l
dependent on an oxide f i l m f o r p ro tec t ion from t h e i r normal environ-
ments.
conducive t o the formatLon of such p ro tec t ive f i l m s , experiments were
put i n hand t o study the phenomenon. Exploratory r e s u l t s , designed
t o assess the general s ign i f i cance of the problem have shown t h a t
s o l i d s o l u t i o n a l loys , e.g., t h e a u s t e n i t i c s ta inless steels and
I N 1 0 2 (Figs . S ( a ) and (b)) are not s i g n i f i c a n t l y a t tacked , whereas
t h e p r e c i p i t a t i o n hardened n icke l chromium a l l o y s undergo se r ious
i n t e r n a l ox ida t ion (Fig. 5 ( c ) ) . Se l ec t ive oxida t ion of the chromium,
aluminium and titanium does not g ive a p ro tec t ive f i l m and a t t a c k
proceeds by i n t e r n a l ox ida t ion which i s d i f f u s i o n cont ro l led . Such
a t t a c k i s p a r t i c u l a r l y dangerous where t h e elements t h a t are oxidsed
play a v i t a l r o l e i n t h e s t r eng th of t h e a l loy , as i s t h e case with
t h e "Nimonic" a l l o y s and related mater ia l s .
A s i t was thought t h a t t he HTR environment might not be
Fur ther work i s requi red t o de f ine t h e working limits of those
ma te r i a l s t h a t have shown promise i n t h e exploratory tests, and both
s t r e s sed and unstressed cor ros ion tes ts are i n hand. A s t h e a t t a c k i s
b a s i c a l l y d i f f u s i o n con t ro l l ed it should be amenable t o p red ic t ion by
studying i t s effect a t higher temperatures and analysing the r e s u l t s
using t h e accepted laws of d i f fus ion and r e a c t i o n r a t e s .
It may w e l l be poss ib le t o p r o t e c t those a l l o y s t h a t are at tacked
by appropr ia te coat ings. Two p r i n c i p l e s seem worthy of study. One,
by using n icke l o r coba l t which being noble t o the environment would
l i m i t oxygen and carbon concent ra t ion and the re fo re reduce d i f f u s i o n
281
r a t e s :
coa t ings which n i g h t form a p ro tec t ive oxide f i l m .
t h e o t h e r with chromim, or possibly aluminium containing
Molybdenum and i t s a l l o y s deserve s p e c i a l mention. Thermo-
dynamicaliy t h e metal i s s t a h l e t o the HTR environment a t temperatures
above 400-5OO0C.
oxida t ion does take place, MOO alone w i l l be formed, which un l ike
MOO i s not v o l a t i l e . Oxidation rates a t these temperatures are very 3 l o w and s ince t h e molybdenum would no t be used f o r components
opera t ing continuously below 700 C ox ida t ion would not appear t o
present any problem. Furthermore, s ince d i f f u s i o n r a t e s i n
molybdenum are neg l ig ib l e a t temperatures below 1000 C ca rbur i sa t ion
o r i n t e r n a l ox ida t ion of a l loy ing elements such a s zirconium should
not prove s ign i f i can t . N o a t t a c k on e i t h e r t h e unalloyed metal o r
on TZM (Fig. 5 ( d ) ) a t temperatures up t o 850°C w a s observed i n any
of the exploratory experiments r e f e r r e d t o above.
Furthermore a t t he lower temperatures, where
2
0
0
Because of t he s p e c i f i c thermodynamic c h a r a c t e r i s t i c s of t h e
impur i t i e s it should be poss ib l e t o develop high s t r e n g t h a l l o y s
using only those elements t h a t are stable t o t h e HTR environment. For
example n icke l , coba l t and i r o n can be considered a s forming the b a s i c
a l l o y with tungsten and molybdenum providing s o l i d so lu t ion
hardening. hardening cha rac t e r i s t i c s . Such a l l o y s being thermodynamically
s t a b l e both with r e spec t t o oxygen and carbon would n o t be expected
t o d e t e r i o r a t e i n serv ice , any l i m i t a t i o n being confined t o t h e i r
mechanical proper t ies .
Copper and t i n would be expected t o provide p r e c i p i t a t i o n
The absence of p ro tec t ive su r face f i l m s focusses a t t e n t i o n on
f r i c t i o n and se i zu re between mating p a r t s which might cause
maintenance d i f f i c u l t y .
has shown t h a t with an appropr ia te design philosophy, s e r ious
problems can i n general be avoided.
work f o r t h e Dragon Reactor it w a s found t h a t a simple c o r r e l a t i o n
ex i s t ed between t h e temperature a t which a pol ished metallographic
sec t ion of t h e metal s t a r t e d t o show thermal e tch ing i n vacuo, and
Experience i n t h e Dragon Reactor Experiment
During component development
282
t he temperature a t which s t a t i c s e i zu re takes place. This t es t i s
very e a s i l y carried o u t and provided an exce l l en t guide a s t o t he
m a x i m u m temperature a t which any p a r t i c u l a r metal o r combination of
metals could be used without s i g n i f i c a n t danger of seizure.
Where mechanisms o r machine motions are involved, temperatures
can usua l ly be kept low enough t o adopt t he already proven methods of
l u b r i c a t i o n even i f cool ing must be arranged.
S l id ing motions caused by expansion w i l l r equ i r e some a t t e n t i o n
where they l i e ou t s ide t h e present range of experience. Demountable
duct l i n e r s and p i s ton r i n g s e a l s may f a l l i n t o t h i s category b u t
w e a r r e s i s t a n t sur face coa t ings on a stable base mater ia l can be
expected t o m e e t t he needs, p a r t i c u l a r l y when the design condi t ions
are eased by reducing temperatures by s u i t a b l e hea t breaks. A n
appropriate app l i ca t ion of a dry lub r i can t such as molybdenum
disulphi.de (MoS ) can a l s o be expected t o play i t s par t . I n general
t h e temperature of such features can be maintained below 600 C without
s e a l cool ing flow, design arrangement can a l s o ensure t h a t any leakage
w i l l involve the passage of cool gas, and hence lower temperatures
would apply.
0 2
Where structural s h e l l s are no h o t t e r than 300-400°C then conven-
t i o n a l mild steels with good f a b r i c a t i o n q u a l i t i e s would be chosen.
Up t o about 550°C low a l l o y steels, such a s the p l a i n molybdenum,
chrome molybdenum and n icke l a l loy steels would appear t o be
appropriate. This would inc lude recupera tor tubes, t u rb ine s h e l l s and
much of the removable duct s h e l l s car ry ing i n t e r n a l insu la t ion .
0 Where the temperature of t h e ma te r i a l i s higher , up t o 750-800 C a
n icke l base a l loy such as I N 102 looks a t t r a c t i v e wh i l s t s a t i s f y i n g
the previous arguments on s t a b i l i t y .
Higher temperature needs, such as i n the H.P. tu rb ines , are more
l i k e l y t o r equ i r e smaller members such as s t a t o r blade carriers and
s h e l l l i n i n g s , and i n the h o t t e s t zones molybdenum TZM w i l l more than
1000 MW (E) DIRECT HELIUM CYCLE HIGH TEMPERATURE REACTOR
GENERAL ARRANGEMENT VERTICAL SECTION -
FIG. I
I
2
3
4
5
6
7
8
9
10
I1
12
REACTOR PRESSURE VESSEL
POWER TURBINE PRESSURE VESSEL
RECUPERATOR AND PRECOOLER CAVITY
TURBO - MACHINERY AND INTERCOOLER CAVITY
FUELLING STANDPIPE POSITIONS
DUCT FROM H P TURBINE
DUCT m RECUPERATOR
L P TURBINE
SHAFT SEAL
SEAL LEAK COLLECTION SHELL
GENERATOR
SPACE FOR H~USINC m s t u SHUT-DOWN COOLING LOOPS AND OTHER PLANT ITEMS
IC00 MW(E) DIRECT HELIUM CYCLE HIGH TEMPERATURE REACTOR
GENERAL ARRANGEMENT. PLAN AND SECTION THROUGH POWER TURBINES DRAGON PROJECT FIG. 2
28 5
c3 3
7 1
FIG. 3 THEORETICAL AND PRACTICAL CYCLE DATA
Fig. 4 Core Support Columns
( a ) S t a i n l e s s S t e e l 347 type 18/8 N b 7 5 0 ~ ~
(b) Nickel Alloy I N 102 750 '~
Fig. 5 ( a ) and (b) Metallographs of Etched Sect ions Showing Attack of Unstressed Specimens Exposed t o Helium Containing 250 vpm CO 250 vpm H and 50 vpm H 0 f o r 3,000 hours 2 2
Fig.
0
(c) Nimonic 105 85OoC
(d ) Molybdenum Alloy TZM 850'C
(d) Metallographs of Etched Sections Showipg Attack of Unstressed Specimens Exposed t o Helium Containing 250 vpm CO 250 vpm H2 and 50 vpm H 2 0 f o r 3,QOO hours
288
DISCUSSION
R. Huddle: I should l i k e t o add a word t o what George Lockett has
s a i d . The des ign presented was developed on t h e b a s i s t h a t it w a s going
t o be d e t a i l e d and b u i l t . It i s not a n academic des ign - each and every
p a r t can be made from materials t h a t e x i s t today. Some may need f u r t h e r
proving, bu t it i s a f r a c t i o n a l pe r tu rba t ion , ready f o r d e t a i l i n g and con-
s t r u c t i o n . Regarding materials, emphasis has been placed on s t a b i l i t y and
r e l i a b i l i t y . The only r e a l l y unconventional materials are s i l i c o n n i t r i d e
(which i n c i d e n t a l l y i s marketed he re by Haynes S t e l l i t e ) and molybdenum - two m a t e r i a l s used f o r duc ts and l i n e r s .
we g e t a n oppor tuni ty t o do so.
We can b u i l d it now - l e t ' s hope
M. Bender: Considering t h e r e l a t i v e l y low thermal e f f i c i e n c y (45$) , w h a t i s the economic i n c e n t i v e f o r gas t u r b i n e sys tems? Does the t a r g e t
have t o be 50% e f f i c i e n c y o r more?
G. E. Locket t : There i s no s p e c i f i c t a r g e t e f f i c i e n c y . The r e s u l t s
of s tudying t h i s r e fe rence des ign show t h a t t h e t h e o r e t i c a l cycle wi thout
bypassing and h e a t l o s s e s , compared w i t h t h e p r a c t i c a l case, reduces t h e
p l a n t e f f i c i e n c y from 47.47 t o 45.24$. The economic i n c e n t i v e i s t o re- duce t h e gene ra t ing cos t by reducing c a p i t a l cos t and f u e l cyc le cos t
whenever poss ib l e . The r educ t ion i n p l a n t and b u i l d i n g s i z e compared wi th
t h e steam cyc le i s expected t o do t h i s without any emphasis on e f f i c i e n c y .
However, any improvement on thermal e f f i c i e n c y w i l l permit a given power
output t o be obta ined from a smaller r e a c t o r core.
a t tempt ing t o g e t a n a p p r e c i a t i o n of p r a c t i c a l p e n a l t i e s and t o expose any
previous ly unseen problems.
This e a r l y s tudy i s
K. 0. Hin temann: I n f o s s i l - f u e l e d , c losed-cycle gas tu rb ine p l a n t s
t h e a i r h e a t e r t akes almost ha l f of t h e c a p i t a l cos t .
roughly comparable i n gene ra t ing cos t w i th a steam cycle .
gas t u r b i n e p l a n t t h e "air hea ter ' ' i s rep laced by t h e r e a c t o r .
t h e r e must be a n economical i n c e n t i v e provided t h e r e a c t o r i s not ve ry
much more expensive.
Such a p l a n t i s
I n a nuc lear
Therefore ,
289
M. I h l l e Donne: What material d id you consider for t h e duc t ing a t temperatures of about 190OoC, which i s t h e helium tempertiture a t t h e reac-
t o r o u t l e t t h z t you assumed ?
G. E. Locket t : We have considered t h e use of s i l i c o n n i t r i d e mostly
on t h e i n s i d e of t h e tubu la r metal s h e l l s . The core support mounting is
a l s o based on the use of s i l i c o n n i t r i d e .
W. Twardziok: Is emergency cool ing accomplished with t h e high pres-
sure turbo s e t ? How can you sepa ra t e t h e sys tems?
G. E. Locket t : There are fou r turbo-compressor u n i t s feeding two
back-to-back p a i r o f power tu rb ines , thus the re are four p a r a l l e l pa ths ,
bu t t h e r e i s a l i n k i n g po in t between t h e back-to-back power tu rb ine ex-
hausts . For normal opera t ion i t becomes e f f e c t i v e l y a two loop system
wi th two turbo-compressor sets i n each.
i t i s poss ib l e t h a t t h e p l a n t would be run using one genera tor only wi th
i t s a s soc ia t ed two turbo-compressor loops. To satisfy t h e problem of
emergency cooling, failure of one of t h e turbo-compressor u n i t s should
not prevent t h e remaining uni t from cont inuing t o run - a t l e a s t t o an
adequate ex ten t .
bu t it would be necessary t o c lose t h e blocking valve i n t h e f a i l e d turbo-
compressor loop t o prevent backflow. There w i l l remain, however, a bypass
flow rou te around the tu rb ine of t h e good turbo-compressor u n i t . This may not be too important i f appropr i a t e r e s i s t a n c e i s engineered i n t o the
l eak ing po in t between t h e two power t u r b i n e exhausts . It i s poss ib le t o
reduce t h e temperature of t h e bypass flow by p a r t l y opening t h e c o n t r o l
va lve between t h e high pressure compressor o u t l e t and t h e high pressure
i n l e t of t h e f a i l e d u n i t . There remains, of course, t h e p o s s i b i l i t y o f
s t a r t i n g up t h e o the r p a r t of t h e system as convenient i n preference t o
using one-half of t h e f a i l e d loop p a i r a lone.
as t o whether a n a t tempt should be made t o keep t h e genera tor running a t low output i n order t o s a t i s f y t h e base load. F’rom t h e ope ra t iona l po in t
of view, it would be more s t ra ight forward t o use both genera tors even a t power outputs of below 50s so t h a t a fa i lure i n one-half o f t h e system
w i l l a l low it t o be f u l l y shut down and allow t h e o the r ha l f t o continue
For load outputs of 50$ or l e s s ,
The behavior has not y e t been s tudied i n any depth,
Fur ther ques t ions ar ise
0 genera t ing without i n t e r rup t ion .
290
W. Twardziok: What i s t h e overspeed of t h e power t u r b i n e when you
have a load dec rease?
G. E. Locket t : I n t h e event of l oad l o s s , t h e power tu rb ine over-
speed need not exceed 10%. t u r b i n e and genera tor r o t o r be ing about 10% per second.
f i c u l t y i n opening bypass va lves qu ick ly t o d i v e r flow around t h e power
t u r b i n e i f mul t ip l e poppet va lves are used as shown i n t h e a t t ached f i g u r e .
These can ope ra t e t o d i v e r t flow i n 30 t o 50 mil l i seconds .
0 .2 seconds i s made be fo re t r i p p i n g t h e bypass and a l i b e r a l allowance made
for incomplete bypassing, a n overspeed of about 7$ might be reached.
A t y p i c a l a c c e l l e r a t i o n of t h e coupled power
There i s no d i f -
If a pause of
- . . . .. . . . . .. ... . . . - -~ .
291
PRESSURE VESSEL TECHNOLOGY
AND SAFETY TOPICS
(Session I V )
292
Chairman : T. A. Jaeger, Bundesansta 1 t F i r Ma teri alpruf ung
Co-Chairman: H. J. deNordwall, Oak Ridge National Laboratory
Paper l/125
/ I (t 5 F. P. 0. Ashworth
OECD Dragon P ro jec t QLi .
ABSTRACT
The methods of assess ing the f i s s i o n product r e l e a s e and t h e
They a re appl ied t o a no t iona l core t o demonstrate t he g raph i t e cor ros ion i n a High Temperature Gas Cooled Reactor are reviewed. ava i l ab le margins and t o i n d i c a t e t h e p r i o r i t i e s of information.
These p r i o r i t i e s are shown t o be t h e ob jec t ives of the f i s s i o n product and corrosion work underway i n t h e Dragon Reactor Experiment programme.
293
294
INTRODUCTION
Safety arguments f o r r e a c t o r s a r e developed alongside t h e
technology i n t o what becomes a r igorous examination of the p r i n c i p l e s
and p o t e n t i a l of t he system. I n a r e s t r i c t i v e sense t h i s i s d i r e c t e d
towards assess ing p o t e n t i a l hazards. However, t h e t echn ica l
pene t ra t ion requi red provides a unique method of assess ing a l s o t h e
s tandards requi red of the experimental work, t h e ca l cu la t iona l methods,
qua l i t y con t ro l s and the opera t iona l p rac t i ces .
The ob jec t of t h i s paper i s t o examine what these requirements
are f o r t he f irst HTR i n the UK and t o relate them t o t h e present
s ta tus of f u e l development a s descr ibed by D r . Graham, the f i s s i o n
product release s tud ie s ( D r . F lowers) , core design ( M r . Smith) and
management of the reactor experiment as described by Mr. Chapman.
The paper deals f i rs t w i t h t he best present estimates of f i s s i o n
product r e l e a s e and corrosion i n design and t r a n s i e n t condi t ions ,
explores i n each case the l i m i t a t i o n s and ava i l ab le margins which
arise from present da t a and then r e l a t e s t hese design and opera t iona l
r e s t r i c t i o n s t o t h e Dragon Reactor Experiment and i t s a t tendant
re search work.
METHODS OF ASSESSMENT
Safety begins a t t h e design s t age i n a way which i s more obvious
than f o r previous gas-cooled r eac to r s . Designers, s a fe ty assessors
and opera tors demand t o know the l i m i t s imposed by the p a r t i c l e
coa t ings and the g raph i t e can which c o n s t i t u t e t he b a r r i e r s t o f i s s i o n
product r e l e a s e unique t o an HTR because these appear a t f i r s t s i g h t
t o be vulnerable t o imperfect ions i n manufacture, t o cor ros ion and t o
mechanical damage.
The a r ray of accident s i t u a t i o n s which are judged necessary t o be
considered i s smar i sed i n Table 1.
The s t a r t i n g po in t i s a re ference core devised t o r ep resen t a s
r e a l i s t i c a l l y a s poss ib le the equi l ibr ium composition of f u e l channels
of var ious ages, nominal temperature d i s t r i b u t i o n s and f i s s i o n product
c
Table 1. Reactor Conditions t o be Analysed
Si tua t ion Typical Faul t s
Normal Operation Radiation doses not riot exceed some a r b i t r a r y f rac t ion of t h e ICRP recommended annual dose.
Category A Accident Could occur several t i m e s i n a s t a t i o n l i f e . Radiation doses do not exceed ICRP recommended annual doses.
Category B Accident Probabi l i ty of occurrence no more than once i n a s ta t ion l i f e .
Category C Accident
C i r c u i t Access
Probabi l i ty of occurrence i s so low as t o be discounted. Analysis of safeguards and consequences of accident necessary t o support the judgement of t h i s probabi l i ty .
(i) Circulator inspection o r removal.
(ii) Inspection and repair of s t a t i c i n s t a l l a t i o n s such a s hot and r e t u r n gas ducts, hot plenum insulat ion.
(iii) Large scale i n s t a l l a t i o n s designed t o be removed with accompanying long shutdown (boi le rs ) .
Fuel pin f a i l u r e s leading to small sca le increases i n a c t i v i t y re leases .
( a ) Pressure c i r c u i t breach of about 45 square inches, equivalent area.
Coolant s ta rva t ion of a s ing le channel with delayed t r i p .
Fa i lure of a s ingle b o i l e r tube with feed water and r e a c t o r t r i p .
(b)
(c)
( a ) Boi ler tube f a i l u r e with simultaneous c i r c u i t depressurisat ion through r e l i e f valves.
( b ) Major breach of primary c i r c u i t .
( c ) Gross overheating of several f u e l columns.
Once i n 2-3 years.
9nce o r t w i c e i n s t a t i o n l i f e .
Very infrequent.
296
Q inventor ies . Onto t h i s core are imposed the estimated peak systematic
and peak random temperatures which a r i s e from f l u x t i l ts , changes i n
gap s i z e s during i r r a d i a t i o n , coolan t by-passing, etc. The f u e l
compacts are charac te r i sed by t h e as-produced uncoated f r a c t i o n of
p a r t i c l e s and the cu r ren t p a r t i c l e f a i l u r e limits i n terms of burn-up,
dose and temperature.
The rou te f o r es t imat ing t h e f i s s i o n product release i s shown i n
Fig. 1.
and the ca l cu la t ions are en tered with es t imat ions of s ing le channel
r e l eases .
failure, i f any, of p a r t i c l e coa t ings which toge ther w i t h t he
production q u a l i t y c o n s t i t u t e t he source terms. Following the
es t imat ion of f i s s i o n product l nven to r i e s a t each t i m e s tep, the m e t a l
release f r a c t i o n s are estimated using a model of t h e d i f f u s i o n and
evaporation processes i n t h e f u e l and g raph i t e reg ions of t h e channel.
Iodine and f i s s i o n gas releases are s i m i l a r l y ca l cu la t ed with t h e
important d i f f e rence t h a t hold-up i s con t ro l l ed almost e n t i r e l y by
d i f f u s i o n i n the kerne l ma te r i a l of t he p a r t i c l e s .
The d a t a requirements from t h e core design are first spec i f i ed
A t t h i s po in t t h e d a t a i s used t o c a l c u l a t e t he serv ice
If abnormal condi t ions a r e t o be examined, the t r a n s i e n t da t a are
fed i n t o the channel da t a , and i n t h e course of t he ca l cu la t ion , t he
nuclear da t a , the d i f f u s i o n c o e f f i c i e n t s of the f u e l and g raph i t e
reg ions and t h e i r temperature and concent ra t ion dependences are
entered.
A f t e r t he s tage of a x i a l i n t e g r a t i o n , a comparison of var ious
channel concepts i n terms of t h e i r f i s s i o n product r e l e a s e
c h a r a c t e r i s t i c s can be made, which r e t u r n s t o the designer and t h e
f u e l manufacture a s a coarse s e t t i n g of performance and qua l i ty l i m i t s .
The next s t age i s t h e r ep resen ta t ion of the complete equi l ibr ium
core by weighting each c h a r a c t e r i s t i c channel r e l e a s e and t h i s l eads
t o t h e comparison of t o l e r a b l e release r a t e s i n terms of c u r i e s per
year o r e f f e c t i v e re lease- to-b i r th r a t i o from the core.
This comparison allows the s e t t i n g of c l o s e r l i m i t s on the channel
performance and t h e f u e l spec i f ica t ion . It provides a q u a n t i t a t i v e
297
6d assessment of t h e merits of each type of coa t ing and t h e requirements
of t he experimental programme t o determine d i f f u s i o n and evaporat ion
data. F i n a l l y , it provides an es t imate of ava i l ab le marqin, defined
a s the r a t i o between t o l e r a b l e and predic ted r e l e a s e , which can be
used as an opt imisa t ion parameter, o r r e f e r r e d back through the channel
performance t o t h e p a r t i c l e qualit!( con t ro l and t o t h e opera t ion of
t he reac tor .
The corresponding rou te f o r corrosion es t imat ion i s shown i n
Fig. 2. The same re ference core da t a i s used a s inpu t b u t it i s more
convenient t o cha rac t e r i s e t h e core by graphi te surface zones each
with a p a r t i c u l a r a x i a l p ro f i l e . E f fec t ive ly , a histogram of sur face
temperatures i s u'sed i n the ca l cu la t ion of i n t eg ra t ed core chemical
r e a c t i v i t y . The t o l e r a b l e t o t a l water inleakage i s set by t h e
t o l e r a b l e corrosion a t t h e h o t t e s t g raph i t e surface and t h i s i s
entered toge ther with t h e in t eg ra t ed core r e a c t i v i t y i n t o t h e
es t imat ion of t o l e r a b l e inleakage.
The output provides an es t imat ion of t h e ava i l ab le cor ros ion
margin a t any t i m e and pos i t i on i n t h e core which, because the
r eac t ions are first order t o a c l o s e approximation, i s simply
expressed a s a t o l e r a b l e exposure i n micro-atmosphere days.
A t t h e high water concentrat ions which could occur following a b o i l e r tube fa i lure , t h e steam graph i t e r e a c t i o n r a t e s are determined
by the t r a n s p o r t processes of r e a c t a n t s and r e a c t i o n products wi th in
t h e graphi te as w e l l as t h e r e a c t i o n rates. Therefore it i s necessary
t o c a l c u l a t e t h e chemical r e a c t i v i t y of each a x i a l zone accounting f o r
these processes a t var ious times during t h e inc iden t t o take account
of the changing d i s t r i b u t i o n s of h e a t and temperature and t h e
a l t e r a t i o n s of coolant composition and mass flow.
embodied i n the TUBER code.
This r o u t e i s
APPLICATION TO A REFERENCE CORE
The da ta f o r a p a r t i c u l a r core design i s out l ined i n Fig. 3 and
T a b l e 2. It was chosen d e l i b e r a t e l y , a s a non-optimised design t o
298
Table 2. Reference Core Data
Core Power Power Density Core Height ( f u e l l e d ) Core Diameter N u m b e r of channels Age f a c t o r Radial Form Factor
Channel Diameter Outer Fuel Pin D i a m e t e r Inner Fuel Pin D i a m e t e r Graphite Tube Thickness ( inner and o u t e r ) Fuel Density Peak Channel Power (new f u e l ) Peak Channel D w e l l T ime
1500 MW(th) 7.5 kW/litre 500 an 768 an 4,630 1.35 1.37
6.5 an 5.8 cm 2.5 cm 0.5 an
1.0 g /m3 (heavy metal) 0.6 MW 730 days
~
Core Zones Radius Number of Channels Power Factor
cm
- 1 55 96 1.0
2 111 288 0.96
3 166 4 8 3 0.895
4 2 2 1 670 0.79
5 276 861 0.67
6 38 4 2,234 0.45
Table 3. Available Margins f o r Reference Core
Access (1 week, Fa i led Boiler Tube Depressurisat ion
through Safety Valve Stack Discharge)
Continuous Release Shielding 1o Depressurisat ion through 45 sq i n Hole
(Ground Level 1 hon-Unif om Nuclide (Stack 10 m No F i l t r a t i o n ) Disuribution)
~
Caesium- 137 52 2.2 3 30 >300
Strontium-90 30 4.1 75
Iodine-131 0.9 2.3 2.0 25
299
@ demonstrate how the r e l e a s e and czr ros ion es t imates influence the
design and da ta requirements. The serv ice f a i l u r e of f u e l was
est imated from t h e t o t a l f i s s i o n gas and carbon monoxide pressure
developed a t a p a r t i c u l a r temperature and burn-up, using a s a
c r i t e r i o n of f a i l u r e the t i m e a t which the compressive stress i n t h e
s i l i c o n carbide diminishes t o zero. This proport ion was added t o t h e
assumed production de fec t s and shown i n Fig. 4 which shows t h i s de fec t
f r a c t i o n i n the h o t t e s t 20% of the peak channel. The remainder of
t h a t channel and channels i n each zone were examined i n the same way.
'The es t imat ing rou te was fo1:lowed down t o t h e f r a c t i o n s of
caesium-137 and strontium-90 re leased p e r year and the Release t o
B i r th Rate r a t i o f o r Iodine-131. The r e su l t s a r e shown i n Figs . 5,
6 and 7 , where these f r a c t i o n s a r e p lo t t ed a s func t ions of t he
s t a r t - o f - l i f e de fec t f r a c t i o n . A t t he 5 i n 10 de fec t f r a c t i o n , the
r e l e a s e s due t o serv ice d e f e c t s a r e superinposed.
4
This b r ings out c l e a r l y the f a c t t h a t end-of-l ife f a i l u r e t o
l e v e l s of 2-3% of the f u e l par t ic l -es has a r e l a t i v e l y small e f f e c t
on the r e l e a s e t o t h e c i r c u i t of caesium and strontium. This i s due
t o the t ransmission delay imposed by the graphi te sleeve.
These predicted r e l e a s e s a r e r e l a t e d t o the t o l e r a b l e l e v e l s i n
t e r m s of t he ava i l ab le margins i n T a b l e 3, where i t can be seen t h a t
these a r e considerable margins even f o r t h i s unoptimised design and
p a r t i c l e f a i l u r e f r a c t i o n . Only i n t h e case of t h e continuous release
of iodine-131 i s the margin less than one. I n analysing the t o l e r a b l e
l e v e l , an e f f e c t i v e s tack he ight of 10 metres was assumed, with no
f i l t r a t i o n and no decontamination i n t h e helium l eak path between the
primary c i r c u i t and the s tack exit.. The r e s u l t s from the Dragon
Reactor leakage and a c t i v i t y measurements are d i r e c t l y r e l evan t and
w i l l be supplemented with d e l i b e r a t e leak behaviour experiments.
Therefore a p a r t from the development of f u e l and production methods,
engineered safeguards are ava i l ab le t o improve t h i s margin 20 o r 30
t i m e s without except ional expense.
300
This f a c t o r i s necessary t o allow f o r any conservat ive downwards adjustment of the t o l e r a b l e continuous r e l e a s e t o atmosphere.
Corrosion Analyses
The design cr i ter ia of cor ros ion are the t o l e r a b l e graphi te sur face a t t a c k o r loss of sec t ion a t t h e h o t spot , t he bulk corrosion
and loss of mechanical s t r eng th of t he g raph i t e below 800 C and the corrosion of t he f u e l mat r ix i n reg ions where t h e graphi te temperatures
a r e l o w enough t o allow penet ra t ion of r eac t an t .
g r e a t e s t r i s k i s where the s leeve temperatures are a t 750 C and the
f u e l 50 C o r more h o t t e r .
0
The reg ion of 0
0
O f these cr i ter ia , i n normal opera t ion , t h e present view i s t h a t t he loss of sec t ion a t t h e hot-spot i s t h e most severe. The l i m i t i s
set a t 100 mg/cm , corresponding t o an average removal of 0.6 mm from
a 5 mm tube, with l o c a l p i t t i n g reaching up t o approximately 2 mm.
2
This l i m i t , t he re fo re , toge ther with the temperature d i s t r i b u t i o n s
of the r e a c t o r zones a r e entered i n t o the cor ros ion c a l c u l a t i o n route . The r e s u l t s of t h i s ca l cu la t ion are shown i n Table 4. The g raph i t e
chemical r e a c t i v i t y was assumed t o be t h a t measured f o r Gilsocarbon
(1.2 x mg c m h patm a t 1273OK). The f a c t t h a t t h e
c a l c u l a t i o n assumes t h a t a l l t he water r e a c t s with t h e core , whereas
some 20% i s removed by the p l an t , accounts f o r t he margin ava i l ab le a t t h e hot-spot, which was taken t o be a t t h e peak random temperature
of the cen t r e channel. The ava i l ab le margins i n t h e peak channels of
t h e outer zones always exceed t h i s value, t ak ing the longer dwell
t i m e s i n t o account a s well.
-2 -1
The r e a c t o r can be operated with an in t eg ra t ed water inleakage of up t o 300 kg/year before it i s necessary t o discharge cen t r e zone
channels of high burn-up because of corrosion l imi t a t ions .
The extreme case of a spontaneous b o i l e r tube f a i l u r e which could
i n j e c t water a t r a t e s between 10 and 40 kg/s up t o a t o t a l of 2,000 kg
has been considered by Kinsey and Rgmberg.
r e a c t i o n with the core , no a l t e r a t i o n of t h e graphi te temperatures
was assumed, and no f a s t water de t ec t ion and dumping taken i n t o
Because of the r ap id
301
0 account. The l i m i t of 2,000 kg was chosen a r b i t r a r i l y ; obviously I I t he t o t a l removal of graphi te under these assumptions i s approximately
l i n e a r l y proport ional t o the t o t a l r eac t an t . The t o t a l g raphi te
removal was 1,800 kg w i t h a m a x i m u m l i n e a r a t t a c k a t the hot-spot of I ~
L about 80 mg/cm . The maximum a t t a c k of t he p a r t i c l e s by water
pene t ra t ing t h e s leeves i n lower temperature reg ions was the removal
of about 2 mm of t h e mat r ix ma te r i a l and 10 microns of t h e outer
pyrocarbon of t h e p a r t i c l e s i n t h a t region. The reduct ion of the
contaminants by t h e clean-up p l an t t o 1% of t he i r peak values took
8 hour s . Two conclusions emerge from t h i s work. F i r s t , t h e a t t a c k i s
nowhere severe enough t o cause s t r u c t u r a l failure of t he f u e l pins.
I n f a c t a l a r g e proport ion of the core remains wi th in the t o l e r a b l e
corrosion margins, and could be operated. Second, t h e t o t a l removal
of caesium and strontium i s wi th in the ava i l ab le margin of r e l e a s e
through a relief valve, although t h e complete case of subsequent
dep res su r i sa t ion has not been analysed.
DISCUSSION
The f i s s i o n product r e l e a s e and corrosion es t imat ions f o r an HTR
were s ingled out of t he wider s a fe ty analyses because they r ep resen t
t h e areas of proof which d i f f e r most from other-gas-cooled reac tors . A measure of confidence i s created by the f a c t t h a t the inpu t da t a i s
being obtained from measurements i n condi t ions and geometries which
do not involve l a rge ex t rapola t ions . It is , however, worth examining
t h e e f f e c t of e r r o r s i n t h i s data.
I f the value of t he graphi te d i f f u s i o n c o e f f i c i e n t f o r strontium,
f o r example, were increased by a f a c t o r of x 3, t h e re leased f r a c t i o n
per year would increase by a f a c t o r of about 1.5, and i f , separa te ly ,
t h e evaporation c o e f f i c i e n t w e r e increased by t h e same f a c t o r , t he
release would be increased by x 2. Both are requi red , therefore , t o
about t h e same accuracy as t h e s t a r t -o f - l i f e source t e r m . For both
these metals, t he e f f e c t of end-of-life f a i l u r e of f u e l i s shielded
by t h e delay t i m e i n t he g raph i t e and a f a c t o r of x 3 a t 80%
302
i r r a d i a t i o n f o r example i s judged not t o czuse an increased r e l e a s e
of more than 20%.
However, t h e iod ine r e l e a s e i s more s e n s i t i v e , and the loca t ion
of de fec t ive f u e l t o wi th in st small number of channels (say 25) would
provide the opera tor with p rec i se knowledge of t he end-of-l ife
behaviour f o r which p red ic t ions must i ncu r p e n a l t i e s i n terms of
t o l e r a b l e f u e l l i fe .
An important parameter i n t h e es t imate of iod ine a c t i v i t i e s i s
the temperature dependence of re lease . A value of 68 kcal/mol f o r
t he d i f f u s i o n c o e f f i c i e n t of i od ine i n the f u e l g ra in i s based on the
measurements of xenon d i f f u s i o n i n s i n g l e c r y s t a l UO
of changing t h i s value i s shown below on the r e l e a s e from the peak
channel of t h e core def ined i n t h e previous sec t ion .
The e f f e c t 2 -
Act iva t ion energy 40 68 80 kcal/mol
Iodine-131 r e l e a s e from 140 120 80 c u r i e s / s x lo-’ channel a t 20% i r r a d i a t i o n
The corrosion p red ic t ions are l i n e a r l y proport ional t o the water
i n g r e s s r a t e assumed and the in -p i l e g raph i t e r e a c t i v i t y - and
logar i thmica l ly dependent on temperature. However, t h e adequacy can
be checked d i r e c t l y by i n j e c t i o n experiments i n the Dragon Reactor,
and the designed d i s t r i b u t i o n s of t he graphi te temperatures which are
monitored i n t h e core. A p a r t i c u l a r example i s the app l i ca t ion of the
cor ros ion es t imates t o t h e Charge 3, Core 6 w h i c h p red ic ted a core
chemical r e a c t i v i t y of 2.4 h- l , assuming a l l t h e graphi te t o be G 5
ma te r i a l , and 7.2 h f o r Gilsocarbon graphi te , using out-of-pile
ox ida t ion data . The measured value was 4.0 h . The majori ty of
t he g raph i t e was, i n f a c t , Gilsocarbon and the r e s u l t i s reasonably
good when a probable e r r o r of 550 C a t t h e hot-spot i s taken i n t o
account. Previous c o r r e l a t i o n s f o r experiments i n Charges 1 and 2
have been reported showing the same o r b e t t e r agreement .
-1
-1
0
F i n a l l y , t he i n t e r a c t i o n between corrosion and f i s s i o n product
r e l e a s e i s an a rea where c a l c u l a t i o n s r equ i r e c lose support from n
303
6.$ experiments; t h i s inc ludes t h e removal of plated-out metal f i s s i o n
products and iod ine from primary c i r c u i t sur faces during a b o i l e r
tube f a i l u r e accident. The ava i l ab le margins i n these cases a r e
l a rge and r ep roduc ib i l i t y b e t t e r than a f a c t o r of 5 i s probably not
important. The planned work a t Dragon i s mentioned below.
DRAGON REACTOR EXPERIMENTS
The instrumentat ion and sampling systems i n use inc lude t h e
following:
( a ) t h e purge sampling system which enables t h e f i s s i o n gas
a c t i v i t i e s t o be monitored from each of the purged f u e l elements,
( b ) two f a s t purge sampling l i n e s through which the gas t r a n s i t
t i m e i s about 2 seconds,
( c ) t h e Dracule probe which enables t h e core exit gas t o be sampled
a t r a t e s up t o 100 l i t r e s / m i n and i n which plate-out probes of
var ious ma te r i a l s can be i n s e r t e d ,
( d ) the fas t response loop f o r sampling the bulk coolant a c t i v i t y
and f o r t he i n j e c t i o n of gaseous impur i t i e s ,
( e ) the centre-spike i n j e c t i o n f o r s i n g l e element cor ros ion tests
and tests of t h e iMluence of corrosion on the r e l e a s e of metal
f i s s i o n products,
(f) various coolant sampling f i l t e r s .
These are shown schematically i n Fig. 8.
The f a c i l i t i e s have been i n s t a l l e d progressively with the
ob jec t ive of using the r e a c t o r t o prove t h e p red ic t ion methods and
two exe rc i se s are a t p resent i n progress.
The f irst i s t o log the exposure of each element t o oxida t ion
by synthes is ing the core chemical r e a c t i v i t y R from t h e temperature
scans and the r e a c t i v i t y of each g raph i t e component. The l i m i t of
impurity i n j e c t i o n t o l e r a b l e a t any t i m e i s then estimated.
I n j e c t i o n i n t o t h e bulk coolant provides a measured value of Re and
C
304
i n j e c t i o n i n t o the cen t r e element of continuous high concentrat ions
(1,000 patm) provides an in -p i l e c a l i b r a t i o n of t h e oxidat ion r a t e s
by t h e subsequent measurements of weight loss and corrosion p ro f i l e .
This f a c i l i t y i s used simultaneously t o simulate t h e leakage of
coolant through f u e l p in end-cap f e a t u r e s and the consequent corrosion
of t he matrix.
The r e a c t o r i s now opera t ing wi th new, uncontaminated hea t
exchangers and w i t h su r f aces elsewhere w e l l monitored f o r deposited
and induced a c t i v i t y . This represented a good s t a r t i n g poin t f o r
t he second exerc ise , t h e t e s t i n g of a c i r c u i t a c t i v i t y con t ro l method.
The procedure i s :
( a ) t o c o l l a t e t he information a v a i l a b l e from f u e l production concerning the quant i ty and d i s t r i b u t i o n of exposed f i s s i l e
ma te r i a l i n each element,
( b ) t o r e l a t e t hese source terms by t h e in -p i l e purge sampling
of f i s s i o n gases,
(c ) t o c a l i b r a t e t h i s gas sampling with re ference f u e l elements
containing a known proport ion of uncoated kerne ls ,
( d ) t o p r e d i c t t h e metal r e l e a s e s i n t o t h e graphi te and coolant
from t h e re ference element,
( e ) t o check these p red ic t ions f o r bo th t h e re ference and c e r t a i n
o the r elements by pos t - i r r ad ia t ion analyses.
These exe rc i se s enable both the corrosion and a c t i v i t y r o u t e s
t o be checked. The f irst r e s u l t s i n both are encouraging.
The behaviour of f i s s i o n products once they have l e f t t he
graphi te sur faces are inves t iga t ed i n a t h i r d system of measurements.
The bulk gas a c t i v i t y i s monitored f o r gases, i od ines and metals i n
the f a s t probe and t h e plate-out probe, and the da t a i s used t o
determine t h e plate-out behaviour and eventual-ly the decontamination
f a c t o r s f o r iod ine and metals.
305
Because the migrat ion of strontium and caesium t o the coolan t i s
long compared t o t h e average f u e l element dwell t i m e s , a proposal by
D r . Freck of t he Central E l e c t r i c i t y Generating Board t o pre-load
a g raph i t e f u e l tube with strontium-85 and t o monitor t h i s gamma-
a c t i v i t y i n t h e probe i s being pursued, and i s planned t o be in se r t ed
i n September 1970. F ina l ly , t h e inf luence of cor ros ion on t h e
evaporat ion of strontium-85 from pre-loaded graphi te w i l l be ca r r i ed
out i n t h e cen t r e spike i n j e c t i o n f a c i l i t y .
CONCLUSIONS
T h e methods of assessing t h e behaviour of f i s s i o n products
and the cor ros ion i n an HTR which w i l l form p a r t of t h e sa fe ty
arguments used by the Design and Construction Companies have been
described. The f i s s i o n product and chemistry programmes f o r t he
Dragon Reactor have been planned t o prove these methods as r ap id ly
as poss ib le i n condi t ions which simulate a power r e a c t o r a s c lose ly
a s possible .
Present da t a has been appl ied t o a no t iona l r e a c t o r core t o
i n d i c a t e t h e ava i l ab le margins. These are adequate except f o r the
continuous r e l e a s e of iod ine f r o m , f u e l which f a i l s during i r r a d i a t i o n ;
proof of back-up safeguards i n a helium system i s underway.
corrosion margins both i n 'normal' opera t ion ( 'normal ' in leakage i s an e l u s i v e quant i ty) and i n acc ident condi t ions also appear adequate
using present information.
The
The present cycle of p red ic t ion and measurement i n the Reactor
Experiment w i l l provide a major p a r t of t he confidence i n these
methods . ACKNOWLEDGMENT
The confidence i n t h e sa fe ty of an HTR stems from the work of
t he e n t i r e Project .
i n t h i s lecture, p a r t i c u l a r acknowledgment i s due t o the Dragon
Operations Group, t h e Mater ia l s Divis ion and the team a t Harwell l ed
by D r . Flowers. I would l i k e t o thank, i n p a r t i c u l a r , D r . Rowland,
I n the i n t e r p r e t a t i o n of t h e sa fe ty aspec ts made
306
Messrs. W. Browning and D. Kinsey f o r t h e i r valuable cont r ibu t ions
and M r . R. Gray and Mrs. Macey f o r t h e i r e f f o r t s i n preparing t h i s
WNALTI OI S m - D Q N FOR BOILER t- IAI- 3ML3R LBM SFECIPICATIOII ( SIZS AND DURATION )
s p E c I ? I C A T I ~ , CAF'ACITY AND REcEIQwIoII CYCLB
Fig. 2. Route for Assessment of Circuit Chemistry Ana Core Corrosion.
308
1 0 4
1 o-2
E 9 ti E
10-5
-4 10
I I I I
~ AXIAL E3IGtW Z -- 20 40 60 BO 1 0
Fig . 3 . Peak Sys tema t i c Fue l and Graphit , : Su r face Tem- p e r a t u r e s f o r t h e Peak Channel O E t h e Refer- ence Core.
I I
/ f
400
2w
0
Fig. 4. Es t ima ted P ropor t ion of Exposed Fue l During S e r v i c e (Peak Channel Hot-Spot).
0 20 40 60 l a l % IRRADIATION
. . . . . . . - . - .. - -.-
309
U h
F i g . 5. E f f e c t i v e Uniform F a i l e d P a r t i c l e F r a c t i o n Throughout L i f e .
F i g . 6 . E f f e c t i v e Uniform F a i l e d P a r t i c l e F r a c t i o n Throughout L i f e .
8 1 3 7 , 8. 140
t i v a t i o n products mbably in d u t
Cr 51, UI 54. le 51. Sb 124, Co 60, A8 1 '
3 10
E f f e c t i v e Uniform F a i l e d P a r t i c l e F r a c t i o n Throughout L i f e .
- W S T SAHPLIII: ARD
COUNTING F A C I L I T Y
\ FAST RaSPOaB L O O P FOR COOLANI CAS A C T I V I T Y AND c m L COYP(ISIT1ON.
\ IMPURITY I N J E C I ' I O N F A C I L I T Y
X O B E AND KE-EWlQAM UATZR - I N J E C T I O N F A C I L I T Y FOR PLATI: OITT RE-DISTRIBUTION DATA
RGPERENCE RELEASE ELEKEHPS
C E I W E S P I X B I N J E C T I O N FOR
S I N G L E E L E M E M C O R 7 0 i I O N WITS
Fig . 8. S a f e t y Programme of Dragon.
1
Paper 2/118
THE RELATION-,C~LEISSION, PRODUCT RELEASE~LIMITATIONS. TO THE DESIGN AND OPEUT310N,0F- A- LARGE.. H. T . R., STATJON
*- _.-. m ~ < T J i l w r r . r . ~ r -
ABSTRACT
The key f ea tu res concerning f i s s i o n product r e l e a s e
Release of I 3 ' I dur ing normal opera t ion due t o helium leakage.
from a power HTR a re : -
( a )
( b ) Plate-out of 13 '1 and 137Cs on primary c i r c u i t surfaces .
Release of ''SI- during a r eac to r depressurisa- t i o n , possibly following a leakage of steam i n t o t h e c i r c u i t .
( c )
By consider ing the va r ious d i f fus ion and evaporation processes involved i n the t r a n s p o r t of t h e s e p a r t i c u l a r f i s s i o n products from t h e i r po in t s of o r i g i n it i s possible t o relate the f u e l element des ign , and i n p a r t i c u l a r t h e coated p a r t i c l e breakage f r a c t i o n , t o the s e v e r i t y of those f e a t u r e s .
The most important parameters required f o r t h i s calcu- l a t i o n a re : -
d i f f u s i o n c o e f f i c i e n t s f o r I*, C s and S r i n f u e l tube g raph i t e s , as funct ions of temperature, concentrat ion and impurity con ten t ,
adsorp t ion isotherms f o r 12, C s and Sr on f u e l tube g raph i t e s , a s func t ions of t h e same v a r i a b l e s ,
steady state R/B va lues f o r short- l ived gases d i f fus ing from broken particles,
plate-out f a c t o r s descr ib ing the d i s t r i b u t i o n of re leased I and S r between t h e helium coolant and t h e primary c i r c u i t sur faces t o which access m y be required f o r maintenance purposes,
' l i f t - o f f ' f a c t o r s descr ib ing t h e e x t e n t t o which S r and I2 adsorbed on g raph i t e o r s t e e l
311
312
su r faces w i l l be t r a n s f e r r e d t o t h e coolan t during a steam i n g r e s s o r d e p r e s s u r i s a t i o n acc ident .
O f these parameters ( a ) , ( b ) and ( c ) are known w i t h ‘ o r d e r of magnitude’ accuracy, and th.e a v a i l a b l e data toge the r w i t h some r e c e n t Harwell measurements are summar- ised. By means of t h e f i n i t e d i f f e r e n c e code, FIPDIG3, t h e best estimates o f these data are used t o compute the releases of 1 3 ’ 1 , 137Cs and i n t o t h e c o o l a n t of an HTR over i t s whole l i f e , and t o assess the consequences of overheated channel acc iden t s .
Parameters ( d ) and ( e ) are u n c e r t a i n t o t h e e x t e n t of a t l ea s t two o r d e r s of magnitude, and f o r t h e purpose o f these c a l c u l a t i o n s it has been necessary t o take somewhat a rb i t ra ry va lues f o r them.
Having a r r i v e d a t va lues f o r plated-out and helium- borne a c t i v i t y corresponding t o a c e r t a i n broken par t ic le f r a c t i o n , deduct ions are made concerning t h e permiss ib le breakage f r a c t i o n i n a 3000 MW(T) s t a t i o n .
I t i s appa ren t f r o m t h i s type of c a l c u l a t i o n t h a t a t t a inmen t of t h e necessary c l e a n l i n e s s of primary c i r c u i t and environment r equ i r e s high s t a n d a r d s of particle i n t e g r i t y . I n view of the c o s t pena l ty a s s o c i a t e d wi th manufacture and q u a l i t y c o n t r o l a t very high s t anda rds it i s considered worthwhile t o improve ou r knowledge of the c r i t i ca l parameters l i s t e d above i n o rde r t o reduce t h e u n c e r t a i n t y i n ou r e s t ima te of permiss ib le breakage frac- ti on.
I n a d d i t i o n t o l abora to ry measurements of parameters ( a ) , ( b ) and ( c ) it i s proposed t h a t a r e a c t o r loop be const .nicted a t Hanvel l f o r t h e purpose of measuring ( d ) and ( e ) d i r e c t l y under real is t ic c o n d i t i o n s , and t o provide d i r ec t checks of FIPDIG3 conclusions.
The proposed loop , known as P lu to B , w i l l comprise a nea r ly isothermal. f u e l s e c t i o n , a c r o s s f low b o i l e r of real is t ic des ign and a helium c i r c u l a t i o n system which produces heat f luxes o f t h e r i g h t o rde r i n both f u e l ele- ment and b o i l e r . By means of t h i s equipment it w i l l be poss ib l e t o o b t a i n p la te -out f a c t o r s , p la te -out d i s t r i b u - t i o n p r o f i l e s and l i f t o f f f a c t o r s which w i l l be very much more convincing than ou r p re sen t estimates o f those qiiant i t i e s.
313
1 IIWRODUCTION
F i s s ion products c o n s t i t u t e a formidab-e problem i n harnessing of
nuc lear f i s s i o n t o power production, and the so lu t ions of t h i s problem represent a very s i g n i f i c a n t p a r t of t h e high c a p i t a l c o s t of nuc lear power s t a t i o n s . products a r e confined wi th in sealed m e t a l l i c cans, and although many of
them are v o l a t i l e substances t h e r e l i a b i l i t y of the cans i s high enough
t o reduce the f i s s i o n product r e l ease t o neg l ig ib l e proportions. The engineering problem reso lves i n t o one of rapid de t ec t ion and replace- ment of leaking cans, combined wi th very high s tandards of can manufac- t u r e .
I n t h e c u r r e n t gene ra t ion of power r eac to r s t h e f i s s i o n
A new s i t u a t i o n has a r i s e n with t h e HTR. Although t h e primary f i s s i o n product containment i s s t i l l a sealed can, i n t h i s ca se a combination o f PyC and S i c coa t ing s h e l l s , t he f a i l u r e of a can leads
less d i r e c t l y t o contamination of t h e coolan t c i r c u i t . T h i s i s because a barrier of graphi te i s placed between the coated p a r t i c l e and t h e
coolant. Consequently, t h e r e i s a time de lay , varying from one f i s s i o n product t o another , between can f a i l u r e and r e l ease of radio- a c t i v e material.
Another consequence of t h e HTR type of f u e l canning i s t h a t can f a i l u r e i s more predic tab le than before. about 10" coated p a r t i c l e s , so t h a t t h e r e i s a very good chance t h a t
manufacturing de fec t s w i l l r e s u l t i n a reproducible cons tan t f a i l u r e f r ac t ion . Warning of f a i l u r e due t o abnormal r eac to r opera t ion must a l s o occur i n much smaller increments and i n a more progressive manner than i n a conventional reac tor .
A power r eac to r w i l l contain
It i s i n t e r e s t i n g t o observe t h a t , rather than reduce t h e emphasis on f i s s i o n product behaviour, t h e b e n e f i t s r e fe r r ed t o have caused a large expansion i n t h e quan t i ty of information demanded by des igners and sa fe ty assessors . There a r e two main reasons f o r t h i s . F i r s t l y
t h e non-metallic f u e l can i s regarded as reaching a l a v e r s tandard of l eak t i g h t n e s s than me ta l l i c cans , although t h i s i s not necessa r i ly a
v a l i d gene ra l i s a t ion , and secondly designers a r e pred ic tab ly anxious
314
t o take f u l l advantage of t h e new-found second l i n e of defence i n f i s s i o n product r e t e n t i o n , by pushing p a r t i c l e temperatures t o t h e i r
l i m i t and by taking c r e d i t f o r r e t e n t i o n i n t h e g r a p h i t e f u e l tube. The p o s s i b i l i t y of omi t t i ng the S i c c o a t i n g from p a r t i c l e s i s an
example of t h e l a t t e r approach, because the f u e l tube then becomes t h e
primary, and a very e f f i c i e n t , barr ier t o S r release.
Consequently, a d e t a i l e d i n v e s t i g a t i o n o f f i s s i o n product behaviour i s i n progress . I t cove r s t h e va r ious d i f f u s i o n and evapora t ion
processes by which n u c l i d e s could move from t h e fuel k e r n e l s t o the
ou t s ide atmosphere o r t o t h e s team-rais ing machinery, and it seeks t o i n f e r t h e accep tab le s t anda rds of manufacture and ope ra t ion of t h e fue l .
2 . A S W Y OF THE PROBABLE FISSION PRODKT RELEASE RESTRICTIONS
The f irst s t e p i n a t tempt ing a n estimate of t o l e r a b l e coated par t ic le damage i s t o decide which f i s s i o n products and which modes o f
release are l i k e l y t o be l imi t ing .
A s u f f i c i e n t l y a c c u r a t e dec i s ion may be made, i n t h e f i rs t i n s t a n c e , by comparing a n ' i ndex of haza rd ' , g iven by t h e product of t h e ICRP recommended i n g e s t i o n l i m i t , the t .ypica1 r e a c t o r inventory and t h e release p o t e n t i a l f o r every f i s s i o n product i n turn. T h i s has
been done f o r t h e case o f a n HTR, ope ra t ing on a 1500 day f u e l d w e l l
time w i t h a 0.5 c m t h i c k f u e l free zone, u s ing t h e func t ion erfc - as a rough measure of release po ten t i a l . D i s t h e d i f f u s i o n cons t an t of the f i s s i o n product i n nuc lea r g r a p h i t e , x i s t h e f u e l free zone th i ckness and t i s t h e d w e l l time. A c a l c u l a t i o n of t h i s kind leads
t o t h e conclus ion tha t t h e nuc l ides l i s t e d i n Table 1 , i n o r d e r of decreas ing hazard index, c o n s t i t u t e t he major part of t h e f i s s i o n product release problem.
X
f i
Using t h e computer code ICON' ' ) the inven to ry o f these nuc l ides i n a 3000 W(T) r eac to r , a t a n equi l ibr ium s ta te of r e f u e l l i n g and w i t h a n i n i t i a l loadil?g o f 33 tonnes of 5% enriched uranium, has been c a l c u l a t e d f o r i n c l u s i o n i n Table 1.
l 'able 1.
315
S i g n i f i c a n t F i s s ion Products
Nuclide
31 Iodine 3310dine 88Krypton 'OS t r o n t ium 29Tellurium(m) 32Tellurium 34~aesium 3210dine 37~aes ium 341 odine 7K ry p t on
Inventory (Cur ies ) of a 3000 MW HTR a t Refue l l ing Equilibrium
7
8
7
6
6
8
8.3 x 10
1.6 x 10
6.6 x 10
5.5 x 10
6.2 x 10
1.2 x 10 c
4.4 x lo3 8
6
8
7
1.2 x 10
7.4 x 10 2.0 x 10
5 . 5 x 10
The problem of y rad ia t ion from primary c i r c u i t components, a l though not d i r e c t l y r e l a t ed t o t h i s hazard index, i s l a rge ly due t o 134Cs, 137Cs and 1 3 1 1 , and so both a spec t s a r e covered by a considera- t i o n o f t h e nuc l ides i n Table 1.
I t i s convenient t o group toge ther those nuc l ides which show sin-&lar d i f f u s i o n c h a r a c t e r i s t i c s i n HTR f u e l , and t o r ep resen t each group by i t s most hazardous member. w i l l t he re fo re be concerned only w i t h 1 3 ' 1 , 88Kr, 'OS, and 137Cs, and w i t h the gaseous precursors
I n the f o l l w i n g d iscuss ion we
and 137Xe.
I n making es t imates of t h e q u a n t i t i e s of these f i s s i o n products which w i l l d i f f u s e through and evaporate from t h e f u e l tubes i n a l a rge HTR it i s u s e f u l t o have a guide t o the maximum permissible r e l e a s e s of each nucl ide , so t h a t a minimum coated-par t ic le performance may be
spec i f ied . t h a t , t o some ex ten t , d e f i c i e n c i e s i n coated p a r t i c l e s may be o f f - s e t by such expedients as iodine f i l t e r s i n t h e r eac to r vent system o r l o c a l
The provis ion of such a guide i s made d i f f i c u l t by t h e fact
0
316
s h i e l d i n g of maintenance areas, and only a c o s t op t imisa t ion can r e so lve
such f l e x i b i l i t i e s . Never the less a prel iminary c a l c u l a t i o n of maximum
permiss ib le releases, based upon a clear set of reasonable assumptions, serves as a convenient i l l u s t r a t i o n i n t h i s paper.
The fol lowing assumptions are made f o r a twin 1500 W ( T ) s t a t i o n ,
o f 30 y e a r s l i fe : -
The maximum permiss ib le pub l i c i s 0.5 rem/year ICRP . ( 2 )
l e v e l of e x t e r n a l r a d i a t i o n t o t h e
whole body), as recomnended by t h e
The maximum permiss ib le annual dose l i m i t f o r i n h a l a t i o n and i n g e s t i o n by the publ ic i s one t e n t h of t h e ICRP recomenda- t i on . It i s convenient t o express t h a t recommendation i n terms of 'Derived Working L i m i t s ' , which g i v e t h e correspond- ing milk contaminat ion l e v e l s f o r I , S r and Cs s i n c e m i l k
consumption r e p r e s e n t s t he g r e a t e s t i n g e s t i o n r i s k (Table 2a) .
Dose rates from primary c i r c u i t components should no t exceed
200 mR/hour a t p o i n t s which may r equ i r e even very in f r equen t access, one week a f t e r shutdown.
The helium leakage i s on average O.% p e r day.
The s t a t i o n boundary fence i s a t 500 metres.
Leaks are discharged from a stack of 10 metres e f f e c t i v e he igh t , through a f i l t e r g iv ing a f a c t o r of t e n decontamina-
t i o n f o r C s and S r , bu t n o t f o r I
Pla te -out of 12, C s and S r , i s uniform over t h e b o i l e r
s u r f a c e s , the t o t a l b o i l e r volume b e i n g 5 x 10 c m . 2'
8 3
The p la te -out f a c t o r f o r these elements i s 1000 under normal ope ra t ion o r d e p r e s s u r i s a t i o n , and 1 0 0 dur ing a b o i l e r tube f a i l u r e o r channel overheat ing.
The maximum p o s s i b l e prirrary c i r c u i t breach has a diameter of 20 cm.
8
31 7
Table 2. Assumed Tolerab le Release Limits
Nuclide
( a ) Continuous Release
Derived Working L i m i t s fo r Radioactivity i n Milk.
Annual Average Act iv i ty
1311
137cs "S r
I
1311
90s r
3
3
3
0.03 C.sec/m
0.93 C.sec/m
0.00083 C. sec/m
400 @ / l i t r e
800 pC/g C a
30,000 @ / l i t r e
( b ) Accidental Release
Derived Emergency Reference Levels of Cloud Dosage, based on
inha la t ion hazard.
Nuclide I D.E.R.L. ( A i r ) I
318
(10) F a i l u r e of a s i n g l e b o i l e r t ube w i l l no t cause p re s su re re l ief va lves t o l i f t .
( 1 1 ) I n h a l a t i o n and whole body exposure limits f o r acc iden t s i t u a - t i o n s are t h e Emergency Reference Levels recommended by t h e
Medical Research Council ' 2 ) .
countermeasures such as evacuat ion , o r banning of f o o d s t u f f s , a re u n l i k e l y t o be necessary. The s i g n i f i c a n t l i m i t s i n t h i s group are
These are Levels below which
25 rad t o t h e thy ro id
1.5 rad/year t o bone
15 r a d whole body dose
10 rad whole body dose
1311
90s r 88Kr
' 37cs I n g e s t i o n i s n o t counted a l i in i ted r i s k i n a c c i d e n t
s i t u a t i o n s s i n c e doses from t h a t source m y be avoided by temporary banning of foods tu f f s . The Emergency Reference Levels have been expressed as 'Derived Emergency Release
Levels ' i n Table 2b.
On t h e basis of these assumptions, p o t e n t i a l hazards from normal
ope ra t ion , and from c e r t a i n acc iden t c o n d i t i o n s , have been assessed , and a maximum permiss ib le release from the c o r e c a l c u l a t e d i n r e s p e c t of each case. The most l i m i t i n g cases f o r each i s o t o p e are summarised i n Table 3.
S i n g l e channel overhea t ing and b o i l e r tube f r a c t u r e a c c i d e n t s do n o t r e s u l t i n l i m i t s a s severe as those i n Table 3 .
It must be stressed that t h e s e a r e merely i l l u s t r a t i v e c a l c u l a t i o n s , and t h a t l a r g e u n c e r t a i n t i e s r e m i n i n some of t h e assumptions made. I n t h e case of normal 1 3 1 1 release t h e main u n c e r t a i n t y i s probably t h e
p la te -out f a c t o r , and the same a p p l i e s t o 'OS. release during depres- s u r i s a t i o n . t i o n i n the c i r c u i t a r e t h e d i s t r i b u t i o n of p l a t e -ou t , t h e e x t e n t t o which des ign can a l l e v i a t e maintenance d i f f i c u l t i e s , and t h e presence
o f a c t i v a t e d i m p u r i t i e s a longs ide t h e f i s s i o n products.
The u n c e r t a i n t i e s a s s o c i a t e d wi th I 3 l I and 137Cs y radia-
319
Nuclide
1311
88Kr
3 7 ~ s
1 311
' O S ,
88Kr
Table 3. Derived Maximum Permissible Core Releases i n t o t h e C i r c u i t f o r each of t h e 1500 nini\r(T) Reactors
Derived L i m i t Context
R/B = 2 x Leakage i n n o r m 1 opera t ion
R/B = 4 x Leakage i n normal opera t ion
5 Curies/year C i r c u i t contamination
R/B = IO-^ C i r c u i t contamination
36 Curies/year
R/B = 3 x
Depressurisat ion acc ident without l i f t - o f f
Depressurisat ion acc ident without l i f t - o f f
3. PARAMETERS WHICH CONTROL FISSION PRODUCE RELEASE FROM PARTICLES INTO THE REACTOR COOLANT
The sources of f i s s i o n products i n any conf igura t ion of f u e l mat r ix , g raph i t e and coolant w i l l be the e f f e c t i v e proport ion of exposed k e r n e l s and the f r a c t i o n a l uranium contamination of t he o u t e r pyrolytic carbon coatings. I n order to assess the release of a given
f i s s i o n product i n t o the coolan t during a given f u e l element opera t ion , it i s necessary t o evaluate the inf luence of a number of r e l ease b a r r i e r s f o r t he chosen s e t of circumstances.
The barriers which are known t o opera te , and which w i l l be con- sidered, are :-
( a ) d i f f u s i o n from p a r t i c l e s having imperfect coa t ings ,
( b ) d i f fus ion from reco i l s i tes r e s u l t i n g from uranium contamination of t he p a r t i c l e ou te r coa t ings ,
( c ) d i f f u s i o n through t h e f u e l mat r ix ,
320
( d ) d i f f u s i o n through the g r a p h i t e w a l l o f t h e f u e l p in ,
( e ) evaporat ion from the o u t s i d e o f t h e g r a p h i t e w a l l i n t o the
helium coolant .
Some a d d i t i o n a l f i s s i o n product de l ay could occur i n the gap between mat r ix and f u e l tube. I t i s n o t poss ib l e t o take t h i s i n t o account a t p re sen t , s i n c e experiments show t h a t t h e ma jo r i ty of t ransmiss ion of metals occurs a t t h e i n e v i t a b l e , b u t i l l - d e f i n e d , con tac t po in ts .
I n o r d e r t o make use of models t o c a l c u l a t e t h e o v e r a l l e f fec t on products of these barriers, t he fo l lowing parameters are requi red f o r each s i g n i f i c a n t f i s s i o n product :-
Diffus ion c o n s t a n t i n the bare k e r n e l , as a func t ion of burn-up and tempera ture , or empi r i ca l data on f r a c t i o n a l release from bare k e r n e l s as a func t ion of t hose v a r i a b l e s .
D i f fus ion c o n s t a n t from r e c o i l si1;es i n t h e o u t e r pyrocarbon
l a y e r of particles a s a func t ion o f temperature and concen- t r a t i o n , o r empi r i ca l d a t a on f r a c t i o n a l release from i n t a c t
p a r t i c l e s of known contaminat ion .Level.
Di f fus ion c o n s t a n t i n the m t r i x material as a func t ion of
temperature and concen t r a t ion , i n r e spec t of both ' through d i f f u s i o n ' and d i f f u s i o n from r e c o i l s i tes .
Di f fus ion cons t an t i n the f u e l tube graphi te as a func t ion of temperature and concent ra t ion . It i s necessary t o cons ide r t h e o t h e r f i s s i o n producLs, and impuri ty l e v e l s , when de termining conc e n t ra ti on.
Adsorption i so therm describing t h e equ i l ib r ium p n r t i t i o n of
t he f i s s i o n product between g r a p h i t e sur face and t h e ad jacen t helium boundary l a y e r , a s a functj-on of temperature . Like
( d ) t h i s r e q u i r e s a cons ide ra t ion of o t h e r spec ie s present , and ex ten t of o x i d a t i o n of t h e sur face .
Di f fus ion c o n s t a n t i n t h e helium houndary l a y e r a s a func t ion o f temperature . A knowledge of the boundary l a y e r t h i ckness , based on helium Reynolds Number i s a l s o necessary.
321
A knowledge of these parameters , t aken i n conjunct ion w i t h an es t i -
mated temperature-time h i s t o r y and t h e geometr ica l c o n s t a n t s of a f u e l element, a l lows t h e use of computer codes (394) t o c a l c u l a t e t he release
as a func t ion of element l i f e . A p a r t f r o m t h e margin of u n c e r t a i n t y on t h e s e parameters , t h e remaining f a c t o r s which a f fec t t h e accuracy of t h e c a l c u l a t i o n s a re u n c e r t a i n t i e s about t he e x t e n t of par t ic le d e t e r i o r a - t i o n i n service and about the e x t e n t of S r and C s removal from the f u e l tube o u t e r s u r f a c e s due t o co r ros ion by coo lan t impur i t i e s . phenomena must be considered i n a d d i t i o n t o the d i f f u s i o n and evapora- t i o n steps eva lua ted here .
Such
4. PRESENT STATE OF KNOWLEDGE OF KEY PARAMETERS
4.1
measured i n i r r a d i a t i o n experiments , b u t t he a c t u a l number and s e v e r i t y of t h e imperfec t ions has been determined only a p p r o x i m t e l y dur ing
p o s t - i r r a d i a t i o n metallography. For t h i s reason, i n the fo l lowing parametr ic survey of f i s s i o n product release from f u e l e lements , t he
coa ted particles are cha rac t e r i zed by a t t r i b u t i n g t o them a c e r t a i n
R/B va lue f o r each nucl ide , assuming t h a t it remains cons tan t dur ing i r r a d i a t i o n . Fu r the r i r r a d i a t i o n , us ing uncoated ke rne l s , would be
requi red t o re la te these va lues t o a c t u a l numbers of completely broken
coa t ings ;
- Release from Particles having Imperfect Coat ings has been
however, due t o the w i d e spectrum of s e v e r i t y of imperfec- t i o n s , it i s t o specify batches of f u e l according
t o t h e i r R/B f o r 133Xe, 85Kr and "Sr, a f t e r a few days a t tempeGature. f a i l u r e are avoided, and t h e a v a i l a b l e d a t a a r e s u f f i c i e n t t o a l low t h e d e r i v a t i o n of f r a c t i o n a l release f o r o t h e r s i g n i f i c a n t n u c l i d e s
fram r e s u l t s on these t h r e e r e p r e s e n t a t i v e spec ies .
I n thak way, t h e detailed mechanics of coa t ing
The experimental data on medium and shor t - l i ved K r and X e i s o t o p e s shows t h a t R/B v a r i e s as I/&, and t h a t ( R / B ) 1 3 3 X e f o r bare k e r n e l s i s between 1% and 3 6 a t 14OO0C ( P l u t o V and VI)(5). Bildstein") has shown, by X e p re s su re measurements, t h a t 7%-8@ of
s t a b l e rare gases were r e l eased i n t o t h e a c c e s s i b l e voidage of Dragon UO The R/B f o r a K r o r X e i s o t o p e l e a v i n g coa ted p a r t i c l e s w i l l depend upon t h e e f f e c t i v e broken p a r t i c l e
More r e c e n t l y
coated p a r t i c l e s a t around I50O0C. 2 @
322
f r a c t i o n , $I, the decay cons t an t , t h e d i f f u s i o n cons t an t and t h e e f f e c t i v e g r a i n r ad ius ' a ' , i.e.
whe:re A = d$ 3 - (Coth A - A) R B - -
Z u m d 7 ) has shown t h a t Dxe i n UC2 crystals i s g iven by the
equat ion :
68000 2.3 RT 1ocl0D = - 5.34 - --
-16 2 which g i v e s D ( 1 25OoC) = 8 X 10 c m /sec:. X e
2 I f w e s e t (D/a ) a t 1250°C equal t o i n o rde r t o correspond X e t o releases a t l eas t as large as t h o s e seen i n P lu to V and V I , a va lue of c r y s t a l l i t e r ad ius ' a ' equal t o 2.8 I-1 i s der ived.
An empi r i ca l va lue of D/a2 should be obtained f o r a p a r t i c u l a r type of kernel, a t a p a r t i c u l a r burn-up, by observa t ion of R/B f o r a t l e a s t one rare gas i s o t o p e , bu t it i s perhaps u s e f u l t o g i v e , as i n Table 4, t h e equ i l ib r ium (R/B) ,2500c va lues which correspond t o a 2.8 p e f f e c t i v e r ad ius c r y s t a l l i t e w i t h $ = 1. I n e s t i m a t i n g R/B f o r krypton i s o t o p e s it i s assumed t h a t DKr M 4 x DXe, as i s ind ica t ed by va r ious coa ted par t ic le i r r a d i a t i o n r e s u l t s a t O.R.N. L. and Dragon. The measurement of R/B f o r a long-lived nuc:Lide, such as "Kr o r 137Cs, i s r equ i r ed f o r t he e s t i m a t i o n of $I.
The va lue of e s t a b l i s h i n g a n empirical D/a2 f o r a p a r t i c u l a r batch
of fuel a t a p a r t i c u l a r burn-up l i e s i n the f a c t t ha t t he ' a ' parameter, r ep resen t ing the e f f e c t i v e c rys t a l l i t e r ad ius , i s l i k e l y t o be s e n s i t i v e t o manufacturing rou te and burn-up. The a c t i v a t i o n energy i s less l i k e l y t o be affected.
Experimental r e s u l t s on release of i od ine and metallic f i s s i o n products from bare kernels are aga in very sparse . I n P l u t o Loops V and V I , where e s s e n t i a l l y bare k e r n e l s were i r r a d i a t e d , t h e 1 3 1 1 and 13'Cs
r e s u l t s were low due t o hold up of these i s o t o p e s i n t h e mat r ix g raph i t e .
323
0 Never the less f r a c t i o n a l releases of a f e w p e r c e n t were recorded. The fact t h a t UC ke rne l s were used i s no d isadvantage , s i n c e t h e ke rne l s of f a u l t y p a r t i c l e s w i l l be reduced t o UC, i n t h e reac tor .
2 On t h e o r e t i c a l
L.
grounds, we would expect 1 3 1 1 t o show a d i f f u s i o n behaviour i n UC, - L -15 2 ('1 o f 5 x I O c m /sec a t Ba rather similar t o 133Xe, and t h e measured D
1250°C sugges ts 10% release of a l l s i g n i f i c a n t C s , S r and B a i s o t o p e s from 2.8 p r a d i u s UC2 c r y s t a l l i t e s . t i o n of C s can be assumed f o r p a r t i c l e s w i t h imperfec t ions i n a l l coa t ing
l a y e r s , o r of S r and Ba f o r p a r t i c l e s w i t h imperfec t ions i n t h e Sic
l aye r .
I t t h e r e f o r e appears t h a t no re ten-
With these assumptions about t h e behaviour of imperfec t p a r t i c l e s , t he releases from a c t u a l assemblies of p a r t i c l e s may be predic ted from measurements of 133Xe, 85Kr and 89Sr r e l e a s e , as i n d i c a t o r s of t h e two d i f f e r e n t types of imperfect ion. Thus rare gas r e l e a s e s may be de r ived from (R/B)133Xe us ing Table 4 as a guide , 1 3 ' 1 and 137Cs releases may
85 be equated t o (R/B)133Xe and (R/B) K r r e s p e c t i v e l y , and lw23a and 90Sr 89 releases may be equated t o (R/B) S r .
4.2 Release from Uranium Contamination i n Par t ic le Coat ings
On t h e basis of a 2.8 p e f f e c t i v e c r y s t a l l i t e r ad ius i n k e r n e l s (R/B133Xe 0.25 a t 125OoC), the f r a c t i o n a l release o f 1 3 1 1 and rare gases
due t o Uranium contaminat ion of pyrocarbon, i s less than t h a t due t o a n equal f r a c t i o n of exposed kerne ls . For t h i s reason release from uranium contaminant i s unimportant un le s s it exceeds t h e q u a n t i t y i n exposed
fue l .
Information on release from r e c o i l s i t es i n pyrocarbon comes from two sources ; f r a c t i o n a l releases measured a f t e r loose p a r t i c l e irradia-
t i o n s i n which no imperfec t p a r t i c l e s were p resen t , and l a b o r a t o r y measurements o f d i f f u s i o n cons tan ts .
Most ba t ches of particles used i n DRAGON i r r a d i a t i o n s s i n c e around
1967 have been sampled and a counted. A c o r r e l a t i o n between a count and a c t u a l amount of uranium p resen t i n t h e o u t e r p y r o l y t i c carbon l a y e r has been demonstrated.
324
Table 4. ( R I B ) Rare Gas from Bare Kernels of 2.8 p Effec t ive Crys t a l l i t e Radius a t 1250'C
'S,r 8 7 K r
8%r
89K r
Species
1
4.8 x
7.2 x lod2
9.9 x lod3
4.1 loe3
R/B
' l ~ r
1
2.5 x 10-1
6.'5 x
5.4 x
1.3 x
1.0 x
4 4.7 x 10
-3 2.1 x io
Species 1 R/B
I n Table 5 t he r e l e a s e s of some rare gases and metals observed i n three experiments w i t h loose p a r t i c l e s a t about 1250 C maximum a r e shown. I n t h e absence o f any b u r s t s of gas, o r metallographic evidence of coat- i n g damage, we conclude t h a t t hese a r e r e l eases from r e c o i l s i t e s i n the
ou te r pyrocarbon. The evidence t o da te thus sugges ts t h a t r e l e a s e of t h e metals i s complete, bu t t h a t the rare gases , p a r t i c u l a r l y the short- l i ved i so topes , a r e g r e a t l y a t tenuated. T h i s r e s u l t i s i n agreement w i t h w h a t i s known of d i f f u s i o n cons t an t s i n py ro ly t i c carbon.
0
For matrix f u e l t h e r e c o i l s i t es a r e l i k e l y t o be somewhat d i f f e r - e n t from those i n loose p a r t i c l e experiments, but no da ta a r e a v a i l a b l e on present matrix mater ia l s .
4.3 Diffusion through the Matrix Graphite
The physical p rope r t i e s of t h e matr ix a r e a s y e t i n s u f f i c i e n t l y f i n a l i s e d t o warrant any very p rec i se c a l c u l a t i o n s on i t s permeabili ty t o gases and metals. I n view of t he f a c t t h a t t h e delaying e f f e c t of t h e matr ix i s less important than t h a t of t h e f u e l tube , because it i s a d i s t r i b u t e d source, it w i l l be s u f f i c i e n t l y accura te t o assume t h a t t h e
325
Table 5. Releases At t r ibu ted to Coating Contamination a t 125OOC
Dragon Experi-
ment
LEHPD 2
Studsvik 16R
HTE (Rod 3)
F rac t iona l 1 Frac t iona l Release ( 2 5%)
Contam- u- 1 8 9 ~ r
matrix behaves exac t ly l i k e the f u e l tube graphi te . t h i s bas i s how l i t t l e effect upon release of metals i s expected from a t y p i c a l matrix a t 1200 C.
Table 6 shows on
0
4.4 Diffusion Constants f o r F i s s ion Products i n Fuel Tube Graphi te
4.4.1 Strontium There i s a s t rong concentrat ion and temperature dependence of D , and the a v a i l a b l e da ta i s i n s u f f i c i e n t t o a l l o w a
s u i t a b l e funct ion t o be f i t t e d accu ra t e ly over wide ranges of t hese var iab les . measurements i n t o two groups, f o l l a v i n g the example of Besenbruch(8), and t o cons t ruc t Arrhenius type equat ions represent ing the regions above and below 1 mg/g.
A t t h e present time we have chosen t o d iv ide the
Above 1 mg/g the work of Faircloth(’) , Bromley ( 10) , Z u m w a l t ( 1 1 ) and Riedinger ( I 2 ) g ives , very approx imte ly , a l i n e a:; follows :-
2 3 4a99 l o ( D i n c m /set) ( 2 ) T 1 0 g l o D = - 1.90 -
326
a t 1 2 0 0 ~ ~ 2 -1 Dma t r i x
(approx. cm sec )
Table 6. F r a c t i o n a l Releases from a Graphi te Mat r ix
D/a ( a = 0.5 c m ) Nuclide
40Ba
8 9 ~ r
’OS r
37cs
- 7.
o - ~
2. IO-’
-9 0
3.
3.
3.
8.
7.
7.
F ( e q u i l . )
0.5
0.9
1
1
T ime t o reach F/2 (days)
13
30
30
1
The data were obta ined on a v a r i e t y of g r a p h i t e s , such a s PGA, EY9
and HX30, and i n gene ra l range over a ten-fold v a r i a t i o n i n D a t a g i v e n temperature. Below 1 mg/g w e have d i f f u s i o n c o n s t a n t s
der ived f r o m p r o f i l e s i n f u e l t ubes ( 3-1 7 ) , some out -of -p i le r e s u l t s from GGA ( 1 1 ’ 1 2 y 1 8 ) , and some recen t work by Sanda l l s ( 1 9 ) . I n view of t h e u n c e r t a i n t i e s of temperature and f u e l f a i l u r e ra te i n t h e p r o f i l e measurements, and of concen t r a t ion l e v e l s i n t h e
GGA d a t a , we have used Sandal l s ’ data , which i s w e l l represented by t h e equation:-
1 1200 1 0 g l O D = 1.164 - -- ‘r ( 3 )
T h i s work was done on AGL9 Gilsocarbon g r a p h i t e and was reproducib le wi th in a f a c t o r of two i n D. The f ac t that, c o e f f i c i e n t s de r ived from t h e p r o f i l e measurements are i n gene ra l a f a c t o r of t e n lower than Sanda l l s ’ r e s u l t s sugges ts t h a t t h e concen t r a t ion dependence of D r e q u i r e s f u r t h e r examination, e s p e c i a l l y wi th a view t o confirming behaviour a t t h e f u l l burn-up concen t r a t ion (R/B = 10 )
of around 1 pg/g. The g r a p h i t e c h a r a c t e r i s t i c s , such as su r face
-3
327
) + 1 1200 10gloD = (1.164 - - T
a rea and impurity conten t , may a l s o be s i g n i f i c a n t , and i n
p a r t i c u l a r it should be noted t h a t t h e AGL 9 graphi te conta ins
30 ppm of calcium.
3 4.4 x I O - ~ ( C - I O ( 4) 6210 e (T - 3.064). 3
4.4 I O - ~ ( C - I O ) l + e
For t h e purpose of running FIPDIG 3 a t t h i s time, t h e follow- i n g func t iona l representa t ion of D was used, taking i n t o account
t he t o t a l concentrat ion of a l l strontium and barium iso topes : -
r 1
L d
where C = concentrat ion i n pg/g
D i n c m /sec
T i n OK
2
This equat ion connects t he two Arrhenius funct ions by a f a i r l y
s teep s t e p a t 1 mg/g loading. I n Fig. 1 a r e shown a l l of t h e
ava i l ab le measurements f o r D toge ther w i t h the two Arrhenius
l i n e s ( A and B ) comprising eq. 4. Sr’
4.4.2 Caesium A s with S r , t h e r e i s a s t rong temperature and concent ra t ion dependence. There a r e data a t t r a c e r concentra- t i o n ( 1 pg/g) from t h e work of Bryant p ro f i l e s ‘ 21 ’ 7, which g ive approx imte ly a l i n e
( 2 0 ) , and f r o m f u e l tube
10390 10gloD = 0.19 - - T
I n t h e region 100-1000 pg/g we have data ( 1 9 ) on AGL 9 g raph i t e , g iv ing a l i ne : -
3940 log D = - 1.158 - - T 10
328
to T ) + 10390 log D = (0.19 - -
(10) which l i e s c l o s e t o p o i n t s ob ta ined on o t h e r g r a p h i t e s by Bromley . Riedinger ( 2 2 ) g i v e s two r e s u l t s l y i n g midway between these groups.
G 450 0 .147(C - 30) (7 - 1.348) . e
1 -:- e ( 7 ) 0.147(C - 30)
Again there i s no informat ion on how these reg ions connect , bu t t h e C s adsorp t ion i so therms do show some evidence of a change i n
s i te energy a t around 30 rJ,g/g(20). We have t h e r e f o r e i n s e r t e d a s t e p f u n c t i o n a t t h a t p o i n t , t o g ive f i n a l l y : -
L J
where C = concen t r a t ion i n Wg/g
D i n c m /sec
T i n OK
2
Fig. 2 shows a l l t h e a v a i l a b l e po in t s l’or D t o g e t h e r w i th t h e two
l i n e s ( A and B ) corresponding t o equ. 5 and 6 . cs
4.4.3 Iodine There appear t o be no d i f f u s i o n d a t a f o r iod ine a t r e l e v a n t temperatures , bu t work a t lower temperatures i n d i c a t e s
t h a t a t h igh concen t r a t ions it diffuse! ; l i k e a gas (23) . f o r e , treated it l i k e N 2 gas‘24) and in t roduced a p res su re and tempera ture dependence assuming t h a t gas-gas c o l l i s i o n s i n pores c o n t r o l t he d i f f u s i o n and t h a t c o l l i s i o n c ros s - sec t ions are energy independent.
We, the re -
-3 2 Longstaff g i v e s a n apparent D of 3 x 10 c m /sec a t 1 atm and room temperature , f o r a non-impregnated g r a p h i t e w i t h no t o t a l
p re s su re g rad ien t . A s s u m i n g a connected po ros i ty of 8% w2 have
i.e. D = 1.32 x IO-’ x T3/2cm2/sec
329
A t t h i s l e v e l of D t h e r e i s no s i g n i f i c a n t delay of 1 3 ' 1 i n 5 nun of
f u e l tube above 8Oo0C.
4.4.4 Rare Gases There are no data a t real is t ic temperatures and pressures but i n t h i s case we can be more conf ident of t h e ex t r a - po la t ion formulae. ( 24) The expression used was exac t ly as f o r I2 .
I n svmmary it may be said t h a t t he c u r r e n t l y ava i l ab le da ta
on d i f fus ion of metals and iod ine i n fue l tube g raph i t e i s of o rde r of magnitude accuracy only. with a view t o improving t h i s s i t u a t i o n , a r e
Fea tures which a r e under examination,
( a )
( b ) The occurrence of mul t ip le d i f f u s i o n processes.
( c )
The e f f e c t of concentrat ions on D .
The e f f e c t of helium impur i t i e s on D.
( d ) The d i f f e rences between the va r ious poss ib le f u e l tube graphi tes .
4.5 Adsorption Isotherms f o r F i s s ion Products on Fuel Tube G r a p h i t e
4.5.1
of tungsten e f fus ion c e l l s ' 1 8 ) , g ive the following Fruendlich isotherm f o r TS - 688 graphi te : -
The GGA d a t a on S r adsorp t ion recent ly improved by t h e use
w i t h P = ( a t m )
c = p mole/g
a = 10.27
b = - 38.1
c = - 0.745
d = 4.13
The equat ion con ta ins a co r rec t ion t o allow f o r the change i n sur face a rea caused by gr inding t h e g raph i t e t o 37-74 p p a r t i c l e
s i z e ; it i s considered t o represent t he experimental points t o
330
with in a f a c t o r of f ive. Recent r e s u l t s from Hanvell confirm these data ( 2 5 ) with in a f a c t o r of 3 .
I n view of t h e fact t h a t t hese measurements do not extend t o the required l e v e l of 1 pg/g t h e r e i s :some considerable r isk i n ex t r apo la t ing as a Freundlich isotherm; the re fo re , a t a concentra- t i o n of 30 pg/g t h e equat ion has been changed t o a Langmuir i so- therm f o r ex t r apo la t ion purposes. T h i s m y be a r e a l i s t i c approxi- mation because some r e a c t o r g r a p h i t e s conta in around 30 pg/g of calcium, which would be expected t o have the e f f e c t of producing an apparent Langmuir isotherm. The f i n a l equat ion used is:-
) 47000
T 15.17 - - ( 10)
1 o3 + ( c + d T) I n + exp(1n C +
c = concent ra t ion (p mole/g)
The hea t of adsorp t ion i n t h e Langmuir region has been set a t 94 k.cal/mole, i n l i n e w i t h the low concent ra t ion va lue measured a t
GGA . 4.5.2 graphi te . The following approximate equat ion w a s f i t t e d t o h i s
For C s Adsorption w e use the data of Mils tead (26) on TS - 668
r e s u l t s :-
63500 + 4.48 I n C ‘04’0 + I n C] + exp[ 11.6 - --y ( 1 1 ) 1 where P = (atm)
c = concent ra t ion (pg/g)
I n t h i s case t h e experimental po in t s do suggest a change of slope a t 30 pg/g.
involved lump specimens of g r a p h i t e , SI) a surface a rea co r rec t ion i s unnecessary.
(27 ) g ives d a t a f o r adso rp t ion of I 4.5.3 Salzano Carbon type TSX g raph i t e , i n the temperature range 100-800 C.
The i s o p i e s t i c technique used f o r t h i s work
on National 0
2
331
The concent ra t ions used a r e q u i t e comparable t o those expected i n f u e l tubes. temperature, and i n p a r t i c u l a r t he e f f e c t of H 0 corrosion was t o loiver pressures by up t o a f a c t o r of ten. therm t o depend a l s o upon impuri ty l e v e l s , but i n t h e absence of o t h e r information the formula
Sa lzano ' s isotherms a r e very dependent upon outgassing
2 W? might expect t h e iso-
c2 f i 7.8 x x exp (- P = 20000)
T
where P = ( a t m )
c = concentrat ion t pg/g)
0 T = K
0 was used. It app l i e s t o g raph i t e outgassed a t 900 C.
I n sumary it i s c l e a r t h a t the metal adsorp t ion isotherms a r e inw-lequately defined i n t h e s i g n i f i c a n t concent ra t ion region around
1 pg/g. gated.
The poss ib le e f f e c t of impur i t ies has y e t t o be i w e s t i -
5. METHOD OF CALCULATION OF CORE RELEASE
The one dimensional t i m e dependent f i s s i o n product d i f fus ion code F I P D I G has been f u l l y described by P r e i n r e i ~ h ' ~ ) . used t o c a l c u l a t e f i s s i o n product concent ra t ion p r o f i l e s and r e l ease rates f o r any arrangement of f u e l zones and fue l - f ree zones i n s l ab , c y l i n d r i c a l o r sphe r i ca l geometry. The source term and zone temperatures may be var ied w i t h time. I n i t s o r i g i n a l vers ion the code used d i f fus ion and evaporation cons tan ts which were independent of time, and the re fo re of concent ra t ion , although provis ion was made f o r a sc r ib ing d i f f e r e n t va lues t o each of t he temperature zones. The evaporation cons t an t s used i n t h i s e a r l y work were not related t o the respec t ive adsorpt ion isotherms, bu t
were b e s t es t imates from the inadequate experimental data ava i lab le .
The programme can be
A modified form of F I P D I G , known as F I P D I G 3, i s a t present i n use a t Hanvell ( 2 5 ) . T h i s code incorpora tes t h e temperature and concent ra t ion
332
dependent func t ions f o r t h e d i f fus ion and evaporat ion cons tan ts wi th in the o r i g i n a l FIPDIG framework, and the re fo re takes i n t o account auto- mat ica l ly the changes i n D and H. The evaporat ion constant H i s derived from t h e equi l ibr ium partial pressure of t h e f i s s i o n product a t t h e
evaporating su r face by means of an approximation of t he type:-
0.8 O o 3 f ( c ) cm -1 11 = 0.023 (Re) (Sc) - d C
where: D = d i f f u s i o n c o e f f i c i e n t of evaporating spec ies i n boundary l a y e r
d = hydraul ic diameter of coolant channel ( taken a s 0.5 c m )
R e = Reynolds Number of coo lan t ( taken as 40,000)
Sc = Schmidt Number of coo lan t
c = concent ra t ion of evaporat ing spec ies i n su r face of f u e l tube
f ( c ) = gas phase concentrat ion of t ha t species i n equi l ibr ium w i t h
t he surface.
The value of D i s obtained f o r t h i s purpose from a simple k i n e t i c theory c o r r e l a t i o n :
RT(M, + ni2) ?5
1 :I D = 8 0 2 n ( 2 T c M M-)
where C, = mean molecular diameter
n = number o f gas molecules per cc
M M = molecular weights o f helium and t h e f i s s i o n product 1 ’ 2 respect ively.
I n FIPDIG 3 the values of D and H appropr i a t e t o a p a r t i c u l a r time-step are obtained by i n s e r t i n g a concent.ration term, r e l a t i n g t o the sum of a l l s t a b l e i so topes of the element, i n t o equations such as 3 , 5 , 8 and 9. The time-step i s then computed a second time, using
333
0 these values i n conjunct ion w i t h t he y i e l d and h a l f - l i f e data of t h e p a r t i c u l a r i so tope under examination. the
y i z l d s of s t a b l e barium have a l s o been added i n t o the f irst s t ep , s ince it m y be expected t h a t S r and Ba d i f f u s e a t s i m i l a r r a t e s .
I n the case of 89Sr and
By means of FIPDIG 3 a time dependent f i s s i o n product r e l ease may
be computed f o r regions of a power r e a c t o r core , t h e reg ions being chosen so tha t t h e r e i s l i t t l e v a r i a t i o n of temperature o r power h i s t o r y wi th in each one. r e l ease from the core f o r a p a r t i c u l a r management scheme.
A summation o f such r e s u l t s g ives t h e o v e r a l l
Rather than present a c a l c u l a t i o n f o r a single special case , t h e
following sec t ions a r e an a t tempt t o use FIPDIG 3 t o i l l u s t r a t e t h e magnitude of core r e l ease of t he key f i s s i o n products r e s u l t i n g from a s e l e c t i o n of operat ing temperatures. Temperature i s the most important s ing le v a r i a b l e a f t e r broken p a r t i c l e f r a c t i o n .
6. PARAMETRIC SURVEY
An e x t e r n a l l y cooled f u e l pin, w i t h t h e following dimensions w i l l
be evaluated :-
Fuel Matr ix I.D. 26 mm
Fuel Matrix O.D. 42 mm
G r a p h i t e Sleeve I .D. 42 mm
Graphi te Sleeve O.D. ( a ) 50 mm
( b ) 52 mm
Power/unit l ength ( cons t an t ) 0.5 kw/cm
The v a r i a b l e s chosen were :
Equivalent broken p a r t i c l e f r a c t i o n , denoted by #: and
Graphi te s leeve th ickness : 4 and 5 nnn
Species : C s 137, S r 90, I 131
and r a r e gases
334
The tempera tures were chosen a s r e p r e s e n t a t i v e o f t h e range o f
i n t e r e s t , w i t h the g r a p h i t e sleeve th i ckness d iv ided i n t c two p a r t s t o s imula te t h e temperature g r a d i e n t . Power, temperature and $ w e r e
assumed independent of t i m e .
o u t e r s leeve T TFue 1 s l eeve Case
C 0
A 1400 1 1 0 0 1000
B 1200 9 25 8 50
C 1000 840 800
T h i s survey r e p r e s e n t s 12 c a l c u l a t i o n s f o r each nucl ide. I n addi- t i o n , s i n g l e runs were performed t o check t h e e f f e c t of t he d i f f e r e n t h a l f - l i f e i n t h e case of Sr. 89
I n the cases of t h e metallic f i s s i o n products t h e f i s s i o n product source term i s equal t o t he equ iva len t broken p a r t i c l e f r a c t i o n , bu t f o r
1 3 1 1 and t h e shor t - l ived rare gases there i s a s i g n i f i c a n t de l ay and decay i n t h e k e r n e l s of broken p a r t i c l e s . effect i n the parametr ic survey we de f ine t h e * e q u i v a l e n t broken p a r t i c l e
f r a c t i o n ' , $, as being equa l t o t h e s teady s ta te R/B of 13'Cs and 85Kr
from the particles, and fur thermore w e assume t h a t t h e e q u i v a l e n t g r a i n r ad ius of t h e ke rne l , ' a ' , i s such as t o g i v e R/B = 0.25 f o r 13%e release from a broken par t ic le a t 1250 C.
broken p a r t i c l e f r a c t i o n of 10
137Cs, R/B = 2.5 x f o r 133Xe and 1 3 1 1 , and smaller R/B v a l u e s f o r the shor t - l ived gases. A f u r t h e r parameter, the equ iva len t Sic damage
f r a c t i o n $', should a l s o be s t a t ed , t o cover t h e i n s t a n c e when S i c damage exceeds s i g n i f i c a n t l y t h e complete c o a t i n g danage. $' i s def ined a s t h e s t eady s t a t e R/B o f 89Sr o r 'OS, from a n assembly of p a r t i c l e s and should be used i n p lace of q5 when p r e d i c t i n g releases of metals o t h e r t han C s .
I11 orde r t o inc lude t h a t
-
0 Thus a t 125OoC, a n equ iva len t -4 would resul t ; i n R/B = lo4 f o r the
I n t h e present e x e r c i s e it i s assumed f o r convenience t h a t $ = $ ' , implying t h a t there a re no particles w i t h d e f e c t i v e S i c and i n t a c t
pyc.
335
6.1 Discussion of Resul t s on C s and S r
The r e s u l t s of t h e survey a r e .shown i n Figs. 3-6.
The dominant e f f e c t i s temperature, due t o the l a r g e en tha lpy of
evaporation a t t h e cooled su r face and t o the l a r g e a c t i v a t i o n enthalpy of the d i f f u s i o n processes. 150 i n f u e l s leeve temperature i s worth about two o rde r s of magnitulde i n i n t e g r a l f r a c t i o n a l r e l ease a t t h e
2000 day poin t , and considerably more a t s h o r t e r times.
0
The i n t e g r a l f r a c t i o n a l re lease of 137Cs o r 'OS, i s seen t o r i s e sharp ly w i t h time and t o l e v e l o f f eventua l ly a t t he va lue of $. t he h ighes t temperature considered here (curve A ) , t h e f r a c t i o n a l r e l ease comes c lose t o $ a t 200d days, whereas curves B and C a r e f a r below. a t successive t imes, f o r t h e t h r e e temperature condi t ions. On the b a s i s of t h e data used it appears t h a t a t long i r r a d i a t i o n t imes the
l a r g e b e n e f i t s ob ta inable by lowering o u t e r f u e l tube temperatures r e s u l t more from t h e f a l l i n t h e H value than from the l a v e r D. curves are s imi la r .
A t
F igs . 7-9 show a sequence of p r o f i l e s of 137Cs concent ra t ion
The survey shows the f r a c t i o n a l r e l ease t o be d i r e c t l y propor t iona l t o t h e @ value. l e s s than 1 pg/g, making t h e d i f f u s i o n c o e f f i c i e n t s independent of concent ra t ion and g iv ing a Langrnuir adsurpt ion isotherm f o r t h e evapora- t i o n step. The use of much l a r g e r @ values might a l t e r t h i s p i c t u r e , a s the Freundlich adsorp t ion regime i s entered and the D beings t o r i s e , bu t on t h e basis of t h e present assumptions t h i s would require practic-
a l l y lOQ% broken p a r t i c l e s . proceeds, t o s imulate p a r t i c l e damage, may t he re fo re be estimated from Figs. 3-6 by d i r e c t surmnat.ion o f t h e d i f f e r i n g p a r t i c l e h i s t o r i e s .
T h i s i s because t h e metal concent ra t ions involved a r e
The e f f e c t of changing $ as i r r a d i a t i o n
The t i m e dependences of t h e 137Cs and 'OS, r e s u l t s a r e very
s imi la r . T h i s may be considered somewhat u n r e a l i s t i c on the grounds t h a t a t mg/g loadings C s i s known t o d i f f u s e f a s t e r t han S r , but as explained e a r l i e r the ava i l ab le da t a a t pg/g loadings a r e i n s u f f i c i e n t
t o support any more re f ined assumptions.
336
S ir 90
2.0 x
4.9 x
1.3
The e f f e c t of a change from I mm t o 5 mi i n f u e l s leeve th i ckness @ i s seen t o be g r e a t e r a t t h e laver tempera tures and e a r l y i n t h e element l i fe . I t i s less important t han f u e l s l eeve temperature i n determining metal release.
"31- must be r e l eased t o a lesser e x t e n t t han gGSr, due t o decay dur ing passage through the f u e l s leeve. A s a n example, one p o i n t on the
parametric survey (Case B ) was repeated us ing S r decay cons tan t .
Table 7 shows the r e su l t .
89
15 38
100
For t h i s reason t h e hazard from 89Sr evapora t ing as metal can be
1 000
2Ooo
neglec ted i n comparison t o t he 90Sr.
1.3
1.3
Table 7 . Rat io of 89Sr t o F r a c t i o n a l Release
I n t e g r a l F r a c t i o n a l Release ($ = 10'3,0.5 c m f u e l t ube )
'OS r /89~ r
1311 6.2 Discussion o f Resu l t s on
The FIPDIG 3 programme, using t h e d a t a on iod ine d iscussed ear l ier , 0 showed t h a t a t g r a p h i t e tempera tures above 800 C there i s n e g l i g i b l e
de lay i n t h e f u e l s leeve. q u i c k l y reaches t h e va lue p e r t a i n i n g t o t h e p a r t i c l e s themselves. Fig. 10 shows t h i s r e s u l t f o r a s e l e c t i o n of' temperature and (R/B)
p a r t i c l e combinations. Under these assumpti.on5 t h e c o n t r o l l i n g f a c t o r i s t h e (R/B 1 particles 9 which depends on t h e q5 and D,/a d iscussed ear l ier .
The f r a c t i o n a l release of 1 3 ' 1 t h e r e f o r e
2 parameters
337
I f we take "equivalent fa i led p a r t i c l e " f r a c t i o n s , $5, equal t o crs -3 -5 10 and 10 , assume an cqulva len t g r a i n rad ius a equal t o 2.8 p and
assume a l s o t h a t Dxe = DI, then the r e s u l t s shown i n Table 8 a r e obtained covering t h e parametric survey condiLions.
The temperature dependence of 1 3 1 1 r e l ease i s thus r a t h e r less than t h a t found f o r t h e metallic f i s s i o n products, and the s teady s t a t e R/E
i s con t ro l l ed by the p a r t i c l e ke rne l temperature r a t h e r than the f u e l
s leeve temperature. The s l eeve th ickness i s on t h i s b a s i s unimportant, and t h e r e i s a l i n e a r dependence upon t h e equivalent broken p a r t i c l e f r a c t i o n .
Table 8. R/B f o r 1311 under t h e Parametric Survey Condit ions
-16 1200 I 3.6 x 10
( R'B p a r t i c l e s (= f r a c t i o n a l release from
e l emen t )
-5 $5 = 10 -3 I $ 5 = 10
-6 8.4 x 1 8.4 x 10
6 . 3 I n e r t G a s Releases
The rare gases , l i k e iod ine , a r e con t ro l l ed l a r g e l y by d i f f u s i o n wi th in the kerne ls of broken p a r t i c l e s , bu t the s h o r t e s t h a l f - l i f e members s u f f e r some decay a l s o during t h e i r passage through t h e f ie1 s leeve wal l . c a ses con t ro l l ed by t h e ha l f - l i fe rather than the d i f f u s i o n c o e f f i c i e n t , t hese times are always s h o r t compared w i t h t h e f u e l element l i f e t ime . Consequently no FIPDIG cases were run on gas r e l ease ; va lues , f o r t he f u e l element condi t ions covered i n our parametric survey,
Since t h e t i m e t o reach a s teady s t a t e R/B i s i n most
steady s t a t e R/B
338
were computed from DKr,Xe i n UC2 kernels"' and i n r e a c t o r grade g raph i t e (equ. 8).
rad ius ' a. breakage f r a c t i o n , r e s u l t s are given only fo r @ = A f u e l sleeve th ickness of 5 mm i s taken s ince t h e r e s u l t i s rather i n s e n s i t i v e t o a change from 5 t o 4 mm.
As f o r 12, we have assumed a 2.8 p ' e f f e c t i v e g r a i n Since t h e release is propor t iona l t o $, the equivalent
The dep le t ion of mre gases d i f f u s i n g through the f u e l s leeve w a l l ( 2 8 ) . i s given by .-
-AT - e FO
Fi - -
where Fo = c u r r e n t leav ing
F . = current en te r ing
h = decay cons tan t 1
0*693 - apparent delay t i m e x T = - - - - h d r n
X = graphite th ickness
D = d i i f f u s i o n c o e f f i c i e n t (equ. 8)
T h i s equat ion assumes a cons t an t cu r ren t of' gas en te r ing t h e i n s i d e face and a z e r o concent ra t ion a t t h e outs ide face.
Table 9 shows how, f o r 5 mm of graphi te a t 1000°C, t he s leeve deple t ion f a c t o r v a r i e s w i t h d i f f u s i o n coef ' f ic ien t and decay constant .
I n Table 1 0 the ( R/B)element va lues a r e given, w i t h t h e
( R'B p a r t i c l e s 9 f o r t he parametric survey c:ases.
T h i s t a b l e serves t o i l l u s t r a t e t h e temperature and h a l f - l i f e dependence of (R/B )element , although i n an absolu te sense it holds only f o r t h e p a r t i c u l a r values of $ and 'a ' assumed.
brs 339
Table 9. Depletion Factor f o r Rare Gas Diffusion through 0.5 c m Graphite
I so tope
Xe 133
135
137
138
139
1 4 0
141
K r 85m
87
88
89
90
91
92
Decay Constant sec- 1
1.52
2.11
2.96
6.79
1.69
4.33
4.08
4.41
1.48
6.95
3.63
2.10
7.08
2.31
- 6
- 5
- 3
- 4
- 2
- 2
- 1
- 5
- 4
- 5
- 3
- 2
- 2
- 1
Depletion Fac tors ( 1000°C)
-3 D = l x 1 0
1
1
0.99
1
0.30
0.094
0.0002
1
1
1
0.84
0.25
0.043
0.002
6 x
1
1
1
1
0.86
0.52
0.03
1
1
1
1
0.78
0.36
0.09
-2 2 - 1 3 x 10 c m sec
1
1
1
1
1
1
0.32
1
1
1
1
1
1
0.5
Table 10. Calculat ion of the R/B Values for Rare Cases Escaping from a Fuel Element under the Conditions chosen f o r the Parametric Survey
(R/B)par t ic les !
-3 Equivalent Breakage Fract ion (@) = 10 F u e l Sleeve Thickness = 0.5 cm Equivalent UC Grain Radius ( a ) = 2.8 p 2
(R/B)par t ic les
M c l i d e
( R’B ) element
1 3 3 ~ e 6 .8 x
1.7
1.5
2.8
3.6 x
1.3 x
10 -3
1.3
2.0
2.7
1.1
5.7 x
element
6.8 x
1.7 lob4
1.5
2.8
1.8 x
3.9 x
10 -3
1.3
2.0
2.7
8.3 x
1.9 x
Fue 1 1 2 0 0 3 Sleeve (inner) 9250C Sleeve (ou te r ) 850 C
(R/B p a r t i c l e s
1.7
4.4
3.7 x
7.1 x
9.2
3.2 x lo-‘
loM3
3.4
4.9
7.1 x
2.7 x
1.4 x
( R/B e 1 ement
1.7 lob4
4.4 loe5
3.7 x
7.1 x
4.8
9.6
-3 10
3.4
4.9
7.1 X
2.0 x
4.7
Fuel Sleeve ( inne r ) Sleeve (ou te r )
2.6
6.8 x
5.7
1.0 x
1.4
4.9 x
10
5.0 x
7.5 x
1.0 x
-3
4.3
2.2
2.6 IO-^
5.7 IO-’
6.8 x
1.0 x
7.2 x
1.5 -3 10
5.0 x
7.5 x
1.0 x lo+
3.2
7 . 3 x
341
137 The two rare gases of g r e a t e s t in terest a r e 'OK, and X e , on account of t h e i r long-lived daughter products. gases i n t o the primary c i r c u i t causes a corresponding f r a c t i o n a l r e l e a s e of ' O S , and 137Cs t o be deposi ted uniformly. e a r l y i n the l i f e of an element, t hese mlttals a r i s e l a r g e l y from the
gas r e l eases , whereas l a t e r on t h e d i r e c t metal evaporat ion w i l l probably predominate.
( R'B ) element from which it i s c l e a r t h a t a t lower temperatures t h e gas con t r ibu t ion predominates f o r a longer period.
The r e l e a s e of t h e s e
It follows t h a t
To i l l u s t r a t e t h i s po in t the appropr ia te va lues from Table 10 have been p l o t t e d i n Figs. 4 and 6 ,
7. SPECIFICATION OF PERMISSIBLE 'EQUIVALENT BROKEN PARTICLE FRACTION'
The r e s u l t s given i n the previous s e c t i o n r e l a t e t o hypothe t ica l core reg ions of cons tan t power and temperature. reasonable assumptions we can est imate from them t h e approximate behaviour of r eac to r cores i n which t h e spec i f i ed temperatures r e l a t e t o t h e h o t t e s t point of t he peak power channel. Let u s cons ider a 1500 W(T) core w i t h a 1500 day mean f u e l dwell time.
By making a number o f
7.1 'OS, and 137Cs
Let A1500 = no. of Curies re leased i n 1500 days per 0.5 kW of
elemeint length ( from the parametric survey)
Now assume:-
( a ) A random reloading pa t t e rn .
( b ) No v a r i a t i o n of f u e l - tube temperature along t h e core r a d i u s o r as a funct ion of t i m e .
( c ) The fract ionial r e l ease from a channel i s always one f i f t h of t h e fractionial release a t t h e h o t t e s t po in t , due t o t h e a x i a l tempera t u r e p r o f i l e .
Then the Curies/year re leased from t h e co re a t r e f u e l l i n g e q u i l i - brium i s given by
3 1 A1500 1500 0.5 5
x - 365 1500 x 10 x --
342
- A 210
Table 1 1 . E s t i m t e d Core Release Rates of Metals
(q5 = 10 and f u e l tube th ickness = 0.5 c m ) -3
Cur.ies/year from a 15OO MW(T) co re Parametric Survey
Case (related t o h o t t e s t f u e l tube pos i t ion)
Table 1 1 shows the r e s u l t of such an e s t ima te , using only t h e da ta
obtained w i t h an ' equiva len t fa i led f r a c t i o n ' of
f u e l tube.
7 .2
and a 0.5 c m thick
'311 and S i g n i f i c a n t Rare Gases
I n der iv ing R/B f o r iod ine and gases from t h e parametric survey
r e s u l t s (Tables 8 and 10) it i s necessary t o apply a co r rec t ion f o r t h e
spectrum of coated p a r t i c l e temperatures i n t h e core. p a r t i c l e temperature g ives approximately a l'actor of two reduct ion i n R/B, on t h e basis of t h e data used i n t h e survey.
f a c t o r of two i n R/B, both a x i a l l y and r a d i a l l y , as compared t o R/B a t t h e h o t t e s t f u e l t ube pos i t i on of t h e peak power channel.
A 100°C drop i n
We have allowed a
Table 12 g ives t h e r e s u l t i n g values of (R/B) core.
If we now convert t he r a r e g a s R/B estimates t o (Curies/year) of t h e daughter products i n a 1500 W ( T ) r e a c t o r , we ob ta in the r e s u l t s given i n Table 13, which must be added t o those o f Table 1 1 t o ob ta in o v e r a l l C s and S r releases.
Q
343
Parametric Survey Case
A
B
C
Table 12.
Curies/year from a 1500 MW(T) core
’OS r 37cs
3.5 6 . 7
0.83 1.7
0.13 0.25
Parametric Survey Case ( re la ted t o hot tes t fuel tube i n peak channel)
A
B
C
Est imted Core R/’B Values fo r Non4.!.itals
~~
5.0
1.2
-6 2.0 x 10
Table 13. Estimates of Metals Released a s Precursors
($ =
344
Case
A
B
C
8. COMPARISON OF ESTIMATED AND PERMITTED RELEASES
-3 By comparing the es t imates of f i s s i o n product r e l e a s e a t $ = 10
w i t h t h e permissible releases derived i n Sec t ion 2, we can i n f e r t h e values of $ which would be permissible , on the basis of the assumptions made, i n a reac tor w i t h peak condi t ions corresponding t o the parametric survey temperatures ,
1000-1 1 0 0
850-925
800-840
Tfue l ( O C )
1 4 0 0
1 200
1000
I n Fig, 1 1 t h i s comparison i s made, and i n Table 14 the der ived va lues of permissible $ a r e given.
Table 14. Permissible Values of 'Equivalent Broken P a r t i c l e Frac t ion ' Corresponding t o the P a r t i c u l a r Assumptions Made
Nuclide
1 311
88K r
37cs
90s r
1311
"K r
L i m i t i n g Context
Noma1 leakage
Normal leakage
C i r c u i t contamination
C i r c u i t contamination
Depre s s u r i s a t ion
Depre s s u r i sa ti on
A
($ permitted
B
5
0.3
10
2 x 10
-3
4
1 o-2
0.25
C
1
1.7 x
1 o - ~ 0.13
1
c
345
Thus a t t h e highest s e t of temperatures (Case A ) t h e plate-out of 137Cs i s t h e l i m i t i n g f ac to r ; s e t (Case C) the p la te -out of '''1 i s l i m i t i n g , requiring $I < 10-3e P a r t i c u l a r l y s t r i k i n g i s the rap id increase of metal evaporation w i t h
increas ing o u t e r fuel tube temperature. between A and B , t h e r e i s a f a c t o r of 50 i n t h e consequent limits on $.
it requi res $I < 2 X A t t h e lowest
0 With only 50 C d i f f e rence
I n order t o r e l a x the l i m i t s , t ak ing Case B as a f a i r l y real is t ic example of peak channel conditions, the first s t e p would be t o increase t h e c i r c u i t r a d i a t i o n l e v e l to le rance above the assumed 200 mr/hr. The
second s t ep , of similar importance, would be t o inc rease the he ight of t he v e n t i l a t i o n stack, o r t o show t h a t I2 plate-out i s g r e a t e r than 10 : 1 , o r t o i n s t a l l a form of iod ine f i l t e r i n t h e stack. By these means it appears t h a t the l i m i t i n g $I value could be r a i s e d t o , say,
3
i f t he economic f a c t o r s demanded it.
It i s i n t e r e s t i n g t o note that t h e t o l e r a b l e f r a c t i o n of fa i led
Sic c o a t s i s higher than t h e t o l e r a b l e f r a c t i o n of complete coating f a i l u r e s . i n t e g r i t y of S i c coa t s , t he permitted va lue of $I' i s as high as i n case B.
Thus, using the S r release as a c r i t e r i o n of t h e necessary
Another f a c t o r which may f u r t h e r re lax the S i c i n t e g r i t y require- ment, as determined by the depressur i sa t ion acc iden t , i s t h e poss ib le raising of t h e 'OS, D.E.R.L. from 0.00083 t o 0.09 Curie.sec per cubic metre. Such a change would, on present assumptions, remove the
necess i ty of Sic coatings, but considerable improvement i n accuracy of key data i s required before t h a t p o s s i b i l i t y could become a real option.
9. DISCUSSION OF FUTURE DATA REQUIREMnVTS
There is a t least a f a c t o r of t e n uncer ta in ty i n computed r e l eases of Sr and C s , due t o u n c e r t a i n t i e s i n t h e d i f f u s i o n and adsorption cons tan ts of t hese metals i n graphi te as func t ions of temperature and concentration. A p a r t i c u l a r l y important task i s t h a t of deciding the shape of t h e adsorption isotherms below 10 pg/g loadings, and of i nves t iga t ing t h e e f f e c t of impur i t i e s such a s calcium on them. Work
346
i s i n progress on t h e s e problems both a t CGA and a t Hanvell.
Another area r equ i r ing f u r t h e r experimentation i s the measurement of the release rates of iod ine and rare gas i so topes f r o m assemblies of uncoated o r damged f u e l p a r t i c l e s . T h i s information i s important i n es tabl ishment t h e v a l i d i t y of t h e suggested procedure of pred ic t ing iod ine and short- l ived gas R/B values from measurements of 133Xe release. Experiments of this kind should a l s o be used t o d iscover the ex ten t t o which t h e e f f e c t i v e c r y s t a l l i t e s i z e i n kernels can be increased i n order t o decrease the s teady state releases of those f i s s i o n products.
Assuming t h a t a l l these measurements are made s a t i s f a c t o r i l y , we may expect computations of the FIPDIG 3 typhe t o p r e d i c t accu ra t e ly t h e co re r e l e a s e s of s i g n i f i c a n t f i s s i o n produc.ts. However, it w i l l be necessary t o check the p red ic t ions a g a i n s t r e a l i s t i c s imulat ions of
typ ica l HTR core condi t ions.
The e x t e n t and t h e d i s t r i b u t i o n of f i s a i o n product plate-out w i th in the co re and primary c i r c u i t i s almost as important as t h e co re release; it i s i n t h i s area t h a t ou r e s t i m a t e s of hazards from normal helium leakage and from y a c t i v i t y of components r equ i r ing maintenance, may be i n e r r o r by up t o two orders of magnitude. Unfortunately t h e p red ic t ion of plate-out f a c t o r s and plate-out p r o f i l e s i s a pecu l i a r ly d i f f i c u l t task, because adsorp t ion isotherms f o r t h e f i s s i o n products on metal sur faces a r e s e n s i t i v e t o t h e sur face condi t ion , and the mass t r a n s f e r c o e f f i c i e n t s of f i s s i o n products i n a c r o s s f l o w steam b o i l e r are dependent upon p a r t i c l e s i z e i n an almolst unpredictable manner.
I n view of t h e c o s t pena l ty assoc ia ted w i t h manufacture and q u a l i t y con t ro l of coated particles t o very high s tandards, and w i t h guarantees of very low f a i l u r e rate i n s e r v i c e , it i s e s s e n t i a l t o have accura te information on the gas-borne and plated-out a c t i v i t y r e s u l t i n g from a known f r a c t i o n of failed p a r t i c l e s .
10. PLUTO LOOP El
I t i s intended t h a t a r eac to r loop, known as P lu to B , be constructed a t Hanvell during t h e next two years f o r t h e purpose of checking FIPDIG 3
p red ic t ions and i l l u s t r a t i n g t h e plate-out t,o be expected i n a large HTR.
347
By means of t h i s equipment it w i l l be poss ib le t o ob ta in plate-out f a c t o r s , d i s t r i b u t i o n p r o f i l e s and acc iden t l i f t - o f f f a c t o r s which w i l l be ve ry much more convincing than ou r present e s t ima tes of those quant i t i e s .
The loop w i l l comprise a t e n inch fbel p in w i t h ve ry small axial temperature g rad ien t , a cross-flow b o i l e r of r e a l i s t i c design and a helium c i m u l a t i o n system which w i l l produce heat f luxes of t h e r i g h t order i n both f u e l element and b o i l e r surfaces.
Fig. 12 shows a schematic c i r c u i t of Pluto B. The f u e l p in i s made
t o operate l i k e t h e h o t t e s t p in i n a r eac to r channel by heat ing the
helium e l e c t r i c a l l y t o simulate t h e o t h e r 9% of the f u e l length. helium flow rate and pressure i s comparable t o t h a t required i n a s imilar ly s ized channel of a power reactor. a f u l l l ength v e r t i c a l s ec t ion of a cross-flow b o i l e r i s simulated by means of a water-cooled u n i t as shown i n Fig. 13. (30)
the re fo re metal sur face temperatures , are c o n t r o l l a b l e over a range of va lues appropr ia te t o the d i f f e r e n t parts of a steam boi le r . bear ing c i r c u l a t o r r e tu rns the helium t o t h e e l e c t r i c a l heater a t 3OOoC.
Table 15 summarises some key parameters i n the loop design.
The
Downstream of t h e f u e l ,
Heat f luxes , and
A gas
The f i rs t task of P l u t o B w i l l be t o present a p i c t u r e of t he gradual build-up of 13’Cs, 134Cs, ’OS, and 1 3 1 1 on t h e b o i l e r sur faces , using a f u e l p in conta in ing a known f r ac t ion of uncoated f u e l particles.
Continuous measurement of helium-borne a c t i v i t y and of chemical impuri- t i es w i l l be mde. The depos i t i on sur faces w i l l be p a r t i c u l a r l y easy t o examine, s ince ind iv idua l t ubes may be removed and replaced from outs ide the pressure vessel .
Other tasks w i l l be s imulat ion of dep res su r i sa t ion acc idents , t o measure any desorbed o r dis lodged material, channel overheating acc idents , t o measure increased evaporation from the f u e l , and steam ingress acci- dents , t o measure changes i n helium-borne a c t i v i t y .
I n s u m r y t h e P lu to B loop w i l l serve t o check t h e assumptions made
i n our hazard assessment and parametric survey of f i s s i o n produce release.
348 Table 15. Design Parameters f o r P lu to Loop B
Parameter
Normal Operation 0 Gas Temperature C O u t l e t
from C i r c u l a t o r
I n l e t t o f u e l Ou t l e t from f u e l
I n l e t t o Heat Exchanger O u t l e t from Heat Exchanger
Gas Pressure p s i ( a b s )
Gas Flow Rate (g/sec) Fuel Element O.D. c m Channel Diameter c m Fuel Rating Kw/cm P in Length c m P in Power Kw
E l e c t r i c a l Heating Power kW
Clean-up By-pass Flow % B o i l e r o r depos i t ion
(i) Reheater: H e temp. C Average hea t f 1
watts/cm Tube diameter c m Latera l / longi tudina l
p i t c h cms Tube material
s e c t i o n 0
!P
( i i ) Superheater : H e tgmp. C
Average hea t f l ux wat t s/cm2
Tube dia . and p i tch ing Tube material
0 (iii) Evaporator: H e temp. C
!F Average hea t f 1 wat t s/cm
Tube diameter and p i tch ing
Tube materia1 ( i v ) Economiser: He temp. C
Average hea t f l u x
Tube d iameter and
Tube material
0
wat t s/cm2
pi tch ing
P lu to Loop B Design Value
390
840 Design m a x i m
900 Design maximum
880 Design maximum 300 Design maximum
1 ooo 150
6.5 (max.) 7.0 (max.) Up to 1.6 25 up t o 40
400
0.7
75C1-690 Design Value
33.0 2.54
A s required A s required
690-550
26.0 A s r ehea te r A s required
550-460
20
A s r ehea te r A s required
460-300
15.13
A s rehea ter A s required
n
349
1 1 . CONCLUSIONS
(a ) The most important f i s s i o n product hazards i n the HTR a r e
1 3 ' I, 1331 Y 137Cs, 134Cs, 90Sr, 88Kr, '%r and 137Xe.
( b ) Release of C s and S r , while b a s i c a l l y c o n t r o l l e d by t h e f r ac - t i o n of broken p a r t i c l e coa t ings , i s s t rongly inf luenced by f u e l tube sur face temperature. The l a t t e r temperature should be given some cons idera t ion toge ther w i t h t h e p a r t i c l e temperature when s e t t i n g design limits.
( c ) Release of I and rare gases i s con t ro l l ed by t h e f r a c t i o n of 2 broken p a r t i c l e coa t ings and by the particle temperature. Gaseous precursors may be t h e major source of metal f i s s i o n product r e l ease during e a r l y f u e l pin l i f e , p a r t i c u l a r l y a t t h e laver temperatures.
( d ) Data on d i f fus ion , adsorp t ion and plate-out of f i s s i o n products
i s a t present i n s u f f i c i e n t l y accura te and complete t o a l low a conf ident assessment of a l lowable p a r t i c l e breakage f r ac t ion . However, on t h e b a s i s of reasonable assumptions, a l lowable f r a c t i o n s have been est imated f o r a v a r i e t y of opera t ing temperatures.
( e ) A new in-pi le loop, t o be b u i l t a t Hanuell, i s described. Its
funct ion w i l l be t o confirm o r c o r r e c t assumptions and c a l c u l a t i o n s of t h e type presented here.
ACKNOW LEDGERENT S
E s t i m a t e s of permitted r e l eases of ind iv idua l f i s s i o n products corresponding t o t h e p a r t i c u l a r assumptions made, a r e based p a r t l y upon work by M r . D. Tat tersal l and co l leagues a t the Cen t ra l E l e c t r i c i t y Generating Board.
The a u t h o r wishes t o acknowledge the a s s i s t a n c e of Mr. R.L.
Fa i r c lo th and Mr, F.C.W. Pummery i n t h e computations, and of Mr. F. P.O. Ashworth i n va luable discussions.
350
1.
2.
3.
4.
5.
6.
7.
8.
9.
10.
11.
12.
13.
14.
15.
16
17.
18.
REFERENCES
R.L. F a i r c l o t h and M.J. Hopper, A Descr ipt ion of t he F i s s ion Product Inventory Code, ICON, AERE-R 6242 (1969).
H.J . Dunster, The Applicat ion and I n t e r p r e t a t i o n of ICRP Recom- mendations i n t h e U.K.A.E.A., AHSB(RP)R78, 3rd Edi t ion (1968).
G. Pre inre ich , The FIPDIG Code, Dragon P ro jec t Reports 565 and 628 ( 1968) . J. Appel and B. ROOS, The FIPER Code, GA 8399
P.E. Brown, H.J . de Nordwall and I. Dosudil, Pos t I r radSat ion Analysis of Charges V and V I of P lu to Loop A , AERE-R 4856 (1965).
H. B i lds t e in , paper presented a t t h e Dragon Fuel Symposium, November 1969 . L.R. Zurmva l t , P.E. G e t h a r d and E.E. A n d e r s o n , F i s s i o n P r o d u c t Release from Single C r y s t a l UC, Par t ic les , GA 4267 (1963).
G.E. Besenbruch (GGA), personal communication.
L.
R.L. F a i r c l o t h , F.C.W. Pumnery and B.A. Ro l l s , Di f fus ion of Ba, S r and Ce i n var ious grades of r eac to r g raph i t e , AERE-R 4994 (1965).
J. Bromley, A.R. Paddon and N. Moul, Di f fus ion of C s , S r and Ba through Porous Graphi tes , AERE-R 3471 ( 196 1 ) . G.E. Besenbruch, J.H. Norman, C.L. Al len and W.H. Weitzel , Trans.Am.Nuc.Soc., 12 ( 1 1 , 81 , 1969. HTGR Chem. Q u a r t e r l y Report (GGA) Novemberdanuary 1962.
H.J. de Nordwall e t a l , AERE-R 4434 ( 1964).
H.J. de Nordwall e t a l , AERE-R 5040 ( 1965) . H.J. de Nordwall e t a l , AERE-R 5404 ( 1967) . H . J . de Nordwall e t a l , AERE-R 5405 ( 1967).
Report on P lu to Loop A Charge 111,
Report on P lu to Loop A Charge VIII,
Report on P lu to Loop A Charge XV,
Report on P l u t o Loop A Charge XVI,
P.E. Brown and R.H. Flowers, unpublished r e s u l t s on Dragon f u e l tube ana lys i s .
HTGR Base Program Quar t e r ly (GGA) December-February 1969, GA-9227. @
351
19.
20 . 21 . 22.
23.
24.
2-50
26
27
28 . 29
30
F.J. S a n d a l l s , AERE Hanvell, t o be pubiished.
Bryant. Nuc.Sci. and Eng., 15, 288, 1963.
H.J . de Nordwall, personal c o m u n i c a t i o n concerning GAIL IV Loop.
A.B. Ried inger , C.E. Milstead and L.R. Z m l t , Proc. 5 t h Carbon Conference, Vol. 11, 1963.
T. Mukaibo, Chem.Soc.Jap.Bul1. , 36, 629, 1963.
B. Longs taf f , T.R. J enk ins , J.B. Morr i s and L.W. Graham, J.App1. Chem., l7, 172, ,1968.
R.L. F a i r c l o t h , AERE, Harwell, work i n progress .
C.E. Mi ls tead , Carbon, 2 , 199, 1969.
F.J. Salzano, Carbon, 2, 73, 1964.
Following a sugges t ion by L. Jones , The Nuclear Power Group Ltd.
W.G. Marley, AERE Hanvell, personal comunica t ion .
R. Forgan, Research Reac tors Div is ion , AERE Harwell, t o be publ ished.
104 TOK
Fig. 1 Stmntium di f fus ion i n reactor graphite.
-
n
. N E W n
104 - TOK
Fig. 2 Caesium di f fus ion i n reactor graphite.
Fig. 3 Integral fractional release of 1 3 7 ~ s when' @ = 10-5.
Fig. 4 Integral fractional release of 13'cs when @ = 10-3,
TIME DAYS
Fig. 5 In tegra l f r ac t i ona l release of ' O S ~ when @ = 10-5,
TIME D A Y S
Fig. 6 In tegra l f rac t iona l re lease of ' O S ~ when @ = 10-3.
2 1 1 FUEL TUBE
DISTANCE FROM CENTRE IN CM.
1'3 7c Fig. 7 Time dependent concentration profiles for
when $ = - Case A.
2 1 1 SPINE 1 I FUEL I FUEL TUBE
DISTANCE FROM CENTRE IN CM.
Fig. 8 Time dependent concentration profiles for 13'cS when q5 = - Case 9.
- I I SPINE I I FUEL I FUEL T U A E
0 . 0 0 0 . 5 0 1 . 0 0 1.50 2 . 0 0 2 . 5 0
DISTANCE FROM CENTRE IN CM.
Fig. 10 R/B for 13'1 leaving the fuel tube. Fig. 9 ~ i m e dependent concentration profiles for 1 3 7 ~ s when @ = 10-3 - Case C.
I I PERMITTED RELEASES
I ESTIMATED RELEASES -I
PARAMETRIC SURVEY CASE
(0 = 10 -3 . F U E L TUBE THICKNESS =0.5cm)
Fig. 1 1 Comparison of permit ted and estimated f i s s i o n product., r e l eases .
HEAT LOSS HEAT LaSS 16 k W 6kW
3OO0C I 780'~ f 70I0r
- CONTROL - HEATER
3OO0C HEAT INPUT APPROX. 400 kW (MAX), t
SPECIMEN POWER 30kW
INPILE SECTION
Fig. 12 Schematic c i r c u i t o f P lu to B loop.
I
T W S F E R GAS MUINC
Fig.
SERVK€S WOWN ARE TYPICAL FOR A L L TUBE MANIFOLDS I
13 The depos i t ion u n i t of Pluto B loop.
I"
OUT
359
DISCUSSION
T. A. J aege r : I would l i k e t o h e a r some more d e t a i l s about t h e f i n i t e
d i f f e r e n c e code FIPDIG3, and I would be i n t e r e s t e d t o hear whether you have
a l s o cons idered u t i l i z i n g for t h e s e c a l c u l a t i o n s t h e f i n i t e element method
which; e .g . has been s u c c e s s f u l l y app l i ed t o hea t d i f f u s i o n problems i n
complicated geometr ies .
R . H. Flowers: The FIPDIG3 code c a l c u l a t e s concen t r a t ion of a f i s s i o n
product a long a f u e l element r a d i u s a t any number of s p e c i f i e d times a f t e r
s t a r t up. I t i s p o s s i b l e t o vary f i s s i o n r a t e , number of broken f u e l
p a r t i c l e s and zone temperatures throughout t h e course of t h e c a l c u l a t i o n ,
and t h e d i f f u s i o n and absorp t ion c o e f f i c i e n t s a r e computed a t each time
s t e p from appropr i a t e f u n c t i o n s of temperature and concen t r a t ion . The
" f i n i t e e lement" method has no t , a s y e t been app l i ed t o t h e problem, but a
two dimensional ve r s ion of FIPDIG3 may e v e n t u a l l y be used t o r ep lace t h e
manual a x i a l i n t e g r a t i o n descr ibed by Mr. Ashworth.
S. I . Kaplan: Do you in t end t o conduct dus t depos i t i on experiments
i n your loop (P lu to B ) ?
R . H. Flowers: Y e s , t h e o b j e c t of us ing an expensive c ross f low
depos i t i on u n i t i s t o ob ta in r e a l i s t i c p la te -out p r o f i l e s f o r f i s s i o n
products c a r r i e d on p a r t i c l e s of g r e a t e r than molecular s i z e . The molec-
u l a r s i z e . The molecular s p e c i e s could be e q u a l l y w e l l s t ud ied i n a
t ubu la r depos i t i on tube. W e i n t end t o run t h e loop under sets of w e l l -
de f ined oxygen p o t e n t i a l s and water i n g r e s s r a t e s i n o rde r t o produce
d u s t of r e p r e s e n t a t i v e s i z e d i s t r i b u t i o n and q u a n t i t y . Of course, i f
l a b o r a t o r y measurements of dus t samples, taken from pro to type r e a c t o r s ,
become a v a i l a b l e i t might be va luab le t o i n j e c t a s i m i l a r mixture i n t o
t h e loop t o f i n d ou t t h e p l a t e -ou t p a t t e r n on a c ross f low steam b o i l e r .
D. D. Tytga t : To what e x t e n t w i l l t h e i r r a d i a t i o n cond i t ions i n t h e
P lu to B loop be comparable t o t h e HTR power r e a c t o r ?
R. H. Flowers: The loop w i l l i r r a d i a t e a s h o r t l eng th of a r e a l i s t i c
f u e l element a t t h e chosen temperature , wi th helium coo l ing under t h e
c o r r e c t load conri i t ion. The helium w i l l be cooled from around 750' C . @
3 60
t o 300' C . i n a c ross f low water-cooled depos i t i on u n i t , t h e tube su r face
temperatures and hea t f l u x e s being a d j u s t a b l e t o match t h e des i r ed steam
b o i l e r cond i t ions very c l o s e l y i n a l l important r e spec t s .
L. R . Zumwalt: 1. Do you have any evidence for o r u t i l i z e a " f a s t "
d i f f u s i o n c o e f f i c i e n t f o r t h e d i f f u s i o n of metals ( C s and S r ) i n g r a p h i t e ,
2. How do you e s t i m a t e t h e evapora t ion c o e f f i c i e n t f o r metal f i s s i o n
products from g r a p h i t e a s used i n your c a l c u l a t i o n s ?
R. H. Flowers: W e have seen long "tai1.s" on d i f f u s i o n p r o f i l e s ob-
t a i n e d from i n p i l e experiments and t h e s e might be t h e r e s u l t of r a r e gas
p recu r se r d i f f u s i o n . However, some r e c e n t ou t -of -p i le i s o t o p i c d i f f u s i o n
experiments a t Harwell , us ing s t ron t ium i n t h e concen t r a t ion range 0 - 100
mg/g, have y ie lded unambiguous p r o f i l e s corresponding t o a s i n g l e d i f f u s i o n
r a t e . W e a r e hopeful t h a t t h e e a r l i e r r e s u 1 . t ~ w e r e anomalous "precurser"
or concen t r a t ion e f f e c t s , but i t i s t o o e a r l y t o be d e f i n i t e on t h a t po in t .
Evaporat ion c o e f f i c i e n t s a r e obta ined by assuming t h a t t h e equi l ibr ium
metal vapor p re s su re e x i s t s a t t h e g r a p h i t e su r face . A convent iona l mass
t r a n s f e r equat ion of t h e type kd/D = .023 R e Sc i s then used t o g ive
t h e evapora t ion c o e f f i c i e n t .
0.8 0 . 3
J . H. Norman: Would you compare f i s s i o n product r e l e a s e f o r a
r e a c t o r wi th tubu la r e lements and wi th te lephone d i a l e lements f o r
s i m i l a r power o u t p u t s ?
R . H. Flowers: In surveys of f i s s i o n product r e l e a s e from c o r e s
comprising elements of d i f f e r e n t geometr ies , i t i s always found t h a t t h e
f u e l tube su r face temperature c o n t r o l s t h e C S and S r emission, while t h e
coa ted p a r t i c l e temperature (and, t h e r e f o r e , s i m i l a r i o d i n e and r a r e gas
r e l e a s e ) showed a g r e a t e r metal r e l e a s e from t h e t u b u l a r element. The
t u b u l a r element had a somewhat h ighe r l i n e a r power r a t i n g , however.
Paper 3/104
\ 0 * FISSIOil PRODUCT TUXSPORT I i J HTGR SYSTEIyls - A SUI@I4lpI *-- A,-- ~ - ' -%-.--= I ~ - suz*r. W&F* *&&,*n*&, iw-i**ii'*" *
F. E . Vanslager and I/. E. Be11 Gulf General Atomic Incorporated
San Diego, California 92112
0. Sisman and M. T. Morgan Oak Hidge National Laboratory Oak Ridge, Tennessee 37830
ABSTRACT
A br ie f summary of f i s s ion product t ransport i n a gas- cooled reactor i s preseuted. Analytical methods applicable t o reactor s i tua t ions a re presented along w i t h a var ie ty of old and new experimental data t o i l l u s t r a t e the calculat ional techniques. These methods indicate t h a t the gaseous ac t iv i ty i n a well-designed gas-cooled reactor system can be e a s i i j held t o acceptable leve ls and w i l l consis t almost en t i r e ly of noble gases. noble gas precursors a s well a s from the halogen precursors which a re found t o have release ra tes essent ia l ly equal t o noble gases. cautions are taken, w i l l not be released from the f u e l elements i n suf f ic ien t quant i t ies t o s ignif icant ly increase the plateout levels above t h a t resu l t ing from these gaseous precursors.
Some plateout a c t i v i t y w i l l r e s u l t from these
The other f i s s ion products, provided n o m 1 pre-
INTRODUCTION
The in t en t of t h i s paper i s (1) t o point out the main features of f i s -
sion product behavior i n EPM;R systems, (2) t o suwDarize recent develop- ments i n the analysis of f i s s ion product release and plateout, and (3) t o summarize the r e su l t s of recent investigations of f i s s i o n product release.
A typ ica l HTCTR system might have f'uel consisting of uranium and thorium dicarbide kernels (microspheres) overcoated with layers of pyro- l y t i c carbon and dispersed i n a bonding or f i l l e r matrix of carbonaceous
* Work supported i n par t by the U. S. Atomic Energy Commission.
361
362
material. s i l i con carbide layers are often irxorporated i n the f u e l pa r t i c l e coat- ings. graphite blocks which are cooled by 8 circulat ing helium coolant stream.
Oxide kernels, as well a s dicarl=:ide kernels, can be used; a lso,
The f ie1 mater ia l i s contained i n fuel elements consisting of
The primary ba r r i e r t o the release of f i s s ion products i n to the helium
coolant system is the coating on each individual f u e l pa r t i c l e . t i ve secondary ba r r i e r f o r metall ic f i s s i o n products i s the retent ion and sorption property of the f u e l matrix mater ia l and the f u e l element s t ruc- t u r a l graphite.
the helium coolant stream. i n t o the coolant a re maintained a t a sa t i s fac tory l eve l by employing a bypass cleanup system. processes a portion of the coolant stream through a series of adsorp- t i on beds culminating i n a cryogenic bed which removes essent ia l ly a l l of the f i s s i o n products i n t h i s helium s t r e a m .
An effec-
These ba r r i e r s l i m i t the release of f i s s ion products i n t o Gas-borne f i s s ion products t ha t a re released
This helium pur i f ica t ion system continuousljr
I n addition t o the helium pur i f ica t ion system, the steam generators and other reactor components a re e f fec t ive i n removing (by plateout) f i s s ion products other than the noble gases.
t u t e the majority of the gaseous a c t i v i t y i n ? a reactor c i r c u i t . Consequently, the noble gases consti-
DIFFUSION OF FlSSION PRODUCTS
The t ransport of f i s s ion products i n a stagnant medium i s generally described by a diffusion equation of the form
where C i s the concentration, t i s the time, D i s the diffusion coeffi-
c ient , A i s the decay constant, and B i s the b i r th r a t e per un i t volume. I n coated fie1 pa r t i c l e s with spherical symmetry and a constant diffusion
coeff ic ient , t h i s equation takes the form
363
0 This equation can be used t o t r e a t the formation, diffusion, and decay of a f i s s i o n product nuclide i n e i t h e r the kernel or coating, or both. Gen- e ra l ly , a buffer layer of low-density pyrolytic carbon e x i s t s between ker- n e l and coating, but t h i s can be neglected.
For the case where the b i r t h r a t e is constant throughout a pa r t i c l e (e.g., a bare uranium carbide pa r t i c l e ) , the solution t o Eq. ( 2 ) , assuming
time-independent properties and zero i n i t i a l and outside concentrations, i s readi ly obtained.
terms of the R/B value, which i s the instantaneous release rate divided by the b i r t h r a t e .
The release of f i s s i o n products is usually expressed i n
This R/B value a s a function of t i m e i s given by
where a i s the outside radius of the pa r t i c l e . This expression s t a r t s a t zero a t time zero and reduces t o the first t e r m a s t approaches in f in i ty . That is,
This equation represents the steady-state behavior. The so l id l i ne on Fig. 1 is a p lo t of Eq. (4) and i l l u s t r a t e s t h a t the release from uncoated (bare) pa r t i c l e s should be proportional t o the square root of the f i s s i o n product ha l f - l i f e f o r R/B values l e s s than 0.1.
If there i s a pyrolytic carbon coating on the pa r t i c l e , Eq. (2) must be solved with a s tep change i n the b i r t h r a t e a t the kernel/coating interface--down t o a value indicative of coating contarnination. The dashed l i n e s on Fig. 1 i l l u s t r a t e the txhavior t h a t would be expected f o r
d i f f e ren t values of the ' b i r th r a t e r a t i o B2/B1, where B2 and B1 are the b i r t h ra tes i n the coating and the kernel, respectively. noted t h a t the behavior is qui te d i f fe ren t i f there is no contamination i n
I'c should be
@
3 64
the outer coating; i . e . , B /B = 0. However,, it should a l so be noted t h a t @ the posi t ion of the curve f o r B2/Bl = 0 depends on the r a t i o of the kernel and coating diffusion coeff ic ients , the sorptive a b i l i t i e s , and tlie r a d i i of
the two regions. cussed i n d e t a i l by Dunlap and Gu1den.l)
2 1
(The equilibrium R/B value f o r coated par t ic les i s d i s -
Numerous experiments on noble gas f i s s ion product release from coated pa r t i c l e s have been conducted.
t h a t were car r ied out by Gulf General Atomic (GGA) are shown i n Fig. 2 i n p lo ts of the steady-state Kr-b5m R/B values vs operating t i m e f o r the
The r e su l t s of some typica l experiments
GR2-284-6F2 f u e l capsule ( C e l l I),2 the GAIL IIIB l0opy3 the GAIL IV loop, 4
and the Peach B o t t o m r e a ~ t o r . ~ The data f o r the 6F2 capsule and the
GAIL IIIB and GAIL rV loops a re a l l a t roughly comparable temperatures. However, the Peach Bottom reactor r e su l t s should be multiplied by approxi- mately a f ac to r of 2 t o account f o r a somewhat lower temperature than f o r the capsule and the GAIL t e s t s . The increase i n the K/B values wi th time i s probably indicat ive of coating f a i l u r e . the 6 ~ 2 capsule, i n GAIL IIIB, and i n the Peach Bottom reactor (Core I) had an ear ly type of coating and showed a re la t ive ly high degree of f a i lu re ,
whereas the coated pa r t i c l e s used i n G A I L IV had a l a t e r , improved type of coati% and showed a low degree of f a i l u r e .
33e coated pa r t i c l e s used i n
Figures 3 and 4 a r e p lo t s of the end-of-l ife R/B data vs ha l f - l i f e of 1
the f i s s i o n products. h a l f - l i f e ) dependence and the l i nes were drakm with t h i s slope.
l i f e dependence indicates t h a t the release i s from e i t h e r bare kernels or
high contamination i n the coatings. I n no case vas there an indication of the sharp increase i n release of long-lived f i s s ion products i n the manner indicated by the dashed curve with B2/Bl = 0 (see Fig. 1).
these experiments the geometrical and operational complexities of the
experiments should be borne i n mind. s ta ted t h a t a var ie ty of d i f f i c u l t i e s usually affected the accuracy of the
data points. )
The data generally show a (tl)" (square root of - 2
!I!his ha l f -
( I n a l l of
Without going i n t o de t a i l s , it can be
365
To more fu l ly understand the release process, the end-of-life Kr-85m R/B values a t 1300uC f o r a number of ORNL, Dragon, and GGA experiments are
assembled i n roughly chronological order i n Fig. 5. the r e su l t obtained by GGA the resu l t s obtained by ORNL f o r an uncoated carbide7 and a mechanically uncoated carbide.
Dragon Project. the 205; par t ic le f a i lu re . c les obtained from the GA 309 sweep capsule The next two are the resu l t s obtained from 1962 t o 1964 f o r the GAIL I I IA and I I I B in-pile loop experiments. 3’10 three-compartment 6~ sweep capsule2 i r radiated i n 1963. ment of t h i s experiment had fue l coated with multiple Layers of s i l i con carbide and pyrolytic carbon. Since only approximately one-fourth of the par t ic les f a i l ed during the i r radiat ion, the Kr-85m R/B value was arb i - t r a r i l y multiplied by a fac tor of 4 t o indicate release from the kernels alone.
The first point i s 6 for an uncoated carbide while the next two a re
The next point i s a Pluto I I IA result’ obtained by the 8
This re su l t was multiplied by a factor of 5 t o account f o r The next s ix are early resu l t s on coated pa r t i -
se r ies i r radiated i n 1960-61. 6
The next three are resu l t s from the The f i r s t compart-
The next point i s fram the GAIL IV experiment4 i r radiated from 1964 t o 1966. end-of-life, t h i s value was a rb i t r a r i l y multiplied by 125. The l a s t point
i s from Peach Bottom Core I result^.^ s u l t was increased by a fac tor of 2 t o account f o r the lower temperatures. This temperature correction i s obtained by assuming t h a t the release ra te has an exponential temperature dependence with an act ivat ion energy of
approximately 30 kcal/g mole.
Since it was Imoim t o have a par t ic le fa i lure of only O.@ a t
A s mentioned previously, t h i s re-
6
It can be seen from Fig. 5 that a l l of the end-of-life Kr-85m R/B values a re approximately the same i f one makes corrections f o r the amount of f a i l ed par t ic les . Therefore, it i s l ike ly tha t the end-of-life release
i s from exposed kernels ra ther than from diffusion out of contaminated coatings. to r t ion t o gross d is tor t ion with the f i n a l kernel volume more than twice the or iginal kernel volume.
dimension (a) i n Eq. (3) i s much smaller than the radius of the kernel.
Also, it was noted tha t par t ic le damage ranged from minor dis-
Therefox, it i s l ike ly tha t the character is t ic
356
The s imi la r i ty of the releases from a l l of these experiments indicates t h a t there i s a noble gas release r a t e charac te r i s t ic of f a i l e d fue l , and t h a t the r a t e i s r e l a t ive ly independent of i n i t i a l material o r of the degree of f a i lu re . Therefore, the reactor &signer can es tab l i sh the design noble gas release leve ls by determining the amount of f u e l
f a i lu re t o be expected and using a release curve obtained from an
appropriate experiment having approximately :E'ully f a i l e d fue l . ignores precursor contributions, the number of noble gas atoms i n the coolant
stream i s then governed by the equation
If one
where n i s the t o t a l number i n the coolant stream, f i s the f rac t ion of
the f i s s ions occurring i n f a i l e d fue l , and F i s the f r ac t iona l removal r a t e by the pur i f ica t ion system.
Although the s i t ua t ion i s r e l a t ive ly siciple from the reactor design
point of view, the d e t a i l s of the noble gas i-elease process need t o be b e t t e r understood.
reason f o r the d i f f e ren t krypton-to-xenon release r a t io s obtained from d i f f e ren t experiments. The above-mentioned CIGA experiments r a i se the possi- b i l i t y t ha t t h i s r a t i o i s approxbatelj . 2-1/2 for badly f a i l e d f'uel and 4-1/2 f o r r e l a t ive ly i n t a c t fue l . carbide par t ic les7 has indicated tha t there is no difference between the kry-pton and xenon release r a t e s .
For example, there i s not; a c l e a r understanding of the
However, an ORNL experiment on uncoated
There is a l s o disagreement among the vai*ious invest igators about the
in te rpre ta t ion of a ha l f - l i f e independent %ecoil" release, a s opposed t o diffusive release. Vanslager has maintained t h a t the word "recoi l" does not adequately describe the release process, since the recoi l ing pa r t i c l e inevitably ends up back i n a so l id u a t e r i a l from which it must be subse- quently released. These problems, and many others, warrant fur ther
investigation.
The normal reactor operating temperatures a re generally high enough so t h a t the release of halogens from the f u e l pa r t i c l e s is essent ia l ly
367
0 i den t i ca l t o tha t of the noble gases. of the iodine release r e su l t s obtained from decay experiments and diffusi-on tube r e su l t s . It can be seen tha t , withill experimental accuracy, the re- lease of iodine from the f'uel pa r t i c l e s i s ident ica l t o t h a t of xenon.
Figures 3 and 4 a l so include some
Farther ve r i f i ca t ion of the s l h i l a r i t y cf xenon and iodine release was obtained by recent work a t 0,WL. The release from pyrolytic carbon- coated i x a r i i u m carbide pz r t i c l e s with intent ional ly cracked coatings was
investigated a t a var ie ty of temperatures.
by holding the cooling gas flow constant and rais ing the temperature i n 200°C steps by increasing the f lux . the helium purge stream were measured a t steady-state conditions and a f t e r a sudden capsule withdrawal, t o determine iodine release. The continuing xenon release a f t e r withdrawal is frm iodine decay. a typ ica l p lo t of Xe-133 and Xe-135 decay a t 14OO0C, indicates t h a t the release of iodine frm f a i l e d pa r t i c l e s is similar t o t h a t of senori.
A s e r i e s of t e s t s vas conducted
The Xe-133 and Xe-135 releases i n t o
Figure 6, which i s
The released iodine is not adsorbed, or delayed t o any s igni f icant extent , by the f u e l element s t ruc tu ra l graphite. However, the metal sur- faces of the reactor c i r c u i t are quite e f fec t ive i n removing iodine. The
GAIL loop experiments have indicated t h a t the majority of "the iodine is re- moved i n a s ingle pass around the c i r c u i t . Computer programs have been developed'' t o handle t h i s mass transport problem. kctivity - Distribution), under development a t GGA, solves equations of the form
The PAD code (Plateout
aN 4k.KcMp
d(1 - ~ M . j M s . ) J J 3 sN
A = a t
HEMP
(1 -xMj/Ms.) (&) ' a. 3 = % + AiNi +
J j a t
where
S = source terms fo r coolant concentration and surface concen- J Mj t r a t ion of f i s s ion product j ,
368
N Ni = atom concentration of f i s s ion product j and i t s precursor i i n the coolant stream, j’
Mj, Mi = atom surface concentration of f i s s ion product j and i t s precursor i on the plateout surface,
hj’ hi = decay constant of f i s s ion product j and i t s precursor i,
x, t = a x i a l distance and time coordinates,
k = the mass transport coeff ic ient ,
d = the channel diameter,
V = the coolant flow velocity, anti
K ~ M : i s an expression f o r the desorption of f i s s ion
(1 - CMj/MSj ) product ,j from the surface i n t o the coolant. The PAD code can handle an a rb i t r a ry number of species in te rac t ing through the summation term.
Figure 7 i s a p lo t showing a typ ica l calculated iodine d is t r ibu t ion around a reactor c i r c u i t . It can be seen t h a t the iodine concentration i s great ly reduced by the reactor c i r c u i t components. For t h i s case the loop removal r a t e i s considerably grea te r than the pur i f ica t ion system removal rate and, consequently, the t o t a l amount of loop plateout i s ade- quately approximated by assuming instantaneous compleke plateout i n the c i r - c u i t .
estimated by employing a mass t ransport plateout code such a s PAD.
The c i r c u i t d i s t r ibu t ion of iodine, however, can only be accurately
The a l k a l i metals rubidium and cesium are of intermediate v o l a t i l i t y
a t normal reactor operating conditions. re la t ive ly unimportant, and t h e i r release c2.n be bounded without serious
consequences by using noble gas release r a t e s from the fue l . Cs-134
maintenance operations.
The short-l ived isotopes a re
However, * and Cs-137 a re of spec ia l i n t e r e s t because of t h e i r e f f e c t on
* Cs-134 is formed by a n (n,y) reaction on f i s s ion product Cs-133.
369
The release of these m e t a l s from the fuel pa r t i c l e s i s l i ke ly described by diffusion equations such a s Eq. (2 ) . However, the long-lived species Cs-137 and Cs-134 w i l l normally not reach equilibrium during the core lifetime. Consequently, the t rans ien t solut ion t o the equation i s required. t i o n and added complications when considering a multiregioned f u e l pa r t i c l e ,
the exact so lu t ion i s not readi ly ava i lab le . t i o n t o the equation i s of ten attempted.
by GGA, i s a numerical solut ion t o the general diffusion Eq. (1).
w i l l t r e a t any of the three basic one-dimensional geometries, i . e . , s lab geometry, r a d i a l cy l ind r i ca l symmetry, or spherical symmetry.
Unfortunately, because of slow convergence of the series solu-
Therefore, a numerical s o h - The FLPER code, ''' l3 developed
The code
Figure 8 shows some t yp ica l experimental Cs-137 data obtained from an out-of-pile i s o t h e m a l anneal of an i r r ad ia t ed fuel p a r t i c l e . The so l id l i n e i s the r e s u l t of a FIPEH analysis of the experiment using published
d i f fus ion coefficients'" f o r the p a r t i c l e coating. reasonable approximation has been obtained. However, computer t i m e l imi ta - t ions preclude performing a FIFXR analysis of a l l of the f u e l pa r t i c l e s i n a reactor core (each has a s l i g h t l y d i f f e ren t temperature and power h i s to ry ) . solut ion i s required. constant" model, i n which the release r a t e from the f u e l pa r t i c l e s i s assumed t o be d i r e c t l y proportional t o the inventory. A two-release-constant model presently under invest igat ion by GGA i s defined by the coupled equations
It can be seen t h a t a
Therefore, a closed-form approximation t o the f u l l numerical
Such an approximation i s provided by the "release
\
- = dnl B1 - Rlnl - Anl d t
- - dn2 - B2 + Rlnl - R,p2 - h2 d t
(7)
where n
pa r t i c l e , B1 and B2 a re the respective b i r t h rates, R1 and R2 are the respective release constants, and h i s the decay constant. release-constant model normally used i n reactor calculat ions is, of course,
defined by the first equation.)
and n2 are the t o t a l inventories i n regions 1 and 2 of the f u e l
(The s ingle-
1
The dashed l i n e s of Fig. 8 are the
370
two-release-constant approximation t o the annealing-experiment data. can be seen t h a t these curves provide a reasonable approximation t o the
ac tua l s i tua t ion and can therefore be used for reactor calculations of the release from the f u e l pa r t i c l e s .
It
After the release from the f u e l pa.rticl.es, there a re sorption and d i f -
fusion i n the f u e l element materials and evaporation i n t o the coolant stream. The complexity of the temperature/time histclry and the temperature depend- ence of the material properties again require a numerical solution t o
Eq. (1). approximation t o the release from the f u e l par t ic les , provides a reasonable
treatment of the problem. In general, the t ransport process i s complex and, under some 'circumstances, involves concentration-dependent diffusion coeff ic ients and multiple diffusion processes. The overal l transport process is highly temperature-dependent.
The FIPEH code, with a source given by the two-release-constant
The loss from the f u e l element surfaces is by evaporation described by Freundlich adsorption isotherms .15 A t mcderate temperatures the overal l diffusion and evaporation process represents a major ba r r i e r t o cesium loss from the core. Consequently, i f the reactor temperatures a re low enough, the d i r ec t loss w i l l be negligible and the noble gas precursors w i l l const i tute the major source of Cs-137 a c t i v i t y . a b i l i t y , Figs. 9 and 10 present some cesium a c t i v i t y prof i les measured on
the Peach Bottom DO6-01 f u e l element and the GAIL IV f u e l element.16 Each s e t of p ro f i l e s i s from a d i f fe ren t elevation along the length of the fue l elements. It can be seen from these steeply sloping prof i les t h a t the
d i r e c t loss of cesium i n these experiments was negligible.
A s an i l l u s t r a t i o n of t h i s re tent ion
The curves i n Figs. 9 and 10 a re the r e su l t s of an attempt t o f i t the data w i t h the FLPER code. The cesium diffusion coeff ic ient was the same for both of these experiments and, f o r some reason, appeared t o be very small
and t o have the extremely low ac t iva t ion energy of 3 kcal/g mole. Over t h e temperature range investigated, the temperature dependence of the diffusion coeff ic ient can ac tua l ly be approximated by a temperature t o the 3/2-power
dependence, indicating tha t the rate-l imiting s tep i s possibly gas-phase
transport a t the low concentration levels of these experiments. (It should
371
be noted t h a t these data cover three d i f f e ren t types of graphite, two of which were impregnated.) of the t rans ien t FIPER code r e su l t s ra ther than a confirmation of a diffusion process; it i s hoped tha t this d i f f i c u l t y can be resolved by examination of addi t ional Peach Bottom elements.
These curves should be considered an i l l u s t r a t i o n
The d is t r ibu t ion of cesium a c t i v i t y around the coolant c i r c u i t i s
determined by mass transport calculations such as the PAD code. In general, it i s mass-transport-limited ra ther than saturation-limited. m e n t ~ ' ~ have shown t h a t an approximately exponentially decreasing d is t r ibu- t ion i s obtained i n isothennal regions w i t h spikes a t points of abrupt flow
changes.
Loop experi-
A s i l i con carbide coating i s an extremely e f fec t ive ba r r i e r f o r cesium a s well as other metall ic f i s s i o n products.
The alkal ine ear th metals s t r o n t i m and barium are only moderately vo la t i l e a t normal reactor operating temperatures. Therefore, the release of isotopes other than Sr-u9, Sr-90, and Ea-140 can usually be ignored. "he 12.b-day Ba-140 chain i s important f o r reactor maintenance considerations because of the high-energy gamma rays emitted by the La-140 daughter. 30-year Sr-90 chain is important f r o m the standpoint of reactor safety.
This nuclide i s a bone-seeking beta emit ter which has a re la t ive ly high y ie ld and long ha l f - l i f e .
The
The alkal ine ea r th metals, being smaller i n diameter than the alkali metals, show considerably more so lub i l i t y i n pyrolytic carbon and thus grea te r release from coated pa r t i c l e s than t h a t i l l u s t r a t e d by the r e su l t s of the Cs-137 anneal i n Fig. 8. in-pi le re tent ion data given i n Table 1.
holdup i n the f u e l material and i n the graphite s t ruc tu ra l members. S i l i - con carbide coatings e f fec t ive ly r e t a i n the alkal ine ear th metals a s indi-
cated by ORNL data given i n Table 1 and by GGA data given, f o r example, i n Ref. 18.
This i s shown, f o r example, by the ORNL However, there i s s t i l l s ign i f icant
\
372
Figure 11 shows the r e su l t s of a s e r i e s of out-of-piie strontium d i f - fusion experiments performed a t W. The so l id l i nes on these p lo ts are the
r e su l t s of a FI?ER analysis using the GGA reference design diffusion coef- f i c i e n t data. It can be seen t h a t a reasonable f i t t o the data has been obtained, coilsidering the experimental d i f f i c u l t i e s and uncertaint ies .
Barium, compared t o strontium, has an even longer diffusional holdup;
thus, E .8-day Ea-140 w i l l decay very s igni f icant ly during t r a n s i t through
the s t ruc tu ra l graphite. the major source of Ea-140 a c t i v i t y i n a noma1 reactor s i tua t ion .
*
I
The Xe-140 precursor will therefore const i tute
Mass transport calculations a r e performed t o determine the a c t i v i t y
However, f o r Sr-90 an attempt must d i s t r ibu t ion i n the reactor c i r c u i t . a l s o be made t o determine the physical form of the deposit i n order t o analyze accident s i tuat ions, e.g., the rapid depressurization accident which could lead t o e jec t ion of Sr-90 from the reactor containment. revola t i l i za t ion of Sr-90 from metal surface:; i s re la t ive ly negligible. Therefore, the major concern i s with aerosols o r wi th the f l u i d shear removal of dust pa r t i c l e s containing Sr-90. a s t o preclude the release of Sr-90 from the containment, the Sr-90 d is - t r ibu t ion i s of minor importance t o the reactor design.
The
If a plant i s constructed so
The good retent ion of strontium, a s well. a s of other f i s s i o n product metals i n H E R f u e l elements, i s confirmed i n the Peach Bottom reactor .
The f r ac t iona l release of Sr-90 i n t o the main coolant a f t e r 300 ef fec t ive full power days was measured t o be 1 x 10
f u e l particles.5 decay from the Kr-90 precursor.
-6 , even with essent ia l ly uncoated
This release of Sr-90 can be completely accounted f o r a s
NONVOIATIIZ AND REFRACTORY METAL REXUsE
Most of the remaining f i s s ion product metals are retained i n high degree by t h e f u e l and a r e essent ia l ly nonvolatile a t normal reactor opera-
t ing temperatures. This i s shown, f o r example, by the ORNL retent ion data
for Zr-95, Ce-144, and RU-106 given i n Table 1. Ruthenium-106 and Zr-95 a re often used t o determine the t o t a l amount of f i ss ions tha t have occurred i n a Y
The reference diffusion coef f ic ien t data f o r s t ontium i n graphite are described by t h e equation In D = 5.7 - 3.0 x 10 E
T
373
@ reactor experircent; i . e . , the assumption i s made t h a t there i s essent ia l ly
no loss of these species during t h e experiment. t h i s assumption.
The data i n Table 1 verify
HEAVY METAL RELEASE
The uranium and other heavy metals are a l so re la t ive ly nonvolatile a t normal reactor operating conditions. is some amount of migration i n t o the pyrolytic carbon coatings on the f u e l pa r t i c l e s . The only important e f f ec t should be an increase i n the halogen and noble gas release from the f u e l pa r t i c l e s . This could be important since, i n a properly designed reactor system, the predominant source of a c t i v i t y i s from the halogen and noble gas precursors of the metall ic f i s s ion products.
However, a t high temperatures there
Figure 12 shows experimental data on the release of noble gases from par t i c l e s subjected t o a high-temperature anneal u n t i l there i s some uranium migration through the pyrolytic carbon coating.19 upper r igh t portion of the f igure represent the release from f u e l pa r t i c l e s
i n a carbon matrix apparently saturated w i t h uranium. r igh t i s the release from the pa r t i c l e s alone, i . e . , from saturated pyro- l y t i c carbon coatings. carbon have led t o an increased R/B by providing a shorter diffuc ,ion distance f o r the f i s s i o n products (dis t r ibuted relat ively uniformly by the recoil
process) . f o r the difference i n the matrix granule s izes , would be comparable t o the end-of-life releases plot ted i n Fig. 5 . Therefore, t h i s experiment does not
represent a new fa i lu re mechanism, but ra ther i s an i l l u s t r a t i o n of the sur- rounding granule s ize e f f e c t on noble gas R/B values.
The data points i n the
The lover point a t the
It can be seen t h a t the smaller granule s izes of the
Thus, the release from these "fai led" pa r t i c l e s , when adjusted
I n a well-designed reactor system the f i s s ion product a c t i v i t y can be eas i ly held t o acceptable levels and w i l l r e su l t primarily from t h e release
of noble gases and halogens from the fuel elements.
w i l l consis t almost en t i r e ly of noble Gases, since the halogens w i l l be
The gaseous a c t i v i t y
a
374
removed (by plateout) very- e f fec t ive ly by the loop components. out a c t i v i t y d is t r ibu t ion can be reasonably approximated i f suf f ic ien t experimental information i s obtained.
This plate-
The other f i s s ion products, provided normal precautions a re taken, w i l l not be released from the f u e l elements i n quant i t ics large enough t o s ign i f icant ly increase the plateout l eve l above t h a t resul t ing from the
gaseous precursors. Some of these precautions are: ment temperatures, (2) t o minimize f u e l pa r t i c l e f a i lu re , and ( 3 ) t o pro- vide suf f ic ien t sorptive mater ia l t o r e t a i n the metall ic f i ss ion products.
A s i l i con carbide coating on the f u e l pa r t i c l e s i s a l so an effect ive primary ba r r i e r t o the release of metall ic f i s s ion products.
(1) t o l i m i t f u e l ele-
1.
2.
3 -
4.
5.
6.
7.
8.
11. W. Dunhp and T. D. Gulden, Nucl. Sei. Eng. 2, 40'7 (1968).
F. E. Vanslager e t a l . , F ina l Report on the GA2-2uh-6F2 Fuel I r rad ia- t i on Experiment, W - 5 9 2 5 , General Dynamics Corporation, General Atomic Division (1965).
R. F. Turner e t a l . , I r rad ia t ion Test of the GAIL I I I B Fuel Element i n the General Atomic In-Pile Loop, USAEC Report GA-53111, General Dynarnics Corporation, General Atomic D:ivision (1964).
E . 0. Winlcler e t a l . , I r rad ia t ion Test and Post i r radiat ion Examina- t i on of the GAIL IV Fuel Element i n the General Atomic In-Pile Loop, USAEC Report a-7997, General Dynamics Corporation, General Atomic Division (1967).
40 -hDd ( e ) Pro t o t n e High -Temperature Gas -Cooled Reactor Post c on s t ruc ti on Research and Development Program. Period Ending October 31, 1969, U W C lieport GA-9797, Gulf General Atomic Incorporated (1969) .
Quarterly Progress Report For t h e
L. R. Zumwalt , E. E . Anderson, and P. I:. Gethard, Materials and Fuels for High-Temperature Nuclear Energy Applications , Proceedil?e;s of the National Topical Meeting of the American Nuclear Society, Chapter 9, M.I.T. Press, Cambridge, Mass., 1964.
P. E . Rea.gan, J. G. Morgan, and 0. Sisnlan, Nucl. Sci. Eng. 9, 215 (1965 )
P. E. Reagan, E . L. Long, Jr., J. G . Morgan, and T. 11. Fulton, ORNL unpublished data.
0 9*
10.
11.
12.
13
14.
1-5
16.
17 9
18.
19
375
E. Groos and H. J. de Nordmll, Post i r radiat ion Radiochemical Analysis of the Loop Pluto I11 A, United Kingdom Atomic Energy Report AEFiE-Bb~t34 (1964).
D. R. Lofing and L. R. Zumwalt, H3GR In-Pile Loop Experiment Act ivi ty Analysis GAIL I11 - A Fuel Element, U W C Report W4D-3376, General Dynamics Corporation, General Atonic Division (1962).
T. S . Kress and Paul Nelson, Jr., Numerical Solution of t h e Isothermal - Fission-Product Deposition Equations: the program pX3DE?-II, -7).
J. Appel and B. Ibos, Nucl. Sci. Eng. &, 201 (1968).
B. 14. Roos and J. E . Welch, FIPER 1, A FORTRAN IV Program for the Zelease of Fission Products from a High Tempemtun? Gas-Cooled Nuclear Power Reactor, USAEC Report GA-8564, Gulf General Atomic Incorporated (1968) . P. E . Gethard and L. R. Z m w a l t , Nucl. Appl. - 3 , 679-685 (1967).
H E R Base Program Quarterly Progress Report For the Period Ending USAEC Report GA-9372, Gulf General Atomic Incorporated
W. E. Bell, E. E. Anderson, and C. E. Milstead, Post i r radiat ion Chemical Examination of the GAIL N Fuel Element, U W C Report
General Dynamics Corporation, General Atomic Division
T. S . Kress, Parameters of Isothermal Fission-Product Deposition (Thesis ) , ORNL-Tl4-1330 (1965 ) . HrCrR Base Program Quarterly Progress R e p o r t f o r the Period Endin& February 2b, 1967, USAEC Report GA-7801, General Dynamics Corporation, General Atomic Division (1967) . G . E . Besenbruch, C . C . Adams, J. N. Graves, arid R. Zamcki, Gulf General Atomic Incorporated, pr ivate comunication.
376
Table 1. Retention of Fission Product Metals fmm Coated and Uncoated Fuel Particles m n g Irradiation (ORNL ~ t a )
coating
Buffer
Bare
Bu-Is0
FyC
FyC-Sic
b
NA denotes not available. bFailed
End-of-life P,/B fo r k-88 was 3 x 10-5. L d - o f - l i f e R/B fo r e - 8 8 was io-8.
a
C
R / B - R E L E A S E RATE B I R T H R A T E
1 .o
10-1
10-3
1 o - ~
10-5
1 o -6
10-7
Zr-95
0.96
0.95
1.0
1 .o
1.0 -
Fl2
~e-144 -- -- 0.96
NA
0.93
1.0
1.0 --
t ion I
sr-89 -
NAa
0.067
0.24
0.53
NA
und i n Ba-140
m 0.21
NA
0.56
1.0 - 0.97
1.0
10-1 1 oo l o 1 1 o2
Fig. 1. Steady-State R/B Values vs &ilf-Life and Coating Contamination.
Fig. 11. Strontium Diffhsion Prof i les a t 1 0 0 0 ~ ~ .
TOTAL U - 2 3 5 I N THE COKE (/.LG)
Fig. l.2. Steady-State Kr-85m RIB Values v s U-235 Concentration i n the Carbon Matrix.
384
A
DISCUSSION
R . H . Flowers: You showed a number of r e s u l t s on t h e R/B r a t i o f o r
Krypton 85 from d i f f e r e n t ke rne l s , a l l being c l o s e t o 10 . Was t h e r e a
s o l -gel ke rne l among them?
-2
F. E . Vanslager: I am n o t su re .
R . H . Flowers: Have you had any experimental confirmation of r e s u l t s
ob ta ined with t h e FIPER code on problems involv ing an evaporat ion s t e p .
F. E . Vanslager: A t t h i s t i m e t h e comparison of FIPER wi th exper i -
mental r e s u l t s i s l i m i t e d t o d i f f u s i o n p r o f i l e s .
E . Formann: Do you r e l a t e r e l e a s e of m e t a l l i c f i s s i o n products t o a
g r a p h i t e s p e c i f i c a t i o n ?
F. E . Vanslager: No. In gene ra l w e do our exper imenta t ion on t h e
kind of g r a p h i t e t h a t w i l l be used i n t h e a c t u a l r e a c t o r . Therefore , w e
have removed t h i s a s a v a r i a b l e and have no need t o s p e c i f y f i s s i o n product
r e t e n t i o n p r o p e r t i e s t o t h e g r a p h i t e manufacturer .
H. J . deNordwall: The observed S r d i f f u s i o n c o e f f i c i e n t s a r e n o t
p r e c i s e enough t o d i s t i n g u i s h d i f f e r e n c e s between g r a p h i t e s . However,
s i n c e d a t a f o r pyrocarbon, a l l s t r u c t u r a l g r a p h i t e , and powdered carbon
a r e p r e s e n t l y represented by t h e same l i n e d e s c r i b i n g t h e v a r i a t i o n of D
wi th temperature , w e f e e l t h a t d i f f e r e n c e s between g r a p h i t e s w i l l be minor.
F. E . Vanslager: I agree .
D. B. Trauger: Previous ly t h e r e have been p r e d i c t i o n s t h a t cesium
i o d i d e might be t h e p r e v a i l i n g form f o r t h e s e two elements. What i s t h e
p re sen t t h ink ing?
F. E . Vanslager: Because of t h e s t e e p l y s lop ing concen t r a t ion
p r o f i l e s measured i n t h e G A I L I V and Peach Bottom elements , t h e present
t h ink ing i s t h a t t h e cesium migra t ion i s more l i k e l y t o have been a s
e lementa l cesium r a t h e r than a s cesium iod ide .
A H. J . deNordwal1: Recombination of C s smd I does n o t seem t o occur
i n t h e g a s phase.
385
F. P. Ashworth: Dragcn p la te -out probe da ta i n d i c a t e s t h a t i o d i n e
e x i s t s i n t h e coo lan t i n t h e monoatomic form wi th a sinall amount (say 10%)
c o n t r i b u t i o n from a l a r g e r molecule such a s I 2 '
L. R . Zumwalt: A po in t f o r c l a r i f i c a t i o n : Would uranium migra t ion
through f u e l coa t ings post a problem regard ing f i s s i o n product r e l e a s e
a t t h e f u e l temperatures contemplated f o r normal HTGR ope ra t ion?
F. E . Vanslager: No, The d a t a presented i n t h e s l i d e g iv ing
uranium migra t ion through t h e p a r t i c l e coa t ings were obta ined by hea t ing
p a r t i c l e s t o temperatures above 2000O C . A t r e a c t o r temperatures of t h e
o rde r of 1300° C . , t h e uranium migra t ion should be n e g l i g i b l e .
H. J . deNordwal1: What i s t h e evidence f o r t h e Iodine 131 a c t i v i t y
i n t h e gas phase a s d i s t i n c t from t h e s u r f a c e concen t r a t ion ( f a l l i n g a s
p red ic t ed ) ?
F. E . Vanslager: There were p la te -out probes l o c a t e d a t t h r e e
d i f f e r e n t p o s i t i o n s i n t h e G A I L loop. From t h e s e probes t h e p a r t i a l
p re s su res of Iodine 131 could be c a l c u l a t e d a t t h e s e p o s i t i o n s . Inva r i -
a b l y t h e lowest temperature probe i n d i c a t e d a l a r g e reduct ion i n gaseous
i o d i n e concen t r a t ion due t o p la te -out i n t h e hea t exchanger.
E . Hoinkis : I n your d i f f u s i o n equat ion t h e r e i s no term t o t ake
i n t o account t r app ing of d i f f u s i n g atoms. Could you p l ease comment on
t h i s ?
F. E . Vanslager: The equa t ions presented a r e r e l a t i v e l y gene ra l
equat ions , and, of course , cover t h e two c a s e s of t r app ing p ropor t iona l
t o t h e concen t r a t ion or of cons t an t t r app ing . Other t ypes of t r app ing
terms a r e inc luded whenever needed.
F. H. N e i l l : Where do you b e l i e v e i s t h e g r e a t e s t need f o r a d d i t i o n a l
experimental d a t a f o r t h e complete understanding of f i s s i o n product t r a n s -
p o r t and depos i t i on?
F. E . Vanslager: Personally,my g r e a t e s t need a t t h i s t i m e i s f o r
d e t a i l e d f i s s i o n product d i s t r i b u t i o n s i n loops and r e a c t o r s i n o rde r t o
e s t a b l i s h t h e c o n s t a n t s for t h e mass t r a n s p o r t codes. Addi t iona l i n f o r -
mation on t h e phys ica l form of t h e f i s s i o n product d e p o s i t s i s a l s o
needed, s i n c e t h i s can g r e a t l y a f f e c t t h e d i s t r i b u t i o n of a c t i v i t y . @
386
A
R . E . Blanco: I would l i k e t o ask the same ques t ion I asked D r .
Ashworth. What i s the mechanism and bui ldup r a t e of t r i t i u m i n the gas
c o o l a n t ? I r e a l i z e t he r e l e a s e l i m i t s f o r t r i t i u m a r e high, bu t they may
be lowered i n the f u t u r e . A r e there any p lans f o r t r i t i u m removal from
t h e gas coo lan t?
F. E . Vanslager: The three major c a l c u l a t e d sources of t r i t i u m i n
an HTGR a r e from l i t h i u m contaminat ion, t e r n a r y f i s s i o n , and He-3 a c t i v a -
t i o n . I n gene ra l t h e amount of t r i t i u m a c t u a l l y found i n t he coo lan t i s
a ve ry small f r a c t i o n of t h e c a l c u l a t e d amount produced. The g r a p h i t e and
f u e l would appear t o be q u i t e e f f e c t i v e i n r e t a i n i n g t r i t i u m . A t y p i c a l
HTGR p u r i f i c a t i o n system i s designed t o remove hydrogen ( t r i t i u m ) from
t h e c i r c u l a t i n g coo lan t , and d i s p o s a l can normally be accomplished i n any
d e s i r e d manner without undue compl ica t ions .
C. B. von d e r Decken: We d i d measure t r i t i u m i n t h e primary and
secondary c i r c u i t of t h e AVR. E s t i m a t e s hakre shown t h a t t h e q u a n t i t y
corresponds t o the sources , i . e . by f i s s i o n and by l i t h i u m i m p u r i t i e s .
A s a l r eady mentioned w e a r e doing experiments which should make c l e a r
t h e process of d i f f u s i o n i n t o t h e secondary sys t ems .
F. P. Ashworth: , , T r i t i u m concen t r a t ions measured i n Dragon vary
between a f a c t o r of 10 and 50 lower than va lues predicted from t h e
l i t h i u m impur i ty i n the g r a p h i t e .
J . D. Har t : What a r e the chemical forms of the r e l e a s e d f i s s i o n
products? Would these forms be dependent upon the o t h e r i m p u r i t i e s i n
t he coolan t , and would chemical form a f f e c t p la te -out and l i f t - o f f
c h a r a c t e r i s t i c s .
H. J. deNordwal1: W e can only guess at. presen t . Assoc ia t ion of
metal f i s s i o n product atoms w i t h o t h e r atoms must a f f e c t cohesion, so
c o r r e c t i d e n t i f i c a t i o n of molecules i s important .
A
Paper 4/111
S H E A R-FAILU R E S I N _E&D-S,La B,S,O PRESTRESSED CONCRETE PRESSURE VESSELS
6a 0
T h i s repc t desc
M. A . Sozen W . C . Schnobr ich n l S . L . Paul G!
2
ABS TRAC T
ibes t h e behav io r o f PCRV's p r e s s u r i z e d i n t e r n a l l y t o f a i l u r e . o b j e c t o f t h e t e s t s was t o i n v e s t i g a t e t h e
s i x smal l - sca le The p r imary i n f 1 uence o f
p e n e t r a t i o n s on t h e shear s t r e n g t h o f t h e end s l a b . Msasured s t r a i n s and c a l c u l a t e d s t r e s s e s i n t h e end s l a b a r e d i scussed q u a n t i t a t i v e l y t o " e s t a b l i s h " t h e mechanism o f t h e observed f a i l u r e s .
INTRODUCTION
A s e r i e s o f t e s t s o f s m a l l - s c a l e p ressu re v e s s e l s d e s c r i b e d i n
r e f e r e n c e 1 demonstrated t h a t t h e f l a t end s l a b o f a c y l i n d r i c a l p r e -
s t r e s s e d c o n c r e t e p ressu re vesse l tends t o r e s i s t t h e i n t e r n a l p ressu re
as an i n v e r t e d dome a f t e r t h e i n i t i a t i o n o f c r a c k i n g . Thus, t h e u l t i m a t e
c a p a c i t y o f t h e end s l a b i s r e l a t e d t o t h e s t r e n g t h s o f t h e e s s e n t i a l
e lements o f t h e dome system. The s t r e n g t h o f t h e system may be l i m i t e d
by (a ) t h e f r a c t u r e o f t h e l o n g i t u d i n a l r e i n f o r c e m e n t , which p r o v i d e s
t h e v e r t i c a l r e a c t i o n , ( b ) t h e f r a c t u r e o f t h e c i r c u m f e r e n t i a l r e i n f o r c e -
ment, which p r o v i d e s t h e hoop f o r c e s , and ( c ) by f a i l u r e o f t h e c o n c r e t e
i n t h e dome.
I n t h e s e r i e s o f vesse ls t e s t e d , t h e s l a b f a i l u r e i n mode(c) was
a s s o c i a t e d w i t h t h e development o f i n c l i n e d c racks which carved a dome
o u t o f t h e t h i c k end s l a b l e a d i n g t o h i g h normal and s h e a r i n g s t r e s s e s i n
t h e conc re te . The presence o f p e n e t r a t i o n s i n an end s l a b s u s c e p t i b l e t o
i n c l i n e d c racks was expected t o agg rava te t h e s t r e s s c o n d i t i o n s i n t h e dome.
The s e r i e s o f t e s t s and a n a l y s i s b r i e f l y r e p o r t e d i n t h i s paper were c a r r i e d
o u t p r i m a r i l y t o i n v e s t i g a t e t h e i n f l u e n c e o f p e n e t r a t i o n s on t h e s t r e n g t h o f t h e end s l a b s f a i l i n g i n shear. 63
388
TEST VESSELS AND PROCEDURE
Dimensions.--The d imens ions o f t h e t e s t vesse l a r e shown i n F i g . 1 .
Vesse l P V 1 6 had a s o l i d end s l a b w h i l e t h e end s l a b s i n t h e o t h e r f i v e
specimens were p e r f o r a t e d w i t h 2 - i n . o r 4 - i n . d iamete r p e n e t r a t i o n s as
i n d i c a t e d .
Concrete.--The c o n c r e t e was made w i t h Type I11 cement, c rushed
l i m e s t o n e (one - in . maximum s i z e ) , and Wabash R i v e r sand. The average
compress ive s t r e n g t h s for each vesse l de te rm ined by t e s t s o f 6 by 12 - in .
c y l i n d e r s a r e l i s t e d i n Tab le 1 . T e n s i l e s t r e n g t h s , l i s t e d i n t h e same
t a b l e , were based on s p l i t t i n g t e s t s o f 6 by 6 - i n . cy1 i n d e r s .
P res t ress ing . - -The c i r c u m f e r e n t i a l p r e s t r e s s i n g f o r c e was p r o v i d e d
by 0.25-in. round h i g h t e n s i l e s t r e n g t h s i n g l e w i r e wrapped c o n t i n u o u s l y
a round t h e v e s s e l a t a s p a c i n g o f 0.25 i n . The e f f e c t i v e p r e s t r e s s i n g
f o r c e s i n t h e w i r e a r e l i s t e d i n Tab le 1 .
The l o n g i t u d i n a l p r e s t r e s s i n g f o r c e was p r o v i d e d i n each v e s s e l by
60 S t r e s s t e e l r o d s h a v i n g a d iamete r o f 0.75 i n . Tab le 1 l i s t s t h e t o t a l
e f f e c t i v e f o r c e fo r each v e s s e l .
Seal.--A 1 /16 - in . t h i c k neoprene l i n e r was used t o s e a l t h e t e s t
v e s s e l s . A s t i f f e n e d 0 .5 - in . s t e e l p l a t e c l o s e d t h e open ings on t h e
p r e s s u r i z e d s u r f a c e o f t h e end s l a b . The p l a . t e r e a c t e d a g a i n s t t h e i n n e r
s l a b s u r f a c e .
Measurements . - - I n a d d i t i o n t o t h e p r e s s u r e i n t h e vesse l and d e f l e c -
t i o n s o f t h e o u t e r s u r f a c e , s t r a i n s were measured on t h e p r e s t r e s s i n g
r e i n f o r c e m e n t , on t h e i n n e r and o u t e r s u r f a c e s o f t h e end s l a b , and on
t h e w a l l s o f t h e p e n e t r a t i o n s . Crack t r a j e c t o r i e s were r e c o r d e d by
o b s e r v i n g t h e o u t e r s u r f a c e o f t h e end s l a b d u r i n g t h e t e s t and by
e x a m i n a t i o n o f t h e d e b r i s a f t e r t h e t e s t . T r a j e c t o r i e s o f t h e i n c l i n e d
c r a c k s i n t h e s l a b were e s t a b l i s h e d by c u t t i n g s e c t i o n s i n t h e end s l a b
i f t h e end s l a b s u r v i v e d t h e t e s t i n one p i e c e .
389
Pressu r i z ing . - -The t e s t v e s s e l s were i n i t i a l l y f i l l e d w i t h wa te r and
t h e n p r e s s u r i z e d w i t h n i t r o g e n gas. The p r e s s u r e was a p p l i e d i n i n c r e -
ments r a n g i n g f r o m 250 t o 100 p s i . Each t e s t t o o k a p p r o x i m a t e l y s i x hou rs .
BEHAVIOR OF THE TEST VESSELS
The response c h a r a c t e r i s t i c s o f t h e t e s t v e s s e l s w i t h p e r f o r a t e d end
s l a b s d i f f e r e d l i t t l e f r o m t h o s e o f t h e t e s t vesse l w i t h t h e s o l i d end
s l a b . The observed i n f l u e n c e o f v a r i o u s p a t t e r n s and s i z e s o f p e n e t r a -
t i o n s on t h e s t r e n g t h o f t h e end s l a b , t h e mechanism o f f a i l u r e , and
o v e r - a l l s t i f f n e s s was s m a l l i n r e l a t i o n t o t h e p r o p o r t i o n o f t h e s l a b
c r o s s s e c t i o n removed. A g e n e r a l p e r s p e c t i v e o f t h e t e s t r e s u l t s b e h a v i o r
may be o b t a i n e d f r o m a c o m p a r i s i o n o f t h e p r e s s u r e - d e f l e c t i o n c u r v e s i n
F i g . 2 w i t h t h e h e l p o f t h e i n f o r m a t i o n i n F i g . 1 .
A l l s i x v e s s e l s f a i l e d i n shear as a d i r e c t r e s u l t o f t h e
o f i n c l i n e d c r a c k s , I n ' t w o cases (PV18 and PV19) t h e sea l f a i
t h e s t r u c t u r a l mechanism was comple ted . The o t h e r f o u r f a i l e d
Crack Development
deve 1 opment
e d b e f o r e
e x p l os i v e l y .
The p e n e t r a t i o n s i n t h e end s l a b p e r m i t t e d t h e measurement o f s t r a i n s
a t v a r i o u s l e v e l s i n t h e end s l a b . D e s p i t e t h e f a c t t h a t t h e s e s t r a i n s
do n o t r e p r e s e n t average d e f o r m a t i o n c o n d i t i o n s a t a g i v e n l e v e l , t h e y do
p r o v i d e a v e h i c l e fo r examin ing i n t e r n a l s t r a i n s l e a d i n g t o c r a c k i n g .
Ev idence d i s c u s s e d i n r e f e r e n c e 1 i m p l i e d t h a t i n c l i n e d c r a c k s i n
t h e end s l a b formed i n i t i a l l y a t a p p r o x i m a t e l y m i d - h e i g h t and t h e n p r o -
pagated toward b o t h su r faces ' o f t h e s l a b .
w i t h t h e h e l p o f s t r a i n measurements made i n a p a r t i c u l a r t e s t v e s s e l ,
P V l 7 .
T h i s i m p l i c a t i o n can be checked
S t r a i n s were measured on t h e w a l l s o f t h e p e n e t r a t i o n i n v e s s e l P V 1 7
a t l e v e l s A , 6 , and C as shown i n F i g . 4. A s e t o f i n d i v i d u a l s t r a i n
measurements a t l e v e l B , near t h e m id -dep th o f t h e end s l a b , i s shown i n
F i g . 4. The s t r a i n s v a r i e d smooth ly and v i r t u a l l y a t a l i n e a r r a t e w i t h
i n t e r n a l p r e s s u r e up t o 1500 p s i . A t p r e s s u r e s above 1500 p s i , some gages
i n d i c a t e d r e v e r s a l s and some gave e r r a t i c r e a d i n g s , i n d i c a t i n g t h e d e v e l o p -
ment o f a s t r a i n d i s t r u b a n c e a t or near l e v e l B . 63
390
F i g u r e 5 i s a r e p r e s e n t a t i o n i n p o l a r c o o r d i n a t e s o f s t r a i n s a t
l e v e l s A , B , and C i n v e s s e l P V 1 7 . S t r a i n s a r e p l o t t e d w i t h r e f e r e n c e t o
t h e o r i g i n . The r a d i i i n d i c a t e magn i tudes arid t h e ang les w i t h t h e h o r i -
z o n t a l a x i s indic;:e o r i e n t a t i o n s t o t h e r a d i a l ( r - e ) p l a n e : a s t r a i n
p l o t t e d a l o n g t h e h c r i z o n t a l a x i s r e p r e s e n t s a r a d i a l s t r a i n w h i l e a
s t r a i n p l o t t e d a l o n g t h e v e r t i c a l a x i s r e p r e s e n t s a v e r t i c a l s t r a i n .
The s o l i d c u r v e s r e f e r t o measured s t r a i n s a t a g i v e n l e v e l d e r i v e d
f r o m t h e averages o f t h e s t r a i n measured i n t h r e e d i r e c t i o n s . The b roken
c u r v e s i n d i c a t e t h e e s t i m a t e d c r a c k i n g s t r a i n , o r t h e sum o f t h e c a l c u -
l a t e d s t r a : . i d u s e d by t h e p r e s t r e s s and a s t r a i n o f 3 0 ~ 1 0 ~ ~ assumed a s
a reasonab le upper bound t o t h e c r a c k i n g s t r a i n f o r c o n c r e t e . The cu rves
f o r t h e measured s t r a i n and c r a c k i n g c a p a c i t y s h o u l d be more p r o p e r l y
t r e a t e d as bands r a t h e r t h a n l i n e s because o f t h e expec ted s c a t t e r .
Comparison o f t h e s o l i d c u r v e s w i t h t h e b roken c u r v e s p r o v i d e
i n f o r m a t i o n on t h e l i k e l i h o o d and o r i e n t a t i o n o f c r a c k i n g a t v a r i o u s
l e v e l s i n t h e end s l a b . The c u r v e s i n F i g . 5 i n d i c a t e t h a t t h e l i k e l i -
hood o f c r a c k i n g was sma l l a t an i n t e r n a l p r e s s u r e o f 1000 p s i . A t
1500 p s i , i t appears t h a t c r a c k i n g was most l i k e l y a t l e v e l B and wou ld
f o r m a t an a n g l e o f a p p r o x i m a t e l y 45 w i t h thl3 h o r i z o n t a l . The obse rva -
t i o n t h a t t h e i n c l i n e d c r a c k was l i k e l y t o s t a r t a t m i d h e i g h t a t an
i n t e r n a l p r e s s u r e of 1500 p s i c o n f i r m s t h e i n l j i c a t i o n s o f i n d i r e c t
ev idence f r o m o t h e r t e s t v e s s e l s wh ich deve loped i n c l i n e d c r a c k s .
0
Fa i 1 u r e Mechan i sm
The t h r e e m a j o r c r a c k systems, r a d i a l , i n c l i n e d , and r e e n t r a n t
c o r n e r c r a c k s , f o r m a t about t h e same p r e s s u r e l e v e l .
The i n i t i a l change i n s l o p e o f t h e p r e s s u r e - d e f l e c t i o n cu rves i n
F i g . 2 a t a p p r o x i m a t e l y 1500 p s i i s a t t r i b u t a b l e p r i m a r i l y t o c r a c k s a t
t h e r e e n t r a n t c o r n e r between t h e s l a b and t h e s i d e w a l l and n o t t o t h e
development of t h e i n c l i n e d c r a c k s . R a d i a l c r a c k s on t h e o u t e r s u r f a c e
o f t h e s l a b formed as t h e p r e s s u r e was i n c r e a s e d above 1500 p s i . I n d i r e c t
ev idence i n d i c a t e s t h a t t h e i n c l i n e d c r a c k s when t h e y began t o p ropaga te ,
391
0 d i d so
PV18). A t pressures above 3000 p s i , t h e moment on t h e wedge shaped
s e c t o r s of t h e end s l a b , bounded by t h e r a d i a l c racks , tends t o overcome
t h e "clamping" moment on these s e c t o r s e x e r t e d by t h e p r e s t r e s s i n g f o r c e s .
Consequent ly, another change i n s l o p e occurs. The r o t a t i o n o f t hese
s e c t o r s about t h e edge o f t h e t e s t vessel would l e a d t o a f l e x u r a l f a i l u r e
b u t s t r e s s e s i n t h e i n v e r t e d dome caused a f a i l u r e i n shear a t a pressure
and d e f l e c t i o n lower than those t h a t would have been developed as a r e s u l t
o f f l e x u r a l f a i l u r e .
r a p i d l y , c a r v i n g an " i n v e r t e d dome" ou t o f t h e end s l a b ( F i g . 3 ,
The " t y p i c a l " c h a r a c t e r i s t i c s o f a shear f a i l u r e i n a s o l i d end s l a b
can be i l l u s t r a t e d i n r e f e r e n c e t o t h e c r i t i c a l c r a c k t r a j e c t o r y i n vessel
P V 1 8 , F ig . 3 . The i n c l i n e d c rack formed a t an ang le o f app rox ima te l y 45 t o t h e h o r i z o n t a l near t h e rnid-depth o f t h e end s l a b . As t h i s c r a c k
approached t h e p r e s s u r i z e d s u r f a c e , t h e r a d i a l compressive s t r e s s e s , as
w e l l as t h e shear and c i r c u m f e r e n t i a l s t r e s s e s , increased e i t h e r t o
d i r e c t t h e c r a c k t o a n e a r l y h o r i z o n t a l pa th o r t o cause f a i l u r e . The
c rack t r a j e c t o r y observed i n P V 1 8 and P V 1 9 i n d i c a t e s t h a t p e n e t r a t i o n s
d i d no t change t h i s p a t t e r n c r i t i c a l l y . The c r a c k t r a j e c t o r i e s shown f o r
vesse ls P V 1 7 , PV20, and P V 2 1 were r e c o n s t r u c t e d f r o m t h e d e b r i s a f t e r
e x p l o s i v e f a i l u r e s and do no t n e c e s s a r i l y i n d i c a t e t h a t t h e i n c ined
c r a c k had n o t extended beyond mid-depth a t t h e t i m e o f f a i l u r e . I t
appears q u i t e 1 i k e l y t h a t t h e f i n a l c o l l a p s e occu r red as a r e s u t o f
h i g h s t r e s s e s on a c i r c u m f e r e n t i a l s u r f a c e c o n t a i n i n g ' the p e n e t r a t i o n s ,
r a t h e r t h a n a t a p o i n t c l o s e r t o t h e p r e s s u r i z e d s u r f a c e as i n t h e case
o f P V 1 6 . A q u a n t i t a t i v e d i s c u s s i o n o f s t r e s s combinat ions i n t h e
" i n v e r t e d dome" carved by the i n c l i n e d cracks i s presented i n t h e nex t
chap te r .
0
STRESSES I N THE END SLAB AFTER DEVELOPMENT OF THE INCLINED CRACKS
The a v a i l a b l e exper imen ta l ev idence i n d i c a t e s ve ry s t r o n g l y t h a t
"shear" f a i l u r e s o f t h e end s l a b s t e s t e d was u l t i m a t e l y caused by t h e
m a t e r i a l f a i l u r e o f t h e conc re te under a complex s t a t e o f compressive
392
s t r e s s e s i n t h e t h r e e o r thogona l d i r e c t i o n s and shear s t resses i n t h e
r a d i a l - v e r t i c a l p lane. Assuming t h a t t h e shape o f t h e i n v e r t e d dome
carved by t h e i n c l i n e d c racks i s known, t o determine t h e f a i l u r e c a p a c i t y
o f t h e dome it i s necessary t o c a l c u l a t e a l l components o f t h e s t resses
i n a l l s e c t i o n s o f t h e dome and compare t h e r e s u l t i n g combinat ions w i t h
a f a i l u r e c r i t e r i o n which takes i n t o account p r o p e r l y t h e i n t e r r e l a t i o n -
s h i p between these s t r e s s e s . To make such a c a l c u l a t i o n w i t h any c la ims
t o c e r t a i n t y o r p r e c i s i o n i s impossib le w i t h i n t h e c o n t e x t o f a v a i l a b l e
knowledge. The f o l l o w i n g a n a l y s i s i s made p r i m a r i l y w i t h t h e o b j e c t i v e
o f i n v e s t i g a t i n g whether t h e e s t i m a t e d s t r e s s e s i n t h e end s l a b a t maxi-
mum pressure a re i n a range c o n s i s t e n t w i t h the observed s t r e n g t h o f
c o n c r e t e sub jec ted t o m u l t i - a x i a l s t resses . The a n a l y s i s i s made f o r a
s p e c i f i c t e s t vessel a t t h e maximum i n t e r n a l s t r e s s measured,
F i g u r e 6 shows o n e - h a l f o f a c ross s e c t i o n th rough t h e end s l a b
a f t e r an i d e a l i z e d i n c l i n e d c r a c k has carved ou t a complete i n v e r t e d
dome. The s t r e s s e s i n t h e dome a r e determined w i t h t h e f i n i t e - e l e m e n t
method, assuming t h e s l a b i s l i n e a r l y e l a s t i c , f o r an i n t e r n a l p ressu re
o f 3200 p s i . The v e r t i c a l and h o r i z o n t a l f o r c e s i n t h e re in fo rcemen t
a r e i n t roduced as i n d i c a t e d i n F ig . 6 and correspond t o va lues measured
i n vessel P V 1 6 a t u l t i m a t e p ressu re .
V a r i a t i o n s a l o n g t h e r a d i u s o f c a l c u l a t e d s t r e s s e s a t m idhe igh t o f
t h e dome s e c t i o n a re p l o t t e d i n F i g . 7 f o r t h e r a d i a l , t a n g e n t i a l , and
v e r t i c a l normal s t r e s s e s and t h e shear s t r e s s i n t h e r a d i a l - v e r t i c a l ~
p lane. D i s t r i b u t i o n s o f these s t r e s s e s over t h e depth o f t h e dome s e c t i o n
a t two d i f f e r e n t r a d i i a r e shown i n F i g . 8 .
C e r t a i n f e a t u r e s o f t h e c a l c u l a t e d s t r e s s d i s t r i b u t i o n s a r e notewor thy
w i t h a v iew t o simp1 i f y i n g t h e i n t e r p r e t a t i o n of t h e s t r e s s c o n d i t i o n s i n
t h e dome.
( 1 ) The f o r c e s r e s u l t i n g f rom t h e i n t e g r a t i o n o f t h e r a d i a l and
t a n g e n t i a l s t r e s s e s over t h e depth o f t h e dome s e c t i o n remain e s s e n t i a l l y
cons tan t a long t h e r a d i u s .
393
( 2 ) A t po in t s away f r o m t h e center o f the dome, the v a r i a t i o n o f
the r a d i a l s t ress over the depth o f the dome sec t i on i s smal l . 0
(3 comparab
cated by
(4 the v e r t
The shear s t ress a t the midheight o f the dome sec t i on i s
e t o both the nominal shear s t ress and the maximum value i n d i -
the f ine-element s o l u t i o n .
A t po in t s away from the center o f the dome, the v a r i a t i o n o f
ca l s t ress over the depth of t he dome sec t i on i s very smal l .
I n e f f e c t , the c r i t i c a l s t resses a t any rad ius could be considered
simply as the average r a d i a l s t r e s s , based on the r a d i a l f o rce obtained
by assuming a constant d i s t r i b u t i o n o f t angen t ia l f o rce along the rad ius ;
a shear s t ress equal to the nominal shear s t ress a t t h a t sec t i on ; and
the v e r t i c a l s t ress equal t o the pressure on the inner sur face o f the
dome.
The h igh r a d i a l and tangen t ia l s t resses near the center o f the dome
are extraneous t o the r e a l problem. So lu t ions o f the same dome w i t h lower
moduli f o r the concrete w i t h i n two i n . of center ind ica ted t h a t these
stresses would be reduced as a r e s u l t o f nonl inear response w i thout
a f f e c t i n g the stresses elsewhere c r i t i c a l l y . I n f a c t , t h i s p o r t i o n o f
the dome could be deleted w i thout c r i t i c a l e f f e c t on the s t resses i n
the dome.
A s s u m i n g t h a t Mohr's f a i l u r e c r i t e r i o n app l ied t o concrete under
combined s t resses, a f a i l u r e envelope can be const ructed us ing the
f o l l o w i n g in fo rmat ion : (a ) A Mohr 's c i r c l e represent ing the s t ress
c o n d i t i o n f o r the cy1 inder-sp l i t t i n g t e s t , (b) a Mohr's c i r c l e represent-
ing the s t ress c o n d i t i o n f o r t he u n i a x i a l compression t e s t , and ( c ) an
approximate slope f o r h igher values o f the p r i n c i p a l compressive s t ress
obta ined from the r e l a t i o n s h i p der ived by Richard e t a1 (Ref. 2 )
rJ1 = f ' t 4.1 m2 C
394
where c1 = a p p l i e d a x i a l s t r e s s i n t e r p r e t e d as t h e maximum p r i n c i p a l
s t r e s s ,
f ' = compressive s t r e n g t h o f t h e c o n c r e t e ,
D = c o n f i n i n g s t r e s s i n t e r p r e t e d as t h e minimum p r i n c i p a l s t r e s s .
The s t r e s s c o n d i t i o n s a t v a r i o u s l e v e l s f o r s e c t i o n s i n t h e dome a t
C
2
r a d i i o f 4.88 and 9.5 i n . f rom t h e dome c e n t e r a re shown i n F ig . 9. The comparison o f t h e Mohr ' s c i r c l e drawn f o r t h e s t r e s s c o n d i t i o n s and
t h e envelope suggest o n l y t h a t , a t t h e t i m e o f f a i l u r e pressure i n
vessel P V 1 6 , t h e magnitudes o f t he c a l c u l a t e d s t r e s s e s a re p l a u s i b l e
i n r e l a t i o n t o t h e i n f o r m a t i o n a v a i l a b l e about t h e s t r e n g t h c h a r a c t e r -
i s t i c s of conc re te under m u l t i a x i a l s t r e s s e s . I t a l s o appears converse ly
t h a t Mohr 's f a i l u r e t h e o r y can be used t o determine t h e s t r e n g t h o f t h e
end s lab . Th is c o n c l u s i o n a l s o promises a lead t o t h e e x p l a n a t i o n o f
t h e r e l a t i v e l y smal 1 v a r i a t i o n between t h e c l l t imate c a p a c i t i e s o f t h e
s l a b s w i t h and w i t h o u t p e n e t r a t i o n s f a i l i n g i n shear. The i n t r o d u c t i o n
o f a p e n e t r a t i o n would increase t h e r a d i a l and shear s t resses a t a p p r o x i -
ma te l y t h e same r a t e . Consequent ly, a l t h o u g h t h e shear s t resses would
i nc rease , so would t h e shear s t r e n g t h . Work i s c u r r e n t l y i n progress
toward t h e t e s t i n g o f t h i s hypo thes i s b o t h exper imen ta l l y and a n a l y t i c a l ly.
ANALYSIS OF STRESS C O N D I T I O N S LEADING TO INCLINED CRACKS
I n o r d e r t o p r o j e c t t h e r e s u l t s o f t h e exper imen ta l i n v e s t i g a t i o n
t o combinat ions o f v a r i a b l e s n o t d i r e c t l y covered i n t h e t e s t s , it i s
necessary t o develop a r a t i o n a l method f o r p r e d i c t i n g t h e c r a c k t r a j e c t o -
r i e s as w e l l a s a n a l y z i n g t h e s t r e s s e s i n t h e end s l a b a f t e r t h e c racks
have formed. To t h i s end, t h e lumped-parameter method developed by
Echever r i a and Schnobr ich (Ref. 3 ) ' i s be ing extended t o p r e d i c t t h e
t r a j e c t o r i e s o f i n c l i n e d c racks . A n a l y s i s of p o s s i b l e c r a c k f o r m a t i o n s
i n vessel P V 1 6 u s i n g t h e lumped-parameter mode1 w i t h a 1 i m i t i n g - s t r a i n
c r i t e r i o n f o r t e n s i l e f a i l u r e o f t h e concret:e i s shown i n F i g . 10. I n
a d d i t i o n t o t h e r a d i a l and t a n g e n t i a l c racks a t t r i b u t a b l e p r i m a r i l y t o
f l e x u r a l s t r e s s e s , t h e a n a l y s i s p r e d i c t s i n c l i n e d o r c o n i c a l cracks a t
app rox ima te l y 45 which f l a t t e n as t h e y approach t h e p r e s s u r i z e d su r face . 0
39 5
S UMMAR Y
The t e s t da ta f rom t h e s i x p res t ressed conc re te p ressu re vesse ls
i n d i c a t e no s i g n i f i c a n t r e d u c t i o n i n s t r e n g t h as a r e s u l t o f pene-
t r a t i o n s th rough t h e Clead. Three major c rack systems develop i n t h e
head d u r i n g p ressu re l oad ing . These i n v o l v e r a d i a l c racks beg inn ing
a t t h e t o p cen te r o f t h e head, i n c l i n e d c racks o r i g i n a t i n g a t mid-
dep th on a f o r t y - f i v e degree l i n e f rom t h e end anchorage down toward
t h e c e n t e r o t t h e v e s s e l , and c o n i c a l cracks a t t h e r e e n t r a n t co rne r .
These c racks change t h e f l a t head o f t h e vessel s t r u c t u r a l l y t o t h a t
o f an i n v e r t e d dome. A Mohr’s c i r c l e f a i l u r e c r i t e r i o n seems p l a u s i b l e
f o r p r e d i c t i n g t h e s t r e n g t h o f t h i s i n v e r t e d dome. An e x p l a n a t i o n f o r
t h e l a c k o f e f f e c t o f p e n e t r a t i o n s on t h e s t r e n g t h i s , t h a t these
p e n e t r a t i o n s increase t h e shear and r a d i a l s t r e s s e s i n t h e same
p r o p o r t i o n , t hus i n c r e a s i n g t h e s t r e n g t h c h a r a c t e r i s t i c s o f t h e
c o n c r e t e as we1 1 . ACKNOWLEDGEMENTS
The work r e p o r t e d i n t h i s paper was c a r r i e d ou t a t t h e S t r u c t u r a l
Research Labora to ry o f t h e C i v i l Eng ineer ing Department, U n i v e r s i t y o f
I l l i n o i s , Urbana as a p a r t o f t h e P res t ressed Concrete Reactor Vessel
Program o f t h e Oak Ridge N a t i o n a l L a b o r a t o r y , sponsored by t h e U.S.
Atomic Energy Commission. The program i s c o o r d i n a t e d by G . D. Whitman
o f t h e Oak Ridge N a t i o n a l Labora to ry .
The i n v a l u a b l e h e l p o f B. Mohraz, A s s i s t a n t P ro fesso r o f C i v i l
Eng ineer ing and R . Higashionna and B. Ka r l sson , Research A s s i s t a n t s
i n C i v i l Eng ineer ing a t t h e U n i v e r s i t y o f I l l i n o i s , i s g r a t e f u l l y
acknowledged.
396
REFERENCES
1 . S . L. Paul e t a l , "St rength and Behavior o f Prest ressed Concrete Vessels f o r Nuclear Reactors , ' ' C i v i l Eng ineer ing Stud ies , S t r u c t u r a l Research Ser ies No. 346, U n i v e r s i t y o f I l l i n o i s , Urbana, J u l y 1969.
2. F. E . R ichard, Anton Brandtzaeg'and R . L. Brown, "A Study o f t h e F a i l u r e o f Concrete Under Combined Compressive Stresses," U n i v e r s i t y of I l l i n o i s Eng ineer ing Experiment S t a t i o n B u l l e t i n No. 185, Urbana, 1928.
3 . G . A . Echever r ia and W . C . Schnobr ich, "Lumped-Parameter A n a l y s i s o f C y l i n d r i c a l Prest ressed Concrete Reactor Vessels," C i v i l Engineer ing Stud ies , S t r u c t u r a l Research Ser ies No. 340, U n i v e r s i t y o f I l l i n o i s , Urbana, December 1968.
Table 1
Circurn. P r e s t r e s s Long. P r e s t r e s s Concrete P r e s t r e s s Indec Maximum
Re ached Mark Force pe r Wi re T o t a l Force Comp. S t r e n g t h Tens. S t r e n g t h Circurn'? Long. Pressure
k i p s K i p s p s i ps i p s i ps i p s i
P V I ~ 6.03 1995 745 0 518 1930 4060 3200
P V I 7 6.33 2080 7180 534 2030 4240 3000
pv18 5.94 1818 7590 447 1900 3700 3000
PV19 5.85 23 00 7470 406 1870 4690 3500
P V 2 0 5.77 2140 6890 469 1850 4360 3300
PV21 5.65 23 00 7400 496 1810 4700 3300
a R a t i o o f t o t a l c i r c u m f e r e n t i a l p r e s t r e s s i n g f o r c e per u n i t h e i g h t o f vesse l t o t h e i n t e r n a l d iamete r .
b R a t i o o f t o t a l h o r i z o n t a l p r e s t r e s s i n g f o r c e t o a rea of cav i t . y a t a t r a n s v e r s e s e c t i o n .
397
0 75" Diameter Stressteel Rods
Bonded Reinforcement 4 0 # 4 Bars on 38" Diameter
( 0 ) Cross Section
4 Prestressing at 025" Spacing
( b ) End Slab Penetrations
FIG. I TEST VESSELS
I I I I I I I .-
DEFLECTION AT CENTER OF END SLAB
FIG. 2 PRESSURE-DEFLECTION CURVES
PV 17 PV 18 PV 16
PV 19 PV 20 PV 21
F IG .3 CRACKS LEADING TO FAILURE
LEVEL A LEVEL B LEVEL C
1/2"
FIG. 4 STRAINS MEASURED AT LEVEL B , TEST VESSEL PV 17 STRAIN x lo5
FIG. 5 STRAINS AT VARIOUS LEVELS IN THE END SLAB OF PV17 IN POLAR COORDINATES
6200 psi -1300 psi
,4900 psi -
p t t t t t t t t t ;. 1 3200 psi
- i 1700 psi
-
IO"
-
4 \REENTRANT CORNER 12.5" CRACK
FIG. 6 SECTION OF IDEALIZED INVERTED DOME
-
RADIAL STRESS ur -
STRESSES AT MID-HEIGHT - -
RADIAL DISTANCE IN INCHES FIG. 7 VARIATION OF CALCULATED STRESSES ALONG THE RADIUS
OF THE DOME
4.2 ksi
X
3.25 ksi
/' & FAILURE SURFACE
2 4 6 8 IO
DISTANCE UP F INSIDE FACE IN
u ( k s i )
( b ) SECTION AT R . 9 5 "
FIG. 8 VARIATION OF THE CALCULATED STRESSES OVER THE DEPTH OF THE DOME
'ROM INCHES
STRESS AT R=4.88"
/'
( a ) SECTION AT R = 4.88
DISTANCE FROM FACE IN INCHES
INSIDE
STRESS AT R = 9.5"
FIG. 9 ESTIMATED STRESS CONDITIONS AT FAILURE OF VESSEL PV16
401
DISPLACEMENT NODES
TRESS NODES
AXIS OF 12.5" - - - 7.5"
SYMMETRY LUMPED PARAMETEL MODEL
- TRACE OF CONICALP CRACKS -re AREA COVERED BY
h\\\y RADIAL CRACKS
CRACK PATTERN
FIG. IO CRACK TRAJECTORIES PREDICTED BY THE LUMPED-PARAMETER ANALYSIS IN VESSEL PV16
402
DISCUSSION
G . 3 . Whitman: The absence of c r o s s head t endor s i n t h e t o p head
does not n e c e s s a r i l y impair t h e s t r e n g t h of t h e head s i n c e t h e circum-
f e r e n t i a l tendons induce t h e p r e s t r e s s i n g f o r c e s r equ i r ed t o achieve
s t a b i l i t y a g a i n s t i n t e r n a l p re s su re loads .
Paper 5/108
J. P. Callahan1 J. M. c o r n 1 G. D. Whitmanl
ABSTRACT
The ef fec ts of the thermal conditions imposed on a prestressed concrete reactor vessel (PCRV) present a major uncertainty i n predicting long-term vessel behavior. search and development programs a r e under way t o provide adequate analyt ical methods f o r predicting long-term be- havior and t o provide the basic materials data needed t o effect ively u t i l i z e such methods. however, t h a t ult imately the va l id i ty of the analyt ical methods and materials data obtained from small specimens must be demonstrated by designing, analyzing, and tes t ing a r e a l i s t i c a l l y s ized and shaped structu?.x under conditions similar t o those i n an actual vessel.
Re-
It i s generally agreed,
Thus, a thermal cylinder model, which simulates a portion of the barrel section of a cyl indrical vessel i s being b u i l t and w i l l be tes ted a t Oak Ridge National Laboratory. The thick-walled cylinder specimen i s 48 in . high, 18 in. thick, and 81 in. OD; it w i l l be made of the same material as used i n the basic t e s t s , and it w i l l be sealed t o prevent moisture lo s s i n the same manner as the basic specimens. The model i s prestressed ax ia l ly and circumferentially, and provision i s made f o r applying an in te rna l pressure loading and a temperature prof i le simu- l a t ing thermal conditions i n an operating PCRV. men w i l l be subjected t o mechanical and thermal loading h i s to r i e s that simulate, on a compressed t i m e scale, the loading h is tor ies that an actual vessel m i g h t experience during the first few years of operation. Near the end of the t e s t the specimen w i l l be subjected t o off-design hot spot conditions t o obtain information on the capabi l i ty of the s t ructure t o endure prolonged accidental over- temperatures. s t ress , s t ra in , temperature, and moisture leve ls a t se- lected locations.
The speci-
The model w i l l be instrumented t o measure
* Research sponsored by the U. S. Atomic Ehergy Commission i n sup-
port of Prestressed Concrete Technology under contract with the Union Carbide Corporation.
lReactor Division, O a k Ridge National Laboratory.
403
404
This paper b r i e f l y discusses the basic materials invest igat ions t h a t are being car r ied out and presents some i n i t i a l results and trends. Tlne thermal cylinder t e s t i s then described and r e s u l t s :From the preliminary design creep analysis of t h e tes t specimen are presented.
INTRODtTC T I O N
The s ingle most important f ac to r making prestressed concrete reactor
vessels (PCRV's) unique i n the technology of prestressed concrete i s the
long-term thermal condition imposed on the s1;ructure by the r e l a t ive ly
high-temperature reac tor process f l u i d . In present vessels, a complex
system of insulat ion and cooling i s provided t o l i m i t maximum concrete
temperature t o 200aF or less, but the long-term behavior of the vessels
can be s ign i f i can t ly a f fec ted by temperatures of even t h i s r e l a t ive ly low
l eve l . Over the 30-year design l i f e of a concrete vessel , these thermal
e f fec ts present a major uncertainty with regard t o understanding and
accurately predict ing long-term vessel behavior and margins of safety.
The f ac to r s t h a t a r e of primary concern t o the vessel designer are
thermal stresses, concrete creep and shrinkage, and changes i n the mechani-
c a l and physical concrete propert ies with time. Each of these f ac to r s i s
dependent on temperature and moisture l e v e l s and/or d i s t r ibu t ions , and
these are, i n turn, i n t e r r e l a t ed i n a complicated way. Creep and shrink-
age can have se-rious consequences f o r a concrete vessel because of the
l o s s of i n i t i a l p res t ress , because of possible l a rge deformations of the
vessel resul t ing, f o r example, i n misalignment of cont ro l rod and fue l ing
passages, and because of res idual s t r e s ses t h a t may be introduced as t h e
loading conditions change. I n t he l a t t e r case, t he res idua l stresses could conceivably be t e n s i l e stresses and could be coupled with i n f e r i o r
concrete s t rength propert ies , which may have come about over a period of
time, resu l t ing i n serious damage t o the vess2l.
In 1965, the Oak Ridge National Laboratory w a s asked by the United
S ta tes Atomic Energy Commission t o formulate i2nd d i r e c t a long-range
basic research and development program t h a t supports the technology of
405
prestressed concrete vessels f o r nuclear reactors . t h i s program1j2 has been aimed a t the problems described above. A two-
pronged approach is being followed t o provide vessel designers with the
information and too l s needed t o understand and predic t long-term vessel
behavior. On the one hand, basic materials invest igat ions are under way t o provide mult iaxial concrete creep data a t room and elevated temperatures f o r t yp ica l concrete mixes; moisture d i s t r ibu t ion tests on small simulated
vessel segments are being performed; physical and mechanical propert ies data are being obtained t o character ize the concrete mixes used; and the
e f f e c t s of sustained and cyc l ic elevated temperatures on these concretes are being studied. These invest igat ions, i n which, f o r the most p a r t , individual var iables are being investigated using small specimens, were formulated t o provide much of the bas i c information necessary t o separate the various in t e r r e l a t ed e f f e c t s associated with long-term vessel behavior.
A major port ion of
The second p a r t of the ove ra l l approach i s the development of complex
ana ly t i ca l methods f o r predict ing the creep, cracking, and ultimate
s t rength behavior of concrete vessels . Hopefully, t he basic mater ia ls data can be u t i l i z e d together with these ana ly t i ca l methods t o cor rec t ly pred ic t the long-term in t e r r e l a t ed e f f ec t s on a concrete vessel . However, t o u l t imate ly demonstrate t he v a l i d i t y and accuracy of the ana ly t i ca l techniques and basic materials data, a r e a l i s t i c a l l y shaped s t ruc ture must be designed, analyzed using the newly developed techniques and data, and subjected t o test conditions simulating those i n an ac tua l vessel .
To meet t h i s need, a r e l a t ive ly s m a l l thermal cyl inder t es t s t ruc ture i s being b u i l t and will be t e s t ed a t ORNL. walled cylinder 48 in . high, 18 i n . thick, and 81 in . OD, and it repre- sen ts a segment out of the cy l ind r i ca l port ion of a cy l indr ica l concrete
The tes t specimen i s a th ick-
vessel as shown i n Fig. 1. The specimen w i l l be subjected t o prestressing, i n t e r n a l pressure, and thermal loading h i s t o r i e s tha t simulate, on a com-
pressed t i m e scale , t h e loading h i s t o r i e s that an ac tua l vessel might experience during the f irst f e w years of operation. Near the end of the test, t he specimen w i l l be subjected t o off-design hot spot conditions t o evaluate the capabi l i ty of the s t ruc ture t o endure accidental over-
temperature conditions.
406
ORNL-CJWG 70-3135
,,,-THERMAL INSULATION
THERMAL CYLINDER TEST SPECIMEN
PRESTRESSED CONCRETE REACTOR VESSEL
Fig. 1. Thermal Cylinder Test Specjmen Relationship t o Pres t ressed Concrete Reactor Vessel.
Table 1. Unconfined Compression 'Test Results
~~
2 8 - h y cure 9 0 - h ~ CUE - U l t i m a t e E l a s t i c Poisson, Ultimate
Strength
Curing Condition Elastic Poisson's Modulus Ratio Strength Nidulus
(lo6 p s i ) ( p s i ) (@ p s i ) ( p s i 1 Ratio
Immersed 5.4 0.24 6460 6 . 1 0.26 8310
A s c a s t 5.6 0.26 6010 6.3 0.26 6870
A i r dry 5.3 0.26 6590 6.0 0.26 7560
407
The specimen w i l l be extensively instrumented t o measure s t r a i n s , stresses, temperatures, and moisture l eve l s with t i m e . The concrete used f o r the specimen w i l l be the same as tha t used i n the bas ic materials
invest igat ions, and a l l surfaces of the tes t s t ruc tu re will be sealed t o duplicate t h e moisture condition of t h e sealed specimens i n the basic
s tudies . Thus the basic materials data can be used i n conjunction with
i n e l a s t i c time-dependent s t r u c t u r a l analysis techniques t o pred ic t the
time-dependent behavior of t he test s t ruc ture .
techniques used w i l l t h e n be evaluated by comparing t h e predict ions with the t e s t results.
The accuracy of t h e
The following sect ion of th i s paper b r i e f l y discusses the basic materials invest igat ions t h a t are being car r ied out . Some i n i t i a l r e su l t s and t rends are discussed. The thermal cylinder t es t i s then described
and discussed i n the t h i r d sect ion and typ ica l r e s u l t s from the prelimi- nary design creep analysis are presented. Finally, the last sect ion contains a brief summary and discussion of the ove ra l l integrated study.
MATERIALS INVESTIGATIONS
A concrete mixture w a s selected t o represent what might be used i n a PCRV i n most sections of the United S ta tes . The mixture i s composed
of a 3/4-in. maximum s i ze Tennessee limestone aggregate and Type I1 Portland cement. The mixture w a s designed and specified by the Waterways Experiment Stat ion
of t he Corps of Engineers, Department of the Army, Vicksburg, Mississippi. This concrete has been used i n a l l the bas ic materials invest igat ions and
i s specif ied f o r the thermal cylinder experiment.
Its design 28-day compressive s t rength i s 6000 ps i .
The following materials invest igat ions are being conducted by the respective organizations i n order t o completely characterize the PCRV concrete :
1. Basic mechanical and physical Oak Ridge National Laboratory propert ies
2. Strength propert ies Oak Ridge National Laboratory and University of California, Berkeley
408
3. Creep f o r mult iaxial loadings University of Texas and Wat e rmys Expe riment Stat ion
4. Moisture movement Waterways Experiment Stat ion
Basic Mechanical and Physica:L Properties
With the exception of the moisture movement study, a l l t e s t s a r e
being conducted using r e l a t ive ly s m a l l cy l indr ica l specimens representing
three curing conditions - a i r dr ied, sealed a t the t i m e of cast ing ( a s
c a s t ) , and moist cured (immersed).
t ies and ult imate s t rengths a r e l i s t e d i n Table 1 f o r these three curing
conditions.
The bas ic measured mechanical proper-
The basic physical propert ies t h a t have been measured f o r the PCRV
concrete are the coef f ic ien t of thermal expeasion, thermal conductivity,
thermal d i f fus iv i ty , and spec i f ic heat.
Thermal length change measurements were made f o r both air-drying
and as-cast conditions as follows:
Specimen
A i r dr ied
A i r d r ied
A i r dr ied
A s ca s t
Temperature Range
73°F - 210°F 210°F - 333°F
73°F - 333°F 8 0 " ~ - 147°F
a( i n . / i n . / OF)
4.3 x 0.6 x io-6 2.3 x 3.7 x
It can be seen t h a t a i r -drying specimens experience a d r a s t i c change i n
the observed coeff ic ient of thermal expansion as the concrete i s heated
above the boi l ing point s ince shrinkage e f f e c t s a r e presumed t o pre-
dominate i n t h i s temperature regime.
Thermal conductivity tests were conducted only on air-drying speci-
mens. w a s measured.
cast ing w a s 1.25 Btu/ft-hr-"F.
1 .12 Btu/ft-hr-OF i n 220 days.
sens i t ive t o temperature changes below 250°F.
A sharp i n i t i a l decrease i n thermal conductivity with moisture loss The value of thermal conductivity measured a t 28 days from
The specimen reached a constant value of
Thermal conductivity was not found t o be
The thermal d i f f u s i v i t y of a i r -dr ied coricrete was found t o be 0.0274
f t2 /hr , and the spec i f ic heat was 0.274 Btu/I.b-OF.
409
Strength Propert ies
The average unconfined compressive s t rengths of 6 in . by 12 in .
cylinders subjected t o a l l three curing conditions are p lo t ted i n Fig. 2.
Since t h e a i r -dr ied specimens f o r these pa r t i cu la r tests were moist cured f o r seven days p r i o r t o a i r drying, t h e i r i n i t i a l r a t e of s t rength gain
was subs tan t ia l ly higher than the as-cast specimens which were sealed i n
epoxy and soldered copper two days a f t e r casting. days t h e sealed as-cast specimens continued t o gain s t rength while the
air -drying cylinders experienced v i r t u a l l y no fu r the r increase i n s t rength, as shown i n the f igure. Heating the as -cas t specimens t o 150°F a t the
end of t h e i r 7-day curing period resul ted i n increased s t rength gain a t
6-months age, but t h e i r 1-year s t rengths were l e s s than those of the
sealed specimens remaining a t 75°F. Heating the air-drying specimens
caused a slight decrease i n t h e i r 6-month and 1-year s t rengths .
However, after 180
An extensive study i s under way a t the University of California t o
obtain as complete an account as possible of the mechanical behavior of
the PCRV concrete a f t e r various forms of thermal exposure. A major e f f o r t
i n the study has thus far been concentrated on the development of s t r a i n
instrumentation and seal ing techniques t o be used a t temperatures above
the boi l ing point of water. cy l indr ica l concrete specimens t h a t appears t o be sa t i s f ac to ry a t t e m - peratures up t o 300°F. E l e c t r i c blankets are used t o heat each specimen
individually.
gage t h a t i s constructed of a ha i rp in w i r e filament embedded i n compacted magnesium oxide powder which i s i n tu rn contained i n a sealed s t a i n l e s s
s teel tube. The ends of the tube are welded t o perforated s t e e l end
p l a t e s which serve t o anchor the gage i n the concrete.
A copper jacket has been developed f o r
S t ra ins are measured using the Microdot embedment strain
A p i l o t t es t of sealed 6 by 12-in. concrete cylinders containing
embedded Microdot gages has been completed. These specimens were cured
i n water a t 70°F f o r 28 days p r i o r t o sea l ing i n copper.
specimens were subjected t o one of t he following temperature conditions:
Individual
1.
2. Three cycles of 70-300-70"F and t e s t ed a t 7O0F,
Maintained a t 70°F (control specimen),
410
7.5
6 .O
.- Y 2 4.5 cn cn W
cn E 3.0
1.5
0
Fig. 2. Ultimate Unconfined Compressive Strength of PCRV Concrete for Various Ages and Moisture Conditions.
ORNL-DWG 70-4415
NO HEAT TREATMENT: -CONTROL SPECIMEN
------- --- -
0 300 600 900 1200 1500 1800 2100 2400 270C ST R A I N ( pin. 1' in . I
Fig. 3. Effect of Temperature on Stress-Strain Character- istics of Sealed PCRV Concrete.
411
3. Three cycles of 70-300-70"F and t e s t ed a t 300°F, 4. Heated continuously a t 300°F and t e s t ed a t 300°F.
The s t r e s s - s t r a in curves of specimens subjected t o t h e f i r s t three
temperature conditions are shown i n Fig. 3. The s t r e s s - s t r a in curve f o r
the specimen continuously heated a t 300°F w a s almost i den t i ca l t o the thermal cycled specimen t e s t ed a t 300°F.
and f u r t h e r t e s t i n g is cur ren t ly under way.
These a re preliminary r e su l t s
Creep Under Multiaxial Loadings
The creep t e s t i n g program consis ts of uniaxial , b iax ia l , and tri- a x i a l s t r e s s ing of specimens both a t room temperature and a t 150°F.
Cylindrical concrete specimens 6 i n . i n diameter and 16 in . long a r e being
t e s t ed as shown i n Fig. 4. Two specimens are subjected t o the same a x i a l
load i n each load frame; however, t h e i r l a t e r a l loading can be d i f f e ren t .
The majority of the specimens were loaded 90 days after cast ing.
nations of load, temperature, and moisture conditions included i n the
program a r e summarized i n Fig. 5 . The air-drying specimens were sealed
i n epoxy and soldered copper j u s t p r i o r t o loading a t 90 days.
Combi-
S t r a in instrumentation consisted of vibrat ing w i r e concrete embedment
s t r a i n gages cas t i n t o each specimen i n both the a x i a l and lateral d i rec-
t i ons as shown i n Fig. 4.
In addi t ion t o creep specimens, i den t i ca l f r e e shrinkage specimens
were included f o r each temperature and moisture condition. After the
creep specimens have been unloaded, creep recovery measurement w i l l be
made.
Some preliminary results from the creep tests being conducted by
the University of Texas are shown i n Fig. 6. the a x i a l s t r a i n measured with time f o r several representative loading
conditions both a t 75OF and l5O"F. Figure 6(b) consis ts of r a d i a l o r
l a t e r a l s t r a i n measurements w i t h time f o r the same loading conditions
and temperatures shown i n the first p lo t .
f o r every combination of loading the higher temperature resul ted i n
s ign i f i can t ly higher creep. A preliminary value of creep Poisson's r a t i o
Figure 6(a) shows p l o t s of
It should be pointed out t h a t
@
6-in. DlAM II
STEEL BALL-
OIL-
STEEL PRESSURE JACKET-
9 S T E E L PACKING RING-
0- RING - R A M -
I U
ai- * Os
F i g . 5 . Conditions for T r i a x i a l Creep T e s t s .
A STRESSES TO BE EMPLOYED IN ROOM ROOM TE:MI? AND ELEVATED TEMI? TESTS.
TEMPERATURE TESTS.
41 3
0 f o r t he as -cas t specimens i s 0.17 f o r 150°F and 0.12 f o r 75°F. par t i cu la r values are s ign i f i can t ly lower than the room temperature e l a s t i c Poisson's r a t i o s of 0.26 shown i n Table 1. The creep tests a r e s t i l l i n progress and these results should be considered t o be only pre- liminary i n nature.
These
Mo i s ture Movement Experiment
Shrinkage, creep, and s t rength of concrete a re a f fec ted by moisture In order t o evaluate these content and changes i n the moisture content.
e f fec ts , a pie-shaped specimen 9 f t long, 2 f t deep, and end widths of 2 f t and 2 f t 8 /in. simulating a moisture stream tube out of the cy l indr i - c a l wal l of a PCRV i s being tes ted . and soldered copper on the la teral surfaces and the simulated i n t e r i o r vessel face. r e l a t i v e humidity. thermal gradient can be imposed on the block.
The specimen w a s sealed with epoxy
The open end i s exposed t o the atmosphere a t 70°F and 50% Heaters and insulat ions were provided so tha t a
The hea ters were a l so used t o simulate the thermal conditions that would ex is t i n an i n f i n i t e l y long cy l indr ica l vessel sect ion by applying heat and maintaining a very s m a l l
temperature difference i n an equivalent circumferential plane during the
i n i t i a l unheated period. Carlson s t r a i n meters, thermocouples, and moisture measuring devices were cas t i n to the concrete.
t u r e content i s measured by a nuclear moisture meter, and a measure of the free water i n terms of changes of the d i e l e c t r i c propert ies of the concrete i s mde using open w i r e l i n e probes developed by Waterways Experiment Stat ion. provided f o r t h a t purpose.
The t o t a l mois-
Monfore humidity gages are also being used i n w e l l s
The moisture movement specimen remained i n unheated condition f o r
I 16 months. During t h i s t i m e t he moisture conditions i n the specimen re- mained r e l a t ive ly stable except i n the immediate v i c in i ty of the open
end. The temperature levels a t , v a r i o u s horizontal distances from t h e heated
end are shown i n N g . 7 f o r periods from 16 hours t o 17 days af ter the
i n i t i a t i o n of heating. t i n u a l concrete expansion since heating, with changes i n s t r a i n ranging
In March 1970, the sealed end of the specimen w a s heated t o 150°F.
The Carlson s t r a i n meters have indicated con-
@
414
160
140
t 20
1 00
80
60
40
800 , I I I ,
Fig. 6. Effect of Temperature, Moisture and Type of Multiaxial Loading on Creep of PCRV’Concrete.
ORNL-DWG 70-4444
0 10 20 30 40 50 60 70 80 90 400 110 DISTANCE FROM HEATED END ( in.)
Fig. 7. Moisture Migration Study Temperature Distribution a t the Center Line.
6d from 280 y in . / in . near the heated end t o p r a c t i c a l l y no change near unheated end. There appears t o be l i t t l e change thus far i n the mo
...
the s tu re
content of t he concrete since the i n i t i a t i o n of heating. The specimen i s scheduled t o continue t o be heated f o r a period of one year.
THERMAL CYLINDER TEST
The object ive of a thermal cylinder t es t i s t o simulate, as closely as possible, t he middle sect ion of the cy l ind r i ca l port ion of the vessel and the conditions imposed on it. The resu l t ing t e s t specimen i s shown, i n simplified form, on the r i g h t i n Fig. 1. The specimen is sealed a t top and bottom t o eliminate any moisture flow axia l ly , and t h e ends a re a l s o insulated thermally. confined pr imari ly t o the rad ia l d i rec t ion , simulating conditions near the middle of the ac tua l vessel . The specimen i s prestressed ax ia l ly and circumferentially, and an in t e rna l pressure can be applied t o the inner surface. The temperature d i s t r ibu t ion i s simulated by heating the inner surface and cooling the outer surface.
The moisture flow and heat flow would thus be
To cor rec t ly simulate t h e thermal gradient and the moisture gradient, t he thermal cylinder specimen should idea l ly be near the s i z e of an a c t u a l
vessel . t e s t specimen, t o provide a basis f o r evaluating the f e a s i b i l i t y and des i r ab i l i t y , as well as the cos t of performing a large-scale thermal test.3
A design study w a s car r ied out, based on a thick-walled cylinder
The specimen chosen w a s 15 f t 9 i n . high and 27 f t OD w i t h a w a l l
thickness of 6 f t . In addi t ion t o prestressing, the cyl inder w a s t o be subjected t o a thermal gradient and an in t e rna l pressure. It w a s t o be
t e s t ed f o r a period of three t o four years under combinations of condi-
t ions representat ive of an ac tua l PCRV.
tes t s t ruc ture and the necessary f a c i l i t i e s , instrumentation, and controls , ready f o r tes t ing , w a s .estimated t o be almost $1 mil l ion.
The t o t a l cost f o r providing the
Thus the design study showed that a large-scale thermal t e s t would be a la rge and very expensive undertaking. be e n t i r e l y dependent on the successful performance of various types of
Furthermore, i t s success would
@
416
embedded instruments whose performance had not been adequately demonstrate under the conditions t h a t would ex i s t . Consequently, a decision w a s made
t o proceed with a smaller thermal cylinder t e s t t o learn more about the behavior of such a specimen and the behavic,r of the necessary types of instrumentation. In addi t ion t o serving as a p i l o t t e s t , the small thermal cylinder tes t w i l l provide data t o meet many of the o r ig ina l objectives es tabl ished f o r t h e la rge thermal cylinder t e s t . moisture gradient could not be simulated cor rec t ly i n the small specimen, it w a s decided t o seal the specimen completely.
Since the
Specimen Description
The ac tua l de ta i led t e s t s t ruc ture i s (depicted i n Fig. 8. The thick- walled cylinder specimen i s 48 in . high, 18 i n . t h i ck , and 81 in . OD. The
design i s based on an in t e rna l pressure of '700 p s i and a normal temperature d i s t r ibu t ion ranging from 130°F on the inner surface t o 75°F on the outer surface. The ends are insulated thermally with loose mineral wool f i b e r
insulat ion a t the top and glass foam blocks a t the bottom.
The cylinder specimen i s prestressed i n the a x i a l and Circumferential d i rec t ions w i t h t he Stressteel-S.E.E.E. s t rand system. The arrangement f o r the circumferential p res t ress ing i s , however, unique i n the small
thermal cylinder. Basically, it consis ts of monostrand tendons wrapped around the outer surface of the cylinder and then tensioned by jacking
them rad ia l ly outward. This system has the advantage of moving the c i r - cumferential tendons out of the w a l l of the cylinder where they would
produce troublesome stress concentrations arid a l s o l i m i t the space avail-
able f o r embedded instrumentation. It a l s o has advantages over conven-
t i o n a l w i r e winding i n t h i s case because (1) it would be d i f f i c u l t t o
wind a cylinder of t h i s s i ze , which i s too la rge f o r a prestressed-concrete-
pipe winding machine and too small f o r conventional tank-winding equipment, and ( 2 ) t h i s lnethod of tensioning allows an accurate measurement t o be made of the tensioning forces ac tua l ly applied t o t h e wrapped tendons. The circumferential system i s a modification of an arrangement proposed
f o r prestressed-concrete reactor vessels by the engineering f i r m of Coyne and Bel l ier i n F r a n ~ e . ~ The anchoring arrangement f o r t h e tendons i n one
417 COOLiNG
WATER N
Fig. 8. Cutaway Drawing of Thermal Cylinder Test Structure .
. .I I 4
Fig. 9. Anchoring Arrangement for Monostrand Tendons i n a Circumferential P res t r e s s ing Band.
of the four circumferential
shown i n Fig. 9.
418
bands and a non'znchor bearing p l a t e are
A heat source i s provided on the inner face and a heat sink on the
outer face of t h e s m a l l cylinder i n order t o es tab l i sh the normal vesse l
temperature difference of 130 t o 75'F i n the cross section. Process water controlled a t the desired temperature w i l l be circulated f o r t h i s
purpose.
Plate- o r panel-type heat exchangers are provided on the inner and
outer surfaces of t he cylinder, t o one-half the flow cross sec t ion of a standard 3/8-in. pipe.
small cross sect ion w i l l permit t he establishment of a high heat t r ans fe r
coeff ic ient f o r flows comensurate with the low hea t t r ans fe r r a t e re-
quired. w a l l s , are spaced 1 l/S i n . apa r t around the circumference of the speci-
men.
The channel. configuration i s equivalent
This
The flow passages, which run v e r t i c a l l y up and down the cylinder
On the inner surface of t he specimen the embossed heat exchanger
panels are f i t t e d t o a 1/8- in . - thick mild s t e e l l i n e r , which simulates
the l i n e r i n an ac tua l PCRV. On the outer surface, the embossed panels
a r e f i t t e d t o a one-piece 22-gage s teel sheet . The embossed panels a r e a l s o made of 22-gage sheet . The hea t exchanger assemblies will serve as
the inner and outer formwork f o r the concretl? and as moisture sea l s on
the inner and outer surfaces. On the inner surface the assembly w i l l be
anchored t o the specimen by 1/4-in. -diam, 1 .L/2-in. -long standard-threaded
Nelson stored-arc studs.
The inner concrete core, o r island, i s provided i n connection with the
pressurizing scheme. The outer surface of the core i s f i t t e d with the same
1/8- in . s t e e l l i n e r and embossed hea t exchanger arrangement as the inner
surface of the specimen, and the two l i n e r assemblies are joined by
closures a t top and bottom consisting of s p l i t c i r cu la r tubes welded t o
the l i n e r assemblies. Thus a small-volume pressure annulus i s provided
f o r applying in t e rna l pressure t o the cylinder specimen. Hydraulic o i l w i l l be used as the pressurizing medium, w i t h the pressure supplied by
bot t led gas through an oil-expansion tank. The sp l i t -p ipe closure a t
419
the top of the pressurizat ion annulus i s provided with threaded connec- t i ons t o permit pressurizat ion and venting and t o provide f o r instrumenta- t i o n leads t o the annulus.
The heat source on the face of the core i s provided t o prevent heat t r ans fe r across t h e pressurizat ion annulus. It w i l l supply the heat
required during heatup and that required t o maintain a uniform core t e m -
perature on the inner surface of the tes t specimen. control po in ts f o r the core heat exchanger and t h e heat exchanger on the
inner surface of the specimen a re ident ica l , a sp l i t - f low arrangement i s
provided f o r the heating water, with the bulk of the flow t o be directed
through the specimen heat exchanger.
Since the temperature
Thin sheet metal sheeting is provided on the bottom of the cy l indr i -
c a l specimen and on the bottom of the center core t o serve as a part of
the formwork and as the bottom mo-isture seal. The top surfaces of the cylinder and core w i l l be coated w i t h l ayers of epoxy and copper f o i l soon after the cylinder and core are cas t . The epoxy-copper combination serves as the top moisture seal . In addi t ion, a l l sheet metal j o i n t s and j o i n t s i n t h e a x i a l tendon ducts w i l l be sealed w i t h epoxy.
P r io r t o casting, the composites of the l i n e r s , the panel c o i l heat exchanger assemblies, the bottom sheet metal surfaces, and the a x i a l tendon assemblies w i l l be assembled on the g lass foam insulat ion blocks, which i n tu rn w i l l be supported on a s t ruc tu ra l s tee l base frame t h a t
w i l l permit handling of the e n t i r e assembly w i t h the concrete i n place.
Tentative Test Schedule
A t en ta t ive t es t program and t i m e schedule f o r the s m a l l thermal
cylinder t e s t has been developed.
curement of the instrumentation and major components of the t e s t s t ruc ture i s complete. Approximately s i x months of addi t iona l time w i l l be required
before the specimen i s cas t . cas t , with temperatures, moisture leve ls , s t r a i n s , and s t r e s ses being
recorded w i t h t i m e .
Design of t he t es t s t ruc ture and pro-
The tes t will begin when the specimen i s
420
A t a concrete age of 90 days, which corresponds t o the age a t loading of the i n i t i a l creep specimens i n the materials invest igat ions,
the pres t ress ing operation will begin. It [is estimated tha t t he pre-
s t ress ing can be completed i n two t o three days.
A f t e r a one-month period during which only the prestressing loads
w i l l a c t on the t e s t specimen, t h e heat ing phase w i l l begin. The design
temperature gradient will be applied by r a i s ing the temperature of the
inner surface of the cylinder from 75 t o 150°F a t a rate of 5°F per day. The outer surface w i l l be maintained a t 75°F. Following completion of
the heating phase, a period of 90 days w i l l pass during which only the
pres t ress ing plus the thermal gradient w i l l be acting.
t h i s period, the in t e rna l pressure of TOO p s i w i l l be added f o r a period
of 180 days.
A t the end of
Following the r e l a t ive ly long-term pressure t es t period, the pressure
w i l l be removed f o r 45 days and then possib1.y reapplied f o r 45 days t o study creep recovery and residual stress e f f ec t s .
For the f i n a l port ion of t he t es t , it i s ten ta t ive ly planned t o hea t
a narrow circumferential band on the inner furface of the specimen t o a temperature of 450°F f o r a period of 90 days and t o then br ing the t e m - perature of the band quickly back t o normal. The purpose of t h i s "hot-
spot" t e s t w i l l be t o evaluate the p o s s i b i l i t y of a prolonged accidental over-temperature resu l t ing i n concrete cracking when the temperature i s lowered. To apply the l o c a l over-temperature, a spec ia l heating cable,
not shown i n Fig. 8, w i l l be wrapped circumferentially around the inner
surface of t h e cylinder p r i o r t o cast ing.
Preliminary Design Analysis
To ver i fy the adequacy of t he design, a preliminary t rans ien t thermal
analysis and a time-dependent f i n i t e element creep ana lys i s were performed.
The creep analysis was used t o pred ic t the stress and s t r a i n behavior of
the specimen s t a r t i n g with the i n i t i a l p res t ress ing and extending through
the 45-day period during which the in t e rna l pressure was removed.
421
In a c t u a l vessel p rac t ice the temperature gradient i s applied a t a
rate of 1°F per day, o r less, w i t h the expectation t h a t t he resu l t ing
thermal stresses w i l l l a rge ly be relieved by creep o r relaxation as the gradient i s applied. In the small thermal cylinder t he gradient w i l l be
applied a t an accelerated rate of 5°F per day. To examine the r e su l t i ng
temperature d i s t r ibu t ions i n the specimen with time, a two-dimensional,
axisyrmaetric, t rans ien t heat t r a n s f e r analysis was car r ied out, and the
results are shown i n Fig. 10. The d i s t r ibu t ions shown a r e through-the-
w a l l thickness a t the specimen midplane. The so l id l i n e s a r e t r ans i en t
temperatures, while the dashed l i n e represents t he f i n a l s teady-state temperature gradient through t h e w a l l . A thermal conductivity of 1.3 Btu/hr-ft-"F and a spec i f ic hea t of 0.2 Btu/lb-"F were used f o r the con- c re te . The insulat ion a t top and bottom w a s accounted f o r by using
equivalent heat t r a n s f e r coeff ic ients .
t u re r i s e on t h e inner surface of the specimen i s l a r g e r than would be
used i n a c t u a l pract ice , t he t r ans i en t temperature curves i n Fig. 10 indi-
ca te t h a t t he resu l t ing temperature d i s t r ibu t ion a t any time i s e s sen t i a l ly
t h a t corresponding t o steady-state conditions.
Although the 5°F per day tempera-
The preliminary time-dependent creep analysis was performed using
the f i n i t e element computer program SAF'E-CREEP,5 which w a s developed f o r
PCRV's by G u l f General Atomic, Inc. This i s a l i n e a r v i scoe las t ic program
based on the superposition pr inc ip le . It i s a two-dimensional analysis t ha t w i l l treat e i ther axisyrmnetric o r plane concrete s t r u c t u r e s . A
spec i f i c s e t of concrete creep data, which includes age a t loading as a
var iable , i s b u i l t i n to the program.
Although any o ther set of creep data can, with very l i t t l e t rouble ,
be programmed i n t o the SAFE-CREEF' program, the preliminary analysis was performed using the data cur ren t ly i n the program.
from t h e basic creep invest igat ions previously described ind ica te t h a t t he ac tua l thermal cylinder concrete w i l l exh ib i t s l i g h t l y less primary
The i n i t i a l creep data
creep than indicated by the da ta used i n the computer program and about
t he same amount of secondary creep.
422
The f i n i t e element layout f o r the analysis i s shown i n Fig. 11. Both
the cylinder and the co1.e are shown divided i n t o a f i n i t e element gr id .
I n these s t ruc tures the idea l iza t ions include membrane-type elements repre-
senting the 1/8-in. - thick mild steel l i n e r s , the panel c o i l heat exchanger
composites, and the sheet m e t a l bottom seals. I n the cy l indr ica l specimen
the s t e e l anchor p l a t e s f o r t he axial tendons a r e represented by s t e e l
elements. The circumferential p re s t r e s s loading on the cylinder was represented by an external pressure.
Typical results from the preliminary time-dependent analysis of the
cy l indr ica l specimen a r e presented i n Figs. 12, 13 and 14. The circum-
f e r e n t i a l and axial stresses on t h e inner and outer surfaces of the cyl in-
der a t midheight are shown i n Fig. 12 as a function o f t i m e since pre-
s t ress ing . The heavy l i n e s are the v iscoe las t ic predict ions while the f i n e l i n e s ind ica te the var ia t ions predicted by a purely e l a s t i c ana lys i s .
The circumferential and a x i a l s t r a i n var ia t ions a t the same points a r e
shown i n Fig. 13, while the circumferential and a x i a l s t r e s ses i n the
s teel l i n e r a t midheight are shown i n Fig. 14.
While the ana ly t i ca l technique used f o r the preliminary analysis i s
only one of several p o s s i b i l i t i e s t h a t w i l l be u t i l i z e d i n the thermal
cylinder invest igat ion, the r e su l t s presented i n Figs. 12, 1.3 and 14 do
give an indicat ion of the general stress and s t r a i n behavior expected
during the tes t . The results show t h a t during periods t h a t are pre-
dominantly load controlled ( f o r example, when only the pres t ress ing forces
a r e ac t ing) the time-dependent behavior is p:cimarily creep with the s t r a i n s changing more rapidly than the stresses. During periods t h a t a r e pre-
dominantly s t r a i n controlled ( f o r example, when t h e thermal gradient plus
the pres t ress ing i s ac t ing) the behavior i s primarily re laxat ion with the
stresses changing more rapidly than the straj-ns.
The e f f e c t of stress relaxat ion on the s t r e s ses due t o pres t ress ing
plus the thermal gradient can be seen i n the circumferential s t r e s s on
the inner surface i n Fig. 12. Calculated on an e l a s t i c bas i s , the s t r e s s
i s almost 3200 p s i compression. Pr inc ipa l compressive stresses a r e
generally l imited t o 0.45fk, where f ' is the specif ied 28-day compressive C
ORNL-DWG 69-4830 il I
Fig. 10. Temperature Dis t r ibu t ions with Time Across Wall of Thermal Cylinder a t Midheight.
NOTE DIMENSIONS ARE IN INCHES
Fig. 11. Axisymmetric F i n i t e Element Layouts f o r Thermal
Cylinder Test Specimen and Core.
434
I I l l l l l l l I
30 days (5 days 90 days 180 days 45 days PRESTRESSING HEATING PRESTRESSING PLUS INTEF'NAL PRESSURE ON INTERNAL PRESSURE
OFF (700psi ) - 3500 l l l l l l 1 1l l I l111 I I l l l l l l l I I I
- 3000 - - v) n
v) -2500 v) W rr
-
5 -2000 1
L -1500
I
t- z
W LL
_----- 2 -1000 a - - - - - u
- 500 --_----
0 l l l l l l 1 I1111111 I I l l l l l l l I I I. - f I I l I I I I l l l l l l l I I I l 1 l 1 I l I I I - -1500 n
Fig. 12. Thermal Cylinder Test Specimen and Core- Predicted Circumferential and Axial Concrete Stress Variation with Time on Inner and Outer Surfaces.
I I I l l l l l l l l I I I I I I I I 1 1 l l 1 1 l 1 I I l l l l l l l I I l l l l l l l I I I - 1000
I I 1 1 1 1 1 1 1 I
1 - 4 0 0 P
I 1 I I l l l l l l l I I I I I I I 1 I I I I I I I I I I 1 1 1 1 1 1 1 I I I l l l l l l I I I
c
200
li I
I
/
EL A ST I c AN A LY s I s
*---A\- -- -
I I l l l l l l l I I I I I I I l l l l l l l I l l l l l l l I I r n t- - - In A -200 5 10 30 35 40 4 5 46 54 64 135 136 144 154 234 316 324 360 a TIME SINCE PRESTRESSING ((lays) X I
Fig. 13. Predicted Circumferential and Axial Concrete S t ra in Variation with Time on Inner and Outer Surfaces of Thermal Cylinder a t Midheight.
425
st rength and i s 6000 p s i f o r the specimen concrete. Thus the compressive 0 stress l i m i t i s 2700 p s i , which i s exceeded by the circumferential s t r e s s calculated on an e l a s t i c basis. With s t r e s s re laxat ion taken i n t o account t h e m a x i m u m stress i s 2550 ps i , compression, which i s below the l i m i t .
This i s generally t h e case i n ac tua l PCRV's. Early designers found t h a t f o r a design t o remain within p rac t i ca l and economic l imi t s , account had t o be taken of the benef ic ia l e f f ec t s of creep. used various methods t o approximately account f o r the e f f e c t s of creep i n t h e i r s t r e s s analyses, notably by simply using a reduced e l a s t i c modulus value, w h i l e o thers have relaxed the allowable stress l i m i t s f o r thermal
plus mechanical load s t r e s ses calculated on an e l a s t i c basis.
Some designers have
To accurately pred ic t the ac tua l stresses, more r e a l i s t i c and rigorous
creep analysis methods must be used. The l i n e a r v i scoe las t ic method em- ployed by SAFE-CREEP i s one poss ib i l i t y . It is known, however, that the
pr inc ip le of superposition used i n SAFE-CREEP does not agree, i n a l l cases, with experimental observations on concrete behavior, and, i n f ac t , one of the object ives of t he thermal cylinder t es t i s t o evaluate the accuracy of t h i s method.
Other ana ly t i ca l techniques, including a v iscoe las t ic analysis with a modified superposition pr inc ip le , the simplified e f f ec t ive modulus m e t h o d , and an analysis based on the rate of creep method w i l l also be
investigated and u t i l i z e d f o r comparisons with the experimental r e s u l t s from t h e thermal cylinder test .6 From these comparisons the most su i tab le creep theory and method of analysis will be iden t i f i ed .
Instrumentat ion
One of t h e bas ic object ives of the small thermal cylinder t e s t i s t o evaluate various types of instrumentation. The information t o be obtained from the tes t consis ts of s t r a i n s , stresses, temperatures, and moisture l eve l s throughout the concrete cylinder, as w e l l as the concrete core;
s t r a i n s on the mild s teel l i n e r ; forces and s t r a i n s i n the pres t ress ing
tendons; and ove ra l l def lect ions of t h e cylinder. With t h i s information obtained as a function of time throughout the tes t , adequate comparisons
can be made w i t h ana ly t i ca l predict ions such as those j u s t shown. @
426
A s near ly as possible the instrumentation w i l l l i e along four r a d i a l l i n e s , 90" apar t , near the midheight of the s t ruc ture . Two of the l i n e s w i l l pass through bearing p l a t e s of the circumferential p res t ress ing
system, while the other two will pass between bearing p la tes .
of l i n e s w i l l contain iden t i ca l instrumentation and w i l l thus provide
dupl icate sets o f data.
Each p a i r
A t o t a l of 231 e l e c t r i c a l instrumentation poin ts
consis t of the following:
Rnbedded vibrating-wire s t r a i n gages, including resis tance thermometers i n each gage
Ehbedded Microdot resistance strain ga,zes
Embedded Carlson-type resis tance s t r a i n gages
Microdot weldable resis tance s t r a i n gal, Tes on the mild steel l i n e r of t h e specimen
Rnbedded stress gages (three d i f f e ren t types)
Resistance s t r a i n gages on pres t ress ing tendons
Load transducers on axial pres t ress ing tendons
LVM"s f o r measuring def lec t ions
Thermocouples
Pressure transducer
is planned. These
Number t o be Used
30
45
6
16
18
20
12
20
33
1
A Troxler probe-type neutron and g a m - r a y back-scattering instrument w i l l be used f o r measuring moisture l e v e l s i n the t e s t cylinder and core. Vert ical holes l i ned with t h i n m e t a l tubing w i l l be cas t i n a t several
locat ions where moisture measurements a r e desired. lowered in to the concrete from the top of the t es t s t ruc ture t o predeter-
mined v e r t i c a l posi t ions.
The probe w i l l be
O f t he three types of embedment s t r a i n gages being used i n the tes t ,
t he vibrat ing w i r e and Carlson-type gages have had widespread use; however, the vast ma.iority of emerience has been f o r ambient conditions. The
427
30 days ! 5 days 90 days 100 days 45 days PRESTRESSING HEATING PRESTRESSING PLUS INTERNAL PRESSURE ON INTERNAL PRESSURE
ONLY (5"F/day) , THERMAL GRADIENT OFF ( 7 0 0 p s i ) (700 psi) I- 1
I I 1 1 l l 1 1 1 I I I
-30.000
-25,000
I .- z -20,000 ln ln w
-15,000 $i
-!O,OOO ELASTIC ANALYSI
-5000
0 0 1 10 30 35 40 45 46 TIME SINCE PRESTRESSING (days)
Fig. 14. Predicted Circumferential and Axial S t r e s s Variation with Time i n S tee l Liner a t Midheight.
1 vB-in.-DIAM STRESSTEEL REGULAR BARS, 72 in. LONG
18 x 36-in. CONCRETE CY LlNDER
'2-in. STEEL END PLATE
. COUPLING
- 530-ton HYDRAULIC RAM
Fig. 15" Relaxation Test Loading Frame. Y
428
Microdot embedment gage has been developed spec i f i ca l ly f o r use i n con- c re t e a t elevated temperatures.
The stress gages t h a t have been thus f a r used f o r embedment in con-
c re t e were unsat isfactory f o r t h i s t es t pr imari ly due t o t he i r la rge s i ze
and l imited s t r e s s range. The Aerojet-General Corporation has developed a stress gage spec i f i ca l ly f o r t h i s appl icat ion. It consis ts of two in- dependent bonded strain-gage bridges i n a szaled s t e e l case. One of the
bridges i s designed t o measure r e l a t ive ly s!nall s t r e s s differences over a prese t 1000 p s i s t r e s s range. Because of the extreme conditions of environment and treatment t o which the gagea are subjected both a t the t i m e of cast ing of t he concrete and i n the approximately two-year duration of t h e tes t , two addi t iona l types of stress gages a re being developed a t
ORNL . The success of the thermal cylinder t e s t depends t o a la rge extent
on the r e l i a b i l i t y and accuracy of the gage employed i n measuring time- dependent stresses and s t r a i n s i n the concrete. Two concrete cylinders,
18 in . i n diameter and 40 i n . long, w i l l be c a s t w i t h the thermal cylinder
i n order t o provide a basis f o r judging s t r e s s c e l l performance while em- bedded i n concrete. embedment s t r e s s and s t r a i n gages of every type t o be included i n the
thermal tes t and w i l l be sealed a f t e r cast ing. One o f the cylinders w i l l
be loaded incrementally i n the frame shown i n Fig. 15 i n order t o provide a ca l ibra t ion of embedded s t r e s s and s t r a i n gages. s t ressed and unstressed cylinders will be heated t o 150°F and the incre-
mental loading of the one cylinder w i l l be 1-epeated. predetermined m a x i m stress, the nuts on the threaded S t r e s s t ee l bars
beneath the middle s t e e l p la te , Fig. 15, wi1 .1 be tightened t o maintain
the loading produced by the hydraulic r a m . Once the r a m has been unloaded the bars w i l l not be retensioned during the extended tes t period. The embedded stress c e l l s w i l l be used t o read any eventual change i n the
s t r e s s due t o concrete relaxation. Both t h e s t ressed and unstressed speci- mens w i l l remain a t the 150°F temperature during the period of the relaxa-
t i o n tes t .
These addi t iona l cylinders w i l l contain representat ive
Eventually both t h e
Upon reaching a
429
SUMMARY
The thermal cylinder experiment i s one of the major pro jec ts i n the
program of PCRV research and development s ince important contributions
w i l l be made t o the fu r the r understanding of long-term vessel behavior.
Basic concrete materials property data u t i l i z e d with advanced ana ly t i ca l methods w i l l be used t o pred ic t t h e stresses and s t r a i n s i n a model t h a t
w i l l be subjected t o a simulated h i s to ry representing the major loading regimes of an ac tua l PCRV including po ten t i a l o f f design thermal loadings.
Aside from the fundamental object ive of es tab l i sh ing the adequacy
of the bas ic info:rmation used i n pred ic t ing vessel behavior considerable
data w i l l be obtained on t h e performance of pres t ress ing hardware and
special instrumentation.
considerable problem and the evaluation of the performance of the speci-
f i e d devices w i l l i n i t s e l f be of major importance t o t h e overa l l program
of PCRV development.
The instrumentation requirements present a
Because of t he subs tan t ia l costs associated with performing a tes t on a large-scale thermal model the small vessel model was selected as a
very reasonable a l t e rna te f o r experimental study a t t h i s stage of tech-
nological development.
vide a comprehensive check on basic information which is presumed t o be
appl icable t o the determination of la rge s t ruc ture behavior. t i o n obtained from t h i s experiment w i l l provide important data which can
be used t o make more quant i ta t ive assessment of the s t rength and dimen- s iona l s t a b i l i t y of concn \ E <essels and the f ac to r of sa fe ty aga ins t
failure from any materj - degradation from t h e thermal environment.
The experiment has been carefu l ly planned t o pro-
The informa-
1. G. D. Whitman, Prestressed Concrete Reactor Vessel Research and Development Program Summary, USAEC Report ORNL-TM-2179, Oak Ridge National Laboratory, 1968.
GCFP Semiann. Progr. Repts. f o r Sept. 30, 1967; March 31, 1968; Sept. 30, 1968; March 31, 1969; and Sept. 30, 1969; USAEC Reports ORNL-4200, -4266, -4353, -4424, and -4508, Oak Ridge National Laboratory .
2 .
430
3. J. M, C o r n and D. W. Goodpasture, Design and Feas ib i l i t y Study of @ a Large-Scale Test Simulating the Time-Ilependent Behavior of a Pre- s t ressed Concrete Reactor Vessel, USAEC Report ORNL-TM-2390, Oak Ridge National Laboratory, February 1969.
4. A. Puyo, Cope and Bellier, Par i s , France, personal communications t o J. M. Corum, Oak Ridge National Laboratory, December 1968 t o February 1969.
5 . F. J. DeArriago and Y. R. Rashid, SAFE-CREEP - A Computer Program f o r t he Viscoelastic Analysis of Axisymnietric and Plane Concrete Structures, USAEC Report GA-8111, General Atomic Division, General Dynamics Corporation, July 31, 1967.
6. G. L. England, Elas t ic and Thermal-Creep Analyses of Cylindrical Model ConcrFte Pressure Vessel, pp. 262-273, GCRP Semiann. Progr. Rept., Sept. 30, 1968, U S E Report ORNLI-4333, Oak Ridge National Laboratory .
431
DISCUSS ION
D. B. Trauger: I t h a s been p o s t u l a t e d t h a t f o r c e r t a i n l i n e r
f a i l u r e s i t may be p o s s i b l e f o r hel ium to p e n e t r a t e t h e c o n c r e t e , and
hence, e f f e c t i v e l y i n c r e a s e t h e loaded a r e a and even c a u s e f a i l u r e .
What i s your o p i n i o n of t h i s p o s t u l a t i o n ?
T. A . J a e g e r : There a r e f i v e l i m i t s t a t e s of a p r e s t r e s s e d c o n c r e t e
p r e s s u r e v e s s e l recognized a s p r e s e n t i n t h e s t r u c t u r a l d e s i g n and one
of t h e s e l i m i t s t a t e s r e f e r s t o c r a c k p r e s s u r i z a t i o n .
M. Bender: Could t h e d a t a , t o t h i s d a t e , g i v e any i n d i c a t i o n a s t o
whether t h e des ign methods a s s o c i a t e d w i t h v e s s e l s a r e c o n s e r v a t i v e o r
n o n c o n s e r v a t i v e . How close a r e w e t o r e s o l v i n g u n c e r t a i n t i e s concern ing
thermal behavior of c o n c r e t e ?
J. P. C a l l a h a n : I t i s d i f f i c u l t a t p r e s e n t t o make b l a n k e t s t a t e -
ments r e g a r d i n g conserva t i sm, o r t h e l a c k of i t i n a n a l y s e s f o r pre-
d i c t i n g long-term v e s s e l behavior . I n f a c t , t h e a u t h o r s f e e l t h a t one
w i l l n e v e r be a b l e t o s t a t 9 unequivocably, t h a t an a n a l y s i s always
g i v e s c o n s e r v a t i v e p r e d i c t i o n s under a l l c o n d i t i o n s . There a r e s e v e r a l
r e a s o n s f o r t h i s . W e must c o n s i d e r : 1. both stress p r e d i c t i o n s and
s t r a i n c o n d i t i o n s , 2 . bo th thermal l o a d i n g s and mechanical l o a d i n g s ,
and 3 . b o t h s h o r t - t e r m i n i t i a l l o a d i n g s and long-term unloadings and
l o a d v a r i a t i o n . A n a l y t i c a l p r e d i c t i o n s which may be c o n s e r v a t i v e w i t h
r e g a r d t o one i t e m i n the p a i r s above might n o t be c o n s e r v a t i v e w i t h
r e g a r d t o the cor responding i t e m . I n o t h e r words, a n a l y t i c a l p r e d i c -
t i o n s can be c o n s e r v a t i v e i n one s e n s e and n o n c o n s e r v a t i v e i n a n o t h e r .
The consequence of t h i s i s t h a t w e can no l o n g e r r e l y on a method be ing
c o n s e r v a t i v e but must s t r i v e f o r methods which a r e a s n e a r l y c o r r e c t a s
p o s s i b l e . The program d e s c r i b e d i n t h e paper i s aimed a t deve loping such
methods and demonst ra t ing t h e i r v a l i d i t y by means of t h e thermal c y l i n d e r
t e s t . S i n c e t h i s test h a s n o t y e t been completed, i t w i l l be some time
before such i n f o r m a t i o n w i l l become a v a i l a b l e .
Paper 6-
ORAL STATEMENT ON THE PAPER BY H. BENZLER AND J. TERPSTFU: "CONCRETE REACTOR PRESSURE VESSELS - 1969 ASSESSMENT"
by D. Tytga t , Euratom
On 18, 19 and 20 November 1969 t h e Commission of t h e European
Communities h e l d a "Second i n f o r m a t i o n m e e t i n g on work r e l a t i n g
t o p r e s t r e s s e d c o n c r e t e p r e s s u r e v e s s e l s and t h e i r t h e r m a l
i n s u l a t i o n " . The a r t i c l e by B e n z l e r and T e r p s t r a r e c a p i t u l a t e s
t h e f i n d i n g s of t h i s m e e t i n g , e s p e c i a l l y t h e p r o g r e s s a c h i e v e d
d u r i n g t h e las t y e a r s and t h e problems s t i l l t o be s o l v e d .
C o n s i d e r i n g t h e time a l l o c a t e d f o r t h i s s h o r t s t a t e m e n t , i t w i l l
n o t be p o s s i b l e t o p r o v i d e a comple te summary o f t h e c o n t e n t s o f
t h e p a p e r , c o p i e s o f which have been made a v a i l a b l e t o t h e
a u d i e n c e of t h i s c o n f e r e n c e . I s h a l l t h e r e f o r e l i m i t my r emarks
t o new c o n c e p t s f o r p r e s t r e s s e d c o n c r e t e r e a c t o r v e s s e l s and
t h e i r t h e r m a l i n s u l a t i o n which were d i s c u s s e d a t t h e r e c e n t
B r u s s e l s i n f o r m a t i o n mee t ing and which may b e o f p a r t i c u l a r
i n t e r e s t w i t h i n t h e c o n t e x t of t h i s mee t ing .
T a y l o r Woodrow C o n s t r u c t i o n L t d . ( U n i t e d Kingdom) have deve loped
a new t e c h n i q u e o f c i r c u m f e r e n t i a l p r e s t r e s s i n g f o r t h e H a r t l e p o o l
n u c l e a r power p l a n t , which i s d e s i g n e d a c c o r d i n g t o t h e pod
b o i l e r s y s t e m , i n which p r e f a b r i c a t e d b o i l e r u n i t s a r e mounted
i n p e n e t r a t i o n s p a s s i n g v e r t i c a l l y t h r o u g h t h e f u l l h e i g h t of t h e
v e s s e l walls. For t h i s d e s i g n , p o t e n t i a l t endon p a t h s are s e v e r e l y o b s t r u c t e d by t h e p r e s e n c e of t h e b o i l e r pods. It w a s
t h e r e f o r e d e c i d e d t o l o c a t e t h e c i r c u m f e r e n t i a l p r e s t r e s s i n g
o u t s i d e t h e main v e s s e l w a l l s , a n d t o keep t h e o u t s i d e s u r f a c e of
t h e v e s s e l c o m p l e t e l y f r ee of l a r g e p e n e t r a t i o n s . With t h e s e
f e a t u r e s , i t w a s p o s s i b l e t o u s e a wire-winding t e c h n i q u e which
had t o be s p e c i a l l y deve loped b e c a u s e no sys tem e x i s t e d which
c o u l d meet t h e n e c e s s a r y r e q u i r e m e n t s . The a r r angemen t chosen
is b a s e d upon t h e u s e of c o n c e n t r a t e d ba.nds o f 0.2 i n d i a m e t e r
low r e l a x a t i o n wire , wound under t e n s i o n i n t o c h a n n e l s preformed
i n t h e v e s s e l w a l l s . The g e n e r a l l a y o u t o f t h e wire-winding
432
433
equipment i s i l l u s t r a t e d i n s l i d e 1 ( F i g . 6 i n pape r No. 5 ) . The two v e h i c l e s of t h e machine a re c a r r i e d on a s t e e l p l a t f o r m which
can b e r a i s e d or l owered . T r a c t i o n i s o b t a i n e d from a c h a i n
e n c i r c l i n g t h e v e s s e l . A s t h e machine p a s s e s a round t h e v e s s e l ,
wire is drawn from a s p o o l mounted on t h e r e a r v e h i c l e and p a s s e s
t h r o u g h a t e n s i o n i n g d e v i c e . The c h a n n e l s f o r t h e wire-winding
bands a re b u i l t i n p r e c a s t c o n c r e t e u n i t s which form e x t e r n a l
s h u t t e r i n g t o t h e v e s s e l .
P h i l i p p Bolzmann AG (Germany) have deve loped a wound m u l t i l a y e r
c i r c u m f e r e n t i a l p r e s t r e s s i n g sys t em w i t h e q u i d i s t a n t wi res and
i n t e r m e d i a t e a n c h o r s i n t h e form o f c lamps which draw a l l t h e
t e n d o n s t o g e t h e r a t s e v e r a l p o i n t s on t h e v e s s e l ' s c i r c u m f e r e n c e
i n a s u b s e q u e n t l y formed f o r c e - l o c k e d bond. Four t e n s i o n i n g
w i r e s a r e wound on s i m u l t a n e o u s l y by a machine. S l i d e 2 ( F i g . 9 i n pape r No. 14) shows a n example of t h e wire-c lamping s y s t e m ,
and s l i d e 3 ( F i g . 2 3 i n pape r No. 14) a working model o f t h i s
t e n s i o n i n g sys t em f o r a p r e s s u r e v e s s e l o f t h e AGR t y p e .
The French Commissar ia t A 1 ' E n e r g i e Atomique (CEA), i n c o l l a b o r a t i o n
w i t h Messrs. Coyne & B e l l i e r of P a r i s , h a s worked o u t p r o p o s a l s
f o r a t e n s i o n i n g sys t em i n which t h e c i r c u m f e r e n t i a l s t r e s s e s a r e
t a k e n up by e x t e r n a l l y l o c a t e d Hoops of h i g h - t e n s i l e s t e e l s t r i p . Each hoop c o n s i s t s o f a band which i s wound r o u n d t h e vessel
s e v e r a l t i m e s . The p r e s t r e s s i s g e n e r a t e d by t e n s i o n i n g d e v i c e s
l o c a t e d between t h e c o n c r e t e s h e l l and t h e hoop; s l i d e 4 ( F i g . 3 i n p a p e r ) . The e f f i c a c y o f t h i s s y s t e m h a s been proved by t e s t s .
a i t h a l l p r e s t r e s s e d c o n c r e t e r e a c t o r v e s s e l s , i t is e s s e n t i a l
t h a t t h e r e a c t o r c o r e be r e a d i l y a c c e s s i b l e from t h e o u t s i d e ,
ma in ly f o r t h e pu rpose o f r e f u e l l i n g .
h a s i n t h i s c o n t e x t s t u d i e d a p r e s t r e s s e d c o n c r e t e v e s s e l w i t h a removable s p h e r i c a l c a p , l i k e w i s e of p r e s t r e s s e d c o n c r e t e , which
i s a t t a c h e d t o t h e v e s s e l ' s s h e l l by means o f a s t e e l hoop
s t r u c t u r e ; s l i d e 5 (Fig. 4 i n p a p e r ) . The hoop s t r u c t u r e is b u i l t up o f p l a t e s and c r o s s - t i e s and c o n t a i n s l a r g e c u t - o u t s
The S o c i a Company ( F r a n c e )
434
which e n a b l e t h e c a p t o b e a t t a c h e d by r.ieans of removable b o l t s .
SFonsored by t h e Commission of t h e European Communities, F r i e d .
Krupp U n i v e r s a l b a u (Germany) have develcrped a m u l t i l a y e r concep t
f o r p r e s t r e s s e d c o n c r e t e r e a c t o r v e s s e l s ; s l i d e 6 ( F i g . A ) .
There a r e f o u r d i f f e r e n t l a y e r s , each o f which h a s a s p e c i a l
pu rpose . The i n n e r m o s t l a y e r - s e e s l i d e 7 ( F i g . B) - is made
o f a h e a t - r e s i s t a n t c o n c r e t e a n d a c t s a s a t h e r m a l s h i e l d . The
n e x t l a y e r is a ce ramic h e a t i n s u l a n t .
The t h i r d l a y e r i s a s p a c e l i m i t e d by an i n n e r and an o u t e r s t e e l
l i n e r and f i l l e d w i t h water a t t h e same p r e s s u r e as t h e r e a c t o r
c o o l a n t . The o u t e r l a y e r i s formed by t h e p r e s t r e s s e d - c o n c r e t e
s t r u c t u r e a n d can be k e p t c o m p l e t e l y f r e e o f t e m p e r a t u r e g r a d i e n t s . Model t e s t s on a 1:5 sca l e have been s u c c e s s f u l l y pe r fo rmed .
The pe r fo rmance o f t h e r m a l i n s u l a t i n g s y e t e m s i n s i d e a c o n c r e t e
p r e s s u r e v e s s e l depends l a r g e l y on t h e n a t u r e and t h e p h y s i c a l
c o n d i t i o n s o f t h e r e a c t o r c o o l a n t .
r e l i a b l e s y s t e m s have been deve loped b o t h i n F rance and i n t h e
Un i t ed Kingdom.
For C02- c o o l e d r e a c t o r s ,
S l i d e 8 shows t h e t f M & t a l i s o l f t sys t em r e c e n t l y employed by CAFL
( F r a n c e ) i n t h e Bugey r e a c t o r . It c o n s i s t s o f p a c k s o f s t a i n l e s s
s t e e l c l o t h s s u i t a b l y s p a c e d by f o i l s and s e a l s and t i e d t o g e t h e r
by b o l t s and a rugged c a s i n g . Other d e s i g n s o f a comparable t y p e ,
however , u s i n g m i n e r a l f i b r e i n s t e a d o f m e t a l c l o t h s , a r e
c u r r e n t l y b e i n g used by Delaney G a l l a y i n s e v e r a l B r i t i s h n u c l e a r
power s t a t i o n s o f t h e AGR t y p e .
A t h e r m a l s h i e l d s y s t e m b a s i c a l l y c o n s i s t s o f t h r e e components
( F i g . 9): - a n i n s u l a t i n g l a y e r , which r e d u c e s t h e h e a t f l u x from t h e
r e a c t o r c o o l a n t t o t h e v e s s e l w a l l s ;
- a metal p l a t e , u s u a l l y t h e l e a k t i g h t l i n e r , which d r a i n s t h e
h e a t l e a k i n g t h r o u g h t h e i n s u l a t i n g l a y e r t o t h e c o o l i n g sys t em; n
435
crs - t h e above-mentioned c o o l i n g s y s t e m , which e v a c u a t e s t h e h e a t
l o s s e s t o o u t s i d e r e a c t o r v e s s e l .
These components a r e n o r m a l l y a r r a n g e d i n s u c h a way t h a t t h e
i n s u l a t i o n is i n s i d e t h e l i n e r , where i t is immersed i n t h e
r e a c t o r c o o l a n t . The c o o l i n g c i r c u i t is u s u a l l y l o c a t e d o u t s i d e
t h e l i n e r , where i t is embedded i n t h e c o n c r e t e . T h i s
" c o n v e n t i o n a l ' 1 a r r a n g e m e n t , shown on t h e l e f t i n F i g . 9 , is t h e
o n l y one a p p l i e d s o f a r i n power r e a c t o r s .
I n t h e a r r angemen t shown i n t h e c e n t r e o f F i g . 9 , t h e c o o l i n g
sys t em h a s moved from t h e o u t s i d e t o t h e i n s i d e o f t h e l i n e r .
The c o o l a n t is t h e same as t h a t o f t h e r e a c t o r c o r e and a t t h e
same p r e s s u r e , b u t a t a lower t e m p e r a t u r e . T h i s sys t em h a s no
s p e c i a l l e a k t i g h t n e s s r e q u i r e m e n t s and i t a l l o w s a h i g h d e g r e e o f
p r e f a b r i c a t i o n . It h a s been deve loped under a Euratom sponsored
c o n t r a c t by Deutsche Babcock and iiu'ilcox and t h e F rench f i r m of
S o c i a .
I n t h e a r r angemen t shown on t h e r i g h t i n F i g . 9 , b o t h t h e c o o l i n g
sys t em and t h e i n s u l a t i o n l a y e r a r e o u t s i d e t h e l e a k t i g h t l i n e r .
I n t h i s c o n c e p t , deve loped by t h e French f i r m of SEEE, t h e l i n e r
is s u b j e c t e d t o e x t r e m e l y s e v e r e t h e r m a l and mechanica l s t r e s s ,
which g i v e s r i s e t o e x t r e m e l y t r i c k y problems. On t h e o t h e r
hand , i t e l i m i n a t e s almost all t h e problems i n v o l v e d w i t h t h e
o t h e r c o n c e p t s , and i t might p rove t o be an a t t r a c t i v e p r o p o s i t i o n
i n t h e c a s e o f wa te r - coo led r e a c t o r s f o r example.
I hope t h a t t h i s s h o r t i n t r o d u c t i o n h a s g i v e n you an i m p r e s s i o n o f
t h e c o n s i d e r a b l e amount of work t h a t h a s been done i n t h i s f i e l d
i n Europe . The u t i l i t i e s i n t h i s p a r t o f t h e wor ld have shown
comple te c o n f i d e n c e i n t h e p r e s t r e s s e d c o n c r e t e p r e s s u r e v e s s e l
from t h e v e r y b e g i n n i n g o f commercial n u c l e a r power g e n e r a t i o n .
The b e s t p r o o f o f t h i s c o n f i d e n c e is c e r t a i n l y t h e number o f
p r e s t r e s s e d c o n c r e t e p r e s s u r e v e s s e l s i n o p e r a t i o n o r under
c o n s t r u c t i o n a t t h e moment - which t o t a l 18 i n a l l .
Thank you f o r your a t t e n t i o n .
.
437
HTGR FUEL E U M E N T DESIGN,
PERFORMANCE AND EVALUATION
(Session V )
438
Chairman : R. F. Turner, Gulf General Atomic
Co-Chairman: J. W. Coobs, Oak Ridge National Laboratory
Paper 1/131
6d HTGR FUEL IRRADIATION P E R F O S - I AND IMPLICATIONS ON FUEL DESIGN* =--*m---,ua+r ---.A"" ...-"a-..%.-m-
i; W . V . Goeddel 'r
E. 0. Winkler
C . S . Luby <\
Gulf Genera l Atomic I n c o r p o r a t e d
San Diego, C a l i f o r n i a
ABS TRACT
The f u e l e lement d e s i g n f o r l a r g e HTGRs i s a hexagonal g r a p h i t e b l o c k c o n t a i n i n g c o a t e d p a r t i c l e s i n bonded f u e l r o d s . The e x c e l l e n t i r r a d i a t i o n performance of t h e m u l t i - l a y e r e d B I S O and TRISO coa ted p a r t i c l e s h a s been demonst ra ted i n 250 s u c c e s s f u l tests t o burnups up t o 59% FIMA, f a s t f l u e n c e s up t o 8.7 x l o z 1 n/cm2, and t e m p e r a t u r e s up t o 1450°C. Beds of c o a t e d p a r t i c l e s bonded i n t o f u e l r o d s w i t h carbon- aceous matrices have been demonstrated t o be s t a b l e d u r i n g 18% FIMA burnup and 6 x l o2 ' n/cm2 f a s t f l u e n c e a t 1250°C. I r r a d i a t i o n t e s t i n g of t h e r e f e r e n c e g r a p h i t e h a s shown i t t o have adequate d imens iona l and s t r u c t u r a l s t a b i l i t y o v e r t h e f u l l r a n g e of HTGR o p e r a t i n g c o n d i t i o n s .
INTRODUCTION
The s u c c e s s f u l development of c o a t e d - p a r t i c l e f u e l s d u r i n g t h e p a s t 1-3 decade h a s l e d t o s i m p l i f i c a t i o n of t h e f u e l e lement d e s i g n f o r HTGRs.
Because of t h e demonstrated e x c e l l e n t s t a b i l i t y of t h e c o a t e d p a r t i c l e s under
t h e combined c o n d i t i o n s of h i g h t e m p e r a t u r e , h i g h burnup, and h i g h f a s t f l u e n c e ,
f u e l e lement d e s i g n h a s been r e l i e v e d of t h e r e q u i r e m e n t s f o r c o s t l y low-per-
m e a b i l i t y g r a p h i t e s and complex f i s s i o n p r o d u c t p u r g h g sys tems.
product c o n t r o l i s now achieved mainly by t h e p a r t i c l e c o a t i n g s , and t h e
d e s i g n e r h a s been g i v e n much g r e a t e r freedom t o o p t i m i z e c o r e performance and
reduce f u e l c y c l e c o s t s .
F i s s i o n
*Work suppor ted i n p a r t by t h e U.S. Atomic Energy Commission under Con- a r a c t s AT (04-3) -633 and AT (04-3) -167, P r o j ect Agreement No. 17 .
439
440
Cores of t h e F o r t S t . V r a i n 330-FnJ(e) and t h e 1100-MW(e) HTGRs are
composed of hexagonal-shaped b l o c k s of c o n v e n t i o n a l needle-coke g r a p h i t e
s t a c k e d i n a close-packed a r r a y of ve r t i ca l columns. 4’5 from t h e long c y l i n d r i c a l e lements used i n the Peach Bottom HTGR a f t e r i t
had been proven t h a t f i s s i o n p r a d u c t contr0.L could b e achieved by means of
t h e m u l t i l a y e r e d p a r t i c l e c o a t i n g s . I n t h e hex-block f u e l e lement , t h e
c o a t e d p a r t i c l e s are c o n t a i n e d i n f u e l r o d s l o c a t e d w i t h i n v e r t i c a l f u e l
channels .
spaced among t h e f u e l channels .
This d e s i g n evolved
Coolant channels p a s s i n g comple te ly through t h e element are i n t e r -
R e s u l t s of many i r r a d i a t i o n tests have confirmed t h e e x c e l l e n t p e r f o r -
mance of HTGR f u e l under some of t h e most s e v e r e d e s i g n o p e r a t i n g c o n d i t i o n s
e n v i s i o n e d f o r HTGR p l a n t s . These r e s u l t s a r e summarized i n t h i s paper , and
t h e d e s i g n b a s i s for t h e hex-block f u e l element g r a p h i t e i s d e s c r i b e d .
COAT ED PART I CL E S
Two t y p e s of c o a t e d p a r t i c l e s (BISO and TRISO) have been developed and
proved f o r HTGR u s e ( F i g . 1). Each has a d e n s e , s p h e r i c a l c a r b i d e k e r n e l and
a n i n n e r c o a t i n g l a y e r of low-densi ty porous p y r o l y t i c carbon ( b u f f e r PyC
c o a t i n g ) .
t r o p i c PyC, whereas t h e TRISO c o a t i n g h a s a s i l i c o n c a r b i d e l a y e r sandwiched
between i n n e r and o u t e r l a y e r s of t h e h i g h - s t r e n g t h , i s o t r o p i c PyC. The S i c
c o a t i n g l a y e r p r o v i d e s added r e t e n t i o n of me ta l l i c f i s s i o n p r o d u c t s . F u e l
k e r n e l s r a n g e i n s i z e from 100 t o 600 Um i n d i a m e t e r , w i t h o v e r a l l c o a t i n g
t h i c k n e s s e s of a b o u t 130 u m . Mathematical st:ress a n a l y s i s models, combined
w i t h t h e r e s u l t s of many i r r a d i a t i o n e x p e r i m e n t s , are used t o d e s i g n t h e
coa ted p a r t i c l e s f o r s p e c i f i c a p p l i c a t i o n s .
The B I S O c o a t i n g h a s a s i n g l e o u t e r l a y e r of h i g h - s t r e n g t h , i s o -
6 -,9
I r r a d i a t i o n t es t r e s u l t s on l a r g e numbers of s t a t i s t i c a l l y s i g n i f i c a n t
samples of B I S O and T R I S O c o a t e d p a r t i c l e s have demonstrated t h e i r s t a b i l i t y
t o burnups g r e a t e r t h a n 20% FIMA ( f i s s i o n s p e r i n i t i a l metal atom) and t o
f a s t f l u e n c e s g r e a t e r t h a n 8 x 10” n/cm2 ( E > 0.18 MeV) a t t empera tures of
1300°C. These tes ts have been conducted f o r t h e most p a r t i n c a p s u l e s i n t h
441
ETR a t NRTS, Idaho ,and t h e GETR a t V a l l e c i t o s , C a l i f o r n i a . Specimen tempera-
t u r e s are c l o s e l y c o n t r o l l e d and monitored by means of thermocouples l o c a t e d
i n t h e c e n t e r of t h e f u e l samples; f a s t f l u e n c e s are determined by a n a l y s e s
of f l u x w i r e s l o c a t e d throughout t h e c a p s u l e s ; and burnups are determined by
p o s t i r r a d i a t i o n i s o t r o p i c a n a l y s e s of t h e f u e l . Each c o a t e d p a r t i c l e t e s t
sample c o n s i s t s of s e v e r a l thousand c o a t e d p a r t i c l e s , a l l of which are examined
b e f o r e and a f t e r i r r a d i a t i o n .
Test r e s u l t s are a v a i l a b l e t o d a t e on about 300 i n d i v i d u a l samples of
c o a t e d p a r t i c l e s , and o v e r 100 a d d i t i o n a l samples are c u r r e n t l y be ing t e s t e d ,
i n c l u d i n g many samples i n test e lements i n t h e Peach Bottom HTGR. lo
coated p a r t i c l e s have s u r v i v e d burnups up t o 59% FIMA, f a s t f l u e n c e s up t o
8 .4 x lo2’ n/cm2, and tempera tures up t o 1450°C. (A sample i s cons idered t o
have s u r v i v e d a test i f more t h a n 99% of t h e p a r t i c l e c o a t i n g s have r e t a i n e d
t h e i r i n t e g r i t y . )
FIMA, f a s t f l u e n c e s up t o 8 . 7 x lo2’ */ern2, and t e m p e r a t u r e s up t o 1300°C.
BISO
TRISO c o a t e d p a r t i c l e s have s u r v i v e d burnups up t o 27%
Photomicrographs of BISO and TRISO c o a t e d p a r t i c l e s t e s t e d under condi-
t i o n s more severe t h a n t h e peak d e s i g n o p e r a t i n g c o n d i t i o n s e n v i s i o n e d f o r
HTGR p l a n t s are shown i n F i g s . 2 and 3 . The r e g i o n s of demonstrated s u c c e s s -
f u l i r r a d i a t i o n performance f o r B I S O and TRISO c o a t e d p a r t i c l e s w i t h r e s p e c t
t o burnup and f a s t f l u e n c e are shown i n F i g . 4. These tes t r e s u l t s i n c l u d e many samples of B I S O and TRISO c o a t e d p a r t i c l e s prepared i n f u l l - s c a l e produc-
t i o n equipment.
FUEL RODS
The HTGR f u e l r o d s c o n s i s t of c lose-packed beds of coa ted p a r t i c l e s
bonded t o g e t h e r w i t h a carbonaceous m a t r i x .
f o r s u f f i c i e n t s t a b i l i t y under i r r a d i a t i o n t o avoid t h e d e l e t e r i o u s e f f e c t s
t h a t have been observed w i t h less s t a b l e f u e l body matrices. Design f e a t u r e s
of t h e f u e l r o d s i n c l u d e u s e of a g r a p h i t i z i n g b i n d e r i n c o n j u n c t i o n w i t h h i g h
h e a t t r e a t m e n t t e m p e r a t u r e s and r a d i a t i o n - s t a b l e g r a p h i t i c f i l l e r m a t e r i a l s .
A h o t i n j e c t i o n molding p r o c e s s i s used t o f a b r i c a t e t h e f u e l r o d s . This
This m a t r i x h a s been des igned
442
p r o c e s s i s a d a p t a b l e t o t h e manufacture of Euel r o d s up t o several i n c h e s
l o n g . F u e l r o d s a re s t a c k e d end-to-end i n t h e f u e l channels of t h e hex-
b l o c k element t o make up t h e r e q u i r e d f u e l (column h e i g h t . T y p i c a l f u e l r o d s
are shown i n F i g . 5.
I r r a d i a t i o n tests t o 6 x 1 O 2 l n/cm2 and 18% FIMA a t 1250°C have shown
t h a t t h e s e f u e l r o d s have e x c e l l e n t s t a b i l i t y under i r r a d i a t i o n .
of c o a t i n g breakage o r of d e l e t e r i o u s i n t e r a c t i o n between t h e m a t r i x and t h e
p a r t i c l e c o a t i n g s h a s been observed . Photographs and photomicrographs of
i r r a d i a t e d f u e l r o d s are shown i n F i g s . 6 , 7 , and 8 .
No evidence
GRAPHITE FUEL BLOCKS
The act ive f u e l , i n t h e form of bonded r o d s , i s s t r u c t u r a l l y conta ined
and a r r a n g e d f o r e f f e c t i v e h e a t t r a n s p o r t t o t h e hel ium c o o l a n t w i t h i n p r i s -
matic g r a p h i t e f u e l e l e m e n t s . The f u e l e lement s t r u c t u r a l g r a p h i t e a l s o
s e r v e s as t h e r e a c t o r modera tor . Each hexagonal f u e l e lement i s 1 4 . 2 i n .
a c r o s s f l a t s and 31.2 i n . i n l e n g t h ( s e e F i g . 9 ) . A s t a n d a r d f u e l e lement
c o n t a i n s 210 a x i a l l y o r i e n t e d f u e l h o l e s , i n t e r s p a c e d w i t h 108 c o o l a n t channels .
Burnable p o i s o n f o r r e a c t i v i t y shimming can 'be i n s e r t e d i n t o any of s i x addi -
t i o n a l non-fueled h o l e s provided a t t h e c o r n e r s of t h e hexagonal e lement .
The f u e l e lements are manufactured from a n u c l e a r - p u r i t y g r a d e of con-
v e n t i o n a l e x t r u d e d needle-coke g r a p h i t e . I n T a b l e 1, s t r e n g t h p r o p e r t i e s of
t h e p r o d u c t i o n f u e l e lement g r a p h i t e f o r t h e F o r t S t . V r a i n Nuclear Genera t ing
S t a t i o n are summarized and compared w i t h v a l u e s e s t a b l i s h e d a s d e s i g n c r i t e r i a .
The l o n g i t u d i n a l minimum s t r e n g t h i s de termined by t e n s i l e t e s t i n g of c o r e
d r i l l e d specimens t a k e n from t h e l o g c e n t e r , where t e n s i l e s t r e n g t h i s normal ly
l o w e s t i n e x t r u d e d g r a p h i t e .
f u e l e lement u s e i n t h e F o r t S t . Vra in HTGR are b e i n g t e n s i l e s t r e n g t h t e s t e d .
One hundred p e r c e n t of t h e p r o d u c t i o n l o g s f o r
11-14 Extruded needle-coke t y p e g r a p h i t e s have been e x t e n s i v e l y i r r a d i a t e d
t o a f a s t n e u t r o n f l u e n c e of g r e a t e r t h a n 8 x l o 2 ' n/cm2 (E > 0.18 MeV) ( t h e
d e s i g n maximum f a s t f l u e n c e f o r HTGR f u e l e l e m e n t s ) . Data maps of i r r a d i a t i
duced d imens iona l change v e r s u s tempera ture and f a s t f l u e n c e based upon /In t h e s e r e s u l t s have been c o n s t r u c t e d f o r u s e i n f u e l e lement d e s i g n and per -
formance a n a l y s e s . These d a t a maps are shown i n F i g s . 10 and 11 f o r t h e a x i a l
and t r a n s v e r s e d i r e c t i o n s , r e s p e c t i v e l y . The shaded area on each map envelops
t h e e n t i r e r a n g e of f l u e n c e and tempera ture exper ienced by f u e l e lements w i t h i n
t h e F o r t S t . Vra in r e a c t o r . G r a p h i t e d imens iona l changes p r e d i c t e d over t h e
f u l l r a n g e of d e s i g n o p e r a t i n g c o n d i t i o n s are w i t h i n a c c e p t a b l e v a l u e s f o r t h e
o v e r a l l c o r e and f u e l e lement d e s i g n s .
I n a d d i t i o n t o g r o s s f u e l e lement d imens iona l change d e s i g n cons idera-
t i o n s , stresses w i t h i n t h e l i g a m e n t s between f u e l r o d s and c o o l a n t channels
are e v a l u a t e d .
i n t h e d i r e c t i o n of h e a t f low between t h e ac t ive f u e l and c o o l a n t channels .
I n a d d i t i o n t o t h e thermal stresses r e s u l t i n g from t h e s e g r a d i e n t s , stresses
are a l s o induced by d i f f e r i n g ra tes of g r a p h i t e d imens iona l change a c r o s s a
l igament because of t h e tempera ture dependence of t h e i r r a d i a t i o n - i n d u c e d
g r a p h i t e c o n t r a c t i o n r a t e .
Ligament stresses occur as a r e s u l t of t h e tempera ture g r a d i e n t s
Although t h e t o t a l s t r a i n d i f f e r e n c e s r e s u l t i n g from c o n t r a c t i o n g r a d i e n t s
a c r o s s l i g a m e n t s are t y p i c a l l y l a r g e compared w i t h t h e thermal s t r a i n d i f f e r e n c e s
(which produce thermal s t r e s s e s ) , t h e c o n t r a c t i o n g r a d i e n t stresses remain
r e l a t i v e l y low because of i r r a d i a t i o n - i n d u c e d c r e e p . 15’16 lifetime stress h i s t o r y f o r a F o r t St. Vrain f u e l e lement a t t h e l o c a t i o n
w i t h i n t h e g r a p h i t e l igament e x p e r i e n c i n g maximum a x i a l t e n s i l e stress. maximum t e n s i l e o p e r a t i n g stresses, a f t e r i r r a d i a t i o n - i n d u c e d c r e e p r e l a x a t i o n
of t h e i n i t i a l thermal stresses, t y p i c a l l y occur a d j a c e n t t o the f u e l h o l e .
S t r e s s e s a t t h e c o o l a n t channel boundar ies are t y p i c a l l y compressive. A s
shown i n F i g . 1 2 , t h e t h e r m a l stress d i s t r i b u t i o n becomes a d d i t i v e t o t h e
cont rac t ion- induced stress d i s t r i b u t i o n when t h e r e a c t o r is s h u t down and
t h e o p e r a t i n g t e m p e r a t u r e g r a d i e n t i s removed. F i g u r e 13 shows t h e a x i a l
stress d i s t r i b u t i o n w i t h i n a F o r t S t . V r a i n f u e l e lement l igament d u r i n g
full-power o p e r a t i o n and a t t h e t i m e i n f u e l l i f e of maximum c o n t r a c t i o n -
induced stress. S t r e s s e s i n t h e transverse ( in-p lane) d i r e c t i o n are t y p i c a l l y
smaller t h a n t h e a x i a l stresses. A l l of t h e s e stresses are w e l l below t h e
F i g u r e 1 2 shows t h e
The
W e a s u r e d t e n s i l e s t r e n g t h s of t h e p r o d u c t i o n g r a p h i t e used f o r t h e f u e l b l o c k s .
444
SUMMARY Q Extensive irradiation tests have confirmed the excellent irradiation
performance of HTGR fuel element materials and components under combined
conditions of high temperature, high burnup, and high fast fluence. This
demonstrated performance of the fuel under the most severe design operating
conditions envisioned for HTGR plants has reaffirmed the basic fuel element
design concept of the hexagonal graphite block containing coated particles
in bonded fuel rods. This fuel element is simple, develops EO high stresses
during operation, and promises to be economic to fabricate and reprocess.
REFERENCES
1.
2.
3.
4 .
5.
6.
7.
8.
R. F. Turner and W. V. Goeddel, Advances in Fuel Element Design and
Materials, GA-7183 (June 1966).
W. V. Goeddel, "Coated-Particle Fuels j.n High-Temperature Reactors: A
Summary of Current Applications," Nucl.. Appl. 2, 599 (1967). S. Jaye and W. V. Goeddel, "High-Temperature Gas-Cooled Reactor Fuel and
Fuel Cycles - Their Progress and Promise," Nucl. Eng. Design 2, 283 (1968).
R. C. Dahlberg, R. F. Turner, and W. V. Goeddel, "Core Design Character-
istics," Nucl. Eng. International 13, No. 163, 1073 (1969). R. F. Turner, W. V. Goeddel, and E. 0. Winkler, "HTGR Fuel Design" ( t o be
presented at the Symposium on Sol-Gel Processes and Reactor Fuel Cycles,
Gatlinburg, Tennessee, May 4-7, 1970, and published in the Proceedings).
J. W. Prados and J. L. Scott, "The Influence of Pyrolytic Carbon Creep
on Coated-Particle Fuel Performance," Nucl Appl. 3 , 488 (1967). J. L. Kaae, "A Mathematical Model for Calculating Stresses in a Pyro-
carbon- and Silicon Carbide-coated Fuel Particle," J. Nucl. Mater. 29,
249 (1969).
J. L. Kaae, "A Mathematical Model for Calculating Stresses in a Four-
Layer Carbon-Silicon-Carbide-Coated Fuel Particle," J. Nucl. Mater.
32, - 322 (1969).
-L__
-
___ . . . . . . . ...
445
0 9 . J. L. Kaae, D . W. Stevens, and C . S . Lucy, " P r e d i c t i o n of I r r a d l a t i o n
Performance of Coated P a r t i c l e F u e l s by Means of S t r e s s - A n a l y s i s Models,"
Nucl. Appl. Tech. ( t o b e p u b l i s h e d ) .
10. K. P. Steward, "Objec t ives and P l a n s f o r F u e l T e s t i n g i n t h e Peach Bottom
HTGR" ( p a p e r b e i n g p r e s e n t e d a t t h i s m e e t i n g ) .
3.1. J. W . H e l m , I r r a d i a t i o n of G r a p h i t e a t Temperatures of 300" t o 12OO"C,
Bhi-1056B (August 1969)
12. P u b l i c S e r v i c e Company of Colorado 330-Mw(e) High-Temperature Gas-cooled
Reac tor Research and Development Program,Quarter ly P r o g r e s s Report f o r
t h e P e r i o d Ending March 31, 1969, GA-9261, pp. 70-72 ( A p r i l 1969) .
13. G . B . Engle , Gulf Genera l Atomic I n c o r p o r a t e d , p r i v a t e communication.
14. H. R . W. Cobb, Gulf Genera l Atomic I n c o r p o r a t e d , p r i v a t e communication.
15. C. R . Kennedy, Creep of G r a p h i t e Under I r r a d i a t i o n , Gas-Cooled Reac tor
Program -- Semiannual R e p o r t , September 30, 1966, ORNL-4036,pp. 192-195
(February 1967) .
16 . T . Y. Chang and Y. R. Rashid , Gulf Genera l Atomic I n c o r p o r a t e d , Visco-
e l a s t i c S t r e s s Analys is of G r a p h i t e S t r u c t u r e s , unpubl i shed d a t a .
T a b l e 1. P r o p e r t i e s of P r o d u c t i o n G r a p h i t e U t i l i z e d f o r t h e F o r t S t . V r a i n F u e l Blocks
~~
D e n s i t y , g/cm
T e n s i l e s t r e n g t h , p s i
L o n g i t u d i n a l mean
L o n g i t u d i n a l minimum
Transverse mean
T r a n s v e r s e minimum
Compressive s t r e n g t h , p s i
L o n g i t u d i n a l
T r a n s v e r s e
Design Cr i te r ia
1.70 min
1500
1000
1000
600
3000
3000
Average Measured
Value
1.77
1920
1690a
1160
1010
4400
4700
aBased on 100% t e s t i n g of 752 l o g s ; t h e u v a l u e is 360 p s i .
Fig. 1. BISO- and TRISO-Coated P a r t i c l e s .
447
M275-48 (P18) (200X)
F ig . 2 . BISO-Coated P a r t i c l e a f t e r I r r a d i a t i o n t o 22% FIMA Burnup and 8.4 x Fas t Fluence a t 1300O C.
n/cm2
M251-94 (P20) (17 5X)
Fig. 3 . TRISO-Coated P a r t i c l e a f t e r I r r a d i a t i o n t o 27% FIMA Burnup and 8 .7 x lo2' n/cm2 F a s t Fluence a t 1300O C.
448
T R l S O
LL
J 9
F A S T FLUENCE ( io2 ' N / C M ~ ) F A S T FLUENCE ( io2 ' N / C M ~ )
Fig . 4 . Regions of Demonstrated Irrad ia t ion Per- formance f o r BISO- and TRISO-Coated P a r t i c l e s .
F ig . 5 . H E R Fuel Rods; These Rods are 1/2 i n . i n Diameter and 3/4 i n . Long.
c c
K340-39 (Q2X) K340-65
Fig. 6. Fuel Rods a f t e r I r r a d i a t i o n t o 5.0 ( L e f t ) and 5 .7 (Right) x lo2' n/cm2 F a s t Fluence and 18% FIMA Burnup a t 1 2 5 0 O C. The ends of severed thermo- couple tubes p r o j e c t from t h e ends of t h e rods . These rods a r e 1/2 i n . i n diameter and 3/4 i n . long.
I
M340-148 (125X) M340-125
F i g . 7. Cross S e c t i o n s of F u e l Rods a f t e r I r r a d i a t i o n t o 5.0 ( L e f t ) and 5 . 7 ( R i g h t ) x 1 O 2 I n/cm2 F a s t F luence and 18% FIMA Burnup a t 1250O C. N o d e l e t e - r i o u s e f fec ts were n o t e d i n the c o a t e d p a r t i c l e s i n t h e s e f u e l rods.
Ip ul 0
c
M340- 14 6 (250X) M34 0- 134
Fig . 8. Enlarged V i e w s of t h e G r a p h i t i c M a t r i c e s of t h e Same Two I r r a d i a t e d Fuel Rods t h a t Are Shown i n Fig. 7.
ELEMENT C O N F I G U R A T I O N W I T H CONTROL P O I S O N CHANNELS
mm:r;;:l,~u~~ H A N D L I N G P I C K U P HOLE
DOWEL P I N
H E L I U M FLOW ( T Y P )
S E C A - A 'DOWEL SOCKET
COOLANT HOLE
HOLE
1
PO l SON
Fig. 9. Standard Hex-Block Fuel Element f o r F o r t S t . Vrain and Large H E R S .
453
TEMPERATURE ( O F )
0
-0.4
- 0 . 8
- 1 . 2
- 1 . 6
- 2 . 0
- 2 . 4
- 2 . 8
-3.2
- 3 . 6
-4 .0
- 4 . 4
-4.8
00
("C)
Fig. 10. Irradiation-Induced Dimensional Change'Contours for Fuel Element Needle-Coke Graphite (Axial Direction). Shaded area defines envelope Of operating condition?.
TEMPERATURE ( O F )
2400 2600 2000 2200
0.8
0.6
0.4
0.2 h
bp 0 Y
-I . 4 -0.2 Y W z
-0.4 5 2 -0.6 -I
0
VI z z 0
- -0.8
-
-1.4
-1.6
600 b 800 '1 200
("C)
Fig. 11. Irradiation-Induced Dimensional Change,Contours for Fuel Element Needle-Coke Graphite (Transverse Direction). conditions.
Shaded area defines envelope of operating
401
30(
2 O(
- - v) n v
,,, loa v) W
LL I- v)
0
-100
- 200
\ I FUEL \ \ I ROD
454
ADD I T I VE THERMAL /S,TRESS AT SHUTDOWN
I I I I I I I
0 1 2 3 4 5 6 7 0 F A S T FLUENCE ( IO2’ N V T )
Fig. 12. Maximum Local Axial Tensile Stress in Fuel Element Graphite for the Fort St. Vrain HTGR. The measured mean tensile strength of the graphite is 1900 psi.
\ \
COOLANT \
\ CHANNEL
\
STRESS, P S I
Fig. 13. Axial Tensile Stress Distribution in Fuel Element Graphite Ligament (Fort St. Vrain HTGR).
H. Krgmer: The two types of p a r t i c l e s , the uranium and thorium, a r e
mixed i n the f u e l rods, and therefore , have t h e same l i fe t ime. Do you
expect d i f f i c u l t i e s from t h i s with regard t o temperature changes and f is-
s i l e mater ia l depletion (high excess r e a c t i v e ) ?
W. V. Goeddel: No. This f a c t o r has been covered i n our i r r a d i a t i o n
The i r r a d i a t e d f u e l rods shown i n the paper contained both tes t program.
types of p a r t i c l e s and were tes ted under thermal gradients more severe
than those i n an HTGR. A s reported, no d i f f i c u l t i e s were encountered.
K. W i r t z : Who is the manufacturer of your graphi te?
W. Goeddel: Great Lakes Carbon Corporation i s supplying the graphite
f o r the Fort St . Vrain HTGR.
K. Wir tz : What i s the clearance between your hexagonal blocks; do
you expect l a te ra l dimensional changes?
W. Goeddel: The clearance between adjacent f u e l element columns i s
about 1/8 inch.
blocks i n t h e r a d i a l direct ion, ranging up t o a maximum of 1%.
s i v e i r r a d i a t i o n data on t h i s type of needle coke graphite indicates t h a t
no expansion of the blocks w i l l occur within the design l i f e t i m e of the
fuel elements in the HTGR.
There w i l l be some radiation-induced shrinkage of the
The exten-
R. D. Vaughan: Which f e a t u r e of the p a r t i c l e or block design cur-
r e n t l y s e t s a l i m i t on the core power r a t i n g you achieve i n your r e a c t o r ?
W. Goeddel: Fuel cen ter l ine temperatures.
G. Meijer: Referring t o the stresses calculated f o r the Fort St .
Vrain f u e l block, can you t e l l us whether you analyzed the stresses f o r
cases l i k e a new f u e l block a t the core boundary and l i k e i n s e r t i n g con-
t r o l rods i n a f u e l block, both giving r ise t o s teep temperature gradi-
ents .
the highest s t r e s s e s a r e experienced?
Can you a l s o t e l l i n what p a r t of the core and f o r what conditions
,
W. Goeddel: We have analyzed the s t r e s s e s f o r these and many other
@ conditions. The highest s t r e s s e s a r i s e i n new f u e l near the core boundary.
Paper 2/107 DEVELOPMENT OF BONDED COATED-PARTICLE 13EDS FOR HTGR FUEL EI;EMEXTS*
-J.wwm-,~.w,s.v&.e- - r - +--- ------- IW- 1~
IJ J. L. Scott? J M Bobbins? J. A. Conlint: J. H. Coobst D. M. Hewette IIf: R. L. Sennz .$
3,
ABSTRACT
Fuel elements proposed f o r advanced HTGR's consis t of hexagonal blocks of graphi te with p a r z l l e l f u e l and coolant channels. The f i e 1 channels a r e loaded with py-rolytic-carbon- coated p a r t i c l e s of f i e 1 and f e r t i l e mater ia ls . We developed and demonstrated a method of bonding the coated p a r t i c l e s i n t o " fue l s t icks" t h a t w i l l keep t h e f u e l bed from f a l l i n g apart during handling or during accidents t h a t might damage t h e graphi te core blocks. The bonded fuel. s t i c k s a l s o f a c i l i t a t e inspection of t he f u e l loading and enhance the t ransfer of heat from the f u e l t o the coolant.
Several problems were overcome i n . developing a sa t i s fac- t o ry binder. When a bed of p a r t i c l e s was impregnated with phenolic r e s i n binder and then heated t o carbonize t h e resin, shrinkage broke coatings on some p a r t i c l e s . t h a t survived carbonization produced weak f u e l s t i cks t h a t dis integrated during i r r ad ia t ion t o HTGR fast-neutron fluences. By using high concentrations of f i l l e r mater ia l i n the binder (40 wt % Poco graphi te powder i n p i t ch or 29 w t $I Poco graph- i t e plus 29% Thermax carbon black i n e i the r p i t c h or resin) we produced f u e l s t i cks t h a t remained i n t a c t throughout irra- d ia t ion . Only one damaged coating was found among 2000 coated p a r t i c l e s examined i n i r r ad ia t ed s t i c k s prepared with these binders.
Modified coatings
INTRODUCTION
Fuel elements containing pyrolytic- carison- coated ( U, Th) 02 or
(U, Th) C2 microspheres have found important appl icat ion i n high- temperature
gas-cooled reactors such as the Dragon Reactor i n England, t he AVR i n
*Research sponsored by the U.S. Atomic Energy Commission under
TMetals and Ceramics Division, Oak Ridge National Laboratory. $Reactor Division, Oak Ridge National Laboratory.
contract with the Union Carbide Corporation.
456
A
457
Germany, and the Peach Bottom, UHTREX, and Fort S t . Vrain Reactors i n t h e United States . The core f o r t h e Fort S t . Vrain Reactor i s composed
of hexagonal graphi te fue:L elements stacked i n v e r t i c a l columns. The
f u e l w i l l be located i n 1/2-in.-diam holes t h a t a r e p a r a l l e l t o the
v e r t i c a l coolant holes i n the element. Core designs f o r la rge HTGR's
a r e expected t o be based on t h e Fort S t . Vrain f u e l element.
t a t e inspection of the f u e l loading and t o avoid s p i l l i n g f u e l i n case
of damage t o a f u e l element, it i s proposed tha t the mixture of coated f i s s i l e and f e r t i l e p a r t i c l e s be bonded together with a carbonaceous
matrix before being inser ted in to the f u e l element.
therefore , was t o develop a bonded f i e 1 body t h a t would withstand i r r a - d ia t ion t o peak HTGR exposures without p a r t i c l e f a i l u r e or severe debonding.
neutron (> 0.18 Mev) fluence up t o 8 X lo2' neutrons/cm2 at temperatures of 600 t o 1300°C.
To f a c i l i -
Our objective,
Typical exposures fo r large HTGR's a r e 20% burnup and a f a s t -
Desiring a simple fabr ica t ion technique, we f i rs t developed a method f o r fabr ica t ing such " fue l s t icks" 'by mixing Asbury graphi te
powder with a phenolic r e s i n and in jec t ing the resu l t ing "grease" i n t o
a mold loaded with loose coated p a r t i c l e s .
f l u i d enough t o penetrate a u - in . - long bed of pa r t i c l e s , t he mix con- ta ined only 15 t o 20 w t % graphi te i n r e s in .2 After t he thermosetting r e s i n had hardened a t 8O"C, it w a s carbonized a t 1000°C. matrix density of such bodies was about 0.6 g/cm3.
problem even i n the carbonizing s tep.
coatings deposited from propylene t h a t some coatings cracked during
carbonizing.
s i s t i n g of an anisotropic sea le r layer and a porous outer layer .
prevented t h e coating from cracking during carbonizing, but weakened
t h e bonded bed.
So t h a t t he grease would be
The f i n a l Shrinkage was a
The r e s i n adhered so f i rmly t o
To prevent t h i s , we developed a s a c r i f i c i a l coating con-
This
Bonded beds of t h i s type were f i rs t t e s t ed i n i r r ad ia t ion experi-
ments i n the ORR. In two separate experiment^,^,^ bonded beds of coated
p a r t i c l e s survived t o high burnup (> 25% FIMA) , and the matrix was re la -
t i v e l y undamaged by the low fast-neutron fluences (< 1021 neutrons/cm2).
More recently, two t e s t s i n HFIR t a rge t capsules showed t h a t severe @
458
degradat ion of bonded beds can occur during i r r a d i a t i o n t o f u l l design
fas t f luences . The f i r s t of t hese HFIR experiments, HT-1, contained
ine r t " p a r t i c l e s t h a t were coated with two-:Layer carbon coat ings p l u s
t h e s a c r i f i c i a l and nonbonding l a y e r s and bonded with t h e same matr ix
material t h a t survived i n t h e ORR
such low-density matr ices r e s u l t s i n considerable d e n s i f i c a t i o n and
shrinkage before o ther e f f e c t s become evident . I n t h i s experiment, a
l i n e a r shrinkage of 10% was observed on samples of t h e matr ix material exposed a t 1000°C a t a fas t -neut ron (> 0.18 MeV) f luence of 7.5 X 1021
neutrons/cm2, and t h e mat r ix of bonded beds d e t e r i o r a t e d so extens ive ly
t h a t t h e beds were no longer bonded a t t h e end of t h e t e s t , as seen i n
Fig. 1. Some p a r t i c l e coa t ings were broken a l so , as shown i n Fig. 2 .
Fast-neutron damage t o
* Ine r t kerne ls are requi red i n H F I R because the gamma hea t ing and thermal f l u x a r e so high t h a t t h e bonded beds would be too hot i f f i s - s ion ing occurred i n t h e bed. I n HT-1 and - 3 experiments t h e i n e r t p a r t i c l e s cons is ted of Z r 0 2 .
/ / I
F ig . 1. Loose Coated P a r t i c l e s and Fragments of Matrix Material A f t e r I r r a d i a t i o n t o a Fluence of 7.5 X neutrons/cm2 a t 1000°C.
459
Fig. 2. Polished Section Showing Typical Appearance of Coated Z r O 2 Pa r t i c l e s Bonded with Resin Containing Asbury Graphite Flour. diated. 6 x lo2’ neutrons/crn2; about 20% of the coated pa r t i c l e s were broken i n two such specimens. A s polished. 1OoX. Reduced 16%.
( a ) Unirra- (b ) After i r r ad ia t ion a t 800°C t o a fast fluence of
460
I n a second i r r a d i a t i o n experiment, HT-3, t h e s a c r i f i c i a l coat ing
concept w a s abandoned. The shr inkage of t h e matr ix during carbonizing
was reduced somewhat by increas ing t h e content of f l a k e g raph i t e from
15 t o 25%. This series of samples a l s o f a i l e d t o survive i r r a d i a t i o n
t o 8.0 X lo2' neutrons/cm2 (> 0.18 Mev) a t 1000°C, as shown i n Fig. 3.
The p a r t i c l e beds completely debonded and rmny p a r t i c l e coat ings were
broken.
DEVELOPMENT AND FABRICATION OF IMPROVED BONDED BEDS
We then sought t o develop a bonded bed having t h e requi red i r r a d i a -
Two obvious ways
(1) t o s e l e c t binders t h a t had
t i o n s t a b i l i t y without regard f o r ease of f 'abr icat ion.
t o improve i r r a d i a t i o n performance were:
high coking values and t h a t y i e l d g r a p h i t i z a b l e coke, and ( 2 ) t o add
l a r g e amounts of g raph i t e or o the r f i l l e r to t h e binder . Such mixtures
are much more viscous than t h e binders containing only 15 t o 25% f i l l e r ;
h igher p re s su res are thus requi red i n order t o i n f i l t r a t e t h e bed of
coated p a r t i c l e s .
To f a c i l i t a t e f a b r i c a t i o n of bonded beds, we designed a mold t o
keep t h e p a r t i c l e bed from expanding and r e s u l t i n g i n a f u e l s t i c k with
l e s s than t h e requi red 62-65 vol % p a r t i c l e loading. The bonding mate-
r i a l or "grease" was forced through t h e p a r t i c l e bed by t h e use of a s p e c i a l l y f a b r i c a t e d pressure device or "greasegun," which i s shown i n
Fig. 4. p a r t i c l e s , and p res su re w a s appl ied by d r iv ing t h e double O-ring sea l ed
p i s ton . Pressure w a s app l i ed u n t i l excess bonding material was forced
out a t t h e e x i t end o f t h e mold.
thermoplas t ic binders t h e neoprene O-rings were replaced with Teflon
O-rings.
The threaded n ipp le was a t tached t o t h e mold containing t h e
When prehea t ing w a s requi red wi th
S o l i d i f i c a t i o n of t h e bonding m a t e r i a l was achieved e i t h e r by poly-
merizat ion of thermoset t ing binders a t W " C , or by cool ing t o room t e m -
pe ra tu re when using p i t c h binder , which i s thermoplas t ic . Af te r t h e
f u e l s t i c k s were hardened by polymerizat ion o r cooling, they were
carbonized by hea t ing t o 1000°C i n an i n e r t atmosphere. The f u e l s t i c k s n
a
461
Fig. 3. I r rad ia ted Bonded-Bed Samples Showing Extent of Debonding After Testing a t 1050°C t o Fluence of 8 X lo2' Neutrons/cm2 i n Experi- ment "-3. bonded bed prepared a t ORNL. coatings and matrix mater ia l from bonded specimen containing TRISO-coated p a r t i c l e s prepared a t GGA.
(a) Loose pa r t i c l e s and fragments of matrix mater ia l from (b ) Loose pa r t i c l e s and fragments of
462
must be heated slowly during carbonization t o avoid cracking or d i s t o r - Q t i o n by gases re leased f r o m t h e binder.
l i n e a r heating r a t e t o reach 1000°C i n 24 hr was sa t i s f ac to ry .
was accomplished i n about 12 h r by simply turn ing of f t he power t o t h e
furnace.
We found t h a t heating a t a Cooling
In OUT e f f o r t s t o improve t h e performance of bonded beds, we
i n i t i a l l y se l ec t ed Poco graphi te f lour* as f i l l e r because of i t s remark-
ab le i r r a d i a t i o n s t a b i l i t y . 7
s i s t i n g of 40 w t % Poco graphi te f l o u r (-40 p) i n thermosetting binders
such as Varcum 82517 or phenolic r e s i n . $ Polymerization of t h e thermo-
s e t t i n g binders was cgtalyzed by t h e add i t ion of 5 w t % (based on binder
weight) maleic anhydride t o t h e Varcum, and 10 wt % t o t h e phenolic
r e s i n . Af te r carbonizing a t l o O o ° C , we found the matrix carbon density
t o be 0.9 g/cm3 compared with 0.6 g/cm3 for t h e matrix made previously.
We found a l s o t h a t a similar body could be imde using thermoplastic
binders such as c o a l tar p i t c h . § made f l u i d by preheating a l l mater ia l s and hardware before in j ec t ion .
With grade 15V p i t c h t h e preheating temperaixre w a s a t l e a s t 150°C. To
r a i s e t h e carbon content fu r the r w e added Themax" t o both t h e thermo- s e t t i n g and thermoplastic mixes.
and 29 w t '$ Thermax carbon black i n Varcum gave a carbonized matrix
dens i ty of 1.25 g/cm3.
as t h e binder. Fuel s t i c k s a t l e a s t 2 i n . long could be made with a l l
of t hese mixes.
We found t h a t we could i n j e c t a mix con-
With therinoplastic binders t h e mix i s
A mix containing 29 w t $J Poco graphi te
A similar mix was i n j ec t ed with grade 15V p i t c h
Grade AXM graphi te from Poco Carbon Cclmpany.
?Furfury l alcohol from Varcum Chemical Company.
ZP-514 Cement Primer from Great Lakes Carbon Company.
§Grade l5V P i t ch from Al l ied Chemical Company.
1lA sphe r i ca l carbon black from R. T. Vanderbilt Company.
*
463
IRRADIATION TESTING OF IMPROVED BONDED BEDS
We have completed an i r r ad ia t ion t e s t , HT-4, of the improved bonded beds i n the t a rge t region of HFIR. For t he experiment we 'used inject ion- bonded p a r t i c l e beds with e i the r grade 15V p i t ch or Varc.um as the binder. F i l l e r materials i n the p i t ch binder were e i ther 40 w t
o r 29 w t '$ Poco graphite plus 29 w t % Thermax carbon black.
29 w t % Poco graphite and 29 w t % Thermax combination was used with the
Varcum binder.
Poco graphi te
Only the
In t h i s experiment we used i n e r t pa r t i c l e s t h a t consisted of carbon
kernels coated with monolayer coatings deposited from propylene a t
1250°C.
increase the i r r ad ia t ion s t a b i l i t y of t he coatings and t o mimimize
s t r e s ses s e t up by d i f f e r e n t i a l thermal expansion of t h e carbon kernels
and monolayer coatings. The composition and heat treatment of the
various specimens a re given i n Table 1.
The coated pa r t i c l e s were annealed a t 2100°C before bonding t o
Capsule Assembly
The capsule assembly consisted of a s ingly contained uninstrumented
capsule with exter ior shape and dimensions bas ica l ly tha t of a t yp ica l t a rge t rod.
p a r t i c l e specimens were loaded in to the cen t r a l 20-in. length of t he capsule.
tu res a r e shown i n Fig. 5. held bonded beds and the loose p a r t i c l e magazine M - 4 were designed t o operate a t 1065°C.
magazines were designed t o operate a t 800°C. i r r ad ia t ed f o r th ree cycles i n the HFIR t a r g e t region.
obtained i n two previous t e s t s HT-1 and -3 i r r ad ia t ed f o r t he same period of time and i n t h e same t a rge t pos i t ion a re shown i n Fig. 6.
Graphite magazines containing the bonded bed and loose
The arrangement of t he magazines and t h e i r respective tempera-
The two center magazines CP-14 and -15 t h a t
The remaining bonded bed and loose coated p a r t i c l e
The capsule assembly w a s The fluences
Pos t i r rad ia t ion Evaluation
After i r r ad ia t ion and disassembly, a l l bonded beds were in t ac t and
could be handled in-ce l l .
i l l u s t r a t e d by the group of specimens shown i n Fig. 7 t h a t were i r rad ia ted
The typ ica l pos t i r rad ia t ion appearance i s
464
Table 1. Bonded P a r t i c l e Specimens f o r HT-4 Experiment
bVarcum 8251 (prepolymerized f u r f u r y l a l coho l from Varcum Chemical
Heated i n argon f o r 30 min.
Company) .
Company) p lus 29 w t % Thermax ( a s o f t s p h e r i c a l carbon black from R. T. Vanderbi l t Company).
C 29 w t $ Poco AXM (-4O-p-size g raph i t e f l o u r from Poco Carbon
dGrade l5V p i t c h ( c o a l t a r p i t c h from Al l i ed Chemical Company). e 40 w t % Poco AXM (-4O-p-size g raph i t e f1o.u- from Poco Carbon
Company).
a t 800°C t o a f luence as g r e a t as 6 X
dimensional changes t h a t occurred a t t h e low and high i r r a d i a t i o n tem-
pe ra tu res were -1.4 and -2.62%, r e spec t ive ly .
temperature t h e shrinkage increased wi th increas ing f luence; a t t h e high
i r r a d i a t i o n temperature t h e shrinkage seemed t o decrease wi th increas ing
f luence.
enced by t h e composition of t h e binder phase or p r e i r r a d i a t i o n hea t
t reatment .
neutrons/cm2. The average
A t t h e low i r r a d i a t i o n
A t e i t h e r temperature t h e shrinkage d id not seem t o be i n f l u -
465
20 m ACTIVE CORE
b P - 4 5 IOESIGN TEMP 4 0 6 5 T )
Fig. 4 . In jec t ion Device for Par t ic le Bonding Material.
NICKEL PINS, TYPE 304 STAINLESS
PYROLYTIC- STEEL, AN0 IRON CARBON FOX FLUX MNlTOR WIRES
MON1TOR.M-2 GRAPHITE fUPPER fEAL PLUG I M 4 HOLDERS-,
I 2 0 m ACTIVE CORE
-35 10 OVERALL
BOTTOM CAP ,ALL!ANUM CAPSULE WALL
,800 T
466
-8 - 4 0 4 8 12 2 -12 DISTANCE FROM CENTER
Fluences Obtained i n Two Previou:; HFIR Target Tests HT-1
LINE OF CAPSULE ( in . )
Fig . 6 . and -3. of the var ious HT-4 magazines a r e shown a t t h e bottom.
The d a t a represent the f luence obtained i n HT-4. The loca t ion
1 R-50105 !
i ' -1 4 ! INCHES
Fig. 7. Appearance of Bonded Beds of Coated Partic.Les Af te r I r r a d i a t i o n i n Capsule HT-4 t o Fluence of 6 X 1021 neutrons/cm2 a t 800°C.
467
We crushed about 25 p a r t i c l e s from each of the loose-par t ic le samples i r r ad ia t ed a t t h e low and high temperatures, and measured the
dens i t ies of the coating fragments i n a density gradient column. We
found t h a t t h e dens i t ies increased 4 and '7% a t t he low and high tempera-
t.ures: respect ively. The l i nea r shrinkage r a t e s corresponding t o these
d e m i t y changes would be about -1 and -2$, which i s i n agreement w i t h
observed shrinkage r a t e s f o r t h e bonded beds. Thus the shrinkage of the bonded beds seems t o be controlled by t h e behavior of the close-
packed p a r t i c l e s .
Metallography of two specimens with the higher loading of carbon
f i l l e r i n the matrix (29 wt $ Poco graphi te powder and 29 w t $ Thermax
carbon mixed with Varcum or grade 15V p i t ch ) revealed only one damaged
coating of more than I200 coated p a r t i c l e s examined i n the two specimens.
Both of these specimens were i r r ad ia t ed a t the higher temperature
(approx 1050°C).
s ive f i n e cracks t h a t had widened and extended, but it was otherwise
similar t o t h e unirradiated control samples as shown i n Fig. 8. The matrix was a l s o wel l bonded t o the p a r t i c l e coatings. The pitch-bonded matrix, on the other hand, showed fewer cracks and d i d not bond t i g h t l y t o the p a r t i c l e coatings. Comparison of the pre- and pos t i r rad ia t ion
microstructures i n Fig. 9 shows t h a t t h e pitch-bonded body i s r e l a t i v e l y unaffected by the high-temperature i r rad ia t ion . Metallography of two
id.entica1 specimens i r r ad ia t ed a t 800°C did not revea l any broken coatings and confirmed the observations c i t e d above. Thus only one
damaged coating was observed out of more than 2000 coated p a r t i c l e s
examined i n four specimens. Metallographic examination of two specimens
of t he t h i r d type (bonded with 40% Poco AXM graphi te i n p i t ch ) i s i n progress, but evidence from the macroscopic and dimensional examinations indicates t h a t l i t t l e o r no damage occurred i n these specimens e i the r .
The matrix of t he Varcum-bonded specimen showed exten-
DISCUSSION AND CONCLUSIONS
I
Although t h e coated p a r t i c l e s i n the HT-4 experiment had monolayer
I
I
coatings deposited over carbon microspheres, we believe t h a t they a re
bas i ca l ly l i k e those two-layer coatings (porous inner-LTI outer) t h a t I @
468
R-SMO7
Fig. 8. Microstructures of Bonded Beds with Varcum Binder Tested i n
The p a r t i c l e s a re 220-p-diam carbon micro- HFIR HT-4. 29 w t % Thermax carbon black. spheres coated with a 75-p-thick LTI monolaye:r coating. and ( b ) i r r a d i a t e d a t 1050°C t o 8 X lOoX. Reduced 18%.
The f i l l e r cons i s t s of 29 w t % Poco AXM graphi te flour and
( a ) Unirradiated, neut:rons/cm*. As polished,
469
R-50106 ~ -w
Fig. 9. Microstructures of Bonded Beds with Pi tch Binder Tested i n HFIR HT-4. 29 wt % Thermax carbon black. spheres coated w i t h a 75-p-thick LTI monolayer coating. and (b ) i r rad ia ted a t 1050°C t o 8 x lo2’ neutrons/cm2. Reduced 22.5$.
The f i l l e r cons is t s of 29 w t $J Poco AXM graphite f lou r and The pa r t i c l e s are 220-p-diam carbon micro-
(a ) Unirradiated, A s polished, 1OOX.
470
f a i l e d i n t h e two e a r l i e r HFIR t a r g e t experiments ( H T - 1 and -3).
carbon microspheres used as kerne ls were of low dens i ty and shrank exten-
s i v e l y during i r r a d i a t i o n , and t h i s shrinkage l e f t t h e monolayer coating
unrestrained. We be l ieve t h e improvement s t ems from the new matrix com-
pos i t ions , which have lower shrinkage r a t e s and do not bond so t i g h t l y
t o t h e p a r t i c l e coatings.
The
Thus t h e r e s u l t s of t h e HT-4 experiment demonstrate t h a t a bonded
bed can be fabr ica ted which w i l l withstand t h e peak temperature and
fluence of an HTGR.
new material , Poco graphi te flour, and were clnly 0.5 i n . long. Addi-
t i o n a l w o r k w i l l be required t o develop longer bodies with equivalent
s t ruc tu res using cheaper r a w mater ia l s and aLtomated f a b r i c a t i o n
processes.
The samples, however, were made with an expensive
It should be noted t h a t t h e bonded beds t e s t e d here d id not contain
f u e l o r coatings with S ic b a r r i e r l aye r s .
a r e much higher than i n an operating HTGR.
w i l l be required t o assess t h e e f f e c t s of t hese va r i ab le s .
Also, t h e neutron dose r a t e s
Pddi t iona l i r r a d i a t i o n s
ACKNOWLEDGMENTS
The authors would l i k e t o acknowledge t h e contrib.utions of
R. L. Hamner, who a s s i s t e d with t h e development of bonding techniques,
t o F. P. J e f f e r s and B. R. Chilcoat f o r t h e i r a s s i s t ance i n specimen
prepara t ion and charac te r iza t ion , and t o S. C!. Weaver, D. E . Rosson,
and W. W. Proaps, who a s s i s t e d with t h e design and assembly of t h e
capsules.
conducted by N. M. Atchley and E . L. Long, Jr..
Metallography of t h e i r r a d i a t e d ar!d con t ro l specimens was
REFERENCES
1. R. C . Dahlberg, R . F. Turner, and W. V. Goeddel, Fort S t . Vrain Nuclear Power S ta t ion ; Core Design Charac te r i s t ics , Nucl. Eng. I n t . - 14( 163), 1073-77 (1969).
2. J. M. Robbins and R . L. Hamner, Bonding of Coated Fuel P a r t i c l e s f o r Fuel Elements, pp. 16-24 i n GCRP Semiann. Progr. Rept. Mar. 31, 1967, OWL-4133.
471
@ 3. P. E. Reagan -- e t a l . , Evaluat ion of Coated me1 P a r t i c l e s Irradiated i n Sweep Capsules i n ORR P o s i t i o n s A9 and B9, pp. 3-7 i n GCRP Semiann. Progr . Rept. Sept . 30, 1968, ORNL-4353.
4. D. R. Cuneo, E. L. Long, Jr., J. H. Coobs, J. A. Conlin, and A. W. Longest, Performance o f Pyrolytic-Carbon-Coated U02 and UC;! Microspheres a t High Burnup, (Summary) Trans. Am. Nucl. SOC. - 12(2), 54849 (1969).
5. J. H. Coobs e t a l . , I r r a d i a t i o n of Loose and Bonded Coated P a r t i c l e s i n HFIR Target , pp. 28-47 i n GCRP Semiann. Progr . Rept. Sept . 30,
-- 1968, ORNL-4353.
6. J. H. Coobs -- e t a l . , I r r a d i a t i o n Experiments i n HFIR, pp. 11-41 i n GCR Semiann. Progr. Rept. Mar. 31, 1969, OWL-4424.
7. C . R. Kennedy, Graphi te I r r a d i a t i o n s i n HFIR, pp. 193-195 i n Metals and Ceramics Div. Ann. Progr . Rept. June 30, 1969, ORNL-4470.
472
DISCUSSION
C . B. von d e r Decken: I t was mentioned t h a t t h e bonding w i l l be
done i n s i d e t h e f u e l e lement b lock and t h a t some c r a c k i n g may occur . Has
such an arrangement been i r r a d i a t e d up t o now?
J . L. S c o t t : N o .
L. W . Graham: What were t h e d imens iona l changes observed i n t h e
Poco-type bonded beds and how s i g n i f i c a n t a r e t h e s e w i t h r e s p e c t t o t h e
f u e l o p e r a t i n g tempera ture i n a power r e a c t o r ?
J . L. S c o t t : The beds which were exposed t o t h e h i g h e s t f l u e n c e and
tempera ture showed a l i n e a r s h r i n k a g e of 2 .8 p e r c e n t . The maximum f i s s i o n
r a t e o c c u r s w i t h a f r e s h f u e l b lock and t h e power d e n s i t y d e c r e a s e s a s t h e
exposure i n c r e a s e s . By t h e t i m e t h e d imens iona l changes become s i g n i f i -
c a n t , t h e h e a t g e n e r a t i o n r a t e s a r e enough lower t h a t t h e tempera ture i s
a l s o lower i n s p i t e of t h e h i g h e r thermal r e s i s t a n c e .
M. D a l l e Donne: I f I have r i g h t l y understood, t h e advantage of
u s i n g a bonded bed i s t o i n c r e a s e t h e thermal c o n d u c t i v i t y . However,
you have l a r g e c r a c k i n g i n t h e m a t r i x s o t h a t t h e i n c r e a s e i n c o n d u c t i v i t y
could be lower t h a n what you would e x p e c t . D o you n o t f i n d t h a t a l o o s e
bed, w i t h a t h i r d p a r t i c l e of s m a l l e r d i a m e t e r (100 micron o r so) t o g e t h e r
w i t h t h e o t h e r two e n v i s i o n e d , could have roughly t h e same c o n d u c t i v i t y
w i t h t h e advantage of having a h i g h e r f u e l d e n s i t y ?
J . L. S c o t t : The p r i n c i p a l reason f o r u s i n g bonded beds i s f o r
s a f e t y , b u t t h e r e a r e h e a t t r a n s f e r advantages a s w e l l . Even though t h e
m a t r i c e s a r e badly cracked,we e x p e c t t h e bed c o n d u c t i v i t y t o be two t o
f o u r times h i g h e r t h a n a bed of l o o s e p a r t i c l e s . For a g iven power d e n s i t y
t h e thermal g r a d i e n t a c r o s s a bed of p a r t i c l e s would be one-half t o one-
f o u r t h t h a t of a l o o s e bed. This would d e c r e a s e t h e change of t h e Amoeba
e f f e c t .
The p a r t i c l e d i a m e t e r s i n p r e s e n t HTGR d e s i g n s a r e 600 microns and
400 microns f o r t h e f e r t i l e and f i s s i l e p a r t i c l e s , r e s p e c t i v e l y . To
markedly i n c r e a s e t h e p a r t i c l e d e n s i t y , a t h i r d p a r t i c l e would have t o be
less t h a n 40 microns i n d iameter . T h i s i s below t h e l i m i t of a u s a b l e
c o a t e d f u e l p a r t i c l e .
473
D. D. Tytga t : 1. To what e x t e n t has t h e Oak Ridge Na t iona l Labora-
t o r y Programme on bonded coa ted p a r t i c l e s included t h e m a t e r i a l s used by
Gulf General Atomic? 2 . I f t h e sepa ra t ion of f e r t i l e and f i s s i l e mater-
i a l s i n Gulf General Atomic f u e l e lements i s obta ined by t h e presence of
a S i c l a y e r dur ing t h e burning r ep rocess ing opera t ion , and no t by a p a r t i -
c le s i z e e f f e c t , why no t adopt t h e same diameter f o r both p a r t i c l e s ? This
would h e l p t h e loading of f u e l e lements .
J . L. S c o t t : 1. Both Oak Ridge Nat iona l Laboratory and Gulf Gen-
e r a l Atomic have t e s t e d bonded beds wi th n a t u r a l g r a p h i t e f i l l e r s and both
use p i t c h b inders . Gulf General Atomic has no t t e s t e d Poco g r a p h i t e be-
cause of i t s high c o s t . 2 . Because of much h igher f i s s i o n d e n s i t y - a n d
burnups i n f i s s i l e p a r t i c l e s , i t i s necessary t h a t they be smal le r than
t h e f e r t i l e p a r t i c l e s f o r h e a t t r a n s f e r reasons .
J. Bugl: So f a r i r r a d i a t i o n t e s t i n g was performed a t 105OOC. D o
you f o r e s e e i r r a d i a t i o n a t temperatures above 1O5O0C?
J . L. S c o t t : Because of t h e high thermal f l u x i n t h e H F I R r e a c t o r ,
f i s s i l e m a t e r i a l burns-out qu ick ly . I n o rde r t o avoid l a r g e temperature
changes, w e depend p r imar i ly on gamma hea t ing f o r our tes ts . When gamma
h e a t a lone i s used, a convenient maximum temperature i s 105OOC. W e
could achieve h igh temperatures i f w e added a f i s s i l e p lus a f e r t i l e
m a t e r i a l combination which would y i e l d a cons t an t f i s s i o n i n g r a t e .
Paper 3/102 THE DESIGN OF PRISMATIC HIGH TEMPERATURE REACTOR FUEL ELEMENTS
- .-.YCllltL->X r '~ _".e - ' - - - I * - * - w ~ t k - * * * -
E. Smith OECD Dragon Pr0jec.t
ABSTRACT
I n t h i s r e p o r t fou r designs of p r i s m a t k f u e l p in s u i t a b l e f o r use i n HTR power r e a c t o r s a r e descr ibed and t h e i r r e l a t i v e thermal per- formance i n a f u l l 8 and continuously gagged ,core with a gas o u t l e t temperature of 800 C i s compared.
The stresses a r i s i n g i n f u e l p ins are descr ibed and the nature of t he change i n these stresses during i r r a d i a t i o n i s discussed. At ten t ion i s drawn t o t h e importance of t h e ma te r i a l p rope r t i e s and t h e i r v a r i a t i o n with i r r a d i a t i o n dose and p a r t i c u l a r l y t o the need f o r def in ing t h e p rope r t i e s of t he f u e l matrix.
INTRODUCTION
Present power r e a c t o r designs based on the HTR concept and using
pr i smat ic f u e l elements envisage a core cons t ruc t ion cons i s t ing of
stacked moderator blocks incorpora t ing more (2r less evenly spaced
coolant channels wi th in which t h e f u e l l e d p ins are located and
supported. The moderator blocks, toge ther with t h e i r charges of f u e l
pins , are designed t o be handled i n t o and o u t of t h e core by the f u e l
handling machinery and t h i s opera t ion may be c a r r i e d ou t e i t h e r on-load
o r off-load according t o the d e t a i l e d design of t h e reac tor . A s a
r e s u l t it i s c l e a r t h a t i n t h i s concept t he residence t i m e of t he
moderator i n t h e core i s the same a s t h a t of t h e fue l . The maximum
c ross sec t iona l dimensions of t h e block are la rge ly d i c t a t e d by t h e
s i z e of ava i l ab le ma te r i a l of t h e prefer red spec i f i ca t ion , bu t may be
modified by handling requirements and the u l t ima te choice of coolant
channel dimensions. Cross sec t iona l shape, ,and prefer red p i t c h o r
spacing of t he channels taken toge ther with cons idera t ions of t h e
l i k e l y inf luence of carbon t o uranium r a t i o wi th in t h e core f u r t h e r
in f luence t h e o v e r a l l design which must a l s o take account of t h e
allowable inter-channel ligament dimensions having due regard t o
474
475
0 manufacturing to l e rances and opera t iona l stress l imi t a t ions . Within
t h e coolan t channels t h e f u e l p in design l i m i t s a r e l a rge ly thermal,
c l e a r l y t h a t design which r e s u l t s i n t h e lowest peak f u e l temperature
and temperature grad ien t f o r a given core pressure drop must be the
d e s i r a b l e t a r g e t , f o r on t h e one hand core power d e n s i t i e s are
maximised and on t h e o the r o v e r a l l r e a c t o r c o s t s a r e minimised. The
f i n a l design optimum w i l l , however, depend on the r e l a t i v e e f f e c t s of
core power dens i ty and core pressure drop on o v e r a l l generat ing c o s t s
and t h e in te r -p lay of l i m i t a t i o n s such a s t h e minimum d e s i r a b l e
th ickness of graphi te sheaths and f u e l bed. It i s the purpose of t h i s
r e p o r t t o examine the r e l a t i v e m e r i t s of var ious f u e l p in designs
aga ins t such a background.
DESCRIPTION OF FUEL PIN DESIGNS
General Descr ipt ion
Current ly t h r e e b a s i c forms of pr i smat ic f u e l p in designs may be
i d e n t i f i e d . They a r e t h e hollow rod, t h e tubular non-interacting rod
and the tubu la r i n t e r a c t i n g rod designs. The hollow rod i s cooled a t
i t s e x t e r i o r sur face only while a l l tubular designs are cooled both
i n t e r n a l l y and ex terna l ly . The tubular non-interacting rod concept i s
f u r t h e r def ined i n two designs; one with s o l i d c y l i n d r i c a l f u e l
compacts incorporated i n t o a tubular t e l e d i a l pin, whi l s t t h e second makes use of unres t ra ined annular compacts wi th in the double wall of
a tubular pin. These designs a r e i l l u s t r a t e d not iona l ly i n Fig. 1.
A s t he names imply, t he i n t e r a c t i n g design allows t h e f u e l body t o
i n t e r a c t with one of i t s containing g raph i t e wa l l s wh i l s t i n t he non-
i n t e r a c t i n g design t h i s r e s t r a i n t i s avoided e i t h e r by incorpora t ing
s u f f i c i e n t l y l a r g e gaps between t h e f u e l and i t s containing wal l s o r
by an inherent feature of t he design i tself as i n t h e t e l e d i a l and
hollow rod concepts.
The e x i s t i n g prefer red proposals f o r a l l t hese designs incorpora te
t h r e e o r fou r equal ly spaced f u l l l ength r i b s i n t e g r a l with t h e
e x t e r i o r sur face f o r c e n t r a l i s a t i o n and loca t ion of t he f u e l p ins
wi th in t h e coolant channel. Axial alignment of t h e r i b s of ad jacent
476
f u e l p ins may be achieved by recess ing one of t h e r i b s i n t o a su i t ab ly
machined s lo t i n t h e coolan t channel wal-1 o r by a keying f e a t u r e
between mating end caps o r tubes.
being considered i n which c e n t r a l i s a t i o n of the f u e l p in i n t h e channel
i s maintained only a t t he extremities of t h e p in , t h e ex te rna l r i b s are
omitted and bowing i s allowed t o occur f r e e l y with the ob jec t of
reducing those Stresses assoc ia ted with t h e r e s t r a i n t of t h e f u e l p ins
by t h e i r i n t e r a c t i o n with t h e wa l l s of t h e channel.
such a proposal i s a t t r a c t i v e s ince it can be shown t h a t the thermal
and i r r a d i a t i o n induced effects lead u l t ima te ly t o a stable configura-
t i o n of t he p in wi th in the channel.
be adversely a f f ec t ed and t h e at ta inment of t h e prime ob jec t ive
(absence of bowing stresses) w i l l depend u l t ima te ly on the degree of
bowing t o be expected i n t h e most adverse cases of c ros s p in f a s t
neutron f l u x and thermal g rad ien t s and the pin/channel r a d i a l clearance.
I n a l l designs it i s the P r o j e c t ' s recommendation t h a t t he average
ou te r g raph i t e w a l l th ickness should not be less than 5 mm t o provide
adequate s t r eng th and robustness after taking due account of l i k e l y
corrosion effects and t o provide an add i t iona l s i g n i f i c a n t delay and
hold-up of f i s s i o n products i n t h e unl ike ly event of f u e l failure.
Al t e rna t ive proposals exist and are
Theore t ica l ly
However peak f u e l temperatures may
A s l i g h t l y th inne r w a l l can be accepted f o r t h e i n t e r n a l coolant
passage of t he tubu la r designs and here t h e recommendation i s a minimum
th ickness of 4 mm. The l igaments between f u e l ho le s i n t h e t e l e d i a l
can be th inner s t i l l , t h e m i n i m u m th ickness probably being d i c t a t e d by
graphi te machining l imi t a t ions .
Tubular des igns may r equ i r e mating f e a t u r e s t o l i m i t c ros s channel
coolant flow, t h i s f e a t u r e t akes t h e form of a simple free f i t
sp igot ted j o i n t between end caps which a l s o serves t o maintain alignment
of t h e c e n t r a l channel.
The Hollow Rod
The hollow rod design c o n s i s t s of a hollow c y l i n d r i c a l g raphi te
rod, closed a t both ends, and housing a number of annular f u e l bodies
t o t a l l y unres t ra ined a t t h e i r i nne r rad ius , (i.e., no i n t e r n a l graphi te
477
0 wal l ) .
i n t e g r a l with t h e tube and one separa te end cap o r i t could have two
separa te end caps. (See Fig. 2.) There are no f u e l g raph i t e i n t e r -
ac t ions i n t h i s design b u t i nc reases i n t h e ex te rna l fue l /g raph i t e
sheath gap and decreasing thermal conduct ivi ty with i r r a d i a t i o n r e s u l t
i n peak f u e l temperatures a t about 4 of t h e res idence t i m e of t he rod
i n t h e core. It will be shown l a t e r t h a t , even without tak ing t h i s
e f f e c t i n t o account, t h e thermal performance of t he hollow rod design
i s inferior t o t h a t of t he tubular designs. The c e n t r a l void i n t h i s
design a l s o provides a low r e s i s t a n c e path f o r p a r a s i t i c coolan t f low
which w i l l occur i n some measure due t o t h e permeable charac te r of the
graphi te wal l s and may increase if t h e end cap s e a l becomes defec t ive .
Such f l o w , occurr ing over t h e h o t t e s t f a c e of t he f u e l body, may enhance cor ros ion of t h i s region; i t s l i k e l y e f f e c t s on f u e l behaviour
must t he re fo re r ece ive c a r e f u l considerat ion.
I n t h i s design t h e graphi te tube may have one closed end
The Tubular-Interact ing Rod
I n t h i s design t h e ou te r tubular graphi te sheath i s s i m i l a r t o
t h a t of t h e hollow rod design and a second separa te inner graphi te
s leeve designed t o " f loa t " between t h e end f i t t i n g s i s added. A s i n
t he hollow rod design one end f e a t u r e may be i n t e g r a l with the ou te r
graphi te tube o r both end caps may be separa te components (see Fig. 3 ) . The i n i t i a l gaps between f u e l body and graphi te w a l l s a r e only
s u f f i c i e n t t o a l low f o r manufacturing to l e rances and non-interact ion a t
e i t h e r f a c e i n going from cold t o peak opera t ing temperatures,
subsequent shrinkage of t he f u e l r e l a t i v e t o the graphi te wal l i s
allowed t o produce stresses wi th in the f u e l mat r ix and the i n t e r n a l
sheath. Clear ly i n t h i s concept i n t e r f a c e gap e f f e c t s are minimised
a t t h e expense of increased f u e l and inne r g raph i t e tube stresses. It
w i l l t he re fo re be necessary t o demonstrate t h a t ne i the r the f u e l nor
t h e f u e l s leeve " f a i l " due t o t h i s i n t e r a c t i o n before such a proposal
can be f u l l y acceptable. It must a l s o be observed t h a t t h e i n t e r a c t i o n
stresses w i l l be a t t h e i r maximum i f a coolant f a i l u r e i n c i d e n t should
coincide with t h a t period of i r r a d i a t i o n i n which the equi l ibr ium
i n t e r a c t i o n stresses a r e a t a peak value (see Sect ion 4).
478
The Tubular Non-Interacting Rod (Annular Fuel)
The non-interacting f u e l rod design incorpora t ing hollow
c y l i n d r i c a l f u e l compacts i s very s imi l a r t o the i n t e r a c t i n g design.
I n t h i s design inner and ou te r graphi te wal l s and one end f e a t u r e may
be i n t e g r a l and one separa te end cap i s provided (see Fig. 4). It w i l l
be shown l a t e r t h a t t h i s design has a thermal performance intermediate
between t h a t of t h e hollow rod and t h a t of t h e tubular i n t e r a c t i n g
design. Design a spec t s r equ i r ing c a r e f u l a t t e n t i o n i n t h i s concept are:
(i) t h a t t he i n i t i a l gaps must be computed c o r r e c t l y t o avoid i n t e r -
ac t ions without too high a thermal penal ty , this r equ i r e s
reliable shrinkage da ta f o r t he g raph i t e and f u e l body over t h e
whole temperature and dose range.
(ii) t h a t , s ince the heat d i v i s i o n between inne r and ou te r channels
changes continuously with t i m e , it i s necessary t o examine i n
d e t a i l , t he thermal, mechanical (s t ress) , and g raph i t e cor ros ion
performance of t h e design over t he f u l l l i f e t i m e of t h e f u e l rod
i n t h e r eac to r core.
T h e Tubular Te led ia l Rod
The t e l e d i a l f u e l rod design has a l l t he thermal b e n e f i t s
assoc ia ted with the use of both inner and ou te r cool ing, the f u e l does
not i n t e r a c t with i t s containing g raph i t e w a l l s and gap growth has
only a l imi ted e f f e c t on thermal performance due t o the smaller
dimensions of t he f u e l body. Bas ica l ly the design c o n s i s t s of a t h i c k
walled cy l inder with evenly spaced f u e l l e d ho le s wi th in t h e wall. The
f u e l l e d holes , which may be d r i l l e d from both ends of t h e cy l inder ,
are closed a t both ends by g raph i t e end caps. (See Fig. 5.)
I n c o n t r a s t t o t h e annular f u e l non-interact ing design, i nne r and
outer channel performance i s not a f f ec t ed by i r r a d i a t i o n shrinkage.
By comparison with t h e o the r f u e l p in designs thermal computation i s
more complicated, s t r i c t l y r equ i r ing a two-dimensional ana lys i s
combined with a x i a l (channel) i n t e g r a t i o n , though t h e present evidence
from l imi ted electrical analogue experiments and two-dimensional A
479
ca lcu la t ions shows t h a t a su i tab le annular model can be chosen which
p r e d i c t s peak f u e l temperatures agreeing wi th in about 10 C. Manu-
f a c t u r i n g c o s t s f o r t h i s design are a l s o expected t o b e somewhat
higher and f o r t he same f u e l space t h e f low a r e a i n a given channel
i s smaller than t h a t of t he o the r t ubu la r des igns r e s u l t i n g i n a
r e l a t i v e l y g r e a t e r core pressure drop.
t he thermal performance of t h e t e l e d i a l i s only s l i g h t l y inferior to
t h a t of t h e tubular i n t e r a c t i n g design, b e t t e r than t h a t of t he
tubular non-interact ing design and markedly super ior t o t h a t of the
hollow rod design.
concept t o the stresses a r i s i n g i n the rod due t o the presence of
connecting l igaments between t h e inne r and ou te r graphi te walls.
0
It will be shown l a t e r t h a t
Careful cons idera t ion must be given i n this
E L A T I V E THERMAL PERFORMANCE OF FUEL PINS
Comparison i n Fixed Channel G e o m e t r y
For a r igorous and t r u e comparison of t he r e l a t i v e m e r i t s of t h e
var ious HTR f u e l p i n designs descr ibed i n t h e previous paragraphs i t
would be necessary t o optimise t h e physical and thermal design of a
power r e a c t o r f o r each proposal using i d e n t i c a l l i m i t a t i o n s with
regard t o m a x i m u m f u e l and graphi te sur face temperatures ( t ak ing
proper account of time-temperature h i s t o r y ) and u l t ima te ly comparing
the o v e r a l l generat ing c o s t of each design. method of comparison cannot be pursued i n t h i s repor t . However, it i s
considered t h a t t h e r e l a t i v e thermal performance of each design can be
i l l u s t r a t e d as follows: a series of r e a c t o r des igns i s assumed, i n
each of which t h e core i s f u l l y and continuously gagged t o g ive a
channel gas exi t temperature of 800 C for a coolan t gas i n l e t tempera-
t u r e of 30OoC. A f ixed channel diameter of 68 mm with a corresponding
equiva len t channel p i t c h fo r t h e core a s a whole of 95 mm, and an
a c t i v e core he igh t t o diameter r a t i o of 0.655 w a s assumed throughout.
The dimensions of channel diameter and p i t ch , toge ther with the
he igh t t o diameter r a t i o of t h e core are used t o determine t h e a c t i v e
For obvious reasons t h i s
0
480
core he igh t ( H ) f o r each case from t h e expression:
2 J - 7 P 2 2 H =- e C (%d e ')
where :
P = Tota l r e a c t o r thermal power (1,500 MW) r
Pc = Mean channel power (MW)
Rhd = Height t o diameter r a t i o
p = Mean channel p i t ch
(0.655)
I d e n t i c a l hea t t r a n s f e r c o r r e l a t i o n s and ma te r i a l p rope r t i e s w e r e used
i n making the ana lys i s which f u r t h e r assumed a channel a x i a l peak t o mean power of 1.20, and a m a x i m u m r a d i a l power f a c t o r of 1.20 f o r a l l
designs, b u t i n i t i a l . age f a c t o r s of 1.15, 1-20 and 1.23 f o r the hollow
rod, tubular (non-interact ing and i n t e r a c t i n g ) rod and t h e t e l e d i a l
respec t ive ly . The b a s i s f o r t h e f u e l space design w a s a hollow rod
f u e l compact with 42 mm O.D. and 25.4 mm I.D<., the c ros s sec t iona l
f u e l a rea i n the hollow rod and tubular desiqns w e r e then assumed t o
be equal and constant. Some depar ture from t h i s cons tan t value of
f u e l space w a s necessary f o r t he first (9-ho:Le) t e l e d i a l design
ana lys i s i n t h i s r e p o r t f o r which a f u e l l e d a rea equal t o 0.804 of
t h a t of t h e hollow rod was assumed. For cons tan t heavy metal dens i ty
t h i s has the effect of i nc reas ing t h e carbon t o uranium atom r a t i o i n
otherwise i d e n t i c a l co res and r e s u l t s i n t h e higher age f a c t o r s
a l ready assumed. A l t e rna t ive ly , t o ob ta in similar carbon t o uranium
atom r a t i o s and hence age f a c t o r i n the te lec l ia l element e i t h e r t h e
heavy metal dens i ty i n t h e f u e l o r t h e f u e l l e d c ros s sec t ion could be
increased by about 20%.
t he core and u l t ima te ly on any assoc ia ted c o s t penal ty a r e amenable t o
ca lcu la t ion .
240 and 295 f o r t h e hollow rod, tubular rods with annular f u e l s , and
t h e t e l e d i a l respec t ive ly .
The more general eff-ects on t h e physics of
Typical N /N r a t i o s f o r the designs discussed are 230, c . u
48 1
The r e s u l t s of t h i s series of ca l cu la t ions , which w e r e made only
f o r ' s ta r t of l i f e conditions' and therefore d id no1 take account of
worsening thermal performance due t o gap development, a r e presented
i n t h e graphs of Figs. 6 t o 9 which show t h e c h a r a c t e r i s t i c s of t h e
' var ious designs f o r a f ixed channel s i z e of 68 mm, t h e independent
va r i ab le i n these curves i s t h e peak channel power. The l imi t ing
fue l and surface temperatures of 1225 C and 1000 C chosen i n t h i s
comparison w e r e based on t h e expectation t h a t peak random tempera-
tures would be about 100°C t o 15OoC and 4OoC t o 8OoC g r e a t e r than
t h e peak nominal values f o r f u e l and graphi te surface respec t ive ly .
It should perhaps be observed t h a t random effects on f u e l temperature,
due f o r example t o fue l /graphi te s leeve gaps and e c c e n t r i c i t y , are
l i k e l y t o be a t t h e i r g r e a t e s t i n t h e hollow rod and tubular non-
i n t e r a c t i n g designs s ince t h e smaller dimensions of the t e l e d i a l and
b u i l t i n r e s t r a i n t of t h e tubular ( i n t e r a c t i n g ) design l i m i t these
effects. It w i l l be seen from t h e graphs t h a t , f o r t h e 68 m channel
f u e l temperature i s the l imi t ing f e a t u r e of a l l designs. A t t h i s
l i m i t t h e core power dens i ty , core pressure drop, peak channel power
and graphi te surface temperatures f o r t he various designs i n a 68 mm
channel are compared i n T a b l e 1.
0 0
Comphrison i n Typical Power Reactor Geometry
Following upon t h e general survey discussed above, a thermal
ana lys i s w a s made tak ing i n t o account dimensional and property changes
during l i f e f o r s p e c i f i c designs of hollow rod, tubular i n t e r a c t i n g
and non-interacting, and t e l e d i a l ( i n t h i s case an 8-hole design) f u e l
p ins i n a t y p i c a l power reac tor .
gagging i n a downflow core a t a coolant pressure of 55 a t m w a s assumed.
B e s t estimate nominal peak f u e l temperatures throughout l i f e w e r e
ca lcu la ted and systematic and random effects, computed separa te ly ,
w e r e added t o the nominal values t o ob ta in Peak systematic and Peak
Random temperatures.
included coolant leakage, hea t leakage, f u e l e c c e n t r i c i t y , gag
adjustment e r r o r and p in power tilt, while t he random effects allowed
f o r two standard devia t ions i n f u e l thickness, gap widths, tube
For a l l designs continuous on-load
The systematic effects taken i n t o account
482
thickness, coolant channel dimensions, e c c e n t r i c i t y , f u e l enrichment,
f u e l dens i ty , instrumentation e r r o r s (gag) , etc. The r e s u l t s of t h i s
survey i n terms of peak f u e l temperature are given i n T a b l e 2.
It i s a conclusion of t h i s p a r t of t he review t h a t from the purely
thermal performance viewpoint t h e tubular elements are a l l g rea t ly
superior t o t h e hollow rod and t h a t t h e tubu:Lar i n t e r a c t i n g design i s
the b e s t of t h e tubular designs.
THE MECHANICAL BEHAVIOUR OF FUEL PINS
The stresses a r i s i n g i n fue l element p i n s may be grouped
conveniently under f o u r headings:
(a ) Membrane stresses i n t h e body of t h e f u e l tubes.
(b ) I n t e r a c t i o n stresses between the p in and i t s boundary w a l l due t o
bowing effects.
(c) I n t e r a c t i o n stresses, i f any, between the f u e l body and i t s boundaries ( t h e f u e l tube wal l s ) .
( d ) Discontinuity stresses a t the ends of t h e pin.
A l l t he se stresses are dependent upon the temperature and f a s t
f l u x gradien ts e x i s t i n g i n t h e components, arid the mater ia l properties.
O f these l a t t e r t h e most important appear t o be shrinkage, coe f f i c i en t
of thermal expansion and the e l a s t i c modulus.
proper understanding of the behaviour of f u e l p ins and t o avoid se r ious
e r r o r t h a t t h e method of ana lys i s should take due account of t h e
v a r i a t i o n of these p rope r t i e s with i r r a d i a t i c , n dose and temperature.
It i s important, f o r a
Within t h e Pro jec t a n a l y t i c a l methods have been developed f o r
es t imat ing the membrane stresses ( a ) and i n t e r a c t i o n stresses (c ) a s
dose dependent func t ions , whereas e x i s t i n g methods f o r t h e i n t e r a c t i o n
stresses ( b ) and the d i scon t inu i ty stresses (d ) are s t i l l under
development.
due t o ( a ) and ( c ) are reached i n t h e dose range 4 t o 8 x lo2' E.D.N.
and w e could expect d i scont inui ty stresses t o behave s imi la r ly .
I n t e r a c t i o n stresses due t o t h e bending of tht2 p in within the coolant
P ro jec t work so f a r has ind ica ted t h a t peak stresses
483
channel may however, be expected t o reach t h e i r peak values a t doses
which w i l l be dependent on i n i t i a l clearances and t h i s dose may o r may
not be i n t h e same range. For some design proposals, f o r example f u e l
p ins without ex te rna l r i b s , i n t e r a c t i o n with the channel wal l s may be
e n t i r e l y absent.
elements f o r use i n the Dragon core none of t h e stresses, ( a ) , (c) o r
( d ) occurring i n the f u e l tubes appear t o give cause f o r concern;
peak t e n s i l e stresses of about 700 p s i , under shu t down conditions and
after operation f o r about 100 days o r more, being t y p i c a l f o r p in
designs not very d i s s imi l a r t o t h e power r eac to r concepts.
o the r hand i n t e r a c t i o n due t o bending (b) can apparently lead t o
r e l a t i v e l y high stresses i f t h e temperature grad ien t and/or f a s t
f l u x gradien ts are s u f f i c i e n t l y la rge , wh i l s t t h e predicted stress (c)
i n t h e f u e l matrix f o r one i n t e r a c t i n g design studied, suggests t h a t
"failure" of t h e matrix might be expected even i n normal service.
Accident conditions such as loss of coolant w i l l r e s u l t i n increased
i n t e r a c t i o n stresses of t h i s type due t o the f l a t t e n i n g of temperature
g rad ien t s between f u e l and graphi te sleeve.
From t h e ca l cu la t ions made so f a r i n support of t es t
On the
With re ference t o the l i k e l y "failure" of the f u e l matrix, it i s
t h e P r o j e c t ' s present opinion t h a t such f a i l u r e w i l l occur e n t i r e l y
wi th in t h e matrix material and t h a t it i s unl ike ly t o produce
s i g n i f i c a n t effects leading t o f u e l par t ic le fa i lure with enhanced
f i s s i o n product release. subjec t of tests t o be ca r r i ed ou t by Dragon and must be pos i t i ve ly
proved before f u l l advantage can be taken of it i n p in design, (i.e.,
i n t e r a c t i n g tubular designs).
This l a t t e r poin t w i l l of course be t h e
The predicted v a r i a t i o n i n t y p i c a l membrane ( a ) and i n t e r a c t i o n
stresses (c) as a func t ion of dose are presented i n Figs. 10 and 11.
Most of t he effects giving rise t o stresses i n t h e f u e l p ins are
common t o a l l designs.
i n t e r a c t i n g tubular design have already been discussed.
design introduces one more addi t iona l effect due t o t h e presence of
t h e ligaments between t h e f u e l l e d holes.
The add i t iona l effects appearing i n the
The t e l e d i a l
I n the ligament reg ion t h e
484
graphi te i s h o t t e r than e i t h e r of t he boundary w a l l s , so t h a t i n i t i a l
thermal effects w i l l g ive r ise t o increased stresses i n the w a l l s ,
t e n s i l e a t t h e ou te r wal l and compressive i n t h e ligament and inner
wall. Subsequent i r r a d i a t i o n induced shrinkage and a r eve r sa l of the
thermal effects a t shut down a f t e r creep r e l3xa t ion effects have been
taken i n t o account, u l t ima te ly r e s u l t i n t e n s i l e f o r c e s i n t h e ligament
reg ion with corresponding compressive stresses i n t h e ou te r boundary
wal l and t e n s i l e stresses i n t h e inne r wall. An i n i t i a l ca l cu la t ion
of these effects suggests t h a t t he stresses ,a r i s ing w i l l be wi th in the
acceptable l i m i t s .
Future r e a c t o r systems w i l l be c a l l e d upon t o fol low load demands
as f u l l y a s possible. Such a requirement toge ther with the small
v a r i a t i o n s i n power inhe ren t i n generat ing a id supply networks impose
c y c l i c stresses on the r e a c t o r components, p a r t i c u l a r l y t h e f u e l
element p ins of t he r e a c t o r core. Wherever :such c y c l i c e f f e c t s may
be imposed it i s i n e v i t a b l e t h a t t h e f a t i g u e performance of the
materials d i r e c t l y involved are questioned and it becomes necessary t o
r e l a t e f a t i g u e performance t o allowable stre:;s l eve l s .
Typically, stresses i n f u e l p ins during steady state opera t ion a t
f u l l power a r e q u i t e modest, about 5% t o 15% of t h e u l t ima te s t r eng th
of t he mater ia l , w h i l s t shu t down (peak) stresses are normally about
50% of the u l t ima te s t r eng th and could rise i n some designs t o about
70% o r so of t he u l t ima te s t rength. Cycl ic power v a r i a t i o n s can then
be expected t o produce stress changes equal to t he product of the
f r a c t i o n a l power change and t h e d i f f e rence between the peak ( s h u t down)
stress and t h e opera t ing stress.
Various types of f a t i g u e test on r ep resen ta t ive graphi te specimens
have been c a r r i e d out by Sud-Aviation on behalf of Dragon Project.
These tests took t h e form of bend tests with a stress v a r i a t i o n
imposed upon a non-zero mean stress.
The r e s u l t s a r e p l o t t e d i n the Goodman t:ype p l o t shown i n Fig. 12 ,
i n which the o rd ina te i s t h e r a t i o of stress amplitude o r range t o
u l t ima te s t r eng th and t h e abscissae the r a t i o of mean stress t o
485
0 u l t ima te s t rength.
On t h e same f i g u r e the reg ion of opera t ion f o r t y p i c a l p in stresses
has been indicated.
a maximum of about 10
( r educ t ion ) should be expected i n t h e lifetime of a f u e l p in i n a
power reac tor .
Fig. 1 2 t h a t t he safe peak stress could conservat ively be as high as
0.7 of t h e u l t ima te s t r eng th of the mater ia l .
E l e c t r i c i t y supply u t i l i t i e s have ind ica ted that 6 power cyc les i n t h e range 1% t o 60% power
It may the re fo re be deduced from the da t a presented i n
Before leaving t h e subject of f u e l p in stresses i t i s important t o
re-emphasise t h a t s i g n i f i c a n t changes i n any of t h e material p rope r t i e s
could ma te r i a l ly a l t e r t he predicted values. For example a reduct ion
i n the creep c o e f f i c i e n t of t h e ma te r i a l s w i l l i nc rease t h e operat ing
stress l e v e l s pro ra ta and inc rease the dose requi red t o reach
m a x i m u m stress leve ls . I n t h i s context i t should be noted t h a t da t a
on t h e material p rope r t i e s of t he f u e l l e d mat r ix are a t t h i s t i m e
somewhat t e n t a t i v e and much work remains t o e s t a b l i s h shrinkage,
thermal expansion and e las t ic modulus data over t h e f u l l range of
temperature and dose. P a r t i c u l a r l y , creep d a t a on mat r ix f u e l s i s
non-existent and i n Dragon ca l cu la t ions t o da t e i t has been assumed
t h a t creep c o e f f i c i e n t s f o r t h e matrix are t h e same as those of
r ep resen ta t ive graphi tes .
CONCLUDING REMARKS
Limited improvements i n €uel element performance can be brought
about by c a r e f u l a t t e n t i o n eo t he r e l a t i v e importance of t h e var ious
ma te r i a l p roper t ies .
advantageous t o have b e t t e r thermal conduct ivi ty i n exchange f o r a
worsening i r r a d i a t i o n shrinkage. It would seem, however, t h a t t he
g r e a t e s t b e n e f i t i s t o be achieved by choosing t h a t f u e l p in which
combines t h e b e s t poss ib le thermal performance with t h e least number
of opera t iona l unknowns r equ i r ing l i f e tests i n t h e core of a reac tor .
O f t h e designs discussed i n this r e p o r t t h e t e l e d i a l and t o a lesser
extent t h e tubular non-interact ing f u e l p in concepts seem t o f a l l
n i ce ly i n t o t h i s category, wh i l s t t o take f u l l advantage of the b e t t e r
For example i n some design concepts i t may be
486
thermal performance of t h e tubular i n t e r a c t i n g design it w i l l be
necessary t o demonstrate i n f u l l l i f e tests t h a t t he i n t e r a c t i o n effects
between f u e l l e d matrix and graphi te sheath do not lead t o an
unacceptable d e t e r i o r a t i o n i n f u e l performanc:e.
The t e l e d i a l design i s only s l i g h t l y less superior i n thermal
performance ar,d w i l l r equ i r e f a r less in -p i l e t e s t i n g t o prove the
i n t e g r i t y of t h e f u e l containing body. The tubular non-interacting
design has a similar thermal performance bu t i t s optimum design w i l l
r e l y upon sure knowledge of t h e r e l a t i v e shrinkage of i t s component
p a r t s , g raphi te and f u e l body. This design may also suffer somewhat
from t h e t i m e dependent charac te r of t h e heat flow i n t o t h e inner and
ou te r channels.
r e l a t i v e l y poor thermal performance and l i k e t h e tubular non-
i n t e r a c t i n g design requires a r e l a t i v e l y p rec i se knowledge of t h e
dimensional changes t o be expected i n t h e f u e l body and graphi te
sheath i f allowable peak random temperatures are not t o be exceeded.
Manufacturing c o s t s , on t h e o the r hand, are Expected t o be l e a s t f o r
t h e hollow rod and t o increase f o r t h e tubulcr designs with t h e
t e l e d i a l as t h e most expensive.
toge ther i n optimised core designs before a f i n a l p i c t u r e of t h e
r e l a t i v e merits of t h e various designs can be obtained.
The hollow rod concept suffers p r inc ipa l ly from i t s
A l l these f z c t o r s must be brought
T a b l a 1. Comparison of t h e Designs i n a 68 rrun Channel (Nominal Peak Fuel Temperature = 1225 C)
( S t a r t of L i f e Conditions)
0
Core Power Core Pressure Peak Channel Peak Surface Density Drop Power Temperature Design Type
C
Hollow Rod 4.45 150 30 4 935
0 kW 2 w/m3 g/cm
Tubular (N.1 . ) 7.80 30 2 46 0 96 5
T e l e d i a l (9-hole 1
9.25 500
Tubular (I) 9.50 36 5
532
526
98 3
9 76
487
T a b l e 2. Comparison of Peak Fuel Temperatures During Life
Approx. Core Design Nominal Systematic Random Power Density
OC OC OC m/m3
Hollow Rod 1320 1400 1545 5
Teledial (8-hole) 1145 1170 1250 7
Tubular 1200 1225 1330 8 non-interacting
Tubular in te rac t ing
1170 1200 1295 9
I
3
I I. MATRIX FUEL COMPACT
2. W T E R GRAPHITE SLEEVE
3. GRAPHITE END CAP
2. The Hollow Fuel Rod
488
3
4
3. The Tubular ( I n t e r a c t i n g ) Fuel Rod
7
6.
4. The Tubular (Non-interacting) Fuel Rod
f
4
I. MATRIX FUEL cop*cI
1. M E R UUPlllTE SLEEVE
3. M E R UUpHm SLEEVE 4. GRlPWTE END CAP
I. MATRIX NEL CCUPACT
1. M E R GRAPHITE SLEEVE
3. GR*PHITE 9ODY 4.GRWMITE END CAP
I MATRIX FUEL COMPACT 1 GRAPHITE
SECTION A - A 3 GRAPHITE END CbP SECTION B-B
5. The Tubular (Teled ia l ) Fuel R A
FULLY GAGGED CHANNELS GAS Cllf 800°C ltO
I l O (
I sac
I SO(
“ lac
1000 Hollow Rod Charac te r i s t ics i n 68 mm Channel 1000
900
ooc
t””i a
IO0 , , I # I 304 nu I I I
200 300 400 500 0 PEAK POWER IN CHANNEL- nw
489
FULLY GAOGEO
900
1'O0 CHANNELS GAS EXIT BOO'C
c ,
I
I I I
400 500 500 800 300
PEAK POWER IN CHANNEL - k w
7. Tubular (Teledial) Characteristics in 68 mm Channel
/ FULLY GAGGW CHANNEL5 GAS EXIT 8OO'C
I 160 k u I
0 400 500 600 100 IO0
PSAK POWER IN CHANNEL - k u
8. Tubular (Non-interacting) Characteristics in 68 nun Channel
49 0
s -60 - t
FULLY GAGGED CHANNELS GA5 BXlT BOO’C
/
s -60-
600
.n f
400
Q
I I I 400 500 6.20 700
PEAK POWER IN C H A N N E L - K U
9. Tubular ( In te rac t ing) CharacLeri:.tics i n 68 mm Channel
m9 / c d
A59UMPTIONS
CONSTANT POWER ISOTROPIC GRAPHITE MATERIAL PROPERTIES VARYING WITH 00% THERMAL, IRRADIATION SHRINKAGE AN0 CREEP EFQCT5 INCLUDED
n 3 I-
OPERATING STRESS
O s -
TYPICAL AXIAL STRESSES IN OUTER SURVACE OF TUBE
w a I- .n
-40 SHUT- DOWN STRESS Y >
6 a
I I I I I 0 5 IO IS 10 25 j-0
DOSE (s IOLa) D.N.E
10. Variation of Membrane Stresses w i t n I r rad ia t ion Dose
A
n
49 1
0.8 O''[
/ I ox) I UTS. (%UT- DOWN)
MEAN STRESS ULTIMATE STRCUGTH
12. Limiting S t r e s s Amplitude as a Function of Mean St ress
PSSUMEO OPERATING TEMPERANRE 0 500 1000 IS00
-----___ AT pa
CIRCUMFERENTIAL FUEL -1r MATRIX STRESSES
IO 1s PO 25 5 I I I
DOSE ( ~1010) 0.E I I
- --,- --- ---
ul yl U a
0 0 5 10-
LIRCUMFERENTIAL GRAPHITE SLEEVE STRESES
I I I 1 1 5 IO IS LO 25
NEUTRON D05E N ( a 10"n cn-1) D.N.E.
Variat ion of I n t e r a c t i o n S t resses with I r r a d i a t i o n Dose 11.
AS1UMPTIONS VARIATIONS IN tT..E. WITH IRRADIATION NEGLECTED OPERATING TEMPERATURES ASSUMED 70 REMAIN CONSTANT MODULUS OF MATRIX
vt x MODULUS OF SLEEVE CREEP COEFF. OF MATRIX.
CREEP COEFF. OF SLEEVE
492
DISCUSSION
J. L. Scot t : Do you o r i f i c e the flow f o r the tubular in te rac t ing or
t e l e d i a l designs ?
E. Smith: Normally, no. Using the ca lca la t ion techniques avai lable
it i s possible t o obtain optimized geometries i n which e i t h e r the f u e l temperature o r the temperature difference between the inner and outer sur- faces i n tubular designs i s minimized. We have noted t h a t i n optimizing f o r minimum temperature differences the penalty on maximum f u e l tempera- ture i s usually q u i t e small, say about 1 0 ° C .
H. Giitmann: I should only l i k e t o answer the questions concerning our calculat ions of the age fac tors . They were deduced from the f i s s i o n cross sect ions applying an average spectrum over the whole i r r a d i a t i o n time. Irradiation-d.ependent disadvantage fac tors were taken i n t o account, We have not y e t performed superce l l calculat ions. Due t o t h i s there i s a c e r t a i n uncertainty i n our age fac tors , but comparisons with the age fac-
t o r s calculated by the consortia have not shown any inconsistency.
J. Scarborough: Have the Dragon f u e l design assessments proceeded t o t h e point of developing reasonable estimates of fabr ica t ion costs f o r each of t h e opt ional designs discussed, and i f so, could you comment on the r e l a t i v e cost of each?
E. Smith: The question on r e l a t i v e costs w i l l be answered more
f u l l y i n a paper t o be given by H. Gctmann of the Dragon Project (paper 6/134, Session V I ) .
assessed, b u t f o r t h e designs discussed i n t h e paper r e l a t i v e production costs do not have a l a r g e influence on overa l l generating costs which are much more influenced by var ia t ions i n allowable core power dens i t ies , carbon t o uranium r a t i o , heavy metal densi ty i n the fueled space, e tc .
However, I may say that r e l a t i v e costs have been
J. D. Thorn: Please explain the bas i s for s e l e c t i o n of l i n e a r sca le
for t h e various geometries, and comment on how fa r the comparisons drawn a r e a r b i t r a r i l y a f fec ted by the choice of scale . Obviously i f d i f f e r e n t s i z e s had been selected d i f f e r e n t answers would have been obtained.
493
E. Smith: I n the preliminary analysis mm f o r the channel s i z e was indeed somewhat
0 presented, the choice of 68 arb i t ra ry and somewhat d i f fe r -
ent quant i t ies would r e su l t fmm a different choice of scale. the analysis was carried fur ther and each of the designs was examined with respect t o thermal performance i n a var ie ty of scales i n which channel diameter and pitch were the principal variable, with a fixed core height- to-diameter ra t io . change the or ig ina l conclusion that tubular designs were far superior t o the hollow rod with the tubular interact ing design as best, closely followed by the te ledial . that the hollow rod would be be t t e r i n smaller channels and that teledial
would be more appropriately disposed i n somewhat larger channels.
However,
The resu l t s of t ha t more complete analysis d i d not
What the additional analysis d id indicate was
J. A. Robertson: I n tubular designs the s p l i t i n heat flow between inner and outer surfaces i s sensit ive t o assumptions about heat t ransfer between fue l rods and graphite containers. Where the s p l i t depends on calculation is it necessary to allow f o r larger uncertainty factors that of fse t apparent benefits of t h i s geometry?
E. Smith: We think not. While variations i n theoret ical assump- t ions appear t o change the inner and outer graphite temperatures there is no evidence of large effects on peak fue l temperature. f ident of our theoret ical prediction f o r the geometries but w i l l be back- ing the calculations up with observations from experiments now i n the
Dragon Reactor and by experiments proposed fo r further charges of the
core. It is, fo r example, our intention t o measure i n some experiments internal, external, and mixed gas e x i t temperatures, and to obtain cool- ant flow s p l i t data f o r additional out-of-pile tests on representative channels.
We a re f a i r l y con-
Paper 4/106
THE DEVELOPMENT AND PERFORMANCE OF HTR CORE MATERIALS ... .xyK
---B* -Ma.. - -- _ _ L. W. Graham
OECD Dragon P ro jec t
ABSTRACT
The cores of pr i smat ic High Temperature G a s Cooled Reactors are composed of structural graphi te f u e l blocks and tubes containing coated f u e l p a r t i c l e assemblies. p a r t i c l e i s described i n terms of t h e p o t e n t i a l sources of f i s s i o n product release together with t h e impl ica t ions of t h e choice of coatings and of chemical and s t r e s s i n g effects occuring during service. The reasons f o r favouring t h e incorporation of t h e f u e l p a r t i c l e s i n t o graphi te matrix compacts are discussed and da ta presented on dimensional changes experienced during i r r a d i a t i o n . For t h e s t r u c t u r a l g raphi te , t h e ava i l ab le commercial materials are adequate f o r t h e ea r ly launching of HTR power systems and t h e se rv ice conditions applying i n these r e a c t o r s o f f e r scope f o r fur ther improvements i n the economy of power production.
The design and performance of t h e coated
INTRODUCTION
The HTR may be viewed as p a r t of t h e l o g i c a l development of gas-
cooled r eac to r technology.
helium, coupled with a core cons t ruc t ion e n t i r e l y of r e f r ac to ry non-
me ta l l i c materials i s not only a t t r a c t i v e from t h e materials viewpoint
bu t l eads t o a design which i s inherent ly safe.
i n the United Kingdom i n t h e mid 1950's which r e s u l t e d i n a proposal
f o r a r eac to r experiment incorpora t ing these p r i n c i p l e s , t h e OECD Higk
Temperature Reactor Pro jec t , Dragon, w a s set up i n 1959. The t a sks of
the Pro jec t w e r e t o cons t ruc t and opera te a r e a c t o r experiment and t o
develop knowledge of t h e system t o such a po.int t h a t t h e Signatory
Countries could assess, design, bu i ld and opera te power producing H T R ' s
t o t h e i r own s p e c i f i c needs w i t h t h e m i n i m u m of addi t iona l research
and development.
The concept of t h e use of an i n e r t coolant,
Following i n i t i a l work
1
During t h e eleven yea r s which have passed s ince t h e formation of
t h e Pro jec t , core material development has passed through severa l
49 4
A
49 5
stages, ranging from those spec i f ica l ly aimed a t achieving successful
operation of t he Dragon Reactor itself through fue l and graphite
development fo r thorium cycle systems, and more recent ly , work specific-
a l l y geared t o the ear ly launching of power reactors u t i l i s i n g low-
enricheu uranium cycles. I n this paper no attempt w i l l be made t o
review each of these stages but the current s t a t e of knowledge relevant
t o power reactor performance w i l l be emphasised.
however, t h a t materials work on the HTR system has passed from
f e a s i b i l i t y s tudies t o the provision of data necessary f o r t he design
and construction of an economic power producing system.
It can be s ta ted ,
Three fac tors may be considered a s having been of paramount
importance i n the t r ans i t i on from the i n i t i a l concept t o engineering
r e a l i t y : t he convincing demonstration of t he use of helium as a
primary c i r c u i t coolant, given by the successful operation of t he Peach
Bottom, AVR and Dragon Reactors; t he development of fission-product-
re ta in ing coated p a r t i c l e fue l and the excellent behaviour of graphite
fue l elements a t high temperatures and high power densi t ies . H e l i u m
technology and core design are discussed elsewhere i n t h i s Symposium
and t h i s paper w i l l be confined t o f u e l and graphite.
COATED PARTICLE FUEL DEVELOPMENT AND PERFORMANCE
Concept
The function of t he coated p a r t i c l e i s t o generate heat whilst
re ta in ing f i s s ion products t o a degree t h a t ensures the safe operation
of a power reactor and permits maintenance of c i r c u i t components which
are subject t o f i s s ion product plate-out. The p a r t i c l e s consis t of
,
I i ~
I I
spherical f issi le or fe r t i l e kernels surrounded by coatings l a i d down
by pyrolysis i n f lu id ised beds.
composition have been developed and although most of t he exploratory
Kernels of both oxide and carbide
work by the Project was devoted t o the development of uranium thorium
dicarbide kernels, a decision w a s made i n 1966 t o concentrate on
uranium dioxide f o r t he exploi ta t ion of low-enriched cycle systems.
Since f i s s ion gives rise t o both a volume increase of t he kernel
material and t o gas re lease, space must be made avai lable within the
49 6
coated p a r t i c l e t o accommodate these effect2,.
favours building porosity i n t o the kernel apd current specif icat ions f o r
power reac tors lay down a nominal value of 20% . choice of coating materials has remained unchanged since the formula-
Accordingly the Project
2 The philosophy of t he
t ions made i n the ear ly 1960's and has been discussed by Huddle 2, 3 . The functions of the several coatings working outwards from the kernel
are b r i e f ly described below:
Pyrolytic carbon (PyC) buffer coatinq - t o a c t a s a catchment fo r
f i s s ion fragment r e c o i l from the kernel. Experience has shown t h a t t o
avoid disruption of this layer (spearhead a t tack) spec i f ic propert ies
of the coating are required and i n t h e case , D f f ue l of uranium dioxide
composition it i s required t h a t t he density ODf t he FyC be approximately
1 d u n . 3
Inner PyC coat inq - t h e f irst of t h e three coatings which make-up the
pa r t i c l e ' s pressure vessel. This again requires spec i f ic propert ies a s
shown la ter , t o m a x i m i s e the useful l i f e of t he p a r t i c l e i n the
environment of a fas t neutron f lux giving rise t o dimensional changes
and consequent s t ress ing.
t o gross diffusion of kernel born material which may a f f ec t t he
in t eg r i ty of t h e s i l i c o n carbide.
usual t o place a PyC sealing layer between the porous buffer and high
density inner PyC t o avoid uranium carbide formation during subsequent
coating operations.
I n addition, t h i s coating serves a s a ba r r i e r
W i t h u r a n i u m dioxide fue l it i s
Si l icon carbide coatinq - the main diffusion ba r r i e r t o metal l ic
f i s s i o n products.
mechanical performance of t h e p a r t i c l e and i n addition a c t s t o give
t h e p a r t i c l e dimensional s t a b i l i t y through i t s s t i f f n e s s and s t a b i l i t y
under neutron i r rad ia t ion .
This coating also plays a s ign i f icant r o l e i n the
O u t e r PyC coatinq - t he t h i r d m e m b e r of t h e ~ r e s s u r e vessel aiding i n
the mechanical performance of the p a r t i c l e but a lso providing chemical
protection fo r t h e s i l i c o n carbide.
497
Fig. 1 i l l u s t r a t e s t he swca l l ed Dragon Reference P a r t i c l e (800 p m kernel 155 p m t o t a l coating thickness) which has acted as a focal point
f o r t he development of low-enriched power reactor studies.
not be assumed, however, t h a t t h i s represents t he optimised p a r t i c l e
f o r t h i s system; it merely ac t s a s a reference and was defined a t a
par t icu lar point of core design development.
a p a r t i c l e used i n a power reactor w i l l be a compromise between the
ul t imate i n performance (small kernel, thick coating) and t h e
engineering and physics paramekers of core design which may tend t o
require maximisation of t he investment of heavy metal i n the fue l space
( l a rge kernel, t h i n coating). Power reac tors of t h e low-enriched
var ie ty now being designed require uranium investments i n the fue l
space i n the range 0.7-1.0 dun approximately 650-800 pm and coating thicknesses from approximately
130-180 pm f o r t he smaller kernel and 160-230 pm f o r t he l a r g e r .
It should
I n f a c t t he geometry of
3 leading t o kernel s i zes of
Fission Product Release Modes
I n considering f i s s ion product re lease i n HTR systems it should
be recognised t h a t a number of ba r r i e r s or delaying features exist
between t h e coated p a r t i c l e fue l and re lease i n t o the environment
i.e., diffusion through the fue l body, escape across the fue l body/
graphite f u e l sleeve gap, diffusion through and evaporation from the fue l sleeve and f i n a l l y plate-out phenomena. Some of these features
can be very powerful i n attenuating f i s s i o n product re lease from the
reactor even i n the presence of coated p a r t i c l e fuel f a i l u r e but they
are discussed elsewhere i n this Symposium.
Concerning the coated p a r t i c l e i tself f i s s i o n product re lease
may be broken down i n t o three poten t ia l sources:
(i) fue l contamination i n the coatings
(ii) diffusion of kernel-born products through the coatings
(iii) escape d i r e c t from the kernel through broken coatings.
498
Release from Contamination
During manufacture a low l e v e l of f u e l contamination occurs i n t h e
PyC coat ing. For t h e s i l i c o n carb ide type f u e l described, t h e only
contamination of importance i s t h a t i n t h e c u t e r PyC layer .
t h i s i s a t a l e v e l around 10 expressed a s a weight f r a c t i o n of f u e l
i n t h e kernel .
i r r a d i a t i o n experiments show t h a t r e l e a s e s of t h e order of 10 r e l e a s e
r a t e / b i r t h ra te (R/B) are observed f o r those spec ies with t h e longes t
ha l f l i v e s a s a r e s u l t of t h i s contamination, due t o t h e r e l a t i v e l y low
t r anspor t r a t e s i n py ro ly t i c carbon. The r e l e a s e of sho r t e r l i v e d
spec ies i s corresponding less due t o t h e delay i n t r anspor t through t h e
PyC.
r e l e a s e s a r e approximately one order of magnitude g r e a t e r , due, it i s
Typical ly -6
I n t h e case of noble gas f i s s i o n products many -7
I n t h e case of f u e l p a r t i c l e s embedded i n g raph i t e matr ices ,
thought, t o release from recoils i n t o t h e surrounding matr ix r a t h e r
than from PyC. For metallic f i s s i o n products t h e higher t r anspor t
r a t e s l ead t o r e l e a s e s which a r e approximately equal t o t h e contamina-
t i o n l eve l .
It can be s t a t e d , however, t h a t t hese l e v e l s of r e l e a s e s a r e of
no embarrassment t o r e a c t o r opera t ion and safeguards are provided by
appropr ia te qua l i t y con t ro l tests i n t h e f u e l production.
A
Release by Diffusion through Coatings
Transport of f i s s i o n products through t h e p a r t i c l e coa t ings i s a
complex phenomenon involving not only d i f f u s i o n i t s e l f bu t a l s o t h e
p a r t i t i o n c o e f f i c i e n t of t h e f i s s i o n product,s between kernel and PyC
coa t ing , between t h e PyC and S i c and f i n a l l y t h e r e l e a s e i n t o t h e
surrounding matrix. 4 Pro jec t by Walther . S i l i c o n carb ide was chosen a s t h e most s u i t a b l e
mater ia l t o se rve as t h e primary b a r r i e r t o m e t a l l i c f i s s i o n products
on t h e grounds t h a t i t was l i k e l y t o possess f a r lower pe rmeab i l i t i e s
t o t h e metals than t h e f l ake - l ike g raph i t e s lxuc tu re of py ro ly t i c
carbon. Fig. 2 i l l u s t r a t e s t h e powerful e f f e c t of a s i l i c o n carb ide
i n t e r l a y e r on t h e f r a c t i o n a l r e l e a s e a t equil.ibrium where t h e
d i f fus ion c o e f f i c i e n t i n t h e S i c i s 10
The system has been t r e a t e d t h e o r e t i c a l l y f o r t h e
4 lower than i n PyC. To provide
499
da ta f o r model ca l cu la t ions , f i s s i o n product t r anspor t i n S i c i s being
i n t e n s i v e l y inves t iga t ed by t h e P ro jec t i n both labora tory measurements
(by determining f i s s i o n product p r o f i l e s i n i r r a d i a t e d coated p a r t i c l e s )
and through t h e pos t - i r r ad ia t ion examination of l a r g e assembles of
coated p a r t i c l e f u e l l e d elements.
f i s s i o n product da t a from a l l experiments so f a r performed by t h e
P ro jec t has f a i l e d t o d e t e c t a r e l e a s e component due t o d i f fus ion
through t h e PyC/SiC/PyC type p a r t i c l e .
only w i t h PyC, however, s t ront ium i s found t o escape r e a d i l y a t t h e
higher opera t iona l temperatures as shown by t h e r e s u l t s given i n
T a b l e 1 f o r two f u e l elements, of a group of nine, i r r a d i a t e d i n t h e
Dragon Reactor f o r 280 f u l l power days. (Burn-up approximately 3.5%
FIMA). Companion experiments t o these having double t h e i r r a d i a t i o n t i m e
a r e being examined cu r ren t ly and it i s planned t o build-up even longer
i r r a d i a t i o n t i m e s i n elements remaining i n t h e Dragon core. I n summary
it may be s a i d t h a t f i s s i o n products release occuring as a r e s u l t of
t he d i f f u s i o n of kernel-born spec ies i s not l i k e l y t o be of major
concern i n currently-envisaged r e a c t o r designs where t h e res idence
t i m e may be of t h e order of 800-1,300 days.
Release from Defective Coatings
I n t h e l a t t e r case , ana lys i s of t h e
I n t h e case of par t ic les coated
From t h e previous sec t ions it i s apparent t h a t t h e f i s s i o n product r e l e a s e f r o m i n t a c t PyC/SiC/PyC coated p a r t i c l e s i s very low and i s not
expected t o con t ro l t h e s i t u a t i o n i n a power r eac to r . Breaching of t h e
coa t ings , however, can be expected t o l ead t o considerable inc reases i n
re lease .
noble gases , are commonly used t o monito;: t h e f u e l performance during
i r r a d i a t i o n experiments.
r e t e n t i o n i s afforded by t h e kernel when breaching of t h e coa t ings
occur. Fig. 3, however i l l u s t r a t e s t h e release of X e i so topes observed
when i n t a c t i r r a d i a t e d p a r t i c l e s of t h e Dragon Reference type containing
kerne ls of UO with 20% poros i ty a r e crushed a t room temperatures.
I n t h e s e experiments, performed f o r t h e P ro jec t a t SGAE, Seibersdorf ,
Vienna, it was found t h a t a t r e l a t i v e l y low burn-up (about 2% FIMA) t h e
These are indeed observed i n p r a c t i c e and, i n t h e case of i
It i s not y e t known i n d e t a i l what degree of
2
observed r e l e a s e w a s s t rongly dependent on temperature whereas a t t h e
500
higher burn-up of 6.5% FIMA t h e release was high and not very teiipera-
t u r e sens i t i ve .
It i s c l e a r l y of g rea t inportance, fnerI?fore, t o def ine t h e
performance l i m i t s of t h e coated p a r t i c l e f u e l i n t e r m s of t h e presence
of f u e l with " f a i l ed" coa t ings s ince it i s t h e f r a c t i o n of such f u e l
i n t h e r e a c t o r which w i l l d i c t a t e t h e magnitude of t h e f i s s i o n product
r e l e a s e source.
f u e l a s a r e s u l t of manufacturing opera t ions b u t t h i s question w i l l be
d e a l t with l a t e r .
Ruptured coa t ings can of course be present i n t h e f r e sh
Coating f a i l u r e s during se rv ice may be divided i n t o txo separa te
a reas although under some condi t ions of opera t ion there i s l i k e l y t o be
i n t e r a c t i o n between t h e two. The two a reas are f a i l u r e s which a r e
e s s e n t i a l l y chemical i n o r i g i n and those w h i c h are mechanical.
C h e m i c a l Failure.--This can occur a s a result : of an i n t e r a c t i o n between
t h e ma te r i a l s of t h e kernel and t h e coatings. , For t h e two main f u e l
types , oxides and carb ides , p o t e n t i a l mechanisms are r eac t ions between
oxygen re leased during t h e f i s s i o n process arid t h e coa t ings f o r t h e
former, and t h e mutual s o l u b i l i t y o r r e a c t i o n s between t h e carbide f u e l
and t h e coa t ings i n t h e l a t t e r .
between t h e PyC and t h e f u e l occurs a t very high temperatures b u t would
l ead t o excessive CO pressures lead ing t o mechanical f a i l u r e . The
temperatures a t which t h i s occurs , however, are considerably above
2000 C and a r e not r e s t r i c t i v e e i t h e r i n fue l manufacture o r i n t h e
opera t ion of r e a c t o r s being cu r ren t ly designed.
I n t h e case of U02, d i r e c t r e a c t i o n
0
A common f e a t u r e of t h e chemical d e t e r b r a t i o n of coated p a r t i c l e
f u e l s observed i n very high temperature irracmiations i s t h e so-called
ttamoeba e f f e c t " i n which t h e kernel moves through t h e coa t ing i n a
un id i r ec t iona l sense. This e f f e c t has been seen i n ea r ly carb ide f u e l s
i n Dragon i r r a d i a t i o n s and has a l s o been r epc r t ed by Goedde15 f o r
carb ide f u e l s .
g rad ien ts across t h e p a r t i c l e s during i r r a d i a t i o n and i n t h e case of
carb ide f u e l t h e d i r e c t i o n of movement i s up t h e temperature gradient .
During t h e l a s t t h r e e y e a r s a sirnilax phenomenon has been observed i n
The phenomenon i s c l e a r l y assoc ia ted with temperature
501
T a b l e 1. Comparison of Strontium Release i n S i c and PyC Coated Fuel P a r t i c l e s
Fract ional Release. a t Fuel Temperature
Fuel Type Isotope 1170-1240 900-1ooo 1040-1150 1160-1230
OC OC OC OC
PYC Sr-90 4.6 x 1.7 IO-* 1.4 x 9.1 loe3
PyC/SiC/PyC Sr-90 4.3 x 3.0 x 3.3 x 4.7 x
*Note Fract ional release measurements made by ana lys i s of graphi te f u e l s leeve surrounding f u e l during i r r a d i a t i o n .
T a b l e 2. Resul ts of Experiments on Amoeba Fa i lure i n UO Coated P a r t i c l e 'Fuel of Dragon Reference Design 2
I r r a d i a t i o n Times t o Onset of P a r t i c l e Surface Rating Estimated Cross
Fa i lure OC OC (days)
Temperature ( W / P a r t i c l e ) P a r t i c l e Gradient Ekp er irnent
Risd LEHPD2 (Denmark 1 1425
HTE (Dragon Reactor 1 1650
HTE (Dragon Reactor) 1725
HTE (Dragon Reactor) 1900
Studsvik 16/1 (Sweden 1 1650
0.68
0.26
0.26
0.26
1.4
250
125
5 0
125
280
140
85
85
8
10
502
UO
Since i n t h e s e experiments t h e f u e l was i r r a d i a t e d i n loose form it has
not been poss ib l e t o c l e a r l y d i s t ingu i sh t h e d i r e c t i o n of t h e kernel
movement bu t i n one experiment t h e r e appeared t o b e a d i s t i n c t tendency
f o r t h e kernel t o move down t h e temperature gradient . The occurrence of t h e amoeba e f f e c t i n UO coated p a r t i c l e fue l i s being s tudied from t h e
t h e o r e t i c a l viewpoint b u t w i l l no t b e pursued i n t h i s paper.
r e s u l t s of some re l evan t experiments w i l l be given showing how t h e
f a i l u r e appears t o be empir ical ly c o r r e l a t e d with t h e parameters
temperature, temperature grad ien t and p a r t i c l e r a t ing . The experimental
da t a r e s u l t s a r e presented i n Table 2 and t h e c o r r e l a t i o n shorn
graphica l ly i n Fig. 4.
coated p a r t i c l e f u e l i n s eve ra l experiments performed by t h e Pro jec t . 2
2 Rather t h e
It should be emphasised t h a t i n a l l t h e s e experiments loose coated
p a r t i c l e s were i r r a d i a t e d , contained i n annulsr cy l inde r s machined i n graphi te . The hea t t r a n s f e r i n such systems i n complex and although
amoeba e f f e c t s should i n p r i n c i p a l be assoc ia ted with t h e condi t ions
wi th in t h e kerne l , i n t h e above ana lys i s t h e (estimated temperature
g rad ien t s r e f e r t o t h e coated p a r t i c l e s . Fur ther , t h e t i m e s r e f e r t o
t h e onse t of p a r t i c l e f a i l u r e observed through an i n i t i a l r ise i n t h e
r e l e a s e of noble gases, and although i n a11 t h e experiments t h e gas
r e l e a s e increased progress ive ly t h e r e a f t e r , only r e l a t i v e l y few
p a r t i c l e s w e r e found t o have completely breached coa t ings a t t h e end
of t h e experiments. For example, i n t h e case of LEHPD2 t h e i r r a d i a t i o n
was continued up t o 240 days achieving 6.5% FIMA burn-up bu t only 1-2
percent of p a r t i c l e s opera t ing under t h e s t a t e d condi t ions were found
t o be f a i l e d a t t h i s s tage. Other p a r t i c l e s i n t h i s experiment
opera t ing a t 130OoC and lower were unaffected. , Further experiments a r e
now underway i n which t h e phenomenon i s being inves t iga t ed i n p a r t i c l e s
embedded i n a g raph i t e matr ix , t h i s s i t u a t i o n being more r ep resen ta t ive
of power r e a c t o r condi t ions.
6
I n using t h e c o r r e l a t i o n i n Fig. 4 , t h e designer would tend t o use
a design l i n e d isp laced somewhat lower than t h a t shown, to m i n i m i s e t h e
degree of amoeba penet ra t ion , so safeguarding t h e mechanical performance
of t h e p a r t i c l e s . Even so it can be shown t h a t with appropr ia te f u e l
503
element design, peak random condi t ions can be achieved i n which amoeba
a t t a c k i s not t h e l i f e - l i m i t i n g f ea tu re .
Mechanical Failure.--In studying t h e stress h i s t o r y of a coated par t ic le
during opera t ion many f a c t o r s have t o be considered. S t r e s ses can f i r s t
occur a s a r e s u l t of e f f e c t s a t tendant upon burn-up i n t h e kernel i t s e l f .
The primary causes which might be expected a r e swel l ing and t h e
generat ion of pressure due t o f i s s i o n gas r e l e a s e and, i n t h e case of
U 0 2 , carbon monoxide. A second source of stress generat ion i s i n t h e
pressure ves se l coa t ings themselves a s a consequence of f a s t neutron
e f f e c t s .
For t h e kerne l , t o avoid t h e bu r s t ing of p a r t i c l e s a r i s i n g from
swell ing, t h e Pro jec t favours t h e use of porous kernels . With t h e l e v e l
of poros i ty a t about 20% no de le t e r ious e f f e c t s due t o swel l ing have y e t
been found i n i r r a d i a t i o n experiments even up t o 6.5% heavy metal burn-
up f o r r ecen t UO
der ive values f o r i n t e r n a l pressures generated by r e l eased f i s s i o n gases,
da t a of t h e type depicted i n Fig. 3 may be used, with due allowance f o r
volume changes within t h e p a r t i c l e .
component can arise due t o t h e formation of carbon monoxide.
recent measurements made i n p a r a l l e l t o those f o r t h e f i s s i o n gases
show t h e presence of CO i n i r r a d i a t e d p a r t i c l e s , revea l ing both a
dependence on t h e l e v e l of burn-up and on t h e temperature a t w h i c h t h e
p a r t i c l e s w e r e crushed. These r e s u l t s a r e shown i n Fig. 5: they
suggest t h a t CO r e l e a s e s may become comparable t o t h e f i s s i o n gas l e v e l s
f u e l s and i n excess of 10% f o r earlier fue l s . To 2
I n t h e case of UO f u e l an add i t iona l 2
Some
a t about 15OOuC f o r p a r t i c l e s with about 6% FIMA burn-up.
noted t h a t t h e CO r e l e a s e s shown i n Fig. 5 are t h e maximum values found.
I f t h e i r r a d i a t e d p a r t i c l e s are maintained a t temperature f o r longer
per iods p r i o r t o crushing, t h e measured r e l e a s e f a l l s , reaching h a l f
t h e values shown a f t e r 2 hours a t temperature. The reason f o r t h i s i s
not understood:
e q u i l i b r i a involved i n t h e amoeba phenomenon.
It should be
it may be r e l a t e d t o t h e establ ishment of chemical
Stresses i n t h e PyC/SiC/PyC coa t ings a r i s e not only a s a
consequence of t h e build-up of i n t e r n a l pressure bu t a l s o from
504
d i f f e r e n t i a l dimensional changes caused by f a s t neutron i r r a d i a t i o n .
I n general , PyC undergoes considerable dimensional changes under these
condi t ions7 whereas t h e p y r o l y t i c S i c i s r e l a t i v e l y s t a b l e . e f f e c t s l ead t o t h e development of c i rcumferent ia l t e n s i l e stresses i n
t h e PyC, which are balanced by i r r a d i a t i o n creep, and r e l a t i v e l y high
compressive stresses i n t h e Sic .
effects of t h e i n t e r n a l gas pressure and delays t h e po in t i n l i f e a t
which t e n s i l e stress i s developed i n t h e Sic . Since t h e dimensional
changes i n PyC are s t rongly dependent on t h e isotropy and i n i t i a l
dens i ty , s p e c i f i c a t i o n of t hese f e a t u r e s play an important p a r t i n t h e
p a r t i c l e opt imisat ion.
8 These
This s t r e s s a c t s i n opposi t ion t o the
To study t h e stress h i s t o r y of coated p a r t i c l e s during se rv ice
and t o a s s i s t i n t h e design of experiments r e l a t e d t o opt imisat ion, 9 a mathematical model has been developed f o r t h e P ro jec t by Walther
(SORIN, I t a l y ) . The r e s u l t s of a t y p i c a l c z l c u l a t i o n showing t h e
general effects expected i n a r e fe rence p a r t i c l e , are shown i n Fig. 6.
It should be noted t h a t cu r ren t low enriched HTR designs are assoc ia ted
with burn-ups i n t h e range 6-9% FIMA and fas t neutron doses between
3 and 4 x 1021 n c m
i d e n t i f y i n g t h e end of t h e use fu l l i f e of ccated p a r t i c l e s have not y e t
been f u l l y v e r i f i e d experimentally. It i s common p r a c t i c e , however,
t o regard t h e p a r t i c l e l i f e f o r power r e a c t o r s i n t e r m s of t h e po in t
a t which a s ta te of zero stress exists i n t h e s i l i c o n carb ide , thus
allowing f o r stress inc reases near t h e end cf l i f e assoc ia ted with
r e a c t i v i t y t r a n s i e n t s . To provide experimental v e r i f i c a t i o n of model
ca l cu la t ions lead ing t o d e t a i l e d p a r t i c l e spec i f i ca t ions f o r u se i n
power r e a c t o r s , t h e P ro jec t has i n hand a l a r g e programme of
i r r a d i a t i o n s i n both t h e Dragon Reactor and i n e x t r a mural experimental
f a c i l i t i e s . This programme covers t h e major va r i ab le s of kernel s i z e ,
kernel poros i ty and coa t ing th i cknesses .
however, t h a t a wide range of ea r ly v a r i e t i e s of coated p a r t i c l e f u e l s
have already completed i r r a d i a t i o n per iods i n excess of 500 days i n t h e
Dragon Reactor without d i sp lay ing progress ive f a i l u r e i n t h e f i s s i o n gas
monitoring system.
-2 ( D I D O Nickel Equivalent) . F a i l u r e cr i ter ia
It should b e pointed out,
0 I n t h e s e experiments temperatures from 700-1200 C
505
-2 have been covered with peak neutron doses of 3 x 1021 n c m
Equivalent and burn-ups i n excess of 10% FIMA being achieved a t t h e
higher temperatures. These r e s u l t s g ive confidence i n t h e a b i l i t y of
coated p a r t i c l e f u e l s t o meet t h e performance requirements of reasonably
p i tched designs.
DIDO Nickel
THE FUEL BODY
Two methods of l oca t ing t h e coated f u e l p a r t i c l e s within t h e f u e l element s t r u c t u r e have been inves t iga t ed by t h e Pro jec t . One technique
termed "meniscus bonding" involves precoat ing t h e p a r t i c l e s with a t h i n
coa t ing of g raph i t e powder/resin mixture, pouring t h e p a r t i c l e s i n t o t h e
requi red f u e l space, and hea t - t r ea t ing t o carbonise t h e r e s i n binder.
This method may b e u t i l i s e d where it i s requi red t o achieve m a x i m u m
heavy metal investment i n t h e f u e l space. It was s p e c i f i c a l l y
developed f o r HTR co re designs i n which t h e moderator s t ack was f ixed
and contained conventional f u e l channels ( t h e so-cal led heterogeneous
type of des ign) . Current designs, however, are of t h e homogeneous
type i n which t h e g raph i t e f u e l conta iners are loca ted i n channels
placed symmetrically i n g raph i t e blocks which are removed toge ther with
t h e f u e l a t t h e end of l i fe . I n these designs, t h e volume of t h e core
ava i l ab le f o r t h e f u e l i s much g rea t e r than i n those of t h e hetero-
geneous type and t h e s p e c i f i c heavy metal investment requirement within t h e f u e l space i s consequently much lower. This r e l a x a t i o n
can b e used t o advantage with t h e a l t e r n a t i v e f u e l body, t h e g raph i t e
matr ix type, i n which t h e coated p a r t i c l e s are embedded i n a g raph i t e
matr ix of r e l a t i v e l y high densi ty .
developed f o r t h e Dragon Reactor i t s e l f and has been found t o perform
exce l l en t ly . It a l s o possesses f ea tu res which overcome some of t h e disadvantages of t h e meniscus bonding:
bed i s improved thus a id ing i n t h e minimisation of f u e l temperatures
and temperature grad ien ts ;
l o s s i n t o t h e primary c i r c u i t i s less l i k e l y i n t h e event of f r a c t u r e
of t h e f u e l s leeve ; t h e g raph i t e matr ix a c t s as a b a r r i e r minimising
mechanical and chemical i n t e r a c t i o n s between adjacent p a r t i c l e s ;
Such a f u e l body was i n fact
10
h e a t t r a n s f e r through t h e f u e l
t h e u n i t i s r e l a t i v e l y robus t and p a r t i c l e
506
f i n a l l y t h e g raph i t e matr ix nay serve t c at ter ,uate t h e r e l e a s e of some
f i s s i o n products even i n t h e event of f u e l f a i l u r e . A potential . d i s -
advantage of t h e matrix f u e l body i s t h a t t o a t t a i n a reasonably high
matrix densicy giving good mechanical and thermal p rope r t i e s , it i s
necessary t o form t h e shape by press ing , involving some r i s k of
p a r t i c l e breakage.
t h e so-cal led overcoat ing rou te i n which the p a r t i c l e s a r e coated with
t h e g raph i t e / r e s in mix t o t h e c o r r e c t degree, giving a cushioning effect
during t h e forming operat ion.
powder type and r e s i n composition, forming pressures can be kept l o w and
p a r t i c l e f r a c t u r e below t h e p re sen t ly requi red f r a c t i o n a l l i m i t of 10 .
To minimise t h i s r i s k t h e P ro jec t has developed
With proper E.t tention t o t h e graphi te
-4
The performance requirements of t h e f u e l body d i f f e r according t o
t h e design d e t a i l of t h e f u e l element a s discussed by Smith", and it i s no t wi th in t h e scope of t h i s paper t o d iscuss a l l aspec ts of t h e
p r o p e r t i e s which have been covered elsewhere . Perhaps t h e most
important requirement i s a knowledge of t he i r r a d i a t i o n induced
dimensional changes s i n c e t h e s e can have a s t rong in f luence on t h e
h e a t t r a n s f e r behaviour through gap development and i n mechanical
i n t e r a c t i o n s with t h e g raph i t e f u e l tubes. I n t h i s contex t it i s t h e
d iamet r ica l dimensional changes which are of most importance. To
i n d i c a t e t h e magnitude of t h e s e Fig. 7 i s presented which shows t h e
dimensional changes observed i n overcoated g raph i t e mat r ix f u e l ,
annul i i r r a d i a t e d i n t h e Dragon Reactor.
t o compacts containing PyC/SiC/PyC f u e l p a r t i c l e s a t 20% volume
loading, o the r r e s u l t s suggest l i t t l e in f luence of volume loadings up
t o 34%. However, it has been found t h a t i n t h e case of compacts
conta in ing f u e l p a r t i c l e s with p l a i n PyC coa t ings , t h e i r r a d i a t i o n
induced shrinkage can be about 30% grea te r .
10
Although t h e s e r e s u l t s refer
GRAPHITE
The main g raph i t e components i n homogeneous H T R ' s under cu r ren t
cons idera t ion are f u e l blocks of about 400 mn width and one metre long
conta in ing a x i a l l y bored f u e l channels l o c a t i n g f u e l tubes o r s leeves
containing the f u e l compacts. I n s p i t e of t h e f a c t t h a t power d e n s i t i e s
507
i n such s y s t q s can be up t o 4 o r 5 t i m e s g r ea t e r than heterogeneous
designs of gas-cooled reactors, with consequent reduct ions i n co re s i z e , -2 t h e peak fas t neutron doses which w i l l b e experienced (3-4 x 1 O 2 l n c m
DIDO Nickel Equivalent) are only one quarter t o one f i f t h of those
faced i n t h e f ixed moderator designs. This i s brought about by not
only because t h e f u e l blocks are discharged toge ther with t h e f u e l bu t
a l s o because t h e f u e l i s spread over a g r e a t e r volume of t h e core.
The s p e c i a l f e a t u r e s of t h e HTR r e l a t i v e t o previous gas-cooled
r e a c t o r s are t h a t t h e g raph i t e s t r u c t u r e opera tes a t higher temperatures
and t h e f u e l s leeves a r e requi red t o ca r ry a s u b s t a n t i a l h e a t f lux .
The P r o j e c t ’ s work on g raph i t e has ranged over a wide f i e l d
covering t h e development and performance of f u e l tubes of con t ro l l ed
permeabi l i ty f o r t h e Dragon Reactor 12’ 13’ l4 t o a s t u d i e s of a very
wide range of ma te r i a l s f o r p o t e n t i a l u s e i n power r eac to r s .
l a t te r , it has been necessary t o cater f o r a number of d i f f e r e n t power
r e a c t o r design p o s s i b i l i t i e s and t o keep i n mind t h e t ime-scale of
design d a t a accumulation and commercial a v a i l a b i l i t y . I n a n t i c i p a t i o n
of commercial exp lo i t a t ion , a dec is ion w a s made i n 1966 t o concent ra te
on one type of g raph i t e t o allow t i m e t o develop t h e necessary design
information. The main veh ic l e s f o r the i r r a d i a t i o n s t u d i e s throughout
have been i n t h e HFR a t Pe t ten i n Holland and i n t h e Dragon Reactor.
Lead experiments had shown very encouraging r e s u l t s i n t h e temperature
range 600-1200°C f o r a g raph i t e based on g i l s o n i t e coke, p a r t i c u l a r l y
i n t e r m s of t he i s o t r o p i c na tu re of the dimensional changes under
i r r a d i a t i o n . Also, t h i s g raph i t e has a high s t r eng th and i s the re fo re
a t t r a c t i v e as a s t r u c t u r a l material i n t h e core. A considerable body
of information has now been gathered on t h e performance under
i r r a d i a t i o n of gi lsoni te-based materials and it i s l i k e l y t h a t t h i s
type w i l l b e chosen i n t h e f i r s t p r i smat ic power H T R ’ s . Reviews of
r e l evan t da t a on t h i s type of ma te r i a l have been given by Evere t t and
Blackstone e t al . , 15’ 16’
of materials produced by severa l European g raph i t e manufacturers. I n
addi t ion , a programme of work i n v e s t i g a t i n g t h e fatigue behaviour of t h e g raph i t e has been i n i t i a t e d i n view of t h e p o t e n t i a l f o r HTR
I n t h i s
covering t h e performance under i r r a d i a t i o n
508
systems t o be employed under condi t ions of power cycling. Some
preliminary r e s u l t s of t h e s e experiments which have been performed f o r
t h e Pro jec t by Sud Aviation, P a r i s , a r e shown i n Fig. 8.
T h e thermal and mechanical performance of severa l types of f u e l
element designs i n which g i l s o n i t e based g raph i t e i s used, i s discussed
by Smith . Such analyses show t h a t t h i s type of mater ia l can be
expected t o g ive s a t i s f a c t o r y and adequate performance i n HTR power
systems. I n t h e f u t u r e , however, two a reas of improvement a r e
envisaged. F i r s t l y , s ince t h e peak neutron doses i n t h e f u e l =criF’
blocks i n pro jec ted power r e a c t o r s i s r e l a t i v e l y low, it i s i?3: unli
t h a t some s a c r i f i c e could be made i n t h e dimensional s t a b i l i t y i f t h i s
was r e l a t e d t o t h e provis ion of a cheaper mater ia l .
reduct ions i n t h e f u e l f a b r i c a t i o n costs clsild then be m a d e as the
g raph i t e i s a s i g n i f i c a n t c o s t item. The second improvement r e l a t e s
t o t h e f u e l s l eeves which have t o ca r ry s w s t a n t i a l hea t f luxes.
Analyses show t h a t f o r g i l s o n i t e graphi te the reversed thermal s t r e s s
occurr ing i n t h e s leeves on shutdown is a more s i g n i f i c a n t component
i n t h e t o t a l stress than t h a t induced by i r r a d i a t i o n effects. This
arises because t h e dimensional changes induced by i r r a d i a t i o n are
small and t h e i r r a d i a t i o n c reep process i s e f f i c i e n t i n r e l ax ing
stresses caused by d i f f e r e n t i a l dimensional changes. On t h e o the r
hand t h e c o e f f i c i e n t of thermal expansion of g i l s o n i t e graphi te i s
high, lead ing t o a r e l a t i v e l y high l e v e l oE thermal stress. Although
t h i s i s r ap id ly r e l i eved during operat ion, i t r e t u r n s on shutdown i n a reversed sense, adding t o t h e r e s i d u a l i r r a d i a t i o n stress. This
s i t u a t i o n could be improved by s e l e c t i n g a g raph i t e f o r t h e f u e l
s l eeve possessing improved thermal stress p rope r t i e s , even i f t h i s i s
a t t h e expense of some loss i n t h e dimensional s t a b i l i t y under
i r r a d i a t i o n . Current g raph i t e i r r a d i a t i o n programmes have been c a s t
with these improvements i n mind.
11
Worthwhile
CONCLUSIONS
Fuel and s t r u c t u r a l g raph i t e material:; development work f o r t h e
HTR has passed t h e s t ages of innovation and f e a s i b i l i t y and most of
509
B A POLISHED SECTION A THE SUPERFICIAL APPEARANCE
-_ - 1 THE EXTERNAL SURFACE
1
J 1
THE INNER PVROCARBON LAYER
THE SURFACE OF THE FUEL KERNEL
c THE FRACTURE SECTION OF A COATING BY *STEREOSCAN '
1. I l l u s t r a t i o n of t h e Dragon Reference Coated P a r t i c l e .
510
t h e cu r ren t experimental work i s assoc ia ted d t h t h e provis ion of
d e t a i l e d design da ta f o r t h e commercial exp lo i t a t ion of t h e system.
For t h e ' fue l , t h e only s i g n i f i c a n t s o u x e of f i s s i o n product
r e l e a s e i s t h e presence of p a r t i c l e s with f a i l e d coa t ings and thus
most e f f o r t i s concentrated on t h e de f in i t i o i l of t h e performance
l i m i t s i n terms of both mechanical and chemical phenomena. I n
consider ing these e f f e c t s , t h e designer should not ignore t h e
importance of opera t iona l r e l i a b i l i t y t o t h e u t i l i t y and t h e incen t ive
t o achieve t h i s by minimising f u e l temperatuces by appropr ia te design.
Commercial g raphi tes a r e a v a i l a b l e on which design da ta ex is t s
and although c e r t a i n improvements could be rn<3.de, these ma te r i a l s are
adequate f o r the cons t ruc t ion and opera t ion of power r eac to r s .
ACKNOWLEDGMENT
I n covering t h e wide f i e l d of HTR co re ma te r i a l s t h e author has
drawn on t h e work of many col leagues both i n t h e Dragon P ro jec t and
i n l a b o r a t o r i e s throughout Europe. Their e n t h u s i a s t i c support i s
g r a t e f u l l y acknowledged.
REFERENCES
1.
2.
3 .
4.
5.
6.
L. R. Shepherd, R. A. U. Huddle, L. A. Husain, G. E. Locket t , F. S. S t e r r y and D. V. Wordsworth, Proc.. 2nd I n t . Conf. on t h e Peaceful U s e of Atomic Energy, 9 , 289 (*L958). -
R. A. U. .Huddle, The Dragon P ro jec t Pro(jramme of Core Mater ia l s Development f o r High Temperature Power Reactors, D.P. Report 673, (October, 1969).
R. A. U. Huddle, Fuel Elements f o r High Temperature Reactors, Paper SM-111/64, I A E A Symposium on HTR .JGlich, (October, 1968) and D.P. Report 605, P t . 11.
H. Walther, Nukleonik, - 11, 1 7 1 (August, 1968).
W. V. Goedell, Symposium on C e r a m i c Matrix Fuels containing Coated P a r t i c l e s , TID-7654, 187 (November, 1962).
K. Bongartz, Heat Transfer Aspects of Coated P a r t i c l e Fuel and T e s t Elements, D.P. Report 585 (1969).
7. M. R. Evere t t , 2.. Blackstcne, L. W. G r a h a m and R. Manzel, Graphi te Mater ia l s Data f o r High Temperature Nuclear Reactors, D.P. Report 699, (December, 1969).
E. H. Voice, M a t . R e s . Bul l . - 4 S331 (1969) a l s o C.P. Report 677. 8.
9. H. Walther, A Model f o r S t r e s s Analysis i n Coated Fuel P a r t i c l e s , U.P. Report 604, (August, 1968) and D.P. Report 683 (October, 1369 1.
10. N. R. Eve re t t , R. Manzel, P. B a r r and K. Mayr, The I r r a d i a t i o n Behaviour of Coated P a r t i c l e Fuel Compacts, D.P. Report 686, (October, 1969).
11. E. Smith, The Design of Pr ismatic High Temperature Fuel Elements, This Symposium, Session V , Paper 132.
12. L. W. G r a h a m , W. Watt, W. Johnson, P. A. P. Arragon and M. S. T. Price, Proceedings of t h e F i f t h Carbon Conference, - 2 387 (1963).
13. L. W. Graham, M. S. T. P r i c e , Proceedings of 2nd SOC. Chem. Ind. Conference on Carbon, London, 446 (Apr i l , 1965).
14. B. Longstaff, T. R. Jenkins , J. B. Morris and L. W. Graham, J. Appl. Chem. - 17, 172, (June, 1968).
15. M. R. Everett , R. Blackstone, L. W. Graham and R. Manzel, Dimensional and Physical Property Changes of High Temperature Reactor Graphites I r r a d i a t e d a t Temperatures i n t h e Range 600-12OOwC, D.P. Report 657, (August, 1969)
16. R. Blackstone, L. W. G r a h a m and R. Manzel, H i g h Temperature Radiation Induced Creep i n Graphi te , D.P. Report 665, (October, 1969 1.
17. R. Blackstone, L. W. Graham, M. R. Evere t t and W. D e l l e , Radiat ion Damage i n Reactor Mater ia ls , - 2 543 IAEA, Vienna (1969).
512
NORMALISED DIFFUSION COEFFICIENT b'= D/a2 A (D- DIFFUSION CO-EFFICIENT, a - FlADlUS, A- DECAY CONST,)
2. Calculated Frac t iona l Release of Kernel-born Fission Products by Diffusion through PyC and PyC/SiC/PyC C2atings.
513
D IRRADIATION TEMPERATURE OC
IO0 9c 80
7a
6C
5c
4c
3c
c
V w
5 2c
a n n W fn 4 W -I
0:
u)
w io 9
w e n 0 7
E 6
o 5
c 0
z I w x 4
3
2
I
I800 1700 1600 1500 1400 3 \
e' '\ '. -8
X X
x 1.5 O/o FlMA BURN-UP
0 6 "/o F l M A BURN-UP
I I I 1 1 1 I 1 1 I I L 0.5 0.6 0.7
lOOU/T *K 3. Release of Xenon Isotopes Observed on Crushing I n t a c t I r r a d i a t e d
Dragon Reference Type Coated P a r t i c l e s a t High Temperatures.
TEMPERATURE OC
4. Onset of P a r t i c l e F a i l u r e Observed dllring High Temperature I r r a d i a t i o n Experiments.
X 1.5 % FlMA BURN -UP
0 6 % FlMA BURN -UP
7 I I I I -I I I I I I
1000 1500 2000
CRUSHING TEMPERATURE 'C 5. Release of Carbon Monoxide Observed on Crushing I n t a c t I r r a d i a t e d
Dragon Reference Type Coated P a r t i c l e s a t High Temperatures.
BURN-UP [PERCENT FIMA]
2 4 6 8 IO 12
c
n
E N I
U 0 7 Y
m
U
0
I-
V
s
z_ d z v) v) W IY c v)
-I
I- z w 0 z U I-
5
3
2
I
0
- I
-2
-3
PRESSURE
I I I I I I IO 20 30 40 50 60
DOSE [ 1020n.cm-2 DIDO NICKEL EQUIVALENT]
Dimensional Changes Observed i n Graphite Matrix Fuel Compacts I r r a d i a t e d i n t h e Dragon Reactor.
-1.0
-2.c
DOSE C 1OZ1n CIII-~DIDO NICKEL EQUIVALENTJ I 2
I
IRRN.TEMP 900 "c
1000 "c I l 0 O 0 C
1200 "c - FUEL COMPACT DIMENSIONS m m
TYPE A TYPE C OD 44.16 44.16 I D 31.60 15-23 L 40 * 28 40.28
6. Calculated S t resses Occurring i n th," Coatings of PyC/SiC/pYC Coated P a r t i c l e I r r a d i a t i o n a t 1200 C. P a r t i c l e Parameters : Kernel U02, 780 p n diameter, 18% porosi ty: coat ings, buf fer
PyC 30 pm 1.1 g/cm3, inner PyC 56 pm 1.8 g/cm , Sic 38 p m , ou ter PyC 34 p 1.8 g/cm3
3
516
- - 1
I 1 1 I I 1 I 1 I I
MEAN STRESS / ULTIMATE STF!ENCTH
8 . Fatigue F a i l u r e Data f o r G i l s o n i t e Graphi te Subjected t o Cycl ic S t r e s s a t Room Temperature.
51 7
DISCUSSION
S. I. Kaplan: What was t h e kerne l composition f o r t h e correlated data on amoeba-effect and f a i l u r e vs lOOO/T? Have you correlated data
for any other kernel composition?
L. W. Graham: The kernel composition was uranium dioxide. I n pre- vious i r r a d i a t i o n experiments a t temperatures above about 16OO0C, we have seen t h i s e f f e c t with Th/U oxide f u e l and i n f u e l s with carbide composi- t ion, but there are not enough points t o s e t up a correlat ion.
H. G. MacPherson: Could you say something about what you found on graphi te fatigud ?
L. W. Graham: There was not time t o include t h i s data i n the pre- sen ta t ion but you w i l l f i n d i t i n the paper. curve suggests t ha t graphite behaves intermediately between a b r i t t l e
cas t i r o n and m i l d s t e e l . produced by power cycling i n HTR f u e l pins i s not ser ious and i s described i n d e t a i l i n E. Smith 's paper.
The shape of the fa t igue
The implication of the data on cyc l ic s t r e s s e s
M. T. Morgan: What causes the disappearance of t h e CO during the measurement when coated p a r t i c l e s a r e crushed a t room temperature, and doesn' t the react ion between U02 and c a r b o y c r e a t e more CO during mea-
surements a t high temperatures?
L. W. Graham: The absence of CO on crushing a t room temperature w a s
a t t r i b u t e d t o absorption e f f e c t s i n the kernel and pyrocarbon. For the
second par t of your question, the p a r t i c l e s a r e crushed i n a mass spec- trometer and the measurement completed i n 1 t o 2 seconds a f t e r crushing. Also the p a r t i c l e s a r e quenched rapidly j u s t a f t e r crushing.
seen addi t iona l CO from the react ion of UOz w i t h the F'yC f o r crushing temperatures up t o about 20OO0C, the m a x i m u m we have looked a t .
We have not
C. B. Zitek: Had any f i s s i l e material been found on the metal sam-
ples ?
L. W. Graham: A very small amount was present; however, much more was found i n or on the graphite samples - l e s s than 10 grams i n a l l the
graphi te i n the core.
Paper 5/126
CHOICE OF FVXL DESIGN FOR HOMOGENEOUS LOW ENRICHED HTR ---*----*-**r=*-- *-.>.,- - ~,” .&.n4w-.,ir,rv .--- +
D.J. Merrett M. Gaube
ABSTRACT
The paper considers firstly the specification of particle for a commercial HTR design and concludes that an 800ym particle will be satisfactory and possess sufficient endurance to meet the economically desirable irradiations.
These particles can be incorporatei. into compacts having sufficient strength, heavy metal density and low breakage fractions to meet engineering a.nd radiological requirements. The irradiation shrinkage behaviour is reasonably matched to that of fuel tube graphite.
The incorporation of these cornpacts into various fuel element geometrics is discussed and it is concluded that all the various configurations available meet limits which are either set by excessive fuel temperature, graphite stress o r compact stress. Bearing these limits in mind, it is concluded that, economically and technically, the tubular interacting design of fuel pin is the preferred choice. A s an alternative, the integral block design also appears to be economically attractive.
518
i .
519
3
INTRODUCTION
Construction of t he f i r s t l a r g e high temperature r eac to r i n the UK
w i l l be undertaken i n 1971 and dec is ions a r e now being made on the bas ic
parameters, s o t h a t t he manufacture and proving of fue l elements and
c e r t a i n of t he engineering f ea tu res may begin. The r eac to r w i l l be of
640 MW output approx and w i l l incorporate prismatic fue l elements of a
design agreed i n i t s e s s e n t i a l f ea tu re s throughout t h e industry.
Several a l t e r n a t i v e designs have been studied i n considerable
d e t a i l over t h e pas t two yea r s and t h i s paper i s a condensation of t h e
work done by TNPG and i t s assoc ia ted companies.
Fundamental t o the fue l element i s t h e requirement f o r high r a t i n g
assoc ia ted with high burnup and l o w c i r c u i t a c t i v i t y without t h e fue l
f a b r i c a t i o n cost becoming t o o g rea t and the re fo re uneconomic. It i s
considered t h a t the r i g h t balance between these demands can now be made.
COATED PARTICLE DESIGN
The design o f a reference coated p a r t i c l e was described i n Ref 1
and the main parameters of a s l i g h t l y rev ised reference design a r e s e t
out i n Table 1. This coated p a r t i c l e has a nominal 800pm kernel and
coa t ing th ickness o f 160-170r.m. There a r e economic incent ives which
lead t o t h e choice of l a rge kernel s i zes . These incent ives stem from
f a c t o r s i n f lu id i zed bed technology, f a b r i c a t i o n c o s t s of t h e coated
p a r t i c l e decreasing as kernel s i z e increases up t o a kernel diameter
around 9 O O p m .
For higher kernel s i z e s the f a b r i c a t i o n cost does not decrease
much more. Moreover, t he coa t ing operation presents some technica l
problems f o r l a r g e r s i z e s and it i s , f o r t he moment, s a fe t o consider
800pm as a manufacturing l i m i t f o r t he kernel diameter.
The p a r t i c l e s i z e inf luences t h e heavy metal loading which has an
impact upon c a p i t a l and generation c o s t s , higher loadings lead ing t o
reduced cos ts . This a l s o pushes one towards l a rge p a r t i c l e s i zes .
520
Accordingly, t he 800r.m kernel has been adopted as a standard and
t h e main concern i s t o spec i fy t h e coa t ing thicknesses.
The main purpose o f the coated p a r t i c l e l aye r s i s t o r e t a i n t h e
f i s s i o n products throughout t h e design l i f e of t he element. The
de ta i l ed func t ion o f t he ind iv idua l l aye r i . 2 ; well known and has been
described before. Their thickness and impoistant parameters a r e t o a
l a rge extent determined by what i s f e a s i b l e i n manufacturing and the
design s e t out i n Table 1 does not necessar i ly represent an optimum
from t h e point of view of endurance.
This p a r t i c l e i s a design which has been developed by Belgo-
Nucleaire and i s very similar t o the one which i s being incorporated
i n t o the TNPG element designs. The mechanical endurance of t h e
p a r t i c l e i s a complex function which, however, i s amenable t o calcula-
t i o n us ing computer techniques and t h i s s ec t ion of t he paper b r i e f l y
reviews t h e r e s u l t s o f one such survey.
COCONUT (Coating Computation f o r NUclear Technology) i s a computer
code which c a l c u l a t e s t h e s t r e s s e s and strains on the coa t ing l aye r s
and has been developed by BelgoNucleaire s ince 1967.
It proceeds through successive time s t eps and has been wr i t t en
for any f u e l , coa t ing ma te r i a l , numbers of l3yers , temperature and
i r r a d i a t i o n evolution.
The s t r e s s e s and strains i n t h e l a y e r s (are generated by t h e
f i s s i o n and CO gas pressure , fue l swelling a:ad the dimensional changes
induced by t h e thermal h i s to ry and the i r r ad : i a t ion damage.
A t each time s t e p t h e s t r e s s e s and s t r a i n s a r e corrected f o r
creep e f f e c t s induced by i r r a d i a t i o n and temperature.
For high power dens i ty conditions, t he s t r e s s e s induced by t h e
thermal f l u x through t h e coa t ing a r e a l s o considered.
Using t h i s model i t can be shown t h a t f a i l u r e of the &C/SiC/p;I.C
p a r t i c l e s occurs where t h e S ic l aye r goes i n t o tension. Up t o t h a t
moment i t i s kept i n compression by t h e combined shrinkages o f the
in s ide and outside HD P y C l aye r s .
- - . . - - . . . .. . . . . . . ,
521
This sudden increase of t he hoop s t r e s ses i n the S i c i s due t o
the hydrostat ic pressure induced i n the coating by the kernel swelling.
Fig 1 Pa r t i c l e S t ress History, shows the va r i s t i on i n hoop and
r ad ia l s t r e s ses of the PyC and S i c layers which character ises t h i s
e f f ec t . It can be seen tha t the increase i n S i c s t r e s s i s very sharp
and, although S i c has a. r e l a t ive ly high t e n s i l e s t rength the point of
f a i l u r e can, t o all i n t en t s , be taken as the time it starts t o go i n to
tension.
The e f f ec t of the kernel swelling, and therefore the f a i l u r e o f
the p a r t i c l e , can be delayed by increasing the buffer layer thickness;
Fig 2 gives the buffer thickness required t o avoid t h i s hydrostat ic
pressure before 4 x 102’EDN; t he percentage of theore t ica l densi ty , o f the maximum fuel burnup,
o f t he temperature and of the buffer layer density ( the curves a re
shown dotted below the m i n i m u m thickness required t o a t tenuate the
f i s s i o n products r e c o i l ) .
t h i s buffer thickness i s a function o f
The l i f e of the p a r t i c l e can a l s o be prolonged by changing the
inner and outer KD PyC and by small changes t o the €ID P y C density but
t he e f fec t of these parameters i s l e s s pronounced.
The cha rac t e r i s t i c s of the p a r t i c l e i n Table 1 have been developed
f o r BelgoNucleaire fabr icat ion process and a re d i f fe ren t from the
cha rac t e r i s t i c s of an optimum p a r t i c l e which might be given by the
parametric study f o r two reasons:
(a) The fabr ica t ion process o f the reference p a r t i c l e i s
f ina l i s ed ; the fabr ica t ion process o f an optimum pa r t i c l e
i s s t i l l under development.
(b) The influence of the var ia t ion o f most of the parameters
i s ins igni f icant and a small change o f Ng/Nu could lead
t o t he same ef fec t on p a r t i c l e l i f e t ime , by a l t e r i n g
fast neutron dose.
The development aspects of p a r t i c l e fuel a r e discussed i n a
companion paper2 t o t h i s conference.
522
Thus it can be seen t h a t t h e r e s u l t of' applying these ca l cu la t ions
t o t h e re ference p a r t i c l e i s t o ob ta in t h e o r e t i c a l burnups of t he
p a r t i c l e of t h e order o f 10% FIMA which corresponds t o about 60 t o
70,000 MWd/teU mean r eac to r discharge i r r a d i a t i o n .
shown on most normal types of f u e l element t h a t t h e t h e o r e t i c a l optimum
burnup o f a f u e l element i s around 60,000 MWd/teU as indica ted by Fig 3. This corresponds t o 3x r a t h e r than 4 x 102'EDN.
taken t h a t t h e coated p a r t i c l e has s u f f i c i e n t endurance t o meet t he
demanded i r r a d i a t i o n which i s a l s o t h a t which i s economically des i rab le .
The d i f fe rence between predic ted FIMA and f a s t neutron dose t o f a i l u r e
and t h e l e v e l s which w i l l need t o be reached i n p rac t i ce i s thus about
I n f a c t it can be
It can therefore be
25%. account of sub-standard p a r t i c l e s . The endiirance predic t ions a r e most firm for elements running at temperatures of approximately 1,200Oc
where t h e r e i s s u f f i c i e n t experimental evidence t o confirm t h e da ta fed
i n t o t h i s computation. Extrapolation t o higher temperatures i s poss ib le
but increas ingly unce r t a in and at the present time it i s concluded t h a t
peak random temperatures of '1,400 C a r e as lar as one would wish t o ex t rapola te . On t h e o ther hand, t h e r e i s s a t i s f a c t o r y i r r a d i a t i o n
evidence f o r p a r t i c l e s a t t h i s temperature $50 t h a t r e l i ance so l e ly on
a computational model i s not necessary. This s t a t e o f a f f a i r s i s
re levant t o t h e choice of f u e l element which i s discussed l a t e r i n t h i s
paper.
This can be regarded as a design margin and should a l s o take
0
Thus, t o summarise, i t i s evident t h a t 800pm kernel coated part-
i c l e s have predic ted endurances o f :
Peak p a r t i c l e burnup
Peak p a r t i c l e f a s t neutron dose approximately 4 x 10 EDN
A t peak p a r t i c l e temperature
approximately 10% FIMA 21
approximately I 200'~
Much i r r a d i a t i o n evidence i s already ava i l ab le up t o these l e v e l s
and more w i l l a r i s e from Dragon, STUDSVIK and OSIRIS by t h e end of 1970. UK programmes w i l l provide s t i l l fu r the r da ta up t o maxima of 8-10$
FIMA/6 x 10 21 EDN by mid-1971 and the re w i l l thus be ample corroborating
523
@ evidence for a reference p a r t i c l e by t h e f u e l f reeze date.
The s i g n i f i c a n t l y lower l e v e l s of endurance which a re economically
requi red for t h e f i r s t - o f f r eac to r should lead t o a very conservative
design i n which the re i s a high degree of confidence.
DESIGN OF mTEL COMPACT
Ref 1 described a design of fue l body i n which the p a r t i c l e s
were bonded together by a t h i n carbonised bond. Further development
of t h i s type of bond has been temporarily suspended s ince t h e method
had l o w thermal conduct iv i t ies and hence gave high f u e l p a r t i c l e temp-
e ra tu re s . It was a l s o d i f f i c u l t t o ensure the bond had s u f f i c i e n t
i n t e g r i t y t o avoid d i s in t eg ra t ion of t he bed under i r r a d i a t i o n condi-
t i o n s , whilst a t t he same time not being s o s t rong as t o adversely
a f f e c t t h e p a r t i c l e s . F ina l ly , t he change t o a more homogeneous type
o f r e a c t o r design reduced t h e requirement for very high heavy metal
loadings, of t h e order o f 1.5 g/cc.
u t i l i s e t h e well proven compact-type of f u e l body which has both high
thermal conductivity and high mechanical i n t e g r i t y .
The present proposals a r e t o
The design of t h e f u e l element a f f e c t s t he spec i f i ca t ion f o r t h e
compact body i n a number o f important ways as discussed below.
Shrinkage Data
One of t he important parameters of t h e fue l compact i s t h e shrink-
age which it experiences under i r r a d i a t i o n . Idea l ly t h i s shrinkage
should be matched t o t h a t o f t h e graphite. I n t h i s manner i t i s then
poss ib le t o prevent t h e opening of t h e i n t e r f a c e gaps, o r i n t h e case
of tubular i n t e r a c t i n g elements lower t h e r e s u l t a n t compact s t r e s s
l eve l s . In p rac t i ce , t h i s matching i s d i f f i c u l t t o achieve. I n t h e
first place t h e graphi te and compact temperatures a r e d i f f e r e n t and
secondly manufacturing a v a i l a b i l i t y r e s t r i c t s t h e s e l e c t i o n of mater ia l
and t h e shrinkage da ta which the re fo re r e s u l t s .
The UK programme has been based on t h e use of i s o t r o p i c Gilsocarbon
as t h e fue l p in graphi te with a needle coke matrix for t he compacts.
524
Gilsocarbon was chosen e a r l y on i n t h e programme on t h e b a s i s t h a t
considerable i r r a d i a t i o n shrinkage d a t a was ava i l ab le t o underwrite
des ign c a l c u l a t i o n s and a l s o t h a t i t had a very l o w shrinkage which
w a s considered t o be a d e s i r a b l e f e a t u r e of f u e l tube graphi te .
The compact, developed at Dragon, on t h e b a s i s of She l l H 100 coke,
underwent some changes both i n ma te r i a l (of ‘be t te r a v a i l a b i l i t y ) and
manufacturing methods t o make i t more s u i t a b l e f o r t h e production-scale
processes of t h e UKAEA Spr ing f i e lds works.
The cur ren t UK s i t u a t i o n i s t h a t t h e t w o materials a r e not exac t ly
matched and, at t h e temperatures of i n t e r e s t f o r peak r a t e d f u e l , t h e
compact shr inks rhore r ap id ly than t h e g raph i t e t o t h e ex ten t of about
1% m a x i m u m d i f f e r e n t i a l by about 1 x 102’EDN, t h e d i f f e rence t h e r e a f t e r
decreasing.
I n an i d e a l world t h i s would not occur, but with g raph i t e
m a t e r i a l s such a r e s u l t i s perhaps as bes t a:; could be r e a l i s t i c a l l y
expected, c e r t a i n l y f o r a f i r s t - o f f commercial system. There i s
obviously room f o r improvement bu t , as w i l l lie shown, t h i s d i f f e rence
does not prevent t h e d e r i v a t i o n of p r a c t i c a l r e a c t o r f u e l designs.
Even i f it were poss ib l e t o match t h e s e t w o parameters exac t ly ,
t h e r e would always be a r e s i d u a l unce r t a in ty due t o s c a t t e r i n t h e
as-manufactured d a t a which might be as much as t20%.
des igning f i e 1 elements t h e d i f f e rences between compaxt and graphi te
behaviour must always be taken account o f , toge ther with t h e scatter
which i s inherent i n product ion q u a n t i t i e s .
Therefore, i n
S t rength
Thermal s t r e s s e s which a r e experienced by t h e compact i n some of
t hese designs range up t o about 800 ps i .
oped from t h e i n t e r n a l temperature drops wi th in a compact, which i n
t h e case o f rod-type elements can be very cons iderable , or, i n t h e case
of t ubu la r i n t e r a c t i n g elements, from t h e i n t e r a c t i o n s t r a i n s with t h e
graphi te . I n these cases , t h e r e f o r e , a reasonable degree of s t r eng th
i s needed. It i s poss ib l e t o a t t a i n UTS va lues o f approximately 2000 p s i
These s t r e s s e s can be devel-
J
. . .
525
0 by going t o matrix dens i t ies of the order of 1.7 g/cc.
pa r t i cu la r ly d i f f i c u l t t a rge t from the point of view of manufacturing,
although it does require r e l a t ive ly high compaction pressures.
high heavy metal loadings a r e simultaneously required, t h i s can r e s u l t
i n large breakage f rac t ions during manufacture.
This i s not a
I f very
Designs such as the t e l e d i a l o r i n t eg ra l block designs do not have
such a requirement and matrix dens i t i e s could conceivably be reduced i n
those cases.
Heavy Metal Loading
A s pointed out above, heavy metal dens i t i e s of 1.5 g/cc a r e not
needed fo r economic homogeneous designs nor, i n f a c t , could they be
achieved with the compact fue l approach. Nevertheless, there i s an incentive t o keep the heavy metal density as high as possible since
bas ica l ly a lower density increases the Nc/Nu r a t i o away from the
economic optimum desired.
The p a r t i c l e design chosen current ly f ixes a pract icable upper
l i m i t o f 1.0 g/cc fo r which a volumetric packing f r ac t ion of up t o 40% i s needed.
t h i s can r e s u l t i n measurable (more than, say, 1 i n 10 ; i t i s
d i f f i c u l t t o measure l eve l s lower than t h i s ) broken f rac t ions of
particles during compaction. If i t is wished t o improve t h i s s i t ua t ion
i n order t o keep the reac tor primary c i r c u i t 'clean' then some reduction
i n packing f r ac t ion i s required. Alternat ively, i t would be feas ib le
t o thicken the p a r t i c l e coating t o make i t stronger.
reduces the heavy metal density and increases costs. The maximum
reduction i n density i s only l i k e l y t o be t o about 0.8 g/cc, but t he
extent of the cost increase i s a c r i t i c a l balance between:
With the matrix dens i t i e s specif ied i n 'Strength' above, 4
Either route
(a) U r a n i u m cos ts (both i n i t i a l and replacement) which a re
determined by reac tor core calculat ions.
(b) Fuel fabr ica t ion costs , pa r t i cu la r ly replacement, which
a re determined by a var ie ty o f overal l system parameters
and a re obviously spec i f ic t o a par t icu lar design.
526
However, f o r t h e gegeral ra.nge of element designs inves t iga ted ,
t h e cost penalty f o r reducing f rom 1.0 t o 0.8 g/cc i s not prohib i t ive
and mainly a r i s e s from fue l cost va r i a t ions . Table 2 shows the manner
i n which c o s t s vary f o r a p a r t i c u l a r pair Gf tubular designs. Fig 4 shows the niannzr i n which fue l c o s t s vary f o r a constant heavy metal
dens i ty but varying Nc/Nu r a t i o . (Note: Cost datums a r e d i f f e r e n t
from Table 2 f o r c l a r i t y ) .
Thus, i t can be concluded t h a t even t h e current s t a t e of develop-
ment w i l l give compacts which have t h e follo.wing cha rac t e r i s t i c s :
Peak shrinkage r e l a t i v e t o f u e l p in graphi te
Compact matrix s t rength UTS (un i r r ad ia t ed ) approx 2000 p s i
Heavy metal loading 0.8 g/cm 4 P a r t i c l e breakage i n manufacture approx 1 i n 10
- I$ t0.25
3
These parameters a r e s a t i s f a c t o r y f o r an economic design now. - The in te rvening time u n t i l 1973 w i l l be used t o underwrite t h e e x i s t i n g
experimental da t a and (hopefully) by refinements t o improve the specif-
i ca t i on.
I r r a d i a t i o n da ta f o r annular compacts i s cu r ren t ly ava i l ab le up t o 21 3 x 10
pos i t ions.
EDN and up t o 12OO0C. This i s s a t i s f a c t o r y for peak r a t e d
FUEL ELEMENT DESIGNS
The d iscuss ion i n t h i s paper i s l imi t ed t o prismatic fue l s . D i s -
cussion of t h e Pebble bed type element i s noli included.
I n a l l cases the elements a r e embodied i.n hexagonal graphi te
blocks and t h e ques t ion t o be answered i s t h e prefer red geometrical
form o f t he elements i n those blocks.
The general form of a l l t h e designs below i s indica ted i n F ig 5 and some of t h e main parameters of t y p i c a l design po in t s a r e s e t out
i n Table 3. chosen with a view t o
t o optimum. Broadly th ree ca tegor ies of embodiment can be discerned:
I n t h e case of t he GGA design t h e f u e l r a t i n g s have been
making t h e Nc/Nu r a t i o 240, t h i s being c lose
527
0 Fuel Rods Cooled on t h e Outside
This s o r t of element i s exemplified by t h e Peach Bottom design,
wh i l s t i n Great B r i t a i n t h e hollow rod design has been evolved. Due
t o f u e l temperature l i m i t a t i o n s incu r red by having t h i c k compacts
and high heat f l u x e s , t h e hollow rod concept can be developed towards
c l u s t e r s o f smaller rods a long t h e l i n e s o f t h e t r e f o i l design as put
forward by BelgoNucleaire. The t r e f o i l i s only a p a r t i c u l a r case of
c l u s t e r designs which a l l f o l l o w t h e w e l l t r i e d rou te o f i nc reas ing
sur face t o volume r a t i o . There a r e t y p i c a l examples o f t h i s approach
i n current UK and US r e a c t o r technology.
Tubular Designs
Improvements t o r a t i n g and decreases i n f u e l temperature can
obviously be achieved by cool ing t h e compact on both s i d e s and one
t h e r e f o r e progresses l o g i c a l l y t o a f u e l p i n which i s tubu la r i n
concept.
I n i t s s implest form t h e compact f i t s loose ly between t h e inne r and
ou te r s leeve and does not i n t e r a c t with e i t h e r . Rat ing improvements may
be obtained by al lowing some degree o f i n t e r a c t i o n with t h e inner
s leeve and t h e r e i s the re fo re an i n t e r a c t i n g ve r s ion o f t h i s concept.
Several v a r i e t i e s o f t h i s type a r e cu r ren t ly be ing canvassed.
A s t e p change can be made by combining t h e t w o tubu la r shea ths
i n t o a solid graphite annulus and embodying t h e fuel compacts i n t o
t h i s s o l i d annulus as d i s c r e t e lumps. Such a design has been put f o r - ward by Dragon Pro jec t and designated t h e t e l e d i a l design.
I n t e g r a l Block Designs
A l l t h e above v a r i a n t s incorpora te t h e fuel p ins wi th in channels
i n t h e f u e l block but by in spec t ion o f t h e last va r i an t i . e . t e l e d i a l
design, i t can be seen t h a t i t i s but a shor t f u r t h e r s t e p t o incor-
pora te t h e compacts d i r e c t l y i n t o t h e block with coolant channels
i n t e r spe r sed . This approach i s exemplified by t h e f u e l element being
developed by GGA f o r t h e Fort St Vrain Reactor. Whilst t h i s cycle i s
a uranium-thorium cycle i t i s i n t e r e s t i n g t o specula te upon t h e appl ic-
a t i o n o f t h e design t o a l o w enriched uranium cycle .
528
Thermal Considerat ions
The Coated P a r t i c l e Design s e c t i o n p o i n t s out t h a t t h e design endur-
ance o f t h e coated p a r t i c l e s i s temperature dependent with t h e h ighes t
degree of confidence at peak p a r t i c l e temperatures i n t h e order o f
1 20OoC.
at higher temperatures and a peak f u e l p a r t i c l e temperature of 14OO0C
may be chosen as t h e upper l i m i t . The main des ign problem with t h e
f u e l element designs considered t h e r e f o r e reduces t o a t t a i n i n g t h e
des i r ab le f u e l temperatures at t h e r a t i n g s .which w i l l give t h e most
economic b e n e f i t s .
However, t h e r e a r e considerable experimental r e s u l t s ava i l ab le
With t h e high thermal conduc t iv i t i e s o f t h e f u e l compacts t h e
temperature drops through them a r e genera l ly small. The gas s i d e surface temperature drop i s a func t ion o f heat t r a n s f e r c o e f f i c i e n t
which i s s e t from economic cons idera t ion . The major unce r t a in ty ,
t h e r e f o r e , i n f u e l temperature i s t h e temperature drop which occurs
between t h e ou te r sur face of t h e compact anti t h e inne r sur face of t h e
g raph i t e tube. Simple mathematics i gnor ing r a d i a t i o n terms show
t h a t t h i s temperature drop can be expressed i n t h e form:
A t = g . Eo+ R (S2- S I g k
where q = heat f lux a c r o s s t h e gap
k = thermal conduct iv i ty of helium i n t h e gap
G = i n i t i a l hot gap dimension
R = r a d i u s of ou ts ide of gap
SI = shrinkage of g raph i t e
E$= shrinkage of compact
0
Typical shrinkage curves f o r g raph i t e a.nd compact give maximum
d i f f e r e n t i a l between S2 and S of about I$, occur r ing at 102’EDN. t h e f i e1 compact dimensions of t h e hollow rod shown i n Table 3, t h i s
d i f f e rence i n shrinkage r a t e i nc reases t h e gap by 200,pm approximately.
For t y p i c a l peak heat f l uxes of ( s ay ) 55 watts/cm2 t h e r e s u l t a n t
i nc rease i n temperature across t h e gap i s approximately 170 C from
start of l i f e .
With 1
0
Simi la r ly , i f one a l l o w s f o r t h e 220% v a r i a t i o n s i n
529
0 these t w o parameters there i s an uncertainty of about 50°C on t h i s
f igure. Such high values of temperature difference constr ic t the
r a t i n g of the hollow rod and, even going t o maximum allowable tempera-
t u re s of 1400 C , the capi ta l and generation costs of t h i s design a re
the highest of those i l l u s t r a t ed . Nevertheless, the simplicity of the
design has a strong a t t r ac t ion and there i s considerable i r r ad ia t ion
experience t o back up the select ion of a design of t h i s s o r t . For a
f i rs t -off s ta t ion , therefore, t h i s design could be an a t t r ac t ive
solut ion since i t gives considerable advantages over current gas-cooled
reactor technology and of fers scope for considerable fur ther develop-
ment.
0
The broad l i nes of t h i s development a re indicated by the other
var iants of fuel elements put forward. A l l attempt t o minimise the
uncertainty i n fuel compact temperature by one of the following routes:
(a) By reducing the magnitude of the problem by reducing e i ther
R ( t o reduce gap widths) o r q.
volumetric fuel r a t i n g q i s inversely proportional t o R a l s o .
Note that for constant
(b) By avoiding i t altogether and allowing the compact t o remain i n direct contact with the graphite sheath.
Method (a) gives the greater scope for design ingenuity. Method
(b) i s represented by the tubular in te rac t ing design. ment of t h i s can be foreseen i n which the compact bed i s cast in tegra l ly
with the fuel pin, but more manufacturing development of t h i s route i s
required.
Further develop-
A s an a l te rna t ive , the graphite and compact data could be ta i lored
for equal shrinkage. T h i s method, although theore t ica l ly a t t r ac t ive ,
has not t o date been act ively pursued since it i s constrained by manu-
factur ing ava i l ab i l i t y of the required materials; furthermore, there
w i l l always be residual uncertainty owing t o s ca t t e r i n the data.
However, i f it i s pursued it would be most f r u i t f u l t o modify the
graphite for s l i gh t ly greater shrinkage. This should a l s o have the
advantage tha t the coefficient of thermal expansion w i l l be reduced with
consequent benefit t o thermal s t r e s s problems (see next sect ion) . @
530
St re s s ing Considerations
Before going on t o consider the performance of various types of e l -
ement i t i s worthwhile b r i e f l y drawing a t t e n t i o n t o t h e problem of
thermal s t r e s s e s i n a l l these designs. The very high heat f luxes in-
volved produce temperature drops throughout t he graphite and r e s u l t i n
thermal s t r a i n s which at t h e high opera t ing temperatures r e l a x out , so
t h a t during r eac to r operation t h e graphi te s t r e s s e s a r e generally very
low. However, at shutdown one g e t s a reversed t e n s i l e s t r e s s pa t t e rn
through t h e thickness of t h e f u e l tube which i s proportional t o coef f i -
c i en t of thermal expansion and which can be of considerable magnitude.
This e f f e c t i s i l l u s t r a t e d i n Fig 6 , which shows typ ica l operating and
shutdown s t r e s s p a t t e r n s for a hollow rod design.
It might be claimed t h a t these thermal s t r e s s e s , being secondary
i n na ture , a r e not harmful and a l s o t h a t t h e graphi te , not being notch
s e n s i t i v e , would not s u f f e r severe cracking anyway. However, t he re i s
no doubt t h a t t h e pred ic ted s t r e s s e s can be very high ( c e r t a i n l y i n t h e
order o f 0.5 x UTS f o r t h e designs of i n t e r ' s s t ) and f o r such a v i t a l
component as a f u e l element i t i s judged pr-udent at t h i s time t o take
account of them.
The graphi te a l s o s u f f e r s from shrinka,ge s t r e s s e s due t o t h e d i f f -
e r e n t i a l temperatures and fast neutron doses which occur throughout t h e
w a l l s o f t he f u e l element. These produce s i m i l a r but generally smaller
s t r e s s pa t t e rns .
Bowing s t r e s s e s can t h e o r e t i c a l l y cause more ser ious e f f e c t s s ince
t h e r e s t r a i n t can s t r e s s one s ide of t h e tube i n a completely t e n s i l e
fash ion . However, these s t r e s s e s a r e gene]-ally l o w compared with
t h e pure thermal s t r e s s e s and, moreover, cain be minimised by
design e.g. i nc reas ing t h e rib/channel cleai-ance.
probably a degree o f s e l f - s t a b i l i s i n g anyway, i n t h a t having bowed
towards a w a l l hot-spots w i l l be developed on t h e f u e l p in opposite t h e
bow which w i l l tend t o s t r a igh ten it out.
1
Moreover, t he re i s
It i s the re fo re concluded t h a t thermal s t r e s s i n g o f t h e graphi te
elements i s t h e main mechanical problem. For comparison purposes
531
simple 2-dimensional analyses a 4 the mid-plane of the fuel pins a re
sat isfactory but th.e more cotnplicated extd e f f ec t s , where steep axiel
temperature gradients and varying r e s t r a in t conditions occur, need
special treatment.
DISCUSSION OF ELEMENT PERFORMANCE
A s mentioned i n Thermal Considerations above, methods (a) and (b)
allow higher ra t ings w i t h lower temperatures and a l l the designs con-
sidered here i l l u s t r a t e various ways i n which t h i s i s obtained. Dealing
with these designs i n turn we may make the following comments:
Trefoil Design
This design reduces both R and q , thereby allowing considerably
higher fuel ra t ings for roughly the same l imi t ing fuel temperature.
Obviously t h i s improvement could be continued by increasing the number
of pins s t i l l fur ther . However, t h i s course of action i s l i ke ly t o
give reducing returns since the fue l fabr icat ion costs w i l l r i s e
steeply with the increasing number of graphite components which have
t o be machined.
numbers of small pins within small channels and a l s o the balancing of
flows between the various sub-channels.
There a re l i ke ly t o be mounting problems for large
The impact o f fuel fabr icat ion costs can be seen (Table 3) from the generation cos ts w h i c h are high compared w i t h o the r equally ra ted
designs. Thus the t r e f o i l may be regarded as indicative of t h i s s o r t of trend.
Tubular Non-Interacting Design
This design halves q although, i n the case shown, the value of R
However, on balance there i s a ne t t reduction i n goes up margirtally.
gap temperature drop which allows reasonably high ra t ings with fuel
temperatures i n the neighbourhood of 12OO0C.
t h i s design i s t h a t , i f i t i s regarded as being essent ia l t o avoid
graphite/compact in te rac t ion , large i n i t i a l gap allowances must be
made t o ensure t h i s condition throughout l i f e and for the expected
The main d i f f i cu l ty w i t h
532
var i ab i l i t y of material parameters.
e f fec ts of two gaps which a re (thermally) i n para l le l .
t o wide var ia t ions i n heat s p l i t and tempera,tures between the two coolant surfaces. These temperature d i f f e ren t i a l s , apart from being
inherently undesirable, can cause severe s t ress ing problems i n the
w a l l s and end caps.
One i s then t ry ing t o balance the
This can lead
Thus, although i n pr inciple the element design can produce
a t t r ac t ive ly high ra t ings , i n pract ice the engineering uncertaint ies
involved i n maintaining the non-interacting concept are l i ke ly t o erode these advantages and there w i l l always be a substant ia l degree
of uncertainty i n thermal performance predictions.
Teledial Design
This takes the t r e f o i l concept fur ther and embodies the compact
In doing s o i t reduces i n t o a single thick annular graphite holder.
both R and q and theore t ica l ly very high ra t ings a re possible with
t h i s design.
redundant s t ructure the graphite s t ress ing p:roblems at the mid-plane
of the element a re qui te severe. Fig 7 shows some f i n i t e element
s t r e s s work which has been carr ied out by Agip Nucleare on a typical
t e l e d i a l design. This indicates t ha t very h:igh t ens i l e s t resses w i l l
occur on shutdown i n the outer r i m of the element and for t h i s reason
we conclude tha t the r a t i n g of the element needs t o be limited.
However, since the design i s essent ia l ly one of a heavily
Accordingly, the design point se t out i n Table 3 has been derated
t o an extent which meets a reasonable graphite s t ress ing cr i ter ion.
Being o f a tubular design, there i s again the problem of predicting
inner and outer surface temperatures and imbalance i n these can a l s o lead t o increased s t r e s s levels. Finally the larger amount of graphite
present tends t o produce marginally worse values of Nc/Nu.
Another aspect of the element i s t h a t the large numbers of very
small compacts require s l i gh t ly higher fue l f’abrication costs t o the
extent of perhaps 10% compared with a hollow rod element.
533
A l l t he se f a c t o r s m i l i t a t e aga ins t obtaining very l o w c a p i t a l and
generation cos ts , although the values s e t out i n Table 3 a r e s t i l l
q u i t e a t t r a c t i v e .
In t eg ra l Block Designs
For t he purpose of comparison we have taken the GGA block as published and assumed t h a t compacts can be f i t t e d i n t o t h i s with a
heavy metal density ad jus ted such t h a t t h e ove ra l l Ng/Nu r a t i o is
about 240 i.e. close t o optimum.
A point of i n t e r e s t is t h a t t he u t i l i s a t i o n of space within t h e
block is very e f f i c i e n t s o t h a t t h e heavy metal density i n t h e compact
can i n f a c t be reduced t o values of t h e order o f 0.6 t o 0.7 g/cc and
s t i l l a t t a i n t h e des i red uranium t o graphi te r a t i o s . Stemming f r o m
t h i s very high space u t i l i s a t i o n it i s poss ib le t o reduce f u e l volu-
metric r a t i n g s s o t h a t t he re a r e s i g n i f i c a n t decreases i n both R and q.
Thus, although t h i s type of element is t h e o r e t i c a l l y subject t o t h e
same s t r e s s i n g problems as t h e t e l e d i a l , t h e very much reduced para-
meters undoubtedly help it t o reach high r a t i n g s o f t h e s o r t s e t out
i n Table 3 before running i n t o s t r e s s i n g problems. The f a c t t h a t a
d i f f e r e n t graphi te with lower coe f f i c i en t o f thermal expansion is
being used w i l l a l s o mi t iga te t h e problem.
~
O n t h e o the r hand t h e s t r e s s e s due t o heat fluxes from t h e compacts
have t o be superimposed upon those developed i n t h e block as a whole
due, f o r instance, t o cross-block temperature and f l u x t i l ts . A
d e t a i l e d s t r e s s ana lys i s i s necessary t o define accura te ly t h e l i m i t i n g
conditions but, on t h e b a s i s t h a t t h e design point i s not l imi t ing ,
Table 3 includes some estimated costs.
It may be assumed t h a t s ince t h e graphi te f u e l p in components had
been de le ted i n t h i s type of design t h e f u e l cos t s may decrease by as much as 20% and the re fo re a f f e c t generation cos t s accordingly.
t h e other hand t i g h t ligament spacing may l ead t o higher r e j e c t r a t e s
which counter-balance t h e advantage. The c a p i t a l and generation cos t s
s e t out i n Table 3 therefore make t h e assumption t h a t i n addi t ion t o
On
534
s t r e s s ing pat terns and temperature l i m i t s being sa t i s fac tory , t he fue l
manufacturing costs a r e broadly i n l i n e with what would be expected
from the other types of designs.
Tubular In te rac t ing Design
In an attempt t o side-step the problem o f gap temperature differ-
ences altogether, t he tubular design can a l l o w the compact t o shrink
on t o the inner graphite sleeve. The outer gap then tends t o be
s t a b i l i s e d in its dimensions and i n any case i n carrying a smaller
heat flux. By use o f t h i s device it is possible t o r e s t r i c t fue l
maximum temperatures by 100 C compared with a non-interacting tubular
design o f t$e same rating. Furthermore, t he uncertaint ies on w a l l
temperatures a re now reduced. erature problem however, one now has t o take account of the s t r e s ses
induced i n the compact during operation. These a r i s e as a r e s u l t of
the d i f f e r e n t i a l shrinkage between compact and graphite; but shrinkage
r a t e s and the e f fec t o f compact creep a re such tha t the peak s t r e s ses
occur f o r a r e l a t ive ly short period of time. Calculations show tha t
they a re l imited t o values o f approximately 0.4 x UTS of the compact.
This s o r t of s t r e s s ing problem is indicated i n Fig 8 and Fig 9, which show the build-up o f nominal s t r e s s and a l s o t he e f fec t of
various uncertaint ies . Note tha t t he compact s t r e s s i s again dependent
on d i f f e r e n t i a l shrinkage r a t e s and is not a f fec ted by t h e f u e l ra t ing.
0
In exchange f o r s t a b i l i s i n g of the temp-
It is also desirable t o show tha t any re(3ctor t rans ien t does not
produce temperature d i s t r ibu t ion i n the graphite w a l l and compact which
can overstress t he compact beyond the normal loperating leve ls discussed
above. This bas ica l ly depends on coef f ic ien ts of thermal expansion
which a re f a i r l y well es tabl ished and s o far d o not appear t o be
1 i m i t ing.
It is possible t o envisage fu r the r development of an in te rac t ing
design i n which the compact is replaced by a Zuel bed which is cast
in tegra l ly in to the graphite sleeves. This type of design would remove
535
gap temperature differentials entirely but once again there would be
the problem of interaction between the compact and the graphite.
state of development of this approach is not yet clear and further work
requires to be done on it before it could be adopted for a prototype
react or.
The
COMPARISON OF DESIGN
All the above designs are capable of being built at the present
time and of using the materials currently available in the UK. All
of them are subject to material limits of one sort or another (fuel
temperature, graphite or compact stress) and Table 3 attempts to quantify the resultant capital and generation costs for designs at the
limiting parameter. These costs should not be regarded as absolutely
accurate since adjustments to the design point could produce different
numbers. Nevertheless, it presents a reasonable guide for comparison
of the various technically feasible designs and probably gives more or
less the correct economic ranking.
However, a selection of element cannot be based solely on economic
criteria alone and a degree of engineering judgement needs to be
injected, particularly to weigh the uncertainties which may be associa-
ted with each design.
As pointed out i n the Coated Pa r t i c l e Design section, there a re
likely to be few uncertainties in particle design apart from endurance
at elevated temperatures of 1400 C and beyond. 0
The Design of fie1 Compact section, in discussing the compact
design, shows that here also there is a high degree of confidence in
the ability to manufacture compacts of the required standard.
main task is to fill in irradiation data uncertainties and confirm the
shrinkage predictions.
The
The graphite which has been the basis of UK work up to the present,
is a fine-grained, high density isotropic graphite based on Gilsocarbon.
This is very well understood in terms of its irradiation performance
and mechanical properties. On the other hand, it is not matched to
536
t he compact i n terms of shrinkages at the point of in te res t . There is, Q therefore, a case f o r invest igat ing graphites with s l i gh t ly d i f fe ren t
cha rac t e r i s t i c s (higher shrinkage t o match gaps/lower coeff ic ient of thermal expansion t o reduce thermal s t resses , ) and it is hoped that t h i s
can be done before 1973. If it can be done, it w i l l r a i s e the l i m i t s of a l l the designs and although it is not l i ke ly t o a l t e r t h e i r economic
rankings it w i l l r e l ieve the pressure on design margins par t icu lar ly
those concerned with graphite and compact s t r e s ses e.g. t e l e d i a l and
tubular interacting. Such work, however, is not e s sen t i a l and designs
can be produced within the current materials r e s t r i c t ions .
The most important uncertainty a f f ec t ing element choice therefore
revolves around the pa r t i c l e endurance at temperatures of the order of 1400 C and above and t h i s therefore puts the main question mark against
the rod type elements which must operate at these temperature limits t o a t t a i n reasonable core ra t ings.
0
The apparent s implici ty of rod designs may therefore be misleading
and the se lec t ion of element probably needs -to be made between:
(a) the t e l e d i a l
(b) t he tubular in te rac t ing and ( c ) t he in tegra l block
as being the elements with most conservative fue l temperatures.
The t e l e d i a l is economically l e s s a t t r a c t i v e but i t s (graphi te
thermal s t r e s s ) l i m i t a t i o n may be deemed t o be the l ea s t worrying of
a l l s ince it is unlikely t o lead t o catastropic f a i l u r e o f t he element.
The tubular in te rac t ing design i s econoniically the most a t t r a c t i v e
and probably represents the ult imate as a long-term development.
t h i s respect, it would a l s o simplify the overal l development programme
if it was adopted as the element f o r the f i r s t s ta t ion . The question
mark over compact s t r e s ses depends upon accwacy of d i f f e ren t i a l
shrinkage data and, f o r t rans ien t considerations, coef f ic ien ts of
thermal expansion.
of a d i f fe ren t graphite) by 1973 there is no problem and it i s t h i s
In
If current data is confirmed ( o r improved by use
8
537
judgement which m u s t be made f o r it t o be adopted f o r a f i r s t -of f
stat ion.
The in t eg ra l block design represents an a l t e rna t ive which
cer ta in ly must be viable at t h e r a t ings being current ly employed and, s ince it i s similar t o the t e l e d i a l i n pr inciple , is t o be preferred
t o t he l a t t e r by reason of i t s r a the r b e t t e r economics. However, it is not qu i te so promising as the tubular in te rac t ing element, particu-
l a r l y i n the long term.
On balance, we conclude tha t t he tubular in te rac t ing element is
t o be preferred as the design of element f o r a f i r s t - o f f s ta t ion .
The in t eg ra l block would be a second choice and, indeed, there is
something t o be sa id f o r the view that each i s a back-up f o r the other.
1. H. B a i r i o t and G.M. Ehsley, Design and Development of Fuel f o r t h e HTR, Paper SM 11 1/24, IAEA, Conference on Advanced and HTGC Reactor Ju l i ch 21/25 October 1968
2. H. Bair iot , L. Aerts, R.A. Skinner and J. Vangeel, Fuel Development f o r a Low Ehriched HTR, Paper A Sect ion V Gas Cooled Reactors Information Meeting OFNL April 27 - May 1 1970.
Table 1. Parameters of Coatings i n BelgoNucleaire 800 p m Kernel Reference P a r t i c l e
Kernel
composition
dens i ty
diameter
Coatings
9 . C b u f f e r layer
th ickness
dens i ty
9 . C t r a n s i t i o n layer
th ickness
dens i ty
Inner HD eVC layer
t h i ckness
densi ty
BAF
Sic layer
th ickness
dens i ty
Outer HE QC layer
t h i ckness
densi ty
BAF
Reference p a r t i c l e
3 3 m 1.05 g/cc
3 O P 1.0 t o 1.7 g/cc
30 pm 1.8 g/cc
1.0 t o 1.1
3 5 w 3.2 g/cc
40 P 1.8 g/cc
1.0 t o 1.1
Table 2. Breakdown o f Costs f o r Two Different Tubular I n t e r a c t i n g Designs at 1.0 and 0.8 g/cm3
I A I B I I Fael pin a r e a cm2 I 8.8 I 11.0 1
HMD g/cc
Nc/Nu
Max. channel power kW
Construction cost E/kW
I n i t i a l uranium E/kW
I n i t i a l fabr ica t ion E/kW
T o t a l c a p i t a l E/kW Replacement uranium C./kW
Replacement fabr ica t ion E/kW
Other running cost E/kW
Total generat ion E/kW
700 2.2 1.2
1.1 1.1
This t a b l e se t s out t h e d e t a i l e d make-up of cost components f o r
c a p i t a l and generation c o s t s of two t y p i c a l designs. The c o s t s i n
E/kW a r e present worth values and a r e shown as d i f f e r e n t i a l s from s u i t a b l e datum costs.
c Table 3. Typical Design Points f o r various Element Types (1)
Hollow Rod Trefoil Tubular Non- Tubular In te rac t ing Teledial In te rna l Block In te rac t ing &hole desigc
Fuel Compact
mm mm
25- 4 42
- 19.0
39.5 54.4
39.5 54.4
- 12.5
- 12.7
Inside diameter Outside diameter
Pin Design
Inside diameter Outside diameter Lengt h Block Design
29.5 64.4 500
24.6 65.6 500
mm mm mm
- 52 500
- 29.0 500
- -
793
loa 41 .o 375 1000
36
422 1000
74. a 36 63.4 377 1000
36
422 1000
74. a 36 76 -6 436 1000
210
36 1 793
15.9 (X loa off) Pins per block Channel diameter mm Dimension across f l a t s mm Length mm Temperatures
Nommal fue l temperatures(2) :C Nominal max sheath C
temperature
Ratings
1185 9m
1085 920
1250 950
1210 a78
1123 910
Not known Not known
Mean fue l r a t i n g MW/Te 43.7 83.50 77.5 77.5 81.5 ( 5 ) 54.4
costs (4)
Mean core r a t i n g ~ / m 3 4.73 a. 60 a. 40 8.40 a. 65 6.11 Limiting fea ture (3) Fuel temp Fuel temp Graphite s t r e s s Compact s t r e s s Graphite s t r e s s Probably graphite
s t r e s s ing - Capital cost d i f f e r e n t i a l % Generation cost d i f f e ren t i a l %
+10 0 +6 +2
0 0
0 0
+5 +4 +3.3 0
- Notes ( 1 )
( 2 )
( 3 )
( 4 ) ( 5 )
These design points a r e typ ica l only, they a re probably close t o optimum within the pa r t i cu la r l i m i t s s e t i n each case
Fuel temperatures a re nominal maximum and do not include random and systematic e f fec ts . up t o about 150°C
Graphite and compact s t r e s ses a re se t at between 0.4 and 0.5 x UTS as a l i m i t . 14OO0C peak random with 12OO0C a more desirable l i m i t .
C o s t s a r e re fer red t o an a rb i ta ry datum
Graphite s t r e s ses t o o high i n t h i s design and downrating t o approximately 55 W/Te
These can r a i s e f u e l temperatures by
Fuel temperature maximum is assumed t o be
1s recommended in which case, costs a r e a s below
IO -
0
SIC THERMAL CR
CAP CLOSURE 0 E f W E i N KERNEL-BUFFEL AND INNER HD PIC
Fig 1 P a r t i c l e S t r e s s History
PIC IRRADIATION CREEP 4 I I ~ ~ ~ / ~ ~ ~ DNE SIC THERMAL CREEP ~
FUEL UOz 90% TD LIAS€ CASE PIC DENSITY 1.8glcm’
e ( I Oe. INNER PIC 10. OUTER P I C
I or rIt-sic , o r S i C - P r c
o--~ 2 3 1 ? rlO’lDtg
r
5 0
4 0
i a w 3 0 > U 2
Y 0 Y) YI w z Y v E 2 0
IO
I
BUFFER DENSITY I . 2 q l c n ’ / /
TEMP. 12OO0C
DOSE 4 ~ 1 0 ~ ~ DNE
I /‘ INIMUM THICKNESS REQUIRED TO ATTENUATE FISSION RECOILS
/
r?. F!M4
/ /
/ / I I I
/ /--
UO, ‘IoTD
85 9 0 95 97 .5 1
KERNEL DENSITY
Fig 2 P a r t i c l e Burnup as a Function of Kernel Density and Buffer La+yer Thickness
DIFFERERENTIAL GENERATION COST f / K W 0 N P W W
L z o D Z - ; s 3 4)s
z ;
0
I s
541
DIFFERENTIAL CAPITAL COST c / K W
N P W W 0 N - -
P z o z ; 3 - g o
> Z - D E
3 I 0 4 '=o
W 0
Fig 3 Graph of Cost v Mean I r r a d i a t i o n
U
2 2 0 2 4 0 260 280 3 0 0
MODIFUEL RATIO ( N ~ / N U )
FUEL TYPE T I DENSITY q / c c 1.0 PIN A R E A C d 11.0
Fig 4 Graph of Cost v Moderator t o Fuel Ratio
542
HOLLOW ROD TELEDI A L TUBULAR INTERACTING AND TUBULAR NON INTERACTING
OPERATING THERMAL STRESS IN 9 - HOLE TELEDIAL AT PEAK LINEAR RATING OF 8 7 0 wattrlcm DOTTED LINES SHOW DISPLACEMENTS STRESS IN psi . NEGATIVE IS COMPRESSIVE
Fig 8 Tubular Interacting Stress Patterns
544
140C
I 2oc
I oo( COMPACT STRESS p s i 80C
6OC
4 0 0
200
I
I I I I I x R E F CASE FOR THREE DIFFERENT
INITIAL CLEARANCES o 4 m m GRAPHITE WALL
2 4 6 8 IO I2 14 I 6 18 2 0
COMPACT HOOP STRESS AT BORE DUE TO INTERACTION AT 60% CORE HEIGHT
DOUBLING RATING INCREASES MAX S T R E S S 160 P S I 17% REDUCING GRAPHITE THICKNESS BY 2 0 %
IO”/, REDUCING RATING BY 10%
WORSENING SHRINKAGES B Y 2 0 %
DECREASING COLD CLEARANCE BY 8 0 p
INCREASING COLD CLEARANCE BY 80,u
REDUCES STRESS B Y 100 P S I
REDUCES S T R E S S BY IS P S I 2%
INCREASES !;TRESS BY 1 4 0 P S I 14%
INCREASES STRESS BY 100 P S I lOyo
DECREASES S T R E S S BY I S 0 P S I I6y0
Fig 9 Sensi t ivi ty of Tubular ]Interacting Stresses t o Parametric Changes
545
DISCUSSION
H. B. Stewart: We gave some a t t e n t i o n t o t e n s i l e stresses that might
arise i n the f u e l compact f o r the tubular i n t e rac t ing f u e l design.
the development of s t r e s s cracking i n some of the compacts present any
problems ?
Would
D. J. Merrett: It is obviously desirable t o avoid compact f r ac tu re
and t h i s i s why we would l i k e t o have high s t rength compacts so that the
p o s s i b i l i t y of f r ac tu re i s very low. If, however, t he re was a fracture ,
there a r e two aspects t o the problem. F i r s t ly , the temperature of the
compact might increase marginally t o a l i m i t which would approach t h a t of
a tubular noninteracting design.
t h i s increase i n temperature would be l imited and i s unlikely t o lead t o any rapid deter iorat ion i n p a r t i c l e i n t eg r i ty , pa r t i cu la r ly with the very
low f u e l temperatures chosen f o r t h i s design.
From Table I11 it can be derived t h a t
Secondly, the fracture might mechanically break a pa r t i c l e . More
evidence i s required on t h i s .
p a r t i c l e s when a compact i s fractured.
matic dis integrat ion ( in t e rna l pressure) of the compact and may be un- representative. A few p a r t i c l e f a i lu re s , however, would not be serious.
Some recent t e s t s have shown a few broken
These f r ac tu re t e s t s were by pneu-
R. A. U. Huddle: I would l i k e t o comment on three points. F i r s t l y , concerning the use of peak nominal.
say f r ac t ion of pa r t i c l e s . It is , therefore, important t o consider
not the nominal but the peak random as it is about f r ac t ion of f u e l that i s at or above this temperature. In comparison, therefore, the only
relevant parameter i s peak random as the difference between the nominal
and random f igures var ies g rea t ly f o r the d i f f e ren t designs.
We a r e interested i n a f a i l u r e of
Secondly, regarding the necessity f o r a high s t rength compact. It
i s beyond my comprehension why one needs high s t rength pa r t i cu la r ly f o r
the t e l e d i a l and any other noninteracting design. I n the in t e rac t ing
design, it i s the creep that matters and t h i s is a very d i f f i c u l t and
time consuming parameter t o evaluate. pacts as it just leads us i n t o v e m serious trouble i n fabr icat ion.
Let's forget high s t rength com-
Lastly, I disagree e n t i r e l y with the statement that f r ac tu re through
a compact w i l l c e r t a in ly break pa r t i c l e s . It is j u s t contrary t o a l l our
experience a t Dragon.
D. J. Merrett: 1. We agree t h a t peak random temperatures a r e impor- that. Parametric surveys have t o be conducted i n terms of nominal tempera- tures; i n picking a preferred design point, tne peak random m u s t be taken
546
i n t o account. t e l e d i a l o r noninteracting designs, and mat;:ix density could be reduced
although one should not loSe s i g h t of the?.mil conductivity advantages.
3. Creep is not a key parameter. O u r s t r e s s calculations have assumed
compact creep data the same as the graphite tube. The s i t u a t i o n i s l i k e l y
t o be b e t t e r than t h i s ; the danger of fracti lre might come from s t r a i n
l imitat ions. 4. High s t rength compacts can be fabricated without "very
serious trouble", as i s outlined i n the next paper.
t o Dr. Stewart, more work is needed i n the aspect of p a r t i c l e f r ac tu re on
breakage o f the compact. On ref lect ion, I agree t h a t Dragon evidence i s more applicable.
2. High s t rength compacts a:re not s t r i c t l y necessary f o r
5. A s pointed out
E. Smith: One must be careful i n applying the material data devia-
t ions s t a t i s t i c a l l y t o deduce allowable design s t r e s s l imitat ions since
some changes ( fo r instance, modules and s t r eng th ) a r e r e l a t ed changes.
W i l l the speaker indicate the cost penal t ies of t he t e l e d i a l design i f graphite stresses a r e not considered to be l imit ing.
D. J. Merrett: I n your f i rs t point, I agree. I n regard t o your
question, i f there were no s t r e s s i n g l i m i t , a close-to-optimum t e l e d i a l
design would be marginally more expensive than a tubular design i n t o t a l
generation aest , t o t he extent of perhaps one pound per kilowatt . This
stems bas i ca l ly from s l i g h t l y worse Nc/NU r a t i o s and s l i g h t l y higher core
pressure drops which have blower consumption penalties.
H. G i i t m a n n : The comparison between the d i f f e ren t designs depends
very much on the underlying assumptions. I n your comparison the t e l e d i a l
design i s r a the r heavily penalized due t o shutdown stress l imitat ions, as
you say. I think t h a t our philosophies a r e disagreeing on t h i s point and
my paper w i l l show a d i f f e ren t outcome of such a comparison. May I ask
you w h a t percentage of the ult imate s t rength you have assumed as design
l i m i t f o r your shutdown s t r e s s e s ?
P. U. Fischer : With bonded rods considerably higher metal loadings
could be reached.
f u e l element designs you presented? How would these a f f e c t the comparison of the various
D. J. Merrett: With our current design and one gram per cc compacts
it is just about possible t o reach optimum J!rc/Nu r a t i o s of around 240. Lower heavy metal dens i t i e s become more d i f f i c u l t t o accommodate, and de-
pending on design d e t a i l s t he re may be ove re l l generating cost penal t ies
approaching a typ ica l m a x i m u m of about 1 .5 pound per kilowatt . of 1.5 grams per cc compact would obviously ease the problem but would
FUEL DEVELOPMENT FOR A LOW ENRICHED HTR I_,,JL’rdilSi”l*.i---̂ - -,-_ l V T l i r . ~ I --,- ”. . * I ..,-Z,4?\c
L. Aerts BN 7 s’ b b o o u H. Bairiot BN R. A. Skinner TNPG W \
J. Vangeel S.C.K.-C.E.N.
BEL#GONUCLEAI RE The Nuclear Power Group Ltd Brussels Knu t s ford
Members of Inter Nuclear
and
Centre d‘Etude de 1’Energie Nuclgaire
Studiecentrum voor Kernenergie Mo 1
Abstract
The approach pursued for the design and development of a HTR fuel was outlined in a paper presented at the Jtilich Symposium held in October 1968 ’. The present contribution describes the continuation of the development work, the design aspects being covered in another pa- per * at the present symposium.
The optimum porosity of the kernel requires further investigation, since there is a discrepancy between the design predictions and some irradiation results. Fabrication techniques have therefore been deve- loped to cover the 85 - 95 % TD range. The kernel properties within this range are compared.
The coating layers follow the scheme proposed by the Dragon Pro- ject. Exemplative results are given on the variations of the dimen- sions and the properties within a batch and from batch to batch.
Various approaches to the manufacture of fuel rods are presently Some results of fabrication trials and proper- being pursued at Mol.
ties investigations are reported. The influence of manufacturing features may be of major importance in the selection of a fuel rod design. The cases of tubular and teledial rods are outlined.
An analysis of available corrosion data has been realized. The influence on the design of fuel pins is commented.
Some unusual irradiation features are reported, a s an illustra- tion of the programme pursued.
547
548
INTRODUCTION
The Belgian nuclear fuel industry has coordinated its actions within
the "Groupement Gen6ral du Combustible Nucl6aire" (G.G.C.N.). Three
companies : "BELGONUCLEAIRE" (BN) , "M6tallu:cgie Hoboken" and "M6tallur- gie et Mgcanique Nuclgaires" (MMN) are performing activities in the
field of HTR fuel.
The very close cooperation with the Belgian Study Centre for Nuclear
Energy (C.E.N. - S.C.K.) and the continuous contacts with the Dragon
Project have assared the availability of the necessary knowhow. A good
example of this ideal environment was the development and the manufac-
ture, in 1964, of plutonium base coated particles, the good behaviour
of which was demonstrated up to extreme burn-up (60 % fima up to lZO0°C)3
and temperature conditions (1850°C up to 20 % fima)4.
In 1967 the decision has been taken to concentrate in Belgium on
the industrial development of HTR prismatic fuel. BELGONUCLEAIRE, a
member of Inter Nuclear, has the leadership of this Belgian program and
insures the complementarity to the fuel development and design activities
of Inter Nuclear.
The fuel elements considered are described and their relative me-
rits compared in two other papers tothis meeting. The present paper
will therefore concentrate on one reference design shortly described
hereafter. But mentions will be made of the others whenever relevant.
For simplicity reasons, the nomenclature used is summarized in Table 1.
n
549
A typical prismatic fuel element is a 1000 mm long hexagonal
graphite brick 420 mm across flats, with eighteen 75 mm diameter
coolant channels. Each channel contains two annular fuel rods 64 mm
OD, 29 mm ID, by 500 mm long, cooled both internally and externally.
The fuel elements stack to form a free standing column of five or
six elements plus reflector and thermal shield units. Beside pro-
viding a structural support for the rods, the bricks provide the
graphite moderator, so that the whole core is replaceable.
A high uranium loading (density! and a long fuel life (MWD/TeU) 5 are desirable to achieve low fuel cycle costs . These considerations
have led to the choice of a fuel kernel of 800 microns diameter and
80 - 90 % TD uranium dioxide, surrounded by a triplex coating of
pyrocarbon and silicon carbide to give a nominal particle diameter
of 1100 microns. The indication of the behaviour of such particles
in a wide range of operating conditions is part of the Dragon Pro-
gram . 6
The fuel particles are embedded in a graphite matrix and packed
into the annular graphite sleeves which serve the dual function of
containing the particles and protecting them from corrosion by impu-
rities in the coolant. The fuel rods are manufactured separately
from the hexagonal brick, which is convenient for quality control and
avoids the rejection of a complete fuel element as a result of a de-
fect in one rod. We are presently using a fine grain isotropic gra-
phite for the sleeves with a trepanned fuel annulus to provide an
integral "closure" at the bottom end. The top closure is provided by
a graphite annular end cap.
OPERATING CHARACTERISTICS OF HTR FUEL
Based on the assessment of various fuel element types 1, 5, the
operating characteristics are summarized in Tables 2 and 3.
550
1 Table 1. Trper of HTR Fuel Elt-nts
Type Symbol Characteristics ~
Hollow rod
Tubular
Trefoil
Teledi a1
HR rods cooled externally only ; annular fuel region
Tu annular rods cooled from both sides
Tr rods cooled externally only ; three rods per coolant channel; plain fuel sticks
Te annular rods with plain fuel sticks
Integral block B1 plain fuel sticks, incorpo- rated directly in the block
Table 2. Derfrable Fuel Endurance L l d t r
Operating temperature 1300" C ':1400° C for HR)
Fraction of defective particles - start of life 10-5 - end of life 10-3
Minimum thermal conductivity 0.2 - 0.3 W/cm°C for HR
0.10 - 0.13 W/cmaC for Tu 0.03 - 0.14 W/cm°C for Te
and Tr
and B1
Heavy metal loading
Heat rating 0.3 W/particle (0.2 W/p for HR)
1.0 g ~ / c : m 3 (less for ~ 1 )
Gas release - R/B ratio 10- =
Burn-up 100 GWd/t (80 GWd/t for HR)
Residence time 800 d (1300 d for HR)
Table 3 . Desirable Graphite Endurance Limits
3 Graphite density 1.8 g,'cm
Mean temperature 800" c Peak surface temperature 1050' C
Thermal conductivity 1.2 W/cma c Maximum thermal expansion coefficient 10-6 1 OC Four point bend strength 200 kg/cm;!
551
REFERENCE SPECIFICATIONS AND MANUFACTURING RESULTS
I n a t y p i c a l HTR power p l a n t t h e f u e l i s subdivided i n t o 10" con-
t a i n e r s ; t h i s shows t h a t HTR f u e l i s a p e r f e c t ca se f o r s t a t i s t i c a l
t r ea tmen t s .
S p e c i f i c a t i o n s can be i s s u e d p r e s e n t l y t o use as a r e f e r e n c e ; but
i n d u s t r y , i n t h e f i e l d of r e a c t o r des ign and of f u e l manufacture , needs
t o check how c l o s e t h e t o l e r a n c e s can be kept and what i s t h e c o s t of
keeping and c o n t r o l l i n g va r ious t o l e r a n c e l e v e l s .
Most of t h e paper w i l l t h e r e f o r e be devoted t o our c o n t r i b u t i o n t o
t h i s a s p e c t . I t must be understood t h a t i t i s t h e p re sen t s t a g e and by
no means t h e f i n a l one o r t h e economical optimum.
KERNEL
Fuel m a t e r i a l
The uranium dioxide has been p r e f e r r e d t o t h e c a r b i d e f o r t h e
fo l lowing reasons :
- t h e dimensional s t a b i l i t y i s b e t t e r a t h igh burn-ups , - t h e oxide w i l l no t i n t r u d e i n t o t h e p y r o l i t i c carbon coa t ings under
7
6 normal temperature g r a d i e n t s , - t h e uranium contaminat ion i n t h e c o a t i n g l a y e r s can be kept t o a
much lower l e v e l dur ing f a b r i c a t i o n , which r e s u l t s i n a lower f i s s i o n
product release,
- t h e oxide i s much easier t o handle du r ing t h e f i r s t f a b r i c a t i o n s t e p s .
The oxide can a l s o be app l i ed f o r t h e thorium c y c l e ; i t i s a
must i n t h e case of plutonium p a r t i c l e s , as was demonstrated by the
J o i n t C . E . N . - BELGONUCLEAIRE Plutonium Group, i n c o l l a b o r a t i o n wi th
DRAGON 8.
552
Kernel s i z e
The f a b r i c a t i o n c o s t o f t h e c o a t e d p a r t i c l e s d e c r e a s e s when t h e
k e r n e l s i z e i n c r e a s e s up t o a k e r n e l d i a m e t e r around 900 mic rons . For
h i g h e r k e r n e l s i z e s , t h e f a b r i c a t i o n c o s t does n o t d e c r e a s e any more.
The p a r t i c l e s i z e i n f l u e n c e s a l s o t h e heavy m e t a l l o a d i n g and t h e
For a same volume l o a d i n g of c o a t e d p a r t i c l e s , t h e f u e l c y c l e c o s t '. heavy metal l o a d i n g d e c r e a s e s by 30 % when t h e k e r n e l s i z e i s p a s s i n g
from 800 t o 550 mic rons ; compensat ing t h i s by an i n c r e a s e of volume
l o a d i n g i s i m p o s s i b l e i n most cases ( C f P a r . 6).
The c o a t i n g o p e r a t i o n p r e s e n t s some problems f o r l a r g e s i z e s ,
i t i s f o r t h e moment s a f e t o c o n s i d e r 900 microns a s a l i m i t f o r t h e
k e r n e l d i a m e t e r .
Fo r t h e s e r e a s o n s 800 mic rons was s e l e c t e d as r e f e r e n c e d i a m e t e r .
The s i z e d i s t r i b u t i o n w h i t h i n a b a t c h and t h e r e p r o d u c i b i l i t y
from b a t c h t o b a t c h are f u n c t i o n of the m a n u f a c t u r i n g t e c h n i q u e . Typi-
c a l r e s u l t s are r e p o r t e d i n Tab le 4 , f o r t h e r o u t i n e powder agglomera-
t i o n t e c h n i q u e ( F i g . 1) and a r e p r e s e n t a t i v ' e g e l p r e c i p i t a t i o n p r o c e s s .
While t h e d i s t r i b u t i o n i s g a u s s i a n i n t h e h t t e r , i t i s n o t i n t h e
former ( F i g . 4 ) .
553
The significance of a close tolerance is unknown. It was reported
earlier that no correlation seemed to exist between the kernel diame-
ter and the coating thickness on particles coated in a same batch. Re-
cent information’ seemed to show the contrary. New. investigations
tend to confirm a likely compensating correlation during the coating
steps with thicker layers on the larger particles.
Density
The optimization of the average density is another field for fur-
ther investigation.Undoubted1y high porosities correspond to more con-
servatively designed particles. However, two factors af.fect adversely
the lower density kernels, all other things,being equal : a lower
strength (leading to a higher contamination of the coating) and an in-
creased number of cracked particles in a compact (due to the higher
volume loading required to reach a given heavy metal loading).
To illustrate this last statement, Table 5 summarizes the result
of a parametric survey‘ performed with the COCONUT code : the buffer
thickness was varied to such an extent that the stress level in the
Sic layer was the same, at the end of life, for all the kernel porosi-
t i e s .
554
Table 4. Kernel Charscteristics
Manufacture Powder Gel agglom.eration precipitation
Diameter ()I)
- average - reproducibility of the average of 400 particles
761 758
- 1 4 i 6 - 6 + 4
Density (g/cm3)
- average - reproducibility (on Hg density samples
10.0 10.8
i 0.2 + 0.1 - -
of u - average - reproducibility
1.985 + 0.005 -
2.005 - + 0.0035
Table 5. Influence of the Kernel Density ( X TD) on the Volume Loading (v/o) of Coated Particles i n the Fuel Region
Contamination l e v e l - before heat treat. fVC 5.8 . 6.9 . t o
2 . 10-6 - a f t e r heat t r e a t . fVC 3.5 . 1.1 . t o
5.6 . I
Table 12. Current Spec i f ica t ions f o r the Reference Fuel -
Layer Thickness (p> Density (g/cm3:
Buffer I + 6 33 - 1 1.0 + 0.08 -
Trans i t ion 30 5 1.6 - 1.7 I Inner PyC 30 + 5 -
Total PyC 95 2 10
36 + 5 -
1.8 + 0.05 -
+ 0.005 3 * 2 - 0.02 I Outer P ~ C 31 + 5 1.8 + 0.05 - -
Total coat ing 170 + 10 I -
'With a kernel 800 bfor a compact 40-50 mm OD and 32-39 mm I D .
diameter and 90 % TD and a 170 p t h i c k coating
564
FUEL RODS
The development work in Belgium is based on tubular fuel, as was
outlined in a previous meeting.
the delay necessary to demonstrate the behaviour of the consolidated
fuel have led to abandon, for the reference fuel, the process des-
cribed in 1968. The standard technique is now the fabrication of
compacts (Fig. 7 ) and their introduction in the graphite sleeve (Fig.8).
The good behaviour of compacts has indeed been demonstrated by Dragon6.
The advancement of fuel design and
565
Since this step is an important part of the fuel fabrication, the
consolidation alternative and an intermediate one are still being
pursued to a small scale.
Table 13.
The main characteristics are given in
Standard Compacts
The coated particles are overcoated by a resin impregnated gra-
phite powder, by the powder agglomeration technique, to a nominal dia-
meter of approximately 1600 microns. The density of the overcoating
layer is 1.6 - + 0.05 g/cm3 after drying, in a rough vacuum, below the melting point of the resin.
The particles are then loaded in the dies on a weight basis and
preheated to 100" C.
constant until a given height is reached. Upon completion of the
cycle, the block is transferred to an ejection press for hot ejection.
The pressure is applied gradually and remains
The heat treatment requires a close control of the heating cycle
up to 950" C and is performed in a continuous furnace in flowing inert
gas. The final treatment consists in
a vacuum degassing in a batch furnace for 2 hours.
The cycle duration is 8 hours.
Various raw materials are being tested in the frame of our pro-
gram (Fig. 9) . Standard specifications follow roughly the figures given in
Table 13.
tical background-is needed in this field, to assess the economic impli-
cations of the tolerances.
Representative results are given in Table 14; more statis-
566
I n S i t u Compaction
The c o s t of t h e process would be decreased and t h e dimensional
t o l e rances eased i f t h e compaction could be r e a l i z e d d i r e c t l y i n the
g r a p h i t e s l eeve . Pre l iminary t r ia ls have i n d i c a t e d t h e advantages
and drawbacks of t h i s technique, among which one may i n d i c a t e :
- t he absence o r t h e r educ t ion t o a low l e v e l of t he gap between the
f u e l and g r a p h i t e s l e e v e ;
- t he p o s s i b i l i t y of o b t a i n i n g a h ighe r HML (1 .3 t o 1 . 5 g U/cm 3 1;
- t h e l i m i t a t i o n of t h e m a t r i x d e n s i t y t o 1 . 3 t o 1 . 4 g/cm3 ma t r ix ;
- t h e presence of r a d i a l c racks through t h e compacts; t hese c racks
a r e however not' a f f e c t i n g t h e i n t e g r i t y of t h e coated p a r t i c l e s .
Advanced Consol ida t ion Processes
A l a r g e e f f o r t has been devoted i n 1967168 t o t h e s e l e c t i o n of
The only t h e c o n s o l i d a t i o n process t o o b t a i n 1 . 5 t o 1 . 6 g/cm3 HML.
r e t a i n e d technique c o n s i s t s i n t h e u t i l i z a t i o n o f a h igh v i s c o s i t y
phenol ic r e s i n mixed wi th g r a p h i t e powder and the i n t r o d u c t i o n of t he
p a r t i c l e s under in f luence of c e n t r i f u g a l f o r c e s .
Af t e r hea t t rea tment and degass ing , t h e ma t r ix m a t e r i a l con ta ins
80 % g r a p h i t e and has a d e n s i t y of 1 . 0 t o 1 . 2 g/cm3 ma t r ix , depending
on HML.
The a p p l i c a t i o n of t h i s technique , which al lows a l s o t o incorpo-
ra te d i r e c t l y t h e f u e l i n t o the g r a p h i t e s l e e v e and has t h e r e f o r e the
same advantages a s mentioned i n the prev ious paragraph, depends en-
t i r e l y on t h e i r r a d i a t i o n behaviour of such Euel beds. Furthermore,
i t s a p p l i c a t i o n i s r e s t r i c t e d t o f u e l concep'cs i n which t h e r a t i n g i s
n o t l i m i t e d by f u e l temperature ( e .g . Te and B l ) .
5 67
Furnace Overcoating
One of t h e c o s t l y s t e p s of t h e compact f a b r i c a t i o n i s t h e over-
coa t ing . I n o rde r t o decrease t h e c o s t , t h e powder agglomerat ion
overcoa t ing (Cf page 2 8 ) has been p a r t i a l l y rep laced by a low d e n s i t y
PyC l a y e r on top of t h e coa t ing . This overcoa t ing has the f u r t h e r
advantage o f p r o t e c t i n g the p a r t i c l e s from t h e f o r c e app l i ed by t h e
m a t r i x du r ing compression and al lows t o reach h ighe r volume loadings .
The a p p l i c a t i o n of t h i s technique depends e n t i r e l y on t h e i r r a -
d i a t i o n behaviour of t h i s type of f u e l beds.
CORROSION STUDIES
Corrosion s t u d i e s by Dragon have been summarized and have shown
t h a t t h e concen t r a t ion of water decreases r a p i d l y w i t h i n t h e c ros s -
s e c t i o n of t h e g raph i t e shea th surroundihg t h e f u e l over much of t h e
shea th temperature range: a mathematical model has provided a means
of c a l c u l a t i n g t h e p r o f i l e of co r ros ion a t t a c k i n depth beneath t h e
shea th s u r f a c e f o r given g r a p h i t e p r o p e r t i e s and has o u t l i n e d a
s imple means of c o r r e l a t i n g from 1 atm experimental r e s u l t s t o t h e
expected behaviour a t r e a c t o r p re s su re .
TNPG have extended t h i s work t o a r e a s not p rev ious ly covered
a n a l y t i c a l l y :
a ) t o provide a method of c a l c u l a t i n g t h e d i s t r i b u t i o n of co r ros ion
through t h e f u e l rod c ros s - sec t ion wi th p a r t i c u l a r r e fe rence t o
t h e lower temperature f u e l rods where g e t t e r i n g of t h e water i s
incomplete w i t h i n the g r a p h i t e s l e e v e s e c t i o n (Cf page 3 3 ) ;
b) t o provide a mathematical means f o r a l lowing f o r t h e changes i n
g r a p h i t e p r o p e r t i e s t h a t a r i s e from co r ros ion i n t h e i r e f f e c t on
subsequent co r ros ion i . e .
568
i)
ii)
iii) to compute i) and ii) for various pressures from the 1 atm
on the resultant depth of corrosion attack,
on the change in corrosion kinetics with burn off,
pressure of experiments up to the reactor pressure case which
cannot readily be examined experimentally (Cf pages 41. to 4 3 ) .
Two reaction regimes are important :
a) the chemical regime where the reaction rate is constant within the
graphite section, diffusion replenishment of water always being
rapid in relation to the point reaction rate;
b) the 'in-pore diffusion' regime where diffusion replenishment is
slow and reaction depletes the local water concentration at some
zone within the graphite to a very small! fraction of the surface
water concentration, but where no water depletion occurs in the gas
external to the geometric surface of the specimen.
Two-Zone (Sleeve and Fuel Matrix) Corrosion with Linear Temperature Gradients without Imposed Flow
In a reacting porous graphite medium Wicke has shown that the con-
centration of corrodent under diffusion conditions is governed by:
Transforming this using :
via a Bessel equation : .-I
2 dLY d Y 2 Y - 2 + Y d y - y 3 ' = o
dY
has a solution :
( 3 )
I
Y (y) = A K (y) + B I (y) 0 0
( 4 )
569
Since the properties of the two regions are different separate
solutions are obtained for the two regions and by applying four boun-
dary conditions, four linear simultaneous equations are obtained
Gpplying the sheathlfuel boundary condition :
f d7) y=y1 =D(") 2 dY Y'Y1
these simplify to :
: on
(5)
Definition of Symbols :
7 = mole fraction of oxidant at a point, relative to its concentration at the outer surface,
5 - - distance of the particular point from outer surface, d, cm , wall thickness, L1, cm
T O = Thiele modulus or catalyst number,
k mo 9 g = L1 Def f
Y
= rate constant per gram for graphite chemical reaction rate 0 3 -1 -1 mo k
at T K,cm g sec , 0
- 3 Pg = apparent density of graphite, g cm ,
2 -1 n = diffusion coefficient of water in STP helium, cm sec ,
570
a
Q
R
T
T 0
Y
YO
A and B
e f f e c t i v e d i f f u s i o n c o e f f i c i e n t oJ wate the porous g r a p h i t e s t r u c t u r e , cm’- s ec , D and D being t h e p a r t i c u l a r values w i t h i n t h e shea th and f u e l m a t e r i a l ,
i n helium whi th in -€ 2
-2 , and d e s c r i b e s t h e i n c r e a s e i n r e a c t i o n r a t e due t o 2 R T
0
temperature g r a d i e n t ,
-1 mean a c t i v a t i o n energy of ox ida t ion r a t e k c a l . mole ,
Gas c o n s t a n t ,
0 Temperature a t po in t i n ques t ion , K ,
0 Temperature at outer surface, K ,
QO a
- Y
are func t ions independant of y but dependant of d i s t a n c e up A and B B a r e t h e corresponding s p e c i f i c va lues
2 1’ 2 t h e channel : f o r t h e s h e a t h and f u e l zones r e s p e c t i v e l y ,
1 K (y> and I (y> are modif ied Bessel func t ions of o r d e r zero wi th K and I being t h e corresponding f i r s t o r d e r func t ions , 0 0
1
and y are t h e boundary i t e m s of y a t t h e shea th i n n e r f ace and Y 1 2 f u e l c e n t r e l i n e r e s p e c t i v e l y ,
P = t o t a l gas p r e s s u r e , a t m . ,
0 -2 -1 = chemical r e a c t i v i t y of t h e g r a p h i t e a t T K , mg cm h ,
-1 p a t i n H 2 0 , kT
= l o c a l burn o f f a t any p a r t i c u l a r p o s i t i o n . BL
571
These were solved us ing a Gaussian e l imina t ion procedure t o cal-
c u l a t e t h e v a r i a t i o n of co r ros ion r a t e wi th depth beneath t h e s u r f a c e
of t h e p i n shea th and t h e f u e l compact material .
F igu res 10-13 show t h e co r ros ion p r o f i l e s c a l c u l a t e d f o r a series
of channel p o s i t i o n s i n an e a r l y HTR des ign and show
t r a n s i t i o n from two zone t o in-pore d i f f u s i o n co r ros ion a s temperatu-
res r ise a long t h e channel .
c l e a r l y t h e
With regard t o r e a c t o r a p p l i c a t i o n , c a l c u l a t i o n o f t h i s two zone
c a s e i s dependant on t h e allowed water conten t and hence on t h e cor -
ro s ion assessment of t h e o v e r a l l co re . F igures 10-13 are thus only
i n d i c a t i v e of behaviour. There i s a l s o a need f o r improved d a t a on
t h e parameters r e l e v a n t t o co r ros ion f o r shea th and f u e l material .
This method of a n a l y s i s i s only v a l i d where t h e r e i s no s i g n i f i -
c a n t change i n r e l evan t g r a p h i t e p r o p e r t i e s as a r e s u l t of co r ros ion :
f o r t h e p r e s e n t two zone cases computed so f a r , t h e e x t e n t of l o c a l
co r ros ion i s low enough t o avoid s i g n i f i c a n t change i n p r o p e r t i e s .
Table 14. Experimental Resu l t s on Compact Manufacturing
Aver. Cont ro l Method Spread. Accuracy C h a r a c t e r i s t . S p e c i f i c a t . I o b t a i n .
+ 1 % Y count ing U235 content N + - 4 % N + - 2 % -2% + 0% - 1.0+ 0.05 0.97 0.96 - 0.98 + 0.02 talc. - - HMTA
Weight N + - 2.5% N + - 3% -4% +2% - Outer @ N + - 0.05 N + - 0.04 -0.03 W.01 - Inner 8 N + - 0.05 N + - 0.02 -0.01 N.01 - Height (mnd N + 0 .5 N + - 1.5 -1.5 +1.5 - Contam.fVC < 10-7 10-5 - 10-8 unknown d count ing F r a c t i o n broken p a r t . 2 x < 0 - 3 x unknown d e s i n t e g r . I
N i n d i c a t e s t he nominal va lue f o r each c h a r a c t e r i s t i c .
572
A
Corrosion Ca lcu la t ion where Local Proper ty Changes occur
The above mathematical model does no t iillow f o r a v a r i a t i o n i n
g r a p h i t e s t r u c t u r e a r i s i n g from corros5on. However a t t he h igh l o c a l
burn o f f s nea r t h e e x t e r n a l s u r f a c e of h igh temperature f u e l s l e e v e s ,
t h e p o r o s i t y of t h e g r a p h i t e s t r u c t u r e w i l l be opened up al lowing
easier i n - d i f f u s i o n of water.
I n t h e a n a l y s i s above, t h e t e r m rp i nc ludes a f a c t o r D e f f which i s t h e e f f e c t i v e d i f f u s i o n of water i n the porous medium.
This can a l s o be w r i t t e n :
1 . 7 5 T D = D A(- (-1 e f f o 2 7 3 . 2 ) P (10)
where
d i f f u s i o n c o e f f i c i e n t of H 0 i n H e i n porous medium of g r a p h i t e
d i f f u s i o n c o e f f i c i e n t of H 0 i n He: i n f r e e gas cond i t ions
h = 2
2
Using t h i s and t h e t rea tment of Wicke i t can be shown t h a t :
O f t hese only k and A could change as a r e s u l t of l o c a l co r ros ion . T
There i s evidence from Dragon work t h a t l a r g e changes i n A a r i s e from
co r ros ion : w h i l s t k must be expected t o change the e x t e n t i s unknown
and i n t h i s a n a l y s i s changes have been a sc r ibed t o h only (but could
a l t e r n a t i v e l y be considered as a change on the r a t i o of k f o r t he
T
T - corroded s t a t e compared t o t h e uncorroded) . A
573
From equat ion 11 and f o r i so the rma l cond i t ions each p r o f i l e of l o g
(cor rodant concen t r a t ion ) p l o t t e d a g a i n s t depth i s a s t r a i g h t l i n e of
c h a r a c t e r i s t i c s lope f o r t h e p a r t i c u l a r A value .
0
The l o c a l burn o f f a t t h e s u r f a c e i s dependant on ly on t h e chemi-
c a l r e a c t i v i t y of t h e g r a p h i t e and a t cons t an t temperature and coolan t
water con ten t i n c r e a s e s l i n e a r l y wi th t i m e , u l t i m a t e l y reaching
1000 mg/g
t h i s s u r f a c e a co r ros ion p r o f i l e which i s a composite of a l l t h e cumu-
l a t i v e co r ros ions a t each p o i n t a l lowing f o r t h e changes i n g r a p h i t e
p r o p e r t i e s t h a t have occurred p rogres s ive ly up t o t h e p o i n t burn up
reached. Fu r the r co r ros ion w i l l n o t change t h i s p r o f i l e bu t w i l l move
t h e whole p r o f i l e bod i ly inwards.
-1 , When t h a t s t a g e i s reached t h e r e then e x i s t s beneath
To compute t h i s p rogres s ive b u i l d up of co r ros ion a l lowing f o r t he
change of g r a p h i t e p r o p e r t i e s , a programme has been w r i t t e n which eva-
lua tes t h e p r o f i l e of cor rodant concen t r a t ion f o r convenient ly small
s t e p i n c r e a s e s of s u r f a c e l o c a l burn o f f , s a y 10 mg/g (and hence a spe-
c i f i c t i m e i n t e r v a l ) , t ak ing account of t h e s e l e c t e d t o BL c o r r e l a -
t i o n .
Thus t h e i n i t i a l s t e p s w i l l have t h e s l o p e c h a r a c t e r i s t i c of t h e
of the virgin graphite. However when the local burn off of
layers beneath t h e s u r f a c e reaches t h a t a t which a change i n occurs sr then the s l o p e - f o r t h e a f f e c t e d l a y e r w i l l be decreased t o t h a t 6d
c h a r a c t e r i s t i c of A f o r t h a t burn o f f : hence t h e co r ros ion occur r ing
i n t h i s a f f e c t e d l a y e r i n t h e s p e c i f i c t i m e i n t e r v a l can be c a l c u l a t e d .
Thus f o r each success ive 10 mg/g i n c r e a s e i n s u r f a c e burn o f f ,
t h e cor rodant concen t r a t ion p r o f i l e i s computed t ak ing t h e h va lue
a sc r ibed t o t h e burn o f f t h a t t h e l a y e r had reached a t t h e s t a r t of
t h i s p a r t i c u l a r pe r iod and hence t h e p rogres s ive co r ros ion i n depth
can be c a l c u l a t e d and t h e t o t a l co r ros ion and co r ros ion ra te eva lua ted
f o r each 10 mg/g s t e p . Thus the cumulat ive co r ros ion c h a r a c t e r i s t i c s
are eva lua ted u n t i l t he equ i l ib r ium p r o f i l e i s reached.
574
There is insufficient published evidence to establish an adequa-
te h to B correlation. However some Dragon work did show experi-
mentally determined (local corrosion) /depth profiles for specimens
corroded at 1 atm. He pressure. Therefore various h / B correla-
tions were arbitarily taken and used to compute the expected corrosion
profile for the experimental conditions until a reasonable similarity
of corrosion profile and corrosion kinetics was obtained. This work
indicated that the A / B correlation was: L
i ) far from linear being more sigmoidal in form,
L
L
ii) appeared to tail out to a A value well below unity.
Considerably more data is neededto allow better evaluation of
this h / B correlation and also to determine whether k varies sub- L T
stantially with B L '
Since all the known experimental determinations of graphite cor-
rosion kinetics have corroded the specimens :in low pressure gas and
since the mathematical model shows that rigorous prediction of the
high pressure corrosion kinetics must take account of the variation of
graphite properties with burn off, the model is considered to be of
considerable value for reactor corrosion predictions and ultimately to
have scope for development for reactor operation core corrosion mana-
gemen t .
It is to be noted thatthis treatment is not absolutely rigorous
in that there is a discontinuity in - whereas in the treatment de- scribed on page 3 3 the method used avoids this discontinuity because
the properties of the graphite are considered constant. However com-
parison runs against a rigorous routine have shown that the difference
is insignificant.
dY
575
I RRADI AT1 ON BEHAVI OUR
Our program i s e n t i r e l y focused towards t h e demonstrat ion of t h e
behaviour of HTR f u e l ; i t i s n o t broad enough t o inco rpora t e r e sea rch
a s p e c t s , f o r which w e r e l y e n t i r e l y on t h e Dragon P r o j e c t .
The ma jo r i ty of our i r r a d i a t i o n s are t h e r e f o r e s tandard endurance
tes ts performed i n t h e BR 2 and BR 3 (Mol) and the DRAGON r e a c t o r ;
most of them are s t i l l i n progress o r have been r epor t ed elsewhere.
Only two examples where new r e s u l t s are a v a i l a b l e w i l l be r epor t ed
he re .
T rans i en t Tests
This series of t es t s i n v e s t i g a t e s t h e response of t h e f u e l t o
power su rges , r e s u l t i n g i n e i t h e r a sudden i n c r e a s e of t h e r a t i n g ,
e i t h e r a h igh temperature , e i t h e r a s t e e p temperature g r a d i e n t , o r
more than one of t hese phenomena a t a t i m e . The program s t a r t e d wi th
f r e s h f u e l and extreme cond i t ions :
- power inc reased i n 30 min.,
- a t power du r ing 2 h r s ,
- p a r t i c l e r a t i n g : 0.08 - 0.11 Wlpa r t i c l e and 1 . 3 - 1 . 9 Wlpar ic le ,
- average g rad ien t up t o 400" C/mm ( a t 2200' C),
- max. temperature over 2700" C .
As expected, t h e p a r t i c l e s d i d no t su rv ive t h e extreme g r a d i e n t
and temperature cond i t ions . The se t of r e s u l t s f i t f a i r l y w e l l t he
des ign c o r r e l a t i o n proposed by t h e Dragon P r o j e c t . 6
Evolut ion of Heat Trans fe r C h a r a c t e r i s t i c s
The b o i l i n g water capsu le , u t i l i z e d s i n c e many years for our plu-
tonium program has been modified f o r t h e i r r a d i a t i o n of coated par -
t i c les .
10
576
The internal cavity usually filled with the sodium-potassium
alloy and the fuel rod is occupied by the sample with the gap between
the sample and the heat diffuser filled wtth helium.
The prototype capsule is presently being irradiated and contains
specimens of fuel 15 mm diameter comprising a graphite can and a fuel
stick of coated particles. These fuel sticks comprise holes in which
thermocouples are inserted, so that at all. times and in various sections
along the fuel length, the heat rating, some surface temperature and
the central temperature of the sample are recorded. From those data,
the heat transfer properties can be assessed; it depends on the lo-
cation of the thermocouples (the maximum number of thermocouples
available is 24) whether it is the overall heat transfer coefficient
or the thermal conductivity between two paints of the fuel samples
which is measured. In our present program only centrally located
thermocouples are inserted so that the central temperature of the
specimen and the graphite sleeve temperature are known.
Since the irradiation is being pursued, the available results are
preliminary in nature and cannot be interpreted until postirradiation
examination is performed. As illustration, Fig. 14 shows the evolu-
tion with time of the thermal conductivity, calculated from the ins-
trumentation data; it relates to consolidated fuel specimens of the
type described on page 31 operating in two ranges of temperature
gradients. Fig. 15 compares the rough data obtained under irradiation
(CEB) with the results of measurements performed at KFA (Jtilich) in a
thermal conductivity rig, under very different thermal gradient and
heat rating conditions. Fig. 16, incorporating data of the two spe-
cimens, seems to indicate a thermal gradient dependance.
Although various interpretations of these results are possible at
this stage, a discussion would be premature, the purpose of this pre-
sentation being only to illustrate the utilization of an irradiation
facility.
Q
Q
577
CONCLUSIONS
The purpose of our program is to contribute, to the extent of our
possibilities, to the development effort of the organizations active
in the field of HTR fuel.
A large part of our effort is aimed towards providing statistical
and tolerance data to the fuel and core designers.
The reliability of the fuel behaviour is also being investigated
and demonstrated. Since the design methods and data of Inter Nuclear
Member Companies are utilized to mount the tests and/or to interpret
the results, an important fall-out is also obtained in the design of
the fuel. A particular example was given for the corrosion problem.
Finally our aim is also to test and demonstrate that appropriate
HTR fuel can be manufactured by industrial techniques, on the basis of
the experience made available to the signatories by the Dragon Project.
ACKNOWLEDGEMENT
The authors wish to acknowledge the collaboration of many sources
and individuals of their organization, for helping in carrying out the
program.
A special mention needs to go to the Dragon Project for providing
back ground data,_contributing with stimulating discussions and coope-
rating directly to some parts of the program (e.g. irradiations).
The corrosion work described on pages 32 to 43 was carried out
for TNPG Limited by D. Birch and P. F. Arthur of International
Research and Development Co, Ltd.
578
REFERENCES
1.
2 .
3.
4 .
5.
6.
7 .
8.
9.
H . B a i r i o t , G.M. Emsley and J . M . Thomson, Design and Development of Fuel f o r t he HTR, Symposium on Advanced High Temperature Gas- Cooled Reactors , J u l i c h , Oct. 1968, IAEA - SM 111/24.
D . J . Merret't and M. Gaube, Choice of Fuel Design f o r Homogeneous Low Enriched HTR , Paper presented a t t he present Symposium (Sess ion V - Paper 126) .
M.T.S. Pr ice , H. B a i r i o t and A . Klusmann, Plutonium Fuels f o r Feed and Breed HTR Concepts, Paper presented a t t he Symposium on Advancad a d High Temperature Gas-Cooled Reactors , J u l i c h , 1968.
P. Barr , N. P o l l i t t e t a l . , High Temperature I r r a d i a t i o n Experi- ments on Plutonium Bearing Coated P a r t i c l e Fue l , Paper presented a t t he Symposium on the Use of Plutonium a s a Reactor Fuel , Brusse l s , March 1967.
H . B a i r i o t e t a l . , Some f e a t u r e s of t he low enr iched HTR f o r va r ious f u e l element des igns , Paper presented a t t he present Symposium (Sess ion 6 - Paper 135) .
L.W. Graham, The development and i r r a d i a . t i o n performance of HTR core m a t e r i a l s , Paper presented a t t h e present Symposium (Sess ion VI.
J . M . Thomson, Computation f o r coa ted p a r t i c l e f u e l design, BN 6911-05, Nov. 1969, BELGONUCLEAIRE, B russe l s .
G.W. Horsley e t a l . , The manufacture of plutonium f u e l l e d f i s s i o n product r e t a i n i n g coa ted p a r t i c l e s f o r i r r a d i a t i o n i n the DRE, Symposium on t h e Use of Plutonium as a Reactor Fuel , Brusse ls , March 1967.
H . B i l d s t e i n ( S G A E ) , P r i v a t e communication.
10. A . Lhost, Rigs f o r i r r a d i a t i o n i n BR2 of f u e l f o r f a s t r e a c t o r s , I n t e r n a t i o n a l Conference on F a s t Reactor I r r a d i t i o n Tes t ing , Thurso, Cai thness , Scot land, A p r i l 14-17, 1969.
57 9
Fig. 1. Kernels manufactured by powder agglomeration.
F i g . 9 . Inf luence of the raw m a t e r i a l on the t e x t u r e of t h e mat r ix .
0 2 0.4 0.6
D e p t h i n g r a p h i t e , cm
F i g . 11. Corros ion p r o f i l e a t t h e 37.5 cm
l e v e l a t peak random t e m p e r a t u r e .
D e p t h i n g r a p h i t e , cm D e p t h in g r a p h i t e , cm
F i g . 10 . C o r r o s i o n p r o f i l e a c r o s s a n n u l i a t t h e channe l i n l e t a t peak random t e m p e r a t u r e
F i g . 12 . C o r r o s i o n p r o f i l e a t t h e 100 cm l e v e l a t peak random t e m p e r a t u r e .
D e p t h i n g r a p h i t e , crn
F i g . 1 3 . C o r r o s i o n p r o f i l e a t t h e 137.5 c m l e v e l a t peak random temperaLure .
584
0.02-
DEC
I
c o n d u c t i v i t y of c o n s o l i d a t e d f u e l ( i r r a d i a t i o n tempera-
\ .%- /
I I I I F i g . 14. Evo lu t ion of t h e
:u L U ~ L i l r r a d i a t i o n
4 I
I 1 ! I 20 Lo
I 4
I A
REA+R C Y C ~ E
I I 9o-1zarlmnj 1 ,I 1 ,/, 1
- 1 1 1
thermal c o n d u c t i v i t y of t empera tu re 500-700°C).
I I 10 20 BURNUP
GWd/ t
l _ _ I - I I I I - l _ l 500 640 700 O C
AVERAGE FUEL TEMPERATURE
F i g . 15 . I n f l u e n c e 3f t h e ave rage t empera tu re o n t h e the rma l c o n d u c t i v i t y of c o n s o l i d a t e d f u e l .
585
DISCUSSION
K. Hackstein: You showed a range of coating thicknesses of 10 m i - crons i n your s t a t i s t i c a l t e s t s . coating batches t h i s w a s obtained?
Could you indica te on what s i z e of
H. Ba i r io t : The s t a t i s t i c a l data w e reported were obtained from fabr ica t ion o f f u e l f o r a c r i t i c a l i t y test. nels avai lable , the necessi ty f o r insuring a minimum quant i ty of waste
and the des i re t o gather s i g n i f i c a n t s t a t i s t i c a l data l e d us t o s e l e c t one kg HM as a coating batch s ize . Undoubtedly the range of coating thicknesses would be l a r g e r f o r l a r g e r coating batches.
The l i m i t e d quant i ty of ker-
HTR FUEL AND MATERIALS DEVEL-OP+MENT& IN GE.R,M-ANY, * 1
PRESENT SITUATION AND PROGRAM
B. Liebmann J . Bug1 K. E h l e r s K. G. Hackstein
ABSTRACT
The German HTR program includes fuel and graphite development and i r radiat ion testing. The work is ca r r i ed out jointly by the German industry and the r e s e a r c h center KFA Julich. P r e s s e d spherical fuel e lements have been produced and loaded into the AVR since 1 9 6 9 and will be used for THTR. The experience obtained with the AVR and the r e su l t s of i r radiat ion t e s t s indicate that these elements will per form well in THTR and a r e well suited f o r larger power reac tors . Pa ra l l e l w o r k on pr ismatic fuel e lements has beeil s ta r ted and will be increased in the coming yea r s . Design data on the i r radiat ion induced changes of the physical propert ies of commercial ly available and newlry developed graphites for fuel elements and re f lec tors is provided by irradiation t e s t s up to l ife-t ime doses . In addition a r e sea rch and development program f o r new types of graphite for HTRs has been s tar ted.
INTRODUCTION
The German high temperature r eac to r development is backed up
by increasing efforts in fuel and mater ia l s development. These
a r e concentrated in a cooperative German Fuel and Mater ia ls
586
- . . . . . . . - . . . . . . - - - - - - .
587
Program for HTRs which serves for the development of fuel ele-
merits and graphites with special consideration for the following
reactors and; projects:
AVR 15 MWe in operation
THTR 300 MWe beginning of construction in 1970
HHT 600 MWe design study to be completed in 1973
The work on fuel and fuel elements is carried out by the companies
Brown Boveri/Krupp (BBK), Gutehoffnungshutte (GHH), NUKEM
and the Kernforschungsanlage Julich (KFA). The reactor building
companies BBK and GHH a r e mainly responsible for fuel element
design and specification development. NUKEM fabricates the fuel
and develops fuel element materials and production processes.
Graphites for High Temperature Reactors a r e developed by Sigri
Elektrographit and Ringsdorff-Werke. KFA is responsible for
a l l irradiation tests including post-irradiation examination and
contributes to materials research and development. The work is
sponsored by the German government and supported by close
cooperation with the Dragon Project. The activities can be sub-
divided into work on coated particles, fuel elements and graphites.
Each of these sections includes irradiation testing.
COATED PARTICLES
Fuel Kernel Preparation
The (U, Th)C fuel particles of approximately 0. 32 mm diameter
presently used in the AVR fuel elements a r e still produced by
an agglomeration technique and subsequent melting in a bed of
graphite powder. I t is envisaged that we wil l change to oxide
2
63
588
particles in 1971. These will then be used for follow-up charges
of the AVR as well as for the THTR and HHT. Production
equipment for oxide particles has been set up and is used for the
fabrication of particles for irradiation tests. The particles a r e
produced from an emulsion by a surface tension method and
sintering. In addition sol-gel-processes for UO and (UTh)02
particles of diameters up to 1 mm ha.ve been developed on a
laboratory scale.
@
2
Coating De po s it ion and Characterization
The fuel particles for AVR and THTR have pyrocarbon coatings
only, while direct cycle helium turbine plants a s studied in the
HHT project probably will require a silicon carbide interlayer.
Fluidized beds with a capacity up to 5; and 5 kg per batch have
been developed for production coating. Studies on the influence
of deposition parameters on coating properties a r e presently
concentrated on Sic and on coatings o'btained from propylene.
Emphasis is given to the characterization of coating structures
and properties before and after irradiation. Two new methods
have been added to those existing: and optical method called
Optaf for determining the anisotropy of pyrocarbon and a method
for measuring the modulus of elasticity and the rupture strength
of outer coating layers. Optical determinations of the anisotropy
a r e the only methods which can be applied directly to the coated
particles. The modulus of elasticity and the rupture strength a re
calculated from values obtained by pressing the coated particles
between two parallel plates and measuring deformation and force.
For the pebble bed reactors AVR and THTR, spherical fuel elements
of 6 cm diameter wil l be used. Whether spherical or prismatic fuel
elements wil l be utilized in the HHT wil l be decided at a la ter stage.
Spherical Fuel Elements for Pebble Bed Reactors
Most of the development work on fuel elements has been performed
for the spherical fuel elements of AVR and THTR. At present the AVR
operates with the three types of fuel elements shown in Fig. 1 . The
589
Model Work and Irradiation Testing
Specification tes ts and tes ts for the comparison of the results of
model calculations with actual coated particle performance have been
carr ied out up to doses of n/cm2 (E. 0 , l MeV) and will be
continued on an increasing scale. The influence of time, temperature
and burn-up especially with respect to solid fission product diffusion
is studied in the Dido reactor of KFA which has low fast flux. The
effects of high fast neutron doses a re investigated by tes ts in the
ments of this type have been loaded into the AVR since 1969 and
wil l be used for THTR and a r e considered for HHT.
3
Fig. 2. shows a crossection of one of the UCC fuel elements 2 1 2 n/cm irradiated in AVR for 8-10 % fima and a fast dose of 1 . 2 ~ 1 0
(E) 0, 1 MeV). Spearhead attak has started, but did not lead to
an increased activity in the reactor. Fig. 3. shows particles in
a pressed sphere after irradiation in the test SK 1 to 10 70 fima 2 1 2 and a fast dose of 2 . 2 x 10 n/cm ( E ; 0 , l MeV). The excellent
performance of the two balls irradiated in this test was also
demonstrated by the small fission gas release of R/B =
2 x 10 for 133 Xe, which was well below the specified value -5
of R / B = 5
Fig. 4. gives a survey on the irradiation of spherical fuel
elements in various tests and in the AVR. The numbers in the
circles indicate the numbers of fuel elements irradiated in the
tests. Circles with an arrow indicate the present burn-up and
59 1
dose of tests which a r e still in progress. The guarenteed
values for the fuel elements of THTR have been reached by the
tes ts SK 1 and SK 2. SK 2 wil l reach more than 14 7’0 fima and
a fast dose of 6.4 x 10
SK 3 wil l reach these values by the middle of 1971. In the THTR
le s s than 10 of the fuel elements leaving the reactor will have
reached these values which a re 20 70 above average.Future tes ts
of the SK ser ies wil l include irradiation of feed elements to
70 % fima and a fast neutron dose of 4 x 10 and of breed
elements to 14 70 fima and a fast dose of 8 x 10
2 1 n/cm2 (E> 0 , l MeV) during 1970.
- 4
2 1
2 1 2 n/cm .
In one experiment at Julich spherical elements were tested 37
days at a rating of 8 kW per element (instead of the maximum
design value of 3 . 3 kW) and with surface temperatures of
1400 OC (instead of 1000°C). No damage was observed.
Fig. 5. shows how temperature and rating of a fuel element
during its runs through a pebble bed reactor a re simulated by
the SK tests. The figure demonstrates that the fuel temperature
in the test is always above the fuel temperature in the reference
reactor. This creates more stringent conditions than the r e -
ference case and thus provides for sufficient safety of the de-
monstration.
Tests of the graphite matrix of the pressed elements in the DFR
have demonstrated that no detrimental changes occur a t the
maximum life-time dose of 6.4 x 10 n/cm , 21 2
The experience with the fuel elements of the AVR and the available
results of irradiation tests indicate that the pressed fuel ele-
ments a r e well suited for THTR and larger power reactors.
592
Prismatic Fuel Elemeints
Despite of the encouraging results obtained with the spherical
fuel elements parallel work on prismatic fuel elements has been
started and will be increased in the future . The deve-
lopment of matrix materials and fabrication techniques for fuel
compacts is based on experiences from the pressed spherical
fuel elements and on Dragon know-how. The influence of compo-
sition, temperature of pyrolysis and other parameters on the
properties of materials for compacts and to a smaller extend
for bonded beds a r e being systematically investigated. Annular
compacts and smaller samples for materials development a r e
being irradiated to various doses up to 6 x 10
(E> 0 , l MeV) in Dragon, DFR Dounreay and MTRs.
2 1 2 n/cm
GRAPHITE
Design data on the irradiation induced changes of the physical
properties of commercial types of graphite for prismatic fuel
elements and reflectors is obtained from irradiation tests in
DFR Dounreay, Dragon and MTRs. A Gilso carbon graphite
will used for the inner reflector of the THTR. Its maximum 2 2 2 life dose wil l be 1. 2 x 10 n/cm (Dido Ni) at temperatures
0 between 300 and 1000 C. This dose has been surpassed in
UKAEA tests with AGL graphites and will be reached in our
tes ts with Sigri graphites in May 1971.
In additional programs new graphites for HTRs a r e being deve-
loped and the influence of composition and fabrication parameters
on the irradiation behavior is being tested. Studies on the
fe sibility f repla ing Gilso carbon by various other raw materials 0
and on special forming methods like isostatic pressing and vibra-
tory compaction a re included. The reproducibility of promising
types is being checked by production runs.
24 000 4400 15 000
Fig. 1. Types and Amounts of Fuel
Elements Presently Used in the AVR
594
F i g . 2 . Particle of a n UCC-Fuel
E l e m e n t I r r a d i a t e d in AVR 2 1 2 8-10 70 fima, 1 . 2 ~ 1 0 n / c m (E > 0 . 1 MeV)
A
595
A
Fig. 3. Particle of a P r e s s e d Fuel
Element I r radiated in SK 1 Tes t
1 0 . 5 70 fima, 2x10 2 1 n/crn2 ( E b O . 1 MeV)
Fig. 4. Irradiation Tests of Spherical
Fuel Elements
NORMALIZED TIME FOR THE RUN OF A FUEL ELEMENT THROUGH THE CORE
Fig. 5. Fuel Temperature in the THTR
and in Fuel Demonstration Tests SK 2 and SK 3
597
DISCUSSION
J. H. Coobs: Could you comment on th relative a rits of spherical
and prismatic fuel elements for HTGR's and on the present status of devel-
opment and testing?
B. G. Liebmann: Thank you for this question, which gives me a chance
to make some propaganda f o r the spheres. As far as I can see they have
two advantages: 1. There is production and irradiation experience with
spherical fuel elements. Spherical fuel elements are being produced for
the AVR and have been irradiated up to doses and burnups as guaranteed for the finished core of THTR. For irradiation behavior we do not have
to rely on tests of small fragments of fuel elements which is the case for prismatic elements. We have tested the complete elements. 2. Pebble
bed reactors have the advantage that only a few fuel elements see the
highest temperatures and this only f o r a few days of their lifetime. In
reactors with block type elements the same elements remain under the most
severe conditions for a long time. Also the worst fuel temperatures seem
to be lower in pebble bed reactors than in reactors with prismatic fuel
elements and the same outlet gas temperature. There are, of course, also
disadvantages to pebble bed reactors, but these are not concerning the
fuel elements themselves. As I have said in the paper, we are now also
engaged in the development of prismatic fuel elements. One reason for
this is our belief that international collaboration is required to bring HTR's to a success.
tic fuel elements also.
Therefore, we want to be prepared to produce prisma-
Paper 8/133
J. Baier W. i n d e r Schmitten P. Walger
ABSTRACT
The f a s t - neut ron damage of s e v e r a l types of pyrocarbon coated p a r t i c l e l a y e r s was i n v e s t i g a t e d by two i r r a d i a - t i o n experiments i n t h e Dounreay F a s t Reactor (DFR) . The maximum f a s t dose accumulated i n both experiments was 5.5-1021 n/cm2 and 14.6.1021 n/cm2 ( E > 0 , 1 8 KeV) respec- t i v e l y , t h e temperature 1300OC. The r e s u l t s i n d i c a t e t h a t dens i ty and Bacon an i so t ropy f a c t o r (BAl?) of pyrocarbon l a y e r s determine the i r r a d i a - t i o n behavior . We found, however, t h a t a d e n s i t y of about 1.90 g/cm3 and a BAF of about 1.03 a lone do n o t guaran-
:eIegFE2Y n/cm2. I t i s assumed anocher proper ty which was n o t measured i n t h e experiments t o be important a t such high f a s t f l u x i r r a d i a t i o n s .
a r t i c l e s t o remain i n t a c t a f t e r a dose of
INTRODUCTI OIJ
Stresses i n t h e l a y e r s of coated p a r t i c l e s are mainly due t o t h e f o l l o -
wing e f f e c t s :
- b u i l d up of gas p re s su re between ke rne l and coa t ing
- a n i s o t r o p i c thermal dimensional changes
- i n t e r a c t i o n s between ke rne l and coa t ing arid between t h e coa t ing
layers
- f a s t neut ron induced dimensional changes of pyrocarbon.
I n o r d e r t o s tudy the in f luence of t he f a s t neut ron f l u x on coated par-
t i c l e behavior s epe ra t e ly , two i r r a d i a t i o n experiments i n the Dounreay
F a s t Reactor (DFR) were c a r r i e d out by the Thorium-IIochtenperatur-Reak-
t o r - (THTR) Assoc ia t ion i n t h e l a s t t h r e e yea r s .
598
599
E xp e r imen t DN 1
F u l l power days 50
Maximum f a s t 5,5 10 2 1 dose ( E > 0,18 MeV)
Temperature 1 3OO0C
Burn up < I Z fima
IRRADIATION DATA
DN 2
96
14,6 10 2 1
I 30OoC
ti I fima
The two Dounreay i r r a d i a t i o n experiments d i f f e r mainly i n t h e i r r a d i a -
t i o n t i m e and t h e accumulated f a s t dose. Table 1 shows some d e t a i l s of
t h e i r r a d i a t i o n da ta .
DESCRIPTION OF TEST SPECIMENS
I n both t e s t s a v a r i e t y of d i f f e r e n t p a r t i c l e ba tches was tested.Most
of t h e p a r t i c l e s were of t h e BISO type , i . e . t h e UC2 - k e r n e l w a s
coated by a porous b u f f e r l a y e r and a dense pyrocarbon o u t e r l aye r . F i g . 1 shows a metallographic section of such a particle with dimen-
s i o n s used mostly i n t h i s t es t . The porous b u f f e r l a y e r provides volume
f o r t h e f i s s i o n gases and decouples the o u t e r l a y e r from the ke rne l
mechanically. The o u t e r l a y e r i s the p r e s s u r e ves se l f o r t h e f i s s i o n
gases and t h e d i f f u s i o n b a r r i e r f o r t h e s o l i d f i s s i o n products .
The BISO type p a r t i c l e s i n t h e s e experiments can be d iv ided i n t o seve-
r a l d i f f e r e n t series, i n each of which one parameter i s s y s t e m a t i c a l l y
va r i ed . These parameters a r e ke rne l composition, l a y e r t h i ckness and
p r o p e r t i e s of t h e o u t e r l a y e r pyrocarbon.
From each ba tch 40 s p h e r i c a l p a r t i c l e s wi th equal l a y e r t h i cknesses were
s e l e c t e d f o r i r r a d i a t i o n by means of radiographs. Thus i t was c e r t a i n
t h a t t he r e s u l t s of t he i r r a d i a t i o n were c l ea r - cu t : A l l p a r t i c l e s of a
batch f a i l e d o r a l l p a r t i c l e s remained i n t a c t .
600
F A S T NEUTRON INDUCED D I ? E N S I O N A L CIIANGES
S ince t h e f i s s i o n ra te i s very small i n t h e Dounreay t e s t , t h e o u t e r
l a y e r i s put i n t o stress only by t h e f a s t neut ron induced dimensional
changes of t h e pyrocarbon. Therefore these t:ests can be considered more
as a s p e c i a l material t es t than as a coated p a r t i c l e t es t .
Fast neut ron induced dimensional changes of f r e e pyrocarbon specimens
were measured f o r i n s t a n c e by GGA . Fig. 2 shows t h e s e changes f o r d i f -
f e r e n t types of pyrocarbon. The curves a r e ex t r apo la t ed up t o t h e maxi-
mum dose reached i n D€J 2. They show t h a t a t t h e maximum dose, f o r in-
s t a n c e , a 1,9 g/cm pyrocarbon would s w e l l i n r a d i a l d i r e c t i o n by 330 X whi le i t would s h r i n k i n c i r c u m f e r e n t i a l d i r e c t i o n by about 42 %. These
dimensional changes are even h ighe r a t h ighe r d e n s i t i e s o r BAF - values .
I n pyrocarbon l a y e r s of a coated p a r t i c l e those changes must be belanced
by stresses and creep.
To ana lyze t h e stresses i n t h e l a y e r s of coated p a r t i c l e s models have 3 been developed, f o r i n s t a n c e ) by Prados and S c o t t
and Walther (SORIN)4. These models take i n t o account a l l t h e e f f e c t s
presented h e r e a t t h e beginning, but they can a l s o be used f o r calcula-
t i o n s of t h e stresses induced by dimensional changes only. Ca lcu la t ions
w i t h the models of Prados, S c o t t and Walther have been made and compared
wi th t h e r e s u l t s of t h e experiments desc r ibed here . Our r e s u l t s were
found t o be i n a good agreement wi th t h e c a l c u l a t i o n s .
1
3
Kaae (GGA)
RESULTS
In f luence of t h e o u t e r l a y e r t h i ckness on p a r t i c l e behavior
I n one series of four ba tches t h e o u t e r l a y e r t h i ckness w a s va r i ed from
30 um t o 150 um. A f t e r i r r a d i a t i o n i n DY 2 the p a r t i c l e s of t he four
ba tches were examined under t h e per i scope and a l l of them were found t o
be i n t a c t . I n t h e meta l lographic s e c t i o n , however, r a d i a l c racks were
found i n t h e 115 and 150 um t h i c k l a y e r s which a rose dur ing s e c t i o n i n g .
(Fig. 3 ) . These c racks i n d i c a t e t h a t t h e r e were h igh t e n s i l e s t r e s s e s
i n t h e l a y e r s n e a r l y as h igh as the rup tu re stress. Another e f f e c t is
I I
/
601
@ seen i n F ig . 3: The th i cknesses and t h e p o r o s i t y of the b u f f e r l a y e r of
t h e two p a r t i c l e batches d i f f e r a f t e r i r r a d i a t i o n . The b u f f e r of t h e
p a r t i c l e w i th the t h i c k e r o u t e r l a y e r seems t o be t h i n n e r and less po-
rous than t h e b u f f e r of t h e o t h e r p a r t i c l e which had a t h i n n e r o u t e r
l aye r . This i n d i c a t e s t h a t much more p re s su re i s put on t h e b u f f e r by
the shr inkage of t h e t h i c k e r l a y e r . I n f a c t , model c a l c u l a t i o n s confirm
these observa t ions .
In f luence of t h e pyrocarbon p r o p e r t i e s
The in f luence of pyrocarbon p r o p e r t i e s on the i r r a d i a t i o n behavior of
t h e p a r t i c l e s has been found more important than a l l t h e o t h e r parame-
t e r s s t u d i e d i n both the DN 1 and DN 2 experiments.
The fo l lowing pyrocarbon p r o p e r t i e s were i n v e s t i g a t e d :
1 . Densi ty: measured both on pyrocarbon d i s k s and on c o a t i n g fragments
by t h e s ink-f loat-method,
2. O r i e n t a t i o n an iso t ropy , s p e c i f i e d as Bacon-anisotropy f a c t o r (BAF)
measured by an x-ray d i f f r a c t i o n technique on d i s k s and by an o p t i -
cal method on meta l lographic s e c t i o n s of p a r t i c l e s ,
3. Apparent c r y s t a l l i t e s i z e : measured by an x-ray d i f f r a c t i o n technique
on d i sks .
It w a s n o t p o s s i b l e , however, t o vary a l l t h e s e parameters independent- l y in methane deposited layers and this complicates the interpretation
of t h e r e s u l t s .
The pos t i r r a d i a t i o n examinations show t h a t p a r t i c l e layers remained
i n t a c t on ly when d e n s i t y and B M a r e below a c e r t a i n l i m i t . These l i m i t s
d i f f e r f o r t h e two expe r inen t s , they are shown i n Table 2. A n i n f luence
of t h e c r y s t a l l i t e s i z e could no t be found.
Table 2: P r o p e r t i e s of pyrocarbon l a y e r s which remained i n t a c t i n DFR
experiments
DN 1 Experiment I BAF
Densi ty [ g/cm3 ]
L 1 , 2
1.6 - 2.05
DN 2
c 1,05
1.6 - 1.95
602
Damage mechanism of t h e pyrocarbon l a y e r s
The fo l lowing damage mechanism of t h e p a r t i c l e l a y e r s h a s been observed:
A t one p o i n t of t h e o u t e r s u r f a c e t h e l a y e r c r a c k s towards t h e i n n e r
s u r f a c e and many c r a c k s s t a r t from h e r e and s p r e a d i n r a d i a l d i r e c t i o n s .
The p a r t i c l e looks l i k e an opening f lower . A f t e r c r a c k i n g , t h e stresses
i n tlie pyrocarbon are auch lower t h a n b e f o r e and t h e r e f o r e t h e pyrocar-
bon can change i t s dimensions as shown i n F i g . 2. The F i g u r e s 4 and 5
S!IOT.~ t h i s h i s t o r y s c h e m a t i c a l l y on two p a r t i c l e b a t c h e s ~ 7 h i c h seem t o
have been d e s t r o y e d a t d i f f e r e n t times i n t h e i r r a d i a t i o n h i s t o r y
Tlinensional d ianpes and a n i s o t r o p y changes of i n t a c t p a r t i c l e s
I n t h e DN 2 experiment t h r e e p a r t i c l e s were t a k e n from n e a r l y each b a t c h
and were i r r a d i a t e d as i n d i v i d u a l p a r t i c l e s . The dimensions of t h e s e par-
t ic les have been measured p r e c i s e l y by rad iography b e f o r e and a f t e r i r ra-
d i a t i o n . I n a l l cases a d e c r e a s e of t h e o u t e r d i a m e t e r w a s found. The
porous i n n e r l a y e r d e n s i f i e d about 39 Z and we found a c e r t a i n d e c r e a s e
i n t h e IJC
k e r n e l s d i d n o t change. Some d e t a i l s of two p a r t i c l e b a t c h e s are g iven
i n Table 3 .
Anisotropy h a s been measured on m e t a l l o g r a p h i c s e c t i o n s b e f o r e and a f t e r
i r r a d i a t i o n . As e x p e c t e d , t h e BAF v a l u e s i n c r e a s e d s t ronp , ly ; f o r i n - 21 s t a n c e , from EAF = 1.00 t o BPJF = 1.30 a f t e r a f a s t dose of 14.6010
n / c n .
k e r n e l d iameter t o o , w h i l e t h e d i a m e t e r s of t h e ( U , T h ) 0 2 2
2
Changes of d i n e n s i o n s and d e n s i t y of broken l a y e r s
Pyrocarbon t h i c k n e s s e s of broken l a y e r s were measured and compared w i t h
t h e o r i g i n a l t h i c k n e s s . The comparison shows a s w e l l i n g of pyrocarbon
w i t h an o r i g i n a l d e n s i t y of 2.1 g/cm3 and an BAF v a l u e of 2 . 0 up t o a
f a c t o r 5 t o 6 . The s w e l l i n g of pyrocarbon w i t h lower o r i g i n a l d e n s i t i e s
and BAF - v a l u e s w a s lower. These swell f a c t o r s were found t o be i n a
good agreement :Ji t h e x t r a p o l a t e d d imens iona l change c u r v e s of GGh
( f i g . 2 ) .
1
603
Density measurements were made on pyrocarbon fragments of all the bat-
ches which failed in the experiment DN 2.
Original densities of the different batches lay between 1,6 and 2,l
g/cm3 and after irradiation to 14,6 IO2* n/cm2 densities of all char- 3 ges were in the range of 1.8 to 1.9 g/cm .
Discussion of the results
A s shown before density and BAF value determine the fast neutron irra-
diation behavior of pyrocarbon layers on coated particles. But we found
in the DN 2 experiment that these conditions are necessary but not suffi-
cient. Some batches of particles failed at the same irradiation condi-
tions although their density and anisotropy fulfilled the conditions
mentioned above. However, the conditions used in depositing the outer
layers, especially the deposition rate,differ for the batches which
remained intact and which failed.
In this manner, we came to the conclusion, that there are one or more
other pyrocarbon properties which were not investigated in the present
experiments but which are obviously of great influence under the extreme
irradiation conditions of the Dounreay experiments. Therefore some ef-
fort is now being made on measurements of mechanical properties of par-
ticle layers (Young's modulus) and of the non-crystalline contents
within the pyrocarbon layers .
C ONC LUS I O N S
The irradiation experiment DN 2 shows that coated particle pyrocarbon
layers with certain material properties deposited from methane can with-
stand extreme high fast neutron fluxes up to double the dose reached in
high temperature gas-cooled reactors at the maximum. Those properties
are: density 1.6 to 1.95 g/cm , BAF <1,05 with the additional condition that the deposition rate has to be greater than 100 um/h.
Results of the DN 1 experiment indicate that these values are less cri- tical up to the maximum fast dose of an HTGR. (density: 1.6 to 2.00
3 g/cm , BAF c 1.2)
3
/
604
U n i r r a d i a t e d
REFERENCES
I r r a d i a t e d
Q
B u f f e r I Outer Layer I Thickness
Kernel
Diameter
HTGR Base Program, Quater ly P r o g r e s s Report f o r the P e r i o d Ending May 30, 1969, GA - 9372
Kernel
D i aime t er
J . W . Prados, J .L. S c o t t , Nucl. Appl. 2, 488 (1967)
375
390
J.L. Kaae, J. Nucl. Mat. - 32, 322 (1!)69)
z
4 3 65 -' 3
40 150 -' 4
H. Walther , S t r e s s Analys is i n Coated Fuel P a r t i c l e s , DP Report 604, August 1968
- 28
- 36
n .
+ IS
+ 13
Table 3: Dimensional changes of i n t a c t coa ted p a r t i c l e b a t c h e s a f t e r 14.6 IO"
n/cm2 (E70,18 MeV) a t 130O0C, burn up c 1 2 fima.
Batch
MAUC 51
MAUC 53
Changes of
B u f f e r I Outer Layer
Thickness
n
605
dense, isotrope layer
,buffer l a y e r
-kernel
+ LOO p m
10 pm
65 p m
Fig. 1 . BISO - Coated Part ic le
Fig. 2 . Bulk Dimensional Change Versus Fast Neutron Exposure for Different Pyrocarbons, Irradiated a t 1250°C. (af ter GGA’)
+ 150
+ 100
+ 50
0
- 50
, I I I I I I
0 2 4 6 8 10 12 14 16 - neutron exposure (10 n l c m I
606
Dose: 14.6 * 102 'n /cm2 ( E >0.18 M e V )
Temperature: 1300 O C
Burn u p : 0.2 % f ima
U C 2 - kernel , LOO pmi$ Buffer layer : 40 pm
65 pm Outer layer 150 pm
Fig. 3. Influence of Outer Layer Thickness on Coated Particle Behavior in High Fast Neutron Flux.
Fig. 4 . Damage of Coated Particle Pyrocarbon Layers by Irta- diation Induced Dimensional Channes. (schematic: Drawing).
Fig. 5 . Damage of Coated Particle Pyrocarbon Layers by Irra- diation Induced Dimensional Changes.
607
DISCUSSION
D. M. H e w e t t e : We+have been doing parallel coa ted -pa r t i c l e t es t s i n
t h e H F I R t a r g e t reg ion ob ta in ing results a t s l i g h t l y lower temperatures
(1100°C) t h a n yours b u t a t f l uences near your va lues .
h igh d e n s i t y i s o t r o p h i c propylene coa t ings d e n s i t i e s as h igh as 2.07
grams pe r CMQ and f i n d t h a t these coa t ings surv ive . Tes t s a t GGA suggest
t h a t propylene coa t ings don ' t i nc rease i n an iso t rophy n e a r l y as much as do methane. Do you p l an t o t e s t propylene der ived coa t ings i n t h e f u t u r e ?
We have tes ted
J. Baier : Yes, w e have such p a r t i c l e s i n t h e H F I R HT-5 t e s t and a r e
awa i t ing eva lua t ion . However, w e c a n ' t compare these coa t ings d i r e c t l y
wi th methane because of low c r y s t a l l i t e s i z e s .
D. M. Hewette: The c r y s t a l l i t e s i z e of t h e propylene coa t ings can
be increased by h e a t t rea tment t o g ive va lues t h e same as f o r h igh t e m -
pe ra tu re methane coat ings.
J. Baier : We d i d n ' t i n c r e a s e the c r y s t a l l i t e s i z e by heat t rea tment
i n our f irst experiment. But i n our f u r t h e r experiments w e w i l l do so.
J. L. S c o t t : What i s t h e mechanism of change i n p re fe r r ed o r i e n t a -
t i o n of p y r o l y t i c carbon under i r r a d i a t i o n ?
J. Baier : I cannot f u l l y answer t h i s ques t ion a t t h e moment. It can be assumed, however, t h a t t h e inc rease i n p r e f e r r e d o r i e n t a t i o n i s due t o creep.
D. Tytga t : I want t o complement Dr. Graham's and Dr. Liebmann's
comments on t h e i r r a d i a t i o n i n fast r e a c t o r s . Dr. L. Valette from
Euratom proposed l a s t y e a t a t t h e AIEA, June 1969, meeting i n Vienna t h a t
f o r g r a p h i t e i r r a d i a t i o n s , a good c o r r e l a t i o n e x i s t s between t h e d i f f e r e n t
dimensional changes measured i n d i f f e r e n t r e a c t o r s f o r temperatures as h igh as 12OOoC, i f t h e appropr i a t e cor rec ted temperatures are ca l cu la t ed by using t h e same a c t i v a t i o n energy Q = 1 . 2 e v as Dr. Simmons from Harwell.
This va lue w a s proposed i n i t i a l l y for temperatures up t o about 500°C. It would be i n t e r e s t i n g t o see i f t h e same e f f e c t i s observed f o r pyrocarbon
i r r a d i a t i o n s performed by d i f f e r e n t l a b o r a t o r i e s . Could Dr . B i e r com-
ment on how h is data f i t t e d wi th t h e o thers?
608
J. Baier : We compared ou r dimensional measurements b o t h on broken
l a y e r s and on f ree pyrocarbon specimens wi th t h e ex t r apo la t ed curve o f
GGA and found a r a t h e r good agreement. Our va lues t e n d t o be a b i t lower
than those of t h e ex t r apo la t ed curve.
K. Wirtz: I n one of your experiments p a r t i c l e s w i th h igher coa t ing
d e n s i t i e s cracked t o a h ighe r degree than those wi th longer ones. Do you
t h i n k t h a t wi th h igher temperatures and longe r t i m e s f o r t h e i r r a d i a t i o n
t o t h e same dose, i . e . , i r r a d i a t i o n i n a lower f l u x would g ive b e t t e r re -
s u l t s ? More genera l ly , what i s t h e in f luence of temperature and f l u x
d e n s i t y on your result ? Is t h e i r i n f luence of i n t e r n a l c r e e p ?
J. Baier: The ques t ion concerning t h e in f luence of h igher fast neu-
t r o n f l u x i s no t yet answered by experiment. Therefore , w e are ju s t plan-
ning experiments, f o r in s t ance , i n t h e HFR-Petten up t o same fast f luences
as i n t h e DFR experiments.
bon specimens a s t r o n g in f luence of t h e temperature on t h e dimensional
changes and on creep behavior was found. I n our experiments w e could not i n v e s t i g a t e t h e in f luence of temperature bec'zuse t h e fas t f luence w a s
lower a t lower temperature .
I n t h e work of GGA (Bokrus) on f r e e pyrocar-
L. W. Graham: I would l i k e t o m a k e a cmment on t h e re levance of
i r r a d i a t i o n s under t h e h igh-acce lera ted fast f l u x condi t ions i n DFR. A g r e a t d e a l of work has been publ ished r e l a t i n g t o low temperature i r r a d i a -
t i o n i n DFR on g r a p h i t e s developed f o r t h e AGR. Much of t h e concern i n
t h i s work has been wi th c o r r e c t i o n f a c t o r s which have t o be app l i ed t o
t h e temperatures t o g ive a n "equiva len t i r r a d i a t i o n temperature"; equiva-
l e n t t h a t i s , t o a temperature i n a power r e a c t o r possess ing a much lower
fast f lux . From experiments done on g r a p h i t e i n bo th DFR and on g raph i t e
t e s t r i g s i n t h e HFR-Petten where t h e i r r a d i a t i o n temperatures were t h e
same and h ighe r w e f i n d q u i t e d i f f e r e n t dimensional changes i n d i c a t i n g
t h a t l a r g e equ iva len t temperature co r rec t ions have t o be made f o r h igh
temperature g r a p h i t e i r r a d i a t i o n i n DFR. The c o r r e c t i o n i s a downward
one and can be s e v e r a l hundred degrees cent igrade . It i s d i f f i c u l t t o
j u s t i f y such co r rec t ions t h e o r e t i c a l l y by t h e methods used previous ly f o r
t h e low temperature AGR work. I pe r sona l ly b e l i e v e t h a t t h i s i s a conse-
quence o f t h e temperature dependence o f i r r a d i a t i o n c reep above 500°C.
. . . . . . . . . . . . .
609
A downward equivalent temperature correction describes the correction for the displacement i n the crystals , hut the creep occurs equivalent t o the
ac tua l i r r a d i a t i o n temperature. All t h i s leads me t o believe t h a t i r r a - d i a t ion of graphite n a t e r i a l s a t high temperatures i n the DFIi a r e only of qua l i t a t ive use.
Paper 9/116
I cqG
b'? K. G. Hackstein
ABSTRACT
More than 20,000 of the so ca l led molded f u e l elements were made f o r t he AVR-Reactor. A c r i t i c a l examination o f the most impor t an t data obtained during f ab r i ca t ion of kernels coated p a r t i c l e s and spheres ind ica tes that t he production o f l a rge amounts of t h i s f u e l elements can be achieve@ without ser ious d i f f i c u l t i e s . Further development work has t o be done w i t h respect t o t he reproducib i l i ty o f some properties.
Introduction
I n addi t ion t o a c t i v i t i e s i n the development o f production methods f o r kernels, coated p a r t i c l e s , prismatic f u e l elements including blocks, we a r e now producing f u e l elements f o r the AVR-Reactor.
The Am-Reactor needs about 18,000 f u e l elements per year. Since May 1969 the reac tor has been reloaded with the s o ca l l ed molded fue l elements developed by Nukem.
We now have made more than 20,000 f u e l elements o f t h i s type and will give a s h o r t review of the experience and r e s u l t s during t h i s production.
Fuel Element Design
The spheres contain 6 g heavy metal :in the f o r m o f U r a n i u m / Thorimcarbid ( r a t i o i s 1:5) kernels coated with a dup1ex l aye r o f pyro ly t ic carbon. The thicloiess o f the inner l aye r i s i n the order of 50 microns and the density i s about
and the density w a s designed t o be 2 2,OO g/cm3 f o r t he f irst 1 g/cm 3 . The thickness o f t he outer :Layer i s 120 microns
610
611
5 batches, but w a s then reduced t o 2,00f2,4 homogenized batch w a s 30 - 40 kg coated p a r t i c l e s ) .
g/cm3 (one
Based on i r r a d i a t i o n r e s u l t s it may be necessary l a t e r on t o reduce the density even more, but for t h e burnup conditions t h i s i s not now a very i m p o r t a n t question.
Carbide coated p a r t i c l e s a r e used, because they have been s u f f i c i e n t l y t e s t e d as loose p a r t i c l e s as well as embedded i n spheres. We will employ oxide coated p a r t i c l e s as soon as the i r r a d i a t i o n t e s t s for f u l l burnu fima) and the desired fas t dose (7 I O ” nvt) a r e finished. These t e s t s a r e under way a t Studsvik the fast dose i s now about 3,5 t o 4 IO2 ’ nvt (E 12 - 1 3 76 f i m a .
(more than 12 %
0 , l MeV) and t h e burnup i s
Coated P a r t i c l e s
So fa r we have produced about 600 kg coated p a r t i c l e s o f t he carbide type which have been used f o r b o t h t he e a r l i e r wale paper and molded spheres, but mainly f o r t he l a t t e r . During production the following proper t ies have been measured on the dense melted carbide kernels.
,
Uranium/Thorium r a t i o Carbon content Density Spherici ty
On coated p a r t i c l e s we have measured
Thickness o f the buf fer l aye r Thickness o f t he outer l aye r Density o f t he outer l a y e r Anisotropyfactor o f t he outer l aye r Surface contamination.
Table 1 represents some data o f kernels and coated p a r t i c l e s obtained from 17 batches.
612
T h i s measuremerbs were made on batches o f about 20 kg heavy metal resp. 40 kg coated par t ic les . In addition microradio- graphic and metallographic measurements were made i n order t o detect Uranmigration, cracks etc.
Para l le l t o t h i s the reproducibil i ty of the coating conditions was controlled by measuring the thickness o f the inner and outer layer of 18 single coating batches. One batch was 1 kg heavy metal.
Table 2 indicates that the values and the corresponding standard deviations a re re la t ive ly constant.
Fuel Elements
The pressed spheres contain 76 % natural graphite, 14 % graphitized pe t ro l coke and 10 76 binder coke. During production we have learned tha t the properties o f the fue l elements are depending mainly on the qual i ty of the r a w materials. Therefore the following analyses on graphite powder are made
Structure (Metallography and X-ray) Density Elec t r ic r e s i s t anc e BET-surf ac e Grain-size (by sieve analyses and sedimentation) Buld density Tap density Water content Gas content (H2, N2, O2 per h o t extraction) Impurities . The first parameters, s t ruc ture density blaine value o r BET-surface and e l ec t r i c res is tance have a remarkable influence on the properties of the graphite matrix, w i t h respect t o the density, thermal conductivity and corrosion rat e .
. . . - . . . . . . .~ . . . -. . . . . . . . .
61 3
The f r ac tu re l o a d and espec ia l ly t h e number o f drops necessary t o cause surface damage of the f u e l elements a r e influenced by the grain-size o f t he powder.
The binder i s a l s o very extensively control led with respect t o t h e important chemical, physical properties.
Since the fabr ica t ion methods f o r t he pressed f u e l elements have been described on previous occasions, we will only discuss the more i n t e r e s t i n g analyses o f data obtained during and a f t e r f ab r i ca t ion o f more than 20,000 spheres.
Table 3 shows t h e most important data which we think a r e necessary f o r a c r i t i c a l examination w i t h respect t o qua l i t y and reproducibi l i ty . Each p l o t represents one l o t , which i s 450 f u e l elements.
Table 3 a l s o ind ica tes that some o f t he proper t ies a r e r e l a t i v e l y constant, o thers a r e not. A s pointed out above the sca t t e r ing values o f t he f r ac tu re load and t h e number o f drops the spheres withstand without surface damage a r e corresponding t o t he va r i a t ion o f the grain-size of t he graphit e powder.
A t present t he through-put i s about 130 f u e l elements per day (one shift). We are n o w convinced that a through-put of 800 - I000 o r more pressed f u e l elements per day as necessary f o r THTR-Reactors can be achieved without ser ious d i f f i c u l t i e s but f u r t h e r development work i s s t i l l necessary.
A
614
u) aJ - E
Inner Layer Thickness
40 Cpm I mean value minrmunt
Batch No. 1 2 3 4 5 6 7 8 9 x ) 11 12 13 IC 15 1 6 2 I I I I , ,
5.5-
4.5- N -Value 5.0-.
Density 8.6 - 8 3 - d Cg/cm31 8.0 -
14.0- C - Content 13,0
C% I 12.0- \
7 * max 4 l2 ioao- 0 min 99.5- C % l 99.0 -
No*
I
Kernels -Coated Particles \YM
Total Layer 180 1 Thickness Cpm I
mean value minimum
- real mean value - real mean value
nominal Val 2.00 Outer Layer Density -- namml wl k 2.00 Cg/cm3 I 1.95
I I
1.0
Anisotropy Factor
with 95% probability 95% of all coating
thicknesses must be within the limit
616
e t
9 (3
19 C o r m n &te I 7.
H 9 a t loOo"Cl5, [kg/cm'h] :;- -*
0 9
-- II Gmm Compression ," - I Gmrn
r-- ---2- - Strength m---
Bending Strength [kp/cmy
Tensile ~OJ
----- II Gmm - I Gmin
g,+ e ---- II Gmm - IGmln
61 7
DISCUSSION
J. A. Robertson: What confidence i s t h e r e t h a t ' o p t i c a l methods give
BAF values representa t ive of bulk proper t ies and not of t h e sur face (which
may be a f f ec t ed by metallographic p repa ra t ion )?
B. Liebmann: There i s c e r t a i n l y a problem. The method of surface
prepara t ion m u s t be standardized.
and X-ray methods taken on graphi te d i s c s have, however, demonstrated t h e
p o s s i b i l i t y of r e l i a b l e co r re l a t ion between OPTAF and BAF.
Comparative measurements with o p t i c a l
J. L. Scot t : Do you have any da ta on t h e shrinkage rate of f u e l com-
pacts with lgU/cc compared with unfueled s h e l l s which are molded
K. G. Hackstein: No, up t o now we don't have t h e exact f igures . We
w i l l s tart with i r r a d i a t i o n t e s t s i n the middle of 1970.
H. Kr 'ber: Dr. Hackstein should add a word about what heavy metal
d e n s i t i e s are achievable by pressur iz ing tubu la r rods.
K. G. Hackstein: Up t o now we have reached a heavy metal dens i ty of
one gram per cubic centimeter with p a r t i c l e s having a ke rne l diameter of
600 microns. The free uranium i s less than 10 X
J. D. Hart: I have understood t h a t you determined p a r t i c l e breakage
l e v e l s by measuring t h e d i f fused uranium af te r hea t treatment r a t h e r than by d i s i n t e g r a t i o n methods. Do you be l ieve that you could d e t e c t one
broken p a r t i c l e i n l o4 by t h i s method?
K. G. Hackstein: We can, because the determination of uranium i s
made a f t e r e l e c t r o l y t i c d i s in t eg ra t ions of t h e spheres.
R. F. Turner: Were the compacts which showed high f u e l dens i ty made
by the overcoating process?
K. G. Hackstein: We. use overcoated p a r t i c l e s toge ther with another
part of t he same graphi te powder and press t h i s mixture.
R. A. U. Huddle:
t i o n we have concluded
overcoating process i s
I n our economic assessment of f u e l element produc-
t h a t an a r t i c l e made from powder and made by an
something of t he order of 5-10 times as expensive
618
as a similar a r t i c l e made from conventional graphi te . Would you comment
on the part of t he element you j u s t described. We do not use POCO gra-
ph i te .
K. G. Hackstein: We th ink t h a t i s not. r e a l l y a problem i f you have
a production l i n e running. On t h e o ther s ide , you know t h a t we a r e using
r e f ined graphi te powder dust ; t h i s i s much cheaper from graphi t ized pe t -
r o l coke. I d i d n ' t mention POCO graphi te .
619
ECONOMICS OF HTGR FUEL RECYCLE
AND POWER GENERATION
(Session V I )
620
Chairman: H. B. Stewart, Gulf General Atomic
Co-Chairman: R. S. Carlsmith, Oak Rige National Laboratory
Paper 1/136
THORIUM-FUEL-REPROCESSING RESEARCH AND DEVELOPMENT WORK . .a~a*v -<* .-.. 4 s - 31 AT THE KFA-JUELICH
*40 P. L*J%@mzc:
J . Bohnens t ing l H. K i rchne r D . T h i e l e B.G. Brodda M. Laser U . Wenzel 0. Coenegracht w. Li tzow H. Wiemer E. F i s c h e r E. Merz H . Witte G . Kaiser H . J . Riedel E. Zimmer
#3 ABSTRACT
4%
Research and development work a t t h e KFA-Ins t i t u t e f o r Chemical Technology i s d i r e c t e d towards t h e development of s u i t a b l e r e p r o c e s s i n g methods f o r t h e g r a p h i t e f u e l e l e m e n t s of HTG-reactors. T h i s work i s p a r t o f a j o i n t p r o j e c t i n which a l s o s e v e r a l companies of t h e German che- mical i n d u s t r y p a r t i c i p a t e and which i s sponsored by t h e F e d e r a l M i n i s t r y for ) Educa t ion and S c i e n c e .
E a r l y i n t h e p r o j e c t , s e v e r a l p r o c e s s c o n c e p t s were i n v e s t i g a t e d . F i n a l l y two b a s i c a l l y aqueous process- f low- s h e e t s were e s t ab l i shed , on which a l l f u r t h e r e f f o r t s are c o n c e n t r a t e d .
s t e p s : The f i r s t - c h o i c e p r o c e s s c o n s i s t s of t h e f o l l o w i n g
- Burning of t h e f u e l e l emen t s . - D i s s o l u t i o n of t h e r e s i d u a l o x i d e s e i t h e r i n THOREX-
r e a g e n t , or I n t h e c a s e of h i g h l y r e f r a c t o r y ox ide p a r t i c l e s , i n a n a c i d - s a l t m e l t . - I s o l a t i o n of p r o t a c t i n i u m by a s o r p t i o n t e c h n i q u e . - Thorium and uranium r e c o v e r y and p u r i f i c a t i o n by TBP-ext rac t ion .
- Waste t r e a t m e n t and s o l i d i f i c a t i o n . T h i s p r o c e s s w i l l be demons t r a t ed i n t h e middle of
t h e s e v e n t i e s i n t h e "JUPITER" hot- p r o c e s s i n g p i l o t p l a n t . The c a p a c i t y of t h i s p l a n t w i l l be on t h e o r d e r o f 2 kg of heavy metal p e r day. Next t o t h e b u r n i n g , t h e d r y c h l o r i - n a t i o n of t h e ground HTGR-fue ls c o u l d be a n o t h e r advantage- ous method f o r s epa i r a t ing m a t r i x g r a p h i t e from t h e heavy metals. T h e r e f o r e , t h e CHLORINEX-flow-sheet deve loped by KFA, cou ld r e p r e s e n t a n a l t e r n a t i v e t o t h e Burn-Leach/TBP- E x t r a c t i o n - P r o c e s s .
* Work performed under a j o i n t p r o j e c t sponsored by t h e German F e d e r a l M i n i s t r y f o r Educa t ion and S c i e n c e .
622
I n t h e head-end o f t h i s p r o c e s s , t h e ground mater ia l i s fed i n t o a f i x e d be$ and c h l o r i n a t e d w i t h e l e m e n t a r y c h l o r i n e a t a b o u t 1000 C . The heavy metals a re removed o u t o f t h e c h l o r i n a t o r . The r e m a i n i n g g r a p h i t e i s d i s c a r d e d and s t o r e d , o r perhaps burned . The condensed c h l o r i d e s a re d i s s o l v e d and f u r t h e r separated and decon tamina ted by a s o l v e n t e x t r a c t i o n c y c l e . One a l t e r n a t i v e i n v e s t i g a t e d i s t h e c o n v e r s i o n of t h e c h l o r i d e s i n t o n i t r a t e s and t h e n a p p l y i n g a THOREX-flow-sheet; a n o t h e r p o s s i b l e method i s a s o l v e n t e x t r a c t i o n p r o c e d u r e i n t h e c h l o r i d e sys t em w i t h l o n g c h a i n t e r t i a r y amines d i l u t e d w i t h a r o m a t i c hydro- c a r b o n s .
INTRODUCTION
I n t h e F e d e r a l Repub l i c o f Germany, so f a r , t h e AVR- r e a c t o r i s t h e o n l y h i g h - t e m p e r a t u r e gas -coo led r e a c t o r i n o p e r a t i o n . Dur ing t h e s e v e n t i e s , two more H T G R ' s w i t h t o g e t h e r 900 MWel a re e x p e c t e d t o b e i n s t a l l e d . They w i l l be f u e l e d w i t h c o a t e d o x i d e p a r t i c l e s d i spe r sed u n i f o r m l y i n a g r a p h i t e m a t r i x f o r m i n g a 60 mm diameter sphere. Fo r t h e r e p r o c e s s i n g o f t h i s t y p e o f f u e l , r e s e a r c h and deve lop - ment work e s p e c i a l l y i n t h e head-end s t e p i s needed , due t o t h e f a c t t h a t a s i m p l e m e c h a n i c a l s e p a r a t i o n o f t h e m o d e r a t o r g r a p h i t e and f u e l material i s i m p o s s i b l e . I n a d d i t i o n , t h e u s e o f c o a t e d p a r t i c l e s w i t h t h e i r c h e m i c a l l y e x t r e m e l y r e s i s t a n t c o a t i n g s of py roca rbon and p o s s i b l y s i l i c o n c a r b i d e c a u s e s a d d i t i o n a l problems.
I n o r d e r t o g u a r a n t e e a comple t e f u e l c y c l e t o f u t u r e r e a c t o r u s e r s , a p p r o p r i a t e p r o c e d u r e s f o r t h e r e p r o c e s s i n g of s p e n t f u e l e l e m e n t s must be deve loped i n t h e n e a r f u t u r e . T h e r e f o r e , a l r e a d y i n 1966 a j o i n t p r o j e c t between K F A and seven i n d u s t r i a l companies was i n a u g u r a t e d by t h e F e d e r a l M i n i s t r y f o r E d u c a t i o n and S c i e n c e .
623
T h i s p a p e r d e s c r i b e s t h e work done e i t h e r by t h e K F A a l o n e , or i n c l o s e c o o p e r a t i o n between K F A and i n d u s t r i a l companies . A c t i v i t i e s f a l l i n g e x c l u s i v e l y unde r t h e r e s p o n - s i b i l i t y of o u r i n d u s t r i a l p a r t n e r s w i l l n o t be i l l u s t r a t e d here .
a
SHORT SURVEY OF STUDIES D U R I N G THE EARLY PROJECI' PEF,IOD
Dur ing t h e f i r s t t h r e e years o f t h e p r o j e c t , a r e l a t - i v e l y b road spec t rum o f d i f f e r e n t r e p r o c e s s i n g methods has been i n v e s t i g a t e d on a l a b o r a t o r y s c a l e . I n t h a t t ime w e have been i n c l u d i n g t h e t h o r i u m m o l t e n - s a l t r e a c t o r i n o u r r e s e a r c h program. Also i n t h a t t i m e , we f o l l o w e d t h e o v e r a l l a d v o c a t e d view t h a t f o r f u t u r e u s e ma in ly nonaqueous processes s h o u l d be s u p e r i o r . T h e r e f o r e we f i r s t s t a r t e d w i t h f l u o r i n a t i o n e x p e r i m e n t s t r y i n g d i f f e r e n t f l u o r - i n a t i o n a g e n t s . The s t i l l unso lved v a i n problem i s t h e d i f f i c u l t y o f good uranium y i e l d s due t o t h e o b s t i n a t e ho ldback o f t h e t h o r i u m m a t r i x . T h i s problem d o e s n ' t e x i s t i n m o l t e n s a l t f l u o r i n a t i o n .
1
Other a c t i v i t i e s i n c l u d e d p y r o m e t a l l u r g i c a l and pyro- chemical methods of m o l t e n - s a l t s e p a r a t i o n and p u r i f i c a t i o n p r o c e s s e s a p p l y i n g p a r t i t i o n between l i q u i d metal and s a l t phases. Much e f f o r t was p u t a l s o i n s u c h methods l i k e ox id - a t i v e s l u g g i n g and e l e c t r o r e f i n i n g f rom s a l t melts. All methods y i e l d e d u n s a t i s f a c t o r y s e p a r a t i o n and d e c o n t a m i n a t i o n f a c t o r s as wel l a s s e v e r e material and c o r r o s i o n problems.
We conc luded from t h e r e s u l t s and e x p e r i e n c e g a i n e d d u r i n g t h i s p e r i o d t h a t i n t h e f i r s t r e p r o c e s s i n g p e r i o d o n l y a wet c h e m i c a l p r o c e s s such as s o l v e n t - e x t r a c t i o n can s a t i s f a c t o r i l y separate t h e feed a n d / o r breed mater ia l f rom
624
t h e f i s s i o n p r o d u c t s . T h i s c o n c l u s i o n i s n o t s u r p r i s i n g s i n c e i n 25 y e a r s o f e x p e r i e n c e i n r e p r o c e s s i n g , on ly e x t r a c t i o n p r o c e s s e s have been p r a c t i c a l on an i n d u s t r i a l scale.
N e v e r t h e l e s s w e b e l i e v e t h a t w e g o t a r a the r good r e t u r n o u t o f these s t u d i e s s i n c e t h e y g i v e u s a b e t t e r u n d e r s t a n d i n g o f t h e p o t e n t i a l i t i e s o f aqueous p r o c e s s i n g and i t s a s s o c i a t e d problems. A s t h e r e s u l t o f about f o u r y e a r s of work, two p r o c e s s f l o w - s h e e t s were e s t ab l i shed
f i n a l l y , on which a l l f u r t h e r e f f o r t s are c o n c e n t r a t e d .
For t h e p r e s e n t , a n i s o l a t i o n of decontaminated tho r ium can be renounced . F u r t h e r , t h e p r o c e s s s h o u l d be c a p a b l e of t r e a t i n g f u e l e l e m e n t s a f t e r s h o r t c o o l i n g p e r i o d s . T h e r e f o r e , a p r o c e s s s t e p f o r t h e r e c o v e r y and p u r i f i c a t i o n o f t h e r e l a t i v e l y l o n g - l i v e d 233Pa Inas t o be p rov ided . On t h e o t h e r hand, we are wel l aware o.f t h e f a c t t h a t t h e n e c e s s a r y i o d i n e removal may be t h e o t h e r l i m i t i n g f a c t o r i n p r o c e s s i n g s h o r t - c o o l e d f u e l .
I. BURN-LEACH / TBP-SOLVENT EXTRACTION PROCESS
There seems t o e x i s t no doubt t o d a y t h a t f o r a f i rs t r e p r o c e s s i n g p e r i o d of HTGR-fuel e l e m e n t s t h e most e x p e d i e n t f l ow-shee t w i l l be marked by a b u r n - l e a c h s t e p i n t h e head- end and a TBP-solvent e x t r a c t i o n p r o c e d u r e i n t h e second t o a c h i e v e a good r e c o v e r y and p u r i f i c a t i o n o f t h e v a l u a b l e f i s s i o n a b l e material. Our endeavours are c o n c e n t r a t e d there- f o r e on a f low-shee t c o n s i s t i n g of t h e f o l l o w i n g p r o c e s s - s t eps :
- Burning o f t h e g r a p h i t e - c o n t a i n i n g f u e l e l emen t s - D i s s o l u t i o n o f t h e o x i d e r e s l d u e s
62 5
- I s o l a t i o n o f p r o t a c t i n i u m - Thorium and uranium r e c o v e r y and p u r i f i c a t i o n by a
TBP-solvent e x t r a c t i o n p rocedure - Waste t r e a t m e n t and s o l i d i f i c a t i o n
However, no f i n a l d e c i s i o n can be pronounced on t h e de t a i l ed l ay -ou t of t h e i n d i v i d u a l p r o c e s s - s t e p s a t t h e moment, s i n c e i n s e v e r a l cases a l t e r n a t i v e s are s t i l l under i n v e s t i g a t i o n . T h i s i s t r u e f o r t h e b u r n i n g , d i s s o l v i n g and p a r t l y f o r t h e e x t r a c t i o n . The o v e r a l l a l t e r n a t i v e s are c h a r a c t e r i z e d by t h e well-known THOREX-flow-sheets and t h e KFA/TBP 23/25-f low-shee t .
We i n t e n d t o f i n i s h t h e f low-shee t d e s i g n by t h e end o f n e x t year and t o p u t a s e m i - t e c h n i c a l p i l o t p l a n t i n t o o p e r a t i o n i n abou t 4 y e a r s f rom now. Design work on t h i s p i l o t p l a n t ( " J U P I T E R " ) has s t a r t ed just r e c e n t l y . The s i z e of t h e p i l o t p l a n t w i l l be r a the r small. It i s l i m i t e d by t h e o u t p u t o f t h e AVR-reactor and t h e h o t c e l l f a c i l i t i e s . The d a i l y t h roughpu t b e i n g on t h e o r d e r of abou t 2 kg of heavy metal.
626
Time Schedule for HTGR - Reprocessing R 8 D -Work at KFA - Juelich
Year 1970 71 72 73 I
Dp.roImn AV R Oprolimlco 7COFElO-7 HYld i-om I078 1 Fuel Elements THTR-3OOMW - from THTR-WOMW Cmslruci*n Tma-5y k Opnolion 1978 co W F E l d 1 U h W i d bm 1978
KSH -Reoctor 7
DZO-Th- Breeder 3 I I 1 I I 1 1 I I I I
I I I I I I I 1
I
Ion . cold Run$. I
not nuns Reprocessing Flow - Sheet Il I Lokaidry ExF'm*ni* ! -- CHLORtNEX- Process
F i g . 1: T i m e Schedule f o r Reprocess ing R & D-Work a t t h e KFA-Juelich
A c o n t i n o u s d i s c h a r g e o f spent; f u e l spheres from t h e AVR-reactor i s e x p e c t e d f o r t h e y e a r 1972. I n t h e meantime, t h e s p e n t f u e l e l e m e n t s must be s t o r e d i n a n i n t e r i m s t o r a g e f a c i l i t y t o be e r e c t e d a t t h e r e a c t o r s i t e . Larger q u a n t i - t i e s of s p e n t f u e l from t h e THTR-300 MW-reactor are n o t e x p e c t e d b e f o r e 1977/78. A f u r t h e r i n c r e a s e shou ld a r i s e a t t h e b e g i n n i n g of 1980.
Reprocess ing o f s p e n t f u e l e l e m e n t s f rom HTG-reactors w i l l t h u s be a d e q u a t e l y g u a r a n t e e d a t t h a t t ime, i f a head- end p r o c e d u r e i s a v a i l a b l e , because t h e s o l v e n t e x t r a c t i o n
. .
627
s e p a r a t i o n and p u r i f i c a t i o n may be ach ieved i f n e c e s s a r y i n a n e x i s t i n g PUREX-plant. We are aware t h a t t h i s l ess economic
63 r o u t e r e p r e s e n t s on ly a t r a n s i t i o n a l stage f o r t h e t i m e b e i n g , when o n l y a few tho r ium r e a c t o r s are i n o p e r a t i o n .
We t h e r e f o r e s ta r ted c o n c e p t u a l d e s i g n s t u d i e s on a 2 0 kg/day-combustion p i l o t p l a n t j u s t r e c e n t l y . It i s aimed towards a d e c i s i o n which f u r n a c e t y p e , e . g. f l u i d i z e d bed oven, may be s u p e r i o r f o r t h e bu rn ing . Economic s t u d i e s w i l l r e v e a l t h e b e s t of one of t h e f o l l o w i n g combi- n a t i o n s :
1. F i n a l s t o r a g e of t h e s p e n t f u e l e l e m e n t s a t t h e
2 . I n t e r i m s t o r a g e of t h e s p e n t f u e l e l e m e n t s a t t h e
shaft o r
power p l a n t s i t e .
power p l a n t s i t e and f i n a l s t o r a g e i n an abandoned s a l t mine.
f u e l e l e m e n t s i n a head-end b u r n i n g i n s t a l l a t i o n a t t h e power p l a n t s i t e and f i n a l s t o r a g e of t h e o x i d e r e s i d u e s a t t h e r e a c t o r s i t e o r a n abandoned
3 . I n t e r i m s t o r a g e as w e l l as b u r n i n g of t h e s p e n t
s a l t mine, r e s p e c t i v e l y . 4 . I n t e r i m s t o r a g e as w e l l as b u r n i n g of t h e s p e n t f u e l
e l e m e n t s i n a head-end b u r n i n g i n s t a l l a t i o n a t t h e
power p l a n t s i t e , b u t p r o c e s s i n g of t h e ox ide r e s i d u - es i n a n e x i s t i n g PUREX-reprocessing p l a n t (WAK o r EUROCHEMIC) .
5. E s t a b l i s h m e n t of a b u r n i n g head-end f a c i l i t y i n a n e x i s t i n g PUREX-reprocessing p l a n t .
Combust i o n
For combust ion o f t h e g raph i t e f u e l t h e KFA i s develop- ing a f l u i d i z e d bed combust ion f u r n a c e .
The t h r e e p r i n c i p a l problems are:
1. Crush ing o f f u e l e l e m e n t s 2. H e a t - c o n t r o l o f t h e f u r n a c e 3. Off-gas c l e a n up
The c r u s h i n g of t h e f u e l s p h e r e s i s c a r r i e d o u t i n a hammer m i l l , which has been f u r n i s h e d w i t h a 1 , 5 mm s l o t s i e v e .
The p r o d u c t of t h e hammer m i l l i s f ed i n t o t h e b u r n e r v i a a screw conveye r . The feed r a t e i s c o n t r o l l e d by t h e f l u i d bed d i f f e r e n t i a l p r e s s u r e . The bed t e m p e r a t u r e i s c o n t r o l l e d by o u t e r h e a t i n g and c o o l i n g c o i l s a t 7 5 O o C . Should t e m p e r a t u r e e x c u r s i o n s o c c u r , t h e feed-gas oxygen content, n o r m a l l y k e p t a t 75 %, i s decreased a u t o m a t i c a l l y . The off-gas i s passed through s i n t e r e d metal f i l t e r s , equipped w i t h a n a u t o m a t i c blow-back d e v i c e . To a v o i d l o c a l thermal h o t s p o t s j u s t above t h e bot tom f l o w p l a t e i n b u r n i n g of g r a p h i t e w i t h o u t t h e a d d i t i o n of a l u m i n a , which might c a u s e s i n t e r i n g o f t h e metal o x i d e s , t h e b u r n i n g gas must be d i l u t e d w i t h C 0 2 . T h i s i s a c h i e v e d by r e f l u x i n g par t of t h e o f f - g a s .
An a u t o m a t i c c o n t r o l l e d model of a f l u i d i z e d bed
f u r n a c e has been c o l d t e s t e d e x t e n s i v e l y and i s b e i n g i n s t a l l e d i n t h e h o t c e l l . The c o n s t r u c t i o n o f a 10 " dia-
meter f u r n a c e ( 2 kg heavy metal pe r day c a p a c i t y ) i s i n p r o g r e s s .
Hot c e l l e x p e r i m e n t s on t h e corntiustion o f AVR-fuel s p h e r e s i n a shaf t f u r n a c e model ( 2 s p h e r e s p e r h o u r c a p a c i t y ) r e v e a l e d t h a t f i b e r g lass f i l t e r s r e t a i n t h e r a d i o a c t i v e d u s t s and a e r o s o l s w i t h d e c o n t a m i n a t i o n f a c t o r s o f a b o u t l o 3 - 10 . F o r some i s o t o p e s l i k e ces ium and 4 r u t h e n i u m , t h e d e c o n t a m i n a t i o n f a c t o r s are r e m a r k a b l y lower 2
@
629
Also i o d i n e , i f p r e s e n t , passes t h e s e f i l t e r s anc! can be r e t a i n e d t o a grea t e x t e n t i n c h a r c o a l t r a p s . Because of t h e h ighe r combust ion t e m p e r a t u r e i n t h e s h a f t f u r n a c e ( a b o u t 9 5 O o C ) , t h e o f f - g a s c o n t a m i n a t i o n i s e x p e c t e d t o be somewhat lower i n t h e f l u i d i z e d bed d e v i c e . A s a r e s u l t o f t h e f i rs t h o t c e l l r u n s , a r e v i s e d e x p e r i m e n t a l program on t h e problems of o f f - g a s c l e a n up h a s been s ta r ted .
The re lease o f f i s s i o n gases d u r i n g t h e combust ion of o x i d e f u e l amounts t o 1 - 5 % of t h e t o t a l amount p r e s e n t , whereas carb ide f u e l r e t a i n s o n l y a few p e r c e n t of these f i s s i o n gases.
D i s s o l u t i o n
The combust ion p roduces uranium-thorium o x i d e m i x t u r e s o r mixed uranium-thorium o x i d e s depending whether c a r b i d e o r o x i d e f u e l p a r t i c l e s were employed. For t h e i r d i s s o l u t i o n b o i l i n g THOREX-reagent, a m i x t u r e o f 13 M HNOJ , 0 , l €4
A1(N03)3 and 0,05 M H F , i s w e l l s u i t e d . I n case of c a r b i d e f u e l , t h e d i s s o l u t i o n time amounts t o abou t 1 t o 4 h o u r s depending on t h e burn-up and t h e tho r ium and uranium concent ra t ion asp i red i n t h e f i n a l s o l u t i o n . F u e l w i t h a v e r y h i g h burn-up may l e a v e behind a n u n d i s s o l v e d r e s i d u e o f a y e t u n s p e c i f i e d composi t ion . I f s i l i c o n carb ide c o a t e d f u e l p a r t i c l e s have t o be r e p r o c e s s e d , a small f r a c t i o n o f t h e s i l i c o n (0 ,5 t o abou t 5 $ ) i s found i n s o l u t i o n afterwards. However, it seems t o cause no s e r i o u s problems i n t h e e x t r a c t i o n s t e p . Some annoyance may ar ise from uncomplete burned material d u r i n g t h e f i l t e r i n g and e x t r a c t i o n s t e p s .
Highly r e f r a c t o r y mixed o x i d e p a r t i c l e s r e q u i r e a much l o n g e r d i s s o l u t i o n t ime, ranging from 6 t o more t h a n 50 hour s . The r e a c t i o n seems t o be h i g h l y dependent on t h e compos i t ion , burn-up, s u r f a c e area and d e n s i t y of t h e
630
p a r t i c l e s . I n order t o e x p l o r e t h e d i s s o l u t i o n mechanism t h o r o u g h k i n e t i c i n v e s t i g a t i o n s are i n p r o g r e s s .
Q
A ra ther r a p i d and comple t e d i s s o l u t i o n o f any k i n d of h i g h l y r e f r a c t o r y o x i d e material may be a c h i e v e d a p p l y i n g a n a c i d - s a l t m e l t t r e a t m e n t , c h a r a c t e r i z e d by t h e f o l l o w i n g e q u a t i o n s : Tho2 + 2 K S 0
U 0 2 + 2 K S 0
+ 2 K 2 S 0 4
+ 2 K 2 S 0 4 - U O , ( S O q ) , + 4 K2S04 + SO2
Th (SO4)2 + 4 K2S04 2 2 7
2 2 7 FP(ox ide1 + n K2S207 + m K2S04 -€pP(su lpha te)n + (n+m)K2S04
S y s t e m a t i c i n v e s t i g a t i o n s p roved t h a t a p p r o p r i a t e m i x t u r e s of K 2 S 2 0 7 / K 2 S 0 4 r e q u i r e a minimum amount o f m e l t material f o r a comple t e d i s s o l u t i o n w i t h i n 30 t o 60 m i n u t e s a t a b o u t 7 5 O o C '. Part of t h e K2S04 may be r e c o v e r e d i n a l a t e r p r o c e s s s t e p and r e u s e d , t h u s r e d u c i n g t h e amount of s o l i d waste. After p o u r i n g t h e l i q u i d s a l t melt i n t h e r e q u i s i t e amount o f water, uran ium d i s s o l v e s as u r a n y l s u l p h a t e , whereas t h o r i u m i s q u a n t ' i t a t i v e l y p r e c i p i t a t e d as t h e s p a r i n g l y s o l u b l e d o u b l e s a l t 3 ,5 K2S04 T h ( S 0 4 ) 2 t o g e t h e r w i t h some f i s s i o n p r o d u c t s u l p h a t e s l i k e Ba, Sr. T h i s p r e c i p i t a t e i s washed f r e e from uranium and t h e r e b y t r a n s f o r m e d i n t o t h e compound 2 K2S04 T h ( S 0 4 ) 2 2 H20, which i s t h e n s e p a r a t e d , d r i e d and d i r e c t l y s t o r e d . T h i s method e n a b l e s a s i m p l e t h o r i u m p r e s e p a r a t i o n and i s p a r t o f t h e KFA/TBP 23 /25-p rocess f l o w - s h e e t .
P ro tac t in ium-Recovery
S h o r t c o o l i n g t imes f o r t h o r i u m - c o n t a i n i n g f u e l e l e m e n t s r e q u i r e a s p e c i a l p r o c e d u r e for t h e r e c o v e r y o f t h e 2 3 3 ~ - p r e c u r s o r , 233Pa. The a p p l i c a t i o n of t h e well-known THOREX f l o w - s h e e t p e r m i t s a comple t e r e c o v e r y of t h o r i u m and uranium, bu t no i s o l a t i o n of t h e 233Pa. The sometimes proposed M n 0 2 - p r e c i p i t a t i o n g i v e s u n s a t i s f a c t o r y r e s u l t s .
631
A t h o r o u g h a n a l y s i s of a l l p u b l i s h e d p r o t a c t i n i u m s e p a r a t i o n and p u r i f i c a t i o n p r o c e d u r e s r e v e a l e d t h a t t h e s o r p t i o n on Vycor glass columns shows t h e b e s t promise for a t e c h n i c a l r e a l i s a t i o n .
0
After p r e l i m i n a r y i n v e s t i g a t i o n s w i t h t r a c e r amounts of p r o t a c t i n i u m , a s e r i e s of h o t c e l l e x p e r i m e n t s w i t h h i g h l y i r rad ia ted t h o r i u m f u e l was per formed i n o r d e r t o e s t a b l i s h and e x t e n d t h e t r a c e r e x p e r i m e n t s . It c o u l d be shown a l r e a d y i n t h e f i r s t r u n s t h a t t h i s method o f f e r s a r a the r good p r o t a c t i n i u m r e c o v e r y from THOREX-feed s o l u t i o n s g i v i n g d e c o n t a m i n a t i o n f a c t o r s f o r t h o r i u m , uran ium, ces ium and
3 2 2 Zr /Nb o f a t least 10 , 8 x 10 , 4 x 10 and 6 , r e s p e c t i v e l y . These r e s u l t s are i n agreement w i t h t h o s e of GOODE and MOORE . 4
Exper imen t s have shown a l s o t h a t t h e s o r p t i v e Vycor g l a s s s e p a r a t i o n p r o c e d u r e can a l s o be a p p l i e d i n t h e s u l p h a t e 5 , and p o s s i b l y i n t h e c h l o r i d e sys t em 6 , 7 *
Uranium S e p a r a t i o n and P u r i f i c a t i o n
U p t i l l now, o u r h o t c e l l e x p e r i m e n t s were d e a l i n g w i t h t h e v e r i f i c a t i o n o f t h e well-known THOREX- and INTERIM-23- f l o w - s h e e t . I n g e n e r a l , i t may be s t a t ed t h a t w e o b t a i n e d ra ther s a t i s f a c t o r y r e s u l t s 8 . The measured s e p a r a t i o n and d e c o n t a m i n a t i o n f a c t o r s are i n good agreement w i t h a l r e a d y p u b l i s h e d r e s u l t s based on work done ma in ly i n t h e U S A . There i s no doubt t h a t e i t h e r one of t h e p roposed f l o w - s h e e t s can meet t h e r e q u i r e m e n t s f o r a r e p r o c e s s i n g o f thor ium- c o n t a i n i n g HTGR-fuel. On t h e o t h e r hand , i t i s o u r o p i n i o n t h a t i t would be wor thwhi l e t o d e v e l o p improved f l o w - s h e e t s . Such a p o s s i b i l i t y could be t h e KFA/TBP 23/25-Process .
The c h e m i c a l f l o w - s h e e t s o f t h i s p r o c e s s w i t h t h e
@ p e r t i n e n t mass-streams are shown i n f i g u r e s 2 and 3 .
t MAW 84LLS:aOg HEAVY METAL
KOH: 5 M
+t
URANIUM L E ACHING INSTALL A T ~ O ~
URANIUM 0.5 - 1
THORIUM 0.5 - ( VOLUME 6 1 - 1
VOLUME 0.6 - 0.1 I
DIGESTION POT
THORATE
, I d ” - ,,ug I It d I SUCTION FILTER HNOi ADDITION
HNO3 1 3 M
VOLUME 1.61 I i 3
WASH PROCESS SOLUTION SOLUTION
SOLVENT-EXTRACTION i
Fig . 2: Chemical Flow-Sheet of t h e KFA/TBP 23/ 25-Process , Head-End
AQUEOUS RAFFINATE URANIUM : < 5.6 [
SULFATE : 0.38 VOLUME : 117.65
AQUEOUS STRIP
VOLUME : 58,82 - ORGANIC PRODUCT
URANIUM : 4.75 g /I “03 . 0.29 M
T
1 4 1 3 12 11 10 9 8 7 6 5 4 3 2 1 I
SOLVENT RECOVERY
URANIUM : 9.5g/l “03 : 0.59 M
c=53 EVAPORATOR
1
F i g . 3 : Chemical Flow-Sheet o f t h e KFA/TBP 2 3 / 25-Process , S o l v e n t E x t r a c t i o n
Q
633
The s p e n t f u e l e l e m e n t s a re f i rs t c rushed and t h e n burned. Afterwards t h e r e s u l t i n g ox ide r e s i d u e s are d i s s o l v - ed i n a K2S207/K2S04-mixture. The washed and d r i e d po ta s s ium s u l p h a t o t h o r a t e p r e c i p i t a t e r e t a i n s less t h a n 0 , l % of t h e t o t a l uranium i n p u t and may be d i r e c t l y s t o r e d . The f i l t r a t e , c o n t a i n i n g t h e uranium i s a d j u s t e d t o s o l v e n t e x t r a c t i o n c o n d i t i o n s by a d d i n g n i t r i c a c i d . Details of t h e e x t r a c t i o n p r o c e d u r e may be deduced from f i g u r e 3 and t h e l i t e r a t u r e . The h i g h ac id c o n c e n t r a t i o n of 5 molar HNO i n t h e s c r u b s o l u t i o n promotes a good ru thenium decon tamina t ion . T h i s i s t r u e a l s o f o r Z r / N b and Ce.
0
9
3
The proposed f low-shee t g u a r a n t e e s a uranium r e c o v e r y of 9 9 , 9 % a p p l y i n g 6 t h e o r e t i c a l e x t r a c t i o n - ana 3 t h e o r e t i c a l b a c k e x t r a c t i o n steps. S i n c e t h e a p p l i e d mechan ica l s t i r r e d mixer s e t t l e r s o f t h e CEN-type e x h i b i t e d a stage e f f i c i e n c y of 60 % o n l y , t h e p r a c t i c a l s t a g e numbers needed were 10 and 5 , r e s p e c t i v e l y . Even b e t t e r r e s u l t s may be o b t a i n e d u s i n g a i r p u l s e d m i x e r s e t t l e r s . I n c o l d l a b o r a t o r y t e s t s we cou ld p rove t h e i r s u p e r i o r i t y compared t o t h e m e c h a n i c a l l y s t i r r e d ones .
Cold t e s t s o f t h e f low-shee t are complete and h o t c e l l expe r imen t s are i n p r e p a r a t i o n .
An u n f o r t u n a t e drawback o f t h i s p r o c e s s i s t h e s u l p h a t e c o n t a i n i n g aqueous waste. However, w e hope t o be able t o surmount t h i s d i f f i c u l t y i n o u r waste t r e a t m e n t e f f o r t s a p p l y i n g phospha te glasses f o r t h e i r s o l i d i f i c a t i o n .
634
11. CHLORINEX-PROCESS Q Next t o t h e b u r n i n g , t h e d r y c h l o r i n a t i o n of t h e ground
grzphite-based f u e l e l e m e n t s of HTG-reactors may be a n o t h e r advantageous method f o r r e p r o c e s s i n g t h i s t y p e of f u e l e lement . We a re t h e r e f o r e d e v e l o p i n g a n a l t e r n a t i v e flow- sheet t o t h e burn/leach-TBP s o l v e n t e x t r a c t i o n p r o c e s s c a l l i n g i t CHLORINEX-process.
Because a l l t h e carbon r ema ins i n t h e e l emen ta ry s ta te by t h i s method, t h e o f f - g a s treatment and e s p e c i a l l y t h e ra re g a s r e t a i n m e n t , if n e c e s s a r y , i s s i m p l i f i e d c o n s i d e r a b l y . It may be done by c o l d - t r a p p i n g a f t e r removing t h e e x c e s s of c h l o r i n e by a b s o r p t i o n .
No s e r i o u s problems a re encoun te red i n case of p r o c e s s - i n g s i l i c o n c a r b i d e c o n t a i n i n g f u e l p a r t i c l e s , s i n c e e a s i l y v o l a t i l e SiC14 i s formed and t h u s can b e s e p a r a t e d from t h e heavy metals.
The c r u c i a l problem of t h i s p r o c e s s i s t h e c o r r o s i o n a t e l e v a t e d t e m p e r a t u r e s w i t h c h l o r i n e i n t h e p r e s e n c e o f carbon o r ca rbon monoxide and w i t h c h l o r i d e s . I f w e succeed i n c o n t r o l l i n g t h e c o r r o s i o n problems, t h e c h l o r i n a t i o n r e p r e s e n t s c e r t a i n l y v e r y p romis ing f e a t u r e s f o r f u t u r e a p p l i c a t i o n o f r e p r o c e s s i n g g r a p h i t e c o n t a i n i n g f u e l e l e m e n t s . 10
The p r i n c i p l e s of t h e proposed f low-shee t are shown i n f i g u r e 4 .
635
I
Chlorinex - Process
I 1 1
1 Reoctor
1
1 Storoge
Crushing ond Grinding
1 4
Grophite- Chlorinotion Woste 1
Dissolution I _----- of the Chlorides I 1
Conversion to the Nitrates
I------- Adlust ment
Protactinium
Solvent - d Woste Extraction
b I -
Refobricotion m Fig. 4 : CHLORINEX-Process;
Schematic Process-Flow-Sheet
636
After a n a d e q u a t e c o o l i n g p e r i o d , t h e graphi te-based f u e l e l e m e n t s a re c r u s h e d and t h e n ground i n a gas t i g h t combined m i l l i n g d e v i c e t o a p a r t i c l e s i z e between 50 and 3OO,um w i t h o n l y a small f r a c t i o n o f f i n e s below 50,um. Thus a l l c o a t e d p a r t i c l e s ( w i t h a diameter from 500 t o 800 p m ) are broken up.
The mater ia l i s t h e n f e d i n t o it f l u i d i z e d o r a f i x e d bed and c h l o r i n a t e d w i t h e l e m e n t a r y c h l o r i n e a t abou t 1000°C. The c a r b o n , which i s p resen t ; i n l a r g e q u a n t i t i e s , r e d u c e s t h e o x i d e s . A t t e m p e r a t u r e s a round 1000°C r e a c t i o n s l i k e t h e f o l l o w i n g o c c u r a t a h i g h r a t e .
+ 2 co 4 k ) + 2 Cl;! 4 T h C l Th02 ( s ) + ‘ (g raph i t e )
A HIOOo°C = P- + 24 k c a l .
A t t h i s t e m p e r a t u r e t h e heavy metals and m o s t f i s s i o n p r o d u c t s are v o l a t i l i z e d . The r e m a i n i n g g r a p h i t e may b e
discarded and s t o r e d as aedium l e v e l waste o r b u r n t i n a s p e c i a l u n i t . No s e r i o u s o f f - g a s problem s h o u l d a r i s e i n b u r n i n g t h i s g r a p h i t e , because a l l t h e v o l a t i l e f i s s i o n p r o d u c t s are a l ready released d u r i n g t h e c h l o r i n a t i o n s t e p . The c h l o r i d e s are condensed i n a condense r u n i t . The tho r ium- uranium c h l o r i d e c o n d e n s a t e i s d i s s o l v e d i n 4 M h y d r o c h l o r i c a c i d . T h i s s o l u t i o n i s passed t h r o u g h a s i l i c a g e l or vycor glass column t o a d s o r b and remove t h e p r o t a c t i n i u m .
The p r o t a c t i n i u m - f r e e s o l u t i o n :Is f u r t h e r s e p a r a t e d and decon tamina ted by a s o l v e n t e x t r a c t i o n c y c l e . One a l t e r n a t i v e i n v e s t i g a t e d i s t h e c o n v e r s i o n of t h e c h l o r i d e s i n t o n i t r a t e s and t h e n a p p l y i n g t h e THOREX-f low-shee t ; a n o t h e r p o s s i b l e method i s a s o l v e n t e x t r a c t i o n p r o c e d u r e i n t h e c h l o r i d e s y s t e m w i t h a s o l u t i o n o f l o n g c h a i n a l i p h a t i c amines i n a r o m a t i c hydroca rbons . The p u r i f i e d u r a n y l c h l o r i d e or n i t r a t e s o l u t i o n i.s used for t h e
637
p r o d u c t i o n of p a r t i c l e s w i t h t h e s o l - g e l t e c h n i q u e .
A thoriurn-uranium s e p a r a t i o n i s t h e o r e t i c a l l y p o s s i b l e by f r a c t i o n a l c o n d e n s a t i o n f o l l o w e d by a s u b l i m a t i o n procedure". The uranium c o n t e n t of t h e condensa ted tho r ium c h l o r i d e s h o u l d be lower t h a n 80 ppm c o r r e s p o n d i n g t o 0 . 2 % uranium loss. Despite e x t e n s i v e s t u d i e s we d i d n o t overcome t h e t e c h n i c a l d i f f i c u l t i e s o f f r a c t i o n a t i n g t h e c o n d e n s a t e s .
Crush ing and G r i n d i n q
The g r a p h i t e f u e l spheres ( o r any o t h e r g r a p h i t e f u e l e lement t y p e ) c o n t a i n i n g c o a t e d f u e l p a r t i c l e s a re f i r s t c rushed i n a hammer m i l l . I n a t y p i c a l exper iment about 4 0 % o f t h i s p r o d u c t pas sed a 0,3 mm s i e v e . The o v e r s i z e p a r t i c l e s are t h e n ground i n a second s t e p i n a n impact d i s c m i l l , t h u s a s s u r i n g t ha t e v e r y p a r t i c l e i s broken up. A c i r c u l a t i n g a i r - f l o w d e v i c e p r o v i d e s t h e s t eady removal o f t h e f i n e - g r a i n . T h i s a i r f low can b e a d j u s t e d and c o n t r o l s t h e amount o f f i n e s ( < s o l u m ) below 25 %. T h i s i s n e c e s s a r y , bedause o t h e r w i s e t h e ground material shows bad
f l u i d i s a t i o n cha rac t e r i s t i c s .
- C h l o r i n a t i o n and Condensa t ion
The r e s u l t i n g ground mater ia l i s t h e n c h l o r i n a t e d i n an a p p a r a t u s schematical ly shown i n f i g u r e 5.
638
0 Spherical Fuel
-Chlorine Chlorine +‘lush Gas L -.
F i g . 5: Mills and C h l o r i n a t o r R e a c t o r f o r CHLORINEX-Process
The c h l o r i n a t i o n o f t h e heavy metal o x i d e s i n t h e p r e s e n c e o f g r a p h i t e i s an endo the rmic r e a c t i o n . A t 1000°C t h e r e a c t i o n p r o c e e d s v e r y q u i c k l y , y i e l d i n g uranium r e c o v e r i e s o f more t h a n 99.8 % w i t h i n 1 h o u r .
Though t h e r e a c t i o n r a t e s below 1000°C are s t i l l s u f f i c i e n t l y h i g h , t h i s t e m p e r a t u r e seems t o be t h e optimum, due t o t h e f o l l o w i n g f a c t :
The l o w e s t p o s s i b l e t e m p e r a t u r e o f t h e r e a c t o r i s
639
de te rmined by t h e behav iour of t h e f i s s i o n p r o d u c t s . A t 8OO0C, f o r i n s t a n c e , t h e vapour p r e s s u r e o f some f i s s i o n p r o d u c t c h l o r i d e s (Cs, B a , S r , R E ) i s v e r y low. Though t h e main p a r t o f t ho r ium and uranium o x i d e i s v o l a t i l i z e d a f t e r a s h o r t t i m e , some uranium i s r e t a i n e d as c h l o r i d e by t h e f i s s i o n p r o d u c t s . Q u a n t i t a t i v e v o l a t i l i z a t i o n o f t h e uranium was o n l y p o s s i b l e , if most of t h e f i s s i o n p r o d u c t c h l o r i d e s were vapour i zed .
0
The c h l o r i n a t i o n r e a c t o r c o n s i s t s i n p r i n c i p a l o f an i n n e r porous g r a p h i t e c y l i n d e r , d i r e c t l y heated by c u r r e n t p a s s a g e , and a n o u t e r c y l i n d r i c a l and gas t i g h t ce ramic j a c k e t . The mater ia l i s c o n t i n o u s l y f ed i n t o t h e f i x e d bed r e a c t o r and f l o w s s l o w l y , as t h e r e a c t i o n p r o c e e d s , from t o p t o t h e bottom of t h e g r a p h i t e c y l i n d e r . The gaseous c h l o r i d e s o f t ho r ium, uranium, p r o t a c t i n i u m and s e v e r a l f i s s i o n p r o d u c t s p e n e t r a t e t h e g r a p h i t e walls i n t o t h e o u t e r ceramic t u b e and t h e n l e a v e i t t h r o u g h a c o n n e c t i n g p i p e sidewards.
The f i x e d bed r e a c t o r proved t o be s u p e r i o r ove r t h e f o r m e r l y f a v o r e d f l u i d i z e d bed c o n c e p t i o n s i n c e i t works c o n t i n o u s l y and t h e dange r of i n t e r f e r e n c e i s much smaller even i f t h e f i n e - g r a i n f r a c t i o n may i n c r e a s e c o n s i d e r a b l y .
The c o n d e n s a t i o n o f a l l v o l a t i l i z e d c h l o r i d e s i s ach ieved i n a c o n d e n s a t i o n u n i t , a p p l y i n g gas i n j e c t i o n t o g a i n a snow-type gas phase c o n d e n s a t i o n . After l o n g and l a b o r i o u s t r i a l s , t h i s method a v o i d s c a k i n g of t h e condensa te on t h e walls s e c u r i n g a d e p o s i t o f f i n e and f r ee f l o w i n g powder.
640
Off-gas Trea tment
The o f f - g a s l e a v i n g t h e condense r c o n t a i n s besides
e x c e s s i v e c h l o r i n e and c a r b o n monoxide, t h e r a r e gases, s i l i c o n t e t r a c h l o r i d e , t r i t i u m c h l o r i d e and p o s s i b l y small amounts of i o d i n e and t e l l u r i u m . T h i s o f f - g a s i s sc rubbed w i t h a n o r g a n i c s o l v e n t , for i n s t a n c e h e x a c h l o r o b u t a d i e n e . S iC14 and a small pa r t of t h e c h l o r i n e can be abso rbed i n a r a the r small a b s o r p t i o n column, t h e main p a r t of t h e c h l o r i n e however, i n a l a r g e r a d s o r p t i o n t o w e r . The c h l o r i n e i s t h e n s t r i p p e d f rom t h e s o l v e n t and f ed back i n t o t h e p r o c e s s . The S iC l l l may be separated f rom t h e s o l v e n t by d i s t i l l a t i o n u n d e r r educed p r e s s u r e .
Excess c h l o r i n e may be e l i m i n a t e d by s c r u b b i n g i n a packed column f i l l e d w i t h soda l i m e .
WASTE EFFLUENT TREATMENT AND SOLIDIFICATION
I n c l u d e d i n o u r r e p r o c e s s i n g program i s a h i g h a c t i v i t y waste p r o c e s s i n g and i n t e r i m s t o r a g e f a c i l i t y . It w i l l be o p e r a t e d i n c o n n e c t i o n w i t h a f u e l e lement i n t e r i m s t o r a g e p l a n t f o r t h e s p h e r i c AVR-fuel e l e m e n t s , t h e c o n s t r u c t i o n t o be comple ted by t h e end o f 1973.
The aqueous waste e f f l u e n t s o f t h e "JUPITER"-plant w i l l be t rea ted and s o l i d i f i e d f o r f i n a l s t o r a g e i n t h e f a c i l i t y w i t h a d a i l y t h r o u g h p u t comparable w i t h t h e c a p a c i t y of t h e r e p r o c e s s i n g p i l o t p l a n t . The proce : j s f l ow-shee t c o n s i d e r e d i s shown s c h e m a t i c a l l y i n f i g u r e 6 .
641
r - - - - - gil& 'j-- *-. *' @
.................. J 4
...............
Dm ............................ c
25 Scrub&
I I A ; W o s t e Solidification - Flow Sheet
F i g . 6: Schematic Flow-Sheet f o r Waste E f f l u e n t Trea tment and S o l i d i f i c a t i o n
The h i g h l y r a d i o a c t i v e waste streams as w e l l as f l u s h i n g streams w i t h l o w - s a l t c o n t e n t are f i r s t c o n c e n t r a t - ed i n a n e v a p o r a t o r equipped w i t h a r e c t i f y i n g column. The
low a c t i v i t y d i s t i l l a t e ( a b o u t 0 , l M H N 0 3 ) may be r e u s e d i n t h e r e p r o c e s s i n g p l a n t f o r r i n s i n g , d i l u t i n g , e t c . o r re t reated and dumped. E v a p o r a t o r , condense r and o t h e r p a r t s o f t h e p l a n t are f a b r i c a t e d from t i t a n i u m .
The c o n c e n t r a t e d s o l u t i o n i s t h e n d e n i t r a t e d a p p l y i n g formaldehyde , t h u s minimiz ing a ru then ium v o l a t i l i z a t i o n .
642
S i m u l t a n e o u s l y a f u r t h e r c o n c e n t r a t i o n of t h e s o l u t i o n i s a c h i e v e d . F i n a l l y , t h e r e s u l t i n g c o n c e n t r a t e i s p a s s i n g a p r o d u c t c o o l e r and c o l l e c t e d i n a e t o r a g e t a n k . The l i b e r a t e d n i t r o u s g a s e s are r e c o n v e r t e d i n t o n i t r i c a c i d , which i s r e u s e d a f t e r c o n c e n t r a t i o n .
@
I n t h e n e x t s t e p , t h e c o n c e n t r a t e d s o l u t i o n i s f e d on t o a r o l l e r - d r y e r . The r e s u l t i n g d r y f l a k y p r o d u c t i s mixed w i t h g l a s s - f o r m i n g a d m i x t u r e s and f u s e d i n i n d u c t i v e heated g r a p h i t e c r u c i b l e s and t h e n poured i n s t e e l p o t s . Yost l i k e l y , b o r o s i l i c a t e or p h o s p h a t e g l a s s e s w i l l b e employed.
By p a s s i n g t h e p r o c e s s g a s - s t r e a m s from t h e d i f f e r e n t p r o c e s s s t e p s t h r o u g h t h e d e n i t r a t o r , t h e gas w i l l be purged o f v o l a t i l e f i s s i o n p r o d u c t s . The u n i f i e d o f f - g a s e s are washed, d r i e d and released t h r o u g h t h e s t ack .
643
REFERENCES
a u s Thorium-Reaktoren, Atomwir t schaf t l3, 417 (1968) . 6d 1. E. Merz, Aufa rbe i tung bestrahl ter Brenn- und B r u t s t o f f e
Y. Lepold , W. Li tzow and H. Wit te , 2. U. T i l l e s s e n , 1 E r g e b n i s s e b e i der Graph i tve rb rennung a l s Head-End- ProzeA zu r Wiede rau fa rbe i tung von HTR-Brennelementen, -0
- _ _ Reak to r t agung 1 des Deutschen Atomforums, A p r i l 2 0 - L L , 1970, B e r l i n , S e k t i o n 4.6.
3. 0. Coenegracht , G . Kaiser and E. Zimmer, Das Head-End des KFA/TBP 23/25-Prozesses , Reaktor tagung des Deutschen Atomforums, A p r i l 20 - 2 2 , 1970, B e r l i n , S e k t i o n 4.6.
4 . J. H. Goode and J. G . Moore, Adsorp t ion of P r o t a c t i n i u m : F i n a l Hot-Cel l Exper iments , ORNL-3950 (1967) .
5. G. Kaiser and E. Merz, Adsorp t ion von P r o t a k t i n i u m a u s schwefe l sau ren Ltjsungen a n Vycor-Glas 7930, P roceed ings of t h e 3. I n t e r n . P r o t a c t i n i u m Conference , A p r i l 1 5 - 1 8 , 1969, SchloA Elmau(Germany).
6. Chemical Technolopy D i v i s i o n , Annual P r o g r e s s Repor t , P e r i o d Ending May 31, 1966, ORNL-3945 (1966) .
7. M . Laser, P ro tak t in ium- , Zirkonium- und Niob-Sorpt ion an S i l i c a g e l e n und Vycor-Glas a u s s a l z s a u r e r Liisung, Hauptversammlung der Gesel lschaft Deutscher Chemiker, September 15 - 2 0 , 1970, Hamburg (Germany), t o b e p u b l i s h e d .
8. L. SchSfer , B. Wojtech, B. G. Brodda, H. K i rchne r and H. J. Riedel, Wiede rau fa rbe i tunp t h o r i u m h a l t i g e r Kern- b r e n n s t o f f e nach dem THOREX-ProzeA, Reaktor tagung des Deutschen Atomforums, A p r i l 20 - 2 2 , 1970, B e r l i n , S e k t i o n 4.6.
9. G . Kaiser, E. Merz and E. Zimmer, The KFA/TBP 23/25- P r o c e s s - A S o l v e n t E x t r a c t i o n Reprocess ing Method f o r Thorium-Uranium F u e l s , t o b e p u b l i s h e d .
10. E. F i s c h e r , Entwicklung e i n e s V e r f a h r e n s z u r c h l o r i e - r enden Wiede rau fa rbe i tung g r a p h i t u m h U l t e r Reaktor- brenn- und Bru te l emen te , Ph. D. T h e s i s , Technische Hochschule Aachen (Germany), Februa ry 1970.
11. E. F i s c h e r , M. Laser and E. Merz, C a l c u l a t i o n s on t h e s e p a r a t i o n p r o p e r t i e s o f thorium-uranium f u e l s by c h l o r i d e v o l a t i l i z a t i o n , Nuc lea r Meta l lu rgy l5, 645(19697.
644
DISCUSSION 8 V . C . A . Vaughen: Would you c a r e t o d e s c r i b e t h e decon tamina t ion
f a c t o r s YOU have found i n your bu rn ing s t u d i e s f o r t h e pr imary m e t a l l i c
f i l t e r , t h e secondary f i l t e r s , and th rough t h e p l a n t o f f - g a s ?
E . Merz: I d i d n ' t have t h e t i m e t o go i n t o more d e t a i l i n my
p r e s e n t a t i o n so I w i l l g i v e you a r e f e r e n c e t o t h e f i g u r e s and numbers w e
o b t a i n e d . C o l l a b o r a t e s t u d i e s on t h i s s u b j e c t have been made and a r e
s t i l l under way t o g e t h e r w i t h o u r i n d u s t r i a l p a r t n e r , t h e Nukem Company.
Refe rence 2 of o u r paper d e s c r i b e s t h e r e s u l t s o b t a i n e d s o f a r i n d e t a i l .
L. R . Zumwalt: I n your c l o r i n e x p r o c e s s , of what m a t e r i a l s i s t h e
c h l o r i n a t i o n r e a c t o r made? D o you have any c o r r o s i o n problems i n c i d e n t
t o t h e c h l o r i n e t r e a t m e n t c a r r i e d o u t a t 1 0 0 0 ° C ?
E . Merz: The c h l o r i n a t i o n r e a c t o r c o n s i s t s of a n inne r -po rous
c y l i n d e r made of g r a p h i t e and an o u t e r g a s t i g h t j a c k e t . The g r a p h i t e
i t s e l f w i t h s t a n d s c h l o r i n e v e r y w e l l a t 1000° C. P r a c t i c a l l y no c o r r o s i o n
c o u l d be obse rved d u r i n g long r e a c t i o n t i m e : ; . The problem i s t h e o u t e r
g a s - t i g h t c y l i n d e r . Me ta l s a r e n o t a v a i l a b l e f o r u s e a t t h i s h i g h tempera-
t u r e . P o r c e l a i n o r even b e t t e r g r a p h i t e t u b e s a r e w e l l s u i t e d f o r t h i s
purpose. T h e i r s a f e a p p l i c a t i o n must s t i l l be proven, however, i n h o t
r u n s unde r s e v e r e c o n d i t i o n s .
A . M. Weinberg: How c o m p l e t e l y do you e x p e c t t o r e t a i n r a d i o a c t i v e
g a s e s t h a t come from your i n i t i a l bu rn ing of t h e f u e l e l emen t s?
E . Merz: Our c l ean -up system shou ld p r o v i d e a n e a r l y complete
r e t e n t i o n of r a d i o a c t i v e g a s e s . Dus t s and a e r o s o l s a r e r e s p e c t i v e l y
abso rbed on a s t a c k of f i b e r g l a s s f i l t e r and c h a r c o a l t r a p s . T r i t i u m i s
o x i d i z e d t o T 0 d u r i n g t h e bu rn ing and t h i s can be removed from t h e
g a s s t r e a m by a b s o r p t i o n on molecu la r s i e v e s . I n c a s e a r a r e g a s c o n t a i n -
ment i s a s p i r e d , a l l t h e ca rbon d i o x i d e i s f i r s t abso rbed on l a r g e
z e o l i t e columns, whereas t h e u n p o l a r r a r e g a s e s p a s s t h e s e columns wi th -
o u t a d s o r p t i o n and may be c o l d t r a p p e d and s t o r e d . The z e o l i t e can be
e a s i l y r e g e n e r a t e d by h e a t i n g up. The n e a r l y r a d i o a c t i v e f r e e ca rbon
d i o x i d e i s t h e n r e l e a s e d i n t o t h e open a i r .
a cheap one.
2
However, t h i s method i s n o t
645
M. D a l l e Donne: Coming back t o t h e ques t ion of D r . Weinberg of
burning of t h e g r a p h i t e . I t h i n k t h a t t h i s i s a c r i t i c a l po in t . I f you
have a l l t h e g r a p h i t e of t h e b a l l s , t h e amount of CO produced must be
enormous, SO t h a t you must d i scharge t h e (202 t o t h e atmosphere and you
cannot s t o r e i t . You should, t h e r e f o r e , be a b s o l u t e l y s u r e t o e l i m i n a t e
t h e major p a r t of t h e r a d i o a c t i v i t y from t h e CO inc lud ing t h e a c t i v i t y
coming from t h e nob le gases .
2
2
E. Merz: I agree wi th your comment. This problem r e p r e s e n t s
c e r t a i n l y one of t h e main drawbacks of t h e combustion procedure. On t h e
o the r hand, a n e a r l y complete clean-up of t h e l a r g e of f -gas volumes i s
f e a s i b l e , though i t i s an expensive approach.
w e a r e t r y i n g t o develop t h e Chlorinex process . H e r e t h e of f -gas c lean-
up i s s i m p l i f i e d cons iderably due t o t h e f a c t t h a t only small q u a n t i t i e s
of gases a r e formed.
T h a t ' s t h e main reason why
A . L. L o t t s : Would you comment on what you in t end t o do i n t h e
f u t u r e with t h e U235 which has been i r r a d i a t e d ?
E . Merz: To my knowledge w e have t o d e a l w i th a used f eed and
breed element, and so i n t h i s c a s e w e a r e recover ing both t h e unconsumed
235U a s w e l l a s t h e bred 233U. In c a s e a f eed and breed concept i s appl ied
t h e f e e l element may j u s t be dumped s i n c e most of t h e 235U has d i s -
appeared. Depending on t h e 235U/236U r a t i o i t may be recovered and re-
used. Maybe t h e e x p e r t s could be t te r answer t h i s ques t ion .
C . B. Z i t ek : What i s t h e i n i t i a l carbon burning s t e p being planned
t o be done a t t h e power p l a n t ?
E . Merz: This i s proposed for i n i t i a l ope ra t ion when only a ve ry
few " E - r e a c t o r s a r e i n ope ra t ion . L a t e r t h e head-end f a c i l i t y w i l l be
i n t e g r a t e d , of course, i n t h e a c t u a l reprocess ing p l a n t . The conceptual
design s tudy may even r e v e a l t h a t t h i s concept d o e s n ' t g ive any advantage
a t a l l . I t depends l a r g e l y on t h e t r a n s p o r t a t i o n c o s t s .
E . Merz: Dealing wi th t h e ques t ion of r e l i a b i l i t y of t h e heavy
machinery needed f o r t h e g r ind ing of g r a p h i t e base f u e l elements, one of
t h e most important requirements i n des igning t h e layout of t h e c rush ing
and m i l l i n g appara tus i s good r e l i a b i l i t y . I n our experiments w e found
646
o n l y a s m a l l a b r a s i o n r a t e o f t h e heavy d u t y p a r t s .
c o n s t r u c t e d such t h a t s p a r e p e r t s can e a s i l y be r e p l a c e d by remove
o p e r a t i o n . F u r t h e r , t h e o p e r a t i o n and main tenance i s v e r y s imple .
The machinery i s
R. E. BlsnCG: What t y p e of w a s t e d e n i t r a t i o n and s o l i d i f i c a t i o n
p r o c e s s d i d you select and why d i d you se lec t t h i s method?
E . Merz: The proposed f low-shee t f o r t h e d e n i t r a t i o n and s o l i d i f i c a -
t i o n i s a r e s u l t of a t ho rough s t u d y and e v a l u a t i o n of t h e d i f f e r e n t
methods deve loped and used e l s e w h e r e . C o n s i d e r i n g t h e p r o p e r t i e s of t h e
e x p e c t e d w a s t e s o l u t i o n s a s wel l a s t h e s p e c i a l r e q u i r e m e n t s f o r a f i n a l
d i s p o s a l i n Germany, i t seems t o u s t o secur'? i n an optimum way t h e
h i g h e s t v e r s a t i l i t y , s a f e t y , s i m p l i c i t y , and economy. The r e s u l t s o b t a i n e d
so f a r i n o u r e x p e r i m e n t s j u s t i f y our d e c i s i o n .
po ta s s ium s u l p h a t e t h o r a t e p r e c i p i t a t e i s foreseen f o r a d i r e c t s t o r a g e ;
i t w i l l p robab ly n e v e r be r eused .
F u r t h e r , t h e d r i e d
647
By T i t l e
Review of USAEC - ORNL
HTGR F u e l Recycle Program
D. E . Ferguson,
O a k Ridge N a t i o n a l L a b o r a t o r y
SOME FEATURES O,F-TE& LOW EZBIW-Qi.T-HTR FOR VARIOUS FUEL ELEMENT DESIGNS,-<% __ --
d T ~ ~ ~ ~ it,:, .--_ ~ __ - -_
CParametr ic Fuel Cycle Surveys
G . R ina ld in i , GCR Euratom - I s p r a C. Zanantoni, GCR Euratom - I s p r a
H. B a i r i o t , Belgonucl6aire P. Haubert, Belgonuclgaire
G . Graz ian i , GCR Euratom - I s p r a zqq/d-”J
72-L 6 OQO
G. G h i l a r d o t t i , Agip Nucleare O / b zo620 M. Baur, GGH’ 372 g@d
In t roduc t ion
I n t h e course of t h e i r p re sen t and previous work f o r t h e opt imiza t ion
of low enrichment f u e l cyc le s f o r HTR’s, t h e au tho r s have t r i e d t o a s s e s s t h e f u e l cyc le cos t i n terms of very few parameters which have a paramount
e f f e c t on t h e phys ica l performance of t h e f u e l .
i s made t o p inpo in t such “predominant” parameters which w i l l al low, on t h e b a s i s o f t h e i r choice alone, t o make a good p r e d i c t i o n of t h e phys ica l and
economical performance of t h e f u e l considered.
I n t h i s paper an a t tempt
This work i s based on a number of f u e l cyc le surveys c a r r i e d ou t a t I s p r a i n r ecen t t imes, t h e most r e c e n t w i t h f o u r f u e l element concepts:
t h e hollow rod, t h e tubu la r , t h e t e l e d i a l and t h e t r e f o i l f u e l element.
~ They cover about a l l t h e f u e l element types considered up t o now i n Europe f o r low enrichment f u e l cyc le s i n HTR’s, w i t h the exception o f the multi-
annu la r f u e l element p u t forward i n t h e e a r l y s t a g e s of t h e s t u d i e s on low
enrichment cycles and now abandoned.
The survey descr ibed here w a s performed f o r two va lues of t h e core-
average power dens i ty , vary ing t h e burn-up and t h e moderation r a t i o wi th in
t h e range of i n t e r e s t . The v a r i a t i o n of C/U238 w a s ob ta ined by vary ing
t h e heavy metal dens i ty , while t h e geometry ( f u e l dimensions and l a t t i c e
p i t c h ) was kept cons tan t . This s i m p l i f i e d approach w a s adopted f o r t h e
p re sen t survey, as our prev ious work’ had shown t h a t t h e whole range of
i n t e r e s t i n g va lues of t h e parameters which determine t h e f u e l cyc le phys ics
and economics can be covered i n t h i s way.
649
650
Indeed, two f u e l elements o f q u i t e d i f f e r e n t s i ze , shape and heavy @ metal d e n s i t y l e a d t o t h e same enrichment, conversion r a t i o and age f a c t o r
provided t h e moderation r a t i o (C/U238) and t h e resonance i n t e g r a l a r e t h e
same. This w i l l be explained i n more d e t a i l l a t e r on.
Fuel Cycle Physics
The Calcula t ion Method.--The parameters of a f u e l cycle f o r a given
power dens i ty , buckl ing and d ischarge burn--up were evaluated f o r t h e equi-
l i b r ium condi t ions wi th t h e hypothesis of continuous charge-discharge.
The code MOGA2 (Modified GAffee) was used.
enrichment of t h e f r e s h f u e l and t h e composition of t h e discharged f u e l .
It c a l c u l a t e s t h e necessary
No r ecyc le of t h e spent f u e l was assumed, wi th s a l e of t he produced
Plutonium. The c a l c u l a t i o n s were c a r r i e d out wi th 20 energy groups (8 f a s t ) .
The v a r i a t i o n of t h e e f f e c t i v e c ros s s e c t i o n s w i t h t h e f u e l composi-
t i o n w a s taken i n t o account by means of v a r i a b l e s e l f s h i e l d i n g f a c t o r s .
The dependence of t h e s e l f s h i e l d i n g f a c t o r s upon t h e macroscopic
c r o s s s e c t i o n of t h e c e l l w a s f i t t e d w i t h a simple formula t o a number of
c e l l c a l c u l a t i o n s performed wi th t h e SN code WRETCH3 ( inco rpora t ing WDSN) . For t h e U238 resonances, t h e e f f e c t of t h e double he te rogenei ty of
t h e f u e l w a s taken i n t o account by t h e equivalence theorem:4
e = o + eff po
where
= absorber d e n s i t y i n t h e ke rne l
= mean chord l e n g t h of t h e k e r n e l
= B e l l f a c t o r o f t h e ke rne l
= carbon s c a t t e r i n g c ros s s e c t i o n p e r absorber atom i n t h e lump m = absorber d e n s i t y i n t h e lump e
4, = mean chord l e n g t h i n t h e lump
NO
2, 0
o
N
= B e l l f a c t o r o f t h e lump
= p o t e n t i a l s c a t t e r i n g c ross s e c t i o n of t he ke rne l p e r absorber a t “e
(T PO
651
0 The mean chord l e n g t h t w a s determined wi th t h e L e s l i e approximation
where
= lump-to-lump c o l l i s i o n p r o b a b i l i t y determined by t h e c o l l i s i o n
= absorp t ion c r o s s s e c t i o n of t h e lump p r o b a b i l i t y code Procope5 pf f
The B e l l f a c t o r was determined as a func t ion of o
m eff
and 114, Ne by rn c a l c u l a t i o n s f i t t i n g t h e above-mentioned formula on a number of 0
performed w i t h a ZUT code, modified t o t ake i n t o account t h e double he te ro-
gene i ty according t o t h e Nordheim-Lane theory . 6
The t rea tment of f i s s i o n products w a s q u i t e d e t a i l e d : 25 ind iv idua l f i s s i o n products and two aggrega tes were considered, so t h a t t h e e r r o r i n r e a c t i v i t y induced by t h i s t rea tment as compared t o t h e exac t one was
estimated t o be i n any case sma l l e r t han 0.2$.
Main Assumptions.--As s a i d , t h e f u e l cycle c a l c u l a t i o n s were performed Therefore, t h e r e a c t o r s i z e a f f e c t s t h e f u e l
'. - i n a zero-dimensionkl scheme.
cyc le phys i c s only through t h e buckl ing, which was assumed cons tan t through-
o u t t h e energy range and was va r i ed pa rame t r i ca l ly i n t h e survey.
The equ i l ib r ium K-ef fec t ive w a s assumed t o be 1, i . e . no a d d i t i o n a l r e a c t i v i t y investment i n c o n t r o l rods w a s assumed, a p a r t from t h a t a l ready devoted t o Xe-override.
The charge and d ischarge of t h e r e a c t o r were assumed t o be continuous, t h e r e f o r e no account w a s t aken of t h e LOSS of neut rons due t o t h e reac-
t i v i t y v a r i a t i o n dur ing a re load i n t e r v a l .
t h e approach-to-equi l ibr ium phase of r e a c t o r ope ra t ion . d i scussed i n p a r t 2 of t h i s paper .
Also, no account w a s t aken of
This po in t i s
These approximations a r e qu i t e s a t i s f a c t o r y i n many ins tances , bu t p a r t i c u l a r l y so i f t h e r e s u l t s of t h e p r e s e n t work a r e used t o compare
d i f f e r e n t types of f u e l and t o have an i n s i g h t i n t o t h e e f f e c t o f va r ious
652
phys ica l parameters, r a t h e r than t o make a d e t a i l e d assessment of t h e
f u e l cycle cos t f o r a p a r t i c u l a r , case.
Cross Sec t ion Data.--The Gulf General Atomic c ros s s e c t i o n l ibrairy
was used, i n connection w i t h t h e code GGC I1 (GAM - GATHER Combined) .' Age Factors.--The age f a c t o r i s def ined here as t h e r a t i o between
t h e power i n a channel loaded wi th f r e s h fue:L and t h e power i n that chan-
n e l loaded wi th t h e equi l ibr ium ( l i f e - a v e r a g e ) composition.
A s it i s ca l cu la t ed by t h e MOGA code i n a zero-dimensional scheme,
it does not t ake i n t o account t h e space v a r i a t i o n of t h e f l u x fol lowing
t h e re load of a channel, l e t a lone of a f u e l block o f , say, 18 channels.
This l e a d s t o an underest imate of t h e age f a c t o r p a r t i c u l a r l y a t l o w age
f a c t o r va lues . However, t h i s approximation bas considered t o be sa t i s -
fac tory , because t h e purpose of t h i s survey i s t o show:
( a ) t h e f u e l cyc le phys ics
( b ) t h e dependence of , among o t h e r s , t h ? age f a c t o r upon t h e e f f ec -
t i v e moderation r a t i o ( s e e l i s t of symbols).
t h e l i t t l e e f f e c t of t h e choice of t he shape of t h e f u e l on
Fuel Cycle Economics
The present-worth account ing method was no t used, a s on ly t h e equi-
l i b r ium condi t ions of t h e f u e l cyc le were known.
The f i x e d f u e l cyc le cos t s , 5 .e . t hose depending on the core inven-
t o r y of f u e l , were a s ses sed by a t t r i b u t i n g t o the core a "value" equal
t o t h e average between a core f u l l of f r e s h f u e l elements ( i n c l u d i n g t h e
f a b r i c a t i o n c o s t ) and a core fu l l of spent f u e l elements (deducing the
reprocess ing c o s t ) .
charge-discharge equi l ibr ium cycle wi th enriched uranium feed and s a l e
of t h e discharged Plutonium and Uranium.
The c a l c u l a t i o n s were performed f o r a continuous
Two s e t s of va lues were assumed f o r t h e f s b r i c a t i o n c o s t s and f o r
t h e discharged plutonium va lue : t h e low f a b r i z a t i o n cos t being coupled
wi th t h e l o w plutonium va lue and v ice-versa . 'The high f a b r i c a t i o n cos t
i s r ep resen ta t ive of t h e pro to type r e a l i s a t i o n a , while t he low es t imate
i s c h a r a c t e r i s t i c of a l a r g e market. These two s e t s imply d i f f e r e n t cos t
653
f i g u r e s f o r t h e d i f f e r e n t f u e l elements which w i l l be descr ibed i n t h e
next chapter . Other c a l c u l a t i o n s w i t h economic assumptions i d e n t i c a l f o r
a l l f u e l elements were a l s o performed ( s e e Chapter 5 ) . The r e l e v a n t eco- nomic assumptions a r e l i s t e d below:
Plutonium va lue :
8 (low) and 1 5 ( h i g h ) $ / g f i s s i l e
Fabr i ca t ion cos t :
C F = A + B K + D (v) $/Kg uranium
where
K = c o s t of UF6 ($/Kg uranium)
C - = atomic r a t i o carbon t o uranium (moderation r a t i o ) U
K accounts f o r f a b r i c a t i o n l o s s e s , D f o r g raph i t e f a b r i c a t i o n c o s t . The
va lues a r e given i n P a r t 11, Table 2.
Reprocessing cos t : 60 $/Kg
P l a n t da t a :
g ros s thermal e f f i c i e n c y 4 8
blowers e f f i c i e n c y 9@
e l e c t r . motors e f f i c i e n c y 95% e x t e r n a l pressure-drop 0.3 a t .
Reference p res su re drop f o r t h e f o u r f u e l elements, assuming a n equ iva len t
t r i a n g u l a r p i t c h of 8.87 em:
core- average core-pressure power d e n s i t y drop
Fuel element 1 1 0.07 Fuel element 2 7 0.11 Fuel element 3 7 0.17 Fuel element 4 7 0.14
WI cm3 a t m
These re ference va lues a r e i n c l u s i v e of t h e r a d i a l power shape f a c t o r ,
no t of t h e age f a c t o r .
t h e age f a c t o r f o r each s i n g l e case.
They were t h e r e f o r e multiplied by t h e square of
654
Delays :
Out of core res idence t ime f o r t h e reprocessed f u e l 360 days
f r e s h f u e l s to rage 180 days i n t e r e s t r a t e = 11%
A
Fuel Cycle Survey w i t h Four Fuel Elements
The r e s u l t s of t h e survey repor ted here w i l l show t h e l i t t l e impor-
tance of t he f u e l element shape as far as the f u e l cycle physics i s con-
cerned.
a s it i s shown i n Chapter 5. This l e a d s t o p l o t t i n g t h e r e s u l t s i n terms of very few parameters,
The f u e l elements considered here a r e the four descr ibed i n Fig. 1:
i n t h i s f i g u r e t h e c ros s s e c t i o n of a s i n g l e channel i s shown. Each
g raph i t e block would con ta in a number of t h e channels . The f u e l mat r ix
i s shown by dot ted a r e a s . The f u e l element L has only one ( e x t e r n a l )
coolan t channel. Fuel elements 2 and 3 have i n t e r n a l and e x t e r n a l cool- i ng . The g raph i t e d e n s i t y was assumed t o be:
1.8 g/cm3 f o r t h e cans
1 . 6 g/cm3 f o r t h e bulk
No account was taken of t h e reduct ion of t he e f f e c t i v e g raph i t e den-
s i t y because of c o n t r o l rod holes e t c . This c o r r e c t i o n would n o t have been
meaningful f o r ou r i n v e s t i g a t i o n , par t icular1.y so i f one th inks t h a t no
r educ t ion of t he uranium loading w a s assumed t o account for t he a x i a l d i s -
t ance between t h e fue l ed s e c t i o n s of t h e charinel.
The r e s u l t i n g r e l a t i o n s h i p between heavy metal d e n s i t y i n t h e f u e l
matr ix , moderation r a t i o n C/U8 and e f f e c t i v e moderation r a t i o (C/U8)eff
( s e e below) i s repor ted i n Fig. 2 f o r an equiva len t t r i a n g u l a r l a t t i c e
p i t c h of 8.87 em.
The c a l c u l a t i o n s were performed f o r :
- 2 va lues of t h e core-average power dens i ty : 6 and 8 w/cm3 ( 4 and
- 3 values of t h e average burn-up a t d ischarge : 60, 80, 100 MwdIKg
- 4 values of t h e moderation r a t i o n C/U238:200, 250, 300, 400
- 1 value of t h e Xe ove r r ide requirement:
5 f o r element 1)
6@ of nominal power
655
A cons tan t va lue o f t h e equ iva len t t r i a n g u l a r p i t c h w a s used: 8.87 cm. Indeed, prev ious experience had shown t h a t a parametr ic v a r i a t i o n of t h e
p i t c h would not con t r ibu te any a d d i t i o n a l information concerning t h e f u e l
cyc le . This i s s a t i s f a c t o r i l y descr ibed by moderation r a t i o and resonance
i n t e g r a l only, as f a r a s t h e e f f e c t s of l a t t i c e he te rogenei ty a r e con-
cerned. In o t h e r words, t h e e f f e c t of a p i t c h v a r i a t i o n can be s imulated
wi th a v a r i a t i o n of f u e l geometry and heavy metal d e n s i t y which l e a d t o
t h e same resonance i n t e g r a l and moderation r a t i o . We s h a l l dwell on t h i s
po in t w i t h more d e t a i l i n t he next chapter .
A s f o r t h e e f f e c t of power d e n s i t y on t h e leakage, a one-group Buckling
w a s deduced from a s impl i f i ed a n a l y t i c a l t rea tment f o r a f l a t t e n e d r e a c t o r .
A more d e t a i l e d s tudy would no t have much sense, because o f t h e o t h e r ap-
proximations involved i n zero-dimensional assessments and because a care-
f u l assessment of t h e Buckling would be p o s s i b l e only f o r a d e t a i l e d
r e a c t o r des ign .
The fol lowing values were used:
power dens i ty : 4 5 6 8 w/cm3
Buck1 ing : .52 .59 .65 .77 m - 2
The equ i l ib r ium f u e l cyc le assessment w a s performed wi th t h e method de-
s c r ibed i n Chapter 2. the heavy metal d e n s i t y i n the compacts.
The moderation r a t i o n C i U 8 was va r i ed by changing
A s an example of t h e r e s u l t s , t h e r e l a t i v e f u e l cycle cost* i s p l o t t e d
for one case i n Fig. 3 t o show how f l a t i s t h e behaviour of t h e cos t as a
func t ion of burn-up and moderation r a t i o . On t h e b a s i s of graphs of t h i s
type t h e optimum cases r epor t ed i n Table 1 were chosen.
t h a t even a cons iderable change of burn-up or moderation r a t i o n wouldn't
a f f e c t t he va lues of Table 1 s i g n i f i c a n t l y .
t o a re ference case (one f o r each economic assumption) which i s quoted
wi th 100 i n the table .
Figure 3 shows
The va lues a r e given r e l a t i v e
* Note. Throughout t h i s paper we have followed t h e p o l i c y of p l o t t i n g
r e l a t i v e o r d i f f e r e n t i a l f u e l cycle cos t s , not abso lu t e va lues . This was made not i n o r d e r t o conce i l r e s u l t s , which can be e a s i l y deduced from t h e information provided, b u t because g iv ing abso lu te c o s t s w a s nor t h e pur- pose n e i t h e r t h e most s i g n i f i c a n t a spec t of t h i s paper.
656
The d i f f e r e n c e s between t h e fou r elements i n Table 1 e r e e s s e n t i a l l y
due t o t h e d i f f e r e n t econonic assumptions.
To show how l i t t l e t h e geometry of t h e f u e l a f f e c t s t h e f u e l cycle
cos t , t h e r e l a t i v e c o s t was p l o t t e d i n F ig . 4 f o r a s i p g l e s e t of economic
assumptions ( those corresponding t o low c o s t , f u e l element 2, see Chapter
3 ) .
Figure 4 shows cLearly t h a t t h e f u e l c:ycle economics i s p r a c t i c a l l y
t h e same, f o r d i f f e r e n t geometries, provided t h e moderation r a t i o n C/U8
i s t h e same. This depends upon t h e f a c t t h a t :
- t h e f a b r i c a t i o n and reprocess ing itern of t h e f u e l cycle cos t depend
only on t h e burn-up
- t h e g raph i t e f a b r i c a t i o n i tem depend:; only on C l U 8 and burn-up
- t h e f u e l consumption i tem i s not very much a f f e c t e d by t h e f u e l
geometry, i . e . resonance i n t e g r a l , because t h i s has counterac t ing e f f e c t s
on t h e average enrichment and on the conversion r a t i o . Indeed, i n these
r e a c t o r s which a r e optimized a t high burn-up, f u l l advantage can be taken
of any improvement i n t h e conversion r a t i o . A s a consequence, t h e inc rease
of average enrichment corresponding t o an inc rease of t h e resonance i n t e -
g r a l i s compensated by an inc rease of t h e conversion r a t i o , which l eaves
t h e feed f u e l enrichment about t h e same, t h e r e f o r e t h e f u e l consumption
about t h e same, f o r d i f f e r e n t geometr ies .
These cons ide ra t ions on counterac t ing e f f e c t s suggest t h a t t h e same
compensations might no t occur f o r o t h e r fue l cyc le parameters, l i k e en-
richment, conversion e t c . This i s t r u e , and it w a s found t h a t a wide
s c a t t e r o f t h e resul ts f o r d i f f e r e n t geometries would occur, i f a p l o t
o f conversion, enrichment, age f a c t o r was at tempted versus the modera-
t i o n r a t i o n C / U 8 . Therefore , t h e e f f e c t i v e moderation r a t i o waF i n t r o -
duced, t o account f o r bo th moderation and resonance i n t e g r a l . The e f f e c t i v e
moderation r a t i o i s t h e phys ica l moderation r a t i o where t h e U238 atoms a r e
weighted wi th the resonance i n t e g r a l . Havirlg chosen 60 as a re ference
va lue f o r t h e R.I., t h e e f f e c t i v e moderation r a t i o n was def ined as
C - C 60 U 8 R I (5) - - -
e f f
657
Figure 5 shows t h e s i g n i f i c a n t physics parameters of t h e f u e l cycle ,
p l o t t e d as a func t ion of t h e e f f e c t i v e moderation r a t i o for t h e va r ious
geometries a t BU = 80 Mwd/Kg, 60$ Xenon ove r r ide . The power d e n s i t y i s
6 W/cm3 except f o r f u e l element 1 ( 5 W/cm3).
has very l i t t l e e f f e c t on t h e p l o t t e d d a t a ( f l u x l e v e l , Xe abso rp t ion ) .
This f i g u r e shows how remarkably w e l l any lumping e f f e c t (geometry, heavy
metal d e n s i t y ) can be descr ibed i n terms of t h e e f f e c t i v e moderation r a t i o
only.
However, t h e power d e n s i t y
A General ized Parametr ic Representa t ion of t h e Resu l t s
With t h e above-mentioned r e s u l t s i n mind , a paramet r ic r e p r e s e n t a t i o n
of t h e f u e l cyc le d a t a w a s envisaged, which could a l low t h e FCR des igner
t o deduce t h e e s s e n t i a l information concerning t h e f u e l cyc le physics by
i n t e r p o l a t i o n between a few curves.
c ho s en :
The fol lowing "main" parameters were
burn-up (BU) = 60, 80, 100 Mwd/Kg
buckl ing ( B 2 ) = 0.5, 0.9 m-2
e f f e c t i v e moderation r a t i o (C/U8 x 60/RI) = 200, 250, 300, 400
Besides t h e s e main parameters, o t h e r t h r e e "secondary" parameters a r e
needed t o de f ine t h e f u e l cyc le physics , i . e . :
2/U8 moderation -
power density
core-average carbon dens i ty yv
' P C
The use of t he moderation r a t i o C/U8 i s obviously equiva len t t o t h a t of
t he s p e c i f i c power i n t h e fue l , as they a r e p ropor t iona l a t cons tan t
power d e n s i t y ( a t 7 w/cm', t h e moderation r a t i o s 200, 300, 400, 500 cor-
respond t:, s p e c i f i c power 50, 75, 100, 125 - r e s p e c t i v e l y ) .
P
W 63
It should be pointed ou t t h a t i f C/U% can be regarded as a secondary
parameter from t h e po in t of view of t h e phys ics (see e .g . Fig. 14) t h e
same cannot be s a i d about economics. The important e f f e c t of C / U 8 on
economics i s obvious i f one t h i n k s of i t s equivalence t o s p e c i f i c power.
Figures 6 and 7 a r e repor ted t o show t h i s e f f e c t . They were calcu-
l a t e d w i t h t h e physics d a t a of F igs . 8-19 and t h e economic assumptions
corresponding t o f u e l element 2, low c o s t . @
658
The e f f e c t o f t h e llmainff parameters and of C/U8 on t h e f u e l cycle
physics i s shown i n F igs . 8 t o 19. They can be used t o i n t e r p o l a t e t h e
r e s u l t s f o r any f u e l cyc -e , whatever t h e s i z e , shape and dens i ty of t h e
f u e l element.
The repor ted d a t a 'are r e l a t i v e t o
- power d e n s i t y 7 w/c.m3 - core-average g r a p h i t e d e n s i t y 1 . 4 E ; / em3
However, t h e e f f e c t of t h e s e two "secondary" parameters on t h e f u e l cyc le
physics i s small, as it i s due only t o
- f l u x l e v e l ( X a b s o r t i o n ) : j . and x c - neutron migra t ion a r e a ( l eakage ) :
e V
Therefore t h e f i g u r e s 8-19 can be used f o r a wide range of 2/ For a more d e t a i l e d a n a l y s i s , c o r r e c t i o n s f a c t o r s could be e l abora t ed .
and tc. V
The e f f e c t o f C / U 8 on t h e f u e l cyc le pkl.ysics, i l l u s t r a t e d by Figs .
8-19, i s more c l e a r l y shown i n Table 2.
The meaning of t h e symbols i s a s fo l lows:
'il eta va lue f o r t h e mixture of f i s s i l e i so topes
c carbon absorp t ion
e
e ov
NFHM absorp t ion by non f e r t i l e heavy meta ls (U236, 237, 239 twice,
X Xenon abso rp t ion
abso rp t ion by ove r r ide con t ro l rods X
FP f i s s i o n products abso rp t ion
Pu242)
I n t h i s t a b l e t h e neutron balance i s i r e p o r t e d f o r a given s e t of t h e
"main" parameters and s e v e r a l C / U 8 va lues .
- on the thermal neutron spectrum ( 7 ) - on t h e r a t i o between thermal and ep i thermal flux (NFHM, FP) - on t h e carbon absorp t ion , as obvious ( e )
- on t h e f l u x l e v e l , as it i s p ropor t iona l t o t h e s p e c i f i c power (Xe, Xe o v e r r . )
- on t h e leakage, because of t h e v a r i a t i o n o f t h e migra t ion area, due t o t h e v a r i a t i o n of U238 dens i ty , enrichment e t c . a t cons tan t graph- i t e dens i ty .
659
0 Concluding Remarks
The he terogenei ty of t h e HTR cores cannot be as l a r g e as t o make t h e
f u e l element shape and s i z e r e l e v a n t from t h e po in t o f view o f t h e f u e l
cycle phys ics .
t h e f u e l shape, s i z e and d e n s i t y and l a t t i c e p i t c h , as far as neutron
physics i s concerned.
can be c a r r i e d ou t independent of t he nuc lea r op t imiza t ion . The flexi-
b i l i t y of t h e HTR design makes t h e use of such genera l ized graphs as those presented here p a r t i c u l a r l y u s e f u l .
The des igner has t h e r e f o r e a l a r g e freedom of choice of
Also, t h e thermal op t imiza t ion o f t h e f u e l element
Acknowledgements
The au tho r s g r a t e f u l l y acknowledge t h e keen co l l abora t ion of
M. Pa rucc in i (EURATOM) and F. P a s q u i n e l l i (AGIP Nucleare) , who a s s i s t e d
them wi th computer work and va luable sugges t ions throughout t h e prepara-
t i o n o f t h e paper .
L i s t o f t h e Main Symbols and D e f i n i t i o n s
w power d e n s i t y (-) = power p e r u n i t core volume
W s p e c i f i c power (-) = core-average power p e r u n i t heavy metal g weight
core-average carbon dens i ty (5)
V em3
C
C (3) e f f e c t i v e moderation r a t i o = C / 8 w i t h t h e U238 d e n s i t y
e f f weighted w i t h t h e resonance i n t e g r a l
BU average burn-up a t d ischarge (MWd/Tm)
(%'eff e f f e c t i v e moderation r a t i o = C/U8 w i t h t h e U238 d e n s i t y weighted w i t h t h e resonance i n t e g r a l
R I resonance i n t e g r a l (b ) = U238 abso rp t ion c ros s s e c t i o n
B* buckl ing (m-*) cons t an t over the. whole energy range and in- averaged over t h e whoye e p i t h e m a l range o f l e t h a r g i e s
troduced i n t h e zero-dimensional burn-up code t o account f o r neutron leakage.
X age f a c t o r = reactor-average r a t i o o f t h e beginning o f l i f e t o t h e l i f e - a v e r a g e power i n a f u e l element
660
conversion r a t i o = core average ( l i f e - a v e r a g e ) r a t i o between r a t e of formation and r a t e of d e s t r u c t i o n of f i s s i l e i so topes . Evaluated f o r t h e equ i l ib l ium composition
e t a value (neu t ron regenera t ion f a c t o r ) f o r t h e mixture of f i s s i l e i s o t o p e s . Evaluated for, t h e equi l ibr ium composition
(%I f i s s i l e material weight t o t a l heavy metal weight 6 enrichment =
6 f r e s h f u e l enrichment ($) i
6 average f u e l enrichment (U235 + f i s s i l e Pu) ( l i f e average = core average) ( k )
6 t o t a l enrichment (U235 + f i s s i l e Pu) of spent f u e l (8) f r o r
E spent f u e l enrichment i n f i s s i l e Plutonium (4) f P U
X % Xenon ove r r ide requirement: c a p a b i l i t y of r e s t a r t a f t e r sudden power r educ t ion from l0@ t o ( 1 0 0 - X ) $
REFERENCES
1. C . Zanantoni, Cont r ibu t ion t o t h e d i scuss ion of paper SM-111/63. Advanced High Temperature Gas- cooled Reactors, IAEA, Vienna 1969, pages 726-728.
2. C . Zanantoni e t a l . , I n t e r n a l EURATOM Report t o be publ i shed .
3. C. Zanantoni e t a l . , I n t e r n a l FXJRATOM Report t o be publ i shed .
4. J. Journe t , Resonance Absorption i n Mate r i a l s w i th G r a i n S t r u c t u r e . Equivaience Rela t ion . Dragon P r o j e c t Report 615, Dee. 1968.
5. L . Amyot, P. Benoist , F i r s t F l i g h t C o l l i s i o n P r o b a b i l i t i e s i n P in -
Clus te r s and Rod L a t t i c e s , Nucl. Sc. Eng. 28, 215-225 (1967 and PROCOPE - ELTR 32% (1%7)
6. R . K. Lane, L . W. Nordheim and J. B. Sampson, Resonance Absorption i n Mate r i a l s w i t h Grane S t r u c t u r e , Nucl. Sc. Eng. 14, 39G396 (1.962).
7 . G . D . Joanou, e t a l . , G . G . C GAM-GATHER-COMBINED, GA 4265 and 4132, 1963.
J
661
~ -~
Scale 1:2
rl
fuel elemen n* 1 fuel element n* 2 fuel element n'3 fuel element n.4
Figure 1. The four fuel elements
Table 1. Minimum Relat ive Fuel Cycle Cost with Four Fuel Elements
Type of Fuel 1 2 3 4
4 5 6 8 6 8 6 8 Power Density ( W/ em3)
Low fahri- 6 6 Xe 105 101 102 100 103 101 107 105 ca t ion cos t overr ide
106 Xe 107 103 105 103 106 105 111 110 overr ide
High fabr i - 6oq6 Xe 108 104 1% 100 1% 100 108 105 ca t ion cos t overr ide
106 Xe 110 106 106 103 106 1% 111 108 overr ide
For A l l Types of Fuel
Optimum Burn-up Optimum MWd/ Kg C/U8
LOW c o s t 80 300
High c o s t 100 300
Table 2. Effect of t h e Moderation Rat io on the Neutron Balance Equilibrium Fuel Cycle, Continuous Charge-Discharge
= 250; B2 = 0.5 m-2 C
' 8 e f f BUITI-UP = LOO MWd/Kg: -
power dens i ty = 7 w/cm3 core-average carbon dens i ty = 1.4 g/cm3
Absorptions ($)
C Leakage C Xe & 60 ($) NFHM F P Total (%) overr ide Losses ' 8
SOME FEATURES OF THE LOW ENRICHED HTR w>--~.P*<U--..*^ -..-r--.MIQPyr--*- I ' -
FOR VARIOUS FUEL ELEMENT DESIGX P a r t I1
Comparison of the f u e l element designs
_I_̂----.
L_c_------ G . G h i l a r d o t t i AN
AN :'Agip Nucleare - Milano Members of BN : BELGONUCLEAIRE - Brusse ls INTER GHH : Gutehoffnungshutte - Sterkrade ( NUCLEAR CCR : EURATOM - I s p r a
ABSTRACT
This p a r t i s devoted t o the a n a l y s i s of va r ious types of f u e l on t h e b a s i s of the parametr ic s tudy o u t l i n e d i n P a r t I .
Frame of work
The work i s based on a survey of t he f u e l cyc le c o s t w i th four f u e l element concepts analysed i n a companion paper t o the present symposium1 : the hollow rod , t he t u b u l a r , t he t e l e d i a l and t h e t r e f o i l f u e l e lements . They cover about a l l t he f u e l element t ypes considered up t o now i n Europe f o r low enrichment f u e l c y c l e s i n H T R ' s , wi th the except ion of t he mult iannular f u e l element put forward i n the e a r l y s t a g e s of the s t u d i e s on low enrichment cyc le s and now abandoned. d a t a are a l s o given on the i n t e g r a l f u e l block concept .
Some
The present survey covers :
- two power d e n s i t i e s f o r each f u e l element : 6 and 8 MW/m3 f o r a l l bu t t he hollow rod , f o r which 4 and 5 MW/m3 a r e cons idered ;
- t h r e e burn-ups : 60, 80 and 100 GWd/t ;
- two choices f o r the Xenon ove r r ide requirements : 70 % and 100 % ;
- a range of moderation r a t i o s from 200 t o 400 C atoms/U 238 atoms, ob ta ined by vary ing the heavy metal dens i ty , while t h e geometr ical c h a r a c t e r i s t i c s of t h e f u e l (dimensions and p i t c h ) a r e kept cons tan t
671
672
wi th in each des ign . This s impl i fy ing approach was s e l e c t e d f o r the present survey, s ince e a r l i e r work has demonstrated t h a t the modifi- c a t i o n of f u e l rod dimensions o r p i t c h w i t h i n p r a c t i c a l l i m i t s only induce secondary e f f e c t s ;
- two s e t s of assumptions f o r the f a b r i c a t i o n c o s t s and f o r the d i s - charged plutonium va lue : t he low f a b r i c a t i o n c o s t being coupled wi th the raw plutonium va lue and v i ce -ve r sa . The high f a b r i c a t i o n cos t i s r e p r e s e n t a t i v e of t h e prototype r e a l i z a t i o n s , while the low es t ima te i s c h a r a c t e r i s t i c of a l a rge market.
The c a l c u l a t i o n s were done f o r a continuous charge-discharge equi- l i b r ium cyc le wi th enr iched uranium feed and s a l e of t he discharged plutonium and uranium.
Fuel cyc le cos t
The f u e l cyc le c o s t s a r e a s ses sed f o r ,the four elements considered, t he two power d e n s i t i e s and the t w o Xenon ove r r ide requi rements and f o r two c o s t assumptions. Under the c o s t assumptions descr ibed i n the paper, t h e f u e l cyc le was found t o be 18 % lower f o r t h e l o w f a b r i c a t i o n c o s t assumption than f o r t h e h igh f a b r i c a t i o n c o s t assumption.
Generat ing c o s t
The equ i l ib r ium f u e l cyc le cos t a s a s ses sed i n t h i s study i s not a s u f f i c i e n t c r i t e r i o n f o r t he s e l e c t i o n of t:he f u e l des ign and t h e f u e l cyc le c h a r a c t e r i s t i c s .
The f u e l cyc le c o s t should f i r s t be co r rec t ed f o r t h e approach t o equ i l ib r ium per iod . The inf luence of t h i s per iod i s i l l u s t r a t e d .
Furthermore, t h e c a p i t a l c o s t may be inf luenced by some f u e l c h a r a c t e r i s t i c s such as the power d e n s i t y . This e f f e c t i s assessed f o r t he four element des igns .
Conclusions
The r e s u l t s of the f u e l design and development e f f o r t s 192 impose t o exclude some a reas covered by the present s tudy . This p inpoin ts t o p i c s f o r f u r t h e r development.
673
INTRODUCTION
The purpose of t h i s second p a r t i s t o compare va r ious f u e l des igns , 1 descr ibed i n a companion paper t o the present symposium
t h e in f luence of t he economical environment. The broad f i e l d t o be covered
l e a d s t o the adopt ion of s i m p l i f i e d approaches, backed by previous experien-
ce ; some assumptions w i l l .be mentioned i n t'he paper t o i l l u s t r a t e t h i s .
and t o emphasize
I n t h i s frame, the gene ra l i zed parametr ic approach, o u t l i n e d i n
Pa r t I , i s a pe r fec t b a s i s f o r more e l a b o r a t e developments.
The s tudy summarized i n t h e present paper i s s u f f i c i e n t t o sc reen the
most promising f i e l d s . The rea f t e r , i t i s necessary t o look i n t o more
d e t a i l s , i n order t o s e l e c t a near optimum design f o r each p a r t i c u l a r
c a s e . This d e t a i l e d t reatment can no more be l imi t ed t o economic cons i -
d e r a t i o n s , but has t o be i n t i m a t e l y connected wi th a l l t he design, manufac-
t u r i n g and development a spec t s , some of which being descr ibed i n o the r 1 , 2 papers .
To avoid misleading f i g u r e s and t o give a c l e a r e r view of the impor-
tance of each i tem, the c o s t s a r e being quot:ed i n r e l a t i v e terms ; t h i s
shows b e t t e r whether some t r ends a r e u n i v e r s a l .
DESCRIPTION OF THE FUEL ELEMENTS
1 A s expla ined i n the paper a l r eady r e f e r r e d t o , f i v e f u e l element
designs were i n v e s t i g a t e d , t he hollow (HR), t ubu la r (Tu), t r e f o i l (Tr)
and t e l e d i a l (Te) rods and the i n t e g r a l block ( B l ) . The l a t t e r i s s i m i l a r
t o t he For t S t Vrain f u e l , while t h e four ones f i r s t mentioned have f u e l
rods independent of t he s t r u c t u r a l g r a p h i t e , as i n the DRAGON and the PEACH
BOTTOM r e a c t o r s . The va r ious f u e l s a r e sketched i n F ig . 1 and t h e i r geome-
t r i c a l c h a r a c t e r i s t i c s a r e given i n Table 1.
674
Table 1. C h a r a c t e r i s t i c s of the va r ious f u e l s considered
Hollow Tubular T r e f o i l T e l e d i a l I n t e g r a l rod rod rod rod block
Fuel compact
Ins ide diameter mm Outside diameter mm
Graphite s leeve
Ins ide diameter of the inne r coolan t channelmm Outside diameter of t he s leeve ( f i n s exc 1uded)mm Length mm
Graphi te block
N r . of rods per block N r . of coolan t channels Channel diameter mm Dimensions ac ross f la tmm Length mm Ng/Nu f o r HML = 1.0 g/cm3
25.4 42 .O
-
52 500
36 18 63.4 377 1,000 236,5
39.5 54.4
29.5
64.4 500
36 18 74.8 422
230 1,000
- 19 .o
-
29 .O 500
108 18 41 .O 37 5 1,000 230
- 11.8
18.6
58.8 500
36 18 67 .O 38 5
270 1,000
12.7
-
- -
210 108 15.9 361 7 93 130
The g raph i t e d e n s i t y was assumed t o be 1.8 g/cm 3 and the moderation
r a t i o was v a r i e d i n the survey by changing t:he heavy metal loading (HML
i . e . t he uranium dens i ty i n the f u e l r eg ion ) from 0.6 t o 1 .4 g/cm (Fig .2) .
E a r l i e r s t u d i e s have shown t h a t f r e e z i n g t h e dimensions f o r a survey l i k e
t h i s i s acceptab le , s ince t h e s i z e ranges l e f t open by o the r design l i m i -
t a t i o n s a r e q u i t e narrow.
For each des ign , an equ iva len t t r i a n g u l a r p i t c h w a s c a l c u l a t e d t ak ing
i n t o account t h e s p e c i a l blocks wi th the c o n t r o l rod channels and the edge
f e a t u r e s i n a l l b locks . The resonance i n t e g r a l ( F i g . 3) was c a l c u l a t e d f o r
such an i d e a l i z e d l a t t i c e . For each f u e l type, the resonance i n t e g r a l
depends, i n decreas ing o rde r , on the heavy metal loading, t he th ickness
of t he f u e l and t h e p i t c h .
v a r i a t i o n of t he parameter i s :
3
A s a guide- l ine , t he s e n s i t i v i t y t o a 10 %
675
2.0 barns f o r t he heavy metal loading
2.0 barns f o r the f u e l s e c t i o n th i ckness
1.5 barn f o r the p i t c h .
The design l i m i t s a r e such t h a t the p i t c h (or block s i z e ) and the f u e l
t h i ckness vary u s u a l l y s imultaneously f o r t h e t u b u l a r , t e l e d i a l and t r e f o i l ;
t he e f f e c t s on the resonance i n t e g r a l a r e then p a r t i a l l y compensating each
o t h e r .
i n t e g r a l cannot be v a r i e d by more than 5 barns between extreme cases
wi th in each type of design, a t a f i x e d heavy metal loading. The approxi-
mation of f r e e z i n g dimensions i s t h e r e f o r e not t oo bad, but c e r t a i n l y worth
n o t i c i n g . It i s ‘of t h e same order of magnitude a s t h e d i f f e r e n c e i n the
va lues of t he resonance i n t e g r a l computed a t d i f f e r e n t p laces on the same
i d e a l i z e d l a t t i c e . Furthermore, a sys temat ic e r r o r might be in t roduced
by the s i m p l i f i e d r ep resen ta t ion , s ince most rods a r e a t a d i s t ance of the
ma jo r i ty of t h e i r neighbours by l e s s than t h e equ iva len t p i t c h . Only when
the r e s u l t s of r e p r e s e n t a t i v e physics experiments w i l l be f u l l y assessed ,
It can be considered f o r a l l p r a c t i c a l purposes t h a t resonance
w i l l i t t h e r e f o r e be the time t o broaden surveys as t h e one descr ibed i n
the present paper and t o inc lude v a r i a t i o n s i n dimensions. The b e n e f i t
of e a r l i e r surveys as t h i s one w i l l have been t o r e s t r i c t t he f i e l d s t o
be considered.
METHODS AND ASSUMPTIONS
The f u e l cyc le c h a r a c t e r i s t i c s were determined us ing t h e methods
o u t l i n e d i n P a r t I . -
The parameters which a r e v a r i e d i n t h e survey a r e the fo l lowing
ones :
- C I U : from 150 t o 300 approximately
- burn-up : 60, 80 and 100 MWd/kg
- power dens i ty : 6 and 8 MW/m except f o r t he hollow rod f o r 3
3 which 4 and 5 MW/m a r e cons idered .
676
A s a l ready mentioned i n P a r t I , the f u e l cyc le c h a r a c t e r i s t i c s a r e
determined f o r an equ i l ib r ium f u e l cyc le , wi th continuous charge-discharge
and no r e a c t i v i t y investment o the r than t h a t needed f o r Xenon over r ide ca-
p a b i l i t y . Two assumptions f o r Xenon ove r r ide c a p a b i l i t i e s a r e considered,
a l lowing power r educ t ions of r e s p e c t i v e l y 100 % and 60 % from nominal
power l e v e l .
The f u e l cyc le cos t i s eva lua ted f o r the equ i l ib r ium f u e l cyc le f o r
two economic con tex t s , d i f f e r i n g e s s e n t i a l l y by the f a b r i c a t i o n cos t and
the plutonium va lue . One contex t i s represen . ta t ive of t he near f u t u r e
s i t u a t i o n s which would be faced by the f i r s t power p l a n t s t o be b u i l t :
the f a b r i c a t i o n c o s t i s h igh because the p l a n t s a r e small and the r e sea rch
and development charges s t i l l s i g n i f i c a n t ; on t h e o the r hand, the plutonium
p r i ce (15 $/g) i s r e p r e s e n t a t i v e of i t s present s c a r c i t y .
The second economic contex t would be more v a l i d from the end of
t he 70 ' s on ; t h e f a b r i c a t i o n cos t i s lower (approximately 50 % of the
former) , because r e sea rch and development charges a r e amortized and
because the f a b r i c a t i o n p l an t has increased i . n s i z e i n order t o serve a
l a rge number of power p l a n t s ; on t h e o ther h.snd, t he plutonium p r i ce
(8 $ /g> has dropped t o i t s va lue f o r r ecyc l ing i n water cooled r e a c t o r s .
The f a b r i c a t i o n c o s t , i nc lud ing the c o s t of uranium l o s s e s and the
i n t e r e s t charges during f a b r i c a t i o n can be ex;?ressed a s :
where k i s the p r i c e of uranium a s UF ($/kg LJ). The c o e f f i c i e n t s A , B
and D a r e given a t Table 2 f o r the four f u e l elements and the two economic
con tex t s considered ( t h e f a b r i c a t i o n cos t i s normalized t o 100 f o r the
tubu la r elements a t 6 % enrichment and C / U = ; !30) .
U 6
. . .. -~ - - - - - - - . . . . . . . . . . .
677
Table 2. Values of A, B and D e3 Fuel element A B D
Hollow rod
Tubular
Te l e d i a l
T r e f o i l
30 1.9 x 0.19
28 1.9 x 0.25
35 1.9 x 0.16
28 1.9 x 0.26
The o the r main economic parameters a r e the fo l lowing ones :
- Plan t load f a c t o r : 0.75
- Uranium ore c o s t : $ 8 l l b U308
- Separa t ive work c o s t : $ 26lkg
- T a i l assay of enrichment p lan t : 0.2 %
- Reprocessing c o s t : $ 60lkg
- I n t e r e s t r a t e : 10 %
- Net e f f i c i e n c y : -41.5 %.
The in f luence of t he pumping power on the n e t p lan t e f f i c i e n c y has
been taken i n t o account f o r each case .
The core pressure drop and t h e pumping power (Table 3) have been
determined on the b a s i s of t he fo l lowing assumptions :
- Reactor he ight : 600 cm
- Power shape f a c t o r : 1.3
- Per fec t gagging of t he coolan t f l u x i n order t o keep the o u t l e t tempe-
r a t u r e c o n s t a n t .
I n f a c t , t h e e f f e c t of t he blower power on the n e t p lan t e f f i c i e n c y
i s r a t h e r small , but of course i t has a l s o an in f luence on the c a p i t a l
c o s t of t he p l a n t , v ia the c o s t of t h e blowers themselves.
678
Table 3. Inf luence of t he design and the power dens i ty on the pumping power
HR Tubular Te led ia l T r e f o i l
Power dens i ty ( ~ ~ / m 3 >
4 5 8 6 8 6 8 6
Rela t ive core 25 39 5 6 100 48 8 4 58 104 pressure drop
Re la t ive pumping 62 7 2 68 100 63 90 68 100 power
A
FUEL CYCLE PERFORMAIXE
E f f e c t of C / U 8
A s expla ined i n Pa r t I, the e f f e c t on the moderation r a t i o i s mainly
descr ibed by the e f f e c t i v e moderation r a t i o , i . e . t he moderation r a t i o
c o r r e c t e d by the a c t u a l resonance i n t e g r a l :
The e f f e c t i v e moderation r a t i o i s p l o t t e d on F i g . 4 ver sus the a c t u a l
moderation r a t i o f o r t he fou r f u e l e lements . One can see t h a t , f o r a same
C / U 8 , t he e f f e c t i v e moderation r a t i o i s s i g n i f i c a n t l y higher f o r the tubu-
l a r and the hollow rods than f o r the t r e f o i l and t e l e d i a l .
For a l l designs the optimum C / U i s around 250 except f o r t ubu la r 8
which opt imizes a t a somewhat lower f i g u r e a!; can be no t i ced a t F ig . 5 and
7 , f o r high and low f a b r i c a t i o n c o s t r e s p e c t i v e l y .
moderation r a t i o f o r t he tubu la r f u e l element exp la ins the d i f f e r e n c e .
The optimum C / U
i s q u i t e understandable , s ince t h e r e i s l e s s i n c e n t i v e t o decrease the
amount of g raph i t e which c o n t r i b u t e s s i g n i f i c a n t l y t o the f a b r i c a t i o n c o s t .
The higher e f f e c t i v e
i s higher f o r t he lower f a b r i c a t i o n cos t e s t ima te which 8
A
679
The in f luence of t h e Xenon ove r r ide requirements can be seen a t
F ig . 6 . Going from 60 t o 100 % c a p a b i l i t y i n c r e a s e s the c o n t r o l l o s s e s
and t h e r e f o r e t h e f u e l cyc le c o s t (h igher inventory c o s t , because of h igher
c r i t i c a l enr ichment , and h igher consumption c o s t , because of lower conver-
s i o n r a t i o ) . The c o s t i nc rease depends e s s e n t i a l l y on t h e r a t i n g which i s
p ropor t iona l t o C/U f o r a given element and power d e n s i t y . For t h e f u l l
Xenon ove r r ide requirements , t h e C/U optimizes t h e r e f o r e a t a lower f i g u r e 8 a s can be seen on the graph f o r hollow rod and tubu la r des igns a t t he h igher
power d e n s i t y . The e f f e c t of Xenon ove r r ide on the t e l e d i a l and t r e f o i l
f u e l e lements i s p r a c t i c a l l y t h e same a s t h a t on tubu la r f u e l e lements a t
equal r a t i n g f i g u r e .
E f f e c t of burn-up
Since t h e moderation r a t i o can be e a s i l y a d j u s t e d v i a t h e heavy meta l
d e n s i t y i n t h e compact, i t would not make sense t o envisage t h e e f f e c t of
burn-up on f u e l cyc le c o s t without acknowledging t h e f a c t t h a t a h igher
burn-up f i g u r e puts a lower emphasis on f a b r i c a t i o n c o s t and hence decreases
t h e i n c e n t i v e f o r low f a b r i c a t i o n c o s t s and low C / U I n p l o t t i n g t h e f u e l
cyc le c o s t s ve r sus burn-up on F ig . 8 we have t h e r e f o r e opt imized C/U
each burn-up f i g u r e . It remains of course t o be checked whether t h e heavy
meta l d e n s i t y corresponding t o t h e o p t i m u m C / U i s not t oo h igh ; b u t , i n
any case , a s m a l l v a r i a t i o n i n C / U
c o s t pena l ty , t h e optimum being very f l a t ; bes ides t h e r e i s s t i l l t h e poss i -
b i l i t y of a d j u s t i n g somewhat t h e f u e l geometry i f t h i s were necessary .
F ig . 8 shows t h a t even f o r l o w f a b r i c a t i o n c o s t , t h e optimum burn-up
f i g u r e i s s t i l l r a t h e r h igh , above 80 MWd/kg and t h i s j u s t i f i e s t h e deve-
lopment of a f u e l element capable of wi ths tanding such burn-ups. Of course ,
f o r t h e h igher f a b r i c a t i o n c o s t e s t i m a t e , t he optimum burn-up f i g u r e i s
s t i l l h ighe r .
8 ' f o r 8
8 (and HML) would not e n t a i l a s i g n i f i c a n t 8
680
The f u e l cyc le c o s t v a r i a t i o n f o r a l l f u e l elements i s very s i m i l a r ,
except f o r the hollow rod which opt imizes a t a s l i g h t l y lower burn-up
f i g u r e . The Xenon over r ide requirement has p r a c t i c a l l y no e f f e c t on the
optimum burn-up f i g u r e .
E f f e c t of power dens i ty
The e f f e c t of power d e n s i t y on t h e v a r i a t i o n s of f u e l cyc le c o s t wi th
C/U i s shown a t F ig . 9 f o r t h e hollow rod and the tubu la r f u e l elements
f o r two burn-up f i g u r e s and f o r 60 % Xenon ove r r ide requirement . The
inf luence of power dens i ty i s p r a c t i c a l l y the same f o r the t e l e d i a l ,
when the a c t u a l Gating i s taken i n t o account..
8
The most obvious inf luence of t he r a t i n g i s on inventory cos t
( i n t e r e s t charges on the f u e l t i e d up i n t h e r e a c t o r ) which decreases
when the power d e n s i t y i n c r e a s e s . However, a s a t u r a t i o n e f f e c t develops,
due t o the inc rease i n c r i t i c a l enrichment, as t h e amount of r e a c t i v i t y
t i e d up i n Xenon ove r r ide requirement i n c r e a s e s wi th t h e r a t i n g .
The l a t t e r e f f e c t has a l s o a de t r imen ta l i n f luence on the conversion
r a t i o and consequent ly on consumption charges which tend t o inc rease wi th
i n c r e a s i n g power d e n s i t y .
The above e f f e c t s exp la in the behaviour of t he curves on F i g . 9 :
t h e f u e l cyc le c o s t i s normally higher f o r t he lower power dens i ty but
t he gap narrows as the C / U
f i g u r e , such a s 60 GWd/t, t he d i f f e rence can even be r eve r sed f o r h igh
C / U because the c r i t i c a l enrichment i s lower and consequent ly , the incen-
t i v e f o r h igh power dens i ty l e s s than f o r 80 GWd/t burn-up.
and the f u e l rat:ing go up. For a low burn-up 8
8
The curves on F ig . 9 were p l o t t e d f o r 60 % Xenon ove r r ide requirement
and the higher f u e l f a b r i c a t i o n c o s t e s t i m a t e . F u l l Xenon ove r r ide requi -
rement and lower f a b r i c a t i o n c o s t would agajin lower the incen t ive f o r high
power dens i ty .
681
APPROACH TO EQUILIBRIUM
A s mentioned above, t he parametr ic f u e l cyc le c o s t s t u d i e s do not t ake
i n t o account the a c t u a l i n i t i a l c o s t and t h e approach t o equ i l ib r ium which
can extend over a long per iod i n r e a c t o r where the f u e l res idence time can
be of t he order of 5 years a t equ i l ib r ium.
I n the frame of t h i s s tudy , i t was not poss ib le t o c a r r y an approach
t o equ i l ib r ium study f o r a l l t he c a s e s cons idered . We s h a l l only i n d i c a t e
t h e range of e r r o r which i s caused by t h i s approximation by g iv ing a nume-
r i c a l example where a d e t a i l e d approach t o equ i l ib r ium a n a l y s i s has been
c a r r i e d out ; t he example r e f e r s t o a case wi th a long f u e l res idence time
a t equi l ibr ium.
I n f a c t , t w o e r r o r s a r e involved i n t h i s approximation, one being
made on the f i s s i l e m a t e r i a l components and t h e o the r on t h e f a b r i c a t i o n
and r ep rocess ing c o s t components.
The equ i l ib r ium f u e l cyc le c o s t normally overes t imates the f i s s i l e
m a t e r i a l component because i t a p p l i e s immediately the i n t e r e s t charges on
the equ i l ib r ium core inventory , which i s normally a t a much h igher enr ich-
ment than t h e f i r s t core ; indeed, t h i s f i r s t core has no f i s s i o n product
poisoning and i s normally designed f o r a l i m i t e d burn-up. A l s o t he f i s s i l e
m a t e r i a l consumption i s overest imated, because the equ i l ib r ium conversion
r a t i o i s decreased by f i s s i o n product poisoning. I n the case considered
the f i s s i l e m a t e r i a l component i s overest imated by 9.5 %.
On the con t r a ry , t he equ i l ib r ium f u e l cyc le c o s t underes t imates the
f a b r i c a t i o n and reprocess ing c o s t s components because i t does not account
f o r t he p a r t i a l burn-up of t he f i r s t and probably a l s o the second co re .
I n t h i s p a r t i c u l a r ca se , t h e equ i l ib r ium f u e l cyc le c o s t underest imates
t h i s component by 25 %. The abso lu te magnitude of t h i s e r r o r depends on
t h a t of the f a b r i c a t i o n and reprocess ing c o s t s .
682
Through p a r t i a l compensations of t h e s e two kinds of e r r o r s , t h e e q u i l i b r i u
f u e l cyc le c o s t underes t imates the a c t u a l f u e l cyc le cos t by 10 % f o r t he
h igher f a b r i c a t i o n cos t e s t ima te and 5.5 ”!, fo r the lower e s t ima te ( f o r t h i s
c a l c u l a t i o n t h e plutonium p r i ce w a s kept equal t o $ 8 / g i n both c a s e s ) .
GENERATING COST
To be complete, we should f i n a l l y o u t l i n e the in f luence of the power
dens i ty on the c a p i t a l c o s t of t he p l a n t s . A member company of INTER
NUCLEAR i s i n v e s t i g a t i n g t h i s problem i n d e t a i l and DRAGON has a l s o made
an a n a l y s i s f o r hollow rod and t e l e d i a l f u e l e lements .
being reasonable and coherent , t h e d a t a u t i l i z e d by DRAGON f o r pub l i ca t ion
w i l l be u t i l i z e d as a r e fe rence ; i . e . , t he c a p i t a l c o s t of the p lan t
i n c r e a s e s by 2 t o 3 $/kWe i n s t a l l e d when the power dens i ty i s decreased
from 8 t o 6 MW/m
decreased from 5 t o 4 MW/m f o r t h e hollow rod .
The f i n a l r e s u l t s
3 f o r t he t e l e d i a l and by 4 t o 5 $/kWe when it i s 3
Taking t h e s e da t a i n t o account , and t h e in f luence of power dens i ty
on f u e l cyc le c o s t (F ig . 91, one ob ta ins t h e t o t a l genera t ing cos t
(F ig . 10) of hollow rod and tubu la r des ign . The curves f o r t he hollow rod
a t 5 W/m3 t ake a l s o i n t o account a c a p i t a l c o s t pena l ty due t o a power
d e n s i t y lower than t h a t of t he t u b u l a r e lements .
COMPARISON OF VARIOUS DESIGNS
Tables 4 and 5 summarize the d a t a on f u e l cyc le and genera t ing cos t
i s s u e d from t h i s s tudy and t ak ing i n t o account the des ign l i m i t a t i o n s
o u t l i n e d i n another paper . The f i r s t conc lus ion i s t h a t a l l t h e designs
a r e w i t h i n a q u i t e narrow band. The r e l a t i v e in f luence of t he f a b r i c a t i o n
c o s t and the Xenon ove r r ide requirement i s a l s o very s imilar . The r e l a t i v e
in f luence of t h e power dens i ty i s a l s o q u i t e the same i n a l l des igns ,
except t he hollow rod which p resen t s a h igher s e n s i t i v i t y t o downrating.
1
683
F a b r i c a t i o n c o s t s
Table 4 . Re la t ive f u e l cyc le c o s t
h igh low
% Xe ove r r ide 60 100 60 100
4
5 HR
I
33
32
8
3 4
33
32 33 27 28
27 27
26 26
6
8 Te
6 Tu
32 33 26 27
31 32 25 27
8
F a b r i c a t i o n c o s t s
% Xe over r ide
high low
60 100 60 100
32 33 26 27
31 3 2 25 26
8
6
8
6
8
T r
Te
I I
99 100 93 94
10 2 10 2 95 96
100 101 94 96
100 10 1 9 4 95
99 99 93 9 4
6 T r 33 3 4 27 28
Table 5. Re la t ive genera t ing cos t
4 HR
104 10 5 98 98
10 2 102 96 96 5 I Tu 6 100 10 1 95 95
684
The i n t e g r a l block (Bl) i s not f u l l y assessed ; i t s main advantage
l a y s i n the reduct ion of t he f a b r i c a t i o n cost:.
The t e l e d i a l s u f f e r s from the d i f f i c u l t y of concent ra t ing enough f u e l
i n t o a block ; t h i s leads t o a h igh resonance i n t e g r a l and higher en r i ch -
ments and hence an age f a c t o r prevent ing t o go t o t he optimum ; t he
r e s u l t a n t higher s e n s i t i v i t y of t he p r i c e of enr iched uranium i s undoubtly
a l s o a disadvantage, i n regard t o the unce r t a in ty of f u t u r e evo lu t ion of
t he market. The design could t h e r e f o r e b e n e f i t from manufacturing techni -
ques enabl ing t o inc rease the heavy metal ; some conso l ida t ion processes
mentioned i n a companion paper a r e appl ical i le f o r t h i s purpose, a f u r t h e r
b e n e f i t being the r educ t ion of t he manufacturing c o s t s .
2
The m a i n disadvantage of the t r e f o i l i s h igh f a b r i c a t i o n c o s t , r e l a -
t i v e t o t h e h igh d e n s i t y f u e l s .
The tubu la r p re sen t s i t s optimum a t lower moderating r a t i o ' s than
obta inable by the c u r r e n t f a b r i c a t i o n techniques . Fur ther developments
lead ing t o f u e l s wi th a higher heavy metal loading o r burn-up c a p a b i l i t y
would s t i l l favour the economic incen t ive of t h i s f u e l .
ThE hollow rod p resen t s the gene ra l advantage of the low r a t e d e l e -
ments : lower s e n s i t i v i t y t o t h e Xenon over r ide requirements , smaller s h i f t
of the optimum moderation r a t i o wi th f u e l f a b r i c a t i o n c o s t , e t c . . . On the
o ther hand, t h e genera t ing c o s t i s over 3 % higher than the o the r elements
and t h e p o s s i b i l i t i e s t o improve the economics a r e smal l , s ince the present
l i m i t s on moderation r a t i o ' s and burn-ups a r e near t he optimum f o r t h i s
f u e l . Furthermore, the low r a t i n g adds the highest running-in per iod
penal ty t o the c o s t s mentioned i n Table 5.
REFERENCES
1. D . J . Merret t and M. Gaube, Choice of f u e l design f o r homogeneous l o w enr iched HTR, Paper presented a t t he present Symposium (Session V, h 1 2 6 ) .
2. L. Aer t s e t a l . , Fuel development f o r a low enr iched HTR, Paper presented a t t he present Symposium (Session V, P.124). 8
HOLLOW ROD TREFOIL
TUBULAR TE LEOIAL
Fig . 1. Reference cases cons idered .
686
c/U(
LO I
300
200 3 9 U/cm H ML
F i g . 2 . Re la t ion between the heavy metal loading and the moderation r a t i o f o r t he r e fe rence c a s e s .
687
1 gU/cm 3
HML
F i g . 3 . Resonance i n t e g r a l s f o r v a r i o u s t y p e s of f u e l s .
F i g . 4 . R e l a t i o n between t h e e f f e c t i v e moderation r a t i o , t h e f u e l r a t i n g and t h e moderat ion r a t i o .
FC . COST
1.3
1.2
1.1
1.0
0.9
BURN UP 80 M W j l k g
POWER DENSITY e MW lm3
( 5 MW/ rn3 FOR HOLLOW ROD 1
. Tr
HOLLOW ROD ---- HR
TUBULAR Tu
TELEDIAL __-. Te
TREFOIL . ........ Tr
FC . cos1
1.3
1.2
1.1
1.0
0.9
BURN UP 80 M W j l k g
POWER DENSITY 8 MW ld ( 5 M W l m 3 FOR HOLLOW ROD 1
Tu
/ HR
/ Tu 1’ / 1’ HR
\
HOLLOW ROD --- HR 60% Xe OVERRIDE
- - - HR 100% k OVERRIDE
- Tu 60V. Xe OVERRIDE
- Tu 100% Xe OVERRIDE
TUBULAR
150 200 2 5 0 300 clue
F i g . 5 . R e l a t i v e f u e l c y c l e c o s t v e r s u s C / U 8 f o r h ighe r f a b r i c a t i o n c o s t e s t i m a t e .
150 200 2 50 300 ClUg
F i g . 6 . f u e l c y c l e c o s t .
In f luence of t h e Xe ove r r ide requi rement on t h e
F.C. COST
BURN U P 80 M W j I k g
POWER DENSITY 8 h4wlrn3
( 5 b4w/rn3 FOR HOLLOW ROD
HOLLOW ROD - --- HR
TUBULAR Tu
T E L E D I A L . To
TREFOIL ........-. Tr
Fig. 7. Relative fuel cycle cost versus C / U ~ for lower fabrication cost estimate.
1.2 NUCLEAIRE cOsTl I
HOLLOW ROD -, , ,. HR
TUBULAR Tu
TELEDIAL . , T o ' I
TREFOIL I . . . . . . . . . Tr
1.0 a HIGHER FABRICATION COST I
b ) LOWER FABRICATION COST
Fig. 8. Relative fuel cycle cost versus bu n- p (C/U8 optimised for each burn-up figure).
F. C . COST
1.2
1.1
1.0
1.2
1.1
/ 6 W / C C
80 M W j / K g
6 0 MWj /Kg ----
5 w / c c ,// LW/CC /’
// / I /
200 250 300
Fig. 9 . In f luence of power d e n s i t y on f u e l c y c l e c o s t f o r hollow rod and t u b u l a r e lements .
1.11
1.0
1.01
0.9!
GENERATING COST
80 M W j I kg
60 *la XENON OVERRIDE
-___/----
TUBULAR 8 W I C C
I* 6 W I C C , FUEL CYCLE COST INCREASE
6 W I CC . ID. + CAPITAL COST INCREASE
HOLLOW ROD 5 W I C C
* - 4 W I C C , FUEL CYCLE COST INCREASE
.’ 4 W I CC. ID + CAPITAL COST INCREASE
I I I I
200 250 300 CIUg
F i g . 10. In f luence of power d e n s i t y of gene ra t ing c o s t f o r hollow rod and t ubu la r e l emen t s .
I
692
R . A . TJ. Huddle: All t h e assessments on t h e t e l e d i a l concept have
been c a r r i e d ou t on simple r e fe rence des ign . Now t h e most important f a c t o r
i n fue l f a b r i c a t i o n c o s t s i s t h e amount of g r a p h i t e work one has t o do
f o r a g iven amount of uranium both f i s s i l e and 238. I f one t a k e s
advantage of t h i s by c u t t i n g ou t some of the unnecessary g raph i t e , t h i s
i n t e rven ing su r face for both f u e l and coo lan t , i . e . t h e so c a l l e d
"frog spawn" modi f ica t ion , then your Nc/Nu r a t i o i s reduced and f a b r i c a -
t i o n c o s t s per u n i t of f u e l a r e reduced s i g n i f i c a n t l y . I be l i eve t h a t ,
if t h e f u e l cycle c o s t s were r eeva lua ted with such an optimized type of
t e l e d i a l element, then i t would show up more f avorab ly than wi th t h e
simple r e fe rence design.
C . Zanantoni: I am not s u r e I understand your ques t ion , however,
t h e f a c t i s t h a t t h e f u e l shape has ve ry l i t t l e a f f e c t on t h e f u e l cyc le
c o s t provided t h e Nc/Nu 238 r a t i o i s t h e sar!ie i f t h e same f a b r i c a t i o n c o s t s
assumptions a r e made f o r t h e va r ious f u e l e lements . In my c a l c u l a t i o n s
I have assumed t h a t t h e f a b r i c a t i o n c o s t i s made up of two p a r t s , one
p ropor t iona l t o t h e heavy metal loading and one p ropor t iona l t o t h e
q u a n t i t y of g r a p h i t e .
H. Kramer: The c a l c u l a t i o n s have been made for an onload f u e l i n g
I assume. I expect t h a t t h e c o s t p e n a l t i e s f o r X e ove r r id ing which a r e
small due t o your c a l c u l a t i o n s when decreas:ing power from 60 percent w i l l
be cons ide rab ly h ighe r when power i s decreased t o 40 percent . What
c e r t a i n t y w i l l be s p e c i f i e d f o r HTR p l a n t s ?
C. Zanantoni: I want t o po in t ou t t h a t your 40 percent power and
our 60 percent X e o v e r r i d e a r e t h e same th ing . In t h e nomenclature w e
decided t o adopt t h e p o s s i b i l i t y t o r e s t a r t a f t e r dropping t h e power from
100 percent t o 40 percent , i s what w e c a l l t he 60 percent Xe o v e r r i d e
requirement .
H. B a i r i o t : The c a l c u l a t i o n s were done f o r 60 and 100 percne t X e
ove r r ide requirements . I commented t h a t t h e r e was merely no i n f l u e n c e
of t h e X e ove r r ide requirement on t h e choice of t h e optimum (cu / r a t io ) .
A s could be no t i ced i n t h e F igure 6, t h e r e i s indeed a 3 percent c o s t
pena l ty on t h e f u e l cycle c o s t . This i s d iscussed more i n d e t a i l i n
t h e paper.
69 3
/ \ H . Gutmann: You have poin ted o u t r e l a t i v e l v pronounced i n c e n t i v e " -
looking a t f u e l cycle c o s t on ly t o go from 60 t o 80 Mwd per Te d i scha rge w i n d i c a t i o n . I wonder whether you have taken i n t o account t h e change i n
thermal e f f i c i e n c y due t o h igher age f a c t o r s f o r longer i r r a d i a t i o n ?
C. Zanantoni: Y e s , w e d id . I do n o t t h i n k t h a t t h e d i sc repanc ie s
which may e x i s t between our and your c a l c u l a t i o n s from t h i s po in t of view
can be t h e cause of such d i f f e r e n c e s . The comments by Dr. Merrett a r e
r e l e v a n t t o t h e answer t o t h i s ques t ion . D. J. Merrett: I would l i k e t o comment on t h e op t imiza t ion of f u e l
The opt imiza t ion a t 80,000 MWd/Te i s inf luenced c o s t s wi th f u e l burnup.
by t h e choice of f u e l f a b r i c a t i o n c o s t formulae. The formula chosen
for t h i s e x e r c i s e i s d i f f e r e n t from t h a t used i n t h e U . K . s t u d i e s and
a r r i v e a t a r a t h e r h ighe r optimum than w e would expec t t o f i n d i n t h e
U.K. This i s t h e gene ra l po in t t h a t one would expect t o f i n d d i f f e r e n c e s
between European, U.K. and U.S. market p r i c e s f o r f u e l f a b r i c a t i o n , t hus
making d i r e c t comparison sub jec t t o some d i f f i c u l t y .
C. Zanantoni: We agree completely.
Paper 4/130
COMPARISON OF HTGR FUEL CYCLES FOR LARGE REACTORS ------..",& *, /* -%* m\c"*%-F*- .m"~-~* ---ED.*..--,
R. C. Dahlberg 3
L? '7
h?- ABSTRACT (G/
Minimum fuel cycle costs consistent with design object- ives on power peaking and fast fluence can be achieved in large HTGRs with a fuel cycle defined by a 4 year fuel lifetime, a power density of 8 w/cc, and a C/Th ratio of 250 to 300. This is the basis for current large HTGR design efforts. Recycle of the bred U-233 will be undertaken as soon as the necessary processing facilities are available.
Plutonium is an attractive makeup fissile material in the HTGR. The use of 300 1-1 fuel particles provides a signi- ficant and beneficial self shielding of the Pu-240 resonances, and the resultant indifference value is about $9.80/gm fissile. Moreover, the fuel cycle cost can benefit from a weakness in the cost of plutonium obtainable on the open market. For example, if plutonium were available at $8/gm fissile, as might be the case based primarily on a LWR market, then the fuel cycle cost using plutonium makeup fuel in the HTGR would be reduced by 0.11 m/kwh over the reference case with U-235 as the feed fuel.
At the present time, the low enrichment cycle for a fuel element design similar to that developed for the Fort St. Vrain HTGR results in net depletion and fuel inventory costs which are .2 to . 3 m/kwh more expensive than in the thorium cycle. uranium cycle are not expected to change this cost disadvantage significantly. optimum economics, but the fuel cycle cost is not critically sensitive to the enrichment.
The HTGR concept as developed by Gulf Genera l Atomic i s based on
t h e thorium-uranium c y c l e . F u l l y e n r i c h e d uranium is used as t h e makeup
f e e d mater ia l and t h e U-233 w i l l b e - r e c y c l e d as soon as p o s s i b l e . The
40 MW(e) Peach Bottom HTGR u t i l i z e s b a t c h l o a d i n g w i t h a 3 y e a r f u e l
l i f e t i m e . I n t h e much l a r g e r 330 MW(e) F o r t S t . V r a i n HTGR, a graded
r e f u e l i n g scheme i s employed i n which one-s ix th of t h e c o r e i s r e f u e l e d
each y e a r : t h e f u e l l i f e t i m e i s s i x y e a r s , and t h e power d e n s i t y i s
about 6 . 3 w / c c .
The f u e l c y c l e f o r t h e 1100 MW(e) HTGRs under c u r r e n t d e s i g n i s
p a t t e r n e d a f t e r t h a t f o r F o r t S t . Vra in . The f u e l l i f e t i m e i s reduced
t o 4 y e a r s , however, w h i l e t h e power d e n s i t y i s i n c r e a s e d t o 8 w / c c ,
somewhat g r e a t e r t h a n t h a t f o r F o r t S t . Vra in . During t h e r e c y c l e mode
of o p e r a t i o n y e a r l y r e c y c l e of a l l of t h e b r e d U-233 i s p lanned .
The power d e n s i t y of about 8 w / c c i n t h e c u r r e n t g e n e r a t i o n of
HTGRs y i e l d s f u e l tempera tures which are n e a r c u r r e n t d e s i g n l i m i t s .
Both t h e f u e l c y c l e c o s t and t h e p l a n t c o s t s are reduced with i n c r e a s e s
i n power d e n s i t y . For example, as shown i n F i g u r e 1, an i n c r e a s e from
6 w / c c t o 8 w / c c f o r t h e same f u e l l i f e t i m e lowers f u e l c y c l e c o s t s by
.05 t o .1 m/kwh.
The f u e l l i f e t i m e of 4 y e a r s r e s u l t s i n a f a s t f l u e n c e t o t h e 2 1 f u e l e lements of about 8 x 10 n v t , n e a r t h e d e s i g n exposure . I f t h e
power d e n s i t y were 6 w / c c , t h e f u e l l i f e t i m e c o u l d , of c o u r s e , b e
i n c r e a s e d w i t h o u t exceeding 8 x 1021 n v t .
were f e a s i b l e , t h e n t h e f u e l c y c l e c o s t would b e a b o u t t h e same as f o r
t h e r e f e r e n c e c y c l e . For a g iven o u t p u t , however, t h e c o r e s i z e would
b e l a r g e r and p l a n t c o s t s would b e g r e a t e r .
t end t o f a v o r t h e h i g h e s t p r a c t i c a b l e power d e n s i t y .
I f a 6 y e a r f u e l l i f e t i m e
Thus, t o t a l power c o s t s
The power peaking " l i m i t " i n d i c a t e d on F i g u r e 1, which d e f i n e s
t h e r e g i o n of most f a v o r a b l e power d i s t r i b u t i o n s , re la tes t o t h e age
696
Pe d i
Fo
ag
by Bo
f i
t h
PO
a
Y i f u
i n
sh
A ,
is
of
!AT
U-
thi
d i
ac
sti
so st
re
shi
i n
Thi
ak ing f a c t o r , t h e d i f f e r e n c e i n l o c a l p o w e r d e n s i t y caused by t h e
s t r i b u t i o n of f u e l of d i f f e r e n t a g e s i n t h e c o r e . Experience w i t h
r t S t . Vra in i n d i c a t e s t h a t an a c c e p t a b l e d e s i g n can b e achieved w i t h
e peaking f a c t o r s of 1 .3 t o 1 . 4 . Age peaking i s a d v e r s e l y a f f e c t e d
both long f u e l l i f e t i m e s and low thorium l o a d s ( o r h i g h C/Th r a t i o s )
t h l e a d t o lower convers ion r a t i o s , l a r g e r f r a c t i o n a l changes i n t h e
s s i le l o a d i n g and t h u s l a r g e r changes i n th12 l o c a l power d e n s i t y o v e r
e f u e l l i f e .
w e r d i s t r i b u t i o n f o r a f u e l l i f e t i m e of 4 y e a r s .
A C/Th r a t i o of about 250 t o 275 g i v e s an a c c e p t a b l e
I n summary, a f u e l c y c l e d e f i n e d by a power d e n s i t y of 8 w / c c and
4 y e a r f u e l l i f e t i m e , w i t h C/Th r a t i o s i n the r a n g e of 250 t o 275,
e l d s minimum f u e l c y c l e c o s t s c o n s i s t e n t w i t h d e s i g n o b j e c t i v e s on e l t e m p e r a t u r e s and f a s t f l u e n c e s . A f o u r y e a r l i f e t i m e a l s o r e s u l t s
a n age d i s t r i b u t i o n i n t h e c o r e which h a s f a v o r a b l e symmetry, as
own i n F i g u r e 2. The f o u r f u e l segments , i d e n t i f i e d by t h e l e t t e r s
B , C , o r D , r e p r e s e n t f u e l of d i f f e r e n t a g e s .
A r e p r o c e s s i n g p o l i c y f o r t h e HTGR i s s h o r t l y expec ted t o be
sued by t h e USAEC. However f o r f o r e i g n a p p l . i c a t i o n s , i n t h e absence
e i t h e r a n e s t a b l i s h e d r e p r o c e s s i n g and r e f a b r i c a t i o n i n d u s t r y f o r
GR t y p e f u e l s , o r government p r o v i s i o n f o r r e p r o c e s s i n g services and
233 buyback, two v a r i a t i o n s on t h e r e f e r e n c e c y c l e have been s t u d i e d :
e s t o r a g e c y c l e and t h e throwaway c y c l e . I n t h e s t o r a g e c y c l e , t h e
scharged f u e l i s s t o r e d i n a n i n t e r i m f a c i l i t y u n t i l enough f u e l h a s
cumulated t o w a r r a n t t h e c o n s t r u c t i o n of a p r o c e s s i n g f a c i l i t y . The
o r a g e t i m e would, of c o u r s e , b e a f u n c t i o n of t h e number of HTGRs
I d , b u t a n 8 y e a r s t o r a g e t i m e h a s been assumed f o r t h e s e comparat ive
u d i e s . I n t h e throwaway c y c l e , t h e d i s c h a r g e d e lements are permanent ly
t i r e d w i t h no r e c y c l e of t h e b r e d f i s s i l e material.
A comparison of t h e r e f e r e n c e c y c l e w i t h t h e s e two v a r i a t i o n s i s
own on Table 1 f o r a 1000 MW(e) HTGR. Delayed r e c y c l e would r e s u l t
a p e n a l t y of about .05 m/kwh i n t h e a v e r a g e 1 2 y e a r f u e l c y c l e c o s t .
e p e n a l t y i s n o t l a r g e r because a f t e r 8 y e a r s t h e accumulated U-233
Figure 1
REFERENCE 1000 MW(e1 HTGR FUEL CYCLE Figure 2
0.04
5 0 . 0 3 I
\ v) J
z - 0 . 0 2
I-- 0.01
W 0
v) 0 V
J V >- " -0.01 -I W
z - 0 . 0 2 W >
- 0 . 0 3 a J w
-0 .04
- 0 . 0 5
CORE C O N F I G U R A T I O N ; R E G I O N & SEGMENT I D E N T I F I C A T I O N
30 YEAR REFLECTOR ZONE
698
would f u r n i s h a l l of t h e f i s s i l e r e q u i r e m e n t s of t h e HTGR f o r 3 more
y e a r s , r e s u l t i n g i n good n e u t r o n i c s and a h i g h convers ion r a t i o . The
d e p l e t i o n c o s t s a re , as a r e s u l t , low during, t h i s i n t e r i m p e r i o d . The
s t o r a g e c o s t s , w h i l e s m a l l , are n o t n e g l i g i b l e . I n t h e s e comparat ive
c a l c u l a t i o n s , t h e cumula t ive c o s t s a s s o c i a t e d w i t h s p e n t f u e l d i f f e r e d
between t h e r e f e r e n c e and s t o r a g e c y c l e s o n l y i n t h e i n v e n t o r y c o s t s
a s s o c i a t e d w i t h t h e s t o r a g e c y c l e .
The c o s t p e n a l t y f o r a throwaway c y c l e would be minimized w i t h
low m e t a l l o a d i n g s and long f u e l l i f e t i m e s . However, power peaking
c r i te r ia would l i m i t t h e d e g r e e t o which t h i s could b e c a r r i e d o u t
a l t h o u g h v a r i a b l e o r i f i c i n g as i n F o r t S t . Vra in could b e used t o permi t
h i g h e r peaking f a c t o r s t h a n c o n s i d e r e d i n t h i s paper . The c y c l e shown
on Table 1 i s t y p i c a l of t h e throwaway c y c l e , y i e l d i n g a r e l a t i v e l y
u n a t t r a c t i v e f u e l c y c l e c o s t which i s about . 2 1 m/kwh g r e a t e r t h a n f o r
t h e r e f e r e n c e c y c l e . The s p e n t f u e l s h i p p i n g and d i s p o s a l c o s t s f o r
t h e throwaway c y c l e w e r e assumed t o be about $300/element .
PLUTONIUM U T I L I Z A T I O N I N HTGRS
I n J u n e , 1968, t h e Edison E l e c t r i c I n s i i i t u t e and Gulf Genera l
Atomic i n i t i a t e d a j o i n t e f f o r t i n e v a l u a t i n g t h e u s e of plutonium i n
HTGRs. The f i r s t phase of t h a t s t u d y d e a l t w i t h t h e v a l u e of plutonium
as a makeup f e e d material i n H T G R s , and t h e r e s u l t s of t h a t work i n d i -
c a t e d an i n d i f f e r e n c e v a l u e between $9 and $1.1 p e r gram f i s s i l e (Ref. 1).
The r e l a t i v e l y h i g h i n d i f f e r e n c e v a l u e f o r pl-utonium i n HTGRs i s due t o
t h e f o l l o w i n g f a c t o r s :
1) 93% e n r i c h e d U-235 f u e l a t about $l.l/gm would b e r e p l a c e d
by t h e plutonium;
699
200
Table 1. Var i a t ions On U-233 Recycle I n Reference Cycle Reference Delayed Throwaway
Cycle Recycle Cycle
+.23 +.16 +. 16
Fue l l i f e t i m e , yea r s
Power d e n s i t y , w/cc
F r a c t i o n of co re r e f u e l e d each yea r
C/Th r a t i o
Delay i n U-233 r e c y c l e ( a f t e r i n i t i a l o p e r a t i o n ) , yea r s
Mass flows i n equ i l ib r ium c y c l e , kg/yr
Th-232 loaded
U-233 r ecyc led
U-235 r ecyc led
Fresh U-235 loaded
U-233 discharged
U-235 r e t i r e d
R e l a t i v e f u e l cyc le c o s t s , m/kwh
F a b r i c a t i o n
Reprocessing (and s to rage )
Dep le t ion
Working c a p i t a l
T o t a l
250
C/Th R a t i o 300
350
4
8
114
250
3
8200 190
20
340
195
30
0.0
0.0
0.0
0.0
0.0
+.12 +.05 +. 03
+.06 0.0 -.01 (Assumed Reference Case)
+.03 -.03 -.04
4
a 114
250
8
8200a a -
- 580
180a 45
0 .o 0.0
-.01
+.06
+.05
200
250
300
350
C/Th Ra t io
4
a 114
275
-
7400 - -
570 170
45
-.02
-.14 +.47
-.lo +.21
Fue l L i t e t ime , Years
3 4 5
1.17 1.23 1.27
1.21 1.30 1.39
1.25 1.37 1.47
1.28 1.42 1.55
a These d a t a apply t o t h e pseudo equ i l ib r ium cyc le t h a t exists j u s t be fo re r e c y c l e commences. The long term equ i l ib r ium cyc le i s , of cour se , i d e n t i c a l w i th t h a t of t h e r e f e r e n c e cyc le .
Table 2. R e l a t i v e Fuel Cycle Costs With Plutonium Makeup mlkwh
I Fue l L i f e t ime , y e a r s 3 4 5
700
2) t h e problems i n f a b r i c a t i n g plutonium b e a r i n g e lements
should b e somewhat s i m i l a r t o t h o s e expec ted i n f a b r i -
c a t i n g U-233 e l e m e n t s ;
3) t h e use of c o a t e d f u e l p a r t i c l e s p e r m i t s an a d d i t i o n a l
c o n t r o l of t h e a d v e r s e n e u t r o n i c s e f f e c t s of Pu-240; and
4) t h e b e n e f i t s of t h e f a v o r a b l e n u c l e a r p r o p e r t i e s of
U-233 are s t i l l o b t a i n e d .
The plutonium used i n t h e s e v a l u e a n a l y s e s w a s t y p i c a l of t h a t
d i s c h a r g e d i n LWR f u e l exposed t o a n average of 30,000 MWD/MTU, namely:
PU-239 : 57%
PU-240 : 26%
PU-241 : 13%
PU-242 : 4%
The Pu-240 c o n t e n t of t h i s mater ia l i s q u i t e h i g h , and u n l e s s h i g h l y
s e l f s h i e l d e d t h e a b s o r p t i o n resonance a t 1 . 0 5 e v c o n s t i t u t e s a n
u n a c c e p t a b l e n e u t r o n poison . The u s e of coa ted p a r t i c l e s whose k e r n e l s
r a n g e i n d iameter from 100 t o 300 p p r o v i d e s a s i g n i f i c a n t amount of
c o n t r o l l a b l e s e l f s h i e l d i n g . F u r t h e r s h i e l d i n g o c c u r s i n t h e f u e l r o d s
i n which t h e p a r t i c l e s are bonded.
A s w i t h t h e thorium c y c l e , a 4 y e a r f u e l l i f e t i m e a p p e a r s a t t r a c -
t i ve . Some comparat ive d a t a are shown on Table 2 where t h e r e l a t i v e
f u e l c y c l e c o s t i n a n e q u i l i b r i u m c y c l e i s shown as a f u n c t i o n of b o t h
t h e f u e l l i f e t i m e and C/Th r a t i o . 300 p g r a i n s were assumed, b u t t h e
comparat ive d a t a are n o t s e n s i t i v e t o t h a t parameter . The assumed
r e f e r e n c e c y c l e , namely a 4 y e a r f u e l l i f e t i m e w i t h a C/Th r a t i o of
300, h a s a n a c c e p t a b l e age peaking f a c t o r of 1 .37. T h i s i s shown i n
Table 3 i n a m a t r i x of d a t a s imi l a r t o t h a t shown i n Table 2. Somewhat
smaller age peaking f a c t o r s can b e o b t a i n e d i n a 3 y e a r , C/Th=350 c y c l e
a t a small i n c r e a s e i n t h e f u e l c y c l e c o s t . S m a l l r e d u c t i o n s i n f u e l
c y c l e c o s t can b e achieved w i t h f u e l l i f e t i m e s somewhat l o n g e r t h a n
4 y e a r s a n d / o r C/Th r a t i o s g r e a t e r t h a n 300, b u t t h e age peaking f a c t o r
t h e n exceeds t h e d e s i r a b l e range of 1 .3 t o 1.ii.
701
Mass f lows and o t h e r d a t a f o r cyc le s of major i n t e r e s t a r e shown
on Table 4 . F i s s i l e plutonium r e q u i r e n e n t s f o r a 4 year f u e l l i f e t i m e
are about 380 kg/yr . Yearly requirements f o r a 3 year cyc le would be
somewhat l a r g e r . The i n d i f f e r e n c e va lue f o r f i s s i l e plutonium i n t h e
r e f e r e n c e c y c l e i s $9.80/gm f i s s i l e .
a p p r o p r i a t e t o a 100 )I d iameter Pu p a r t i c l e r a t h e r than a 300 LI p a r t i c l e .
On t h e s u r f a c e , t h e use of 100 1 ~ - p a r t i c l e s looks a t t r a c t i v e ; t h e i n d i f f -
e r ence v a l u e i s l a r g e r than i n t h e r e f e r e n c e c y c l e , o r t h e f u e l c o s t i s
lower. However, p o t e n t i a l problems e x i s t wi th end-of-cycle r e a c t i v i t y
requirements .
Also shown on Table 4 are d a t a
With very small g r a i n s and low C/Th r a t i o s a c r i t i c a l end-of-cycle
conf igu ra t ion cannot be achieved. For example, i t i s d i f f i c u l t t o
achieve a c r i t i c a l loading a t end of cyc le i f t h e C/Th i s 200 and t h e
plutonium g r a i n s i z e i s 100 I.I i n diameter o r less. This problem of
i n s u f f i c i e n t r e a c t i v i t y r e s u l t s from t h e s t r o n g p a r a s i t i c cap tu re of
neut rons i n Pu-240. A s t he plutonium f u e l loading i s increased i n an
a t tempt t o add r e a c t i v i t y a t t h e end of t h e r e f u e l i n g i n t e r v a l , t h e
thermal spectrum i s hardened s o as t o f u r t h e r i n c r e a s e neut ron cap tu re
i n t h e Pu-240 resonance. This problem i s much less seve re when t h e 300
micron g r a i n i s used t o reduce t h e Pu-240 resonance cap tu re .
Deple t ion r e a c t i v i t y l o s s e s shown on Table 4 do no t i nc lude t h e
e f f e c t of burnable poisons t h a t might be used i n a complete des ign .
However Pu-240 acts l i k e a burnable poison s i n c e i t i s converted by
neut ron cap tu re i n t o t h e f i s s i l e i s o t o p e Pu-241. The abso rp t ion prob-
a b i l i t y f o r Pu-240 i s much less when t h e l a r g e r 300 micron g r a i n i s
employed, s o t h i s compensating e f f e c t i s reduced, and t h e n e t d e p l e t i o n
decrement of r e a c t i v i t y i s inc reased . The i n c r e a s e i n r equ i r ed plu-
tonium makeup f o r t h e l a r g e r g r a i n s r e s u l t s from t h e f a c t t h a t t h e
f i s s i l e plutonium remaining a t t h e end of t h e r e load i n t e r v a l i s more
sh i e lded i n the l a r g e r g r a i n . Hence, extra f u e l i s r equ i r ed t o y i e l d
a c r i t i c a l conf igu ra t ion a t end-of-cycle. I n t h i s a n a l y s i s a 10%
i n c r e a s e i n t h e r equ i r ed plutonium feed w a s observed, and the i n c r e a s e
i n f u e l cyc le c o s t r e s u l t s p r i m a r i l y from t h i s added investment i n
p 1Etoniurr..
Table 4. Plutonium U t i l i z a t i o n I n HTGRs
Bases: Equilibrium Cycle 4 Year Fuel L i fe t ime Annual Refuel ing
Pu p a r t i c l e diameter , u 300
C/Th r a t i o
Fuel loaded p e r y e a r , kg
Th-232
U-233 ( recyc le )
U-235 ( recyc le )
250 300 (Reference Pu Feed
Cycle)
F i s s i l e Pu 384 388
F i s s i l e Pu d i scha rged pe r y e a r , kg ( r e t i r e d ) 60 4 4
Age peaking f a c t o r 1.30 1.37 AK due t o d e p l e t i o n over y e a r l y
cyc le .042 .048
R e l a t i v e f u e l cyc le c o s t , m/kwh +.05 0.0
I n d i f f e r e n c e v a l u e , $/gm f i s s i l e Pu 9.00 9.80
Table 5. Comparison of Thorium and Uranium Cycles i n HTGRs
Bases: F o r t S t . Vrain Fue l Element Equi l ibr ium Annual Refuel ing Cycle
Separa t ive Work: $26/kg Ore Cost: $8 / lb u308 I n t e r e s t Rate : 10% Pu P r i c e : $9.50/gm f i s s i l e Power Level: 1000 MW(e)
-. inorium Uranium Cycle Cycle
C/Th r a t i o 250 -
C / U r a t i o 500
Fuel l i f e t i m e , yea r s 4 4 Age peaking f a c t o r 1.37 1 .48 Re la t ive f u e l c o s t components
U-235 d e p l e t i o n 0.0 +.04
Pu c r e d i t 0 .O -.06
U-233 c r e d i t 0.0 +.35
Fuel working c a p i t a l 0.0 -. 07
To ta l 0 .0 +. 26
703
I n summary, t h e 300 u g r a i n w a s chosen as t h e r e f e r e n c e Pu f u e l
t o p r o v i d e e x t r a f l e x i b i l i t y i n meet ing r e a c t i v i t y r e q u i r e m e n t s . The
i n d i f f e r e n c e v a l u e f o r f i s s i l l e plutonium i n t h a t c y c l e i s $9.80. F u e l
c y c l e c o s t s are s e n s i t i v e t o t h e f i s s i l e Pu p r i c e ; a r e d u c t i o n of $l/gm
i n t h e v a l u e of f i s s i l e plutonium would r e s u l t i n a r e d u c t i o n of
.06 m/kwh i n t h e f u e l c y c l e c o s t . I f f i s s i l e plutonium w e r e a v a i l a b l e
a t $8/gm f o r example, t h e e q u i l i b r i u m f u e l c y c l e c o s t f o r a n HTGR
u t i l i z i n g makeup plutonium would b e about .11 m/kwh less t h a n t h e com-
p a r a b l e c y c l e u s i n g e n r i c h e d uranium.
THE LOW EtNRICHMENT CYCLE I N THE HTGR
The u s e of t h e low enrichment c y c l e i n t h e HTGR i s b e i n g cont inu-
a l l y r e - e v a l u a t e d even thougf.1 o u r s t u d i e s have c o n s i s t e n t l y shown
p o o r e r economic performance w i t h t h e low enrichment c y c l e t h a n w i t h t h e
thorium c y c l e (Ref. 2 ) . One advantage of t h e uranium c y c l e would be
t h a t s i g n i f i c a n t p o r t i o n s of a n e x i s t i n g r e p r o c e s s i n g i n d u s t r y might b e
u t i l i z e d . A head-end f a c i l i t y des igned f o r HTGR t y p e f u e l would a lways ,
of c o u r s e , b e n e c e s s a r y , and s p e c i a l r e f a b r i c a t i o n f a c i l i t i e s would b e
r e q u i r e d i f t h e plutonium were r e c y c l e d . However, t h e c o s t s of t h e s e
f a c i l i t i e s w o u l d be less t h a n t h o s e r e q u i r e d t o e s t a b l i s h t h e complete
technology and f a c i l i t i e s f o r t h e r e c y c l e of U-233. The p o s s i b i l i t y
e x i s t s , of c o u r s e , t h a t t h e H'CGR cou.Ld b e based i n i t i a l l y on t h e uranium
c y c l e w i t h a subsequent change-over t o t h e thor ium c y c l e a f t e r many
HTGRs w e r e i n o p e r a t i o n . T h e neces,:;aryibase l o a d would t h e n ex i s t t o
w a r r a n t t h e c o n s t r u c t i o n of p r o c e s s i n g Zac i l i t i es f o r t h e thorium c y c l e .
However, t h e use of i n t e r i m s t o r a g e f a c z l i t i e s t o s t o r e t h e f u e l d i s - I
charged from HTGRs o p e r a t i n g on t h e thor ium c y c l e a p p e a r s t o b e a more
a t t r ac t ive way of b u i l d i n g up t h e b a s e iload.
The thorium c y c l e i n t h e HTGE: h a s a number of i n h e r e n t advantages .
The f u e l i n t h e HTGR i s r a t h e r homogeneously d i s t r i b u t e d i n t h e g r a p h i t e
modera tor , as shown i n F i g u r e 3 . The u s e of thorium, w i t h i t s r e l a t i v e l y
FORT ST. V R A l N
FUEL ELEMENT Figure 4
L O W ENRICHMENT CYCLE.ANNUAL R E F U E L I N G
B A S I S : FORT S T . V R A l N F U E L ELEMENT E Q U I L I B R I U M CYCLE
PO l SON
F U E L HOLE D I A M E T E R , I N
0.. 7 4 0 P l TCH /
FUEL HANDLING PICKUP HOLE
-DOWEL P I N 4 - 0 . 0 7 9 2 YR F U E L
4 YR F U E L -
-
- ACCEPTABLE
- POWER
- I N I T I A L ENR l CHMENT
2 5 0 5 0 0 7 5 0
C / U R A T I O
Figure 3
705
@ low ( i n f i n i t e d i l u t i o n ) resonance i n t e g r a l (about 86b) , r e s u l t s i n f i s s i l e
requi rements which are only a few p e r c e n t ( -5%) of t h e heavy m e t a l load-
i n g .
r e q u i r e e i t h e r a much h e a v i e r enr ichment o r a more he te rogeneous l a t t i c e
c o n f i g u r a t i o n t h a n c u r r e n t l y e x i s t s . Hence, one p o t e n t i a l v a l u e of t h e
uranium c y c l e , namely t h e p o s s i b i l i t y of u s i n g r e l a t i v e l y i n e x p e n s i v e
low enrichment uranium, i s d i f f i c u l t t o a c h i e v e i n an HTGR t y p e r e a c t o r .
The use of U-238 w i t h i t s 277b resonance i n t e g r a l would g e n e r a l l y
It h a s p r e v i o u s l y been shown (Ref. 2 ) t h a t f o r a p a r t i c u l a r age
peaking f a c t o r and f u e l l i f e t i m e , t h e r a t i o of f e r t i l e - t o - f i s s i l e absorp-
t i o n s ( c o n v e r s i o n r a t i o ) and t h e f i s s i l e l o a d i n g i s e s s e n t i a l l y f i x e d .
The r e q u i r e d f e r t i l e a b s o r p t i o n r a t e may t h e n b e o b t a i n e d from e i t h e r a
l i g h t U-238 l o a d i n g w i t h a l a r g e e f f e c t i v e resonance i n t e g r a l o r a h e a v i e r
U-238 l o a d i n g w i t h a smaller i n t e g r a l . The c o n s t a n t U-235 l o a d i n g i s
t h e n purchased a t a h i g h e r o r lower enr ichment , r e s p e c t i v e l y . It h a s
been found t h a t o v e r a r e a l i s t i c range of f a b r i c a t i o n c o s t s , t h e expense
of f a b r i c a t i n g t h e h e a v i e r U-238 l o a d i n g s ( p r i m a r i l y p a r t i c l e c o s t s )
e s s e n t i a l l y c a n c e l s t h e s a v i n g s due t o t h e reduced enrichment c h a r g e s .
These g e n e r a l c o n c l u s i o n s d i s c u s s e d i n Reference 2 , have been
r e a f f i r m e d i n more r e c e n t c a l c u l a t i o n s r e p o r t e d i n Reference 3. These
more r e c e n t s t u d i e s of t h e uranium c y c l e have assumed i n one case t h e
unmodified u s e of t h e F o r t S t . Vrain f u e l e lement , shown i n F i g u r e 3, and i n another case a f u e l e lement i n which a much more he te rogeneous
c o n f i g u r a t i o n could b e achieved .
Relative c o s t s assuming a F o r t S t . V r a i n t y p e element are shown
on F i g u r e 4 . Minimum c o s t s are n o t a s s o c i a t e d w i t h minimum enr ichments .
Low enrichment r e q u i r e s s h o r t f u e l L i f e t i m e s and c o r r e s p o n d i n g l y h i g h e r
h a n d l i n g c o s t s . A f o u r y e a r f u e l l i f e t i m e r e s u l t s i n a d e s i g n w i t h
a c c e p t a b l e f a s t f l u e n c e s , and a C / U r a t i o of about 500 l e a d s t o age
peaking f a c t o r s which are a l i t t l e h i g h b u t n e a r l y a c c e p t a b l e . The
enr ichment , however, i s about 12%. Longer f u e l l i f e t i m e s would r e s u l t
i n s t i l l lower f u e l c o s t s , b u t f a s t f l u e n c e s would b e g r e a t e r t h a n
8 x lo2' n v t . A s l i g h t l y d i f f e r e n t uranium l o a d i n g might r e s u l t i n
706
f u r t h e r s m a l l r e d u c t i o n s i n t h e f u e l c y c l e c o s t , b u t t h e C/U=500 p o i n t
i s n e a r t h e minimum. D e p l e t i o n and i n v e n t o r y c o s t s f o r t h i s low e n r i c h -
ment c y c l e are compared witlh t h o s e of t h e r e f e r e n c e thorium c y c l e on
Table 5 . The c o s t of t h e s e components i n an e q u i l i b r i u m c y c l e i s about
.2 t o . 3 m/kwh g r e a t e r f o r t h e low enrichment c y c l e t h a n f o r t h e r e f e r -
ence thorium c y c l e .
d i f f e r e n c e i n f a b r i c a t i o n and p r o c e s s i n g c o s t s which under p r e s e n t eco-
nomic c o n d i t i o n s might f a v o r t h e uranium c y c l e .
T h i s p e n a l t y i s b e l i e v e d t o b e much l a r g e r t h a n t h e
A s a l i m i t i n g case, a f u e l e lement w a s c o n s i d e r e d i n which a v e r y
low resonance i n t e g r a l could b e o b t a i n e d , f o r example, 30 b a r n s . A
f u e l e lement d e s i g n which would g i v e t h i s
t h e r e s u l t s of t h e a n a l y s i s w i l l i n d i c a t e t h e v a l u e of p o t e n t i a l r e s e a r c h
and development e f f o r t s i n t h a t d i r e c t i o n . B e s t r e s u l t s are compared
w i t h d a t a o b t a i n e d w i t h t h e uranium c y c l e i n t h e F o r t St. V r a i n element
on Table 6. The enrichment w a s reduced t o a b s u t 7% and t h e d e p l e t i o n
and i n v e n t o r y components of t h e f u e l c y c l e c o s t were reduced by .08 m/kwh.
The t o t a l uranium r e q u i r e m e n t s have i n c r e a s e d s i g n i f i c a n t l y however; i n
f a c t , t h e y have doubled. The e f f e c t of j u s t t h e i n c r e a s e d p a r t i c l e c o s t s
on t h e f a b r i c a t i o n c o s t would o f f s e t t h e r e d u c t i o n i n f u e l c o s t s shown
on Table 6 . Average p a r t i c l e c o s t s , as r e p o r t e d i n Ref . 2 , are a b o u t
$60/kg metal, and f o r burnups i n t h e r a n g e of 75,000 MWDIMT, t h i s e x t r a
f a b r i c a t e d uranium would add about .06 m/kwh t o t h e f u e l c y c l e c o s t .
r e s u l t w a s n o t deve loped , b u t
Thus, low enrichment f u e l c y c l e c o s t s i n t h e HTGR are v e r y insen-
s i t i v e t o t h e enr ichment of t h e uranium u t i l i - z e d . The u s e of 12%
e n r i c h e d material i n a F o r t S t . V r a i n type el-ement i s as a t t r a c t i v e as
t h e use of 7% e n r i c h e d uranium i n a more he te rogeneous c o n f i g u r a t i o n .
Both, however, are n o t as economic as t h e thorium c y c l e , a t l eas t under
normal ly expec ted c o n d i t i o n s .
707
c
T a b l e 6 . F u e l Cycle Cos ts f o r Advanced Low Enrichment Fuel Element Design
Annual R e f u e l i n g
F o r t S t . V r a i n Advanced F u e l E 1 e m e n t Element Design
C / U r a t i o 500 250
F u e l l i f e t i m e , y e a r s 4 4
I n i t i a l enr ichment .12 .067
F i n a l enr ichment .012 .0048
Pu d i s c h a r g e d , k g / y r 44 38
Conversion r a t i o
Age peaking f a c t o r
Relative f u e l c o s t s , m/kwh
Uranium d e p l e t i o n c o s t
Pu c r e d i t
F u e l working c a p i t a l
S u b t o t a l
.50
1 . 4 8
0.0
0.0
0.0
0.0
.45
1.48
-0.. 05
-0.03
0 . 0
-.08
REFERENCE
1. GA-9652, F i n a l P r o g r e s s Repor t , EEL Study of Plutonium
U t i l i z a t i o n i n t h e HTGR, C . H. George, August 20, 1968.
2 . GA-9010, A l t e r n a t e F u e l Cycles f o r t h e HTGR, P . U. F i s h e r ,
S. J a y e , H. B. S t e w a r t , October 4 , 1968.
3. GA-9715, The U s e of Lower Enrichment Uranium i n t h e HTGR,
B . W. Southworth and D. H. Lee, J r . , t o b e i s s u e d .
708
DISCUSS ION 8 R.A.U. Huddle: We had a j o i n t program w i t h H. B a i r i o t of B e l g o n u c l a i r e
t o d e v e l o p a Plutonium f u e l . The f u e l was a combinat ion of Pu02 i n ca rbon
b l a c k Pu/C r a t i o 1/20--diameter abou t 300 micron w i t h a PyC/SiC/PyC c o a t i n g .
Two complete f u e l r o d s were i r r a d i a t e d i n Dragon--maximum t e m p e r a t u r e
125OOC. t o a burn u p of I t h i n k 93 p e r c e n t . The f u e l behav io r was excel-
l e n t and t h i s i s undoub ted ly o u r pin-up f u e l . J u s t a word of warning--
d o n ' t t r y t o make a (plutonium) c a r b i d e f u e l . There seems t o be a v o l a t i l e
competent i n t h i s sytem. The plutonium j u s t v a n i s h e s .
D. T y t g a t : Could you g i v e some i n f o r m a t i o n on t h e d e s i g n of your
plutonium c o a t e d p a r t i c l e ?
R . C . Dahlberg: Our s t u d i e s have assumed pure Pu02 k e r n e l s r a n g i n g
i n d i a m e t e r from 100 t o 300 mic rons . These can be d i l u t e d w i t h Th-232
a s n e c e s s a r y t o a c h i e v e d e s i r e d f i s s i o n d e n s i t i e s p rov ided t h e kernel.
d i a m e t e r i s a d j u s t e d t o keep t h e p roduc t of t h e PU d e n s i t y i n t h e k e r n e l
and t h e r a d i u s n e a r l y c o n s t a n t . C o a t i n g t h i c k n e s s a r e expec ted t o be
of t h e o r d e r of 150 micron.
D. T y t g a t : Wi th in t h e THTR A s s o c i a t i o n , one i r r a d i a t i o n of
plutonium c o a t e d p a r t i c l e s h a s been performed r e c e n t l y and r e s u l t s w i l l
b e a v a i l a b l e s h o r t l y from KFA. The c a p s u l e c o n t a i n e d t h r e e d i f f e r e n t
t y p e s of k e r n e l s , each hav ing t h e same amount of plutonium b u t w i t h
d i f f e r e n t d i a m e t e r s .
H. Kramer: How does t h e t e m p e r a t u r e c o e f f i c i e n t change when u s i n g
a Fu r e c y c l e i n s t e a d of uranium m a k e u p ? What a r e t h e r e l a t i v e f u e l c y c l e
c o s t s of a U/Th and a 1 o . v e n r i c h e d c y c l e f o r t h e GGA f u e l e lement d e s i g n ?
R . C . Dahlberg: The t e m p e r a t u r e c o e f f i c i e n t i s more n e g a t i v e w i t h
Pu f e e d than w i t h e n r i c h e d uranium f e e d . In t h e U.S., assuming a f u e l
e l emen t geometry of t h e F o r t S t . Vra in t y p e , t h e low en r i chmen t cyc le
a p p e a r s t o be about 0 . 2 m p e r Kwh more e x p e n s i v e than t h e Th-232/U-235
c y c l e .
H. B a i r i o t : A s w a s mentioned by M r . Huddle, w e manufactured a t
M o l d i l u t e d 300 micron Pu o x i d e k e r n e l s ; t h e y were s u b m i t t e d t o t h e
Dragon p r o j e c t f o r i r r a d i a t i o n e x p e r i m e n t s : up t o 1 8 5 O O C . (2OOGWd/t) i n
t h e S t u d v i k r e a c t o r - - u p t o 600 GWd/t ( 1 2 0 O o C . ) i n t h e Dragon r e a c t o r .
7 09
One ba tch of s i m i l a r 500 p k e r n e l s and two ba tches of und i lu t ed k e r n e l s
were manufactured of coa ted p a r t i c l e s of i d e n t i c a l o u t e r d iameters a l s o
a t Mol and i r r a d i a t e d i n t h e ,J;’lich r e a c t o r w i th in a j o i n t program w i t h
WA (as p a r t of t h e THTR p r o j e c t ) ; p o s t - i r r a d i a t i o n work w i l l s t a r t i n
a f e w weeks. Although more demonstrat ion t es t s a r e r equ i r ed , t h e f e a s i -
b i l i t y of such Pu p a r t i c l e s i s n o t ques t ionab le .
C. B. Z i t e k : I n o p e r a t i n g an HTGR i s there a parameter such a s Bor t h a t has t o be m e t . What parameter i s used i n determining t h e accep tab le
peaking f a c t o r l i n e on t h e d r a f t p resented?
R. C. Dahlberg: There i s no B o r i n HTR. The accep tab le peaking
f a c t o r i s based on c a l c u l a t i o n s w i t h due c o n s i d e r a t i o n f o r experimental
d a t a on d e s i r a b l e f u e l tempera tures and f a s t f l u e n c e s . W e w i l l have
thermocouples t o determine power output of re loaded f u e l .
Paper 5/129
ECONOMICS OF RECYCLE IN LWR'S ,_ AND m-ra,rru*---.riam..*..*= HTGRI-S IN THE U.S. *---n.=u-w- ---A--CONSGYTANT~S POINT OF VIEW
Many inves t iga tors in r ecen t yea r s h a v e reported on the economics of re- cyc le of fissile inventor ies bred in thermal conver te rs . '" United S ta t e s plutonium is s e e n a s LWR recyc le fuel in the m i d - 1 9 7 0 ' ~ ~ and the underlying technology supporting the exte sion of the uranium c y c l e to plutonium recyc le is s t ead i ly developing. ' Furthermore I its economic implicat ions a r e under cont inuous *asses smen t .
In the
5
Similar ly , the neutron economy of the advanced thermal converter favored in t h e U . S . , the HTGR h a s led to a s s e s s m e n t s of optimum fuel c y c l e s for th i s s y s t e m under spec i f i ed economic condi t ions and ava i lab i l i ty of enr ichment plant. ' In Europe , with the except ion of the THTR program I HTR fuel c y c l e development h a s in recent years been reoriented towards the s l ight ly-enriched uranium c y c l e , with somewhat l e s s emphas i s a t t he moment on r ecyc le . In the United S t a t e s , t he thorium c y c l e h a s been favored by the American proponent of t h i s s y s t e m , Gulf Genera l A t o m i c , I nc . 7
By the d a t e of commercial r ecyc le of mixed uranium-plutonium f u e l i n water reac tors in t h e U.S. , more than a d e c a d e of operat ing exper ience wi l l h a v e been obtained in l igh t wa te r fue l technology by u t i l i t i e s , equipment s u p p l i e r s , and reprocessors a l i k e . A s y e t , no major U.S. re- ac to r equipment suppl ie r nor independent fuel fabr ica tor h a s announced a cont rac t with a u t i l i ty for re load plutonium fuel in a commercial l igh t water p l an t , even though the inventory va lue of plutonium in the United S t a t e s a lone wi l l reach approximately $100 million by 1975 and upwards of one bi l l ion dol la rs by 1980.
Against t h i s background of the re la t ive ly lep.gthy schedu le of implemen- ta t ion of r ecyc le in l igh t water r eac to r s , t he USAEC and Gulf Genera l A t o m i c a r e in genera l accord on the des i rab i l i ty of r ecyc le in HTGR's a t t he e a r l i e s t p o s s i b l e t i m e c o n s i s t e n t with the development of r ecyc le technology and a suf f ic ien t reprocess ing inventory. 7 r 8 S tudies have been con'ducted of t h e optimum t i m e for cornmencement of r ecyc le of U from operat ing HTGR's, and the further development of the technology required to ach ieve t h i s goa l h a s been reported.
233
A
71 0
711
The ra t iona le for cont inued commercial development of the HTGR in the United S t a t e s m u s t r e s t on the wi l l ingness of the U .S . ut i l i ty industry t o c o m m i t to th i s advanced sys t em (with appropriate commercial contin- genc ie s ) concurrent ly with the cont inued development required in the fue l c y c l e . The required ut i l i ty support during the HTGR development period , we be l ieve , will depend upon t h e ut i l i ty indus t ry ' s a s s e s s m e n t of the near- term, re la t ive ly a s s u r e d competi t ive economic margin of the HTGR, ve r sus competing commercial a l t e rna t ives , such as l igh t water conver te rs with plutonium r e c y c l e , and l a t e r , thermal or fast b reede r s ,
S ince the wa te r reactor is the immediate competit ion for t he HTGR, in th i s paper w e compare t h e HTGR thorium f u e l cyc le with U 2 3 3 r ecyc le and the LWR uranium c y c l e with plutonium recyc le i n a se l f - cons i s t en t manner u t i l i z ing d iscounted c a s h f low eva lua t ion techniques common for th i s pur- p o s e as a b a s i s forcompar json . A t t h e hea r t of the HTGR evalua t ion a r e the economic dependences a s sumed fo r such par t s of the fue l c cle a s fabr ica t ion , shipping , reprocess ing and refabricat ion , bred U 2'3 v a l u e , and so on . s ide rab le judgment as to the r a t e of industry growth (throughput as a func- t ion of t i m e ) , projected costs for commercial p rocess ing p lan ts , and environmental cons t ra in ts on p l an t s i z e a s t h e s e affect ach ievab le lev- els of heavy metal throughput per un i t of cap i t a l i nves t ed . Bases for t h e s e economic cons idera t ions a r e presented . The v i ew of the ut i l i ty in- dus t ry in a n as y e t undemonstrated fuel c y c l e is presented as conserva t ive s i n c e normal market fo rces a r e not as y e t opera t ive .
Se lec t ion of t h e s e da t a fo r the HTGR fuel c y c l e requi res con-
Of equal i n t e r e s t to u t i l i t i es is the cost s t ruc ture or economic character- i za t ion of the en t i re f u e l c y c l e , par t icular ly t h o s e components t ha t pro- spec t ive ly lie within their control . The f u e l c y c l e cost s t ruc ture for the LWR and HTGR is examined in terms of d i f f e rences in the makeup of the d i r ec t and ind i rec t f u e l costs. In addi t ion , we assess the s e n s i t i v i t i e s of both f u e l c y c l e s to ce r t a in va r i ab le s s l ich as plant capac i ty fac tor , va lue of bred fissile inventory r e l a t ive to U235, U 2 3 2 penal ty effects o n refabricat ion costs, and o ther var ia t ions in the r e spec t ive fuel c y - cles. From t h e s e a n a l y s e s t h e HTGR fabricat ion cost t a rge t for a g iven reprocess ing cost is developed for graphi te fbels to a c h i e v e parity wi th current compet ing l ight water commercial nuclear fue l offer ings , as w e view prospec t ive market deve lopments for e a c h sys tem.
11. Economic Assumptions
A . Thorium Cycle
1. Industry Growth c3
712
The USAEC have undertaken a systems analysis of the U.S . electric pawer industry, whereby optimal "mixes" of fossi l , hydro, and nuclear plant can be simulated under various cGnditions of demand and supply in the respective industries (i.e. , fos s i l , nuclear, e tc . ) and for v rious eco- nomic assumptions (discount rate , amortization period , e tc .) . Numerous c a s e s have been examjned to investigate the effects of varying parameters on the relative cumulative capacity (growth) of water reactors and IITGRs in an economy with a f a s t breeder reactor and one without a breeder reactor. The assumptions relate to uranium f u e l c o s t s , fossi l file! cos ts , electrical energy demand , electrical energy cos ts , and timing of the introduction of the breeder. The ana lys i s is based on a linear pro- gramming model used to calculate the minimum cos t of supplying U . S . electrical needs for the next half century (1970-2020) for a variety of pos- s ib le electricity growth patterns. We have taken a s our bas i s for the HTGR (thorium cycle) market penetration t h e Base cIr normative Case (B-1) for L w R s , HTGRs and commercial LMFBRs by 1984 with certain modifications. The modification of the indicated growth of an HTGR economy is based on t h e f o l l o w i n g N U S a s s u m p t i o n s :
8 , 10
a . u308 will continue to be available for several decades a t prices of $7-9 (1970 dol lars) .
b. Fossil fue l c o s t s will r ise slowly over this same period due to SO2 removal cos t s .
c. A base energy demand of 11.9 years doubling t i m e appears reasonable and consis tent with various other projections.
d . A significant investment (several hundreds of millions of dollars) is required to develop a commercial thorium f u e l s industry supporting an HTGR economy of the projected s i ze .
The Base C a s e under the Commission's ana lyses indicates very l i t t le HTGR penetration until 1980-1989, and from the conditions which we believe ap- propriate above , we have inferred that by 19!30 approximately 7 0 , 000 MWe of HTGR capaci ty (cumulative) will be instal led, in l ieu of 136, 000 MWeof MWe of HTGR capacity indicated for the Base Case . l o We believe th i s capacity by this date to be reasonably consis tent with an initial commercial availabil i ty date for an 1100 MWe HTGR in the United States in the 1976- 1977 period, and commitments of two or three 1100 MWe HTGRs per year during the early phase of market penetration, leading to 7-8,000 MWe of installed HTGR capacity by 1980. These l i m i t s in our opinion consti tute an upper bound.
A s a lower l i m i t , we would expect slower development and acceptance of this new concept after an initial commitment to an HTGR for startup in
713
t he 1976-1977 t i m e per iod. Further commitment to the concep t by e l ec t r i c u t i l i t i e s would come a f t e r 1-2 yea r s of s u c c e s s f u l Fort S t . Vrain opera t ion , s a y by mid to late 1 9 7 3 , a t which t i m e further commercial orders for 1100 MWe HTGRs would b e p laced for 1979-1980 s t a r tup .
These cons idera t ions l ead u s to conclude t h a t growth of HTGRs might be a s low as follows:
MWe of Ins ta l led HTGR Capaci ty
Year Incremental
Avg . Low - - 19 7 6-77 1000 1000
Cumulative Avg . Low - -
1000 1000
1978 - - 1000 1000
1979 2000 1000 3000 2000
1980 2 5 0 0 1000 5500 3 0 0 0
19 81 3 0 0 0 2 0 0 0 8 5 0 0 5000
1982 3 0 0 0 1000 11500 6 0 0 0
19 83 3 0 0 0 1000 14500 7 0 0 0
19 84 2000 1000 16500 8 0 0 0
From the a s sumpt ions support ing the mean , l o w , and high e s t ima tes we pro jec t the cumulat ive c a p a c i t i e s of HTGRs presented in Figure 1 and s u m - marized below.
Low High Average -
1976-77 1000 1000 1000
1980 8 0 0 0 6 0 0 0 3000
19 85 - 20000 15000 9 0 0 0
1990 - 7 0 0 0 0 25000 13000
714
For the throughput dependen t fue l c y c l e p r o c e s s e s d i s c u s s e d be low we h a v e a s sumed t h a t ave raqe c a p a c i t i e s a r e l i ke ly to prevail ; i . e . , 25000 MWe of U.S. HTGR c a p a c i t y by 1990.
2 . Fuel Fabricat ion and Refabricat ion
a . HTGR fue l preparat ion costs for t h e a s s u m e d industry size and equi- v a l e n t capac i ty in tonnes /year of heavy metal (uranium and thorium) a r e from the l i t e ra ture7 ,I1:
HTGR Fuel Preparat ion C o s t s
1980 6000 65 10 2 5
1985 15000 160 10 15
1990 25000 265 10 12
b. HTGR fuel fabr ica t ion costs ( inc ludes fue l preparat ion costs and sh ipment to reactor) are:
R e f . 11, Appendix D Year M We M T/yr Fab Refab*
(-E) (S/Kg)
1975 1000 10 40 360 485
19 80 6000 65 240 170 245
19 85 15000 160 600 120 160
1990 25000 2 65 1000 100 135
* Assumes a 30% cost d i f fe ren t ia l on manufacturing costs.
3 . Fue l Shipment7 l1
a . Fresh fue l sh ipment costs to site are :
Year -
715
Refab 0
Before 1980 2.50 8 .0
After 1980 2.20 7 . 0
b .
Year C o s t ($/‘Kg)
1975-1980 I. 7
1980-2000 1.6
Irradiated fue l sh ipment costs from site to p rocess ing f ac i l i t y are:
-
7 ,, 11 4 . Fuel Reprocess ing
Irradiated f u e l r ep rocess ing costs a f t e r 1982 are :
Year M We M T/yr Reprocess ing Cos t* (S/Kg)
1982 9000 - 96 - 120
1985 15000 - 160 95
1990 25000 - 265 N 7 0
2000 25000 - 265 - 7 0
* From Table 7 . 8 of Reference 7 a t a n a s s u m e d f ixed cha rge r a t e of 30%.
5. Bred Fuel Value
The U233 va lue relative to U 235 (par i ty va lue) is b a s e d on t h e re- fabr ica t ion p e n a l t i e s shown under 2 . b . and a n a s s u m e d loading of 20 gm U233 per kilogram of heavy m e t a l .
716
Year Parity Value
Up to 1977 14/12
1977 to 1988 (no recycle) 1 0/12
1988 on 12/12
6. Thorium Cycle C o s t Summary
To recap our choice of the c o s t assumptions for with recycle I w e have:
Reprocessing Year MWe costs -
$/Kg H i
1975 1000 120
1980 6000 120
1985 15000 95
1990 25000 70
2000 25000 70
SpenT Fuel Shipment $/Kg Hi
17
17
16
16
16
* From cost data of WASH-1085 (Re
Fabri-* cation $/Kg Hi
360
170
120
100
100
, 7) and NUS-
the thorium cycle
u233 Refabri- * cation Parity Value $/Kg Hi
-
245
160
135
13 5
10/12
10/12
12/12
12/12
( R e f . 11, with an assumed 30% Fixed Charge Rate and nominal throughput of 10 MTH per 1000 MWe of instal led capaci ty per year (lead and lag times have been ignored for simplicity) in dcdlars per kilogram of heavy metal, ini t ia l .
The heavy metal m a s s ba lances by batch and year were provided by Gulf General Atomic for a n 1100 MWe HTGR. These were found to be reasonably cons is ten t with t h o s e reported ear l ier (Reference 7) for an 1000 MWe HTGR.
B .Uranium Cycle
In developing the costs for t h e uranium-plutonium cycle in the l ight water reactor , we have used generally prevailing and accepted market data for ore I conversion I enrichment, fabrication, shipping and processing c o s t s . Judgment is required however in the valuation of bred fuel (plutonium) with
717
0 t i m e , and in refabrication costs of urania-plutonia fue ls for light water recycle. The bases for our a s ses smen t of each is d iscussed in turn.
1.
2 .
Bred Fuel Value
The plutonium valuatiori is based again upon commercial introduction of the fast breeder in 1984, on fabrication price differentials to be d i scussed , and on plutonium recycle s tudies in light water reactors by General Electric and Westinghouse under the sponsorship of the Edison Electric Insti tute. in which plutonium prices greater than $7-8/gm (fissile) in the mid to late 1970's (developed in the EEI s tudies) were obtained. The greater weight of evidence in our opinion is with the $7-8/gm range, and it is these values that we have used.
An independent study12 has been conducted
Fuel Fabrication and Refabrication
The plutonium fabrication penalty is based on the Commission's assumed uranium cycle (LWR) industry s i z e of 150 ,000 MWe by 1980 and a fabrication penalty derived by BNWL. l3
We therefore have used these non-market cost data for the uranium cycle:
U ra n iu rn Plutonium Plutonium Year - abrication Fabrication Parity Value
($/Kg'f- ($/Kg)
197 5 73 10 0 0 . 6 5
1980 54 70 0 . 7 5
1985 44 57 0.9
1990 40 52 1.0
2000 40 50 1.0
The heavy metal mass balances were developed by NUS from work sponsored by the Edison Electric Insti tute referred to above. We chose to analyze a boiling water reactor burning natural uranium feed with plutonium makeup - which the industrial ana lys t , t h e General Electric Compnay, found to be the optimal mode of plu- tonium recycle for their system. This is not a self sustaining cycle in that the amount of plutonium produced during any one cycle is not sufficient to provide enough recycle fuel to form a complete
718
replacement batch. Four BWRs (or PWRs) provide only enough plutonium for one B W R in this economy. Thus, either more plutonium m u s t be purchased a s makeup material for a complete replacement loading , or else only part of a reload is made up of plutonium bearing fue l assemblies . The cos t structure and sensi t ivi t ies given in the fol- lowing sect ion apply only to the recycle assembl ies , so tha t we have assumed that additional plutonium is available and will be purchased to complete a fu l l replacement loading.
111. Discussion
We have analyzed both the HTGR and LWR fue l costs with recycle using the NUS computer code model , FUELCOST-11. This code calculates the revenue required to amortize entirely each batch of fuel over i t s lifetime, defined a s the t i m e from the f i rs t payment for the batch until the final dollar credit is received from the spent fuel material. T h e s e "batch cos ts ' ' are com- bined in a manner related to when and how rapidly each batch produces en- ergy in order to yield a fue l cost for the reactor. These cos t s are then discounted to yield a "present worthed" or " level ized" f u e l cos t .
We have incorporated the cost information given in Section I1 of this paper into our calculations to yield thirty year levelized fuel costs. We further allowed the cost assumptions to change in order to determine the sensit ivity of the fue l cost of each system to different assumptions about cost compon- e n t s , a s shown in Tables 1 and 2 .
The sources of the heavy metal mass balances were mentioned in Section I1 of this paper. Since they form an important part of the cost ana lyses , we have tabulated typical equilibrium mass balances for each s y s t e m in Table 3 , although in the economic ana lys i s , detailed treatment by batch was resorted to.
Tables 1 and 2 show the cos t structure and c o s t sensi t ivi t ies of each f u e l cycle a s they apply only to these two specif ic f u e l cyc les . cyc le s , such as an HTGR without U235 makeup (such as P ~ ~ 3 9 - u ~ ~ ~ m a k e - up) or a LWR with recycle of only self-produced plutonium, would undoub- tedly yield different resu l t s . We believe however the c a s e we have selected is the more probable U.S. economy for the near term, based on the General Electric ana lyses .
Other fue l
For the particular fuel cyc les analyzed , we conclude the following:
1. The effect of capaci ty factor on fuel costs is essent ia l ly identical between the two systems. Therefore, neither system shows a cost advantage over the other i n a reas of the world in which the
719
2.
3 .
4.
future plant capacity factor may be quite uncertain. An example of such a situation is one in which a nuclear plant is being inte- grated into a predominantly hydroelectric system, and the nuclear plant is not intended to be base-loaded.
For equal total fuel c o s t s , the HTGR has higher direct c o s t s , which could have certain advantages in the U. S. accounting treatment of nuclear fuel. For example, a utility might choose to finance a larger portion of the HTGR fuel c o s t s through low cost debt financing than is the case with LWR fuel, while at the s a m e t i m e expanding the rate base.
The process costs contribute equally to the fuel cost of each system. One interpretation of th i s result is that each system can benefit equally from economics of scale and from competition which will develop in the process industries.
The uncertainty i n LWR fuel cos t s for a given percentage uncer- tainty in bred fuel value is several t i m e s that for a n HTGR.
We should point out that the fuel cos t s for the LWR economy we have chosen are very dependent on plutonium prices. We have postulated a situation in which the plutonium is produced by other LWR's so that pluto- nium prices would in fact be related to uranium prices. The LWR would exhibit a sensit ivity to U 3 0 8 cos t as a resul t through plutonium purchases. We have not shown th is effect directly in Table 2 , although qualitatively one would expect the resulting sensit ivity to ore price to be greater for the LWR than for the HTGR under these circumstances. We have a l so not considered the l ikely reoptimization of the respective m a s s balances for either the HTGR or LWR which would probably ensue from future higher U 3 0 8 costs and lower fabrication costs.
IV. Summary and Conclusions
In summary, we have analyzed two specific examples out of many possible modes of recycle. We conclude that the balance between depletion costs, process costs and indirect cos t s shows that each system displays different cos t sensit ivit ies. Depending on specific commercial circumstances, either system might show the lowest overall fuel cost or the least sensi t i - vity to uncertainties in a n evaluated result.
A s a final point, we have estimated what the process costs must be in order for the HTGR fuel costs to be equal t o the LWR fuel costs. The HTGR fabrication cost required for parity with LWR fuel offerings is in the range of 250-300 $/Kg H (heavy metal) for a n assumed reprocessing cost of 70 $/Kg H (typical o:E a - 2 5 , 0 0 0 MWe HTGR fue l processing
720
economy). a n d p rocess ing costs wi th h e a v y metal throughput , we conclude that par i ty wi th LWR fue l wi th recycle will be approached wi th a n HTGR indus t ry size of be tween 1 0 , 0 0 0 a n d 1 5 , 0 0 0 MWe, a s suming t h a t p r i ces do not reflect t h e development costs of t h e thorium fue l cycle.
On t h e basis of d a t a i n t h i s paper o n graphi te fue l fabr ica t ion @
REFERENCES
1.
2 .
3 .
4.
5 .
6.
7 .
8 .
9 .
10.
11.
12 .
13.
Symposium on Economics of Nuclear F u e l s , Got twaldov, May 1968, IAEA Proceedings S e r i e s , 1968.
Technical S e s s i o n 2 , In te rna t iona l Nuclear Indus t r ies Fa i r , (NUCLEX 6 9 ) , Basel, 1969.
Symposium on Plutonium a s a Reactor Fue l , Brusse l s , March 1967, IAEA Proceedings Series, 1967.
Proceedings of t h e Plutonium Fue l s Technology Conference , AIME , April 1968.
Pr ivate Communicat ion, Edison Elec t r ic I n s t i t u t e , S t a tus of Plu- tonium Ut i l iza t ion S tudy , February 1969
Symposium o n Advanced a n d High Temperature Gas-Cooled Reac to r s , Ju l i ch , October 1968, IAEA Proceedings S e r i e s , 1969.
U.S. Atomic Energy Commiss ion , An Evaluation of t h e High Tempera- ture Gas-Cooled Reac tor , USAEC Report WASH-1085, July 1969.
Gulf Gene ra l A t o m i c , I n c . , Nat iona l HTGR Recycle Development Pro- gram P lan , May 1969 (to b e i s s u e d ) .
Deonigi , D. E. , 'I Simulat ion of t h e U . S . Power Economy, "Proceedings of t h e American Power Confe rence , Vol . , 3 2 , 1970.
U. S. A t o m i c Energy Commiss ion , Potent ia l Nuclear Power Growth Pat- t e r n s , USAEC Report WASH-1098 (to b e i s s u e d ) .
USAEC Report , Guide for Economic Evalua.tion of Nuclear Reactor P lan t D e s i g n s , NUS-531, January 1969.
Dawson , F .G . , et a l , Resul t s from USAE:C Plutonium Ut i l iza t ion Pro- grams Conducted by BNWL, IAEA Panel on Plutonium Ut i l iza t ion , September 2-6 , 1968.
Keenan, J . D . , Goldsmi th , S . , D e H a l a s , D.R. , Fabricat ion a n d Ir- rad ia t ion Fac tors Inf luencing Plutonium Recycle Economics, BNWL- SA-1079, January , 1967.
HIGH
I I
CALENDAR YEAR
FIGURE 1 ESTIMATES OF CUMULATIVE INSTALLED HTGR CAPACITY (1984 COMMERCIAL INTRODUCTION OF FBR)
TABLE 1
COST STRUCTURE AT EQUILIBRIUIL~~ RECYCLE PERCENT
DEPLETION COSTS, DIRECT
U - 235 Depletion
Pu Depletion
U - 233 Depletion
SUBTOTAL
PROCESS COSTS, DIRECT
Fabrication
Spent Fuel Shipping end
Refirocessing
SUBTOTAL
!NDIRECT CDSTS
ATEN PERCENT UNCERTAINTY IN:
1. $/lb U308
T A B L E 2
COST SENSIT IV IT IES IN RECYCLE
YIELDSTHE FOLLOWING PERCENl UNCERTAINTY I N FUEL COSTS: HTGR LWR 3.0 1.0
2. $/SWU 3.9 -
3. $/gm of bred fuel value 1.6 6.6
4. $/Kg recovery cost (shipping plus reprocessing 0.5 0.6
Metal Loading
T A B L E 3
ASSUMED E Q U I L I B R I U M HEAVY M E T A L MASS B A L A N C E S
1100 MWe HTG R
9900 Kg
U-235 Loading
U-233 Loading
400 Kg
210 Kg
5. Capacity factor 2.9 2.9 Fissile Pu Loading -
6. Fabrication cost 2.8 1.8
Metal Oischarge 9000 Kg
1. Interest rate 3.1 4.6
U-233 Discharged for Recycle 210 Kg
U-235 Discharged for Recycle 30 Kg
Fissile Pu Discharged for Recycle
Burnup, MWD/MTU
-
85,000
1100 MWe LWR*
33,600 Kg
Natural U
il (\3 Iu 1000 Kg
32,500 Kg
0.32 (wgt. %)
640 Kg
27,500
GECR - 5566 Plutonium Utilization in Boiling Water Reactors - Phase I Final Report, work preformed for the Edison Electric Institute
723
DISCUSSION
R . S . Car l smi th : I t should be poin ted out t h a t t h e pene t r a t ion of
H T G R ' s i n t o t h e U.S. market i n t h e AEC s t u d i e s (WASH-1126) i s n o t given
a s a s i n g l e e s t ima te . Severa l e s t i m a t e s were given - some of them lower
than t h e one by t h i s speaker . D o your e s t i m a t e s inc lude t h e e f f e c t of
a " learn ing curve" o r f i r s t -o f - a -k ind c o s t s f o r H T G R ' s i n comparison wi th
t h e e s t a b l i s h e d LWR i n d u s t r y ?
J. C . Scarborough: We have not included t h e e f f e c t of a l e a r n i n g
curve i n our p r o j e c t i o n s , s: ince i t i s no t c l e a r t o us how i n t h e e a r l y
years of HTGR development and commercial a c t i v i t y p r i c i n g w i l l r e l a t e t o
f u r t h e r manufacturing knowledge. I n t h e LWR indus t ry , t h e " learn ing
curve" appears t o have g e n e r a l l y brough h igher p r i c e s , a s Mr. P h i l l i p
Sporn has r e c e n t l y brought o u t .
H. B. S tewar t : Your market p r o j e c t i o n f o r t h e HTGR must be based
on some l i m i t a t i o n such a s t h e i n t r o d u c t i o n d a t e of f a s t b reeder r e a c t o r s .
Can you t e l l u s what you assumed i n t h i s r e s p e c t ?
J. C. Scarborough: Our market p r o j e c t i o n i s based on c e r t a i n modi-
f i c a t i o n s of assumptions employed i n t h e USAEC Base Case a n a l y s i s ; how-
eve r , t h e assumption of commercial i n t r o d u c t i o n of t h e LMFBR i n 1984 w a s
r e t a i n e d . I t i s acknowledges, and t h e s e same USAEC s t u d i e s have shown,
t h a t a s i g n i f i c a n t i n c r e a s e i n cumulat ive HTGR c a p a c i t y may occur i f t h e
1984 r e fe rence LMFBR commercial i n t r o d u c t i o n d a t e i s delayed by s e v e r a l
years . We would a l s o expec t o t h e r commercial arrangements t o be r equ i r ed
i n t h e United S t a t e s , such a s t h e l i c e n s i n g of o t h e r equipment s u p p l i e r s ,
t o support t h e H E R i n d u s t r y size of our more o p t i m i s t i c range of e s t i m a t e s .
R . C. Dahlberg: I assume from t h e l a s t s l i d e t h a t t h e s e n s i t i v i t y
of t h e f u e l c y c l e c o s t t o changes i n o r e c o s t i s much less f o r t h e LWR
than t h e HTGR because i t was assumed t h a t plutonium from many LWR's was
used t o supply t h e f i s s i l e requirements f o r t h e LWR under ques t ion r a t h e r
than simply r e c y c l i n g i n a r e a c t o r t h e plutonium bred i n t h a t r e a c t o r .
Is t h a t c o r r e c t ?
J. C. Scarborough: Y e s , t h e General Electr ic s tudy i n d i c a t e d t h a t 3
t o 4 B W R ' s would provide t h e makeup f eed f o r another comparably s i z e d BWR. @ - H. B. S tewar t : Our c a l c u l a t i o n s , and I t h i n k those of o t h e r s , have
c o n s i s t e n t l y shown t h a t t h e HTGR f u e l c y c l e c , o s t i s much l e s s s e n s i t i v e
t o U 0 c o s t s than t h e LWR. I t h i n k i t i s important t h a t people r e a l i z e
t h a t t h e U 0 s e n s i t i v i t y you have shown i n your t a b l e i s a h igh ly
unusual ca se where t h e f u e l i s predominantly plutonium. D o you wish t o
comment ?
3 8
3 8
J . C . Scarborough: We acknowledge the f a c t t h a t t h e sub jec t of
HTGR f u e l cycle c o s t s e n s i t i v i t y has been e x t e n s i v e l y analyzed and t h a t
HTGR f u e l cycle c o s t i s much less s e n s i t i v e t o U 0 c o s t s than the LWR
without r ecyc le , o r w i t h only self-produced r ecyc le . W e a r e n o t prepared
t o say t h a t t h e case w e have examined i s h igh ly unusual however. Indeed,
if t h e i n d i c a t e d mode of recycle i n a BWR i s i n f a c t s u b s t a n t i a l l y more
a t t r a c t i v e a s t h e General E lec t r i c s tudy sugges ts , than a reasonable case
can be made t h a t t h i s mode would p r e v a i l over the nea r term i n t h e United
S t a t e s .
3 8
P.U. F i sche r : In your comparison of t h e economics of r e c y c l e i n
LWR's and H T G R ' s you have assumed a c e r t a i n range range f o r t h e HTGR
market pene t r a t ion . S ince i t t a k e s s e v e r a l L W R ' s t o produce t h e plutonium
requ i r ed f o r a recycle LWR t h e r e w i l l be a l i m i t e d market f o r plutonium
recyc le . D o you have a f e e l i n g f o r t h e s i z e of t h i s market?
J , C . Scarborough: The plutonium market a s r ecyc le f u e l f o r thermal
conve r t e r s , of course , depends on t h e de facxo commercial i n t r o d u c t i o n of
f a s t b reeder r e a c t o r s , or t h e i n d u s t r y d iscount of t h i s da t e . W e b e l i e v e
t h a t t h e annual market f o r r ecyc le plutonium could range up t o 50 MT
through 1985, though t h i s assumption i s n o t n e c e s s a r i l y c o n s i s t e n t w i t h
t h e scheduled LMFBR commercial i n t r o d u c t i o n d a t e of 1984.
H. Kramer: I would l i k e t o confirm t h e comment of Dr. Stewar t ; due
t o our c a l c u l a t i o n s f o r u sua l f u l l c y c l e s t h e s e n s i t i v i t y of H e HTR i s
less s e n s i t i v e t o i n c r e a s e s i n o r e p r i c e s (by a f a c t o r of 3 ) . Which
mechanisms a r e under ly ing your c a l c u l a t i o n s f o r p r e d i c t i n g t h e market
p e n e t r a t i o n s of the HTR?
J . C. Scarborough: The bases were those assumed by t h e USAEC i n
WASH-1098, P o t e n t i a l Nuclear Power Growth P a t t e r n s , a s modified by t h e f o u r assumptions c i t e d i n our paper. Chief among these i s t h a t low o re
prices (less than $9/lb. unesca la t ed ) w i l l p r e v a i l u n t i l about t h e 1990
t i m e per iod . The more r ecen t uranium exp lo ra to ry d r i l l i n g r e s u l t s upon
725
which our judgement on t h i s po in t i s based were n o t g e n e r a l l y a v a i l a b l e
a s an i n t e r p r e t e d r e s u l t a t t h e t i m e t he ana lyses r epor t ed i n WASH-1098
were performed a f e w years ago. The remainder of t h e a n a l y s i s i s economic;
t he t e c h n i c a l design bases suppor t ing t h e r e s p e c t i v e mass ba lances for
the two systems analyzed have been g e n e r a l l y confirmed by o t h e r work.
6d
C. Zanantoni: What were the assumptions concerning t h e p l a n t c o s t
f o r t h e two t y p e s of r e a c t o r s ?
J. C. Scarborough: Our paper was concerned only w i t h f u e l cyc le c o s t s
a s opposed t o power genera t ion c o s t s , which inc lude deprec i ab le c a p i t a l
p l an t and o t h e r ope ra t ing c o s t s . Es t imates have been made of HTGR and
LWR power gene ra t ion c o s t s by the USAEC (Reference 71, and an eva lua t ion
of commercial t ende r s which inc lude an HTGR and s e v e r a l l i g h t water
r e a c t o r s i n the P a c i f i c Northwest of t h e United S t a t e s should be a v a i l a b l e
i n t h e summer, 1970.
R. S . Car l smi th : In connect ion w i t h s e n s i t i v i t y t o changes i n o re
p r i c e s i t i s perhaps worth reemphasizing t h a t t h e f u e l c o s t s f o r t h e BWR
t h a t was chosen w i l l be very dependent on Pu p r i c e s . I f one i s p o s t u l a t i n g
a s i t u a t i o n i n which the PU i s being produced by o t h e r LWR's; then Pu
prices would be c l o s e l y t i e d t o uranium prices, and t h e BWR would show
an a d d i t i o n a l s e n s i t i v i t y t o U 0 c o s t through i t s purchase of Pu. If
on t h e o t h e r hand, one wishes t o cons ide r a s i t u a t i o n i n which excess PU i s being produced by LMFBR's; then the Pu pr ice would no t rise, and
t h e HTGR's would c e r t a i n l y s h i f t t o a Pu-makeup cycle t o avoid buying high-
c o s t uranium.
3 8
The f i rs t of those c a s e s i s probably of most i n t e r e s t . ORNL c a l c u l a -
t i o n s have been made concerning t h e s e n s i t i v i t y of HTGR and BWR f u e l cnsts
t o a 10% i n c r e a s e i n U 0 c o s t wi th t h e Pu p r i c e maintained a t a p a r i t y
of 1.0 t o 235U p r i c e . Under t h e s e assumptions w e f i n d 6.6% i n c r e a s e i n
BWR f u e l c o s t compared t o a 2.6% i n c r e a s e i n H E R c o s t . A 10% i n c r e a s e
i n s e p a r a t i v e work c o s t would cause a 4.2% i n c r e a s e i n BWR f u e l c o s t (due
t o inc reased PU va lue a s 235U p r i c e i n c r e a s e s ) , compared w i t h a 4.4%
i n c r e a s e f o r t h e HTGR. These c a l c u l a t i o n s were based on t h e NUS mass
ba lances and economic assumptions a s w e l l a s could be determined. Thus
t h e y s t i l l do not t ake i n t o ;account any r eop t imiza t ion of t h e f u e l cyc le .
3 8
Paper 6/134
PARAMETRIC SPRVEY -0NJY-EL-CCyCLES AND TOTAL "GENERATING ,,C-OSTS FOR HTR's WITH HOLLOW ROD, TELEDIAL ANDwTUBULARvTf'Kl?ERACTING FUEL ELEMENTS
- 4 t- .1 0 0
H. Gutmann, J. Daub, J. Pedersen, H. Schober (3&3 OECD Dragon P ro jec t >
D C. Rinaldini, G. Grazial-ii >:fB ! Q
8 ) % /
,-I Euratom I s p r a
J. Journet, J. Malherbe I , a- Commissariat a 1 'Energie A t c l m i q u e
P-
ABS TRACT
Tota l Generating Costs and Fuel Cycle Costs are given f o r Low Enriched Homogeneous Design HTR' s with Hollow Rod and Teled ia l prismatic Fuel Elements which are t h e types considered f o r t he f irst l a rge HTR s t a t i o n s t o be b u i l t i n Europe. the Tubular In t e rac t ing concept which r equ i r e s more extensive proof t e s t i n g before it can be introduced has been inves t iga ted f o r both low enriched and thorium/highly enriched f u e l cycles. The designs are inves t iga t ed with r e spec t t o t h e manufacturing and design l i m i t s a t present recommended by Dragon on heavy metal loading, f a s t neutron dose, surface and f u e l temperature limits. The design assessments are made f o r var ious power d e n s i t i e s on t h e b a s i s of un i r rad ia ted f u e l geometries f o r varying f u e l temperature limits. Supplementary s t u d i e s relate these r e s u l t s t o t h e worst hea t t ransfer condition during i r r a d i a t i o n and include systematic and random e r r o r assessments. t o t a l e l e c t r i c i t y generating c o s t s inc lude present ly real is t ic f u e l f a b r i c a t i o n and c a p i t a l c o s t estimates se lec ted according t o t h e p r inc ip l e t h a t only t echn ica l and economic considerations determine t h e choice of contractors.
A:; a more advanced design,
The
INTRODUCTION
The task of surveying r e a c t o r s with t h e purpose of recommending
an optimum reference design o r choosing between d i f f e r e n t design
concepts makes it necessary t o combine f u e l cycle ca l cu la t ions with
t h e corresponding h e a t t r a n s f e r and c a p i t a l cos t assessments.
Furthermore i t i s essent ia l f o r t h e usefulness of such a survey t h a t
i t t akes i n t o account t h e material and engineering design limits so
t h a t , where necessary, t h e survey cases can be optimised t o t h e l i m i t
726
727
and t h e optimum cases of each f e a s i b i l i t y a rea can be out l ined .
The f u e l cyc les are, the re fo re , shown a s a cons t i t uen t p a r t of
t h e interwoven system of physics , h e a t t r a n s f e r , engineer ing,
material and cost considerat ions. The optimum designs are found as
minimum t o t a l generat ing c o s t p o i n t s wi th in t h e areas of t echn ica l
f e a s i b i l i t y . It has been made c l e a r how these areas and t h e optimum
designs would be a f fec ted by changes i n the permissible f a s t neutron
dose, f u e l temperature, and achievable heavy metal dens i ty ,
The paper concerns i tself mainly with low enriched f u e l cyc les
f o r t he th ree pr i smat ic f u e l element design types a t p resent under
cons idera t ion i n Europe, t h a t i s , Hollow Rod, Te led ia l and Tubular
In t e rac t ing . For the l a t te r t h e low enriched f u e l cyc le s a r e
compared with the corresponding segregated thoriwn/highly enriched
uranium cycles.
FUEL ELEMElNT AND REACTOR DESIGN DATA
The r ep resen ta t ive f u e l cells of t h e t h r e e f u e l element designs
which w e r e i nves t iga t ed are shown i n Figs. 1 and 2. (Gaps are not
quoted. )
p a r t i c l e s embedded i n a g raph i t e matrix. For t h e l o w enriched
i n v e s t i g a t i o n s standard Dragon p a r t i c l e s w e r e used throughout t he
The fue l i tsel f cons is ted of compacts comprising coated
survey. For the thorium/highly enriched uranium cycles breed
p a r t i c l e s of standard s i z e and feed p a r t i c l e s of a smaller s i z e w e r e
consol idated i n t o t h e same compact. The feed p a r t i c l e s w e r e d i l u t e d
with carbon so t h a t equal gas pressure w a s b u i l t up with i r r a d i a t i o n
i n both types of p a r t i c l e s . During reprocessing of t he compacts t h e
g raph i t e mat r ix and t h e o u t e r coa t ing l a y e r s w e r e d i sso lved
e l e c t r o l y t i c a l l y SO t h a t t h e two types of coated p a r t i c l e s assumed t o
be reduced t o t h e i r s i l i c o n carbide l a y e r s being of d i f f e r e n t s i z e
could be separated by s iev ing techniques. The f u e l material d a t a and
coated p a r t i c l e dimensions are given i n T a b l e 1.
The reactor w a s a homogeneous pr i smat ic design with one stand
pipe serving f o r t h e charging .and discharging of f o u r ad jacent f u e l
Table 2. Reactor Data Table 1. Fuel and Fuel Element Design Data f o r t h e Homogeneous HTR
Standard P a r t i c l e s (breed p a r t i c l e s i n case of thorium cycles )
Design type
Coated p a r t i c l e diameter ~1,100 pm
Coating thickness ~ 1 5 0 pm
Kernel mater ia l : Low enriched cycles: u02
Thorium cycles: Tho /UO
Feed Par t ic les (only f o r thorium cycles )
Coated p a r t i c l e diameter
Coating th ickness
Kernel material
c800 pm
3150 pm
UO + carbon 2
Triangular p i t c h of f u e l channel lat t ice: Hollow Rod 90 nun
Te led ia l 95 nun
Tubular 95 nun
Number of f u e l channels per f u e l block 18 ~~~~
Outer diameter of ou ter cooling channel: Hollow Rod 63 nun
Te led ia l 68 nun
Tubular 68 nun
Cooling medium
Moderator mater ia l
Fue 1
Core height/diameter r a t i o
Pressure i n the primary c i r c u i t
A x i a l power form f a c t o r
Radial power form f a c t o r (power f l a t t e n e d )
Direct ion of cooling flow
Cooling of f u e l pins: Teledial and Tubular
Hollow Rod
Cooling gas core i n l e t temperature
Cooling gas core o u t l e t temperature
Cooling gas reac tor o u t l e t temperature
Gas mass flow i n core
G a s m a s s flow i n r e a c t o r
Gross e l e c t r i c a l output per r e a c t o r
Thermal output per r e a c t o r
E l e c t r i c i t y generation
Loading scheme
Xenon overr ide
a Homogeneous HTR with pr ismatic f u e l elements
H e l i u m
Graphite
Compacted coated p a r t i c l e s
0.615
56 atm
1.2
1.2
Downwards
I n t e r n a l l y and External ly
External ly
30 5OC
785OC
7 5OoC
603.8 kg/s
664.6 kg/s
660 MW(e)
1,535 MW(th)
Via h e a t exchangers and steam turb ines
On-load
For a change from 100% t o 40% load
%omogeneous i s t o be understood i n terms of engineering. The design, however, i s heterogeneous from t h e physics point of view.
729
element s t r inge r s . The r e a c t o r d a t a are given i n T a b l e 2. The core
w a s contained i n a pres t ressed concrete pressure vesse l a l s o housing
s i x pod hea t exchangers.
The design l i m i t s a t present recommended by Dragon are given i n 1 T a b l e 3 . Since t h e hea t conduc t iv i t i e s and the dimensions of the
f u e l compacts and f u e l elements change with i r r a d i a t i o n the design
temperatures had t o be viewed with respec t t o t h e i r limits a t t h e
worst poss ib le poin t i n t i m e .
SURVEY PHILOSOPHY AND COST ASSUMPTIONS
It i s of g r e a t i n t e r e s t t o know how a v a r i a t i o n i n t h e th ree
major design l i m i t s , i.e., t h e ones on t h e f u e l temperature, the f a s t
neutron dose and the heavy metal loading, would effect the optimum
design point.
d i sp lay the survey with r e spec t t o these three var ia t ions .
Great care has the re fo re been taken t o layout and
The survey w a s made i n two par t s . P a r t one consisted of t he L physics ca l cu la t ion with t h e f u e l cycle code MOGA , and t h e hea t
3 t r a n s f e r and cos t ca l cu la t ions with t h e Dragon design code TECO . For each design a range of power d e n s i t i e s and N /N r a t i o s w a s
surveyed f o r un i r rad ia ted f u e l geometries and hea t conduc t iv i t i e s
under varying nominal f u e l temperature l i m i t s and f o r a s p e c i f i c
n o m i n a l surface t e m p e r a t u r e l i m i t e s t i m a t e d t o correspond t o the
value given i n T a b l e 3.
hea t t r a n s f e r ca l cu la t ions with DONKEY,3 and TIGER inves t iga t ing the
systematic and random error:; as w e l l as t h e f u e l and surface tempera-
ture h i s t o r y during i r r a d i a t i o n ,
by a combination of t h e outcome of t h e two p a r t i a l surveys.
C H M
The second p a r t of t he survey consisted of 4 5
The f i n a l r e s u l t s w e r e then obtained
The fue l cycle calculal-ions took i n t o account an opera t iona l
margin of 1% r e a c t i v i t y on top of t h e 40-100% xenon over r ide require-
ment. They w e r e performed on a O-dimensional model. The leakage
terms, however, represented two enrichment cores with a r a d i u s of
0.8 t i m e s t he core r ad ius d iv id ing the inner and outer core zone.
The enrichments yielded from these ca l cu la t ions a r e therefore
730
r ep resen ta t ive of 2-enrichment cores. The age f a c t o r s w e r e deduced
from t h e t i m e dependent f i s s i o n c r o s s sec t ions and disadvantage
f a c t o r s .
Since Hollow Rod and Te led ia l are the designs t h a t can be
introduced earliest, we i nves t iga t ed these concepts only with low
enriched f u e l cycles .
which needs more proof t e s t i n g before it can be introduced, w e
s tud ied a l s o segregated thorium cycles .
I n the case of t he tubu la r i n t e r a c t i n g design,
The low enriched f u e l cyc le s w e r e once-through cases under the
assumption t h a t t he discharged f u e l would be reprocessed and credi ted.
The thorium f u e l cyc le s considered a segregated concept with
U-235 make-up inves ted only i n t h e breed p a r t i c l e s and depleted
make-up a s w e l l as bred U - 2 3 3 from the reprocessed breed p a r t i c l e s
once-through recycled i n the feed p a r t i c l e s .
A l l f u e l cyc le c a l c u l a t i o n s w e r e performed f o r continuously
on-load r e f u e l l e d systems and assumed a f i r s t charge of equilibrium
core composition.
I n t h e h e a t t r a n s f e r c a l c u l a t i o n s r a d i a l power form f a c t o r
gagging and a continuous age f a c t o r gagging f o r equal gas o u t l e t
temperature w e r e appl ied when needed. All cases w e r e blower power
optimised which means t h a t blower power was reduced t o t h e poin t where
e i t h e r t h e f u e l temperature o r t h e surface temperature reached i t s
l i m i t .
Q
The f u l l y gagged cases where a temperature l i m i t w a s a l ready
reached a t f u l l blower power r ep resen t a boundary l i n e of t h e
f e a s i b i l i t y area.
The c o s t assumptions are given i n T a b l e 4. It w a s assumed t h a t
t h e f u e l and t h e enrichment s e rv i ce would be bought on t h e world
market.
t h e nuclear i n d u s t r i e s i n t h e United Kingdom and Continental Europe
have been contacted. Because of the involvement of commercial
i n t e r e s t s d e t a i l s of these cost assumptions cannot be disclosed.
For the assessment of t h e f u e l f a b r i c a t i o n and c a p i t a l c o s t s
731
The contractors w e r e chosen on the bas i s of technical and economic
considerations only.
20,000 MW(e! would be in s t a l l ed during the f irst t en years.
w e r e assessed f o r a s i t ua t ion with several power s t a t ions already on
order .
For the fabr ica t ion costs it was assumed t h a t
The cos ts
It should be mentioned t h a t the fabr ica t ion cos ts f o r the low
enriched f u e l cycles, although 2-enrichment cores w e r e considered,
assumed only one manufacturing l ine. This introduced an e r ror of
-0.02 mills/kWh which does not however influence the r e l a t i v e
comparison between the d i f f e ren t designs.
HEAT TRANSFER ASSUMPTIONS AND UNCERTAINTIES ACCOUNTANCY
To ar r ive a t a t rue c:omparison between the d i f f e ren t cases of
the same o r d i f f e ren t design concepts, w e had t o work with the actual
maximum temperatures.
i r r a d i a t i o n effects as w e l l a s both systematic and random errors.
This meant an involvement i n s tudies of
I n our invest igat ions with the Dragon design code TECO, w e
restricted ourselves t o the idea l core of unirradiated nominal design
specification. The temperatures obtained i n t h i s way w e c a l l nominal
temperatures.
ax i a l power form fac to r s and the age factor .
t h a t are referred t o i n Figs. 7-10.
I n t h e i r maximum values they include the r a d i a l and
It i s these temperatures
A separate study, r e s u l t s of which are shown i n Fig. 11, yielded
the i r r ad ia t ion effect.
correspond t o the m a x i m u m nominal f u e l temperatures brought about
above.
dwelling t i m e .
The temperature values a t zero i r r ad ia t ion
The maximum f u e l temperatures occur a t about 30% of f u e l element
Another study investigated the e r ro r s due t o imperfections of
the actual design. This accounted f o r f u e l eccent r ic i ty , coolant
leakage, heat leakage, gag adjustments, block and pin power t i l t s and
corrosion.
peaks gave the systematic peak temperatures.
6
Adding these systematic e r r o r s t o the above temperature
732
A l a s t study covered t h e random effects. It accounted f o r t h e
v a r i a t i o n of t h e f u e l compact th ickness , in t -e r face gap width, tube
thickness , coolan t annulus dimension, f u e l enrichment, f u e l dens i ty ,
and f u r t h e r f o r p in displacement, thermocouple and recorder e r r o r ,
con t ro l rod effects, etc. These e r r o r s on t o p of t he systematic peak
temperature y ie lded t h e random peak temperatures. It i s the la t ter
t h a t have t o be compared with the given temperature design l i m i t s , t h a t are quoted i n T a b l e 3 o r t h e var ied f u e l temperature l i m i t i n
Figs. 12-15.
FUEL CYCLES PHYSICS RESULTS
The physics r e s u l t s of t h e fue l cycle c:alculations are given i n
Figs. 3-6. Comparing t h e r e s u l t s one not ices , as could be expected,
an inc rease i n the age f a c t o r and enrichment. with increas ing
i r r a d i a t i o n , while t he conversion r a t i o decreases.
The d i f f e r e n t carbon/HM-atom r a t i o s (N /N ) were achieved by c: HM varying t h e heavy metal dens i ty i n t h e f u e l pin.
i nc rease with increas ing N /N
conversion r a t i o .
The age f a c t o r s
values r e f l e c t i n g the decrease of t he C H M
I n t h e range between N /N 200-400, th.e conversion r a t i o of t h e C H M
low enriched cases moves c h a r a c t e r i s t i c a l l y between.0.5 and 0.65 f o r
both i r r a d i a t i o n s while t he enrichment ranges between 4.5% and 6.5%
f o r 60 GWd/t and 6.0% t o 8.0% f o r 80 GWd/t.
I n t h e thorium/highly enriched f u e l cyc les one f i n d s higher
conversion r a t i o s and consequently b e t t e r f u e l u t i l i s a t i o n due t o the
higher q-value of U-233 compared with Pu-239 and t h e b e n e f i t of t he
segregated once-through r ecyc le f u e l management.
have, on t h e o the r hand, t he disadvantage of higher age f a c t o r s s ince
t h e U-233 f i s s i o n c r o s s sec t ion i s smaller than the one of Pu-239.
The thorium cycles
HOLLOW ROD AND TELEDIAL COST RESULTS
The t o t a l generat ing c o s t s from t h e survey on t h e un i r r ad ia t ed
f u e l geometries are given i n Figs. 7 and 8. Each of t hese figures i s
ac tua l ly a superimposit ion of a manifold of figures because d i f f e r e n t A
7 3 3
@ nominal f u e l temperature l i m i t s determine d i f f e r e n t cost-landscapes,
each with i t s own full-gagging l i n e which l i m i t s i t s f e a s i b i l i t y area.
Below t h i s boundary i s the f e a s i b l e design a rea of p a r t i a l gagging.
All t hese full-gagging l i n e s f o r d i f f e r e n t nominal f u e l tempera-
ture l i m i t s now appear f o r each design on one and t h e same f i g u r e
because w e have found that. t h e c o s t s i n t h e regions of i n t e r e s t vary
so l i t t l e With t h e f u e l temperature l i m i t s ince the surface temperature
f o r c e s one i n a l l cases t o work near full-gagging. W e have, therefore ,
f o r t h e sake of a much simpler d i sp lay , been able t o superimpose t h e
var ious "cost-scapes" without introducing an e r r o r g r e a t e r than 0.003 mills/kWh.
Each f e a s i b i l i t y a rea i s determined by t h e full-gagging l i n e 3
as mentioned above, and e i t h e r t he manufacturing l i m i t of 1 g/cm
heavy metal o r t h e fas t neutron dose l i m i t of 4 x 1021 EDN which are
a l s o given i n these graphs.
develop,the design f e a s i b i . l i t y area w i l l grow towards higher f u e l
temperature l i m i t s , higher f a s t neutron doses and higher heavy metal
loadings. However, as can be seen from these f igu res , t h e c o s t optima
are already included i n t h e present f e a s i b i l i t y areas as f a r a s f a s t
neutron dose and heavy metal loading are concerned, SO t h a t real c o s t
improvements can be expected only by t h e easing of t h e f u e l temperature l i m i t . T h i s i s e spec ia l ly t r u e fo r the Hollow R o d design w h i c h i s
apparently much more inf r inged by t h i s l i m i t than t h e Teled ia l design.
A s ma te r i a l s and manufacturing processes
All optimum cases occur a t full-gagging and t u r n ou t with Nc/NU
r a t i o s between 200-300.
r e s u l t s with r e su l t s from t h e Consortia t h a t t hese optimum Nc/NU values
are overestimated by approldmately 10-20 due t o our survey running-in
assumption as compared with t h e outcome of proper running-in s tud ies .
W e expect from previous comparisons of o ld
Comparing t h e Hollow Rod and Te led ia l design one sees t h a t t h e
l a t te r , due t o i t s add i t iona l hea t t r a n s f e r surface i n t h e inner
cooling channel, i s less l imi ted on t h e f u e l temperature and f o r t h a t
reason allows f o r much higher power d e n s i t i e s , z 9 MW/m
to t h e < 5 MW/m f o r t h e Hollow Rod.
3 as compared 3
734
Another s i g n i f i c a n t d i f f e rence between the Hollow Rod and t h e
Te led ia l becomes apparent when one s t u d i e s the temperature behaviour
with i r r a d i a t i o n as given i n Fig. 11.
t h e Hollow Rod a t 4 MW/m
t he same. Due t o the l a r g e r dimension of a Hollow Rod f u e l annulus
compared with one of t he e i g h t Te led ia l Fuel. s t i c k s it develops a
l a r g e r gap between f u e l compact and g raph i t e s leeve which r e s u l t s i n a
higher i nc rease of t h e f u e l temperature up t.o a maximum with
i r r a d i a t i o n . The worst po in t i n t i m e i s reached after approximately
30% i r r a d i a t i o n , and t h i s determines t h e r e d design r e s t r i c t i o n due
t o t h e f u e l temperature l i m i t .
The f 'uel temperature curve f o r 3 and t h e Te led ia l a t 9 MW/m3 are roughly
The optimum t o t a l generat ing c o s t s are obtained by combining t h e
r e s u l t s i n Figs. 7 and 8, with those i n Fig. 11 including systematic
and random e r ro r s . They are shown i n Fig. 1.2, while Fig. 13 conta ins
the corresponding f u e l cyc le cos ts .
f u e l temperature l i m i t s t h e core power dens i ty being a curve parameter.
With inc reas ing f u e l temperature l i m i t t h e c D s t curves f o r p a r t i c u l a r
power d e n s i t i e s decrease u n t i l they reach t h e i r t o t a l generat ing cost
m i n i m u m .
The cos.ts are p lo t t ed f o r var ious
From t h e r e on the curves are f l a t because f u r t h e r i nc reases i n
the f u e l temperature l i m i t cannot be u t i l i s e d as w e have already
reached t h e optimum N /N
e f f i c i ency due t o the r e s t r i c t i o n on the sur face temperature.
value and nothing can be gained i n c u
The envelopes of t he ind iv idua l curves are t h e real o v e r a l l
optimum r e s u l t s showing how, i n the case of more and more s t r i n g e n t
f u e l temperature l i m i t s , it pays t o go t o lower power dens i t i e s . W e
have cut-off our Te led ia l i n v e s t i g a t i o n s a t a power dens i ty of
9 MW/m , as w e th ink t h a t above t h i s power dens i ty t h e thermal shut
down stresses across t h e f u e l p in might beco.me too high.
corresponding cut-off f o r t h e Hollow Rod, where t h e hea t from t h e
f u e l p in only flows i n one d i r e c t i o n , was chosen a t 6 MW/m . This
however, would already require fue l temperakure l i m i t s i n excess
of 1450 C where w e have cut-off our figures.
3
The
3
0
735
I n t h e case of t h e Hollow Rod t h e cases with 80 GWd/t show no
t o t a l generating c o s t advantage over t h e ones with 60 GWd/t, and f o r
t h e Teled ia l , t h e c o s t reduction i s not very pronounced. S ign i f i can t ,
however, i s t h e cos t advantage of t he Teled ia l over t he Hollow Rod,
which becomes more and more pronounced t h e f u r t h e r one i s r e s t r i c t e d
on t h e f u e l temperature. To be fa i r , though, w e have t o admit t h a t t he chosen Hollow Rod design cannot claim t o be f u l l y optimised.
ins tance , w e have not included a v a r i a t i o n of t h e p i t c h i n t h i s
survey. However, w e have reason t o be l i eve t h a t t he chosen Hollow
Rod cannot be far from an o v e r a l l optimised design.
could never c lose the s u b s t a n t i a l c o s t gap t o the Teled ia l design of
about 0.2 mills/kWh a t t h e recommended f u e l temperature l i m i t of
135OOC.
For
I n any case it
A comparison of t h e f u e l cycle c o s t s i n Fig. 12 with the t o t a l
generating c o s t i n Fig. 11 shows t h a t t h e former account f o r
approximately 35% of t h e t o t a l costs.
TUBULAR INTERACTING COST RESULTS FOR LOW ENRICHED AND THORIUM/HIGHLY ENRICHED FUEL CYCLES
These s tud ie s d id not cover t h e whole power dens i ty range as the 3 previous inves t iga t ions , b u t w e r e r e s t r i c t e d t o 7 and 9 MW/m .
f u r t h e r has t o be mentioned t h a t t he thorium re su l t s do not have t h e same degree of accuracy as the low enriched ones. This is due t o a
less accurate age f a c t o r assessment and higher uncertaint ies i n t h e
It
f u e l f a b r i c a t i o n costs.
The t o t a l generating c o s t s vs. N /Nm are given i n Figs. 9 and 10. C
The f u e l temperature l i m i t does not pu t a very s t r i n g e n t condition on
t h i s design and it i s more t h e surface temperature t h a t i s l imi t ing on
the temperature side.
However, s ince w e regard t h i s a s a design f o r t h e f u t u r e and
because w e th ink t h a t by then t h e philosophy regarding t h e sur face
temperature l i m i t might have changed, w e have allowed f o r excesses of
the a t present recommended l i m i t of 1050 C by up t o ~ 6 0 C. 0 0
736
The thorium cycle c o s t s i n Fig. IO show a cut-off i n t h e f e a s i b l e
design area which i s determined by t h e manufacturing l i m i t a t 35%
packing f r a c t i o n and t h e assumed r e s t r i c t i o n t o t h e same build-up of
f i s s i o n product pressure per u n i t volume void i n t h e kernel a s i n the
corresponding low enriched case. Though t h i s assumption i s somewhat
of an a r b i t r a r y nature, t h e r e w i l l be a r e s t r i c t i o n of a s i m i l a r
kind and i n fu ture w e simply have t o l e a r n more about it.
The optimum t o t a l generating c o s t s f o r various a c t u a l fue l
temperature limits are given i n Fig. 14, f o r both t h e low enriched
and t h e thorium cycles, while t he corresponding f u e l cycle c o s t s are
shown i n Fig. 15.
Comparing t h e low enriched Tubular I n t e r a c t i n g r e su l t s of Fig. 14
w i t h the T e l e d i a l r e s u l t s of Fig. 12 a t the .same p o w e r d e n s i t i e s one
f i n d s r a t h e r comparable t o t a l generating costs. However, it has t o
be mentioned t h a t while our Teledia l f u e l pili can be regarded as c lose
t o t h e optimum design, our Tubular design could s t i l l be optimised by
going t o lower p i t ches and consequently lower power outputs per f u e l
pin. This i s present ly under inves t iga t ion .
COMPARISON OF REFERENCE OPTIPWM CASES
The design and physics d a t a f o r fou r reference optimum cases of
our survey are compiled i n T a b l e 5.
cost breakdowns. All re ference cases have been chosen f o r t h e same
discharge i r r a d i a t i o n of 60 GWd/t, and t h e recommended f u e l temperature
l i m i t of 135OOC.
Table 6 conta ins the corresponding
The comparison of t h e peak random temperatures i n T a b l e 5 c l e a r l y
shows t h a t t h e Hollow Rod case i s l imi ted on t h e f u e l temperature with
a peak random surface temperature w e l l below i t s recommended l i m i t of
105OOC.
l imi ted on t h e surface temperature, though w e have allowed our
reference cases t o exceed t h i s l i m i t .
I n c o n t r a s t t h e Te led ia l and Tubular In t e rac t ing cases are
The thermal r a t i n g v a r i e s considerably from t h e Hollow Rod t o t h e
o ther low enriched cases which i s r e f l e c t e d i n t h e xenon over r ide
737
0 l o s ses i n t h e neutron balance. The resonances are most shielded i n t h e
case of t h e Hollow Rod r e s u l t i n g i n a lower feed enrichment as w e l l as
a higher m a x i m u m age f a c t o r and f i f a value.
Due t o t h e i r similar resonance sh ie ld ing and equal power density
t h e low enriched Teled ia l and Tubular In t e rac t ing C a s e s t u r n O u t with
t h e same cos t s , T a b l e 6. I n con t r a s t , t h e Hollow Rod, due t o i t s
lower power dens i ty and high c a p i t a l c o s t s i s more expensive by
Z O . 2 mills/kWh.
The thorium case, compared with the low enriched case, has t h e
advantage of a higher f i f a and conversion r a t i o requi r ing only
2.6 wt.% U-235 make-up per heavy metal loaded, T a b l e 5. It suffers,
however, from higher age f a c t o r s and f a b r i c a t i o n c o s t s and g e t s less
f iss i le discharge c red i t . I t s real r e s t r i c t i o n , however, i s t h e
l i m i t a t i o n i n t h e packing f r a c t i o n which has been discussed i n t he
previous section. Under the present set of assumptions t h e optimum
thorium Tubular In t e rac t ing case i s 0.04 mills/kWh cheaper than t h e
corresponding low enriched re ference case. Learning more about t he
above l i m i t s w e f ee l t h a t w e could ob ta in a thorium reference case
with somewhat cheaper costs.
FINAL DISCUSSION AND CONCLUSIONS
A l l t o t a l generating c o s t s m i n i m a are found t o be within the fas t
neutron dose and f u e l dens i ty manufacturing l i m i t a t present recommended.
The optimum heavy metal dens i ty for low enriched f u e l cycles i s approxi-
mately 0.8 g/HM cm3 f o r t h e Hollow Rod design, 0.9 f o r t h e Teled ia l and
0.65 f o r t h e Tubular I n t e r a c t i n g concept. This shows t h a t t h e
Hollow Rod and Tubular designs are more relaxed with r e spec t t o heavy
m e t a l loading requirements than t h e Teled ia l concept. The running-in
assumption of t he survey i s expected t o overestimate t h e optimum Nc/NU
r a t i o by approximately 10-20 as compared with a study where t h e
running-in period would have been properly taken i n t o account. This
means t h a t such inves t iga t ions would recommend heavy metal d e n s i t i e s
t h a t are approximately 0 .1 g/cm3 higher than t h e ones quoted i n t h i s
paper, bringing t h e Teled ia l up t o t h e present manufacturing l i m i t
738
while f o r the Hollow Rod and even more so for t h e Tubular In t e rac t ing
design a comfortable margin would s t i l l remain.
The Hollow Rod design i s t h e most s e n s i t i v e t o t h e f u e l tempera-
ture r e s t r i c t i o n than t h e o the r designs.
t o higher power d e n s i t i e s and r e s u l t s i n a c o s t penal ty of
w 0 . 2 mills/kWh a s compared with t h e Te led ia l design.
regard our Hollow Rod design as f u l l y optimised, we th ink w e are near
enough t o the optimum t o exclude t h a t t h e very pronounced c o s t
disadvantage could be considerably reduced.
This prevents one from going
Though w e cannot
It i s obvious from the r e s u l t s t h a t t h e Hollow Rod design due t o
i t s r e s t r i c t i o n on t h e f u e l temperature s ide could never be used i n
conjunct ion with gas tu rb ines , where w e need high gas o u t l e t - i n l e t
temperatures . The Tubular I n t e r a c t i n g design i s less restricted on t h e heavy
metal loading s i d e than t h e Te led ia l design and less r e s t r i c t e d on the
f u e l temperature s ide than t h e Hollow Rod design. I n these r e s p e c t s
it combines t h e b e s t of both concepts;
temperature, however, it i s more restricted. I n the present survey,
the Te led ia l and Tubular optima have e f f e c t i v e l y t h e same costs. This
i s , however, due t o t h e fac t t h a t t h e chosen Tubular design has not
been f u l l y optimised.
with r e s p e c t t o t h e sur face
The segregated thorium f u e l cyc les , i nves t iga t ed only f o r t he
Tubular I n t e r a c t i n g design, show, a t t h e optimum, a s m a l l t o t a l
generat ing advantage of approximately 0.04 mills/kWh over the
corresponding l o w enriched case. This outcome is , however,
determined by our f e a s i b i l i t y assumptions.
A l l c o s t landscapes show f l a t c o s t m i n i m a vs. heavy metal d-ensity,
which l eaves t h e designer a comfortable margin f o r t he f i n a l choice
of t h e re ference point.
For some designs t h e cost incen t ive of going f r o m 60 t o 80 GWd/t
i r r a d i a t i o n i s not pronounced.
t h i s kind it the re fo re seems advisable t o choose the l o w e r i r r a d i a t i o n
For t h e f irst power p l a n t s of
739
because t h i s would mean a considerable r e l a x a t i o n of t h e fas t neutron
dose requirements and would c u t down t h e i r r a d i a t i o n requi red i n t h e
f u e l and f u e l element tests t h a t have t o be completed before t h e
concept i s accepted.
W e have inves t iga ted cases with f u l l and p a r t i a l gagging and
have found t h a t t h e cos t optima f o r a l l cases inves t iga ted occur a t
full-gagging.
Due t o t h e higher power d e n s i t i e s t h a t can be achieved with t h e
Teled ia l and Tubular I n t e r a c t i n g design a s compared with t h e Hollow
Rod design, t h e i r residence t i m e i n days i s sho r t e r , which increases
t h e s a f e t y margin aga ins t corrosion.
ACKNOWLEDGMENTS
The authors are most indebted t o a l l t he nuclear i n d u s t r i e s and
f u e l f a b r i c a t i o n cen t r e s t h a t have given them t h e i r support with
r e spec t t o f u e l f a b r i c a t i o n and c a p i t a l c o s t assessments. They a l s o
apprec ia te t he g r e a t value of d i scuss ions with M r . S. B. Hosegood,
M r . M. S. T. Price and M r . E. Smith. Special acknowledgment i s a l so
due t o Mrs. E. B e l l , Mrs. K. S. Merrick and M r . M. Paruccini for
t h e i r most valuable assistance.
REFERENCES
I.
2.
3.
4.
5.
L. W. Graham and M. S. T. P r i c e , Dragon Materials Division, Pr iva te Communication.
C. Zanantoni, e t al., MOGA (Version of t h e GGA Code GAF'FEE), forthcoming I sp ra , Euratom Report.
H. Gutmann, J. Daub and U. Weicht, TECO - An HTR Design Survey Code, forthcoming D.P. Report.
J. P. Geffroy, Thermal Design of G a s Cooled Power Reactors - DONKEY 3, D.P. Report 428.
A. P. Bray and S. J. MacCracken, TIGER 11, An IBM-704 D i g i t a l Computer Programme: KAPG2044 (1959) . Temperatures from I n t e r n a l Generation Rates,
740
6. G. Mancini, Temperature E f f e c t s Due t o the Eccen t r i c i ty of Fuel Compacts i n Various HTR Fuel Element Desiqns, forthcoming D.P. Report.
1 T a b l e 3. Dragon Recommended Design L i m i t s
Necessary th ickness of ou te r and inne r f u e l channel g raph i t e cans ( f o r annular f u e l compacts) t o guarantee t h e i r i n t e g r i t y
5 mm
Manufacturing l i m i t on t h e lowest poss ib l e th ickness of 7 mm t h e annular f u e l compact
Manufacturing l i m i t on t h e lowest poss ib l e th ickness of s3 m the f i lament between t e l e d i a l ho le s
b Achievable coated p a r t i c l e packing f r a c t i o n 0.35
Long-term l i m i t on f u e l temperature 1350 C 0
C 0
Long-term l i m i t on cool ing channel surface temperatures 10 50
L i m i t on the f a s t neutron dose 4 x i o 2 1 EDNa
%DN = Effec t ive Dido Nickel Dose ( n v t )
b2 1 gm/cm3 f o r s tandard p a r t i c l e s
Note: A l l t he given design l i m i t s are todays l . i m i t s and are expected t o ease with f u r t h e r f u e l development,
741
Table 4. C o s t Assumptions
Cost Normalisation Point: p r ice l e v e l on 1 s t January, 1969
Item Dragon Assumptions ~~
Plant and Capital
P lan t type
Reactor l i f e
Load f a c t o r
I n t e r e s t r a t e
Tax
Insurance
I n f l a t i o n
Amortisation r a t e
Twin Sta t ion
20 Y
0.75
6% y-1
0% y-l
0% y - l
9.6% y-1
$ 750,000 per twin s t a t i o n and year
Material C o s t s and Credit
U ore cos ts 8 $/lb U308
Th c o s t 17 $/kgTh
Conversion of U 3 8 0 t o UF 6 2.67 $/kg
Separative w r k c o s t s 26.0 $/kg SWU
T a i l enrichment
Transport of f r e s h f u e l 2.9 $figrn
0.2 wt.%
Transport of depleted f u e l elements 8.0 $figm
Plutonium c r e d i t 10.0 $/g f i s s i l e
Depreciation Factors
For reprocessed low enriched uranium 0.8
For twice-through uranium i n case of segregated thorium f u e l cycles
0.5
For once-through uranium i n case of 0.7 segregated thorium f u e l cycles (F ina l Charge)
Fabrication cos ts 200-370 $ /kgm d e w d i n g on throughput, enrichment, and f u e l element dimensions
Refabrication c o s t s ... fabr ica t ion c o s t s x 1.04
Reprocessing cos ts :
depeding on throughput I Thorium cycles (including 18 years 40-50 $/kgrn
of storage of i r r a d i a t e d thorium)
Law enriched cycles 35-45 $/kgm
I n t e r e s t Periods
mela
Conversiona
Enrichment servicea
Fuel elementsa
cooling timeb
I n t e r v a l between discharge of breed p a r t i c l e s and reloading of the bred fuel
17 (20) months
15 (28) months
12 (15) months
6 (11) months
12 (6) months
2 1 months
%‘he f i r s t value i s f o r replacement f u e l , the value i n brackets i s the f i r s t charge fue l .
bThe f i r s t value i s f o r replacement f u e l and i s an average over the r e a c t o r l i fe t ime a s determined by the expected ccnditions f o r the f i r s t HTR power plants. The value i n bracke ts is f o r the f i n a l charge fuel.
742
Table 5. Design and Physics Data for Referen,ze Optimum Cases
~ ~~
Design Hollow Rod Te l e d i a 1 W u l a r In t e rac t ing
L O W L O W L O W Segregated Enriched Enriched Enriched zh/U-235 Fuel Cycle
Design Data
Discharge I r r a d i a t i o n
Power densi ty
Rating
Residence time ( including load f a c t o r )
Plant e f f i c i ency
NC"HM
Heavy metal densi ty
Packing f r a c t i o n
Fuel Temperature
Peak nominal ( f r e s h )
corresponding peak during i r r a d i a t i o n
Peak systematic
2 u peak random
Surf ace Temperature
Peak nominal
Corresponding peak during i r r a d i a t i o n
Peak systematic
2 u peak random
(Gn'd/t) 60
(w/m3) 4.6
( M W / t & 46
(yea r s ) 4.8
0.418
2 50
(g/cm3) 0.78
0.275
(OC)
1026
1121
1256
1350
( O C )
86 1
8 6 1
936
996
60
9
96
2.3
0.417
280
0.90
0.33
1062
1122
1209
1303
898
923
10 13
1078
60
9
96
2.3
0.417
280
0.67
0.23
1080
1096
1183
1283
9 28
964
1054
1106
60
7
62
3.5
0.417
225
0.815
0.35
106 5
1065
1139
1255
920
940
10 28
1090 ~
Physics Data
F a s t neutron dose ( E D N )
Max. age f a c t o r
Fif a
Conversion r a t i o
Feed enrichment ( W t . % )
U-235 make-up per (wt.*) heavy metal loaded
Neutron Balance
? . E
Graphite and leakage lo s ses
Xenon overr ide
Further con t ro l l o s ses
Other non- fe r t i l e l o s ses
Conversion capture
3.0 x 1021
1.20
1.24
0.60
5.1
1.92
0.10
0.01
0.02
0.19
0.60
2.7 x 1 0 2 1
1.16
1.10
0.5')
5.7
1.92
0.12
0.02
0.02
0.17
0.5'3
2.7 x lo2' 1.16
1.10
0.59
5.7
1.92
0.12
0.02
0.02
0.18
0.58
3.3 x 1021
1.60
1.40
0.69
- 2.6
2.16
0.15
0.02
0.02
0.25
0.72 A
743
T a l e 6. Cost B r e a k d m f o r Reference Optinrm Ca.ses
Design Hollow Rod Teledial Tubular Interact ing - LOW tow m w Segregated
Enriched Enriched Enriched Th/U-235 Fuel Cycle
Capi ta l Costs
Tender pr ice mil l ion $
Specif ic tender $/kW price
Custmers on-costs mil l ion $
spec i f i c astomers $ / k ~ on-costs
All-in cap i t a l mil l ion $ cos t s
Specif ic a l l - i n $/kW cap i t a l cos t s
Fuel Cycle Costs
Inventory smw millsmwl
Replacement $ / k W
millsmwh
Total f u e l cos t mills/lrwh
Total f ab r i ca t ion mills/kwh cos t s
Total rewocessing millsmwh
16 1
127
33
26
19 5
152
24
0.37
77
1.14
1.02
0.62
0.07
152
1 19
32
25
184
144
13
0. x)
84
1.26
1.03
0.58
0.07
152
119
32
25
184
144
13
0.20
84
1.25
1.03
0.57
0.07
155
122
32
25
18 7
147
22
0.34
69
1.03
0.74
0.59
0.08 costs
Total U-credit
Total Fu-credit
Runninq Costs
I n t e r e s t and Amortisation on c a p i t a l
Fuel cycle costs
Tax
Insurance
Operating cos t
mil lsrn 0.07 0.09 0.09 0.04
millS/kwh 0.12 0.13 0.13 0.00
mills/kwh 2.26 2.14 2.14 2.19
mills/kwh 1.51 1.46 1.46 1.37
mills/kwh 0.00 0.00 0.00 0.00
millsrnwh 0.09 0.09 0.09 0.09
mills/kwh 0.32 0.32 0.32 0.32
Total Generati- millsmwh 4.28 4.01 ' 4.01 3.97 c o s t s - Total Present $ / k W Worth - 280 269 269 266
744
STRUCTURAL GRAPHITE
(1.8 9/crn3)
SULK GRAPHITE. (1.6 9/cm3 ACCOUNTING FOR ~ I D S )
a HOLLOW R O D FUEL CHANNEL O E S I G U . A P I T T H = ~ ~ O C ~
A L L MEASUREMENTS A R E GIVEN IN mm
b. 8 PIN TELEDIAL FUEL CHANNEI-. A PITCH = 3.5cm
FIG. I
STRUCTURAL G R A P H I T E
( 1 . 8 glcrn3)
BULK GRAPHITE (1.48~lcm' CCOUNTING FOR VOIDS)
A L L M E A S U R ~ M ~ N T S A R E G l v E U I U mrn
FIG '2 T U B U L A R FUEL C H A N C I E L . A P I T C H 0 3.5Cm
L L G E U D - P.D. 3 LAW lm) -- PD, 4 u w / m 3
PO. 5 u w l r n '
U A X I U U M A G E F A C T D R
FACTOR
AGE ]2,0
FlFA
0 . 5
F l F A
60 A N D 8 0 G W d l t
------ - . - -
COUVCRSIOU R A T I O FOR ALL C O R E P O W E R D E U 6 I T I E S
C O U V C R S ~ A 60 G W d / t
RATIO
8 0 G W d 1-
100 Z O O 3 0 0 4.00 uc/ NHM
F I G 3 PHYSICS M T A F O R HOLLOW R O D FUEL E L E U E U T
LEGEND
P O 6h4w/rn3
MAXIMUM AGE. FACTOR
FOR ALL CORE POWER DENSITIES
F lFA
0 . 5
AGE FACTOR
FIFA
CONVERSION RATIO R ) R ALL CORE POWER DFUSlTlES
FIG .4 PHYSICS OATA FOR TELEDIAL FUEL ELEMENT.
FlFA
1.0
0 . 5
ENRICHMENT
(*/o w/w)
MAXIUUU &E FACTOR
FOR ALL CORE: POWER DENSITIES
80 // ~ w d / t
GOGWd/t
FlFA
CONVERSION RATIO FOR ALL CORE POWER DESIGNS
*,t b, U- 235 FEED ENRICH MEN^
I 1 I 1
100
L
200 3 0 0 4 0 0 NC/NHM
FIG 5 PHYSICS DATA FOR TUBULAR INT FUEL ELEMENT WITH L .E . FUEL
c LEGEND
- P.O 7 o uwjrn)
-- P.D 9.0 U W / m3
MAXIMULA AGE FACTOR F(3A 0-
FIFA
0 5
FACTOR
2 0
I 5
AGE I I O
COL~VCRSIOU RATIO
UNIRRADIATED BREED PARTICLES- ----- 8 0 GWd/ t
6 0 G W d / L
- _--- ----
I I I too 300 400 UC/NUU
L I00
F I G 6 PHYSICS DATA FOR TUBULAR INT FUEL €SMENT THORIUM 1 HIGHLY
EURICHLD FULL CYCLES
I R R A D I A T I O U 60 Gwd/ t LEGEND - TOTAL GGNERATIUG COSTS
( U l ~ L S l k w h ) -- FAST UCUTRON DOSL
(102' EON)
'io - - - UAXIUUU WX.4 FUEL TEMP w i r n FULL GAGGING
I
I I I
I
6 -
5 -
4-
3 -
\. .
\.
I I io 09 0 8 0 7 O Q 0 5 --fw (¶/cm3) I 1 1 4 I
1 0 0 2 0 0 500 400 -Nc/NMU
FIG 7 m T A L GENERATING COSTS FOR HOLLOW ROD DESIGN V S NC / NU
IE(E(ADIATI0U 60 G w d / t LEGEND - TOTAL GENERATING
_ - FAST NEUTRON DOSE C~STS(MILLS/ kwh)
( 1 0 ‘ 1 SOU) 3 0 2 0 - - - MAXIMUM NOM FUEL I i ( w / m ’ )
TEMPERATURE WITH FULL GAGGING
I I 9 -
8 -
7 -
6-
S-
Tp = llOO°C
I 3 -
8 -
7 -
6-
5 -
FIG 0 TDTAL GENERATING COSTS FOE\ TELEDIAL DESIGN VS tJC/NU
IRP ID IAT ION 60 G w d / t LEGEND
1 MILLS/kwh
- P D = ~ M W / ~ ~
- - PO= 3 M N / ~ ) --- FAST NEUTRON DOSE
3 9 t -Jm (91 cm’) 0 5 I O 0 9 oe 07 06
I , 400 -)Nc/NHu _. I
2 0 0 300
4 I& CD IRRADIATION 80 G w d / t
MILLS / kwh
4 3 1 ,
FIG 9 TOTAL CEUERATING COST m R TUBULAR INT DESIGN WITH L E FUEL CYCLES W NC&
c
I I I I _
c LEGEND :- - HOLLOW ROD PO 4.0 M W / m 3
TUBULAR LOW ENRICHED MAXIMUM FU€L TEMPERATURE P D 9.0 M W / ~ ~
PD 7 . 0 ~ w / r n ~ TUBULAR THORIUM/URANIUM --
I R R A D I A T I O U 60 G W d
- - - FAST NEUTRON DOS& (1021 EDU)
TC MAXIMUM NOM FUEL TEMPERATURE WITH FULL GAGGIUO
FSASIBLE DLSIGU
t
t “lLLS/kWh
4 . 1 t IRRADIATIOU 80 G W d / t
4.0 I
38 COATED PARTICLES COATED PART IC LGS PACKING FRACTIONS 7 0 35 PACKIUG FRACTIOUS 0 35 1 I ‘ 0,8 97 06 0,s - f ~ ~ ( 9 / ~ ~ ~ )
3 7
100 200 3- 400 - u C / U H M
FIG 10 TOTAL GEUERATIUG COSTS FOR THE TU0ULAR INTERACTING DESIGN WITH THCRIUU/HIGHLY ENRICHED FUEL CYCLES vS NC /UHM
L P D 9.0 MW/m’
110
I \ I \
RESIDENCE TIME
MAXIMUM PIN SURFACE TEMPERATURE
loot
FIG I I MAXIMUM NOMINAL FUEL AND PIN SURFACE TEMPERATURE V S RESIDENCE TIME , Nc/ NHM= 300 , IRRADIATION = 60 G W d / t
IRRADIATION 60 G ~ d / t
\ HOLLOW R O D
T E L E D I A L
IRRADIATION 80 ~ w d / t
t / k w h
\ \
4.6 C , HOLLOWROD
I I I 1 l I 0 0 I 2 0 0 1300
* I d 0 0 ' C
FIG 12 OPTIMUM TOTAL GENERATING COSTS V S FUEL TEMPERATURE
LIMITS FOR THE. HOLLOW R O D A N D T E L E D I A L D E S I G N
IRRADIATION 60 G w d / t
HOLLOW ROO
I I
IRRAOlATlOU 80 G w d / C
\ \ HOLLOW ROD
F I G 13 FUEL CYCLE COSTS RESPONDING TO OPTIMUM TDTAL
GENERATING COSTS V S . FUEL TEMPERATURE LIMITS FOR THE
HOLLOW ROD A N D T E L E D I A L DESIGNS.
I R R A O l A T l O U 60 Gwd/ t
LEGEND
---- TUBULAR LOW
EURICHED FULL - - - TuDULAR THORIUM /uE(AUILICA FUEL
7 u w / n a 9 u w In' - -----
1 I R R A D I A T I O N 80 G W d / C
UILLS/ kwh
F I G 14 O P T I M U M TOTAL G E U E R A T I U G COSTS V S F U E L T E M P E R A T U R E
L I M I T S FOR THE T U 0 U L A R I N T E R A C T I N G O E S I G U
LEGEUO - - - ~ ~ U L A U ~ u r wlrn
LOW CUUICHCD FUEL
-- - TUBULAR INT. WITH
THORIUM /URAUIUM FUEL
I R R A O I A T I O U 80 G w d / L
F I G 15 F U E L CYCLE COSTS CORRESPONDIUG TO O P T I M U M T O T A L
G E U E Q A ~ I ~ J G COS-S V 5 FUEL T E W P E R A T U R E LIMIT3 FOR T H E
TUEULI-T, I ~ ~ T E K A C T I ~ I E CECIC-hI
752
D I S C U S S I O N 8 E'. P. Ashworth: The t o t a l gene ra t ing c o s t s appear t o be i n s e n s i t i v e
both t o t o l e r a b l e f u e l temperature and t o burn-up for a l l t h e s e de isgns .
Could you exp la in t h e s e po in t s?
H. Gutmann: Yes, t h i s i s t r u e f o r t e l e d i a l and tubu la r i n t e r a c t i n g
f u e l e lements ; f o r t h e Hollow Rod i t holds only wi th r e spec t t o burn-up.
The reasons f o r t h e i n s e n s i t i v i n e s s t o buri?-up i s t h a t h igher i r r a d i a t i o n s
g ive h igher age f a c t o r s which subsequent ly loeads t o h igher gagging, and
i n c r e a s e i n blower power and a lower p l a n t e f f i c i e n c y . The i n s e n s i t i v i -
n e s s t o t h e f u e l temperature l i m i t can be c?xplained by saying t h a t t h i s
i s a l i m i t on t h e peak random temperatures and t h e gagging have t o be
ad jus t ed f o r t h i s . Though going t o h ighe r power d e n s i t i e s means an
advantage i n b a s i c c a p i t a l c o s t s , i t a l s o means l a r g e r sys temat ic and
random e r r o r s t o be accounted f o r i n an i n c r e a s e i n t h e d i f f e r e n c e between
f u e l and gas temperatures . I am glad t h a t you have brought t h i s po in t up.
The r e su l t s f o r t h e t e l e d i a l and t u b u l a r i n t e r a c t i n g des igns show t h a t
without l oos ing much i n t o t a l gene ra t ing c o s t , lower f u e l temperatures
can be chosen which would be b e n e f i c i a l wi th r e s p e c t t o f i s s i o n product
r e l e a s e .
D. J . Merrett: Your r e s u l t s a r e ve ry s i m i l a r t o those which were
ob ta ined by TNPG, bu t a s po in ted ou t , w e cons ide r t h a t t h e t e l e d i a l
des ign needs t o be downrated t o produce acc:eptable g r a p h i t e stresses.
Would you c a r e t o comment on whether you s t i l l f e e l t h a t 9MW/cm3 i s an
achievable t a r g e t .
H. Gutmann: You a r e r e f e r r i n g t o t h e d i scuss ions fo l lowing your
paper. I t h i n k t h a t t h e Dragon r e p r e s e n t a t i v e s have made it c l e a r t h a t
w e do n o t sha re your philosophy wi th r e s p e c t t o shutdown stress l i m i t a -
t i o n s . You have s a i d then t h a t TNFG i s des igning a l s o t o 40 percent of
t h e u l t i m a t e s t r e n g t h while Dragon have made t h e po in t t h a t an apprec i ab ly
h ighe r va lue should be acceptab le . We, t h e r e f o r e , do n o t see a need t o
down r a t e t h e t e l e d i a l des ign . When asked by E . Smith you s t a t e d t h a t i f
t h i s r e s t r i c t i o n d i d n o t e x i s t t h e t e l e d i a l would only be roughly 1 pound
per kw more expensive than the t u b u l a r i n t e r a c t i n g design. This i s
753
@ approximately 0.04 w a t t s per kwh. I agree wi th you t h a t t a k i n g i n t o
account d i f f e r e n t l y assumed survey l i m i t s t h e r e i s no d iscrepancy Ire-
tween our r e s u l t s .
P. U. F i s c h e r : I was s u r p r i s e d t o see t h a t lower power d e n s i t y f o r
I t h e thorium a s compared t o t h e low en r i ched case i n your l a s t t a b l e . W e
u s u a l l y f i n d t h a t a h ighe r power d e n s i t y and a f u e l loading t h a t g ives a
lower age peaking f a c t o r l ead t o more f a v o r a b l e power gene ra t ion c o s t s .
H. Gutmann: Our r e s u l t s show t h a t t h e t u b u l a r i n t e r a c t i n g des ign
i s l i m i t e d on t h e s u r f a c e and n o t on t h e f u e l temperature . Already f o r
t h e low en r i ched c y c l e s we have exceeded t h e corresponding tempera ture
l i m i t of 9MW/cm by roughly 56OC. The thorium f u e l cycles have i n t r i n s i -
c a l l y n o t lower but h ighe r age f a c t o r s t han t h e low-enriched c y c l e s .
3
3 Consequently for t h e chosen thorium re fe rence c a s e a t 7MW/cm
exceed t h e s u r f a c e temperature l i m i t by 4OOC. I have t o stress t h a t
w e have chosen a l l our optimum c a s e s t a k i n g t h i s des ign c o n s i d e r a t i o n
i n t o account and n o t o n l y on the b a s i s of lower t o t a l gene ra t ing c o s t s .
I would l i k e t o add t h a t I have made i t c l e a r i n my l e c t u r e t h a t w e
cannot r ega rd our thorium des ign a s an optimum des ign , and I f e e l s u r e
t h a t i n t h e f u t u r e w e would be a b l e t o do much bet ter . We j u s t have
t o l e a r n more about t h e f u e l l i m i t a t i o n s .
w e s t i l l
755
EVENING PROGRAM
Tuesday, A p r i l 28
Dinner Speaker - S. E . Bea l l ,
D i rec to r , Reac tor Div is ion ,
Oak Ridge Na t iona l Laboratory,
" H E R s and Greenhouses
756
GREENHOUSES FOR HTGR’S? - S. E. Beal l , Jr., 03NL
For s e v e r a l years t he United S t a t e s ha:; been undergoing a revolu t ion i n a g r i c u l t u r e b e s t recognizable i n the mechanization of t h e labor- i n t e n s i v e opera t ions such as p lan t ing , cultflvation, and harves t ing , Not
s o recognizable, b u t j u s t as revolut ionary, has been the development of t he chicken indus t ry - b o t h egg and b r o i l e r production. over f i v e pounds of feed t o make a pound of l i v e chicken. You might be su rp r i sed t o know t h g t a t the present t i m e 5: chicken can be grown f o r two
pounds of feed per each pound of chicken; t h i s has come about through a
very vigorous and s tudious a p p l i c a t i o n of a6 ; r i cu l tu ra l engineering. I be l i eve the re are o the r oppor tun i t i e s i n the f i e l d of a g r i c u l t u r e i n which these same p r i n c i p l e s can be appl ied ,
I n 1910 it took
We are a l l familiar w i t h the unpleasant f e e l i n g of l i v i n g i n a cold climate; i t ’ s j u s t a f ac t of l i f e tha t it takes some energy t o maintain
comfort i n a cold environment. If s u f f i c i e n t energy i s not a v a i l a b l e t o rep lace t h a t l o s t t o t h e environment by hea t t r ans fe r , r e s p i r a t i o n , evaporation, e t c . , metabolic func t ions w i l l be d i s turbed and the growing process a f f ec t ed . Both w a r m and cold-blooded animal func t ions appear t o
vary wi th temperatures, as w e s h a l l see i n a moment. Environmental con- t r o l of animal and p l an t enclosures has g r e a t prospects f o r becoming a n important f a c t o r i n t h e a g r i c u l t u r a l revolu t ion . We th ink of environmen- t a l c o n t r o l as con t ro l of t he temperature, humidity, l i g h t , s o i l , and a l l
the th ings which p l a n t s and animals need t o grow vigorously, inc luding a i r . A i r has become a very important p a r t o:? environmental cont ro l . A
fe l low s a i d t h e r e was a t i m e when “sex was d:irty and a i r was c l ean , “ bu t
t h a t ’ s been reversed now! has caused the loss o f e n t i r e crops of tomatoes and carnat ions. I n a con- t r o l l e d environment the a i r would be cleaned before exposure t o p l a n t s ,
There a r e s e v e r a l i n s t ances where pol lu ted a i r
A
I want t o emphasize, though, t h e importence of temperature cont ro l .
My f i rs t s l i de shows some da ta I have accumulated which i n d i c a t e s how i m -
po r t an t temperature can be i n t h e growth of animals. have p l o t t e d percentage of growth a t optimum temperature versus
A s you can see, we
- -_ - - . . . . . . . . . . .
757
temperature. Below 20°C c a t f i s h hardly exhib i t any growth a t a l l , whereas up t o 30°C
t h e r e i s a remarkable increase. The same i s generally t r u e f o r m i l k pro- duction, f o r chicken grovth, and a l s o f o r swine.
Note the curve f o r shrimp, and t h e s teep curve f o r ca t f i sh .
Another f a c t o r which i s important i s the ef f ic iency of feed conver- sion. One has a choice i n growing animals of creat ing the bes t environ-
mental temperature o r let t ing the feed be converted t o produce heat. Using feed as f u e l i s very expensive, about $5 a mil l ion Btu, compared t o $.50 t o $l.OO/million Btu f o r gas, so one can hardly a f ford t o use feed t o keep animals comfortable.
The next s l i d e w i l l show you how the feed conversion e f f ic iency var- ies with temperature f o r some of these animals. ciency of conversion, based on pounds of weight gained per pound of feed
consumed of 3976 f o r chickens, whereas a t 34"C, the optimum temperature, you see tha t the e f f ic iency i s 52s (1 lb of growth per 1 . 9 lb feed) . c a t f i s h it i s even more remarkable. This i s an animal t h a t i s approach-
ing one pound of l i v e weight for every pound of feed, but 65$ conversion i s a more normal eff ic iency. The data f o r pigs a r e crude but an ind iv i - dual hog, a t 3OC, only converts a t an e f f ic iency of 1'78, whereas one kept a t 15 t o 23"C, has a 298 eff ic iency, a 70$ improvement.
milk are a l i t t l e misleading. l i q u i d m i l k per pound o f dry feed, b u t no te t h e d i f f e r e n c e between - 1 3 ° C
and 38"C, a f a c t o r of nearly four.
A t 24OC, we have an e f f i -
For
These data f o r
Efficiency here i s based on pounds of
But what one would l i k e t o do i s t o estimate the value t h a t might accrue from control l ing the environment. i n t h i s fashion. The numbers i n column 1 a r e production r a t e s of food on
The next s l i d e i s an exercise
a per acre bas i s f o r uncontrolled environment, taken from severa l reput- ab le sources. controlled environment. You see t h a t 500 pounds of f i s h per acre i n a natural environment i s a standard production r a t e , whereas i f one controls the temperature a t 32OC and supplies plenty of oxygen and feed, he can
produce 200,000 pounds of f i s h per acre. For b r o i l e r s an increase of a hundred thousand pounds per acre i s possible. For vegetables, tomatoes
a r e the b e s t example:
Column 2 l i s t s yields which have been experienced w i t h a
the highest y ie lds i n the s t a t e of Cal i fornia are
758
Effect of Temperature on Feed Conversion Q Feed Temp. Lbs Feed/Lb Efficiency
(f 1 ( "C ) . Weight Gain -
Chickens' 24 2 . 7 39
30 2.1 48
34
Catfish2 20
29
32
Hogs3
Individual Hog, 3
Group, 3
Group, 8
Group, 15,23
Milk Cows4 (Jersey) -13
10
38
j.. 9
c;. 0
1.. 3
1.. 5
5'. 9
A:. 3
5 .8
3.4
2.1
0.65
0.55
52
25
75
65
17
23
27
29
48
128
180
'Howes, Grub, 1962; k r o t t and Pringle, 1949 'Stram, West and Dunn, 1965 3Sorensen, 1962 4H. D. Johnson, 1965
Reported Yields (Lbs/Acre )
Food Product Estimated Value of Increased Yields Uncontrolled Environment Controlled Environment
Fish 0.01 x i o 5 (1 1
Broilers
Beef
Pork 7.5 x 105 (5 )
Vegetables, e. g., 0.6 x l o5 lbs/acre (6) Tomatoes (One Crop)
1. Nations Agriculture, March 1970 2. Poultry Science, Vol. 37, No. 5 , 1958 3. J. R. Hares, W. R. G r d , Auburn University Experiment Station, 1962 4. Calculated from information by J. B. B i l l a r d , National Geographic, February 1970 5. J. Mentzer, Purdue University Experimental Station 6. USDA Yearbook, 1968, California Yields 7. W. C. Yee, personal communication 8. Heysler and Ruthner, 1968, and M. Bentley, Commercial Hydroponics, 1959
Q
7 59
@ about 60,000 pounds an acre f o r open f i e l d cul t ivat ion.
t r o l l e d environment such as a greenhouse where one can control water, f e r t i l i z e r , C 0 2 , temperature, e t c . , three crops a year are possible and t o t a l production could reach near ly a mi l l ion pounds per a c r e per year. I n f a c t severa l of these foods can be produced today a t a rate of a
mi l l ion pounds per acre per year, and o thers can reach t h i s l e v e l with
the proper appl ica t ion of ava i lab le technology. have estimated the value of the increased production that comes with con- t r o l l e d environment. My estimate var ies from $20,000 an acre for pork t o $100,000 f o r an acre for tomatoes.
Now i n a con-
I n the l as t co lmn I
Now my next s l ide* i s a p ic ture of a greenhouse f u l l of tomato plants which average about twenty pounds t o t h e p lan t and which can produce i n the neighborhood of 600,000 or 700,000 pounds per acre on a three crop per year bas i s . The next s l ide* shows cucumbers grown i n grea t p r o l i f e r - ance, under carefu l ly controlled conditions. An i n t e r e s t i n g point here - i n the f i rs t century it i s recorded by Pliny the Elder i n h i s Natural History t h a t Emperor Tiberius loved cucumbers. w i t h i s i n g l a s s for his gardener t o grow cucumbers i n the o f f season.
ing the daytime the c a r t was r o l l e d out f o r the b e n e f i c i a l e f f e c t s of the
sun, and a t night the c a r t was r o l l e d back i n t o the house. years ago people were growing cucumbers i n greenhouses!
He ordered a c a r t covered
Dur-
Two thousand
It appears that a l l w e need t o accomplish year-round growth and
higher y ie lds of l o t s of foods i s cheap heat, and now, a question for the audience: quant i t ies which might a l s o solve some heat po l lu t ion problems?" months ago Don Trauger and I were out a t Fort S t . Vrain, Colorado, and
there we saw a la rge f e r t i l e area of land being devoted t o a nuclear reac-
tor. This s i t e i s some 2200 acres and i s very prime a g r i c u l t u r a l land. Fort St . Vrain, as you know from a l l that you've heard a t t h i s meeting, i s the High Temperature Gas-Cooled Reactor which Colorado Public Service Company i s building. 330 Mw(electrica1) w i l l be the operating l e v e l and
a t 40$ ef f ic iency it w i l l produce 500 Mw of thermal energy a t 102'F, t o
"Where on e a r t h could we f i n d the source of cheap heat i n l a r g e A few
Wolor photo not included i n t h i s paper
760
be thrown away by means of cooling towers.
how can we miss? towers of t h i s r eac to r , which would cos t atlout a mi l l i on t o a mi l l i on and ha l f d o l l a r s could be e s s e n t i a l l y replaced w i t h "greenhouse cooling
towers. 'I
cooled i n summertime with a device ca l l ed an evaporat ive cooler . The next s l ide i s a p i c t u r e of such a cooler. I t ' s a very cheap affair made from galvanized wire about 2 in . t h i ck s t u f f e d with aspen f i b e r s or Spanish moss. The way it opera tes i s t h a t water, i n our case w a r m water
(102°F) flows i n t o the top of t he pad while a l a r g e flow of a i r i s pul led ho r i zon ta l ly through the pad. Both the a i r and water temperatures i n the f i b e r approach the p reva i l i ng wetbulb temperature. Thus one can maintain
des i r ab le temperatures i n the summertime, and t h i s i s e s p e c i a l l y t r u e a t Denver, Colorado, where the wetbulb temperature runs i n the neighborhood
of 65°F. It i s f a i r l y easy t o show tha t on? can maintain a summertime temperature below 75 degrees i n t h e greenhouse by evaporat ing enough water t o cool t h e water and the a i r . The complete system i s shown on the next s l i d e t o give you a b e t t e r p i c t u r e of how it works. There i s an
evaporat ive pad a t one end and two fans a t the o the r end. The fans draw a t f a i r l y l a r g e r a t e s , l i k e 150,000 lb/hr , -through t h e pad while 40,000 t o 80,000 l b of water/hr flows down through t h e pad. I n t h e summertime the a i r i s blown t o the outs ide , which i s t h e way a cooling tower works, bu t i n t h e winter t ime when you want t o maintain a warm house, then one has t o conserve the hea t i n the a i r by recii 'culating. We have i n s t a l l e d
a p l a s t i c shee t , t o form an a t t i c , t o a l low the r e c i r c u l a t i o n of the a i r back through the warm water coming from the r eac to r s t a t i o n . It i s c l e a r t o us t h a t one can cont ro l temperatures, l e t ' s say, a t 75 t o 80°F i n t he
summertime and above 65°F i n t h e wintertime. expected t o be a problem, we have provided a n opt ion of a row of f inned tubes downstream of the pads so t h a t some dry heat can be added t o keep
the humidity i n t h e 70 t o 80% range. t e m i s t h a t one can b e a t t h e e x i s t i n g cooling towers a t For t S t . Vrain
by about 13°F; t h a t i s , he can send colder water back t o the condenser with t h i s system than he could w i t h t he cool ing towers; t h i s i s important
because it means a g r e a t e r e f f i c i e n c y o f conversion t o e l e c t r i c i t y i n
t h e normally warm summertime.
With f r e e land and f r e e heat ,
We (Garland Samuels and 1 ) propose t h a t t he cooling
We th ink t h a t t he greenhouses could be heated i n wintertime and
I n case high humidi t ies a r e
The remarkable th ing about t he sys-
761
Another very important aspec t of t h i s heat ing-cool ing system i s the
cleaning of t h e a i r by the a i r -water contact ing.
it appears l i k e l y t h a t crops cannot be grown near c i t i e s i n the f u t u r e
unless t h e d i r t y a i r i s cleaned by some process. Water washing i s an ex-
tra b e n e f i t of t he evaporative pads.
A s mentioned e a r l i e r ,
Since For t S t . Vrain i s near Denver, it i s natural t h a t we would
look a t Denver f o r an es t imate of the f r e s h vegetables and poul t ry which
t h e c i t y uses, so we can determine how many greenhouses and poul t ry
houses a r e needed. The U.S.D.A. records of shipments t o the c i t y o f Denver fo r t h e year 1968 show a t o t a l unloading of ou t -o f - s t a t e produce
of 113 m i l l i o n pounds of f r e s h vegetables . I a m not including potatoes
or gra ins . Eveh a t two cents per pound, t he cos t of shipping a hundred
and t h i r t e e n mi l l i on pounds i s about a mi l l i on d o l l a r s a year t h a t could
be saved. Also, assuming t h a t Coloradians e a t chickens as f requent ly as
o the r people i n the United S ta t e s , they could use 20 m i l l i o n b r o i l e r s i n
the environs of Denver, and aga in one can ca l cu la t e nea r ly another mi l l i on
d o l l a r s f o r shipping because few b r o i l e r s a r e grown i n Colorado. So here
i s an opportuni ty for the entrepreneur who is w i l l i n g t o make use of t he
For t S t . Vrain hea t t o produce these foods. On the basis of these sh ip-
ments one can ca l cu la t e t h a t it would take 500 ac res of greenhouses and
maybe 50 ac res of poul t ry houses t o supply the c i t y of Denver. For t S t .
Vrain can ' t supply q u i t e t h a t much heat , bu t i t can supply enough hea t f o r 200 acres . Actual ly , w e can show t h a t 100 acres would be s u f f i c i e n t
t o dispose of a l l t h e 500 Mw heat .
One or two hundred a c r e s a t $175,000 per ac re for greenhouses i s not
an exorb i tan t investment compared t o the investment of the power p l a n t
i t s e l f . One does have t o look ca re fu l ly , though, a t t h e c a p i t a l cos t ,
and I know you wonder whether or not such a t h i n g would pay o f f .
house operators i n the s t a t e of Colorado expect t o spend $.50 t o $1 per
square foo t f o r t h e i r hea t ing equipment.
per acre , which i s a s i zeab le investment.
$4,000 t o $8,000 per a c r e i n hea t b i l l s t o keep t h e i r crops growing a t t h e
maximum r a t e . From my contacts i n the business , I am c e r t a i n they m e
making a p r o f i t even with these l a r g e hea t cos ts .
Green-
This comes t o $25,000 t o $40,003 They expect t o spend from
What about oi.r systern:
7 62
F i r s t , f o r c a p i t a l cos t , t h e a d d i t i o n a l equipment needed t o d e l i v e r t h e
h e a t from t h e r e a c t o r would be pumps, piping, e l e c t r i c a l equipment, a n
emergency h e a t of s e v e r a l hundred megawatts, a l l es t imated t o cos t about
$28,000 a n a c r e (for 100 a c r e s ) .
f o r r e p l a c i n g t h e cool ing tower, I doubt i f Colorado Publ ic Serv ice would
ag ree t o t h a t . If they did, w e would g e t a c r e d i t of about $10,000 p e r
a c r e and reduce our cos t t o $18,000 pe r ac re ; i f they d i d n ' t t h e cos t f o r
h e a t supply would be $28,000 p e r ac re , which compares wi th t h e s tandard
i n s t a l l a t i o n c o s t f o r greenhouse hea t systems.
Although we would l i k e t o t ake c r e d i t
Now cons ider t h e $4,000 t o $8,000 pe r year normal h e a t b i l l . If w e z
can h e a t 200 a c r e s o f greenhouses, w i th f r e e w a r m water, t h e p r o f i t f o r
somebody would be i n t h e neighborhood of a m i l l i o n d o l l a r s a year . I
don ' t propose t h a t a l l of it go t o Colorado Pub l i c Serv ice . I imagine they would be happy t o s h a r e it w i t h t h e gr2enhouse ope ra to r t o e n t i c e
him t o b u i l d nea r them i n a n arrangement such as shown on t h e l as t s l i d e .
Colorado Pub l i c Serv ice could poss ib ly be r i d d i n g i t s e l f o f a c a p i t a l ex-
pense f o r t h e cool ing towers t h a t would be a couple o f hundred thousand
d o l l a r s p e r y e a t a t 14$ annual charge, and a n ope ra t ing expense which I
th ink might be $50,000 a year .
So on paper, a t least , and c e r t a i n l y t h a t ' s no t t h e l as t word, t h i s
system looks f e a s i b l e and p r o f i t a b l e t o t h e grower and t h e u t i l i t y . I
th ink it can be app l i ed t o o t h e r a g r i c u l t u r a l ope ra t ions bes ides green-
houses and, of course, any power p l a n t could be used as t h e h e a t source.
The t i t l e o f t h i s talk as l i s t e d i n your brochure i s "Greenhouses f o r
HTGR's?''. I would l i k e t o remove t h e ques t ion mark, and those who want
t o i n v e s t i n t h e F o r t S t . Vrain Greenhouse Assoc ia t ion meet m e on t h e
r i g h t a f t e r t h i s talk!
L L a 0
" 0
763
10 20 30
TEMPERATURE ("C)
40
Fig . 1. E f f e c t of Temperature on Growth o r Product ion of Food Animals.
,WATER IN
CONTAINER IS v 4 IN. MESH GALVANIZED WIRE
2 "
AIR FLOW
PACKING IS ASPEN FIBERS, SPANISH MOSS, OR OTHER ABSORBENT MATERIAL
Fig. 2 . Pad Assembly.
764
ORNL UWG. 69-13967
V
F i g . 3 . Greenhouse and A i r Flow System.
ORNL DWG 69-113751
I
Ov5c&! _-+OO I SCALE-Fl
EXCLUSION &REA BOUNDARY J
F i g . 4. E x c l u s i o n Area Boundary.
Q
765
PANEL DISCUSSION:
PROSPECTS FOR THE NEXT T E N YEARS
766
J . A. Lane, Moderator
C . L. Rickard Gulf General Atomic
R . D. Vaughan The Nuclear Power Group, L t d .
K. Wirtz Kernf orschungs zentrum Karl sruhe
Oak Ridge Nat iona l Laboratory
767
PANEL DISCUSSION
PROSPECTS FOR THE NEXT TEN YEARS
J. A . Lane, Moderator, ORNL
When MY. Trauger w a s pu t t ing t h i s panel together and asked m e t o be
moderator, I am sure he did s o w i t h the knowledge t h a t I am fond of mak- ing project ions about t he fu ture of atomic energy.
t h a t i n t h a t capacity I would contribute some such project ion for gas- cooled reactors t o the discussion. Unfortunately, t he projections I make
a re not i n the same b a l l park as t h a t being considered by th i s panel. My
projections are very long range, a r e based on very meager information,
and a r e aimed f a r enough i n the fu ture t h a t they cannot be ve r i f i ed while w e are a l l s t i l l around. In contrast , the question before t h i s panel concerns t h e near-term prospects f o r gas-cooled reactors , i s based on
r e a l f a c t s of l i f e information, and i s much more d i f f i c u l t t o answer. Any such project ion we make today, moreover, can or cannot be ver i f ied i n the r e l a t i v e l y near fu ture . In other words, we have t o be careful about what we say! Fortunately, w e have three experts on t h i s panel who a r e idea l ly qua l i f ied t o give you some insight i n to the short-term outlook
f o r gas-cooled reactors , and I w i l l leave it up t o them t o do t h i s .
He probably assumed
Before turning the session over t o them, however, I have one comment t o make about t he ult imate ro l e of gas-cooled reactors ; namely, that the
long-range outlook appears t o be qui te sound. The various s tudies and evaluations of nuclear power systems that have been car r ied out during the last several years, pa r t i cu la r ly those that were done f o r t h e United S ta tes Civi l ian Power Program, a l l show that gas-cooled fast
breeders can contribute s ign i f i can t ly t o the overa l l economics of the
systems. t o l i qu id metal-cooled fast breeders. therefore , gas-cooled breeders should i n the long run become an important
segment of various nuclear power systen-k throughout t h e world.
Their long-term r o l e can be e i ther an a l t e rna te or a partner Because of t h e i r economic merit ,
7 68
The nearer term r o l e of high temperature gas-cooled converter reac-
t o r s , however, i s l e s s ce r t a in because two possible roles e x i s t . On the one hand, HTR's or HTGR's might be developed merely as a stepping stone
t o t h e longer range gas-cooled breeders. This r o l e would be r e l a t ive ly
unimportant i n t e r m s of t o t a l system megawatts. On t h e other hand, a second possible ro l e f o r HER'S ex i s t s ; naniely, t h a t they might become
the main embodiment of advanced converter reactors and introduced as a
means of saving on power costs and a t the same time conserving resources of low cost uranium. The same U.S. Civi l ian Power Studies mentioned
previously showed t h a t t he introduction of advanced converters during the
next decade o r so could save the U.S . power system from $2 t o $8 b i l l i o n
depending on the introduction dates and performance of subsequent f a s t
breeders. counted a t 7% back t o 1970. f o r introducing thermal gas-cooled reactors into the nuclear power sys-
t e m . To make t h e i r m a x i m u m impact, however, they must be b u i l t as soon
as possible and i n large numbers. In the s y s t e m analysis s tud ies men- tioned, more than one hundred 1000 Mwe HER'S were assumed t o be added
t o t h e U . S . power system during t h e period 1976 t o 1990. term r o l e of gas-cooled reactors does not depend upon technical f eas ib i l - i t y o r economics, but upon the a b i l i t y of current equipment suppl iers t o
capture a market fo r and supply so many reactors i n such a shor t period of time.
These a re not ac tua l do l la rs , but ac tua l do l l a r savings d is - Thus there i s a su f f i c i en t economic base
Thus t h e near-
Our next pane l i s t , M r . Corwin Rickard of Gulf General Atomic, should have a l o t t o say on t h i s problem of marketing gas-cooled reactors be-
cause tha t i s h i s company's main business r igh t now.
Corwin Rickard, GGA
1. It has of ten been said t h a t gas cooling of fe rs an open ended poten t ia l f o r improvement i n reactor performance. The reports a t t h i s confer-
ence together with the last ten yea r ' s experience with gas-cooled
reactors has cer ta in ly provided a dramatic i l l u s t r a t i o n of t h i s .
769
2.
We have seen:
a. Plant eff ic iency go from about 25% f o r t he ear ly Magnox reactors
t o 40$ f o r HTGR's
Core power density increase by more than a f ac to r of ten from
less than 1 kw/li ter t o over 8 kw/l i ter with a similar increase
i n power density f o r steam generators, and
Fuel u t i l i z a t i o n improved by more than a f ac to r of two such t h a t
l e s s than ha l f as much uranium need be mined t o start up and operate an H E R plant f o r 30 years, i . e . , about 2000 tons U,O,
for 1000 Mwe. What w i l l t he next t en years bring?
b .
e .
F i r s t , l e t ' s look a t the market. The forecasts indicate t h a t about
l90,OOO Mw's of capacity i n about 150 un i t s w i l l be ordered between now and 1980 i n the U.S. alone. A subs tan t ia l p a r t of these can be gas cooled. Add t o these i n the U . S . t he un i t s t h a t could be gas
cooled i n Europe, Japan, and elsewhere around the world, and it i s easy t o come up with a minimum estimate of 60 units. be twice t h i s number, representing over $25 b i l l i o n i n gas-cooled
reactor plant orders .
It could eas i ly
3. The f i r s t units can be expected t o have charac te r i s t ics l i k e those,
for example, i n the paper by A. J . Goodjohn. Overall p lan t cap i t a l
costs should be l e s s than for LWR's. a.
b . Throt t le steam flow is about one-half
e.
Waste heat is about 3576 less than for LWR's
The steam turbine i s smaller and costs $9 t o $10 mil l ion l e s s
than a LWR turbine i n 1000 Mw s i zes
Liquid and gaseous radioactive wastes a r e s m a l l and economically
controlled t o low l eve l s
d .
e. Pressure times the volume of t he primary c i r c u i t , and the s tored
energy i n the coolant a r e both less than f o r PWR's, thus, both
primary and secondary containments should be easier.
There are a number of other fac tors , as well, t h a t lead t o the
Improve- expectation t h a t plant costs will be less than for LWEi's.
ments w i l l come along as more of t h e units a r e sold.
770
a . Core and steam generator power density w i l l increase by l O - l 5 % without s ign i f icant design change
b . Plant s i zes w i l l increase a t least t o 1500 Mw.
4. Supplier Industry
Unlike some other reactor coolant technologies, gas cooling has
a ready made suppl ier industry with worldwide and redundant cap-
a b i l i t y f o r HTGR-PCRV construction, ste.m generator fabr icat ion, gas
c i rcu la t ion equipment, and other H E R c,3mponents. The s imi l a r i t y
of H E R equipment with conventional power plant equipment should
grea t ly ease requirements f o r industry investment i n new fabricat ion
equipment and should help hold costs doIan as component business in-
creases.
5 . Fuel and Fuel Cycle Characteristics
All of the H E R f u e l element designs look good from the perfor- We seem t o have b:Lock elements, b a l l elements, mance reported here.
and p in elements, bu t from the fabr ica tors point of view, these a r e not any d i f f e ren t than differences say between PWR and BWR elements.
They a l l require about the same i n fabr ica t ion equipment. t en years w i l l surely see a p ro l i f e ra t ion i n H E R f u e l manufacturing
p lan ts .
The next
It would appear t h a t carbide kernel-s, oxide kernels, low en-
riched, high enriched, thorium, Biso, arid Triso fue l s w i l l a l l be
used t o meet d i f f e r ing needs which certE.inly points t o ' t h e advantage
of f l e x i b i l i t y of H E R f u e l .
A t the same time, t h e papers here indicate t h a t performance of
t he f u e l w i l l be fur ther improved toward higher allowable tempera-
tu res permitting higher power density cores, higher ra t ings , and re -
duced f u e l inventory.
plants , w i l l r e s u l t i n a marked decrease i n f u e l cycle costs . This, plus increased throughput i n fabr ica t ion
233U recycle following the excellertt work here a t ORNL should s t a r t during the next t en years.
U.S. AEC t o extend buyback of 233U and g;uarantee HTGR fue l reprocess-
ing provided needed encouragement fo r the pursui t of the U-Th cycle
The Ikrch 1970 announcement by the
@
771
6.
7.
8.
i n t h e U.S which promises s u b s t a n t i a l improvement i n both u r a n i m
u t i l i z a t i o n and f u e l costs.
Pu-Th Cycle
The paper by Dahlberg report ing on EEI s tud ies of Pu u t i l i z a t i o n
i n HTGR's indicates they can make good use of LWR generated Pu. I n
the absence of breeders, the next t e n years should see some HTGR's
benefi t ing from LWR Pu or some LWR's benefi t ing from HTGR's making
good use of t h e i r plutonium.
HTGR Existence with Breeders
It i s of ten pointed out t h a t eventually breeders w i l l help LWR's
by buying t h e i r Pu.
with 233U.
could lead t o a f u r t h e r reduction i n HTGR f u e l consumption and in-
ventory of about 258.
and breeders w i l l happily l i v e together.
Breeders can a l s o help HTGR's by supplying them
The f irst looks a t t h i s are j u s t being taken, but it
For t h i s and other reasons, perhaps HTGR's
One got the impression from t h i s conference that the HTGR steam cycle
development was over and done with and now the R & D w a s turning t o
gas turbine cycles. I bel ieve t h i s impression w i l l be v e r i f i e d dur-
ing the coming ten years. The planned program i n Germany i s cer-
t a i n l y t o be congratulated, as w e l l as the good work i n the U.K. and
Switzerland. The papers brought out the grea t p o t e n t i a l of gas tur- bines-HTGR plants.
a. Capital cost reduction i s expected because of the d i r e c t cycle
and physically smaller turbines. W e know high temperature steam
turbines a r e smaller and cos t less than low temperature saturated
steam turbines. Gas turbines, owing t o the high working pressure
(they are not t ry ing t o get work out of a vacuum the way steam
turbines do) are v a s t l y smaller s t i l l , and therefore , should cost
less. b. Easier and more economical r e j e c t i o n of heat through a i r coolers
may prove e s s e n t i a l i n places where supply of cooling water i s
exhausted.
772
9. Process Heat
The conference, and i n p a r t i c u l a r , t h e exce l l en t paper by Iirxmer igd ica ted the increas ing i -n te res t and need for high temperature
process heat IITGR's. The l as t t e n years s a w t h e bui ld ing and s t a r t u p
of t h e 2500°F UTREX-HER. g r e a t dea l more development i n t h i s a rea , including the new programs
being discussed i n Germany and Japan.
The next t e n years w i l l no doubt b r ing a
GCFR
The Gas -Cooled Fast Breeder Reactor papers have not been presented
ye t , b u t t h e r e are some exce l l en t papers t o be given i n t h i s a r ea to -
morrow af ternoon. Compared t o o the r gas-cooled r eac to r s , t he g rea t a t - traction of the GCFR i s the p o t e n t i a l i t holds for a very large improve-
ment i n fue l u t i l i z a t i o n . For example, while a 1000 Mw HTGR w i l l r equ i r e
about 2000 tons of U3O8 over 30 years , a 1000 Mw GCFR would produce t h e
f i s s i le equivalent of about 1500 tons u308 which i s c e r t a i n l y a worthy goal t o be sought by gas-cooled r e a c t o r development.
Perhaps more important a t t h e present time, however, i s the oppor-
t u n i t y t h e GCFR provides f o r a parallel and a l t e r n a t i v e development t o
t h e L " B R .
Commissioner Johnson has w r i t t e n i n Power Engineering t h a t he woild,
. . . " l ike t o see the GCFR and the LMFBR brought a long toge ther i n devel-
opment.
P h i l i p Sporn stated before the JCAE, "The gas-cooled breeder reactclr
promises s o much i n t h e way of higher s p e c i f i c breeding r a t i o s and lower
c o s t s tha t na t iona l prudence almost demands a cont inuat ion of work on
t h i s a l t e r n a t i v e . . . . ' '
Ralph Davis, Chairman of t h e 41 member u t i l i t y group supporting GCFR development has sa id , "The U.S. n a t i o n a l breeder program would be s t rengthened by including the GCFR. This would provide competit ion of
concepts and technologies and increase p robab i l i t y of developing a
breeder a t t r a c t i v e t o t h e u t i l i t y indus t ry .
a
8
I bel ieve , therefore , t h a t we can look forward t o increas ing ac-
t f v i t y i n GCFR development i n t he years ahead.
773
R . D. Vaughan, TNPG
D r . Rickard has d e a l t so thoroughly w i t h the m a t e r i a l w e have been
d i scuss ing a t t h i s meeting and w i t h t h e American s i t u a t i o n t h a t I t h i n k
i t f a l l s t o m e t o fill out t h e s i t u a t i o n i n Europe and t o b r ing ou t some
of t he d i f f e r e n c e s i n approach which have been adopted over there. I
would a l s o l i k e t o d w e l l a l i t t l e more on some of t h e immediate problems
w e a r e encounter ing i n t h e a c t u a l des ign and cons t ruc t ion of gas-cooled
sys tems . May I d e a l f i r s t wi th t h e shor t - te rm s i t u a t i o n , t h a t i s the next
f i v e years . I n the United Kingdom there a r e e i g h t r e a c t o r s of AGR type
now under c o n s t r u c t i o n and f o u r more a r e s h o r t l y t o be committed by t h e
CEGB. The f i r s t u n i t s of t h i s programme of r e a c t o r s w i l l be going i n t o
commission next year. They a r e of i n t e g r a l des ign w i t h conc re t e p re s su re
v e s s e l s and w i l l have s i n g l e channel access f o r on-load r e f u e l i n g .
The f i r s t high temperature r e a c t o r of commercial s i z e w i l l be ordered
by the CEGB i n m i d 1971, t o be on power l a t e i n 1975. I t w i l l be a s i n g l e
600 MW u n i t a t Oldbury ' B ' and the c o n t r a c t w i l l fo l low compet i t ive
t e n d e r s from t h e two Design and Cons t ruc t ion companies now a c t i v e i n t h e U.K. I n f a c t , t h e CEGB, t o s ecu re t h e best p o s s i b l e des ign , has
a l r eady placed des ign c o n t r a c t s w i t h both of us , and i t i s from i d e a s
being genera ted under these c o n t r a c t s t h a t a formal enqui ry s p e c i f i c a t i o n
w i l l be prepared l a t e r this year .
The CEGB a r e then expected t o r e v e r t t o t h e i r custom of bu i ld ing twin
r e a c t o r s t a t i o n s and t h e pace a t which t h e HTR programme proceeds w i l l
depend ve ry much on our t e c h n i c a l progress i n c e r t a i n s p e c i f i c a r e a s .
I r r a d i a t i o n tests on the f u e l must show s a t i s f a c t o r y behaviour under
t y p i c a l r e a c t o r cond i t ions . W e must a l s o demonstrate t h a t on-load re-
f u e l l i n g i s a p r a c t i c a l p ropos i t i on a s i t has been on t h e magnox r e a c t o r s .
The CEGB a r e ve ry anxious t o k n o w t h a t t h e f u e l and the r e a c t o r a s a whole
i s capable of load fol lowing, and they a r e a l s o p res s ing f o r a des ign i n
which there i s good v e s s e l access so t h a t a l l h igh temperature items can
be in spec ted a f t e r ope ra t ion . I t i s expected t h a t there w i l l be a sub-
s t a n t i a l c o s t d i f f e r e n t i a l wi th r e s p e c t t o the AGR and t h i s w i l l be an
important f a c t o r i n determining how qu ick ly HTR i s introduced.
On the p o s s i b i l i t y of the gas- turb ine HTR, proposa ls have a l r e a d y
774
been prepared f o r t h e cons t ruc t ion of a pro to type u n i t t o fo l low a year
o r two a f t e r t h e f i r s t steam r a i s i n g HTR. Curren t e s t ima tes of t h e
saving o f f e r e d by t h e gas- turb ine s y s t e m a r e f a i r l y modest and amount t o
7 percent on c a p i t a l c o s t and 5 percent on u n i t genera t ion c o s t . W e do
n o t see any j u s t i f i c a t i o n f o r u s ing t h e gas- turb ine cyc le t o r a i s e t h e
thermal e f f i c i e n c y above t h e 42 percent now r e a d i l y ob ta inab le wi th t h e
steam cyc le . The main doubt about t h e gas- turb ine HTR, from t h e po in t
of view of an e l e c t r i c u t i l i t y , i s t h e a v a i l a b i l i t y t h a t can be expected
of i t . In an i n t e g r a l design where most of t h e components a r e tucked
away i n s i d e a conc re t e p re s su re v e s s e l , t h e ease wi th which they can be
removed and rep laced w i l l be c r i t i c a l .
The development work involved i n a gas- turb ine p r o j e c t i s q u i t e
e s t e n s i v e and such a scheme i s u n l i k e l y t o go ahead except a s a co l l abor -
a t i v e p r o j e c t involv ing two or more c o u n t r i e s i n Europe.
On t h e con t inen of Europe t h e f i r s t commercial HTR w i l l probably
be a 300 Mw pebble bed design, developed from the AVR p r o j e c t . I would
expec t and hope t h e second HTR would be a 600 lW u n i t wi th p r i sma t i c
f u e l a long t h e l i n e s adopted f o r Oldbury ' B ; . The s c a l e of t h e programme,
which I expect t o be based on Germany, w i l l then depend on t h e a t t r a c t i o n s
of t h e high temperature r e a c t o r i n r e l a t i o n t o l i g h t water s y s t e m s .
The h igh temperature r e a c t o r must f i r s t l y have lower c o s t s , c u r r e n t l y
e s t ima ted t o be 8 percent on c a p i t a l and 6 percent on gene ra t ion . The
h e a t r e j e c t i o n r a t e , of course , w i l l be much lower, about two-thirds t h a t
of t h e l i g h t water r e a c t o r s . This I understand i s becoming an inc reas ing -
l y important f a c t o r i n t h e U.S . , and w i l l a l s o apply i n Europe.
The h igh temperature r e a c t o r has a lower usage of f i s s i l e atoms than
a l l o t h e r systems except t h e CANDU r e a c t o r and t h e f a s t r e a c t o r s . I f e e l
I must a l s o d i f f e r w i th Mr. Scarborough i n h i s remarks t h i s morning on
t h i s po in t . According t o my c a l c u l a t i o n s , t h e h igh temperature r e a c t o r
uses about two-thirds t h e q u a n t i t y of 235u r equ i r ed by t h e l i g h t water
r e a c t o r , and it i s accord ingly less s e n s i t i v e t o f u t u r e i n c r e a s e s i n ore
c o s t s . Likewise, t h e e f f e c t of a reduct ion i n va lue of plutonium i n t h e
spent f u e l of a high temperature r e a c t o r i s about ha l f what i t would be
f o r a l i g h t water r e a c t o r .
N o w l e t us d e a l wi th t h e longer t e r m , where I am s u r e t h e r e w i l l be
775
I
s n exp?nding market f o r t h e h i g h tempera ture r e a c t o r i f i t m a i n t a i n s i t s
promise on c o s t s .
On the t e c h n i c a l s ide i t i s n o t d i f f i c u l t t o make some r e a s o n a b l e
p r o j e c t i o n s i n t o t h e f u t u r e . I n three o r f o u r y e a r s w e s h a l l be develop-
i n g e x t r u d e d f u e l p i n s , w i t h or w i t h o u t a f u e l f r e e l a y e r on t h e o u t s i d e .
T h i s , of c o u r s e , would n o t a p p l y t o t h e t y p e of f u e l b r i c h which GGA have
developed f o r t h e i r r e a c t o r . But f a b r i c a t i o n c o s t s w i l l b e n e f i t c o n s i d e r -
a b l y a s e x p e r i e n c e i s ga ined and throughput i n c r e a s e s .
Gas t e m p e r a t u r e s today a r e i n t h e r e g i o n of 75OOC. and I should t h i n k
f o r t h e steam r a i s i n g HTR these c o u l d rise t o 8 O O O C . and l e v e l o f f a t t h a t
v a l u e . I can see no reason t o d e p a r t from t h e s u b - c r i t i c a l s team c y c l e
w i t h t e m p e r a t u r e s , a s today, a t 538OC. There i s no doubt t h a t t h e s t a t i o n
o u t p u t can be doubled wi thout any t e c h n i c a l d i f f i c u l t y , and i n f a c t , you
a r e a l r e a d y propos ing t h i s i n t h e United S t a t e s .
With i n c r e a s e s i n g a s p r e s s u r e fr'om 60 b a r t o 80 b a r , I would e x p e c t
w e s h a l l r a i s e t h e c o r e power d e n s i t y from 8kW/litre t o lOkW/ l i t r e , bu t
these p r e s s u r e s and power r a t i n g s w i l l , I t h i n k , be l i m i t i n g . A t t h e same
t i m e , of course , t h e f u e l r a t i n g w i l l be i n c r e a s e d from 80 MW/Te t o 100
MW/Te. I t h i n k t h e i n c e n t i v e t o r a i s e thermal e f f i c i e n c y w i l l n o t be v e r y
g r e a t and i t w i l l remain a t f i g u r e s which a r e c u r r e n t today.
The g a s - t u r b i n e v a r i a t i o n of t h e h i g h tempera ture r e a c t o r I can see
w i l l have an i n t e g r a l d e s i g n a t 80 b a r and t e m p e r a t u r e s r a n g i n g from 8 5 O O C .
t o 900OC. Again t h e i n c e n t i v e s , i n my view, t o go much beyond t h i s temp-
e r a t u r e a r e n o t v e r y g r e a t . The development c o n t e n t of the r o t a t i n g com-
ponents of a g a s - t u r b i n e h i g h t e m p e r a t u r e r e a c t o r i s so h i g h t h a t t h e y
w i l l have t o be des igned and manufactured on a q u a n t i t y b a s i s , a s i n t h e
a i r c r a f t i n d u s t r y . For t h i s reason one o r , a t t h e most, two s t a n d a r d
compressor t u r b i n e d e s i g n s w i l l have t o be adopted. I t h i n k a u n i t of
300 MW would s e r v e v e r y w e l l and t h e s e c o u l d be a s s o c i a t e d w i t h power
t u r b i n e u n i t s of 600 MW t o remain r e a s o n a b l y w i t h i n t h e t e c h n i c a l l i m i t a -
t i o n s of m a t e r i a l s and test f a c i l i t i e s .
There i s one f u r t h e r system of which w e have s a i d l i t t l e a t t h e
moment. T h i s i s t h e gas-cooled f a s t r e a c t o r , f o r which I t h i n k g a s
p r e s s u r e s of 120 b a r w i l l be j u s t i f i e d . A t such p r e s s u r e s a c o r e power
d e n s i t y of 300kW/litre w i l l be o b t a i n a b l e and g a s t e m p e r a t u r e s should
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776
be about 8OOOC. a s f o r t he steam r a i s i n g HTR. n
On t h e commercial s i d e , I t h i n k t h e s i t u a t i o n i n Europe i s c l e a r l y
d i f f e r e n t from t h a t i n t h e United S t a t e s . W e have q u i t e a number of
groups working i n t h e f i e l d a t t h e moment and t h e r e w i l l be a need for
more c o l l a b o r a t i o n , p a r t i c u l a r l y on f u e l des ign , both wi th in t h e UK and
through Europe. The i r r a d i a t i o n f a c . i l i t i e s i n f u e l des igns i s so h igh
t h a t w e must c l e a r l y make every e f f o r t t o evolve one common f u e l design
which can be employed i n d i f f e r e n t r e a c t o r conf igu ra t ions .
I a l s o b e l i e v e t h e r e i s n o t room f o r more than two des ign groupings
i n Europe. There must be two i n o rde r t o s t i m u l a t e competi t ion, but i f
t h e r e a r e t o o many t h e t e c h n i c a l e f f o r t w i l l be spread too t h i n l y and t h e
r e a c t o r des igns w i l l s u f f e r . Co l l abora t ion i s r e l a t i v e l y ea sy i n t h e
s tudy phase when only small sums of money a r e being spent . A v e r y good
example i s t h e GBR Assoc i t ion i n B r u s s e l s , where e x c e l l e n t communications
have been e s t a b l i s h e d wi th a l l design and experimental workers i n t h e i r
f i e l d a c r o s s many n a t i o n a l borders . But t h i s i s a f a i r l y loose a s soc ia -
t i o n . Permanent groupings of t h e va r ious o rgan iza t ions i n t h e f i e l d ,
capable of spending s u b s t a n t i a l sums of money, w i l l on ly come c l e a r when
one or two s p e c i f i c power s t a t i o n s have t o be committed,
Contrary t o Dr. Rickard speaking on t h e U.S. s i t u a t i o n , I t h i n k
t h a t i n Europe t h e r e i s a need f o r more c o l l a b o r a t i o n on f u e l manufacture,
Whereas some competi t ion may be r equ i r ed he re , I t h i n k t h e r e a r e f i v e
groups a t p re sen t i n Europe, and they c l e a r l y cannot a l l compete economi-
c a l l y f o r t h e r e l a t i v e l y small number of o r d e r s t h e r e w i l l be i n t h e next
t h r e e or f o u r years .
3 b e l i e v e t h a t i n f i v e y e a r s ' t i m e order:; f o r h igh temperature
r e a c t o r s w i l l begin t o be placed a s r o u t i n e i n preference t o o t h e r
systems and i t w i l l then be t h e t u r n of t h e f a s t r e a c t o r s t o cha l lenge
t h e p o s i t i o n they have e s t a b l i s h e d . I t h i n k success fu l work on t h e gas-
cooled f a s t r e a c t o r could r e s u l t i n t h e s t a r t on cons t ruc t ion of a proto-
type r e a c t o r providing, of course , governments can f i n d money f o r t h e
p r o j e c t .
about i f some c a l c u l a t e d r i s k s a r e taken, so t h a t e a r l i e r p r o j e c t s g e t
under way and exper ience i s gained a s qu ick ly a s poss ib l e .
Th i s i s a f a i r l y buoyant p i c t u r e , but one which w i l l on ly come
777
0 Karl W i r t z , Karlsruhe
It i s gene ra l ly agreed upon t h a t f o r a n ultimate success of nuc lea r
power product ion breeding w i l l be necessary.
types of b reede r r e a c t o r s - thermal breeders and fas t breeders . no economic thermal power r e a c t o r i s a b l e t o breed, and no proposal has
been made f o r a n economic thermal power b reede r r e a c t o r . It i s not i m - poss ib l e t h a t advanced concepts l i k e t h e Molten S a l t type f i n a l l y w i l l
prove f e a s i b l e f o r economic thermal breeding.
economic thermal breeding would be a major breakthrough and would have
cons iderable advantages compared t o fast breeders .
It m y be obtained by two
So far,
There i s no doubt t h a t
Many s t u d i e s have shown t h a t fast breeders have t h e p o t e n t i a l t o
become economically competi t ive wi th present-day and f u t u r e power con-
v e r t e r s , f o r ins tance , wi th t h e LWR and HTGR types .
The major e f f o r t on FBR's a l l over t h e world i s concentrated on sod-
i u m cool ing, mainly because a t t h e t i m e when t h e s e programs were s tar ted
sodium w a s t h e appropr i a t e choice.
The fo l lowing f a c t s have changed t h i s s i t u a t i o n i n r e c e n t yea r s :
1.
2. The use of p r e s t r e s s e d concrete v e s s e l s f o r gas-cooled r e a c t o r s
3. The f a c t t h a t l a r g e and economic resources of helium became
The development of helium-cooled r e a c t o r technology f o r HTGR's
a v a i l a b l e i n t h e n a t u r a l gas sources , for i n s t ance i n Europe.
4. The p o s s i b i l i t y t o use i n a first gene ra t ion the s a m e b a s i c pin-
type f u e l f o r bo th types of fas t r e a c t o r s under t h e same tern- ' pera tu re condi t ions .
Fu r the r a s p e c t s of gas cool ing for FBR's p o i n t t o a f u t u r e second
genera t ion . The i r p o t e n t i a l i s h ighe r temperatures , t h e poss ib l e use of
gas tu rb ines , and l as t b u t no t l e a s t , t h e h igh thermodynamical e f f i c i e n c y
wi th lower percentages of waste h e a t combined wi th t h e p o s s i b i l i t y of
cool ing a g a i n s t a i r i n s t e a d of water, and thus avoid ing t h e h e a t po l lu -
t i o n problems of r i v e r s on many in l and s i tes .
The GCFBR based on present-day fue l p i n development p re sen t s prl-
mar i ly problems of' c o r r e c t des ign of t h e primary h igh-pressure (-trc:S:
778
There are many arguments t h a t t e c h n i c a l l y it poses problems t h a t are not of a p r i n c i p a l cha rac t e r and should be solved by s t r a igh t fo rward designs.
All s a f e t y problems can be analyzed adequately. The sodium-cooled FIBR, on the o t h e r hand, u n t i l today poses p r i n c i p a l des ign problems connected w i t h t h e in t ima te i n t e r a c t i o n of t h e coolant w i t h t he neut ronic behavior o f the core.
Recent eva lua t ions seem t o i n d i c a t e t h a t even a t equal su r f ace t e m -
pe ra tu re s of t h e oxide f u e l pin, and wi th corresponding steam temperatures, t h e GCFBR o f f e r s the same or even lower c o s t s pe r k i l o w a t t hour than the
sodium-cooled? FBR, mainly because o f lower c a p i t a l cos t s .
1.
2.
3 .
4. 5. 6 .
These favorable a s p e c t s of gas-cool ing of FBR's have s t imu la t ed sev-
e r a l s tudy programs i n Europe as w e l l as i n t h e United S t a t e s . These studies are supported by government laboratl3riesy manufacturers and utili-
t i e s , b u t so far t h e money involved i s only a small percentage of t h e m o u n t spen t for sodium-cooled FBR's. would be mis leading w i t h r e s p e c t t o the resillts of these s t u d i e s , be- cause, as w e mentioned before , the GCFBR p r e s e n t l y can r e l y heav i ly on t h e two major e f f o r t s , t h e HTGR and NaCFBR. This under l ines t h a t it i s
appropr i a t e t o cons ider gas cool ing as j u s t one of the competi t ive cool-
i n g p o s s i b i l i t i e s t o a t t a i n the common goa l - fast breeder r e a c t o r s .
On t h e o t h e r hand, t h e percentage
What has t o be done i n coming y e a r s ? The prospec ts o f GCFBR's cer- t a i n l y j u s t i f y t h e p re sen t modest r e sea rch programs tha t w i l l hope fu l ly
be increased i n coming years . Examples f o r such programs are: Cer t a in h e a t t r a n s f e r s t u d i e s as are going on, f o r ins tance , i n Karlsruhe
The development of higher temperature cladding materials, f o r in s t ance , o f t h e Vanadium a l l o y type and of the advanced s t a i n -
less s t e e l types The development of coated p a r t i c l e s for high fas t f l u e n t e s and t h e research on promising cermets
The r e sea rch on p r e s t r e s s e d concre te vessel des igns
Carbide f u e l development t h a t i s of equal i n t e r e s t t o NaCFBR S tud ie s on a c t i v e and pass ive engineered safeguards, e t c .
779
Moreover, in the coming years there probably will be the strong de-
sire to include a gas-cooled fast breeder reactor prototype power plant
in the present development programs. As we have seen, this is well jus-
tified. In view of the fact that at least five to six major nations are
considering the construction of a prototype sodium-cooled FBR, it should
not be impossible to invest some money to further the later arrived com-
petitor who seems to be equally promising.
would seem to be particularly appropriate. It would make economic sense
for everyone, as it would ensure production of information necessary to
enable both systems to be judged on their economic and safety merits. It
would also comply with the responsibilities of the nuclear community con-
cerning the ultihate goal - a safe and economic FBFL This could be ac-
complished best by developing both coolants. It would also create com-
petition between the manufacturers and give the utilities a chance to
select the type they liked best.
International cooperation
780
FLOOR DISCUSSION
H Kr'ber: I would l i k e t o make some ve ry gene ra l remarks because - a l l the t e c h n i c a l and f i n a n c i a l d e t a i l s w e go t by t h i s e x c e l l e n t presen-
t a t i o n by our p a n e l i s t s , and I would l i k e t o add some very gene ra l remarks.
We a l l followed t h i s meeting, and w e go t a review on t h e work which has
been done i n the d i f f e r e n t o rgan iza t ions on t h e HTR f i e l d . I th ink w e a l l
go t t h e impression t h a t t h e HTR i s now ready from t h e view of t h e develop-
ment work; t h a t now w e can env i s ion t h e phas2 of commercializing thF HTR
system. I th ink we a l l ag ree wi th t h i s now, b u t what has t o be done f o r
e n t e r i n g t h i s commercial pace? I th ink , t h e r e are two main dec i s ions .
One i s t h a t t h e u t i l i t i e s w i l l engage wi th t;iis system and a l s o t h a t t h e
u t i l i t i e s would make dec i s ions . The u t i l i t i e s w i l l have t o t r u s t i n t h e HTR, and w e hope t h a t w i l l be done i n t he next years . The u t i l i t i e s , they
have t o say t h a t t hey w i l l i n t end t o spend t h e money which i s necessary
t o make t h e work on i n d u s t r i a l s c a l e f o r fur- ther developing a l l t h e de-
t a i l s , a l l t h e components which are necessary when in t roduc ing i n t o the
commercial pace, and w e a l l know t h a t t h i s w i l l c o s t q u i t e a l o t of
money. Now what i s t h e s i t u a t i o n ?
I would l i k e t o make ano the r s ta tement Tor, t h a t i s , w e a l l b e l i e v e
t h a t t h e HTR has ve ry good presumptions t o be in t roduced i n t h e energy
market because of s e v e r a l reasons. We know t h a t t h e t e c h n i c a l problems
are a t least i n p r i n c i p l e solved, and they are less t han i n o t h e r reac-
t o r systems, I would say. The economics a r e q u i t e w e l l f o r t h e HTR sys-
t e m . The s a f e t y i s a l l r i g h t s o f a r as w e kr!ow today. The sum of poll^-
t i o n i s be t te r than i n o t h e r systems, and w e a l s o hope t h a t a v a i l a b i l i t y
i s q u i t e w e l l w i th t h i s system, because as we have a l r e a d y heard, t h e
a c c e s s i b i l i t y i s q u i t e good f o r t h i s system, t h e primary c i r c u i t i s q u i t e
pure, a t l eas t as w e know it today. There i s a l s o a b i g development
p o t e n t i a l , and w e have heard about t h e HTR steam cycle , d i r e c t cycle ,
gas-cooled fast breeder , and t h e r e i s process hea t , and i f I may go fur-
t h e r , t h e r e i s a l s o fus ion . We a l l know t h a t helium technology w i l l h e l p
a l s o i n t h i s f i e l d . You see t h e r e i s a very s t r a i g h t l i n e concerning t h e
f u t u r e development p o t e n t i a l . Now I w i l l come back t o t h e s e dec i s ions
*
I
I
0 which w i l l have t o be made on the s i d e of t h e u t i l i t i e s and the companies.
I n t h e United S ta t e s , t he companies . . . have made a c l e a r dec is ion 8 s fa r
as I learned here. They w i l l spend t h e money which i s necessary t o i n t r o -
duce t h i s system, and what w e hope t h a t a l s o t h e u t i l i t i e s i n t h i s country w i l l t r u s t i n t he system and make the r i g h t decisions. In t he United
Kingdom, I a m r a t h e r sure t h a t t h e decisions w i l l a l s o be made wi th in the
next yem. I n t h i s country, I th ink things a r e much e a s i e r than i n t h e
United S ta t e s , and e spec ia l ly i n Germany, because there , t he re i s a long
t r a d i t i o n i n gas-cooled systems. There i s a l o t of experience i n con-
s t r u c t i o n of these kind of r eac to r s , and therefore , w e can be hopeful t h a t
within t h e next year the decisions which I mentioned w i l l be made i n
England. I n Germany, I th ink we a r e not y e t as far. The work i s s t i l l
not set by OUT companies, and we have a l s o t o convince a b i t more of OUT
u t i l i t i e s . We w i l l do our bes t , of course, bu t I th ink t h a t an in te rna-
t i o n a l cooperation, which you a l l mentioned, would he lp th ings very much
and I hope t h a t what you sa id can be r ea l i zed i n the next year, and i f I may make a prospect f o r t h e next year, it i s then t h i s :
t he re i s a b i g p robab i l i t y t h a t within t h e next year t he re w i l l be a de-
c i s i o n whether we w i l l overcome the b a r r i e r t o t h e commercial phase or
we w i l l not.
That I think
P. Fortesque: F i r s t of a l l I would l i k e t o say how much we welcome
Professor W i r t z ’ s remarks. I think a few more voices l i k e t h a t would do us a l o t of good.
r a t h e r broad point about t h e gas-cooled fast r e a c t o r which I think tends
t o be a l i t t l e obscured. A t meetings l i k e t h i s , one hears a g rea t dea l
about projected m i l l s per k i lowat t hour, conversion r a t i o s , and heaven
knows what f o r t he year 1990.
t he whole ingredient. I thlnk i f t h a t were t r u e w e would a l l have nothing
but homogeneous aqueous r eac to r s today. I th ink a very important f ea tu re determining whether v a s t sms of money a r e going t o be expanded by u t i l i -
t i e s on huge p lan ts , a very necessary ingredien t , w i l l be the record of
those p lan ts looking back a t them. Now, i n order t o form such an opinion
you m u s t have a record of more than one type of p lan t t o form t h a t opinion
upon, and the point I wish t o make i s t h a t t o o much preoccupation, ex-
c f l l e n t though a l i t t l e b i t is , too much preoccupation with m i l l s per
What I r e a l l y rose t o say w a s , I wanted t o r a i s e one
Now a l l of t h i s kind of s t u f f i s far from
I
782
k i l o w a t t hour can be obscure. One very good po in t and reason f o r advo-
c a t i n g t h e pursuing of two d i f f e r e n t b reedem i s t h a t only by pursuing
two d i f f e r e n t breeders w i l l i n d u s t r y be a b l e t o accumulate t h e s t a t i s t i c s
necessary t o r e a l l y judge how long those b reede r s w i l l remain on l i n e ,
and i r r e s p e c t i v e of what t h e u l t ima te answer is, a most important degree
of freedom i s taken from t h e users i f he i s only presented wi th one choice
t o make; you have i t or you don ' t . There i s ; one o t h e r s l i g h t l y r e l a t e d
po in t I would l i k e t o m a k e , I th ink , whi le I have got ( t h e microphone).
I not iced Jimmy Lane remarked i n t h e opening t h a t , I th ink he used the
phase, "HTGR i s a s t epp ing s tone t o t h e GCFF:. Well, i n context t h a t i s f i n e , b u t perhaps t h a t i s open t o a l i t t l e mis rep resen ta t ion i f t h a t i s
taken t o mean t h a t w e on ly r ega rd t h e HTGR as a s tepping s tone f o r fast
r e a c t o r s . h r from t h e case; i n f a c t , t h e HTGR i s jus t as much, and even more, bene f i t ed by the coexis tence of breeders as t h e l i g h t water r e a c t o r .
The l i g h t water r e a c t o r s have t h e b e n e f i t of a s ink f o r t h e i r garbage,
t h e Plutonium.
f i t s v a s t l y from t h e f a c t t h a t t h e breeder program, be it gas cooled or
sodium, could i n p r i n c i p l e produce Uranium 233 i n i t s b lankets , and t o
b e n e f i t t o t h e HTGR from use and excess . The 233 i s f a r more than t h e
b e n e f i t of a garbage d i s p o s a l f o r Plutonium and t h e reason goes far be-
yond j u s t t h e physics . We a l l know about t h e physics of t h e b e t t e r f u e l
233. What r ece ives far less a t t e n t i o n i s t h e b e t t e r hea t ing t r a n s f e r
p r o p e r t i e s . Now t h a t i s a n ex t r ao rd ina ry s ta tement , b u t what I mean i s
t h a t t h i s t h e f u e l volume occupancy requirements of U233-fueled HTGR
are much lower than those of a 238 f u e l , l eav ing a much more area f o r
t h e cool passage, and you can g e t very much b e t t e r r a t i n g s indeed wi th
233; so w e regard t h e two p r o j e c t s no t as r i v a l s for 1990 model, b u t as
coex i s t en t , he lp ing , symbiotic, whatever i t is you c a l l them.
The HTGR doesn ' t j u s t provide a sink for garbage, it bene-
B. Chapman: We have had a l o t o f papers i n t h i s meeting on opt imi-
za t ion , b u t a l l o f them, I th ink , have been concerned wi th s teady s ta te .
Now, one of t h e th ings I th ink everybody ag rees on i s a gene ra l i nc rease
i n u n i t s i z e , and what t h a t b r ings wi th it is, t h e problem of t h e fas t
load pickup when you l o s e one s t a t i o n o f f the g r i d .
committed HTR man myself , b u t I b e l i e v e i n th .e philosophy of "know t h i n e
@ enemy," and I think the saturated water systems do have perhaps an e a s i e r
route t o t h i s fas t load pickup problen;. I wonder i f the panel can comment on whether they think t h a t t h i s s o r t of consideration would ser ious ly in- fluence the course of development t o the KTK.
R. Vaughan: I think I could anser that with a question. What par-
t i c u l a r f e a t u r e of the HTGR i s it you f e e l may hamper i t s a b i l i t y t o pick up load and t o b e t t e r other systems?
B. Chapman: Well, I think a t f irst s i g h t one might f e e l t h e reserve provided i n the system by a l a r g e amount of saturated water, and the a b i l i t y t o pick up load by simply dropping pressure would on the face ap- pear t o be an advantage f o r the wet steam system. th i s with the HTGR, you have got t o pick it up p r e t t y w e l l s t r a i g h t from t h e core i t se l f , and t h i s would have q u i t e sharp implications on f u e l de-
sign, I would think.
If you intend t o do
C. Rickard: Yes, I j u s t might say a th ing here. I think the design that w e a r e offer ing, and it i s a l s o t h e case with t h e Colorado PSC, i s designed t o be ab le t o pick up about 5% per minute load v a r i a t i o n and t h a t i s the normal requirement of the systems, and w e haven't i n discussions
with the u t i l i t i e s have not got ten a feed back, a l a r g e advantage i n ex-
cess of that; and the 5% per minute, it seems t o be about normal w i t h con- vent ional plants and t h e i r s i s probably l i m i t e d by turbine temperature changes, and so w e are w i t h the HTGR, w e are f i t t i n g i n t o a normal pa t te rn
tha t has been establ ished previously throughout the country, s o I don't
think t h a t w i l l have an l i m i t i n g e f f e c t on HTGR plant appl icat ion.
R. Vaughan: It i s t r u e w e have made l i f e a l i t t l e more d i f f i c u l t f o r ourselves than it used t o be on t h e Magnox s t a t i o n s by using once- through b o i l e r systems. When w e had natural c i rcu la t ion boi le rs , we had
a reservoi r of the type you were ta lk ing about, and w e have l e t that go i n order t o g e t the economies i n i n t e g r a l design.
taken, I think.
So your point i s well
C. Zitek: What has Peach Bottom's experience been i n load pickup
a b i l i t y ?
784
C. Rickard: I think t h a t Peach Bottorl., when i t ' s operating, has
been b a s i c a l l y base loaded, but it i s a p lan t t o follow load, bu t as far as I know Peach Bottom i s capable of a t least a 3% per minute load change and i t ' s been a b l e t o do t h a t .
P. Fischer: I had seve ra l discussions i n Europe on t h i s top ic . A s far as Peach Bottom i s concerned I think one has t o d i s t ingu i sh between t h e rate which may be a programmed rate increase , and what kind of s t e p
changes it can take, and I th ink Peach Bottom has gone through some rather rough s t e p changes on the system of the Philadelphia E l e c t r i c Company. I t ' s too bad John Kemper i s n ' t here, I think he could give the
d e t a i l s on that . I think, generally, t h a t Peach Bottom can pick up r a t h e r reasonable s t e p changes i n loads without any b i g disturbances t o the temperature, pressure, and key parametem. I think as far as support-
i n g water r eac to r s i s concerned, I th ink , the i n t e r e s t i n Europe i s t o change somewhat f a s t e r than here, bu t I th ink the poin t i s a s a l e s po in t tha t has been maybe a l i t t l e overstated; these 28 per second tha t are
sometimes quoted f o r t h i s sytems a r e over a l i m i t e d range. I t ' s more compared t o a s t e p change, almost, a t tha t ]*ate over say, 30$ load. th ink t h i s i s not w h a t t h e normal g r id w i l l require. I th ink it i s de- signed, it could probably be designed, t o t h e c u s t m e r requirements. I
think, as Rickard said here, I think it i s 3 t o 5%. It might be i n t e r - e s t i n g t o hear whether i n the United S ta t e s , from the u t i l i t i e s s ide , t h e increase t h a t i s expected.
-
I
C. Zitek: I s t i l l th ink t h e l imi ta t ior ! i s on t h e turb ine generator un i t . Water r eac to r s w i l l pick up load as fas t as you want r e a l l y . We have done t h i s . new i n t h i s gas cooled b i t . I a m l ed t o be l i eve t h e waste d isposa l prob-
lem i s much less i n a gas-cooled than i n a water-cooled. not heard that t h i s i s an advantage i n t h e gas-cooled. human cry tha t we have about rad ioac t ive discharge i n t he environment, here i n the S t a t e s a t l e a s t , it would be d e f i n i t e l y t o your advantage t o design a p lan t that has e s s e n t i a l l y zero a c t i v i t y r e l e a s e t o the environ-
ment. I have been pushing f o r t h i s i n the LFMBR's, arL the companies i n - d i c a t e t ha t yes, they could probably do t h i s . Have t h e gas-cooled people thought of doing t h i s as a s e l l i n g po in t?
I have another po in t I want t o br ing in . I a m f a i r l y
S t i l l , 1 have
With the b i g
785
C, Rickard: Yes, I w i l l answer tha t one. It c e r t a i n l y i s an advan- tage i n t h e sense that t o g e t very much lower l e v e l r e l ease , it doesn ' t cos t as much t o ge t them b o t t l e d up and then shipped o f f - s i t e so t h a t you can t u r n tha t advantage i n t o r e a l d o l l a r s i n p l an t construct ion, and we have i n the case, we have now of fered an opt ion going with t h a t t h a t pro- v ides f o r a waste gas system and a l i q u i d waste system, s o that t h e d i s -
charge from the p l an t t o the environment around us i s very, very low, very, very low. Much, much lower than cur ren t discharge l e v e l s .
A. Goodjohn: The gas-cooled r eac to r , of course, doesn ' t generate a l o t of s o l i d and l i q u i d waste. Most of our wastes a r e i n the form of gases, and I want t o comment f i r s t of a l l on the f i s s i o n products. The gaseous f i s s i o n products are removed by a means of a p u r i f i c a t i o n system. I denoted that i n my t a l k on Monday. This p u r i f i c a t i o n system takes about 108 of t h e primary coolant per hour through it and then r e tu rns t h e pur i -
f i e d helium t o t h e PCRV. That p u r i f i c a t i o n system removes t h e dus t , and removes the gaseous d i f f u s i o n product by a means of . . . cold t rapping, and removes t h e hydrogen and tritium by means of a t i t an ium sponge. Now these products normally a r e removed by means of a gas waste system. That
i s , when we have t o regenerate t h a t p u r i f i c a t i o n system. Normally we put the products from our he l iun p u r i f i c a t i o n system i n t o a gas waste
tank, and l e t it go t o the atmosphere under cont ro l led meterological con- ditions. Now i n our opt ion t h a t we a r e providing here , we a r e essen- t i a l l y tak ing the material from our p u r i f i c a t i o n system. s p e c i f i c a l l y of our long-l ived f i s s i o n products, s p e c i f i c a l l y Krypton 85 , w e a r e t ak ing it and pu t t ing it r i g h t back i n t o the PCRV. With t h a t lO$ of t h e primary coolant pe r hour going through the p u r i f i c a t i o n system, t h e Krypton 85 w i l l simply bu i ld up and be r e t a ined i n t h e low tempera- t u r e t r aps . There w i l l be no r e l e a s e of Krypton 85 except as made by t h e normal leakage of containment helium from t h e PCRV. We expect t h a t would
Speaking now
be very, very small, very, very small. Inso fa r as tritium i s concerned - @gain now, when we regenerate t h a t temperature t r a p , normally we would
put it i n the gas waste tank and put it up the s t ack under cont ro l led
meterological conditions. With our zero-pol lu t ion option, we w i l l t ake that t r a p and regenerate it through a n oxid izer and make t r i t i a t e d water.
786
That i s one way t o do it. It then becomes a very concentrated l i q u i d
waste - t r i t i a t e d water, w e , i n f a c t , do not even have t o do that. That
tritium sponge i s r ep laceab le simply by t ak ing it o u t and r ep lac ing it wi th a new sponge. So t h a t , i n f a c t , w e dc) no t have t o r e l e a s e any tri- t i u m t o atmosphere from our p u r i f i c a t i o n system. There w i l l be a small
l e a k of tritium probably, a g a i n from a smal.1 leakage i n t h e PCRV, b u t w e expect t h a t would be very small.
C. Z i t ek : A r e you going t o be able t o measure leakage from t h e con-
ta inment?
A. Goodjohn: That i s always very hard t o do. We designed our con-
tainment t o be subatmospheric, s l i g h t l y , by jus t a f e w inches of water dur ing normal opera t ions . I do not expect t h a t we w i l l g e t ve ry much
leakage from t h e containment.
M. W l l e Donne: I would l i k e t o make more of a comment r a t h e r t han
a ques t ion . I t h i n k t h a t t h e h igh temperature thermal r e a c t o r would have
t h e i n t r o d u c t i o n of t h e gas-cooled b reede r i n r e s p e c t t o t h e sodium cool
breeder f o r t h e fo l lowing reasons : It i s o f t e n s a i d t h a t t h e main advan-
t a g e of t h e sodium breeder i n r e s p e c t t o t h e gas-cooled breeder i s the
smaller des ign inventory . It seems r a t h e r d i f f i c u l t w i t h t h e gas-cooled
breeder t o have a plutonium inventory as s m a l l as t h a t one which i s pos-
s ib le w i t h sodium. This smaller inven to ry would h e l p t h e i n t r o d u c t i o n
o f a sodium b reede r because w i t h a l i m i t e d amount of plutonium coming
from t h e l i g h t water r e a c t o r , f o r ins tance , it i s poss ib l e t o make more
r e a c t o r s wi th smaller inven to r i e s ; b u t i f t h e h igh temperature thermal
r e a c t o r i s one e n t e r i n g i n t o t h e market ve ry s t rong ly , t hen t h e amount of
plutonium a v a i l a b l e for t h e breeder , of coume, w i l l be less and t h e i n -
t r o d u c t i o n of fast r e a c t o r s w i l l be dependent upon t h e doubl ing time r a t h e r than t h e inven to r i e s . I n t h i s case :I: t h ink t h e gas-cooled breeder
w i l l have a n advantage i n r e s p e c t t o t h e sodium breeder , because I t h i n k
t h a t it i s q u i t e l i k e l y t h a t t h e doubl ing t i m e for t h e gas breeder would
be b e t t e r than f o r t h e sodium breeder .
J. Lane: Ac tua l ly i n connect ion wi th the s p e c i f i c inventory our
s t u d i e s show t h a t t h e gas-cooled breeder had! t h e same s p e c i f i c inventory A
787
0 as t h e reference LFMBR, but was a f a c t o r o f 50 t o 80% higher than the
advanced systems; but there is an advanced gas system t h a t a l s o has a
low inventory. The difference i s n ' t t h a t g rea t , i n other words.
D. Tytgat: I have some comments which may be complementing, but
f i rs t of a l l I think w e a l l agree speaking from the European community,
about what has been said by Dr. Krgmer about the fu ture of the HTR. We conclude t h a t t h i s i s a reactor which has E!. high poten t ia l , and we cer- t a i n l y welcome future in te rna t iona l collaboration i n a l l f i e l d s .
could even comment t h a t we a r e always speaking i n i t i a l l y with collabora-
t i o n i n Europe, but a t Euratom w e have excel lent col laborat ion with
USAEC. by having an extensive water-cooled reactor exchange of information,
which I think had a grea t impact on the whole European s i tua t ion .
some small comments on some of the points ra i sed during the meeting;
c e r t a i n l y f o r the matter of prestressed concrete pressure vessel which i s
one of the key new developments i n the U.S., I agree with the words of other colleagues. We cer ta in ly believe i n these pressure vessels i n
Europe, by t h e number of vesse ls which have been b u i l t .
osophy of the United S ta tes f o r the moment i s t o use secondary contain-
ment.
about the ins ta l la t ion , about which we heard from M r . Vaughan, which might be one way t o r e a l l y be sure t h a t a prestressed concrete pressure vesse l has r e a l l y f u l l securi ty . Another point i s concerning the fue l . I had
the impression there might have been i n t h e introduct ion some confusion due t o t h e d i f f e r e n t presentat ion i n t h e f u e l session. That means some presentations were more on f u e l spec i f ica t ion t e s t s , while some other
papers concentrate on f u e l developments. Let us say a t Euratom w e cer-
t a i n l y believe completely i n the excel lent behavior of t h i s coated-
p a r t i c l e fue l , and certai.nly we completely agree on t h e Dragon s i d e too;
and w e have been q u i t e impressed by the work done i n the United S ta tes
on the coated-particle matrix, and the graphite i r r a d i a t i o n r e s u l t s .
A s was pointed out, there may be s t i l l a small gap t o be f i l l e d , but it w i l l be f i l l e d very soon about t h i s s o r t of large-block i r rad ia t ion , but
w e have f u l l confidence tha t they w i l l confirm a l l the p a r t i c l e calcula-
t i o n s up t o now.
We
Previously we could say even t h a t maybe we introduced competition
I have
Maybe the phi l -
Maybe the European philosophy might be more t o take great care
I have one point t o mention maybe on the guarantee.
788
It 'was much i n the d iscuss ion about t h i s guarantee given by Nukem for
the f i r s t 30C megawatt THTR.
s en ta t ives , t h i s may be having some relevance o r meaning, bu t I should
say t h a t we have been working f o r a very long time with Nukem, and we
know t h a t i f they are ready t o give a guarantee, t h a t they r e a l l y be l ieve
and f e e l i t ' s pe r fec t and w i l l g ive a l l s a t i s f a c t i o n t o the e l e c t r i c i t y
producer. Take AVR, which was a very s p e c i a l concept, and the f a c t t h e AVR i s working p e r f e c t l y and going
t o (a 300 megawatt ve r s ion ) proves t h a t even if some p a r t i c u l a r problems were introduced by t h e HTR, they have a l l been solved i n a very s h o r t
time, as a l s o mentioned by t h e panel; and we c e r t a i n l y agree t h a t t h i s
proves t h a t even i f t h e r e are some component developments t o be made, as
Dr KrGner sa id , a l l those problems w i l l be solved.
While maybe for some of t h e American repre-
There a r e o the r po in ts on technology.
R. Huddle: Could 1 jus t b r ing t o your no t i ce a modern ve r s ion o f an
o ld Dragon p ro jec t proverb. One experimental result i s worth a thousand
computer ca lcu la t ions .
J. Bugl: While we have been s i t t i n g here now toge ther f o r t h r e e
days i n a r a t h e r pure environment as we a r e used t o . What I want t o
say i s t h a t w e a r e s i t t i n g toge ther among the family of high temperature r e a c t o r people. Now t o ge t through t o develop such a system, of course,
it needs q u i t e an amount of publ ic money and it needs, of course, a l s o
t h e customer, so i s it s t i l l permitted t o ask, say a r ep resen ta t ive of
t h e USAEC and perhaps a r ep resen ta t ive of a customer o f a u t i l i t y u t i l i -
t i e s t o say a f e w words on what impression they had on our meeting.
R. Pahler : F i r s t of a l l I a m more i d e n t i f i e d wi th t h e HER, I
think, than the AEC; s o I would l i k e t o say t h a t t h e program we a r e
sponsoring on gas-cooled r eac to r s , w e a r e spending $3,000,000 i n 1971 on
our base program, mainly or ien ted f o r f u e l development. We a r e spending
$2,000,000 on formulizat ion which i s our recycled program.
not an announcement, b u t I want t o make a s ta tement which Corwin (Rickard)
r e f e r r e d t o on our U233 buyback pol icy statement was issued.
extend the guaranteed purchase p r i c e f o r U"'?
Now t h i s i s
W i l l it This i s a publ ic r e l e a s e
issued about a month ago, and t h i s i s the Canmission speaking and not
Pahler : "In add i t ion t o guaranteeing the purchase p r i c e of U 2 3 3 , t he
789
@ AEC conducts a research and development program which provides support
f o r t h e high temperature gas-cooled r e a c t o r concept. The AEC budget r e -
ques t f o r the f i s c a l year 1971 provides f o r cont inua t ion of i t s develop- ment e f f o r t s on t h i s r e a c t o r system. Recognizing i t s promise of e f f i c i e n t f u e l u t i l i z a t i o n , high temperature e f f i c i ency , and improved environmental condi t ions over e x i s t i n g r e a c t o r s (and I make tha t s ta tement s p e c i f i c a l l y
back i n the corner w i t h r e spec t t o water r e a c t o r s ) , the AEC plans t o con-
t i n u e support f o r t h e HTGR beyond f i s c a l '71, wi th in t h e l i m i t a t i o n s , of course, of t h e a v a i l a b i l i t y of funds. Through 1977 t h e AEC w i l l accept and m a k e f i n a n c i a l se t t lement f o r HER f u e l s i f commercial reprocessing
is not ava i l ab le . Consideration w i l l also be given to the need for a fur- t h e r ex tens ion of t h i s po l icy a t a l a t e r date ."
refers t o a published p r i c e t h a t w e are coming out with, for reprocessing HTGR f u e l s similar t o what w a s done f o r l igh t -water r eac to r s . I don ' t
know whether it i s i n t h e publ ic record ye t , but it i s soon t o be an- nounced publ ic ly .
Now t h i s l as t s ta tement
L. Graham: I don' t want t o f i n i s h on a f ace t ious note , bu t I wonder whether t h e panel would state what t h e p r o b a b i l i t y of a U.S. r e a c t o r being so ld i n t h e United Kingdom or i n Europe i s i n t h e next 10 years and v i ce versa .
C. Rickard: I think tha t there is c e r t a i n l y always t h a t p o s s i b i l i t y . I think tha t the whole HTGR program is moving forward in a s p i r i t of
cooperat ion and i n the For t St. Vrain r e a c t o r t h e r e a r e a number of com-
ponents which have come from Europe and w e t h ink wi th poss ib ly the bu i ld - i ng of HTGR i n Europe tha t might r ec ip roca te a b i t sometime i n the fu tu re , b u t I think that the main job a t hand i s t o g e t t he f i r s t b i g one s ta r ted .
R. Vaughan: Agreed. No r e a c t o r i s b u i l t i n another country, It i s
b u i l t i n the country on which the ground where it rises from t h e ground. Some features o f i t s des igners , as Rickard has j u s t s a id , may come from
somewhere else, but s t i l l t h e r e a c t o r i s always indigenous a t the end of
t h e day.
K. Wirtz: L e t m e remind you on the past i n Germany, t h e r e have been
b u i l t water r e a c t o r s more or less by American companies, not d i r e c t l y ,
790
bu t i n a way t h a t they are i n l i c e n s e agreement with the German country,
and I th ink t h i s w i l l be the way i n the f u t u r e too, and I guess it i s a good chance it w i l l go both ways.
K. Wirtz: I have one ques t ion which may not be poss ib le t o answer
y e t . The panel has discussed t h e r e l a t i v e merits of helium tu rb ine d i r e c t
cyc le p l an t compared t o a steam cycle. You have mentioned t h a t some i n -
t e r n a t i o n cooperation may be necessary t o b u i l d t h e f irst d i r e c t cycle i n
t h e p l an t . What i s your f e e l i n g t o the s i z e of t h i s p l a n t ? You have t o
have something l i k e an experimental demonstration of such f e a s i b i l i t y of
t h i s d i r e c t cycle helium p l a n t ; and how small can it be i n order t o be
s t i l l b i g enough t o a l low t o draw conclusions which are of some value
l a t e r on l a r g e r s t a t i o n s ?
R. Vaughan: I th ink it m u s t for s e v e r a l reasons be a f a i r l y large
p lan t . F i r s t of a l l , you w i l l remember 1 made t h e poin t that t h e r o - t a t i n g components have t o be developed for mass production.
i s a s t rong word, bu t you know what I mean. Therefore, t h e f i r s t com-
ponents you make must have the dimensions and c h a r a c t e r i s t i c s of those
components you w i l l want f o r your l a t e r s t a t i o n s . So if you are going t o
want 600 or 1200 megawatt un i t s , w e w i l l say 300 megawatts t o t h e com-
pressor u n i t s i n them. That i s t h e s i z e of t h e u n i t s you want t o t e s t and
manufacture. There i s no poin t i n making one which i s one-third t h e s i z e
because you could not j u s t i f y t h e development work economically on t h e
uni t because you would have t o do it aga in for t h e l a r g e unit. Also t h e
o the r purpose of your pro to typa l , t h e value of it i s t o t e s t t h e con t ro l
f ea tu re , and these w i l l vary widely if you go from say a s m a l l u n i t with
two pods t o a l a r g e one with four pods. You have got t o reproduce a s
c l o s e l y as poss ib le t h e dimensions and t h e c h a r a c t e r i s t i c s of your u l t i m -
a t e power s t a t i o n s so I th ink it must be a real prototype; a prototype i n
output as w e l l as i n temperatures and pressures .
Perhaps t h a t
K. Wirtz: S t i l l l e t me say t h a t I a m not sure t h a t wi th j u s t one
p l a n t w e can g e t a l l t h e information we may need, e s p e c i a l l y with r e spec t
t o t h e con t ro l quest ion. It could be t h a t if’ anyone would go r e a l l y i n t o
t h e problems of t he c o n t r o l ques t ion t h a t it could t u r n out t h a t you
could g e t t h i s information through a f a i r l y E m a l l p l an t , s ay of t he p lan t
791
@ w e have envisaged i n Germany; of course, t h i s doesn' t hold f o r t he t u r - b ines and s o on. But my f e e l i n g i s t h a t s o fa r the ques t ion w i t h respec t t o control, t h a t means the in t e rac t ions of t he whole c i r c u i t , haven't been analyzed adequately s o far, a t l e a s t not t o my knowledge, I m u s t say. I would very much l i k e t o have some kind of information about whether f o r t h i s purpose a b i g p lan t would be necessary o r not. a f a i r l y s m a l l p lan t , say 20 t o 50 megawatts, would be adequate.
i
It could well be that
C. Rickard: Yes, I think t h a t I would l i k e t o add, t h e r e i s cer-
t a i n l y something t o say on that argument on t h e m u l t i p l i c i t y of a p lan t and poss ib ly small ones as wel l as l a r g e ones. g rea t , g rea t deal from OUT experience with the 40 megawatt Peach Bottom
plant, and we aTe learn ing a g r e a t dea l more w i t h t h e 330 megawatt For t S t . Vrain p l an t and both of them had r e a l value; so I th ink it would be hard t o say there i s only one approach t o g e t t i n g on w i t h t h e job of combining gas turb ines with HTGR's and I th ink the main t h i n g i s t o ge t moving ahead on t h a t job because there i s very i n t e r e s t i n g p o t e n t i a l i n
t he fu tu re the re f o r t ha t combination of t h e HTGR w i t h t he gas turb ine .
We c e r t a i n l y learned a
R. Cyhan: Somebody asked f o r t h e impression of t h e customer. We
operate the Peach Bottom plant, s o I would l i k e t o make a shor t statement and say t h a t a t Philadelphia E l e c t r i c Company we be l ieve i n HTGR and a r e pu t t ing our hea r t s i n t o making it work and produce power aga in very soon, and t h a t it is making a l l of you proud in your f a i t h of the HTGR concept.
GAS-COOLED F A S T REACTOR DESIGN
SAFETY S T U D I E S AND FUEL DEVELOPMENT
(Session V I 1 1
794
Chairman: C . A. Rennie, P r i v a t e Consul tan t
Co-Chairman: P. P a t r i a r c a , Oak Ridge Na t iona l Laboratory
This paper i s p r i m a r i l y concerned w i t h r e p o r t i n g t h e p r o g r e s s of a 300-MW(e) gas-cooled f a s t b r e e d e r demonstra- t i o n p l a n t d e s i g n , a t p r e s e n t under s t u d y by Gulf Genera l Atomic. The c u r r e n t l y proposed form of t h e p l a n t i s p r e s e n t e d , t o g e t h e r w i t h t h e reasoning behind some of t h e more impor tan t f e a t u r e s . c a l l i n g f o r f u e l and c l a d d i n g tempera tures now no h i g h e r t h a n t h o s e c u r r e n t l y proposed f o r LMFBR a p p l i c a t i o n , r e p r e s e n t s a s i g n i f i c a n t d e p a r t u r e from ear l ie r p u b l i s h e d i n f o r m a t i o n on t h e p r o j e c t , and h a s been i n t r o d u c e d s o l e l y i n t h e i n t e r e s t of f u r t h e r i n c r e a s i n g i n i t i a l commonality w i t h t h e LMFBR f u e l program. It is noteworthy t h a t by i n t r o d u c t i o n of d e s i g n r e f i n e m e n t s d i s c u s s e d , t h i s change h a s been e f f e c t e d w i t h o u t d e g r a d a t i o n of t h e o r i g i n a l performance t a r g e t s . I n a c h i e v i n g t h i s r e s u l t , t h e v e r y c o n s i d e r a b l e importance of p r o p e r o p t i m i z a t i o n of steam and b o i l e r c o n d i t i o n s has been most s h a r p l y evidenced.
The c h o i c e of o p e r a t i n g c o n d i t i o n s ,
I N T R O D U C T I O N
This paper is p r i m a r i l y concerned w i t h t h e c o n t i n u i n g p r o g r e s s on
t h e d e s i g n of a 300-MW(e) gas-cooled f a s t b r e e d e r r e a c t o r (GCFR) demonstra-
t i o n power p l a n t c u r r e n t l y under s t u d y by Gulf Genera l Atomic i n a s s o c i a -
t i o n w i t h a group of 4 1 U.S. u t i l i t i e s .
The d e s i g n i s based on maximum u t i l i z a t i o n of e x i s t i n g f u e l and
component technology , d e r i v e d , r e s p e c t i v e l y , from t h e L i q u i d Metal F a s t
Breeder Reactor (LMFBR) and High Temperature Gas-cooled Reac tor (HTGR)
development programs. I n t h i s r e s p e c t , i t is t o b e d i s t i n g u i s h e d from
s t u d i e s of what could b e done w i t h more r e f r a c t o r y materials, o r even
w i t h t h e b e n e f i t on ly of a l i t t l e f u r t h e r e x p l o i t a t i o n of t h e a n t i c i p a t e d
c a p a b i l i t i e s of t h e s t e e l - c l a d o x i d e t y p e of f u e l .
795
796
I n conformi ty w i t h t h i s more immediate o b j e c t i v e , and indeed recog-
n i z i n g t h e d e s i r a b i l i t y of s t a r t i n g w i t h some d e g r e e of o v e r l a p i n p r i o r
g a s and l i q u i d - m e t a l t echnology, t h e p r e s e n t d e s i g n i s based on t h e u s e of
t h i c k s t a i n l e s s - s t e e l - c l a d oxide f u e l p i n s o p e r a t e d w i t h i n t h e tempera ture
range c u r r e n t l y contemplated f o r LMFBRs.
T h i s , i n f a c t , r e p r e s e n t s a s u b s t a n t i a l l y more c o n s e r v a t i v e approach
t h a n i s r e f l e c t e d i n p r e v i o u s l y p u b l i s h e d i n f o r m a t i o n on t h i s r e a c t o r
program. The r e a l l y i n t e r e s t i n g outcome of t h e more r e c e n t p r o g r e s s
r e p o r t e d h e r e i s t h a t d e s i g n re f inement i n a number of areas t o b e d i s c u s s e d
has r e s u l t e d i n a c t u a l improvement i n o v e r a l l performance i n t h e f a c e of
s u b s t a n t i a l c o n c e s s i o n s , b o t h t o s e c u r e t h e developmental o v e r l a p mentioned
and t o cope more a d e q u a t e l y w i t h t h e metal s w e l l i n g problem, which a t p r e s e n t
is of s o much koncern t o a l l f a s t - b r e e d e r d e s i g n e r s .
I n t h i s p a p e r , t h e p r e s e n t form of t h e p l a n t and i t s c h a r a c t e r i s t i c s
are b r i e f l y d e s c r i b e d , b u t more p a r t i c u l a r l y t h e n a t u r e and r e a s o n s f o r t h e
d e s i g n changes i n t r o d u c e d subsequent t o earlier p u b l i s h e d i n f o r m a t i o n on
t h e subject’” are d e a l t w i t h .
GENERAL PLANT DESCRIPTION
The g e n e r a l form of t h e proposed GCFR de inons t ra t ion p l a n t h a s n o t
changed i n e s s e n c e from t h a t a l r e a d y d e s c r i b e d e l sewhere . T o b e s t
a p p r e c i a t e t h e s i g n i f i c a n c e of t h o s e changes t h a t have been i n t r o d u c e d ,
i t is d e s i r a b l e t o s tar t w i t h a b r i e f d e s c r i p t i o n of t h e p r e s e n t form of
t h e p l a n t as a whole, even though some r e c a p i t u l a t i o n of e a r l i e r publ i skdd
i n f o r m a t i o n i s n e c e s s a r i l y involved .
F i g u r e s 1 and 2 show t h e c o n f i g u r a t i o n O E t h e r e a c t o r and i t s a s s o c i a t e d
pr imary c i r c u i t components, i n c l u d i n g t h e means f o r c o n t a i n i n g them, and
F i g s . 3 and 4 show t h e i n t e r n a l s of t h e r e a c t o r c a v i t y i n more d e t a i l .
Three main l o o p s , each w i t h independent b o i l e r s and c i r c u l a t o r s , are
employed t o g e t h e r w i t h t h r e e a u x i l i a r y l o o p s , each w i t h i t s own c i r c u l a t o r
and h e a t - e x t r a c t i o n system. F i g u r e s 1 and 2 : i l l u s t r a t e t h e c o n f i g u r a t i o n
of b o t h t y p e s of l o o p . A l l b o i l e r s , o r h e a t exchangers , and t h e i r a s s o c i a t e d
A
797
. i r c u l a t o r s are housed i n ver t ica l wells l o c a t e d i n t h e w a l l s of a pre-
s t r e s s e d c o n c r e t e r e a c t o r vessel (PCRV) s u r r o u n d i n g t h e c o r e . Gas f low
is downward through t h e c o r e , and i t is a l s o downward a c r o s s t h e t u b e
banks of t h e h e l i c a l - c o i l e d , once-through steam g e n e r a t o r s t o accommodate
t h e use of upflow b o i l i n g i n t h e s e g e n e r a t o r s . This n e c e s s i t a t e s
a p p r o p r i a t e f low reversals i n t h e g a s p a t h , and t h e s e are o b t a i n e d by
l e a d i n g t h e c o r e e x i t gas up through t h e o t h e r w i s e v a c a n t c e n t e r r e g i o n
of t h e b o i l e r t u b e bank, t h e n down over t h e t u b e s , and up a g a i n around
t h e b o i l e r s h e l l s (which h e l p s t o cool t h e s h e l l s ) , and thence t o top-
mounted c i r c u l a t o r s d i s c h a r g i n g t o t h e r e a c t o r top plenum.
Main c i r c u l a t i o n is by t h e t y p e of i n t e g r a l turboblower u n i t developed
f o r t h e HTGR, which employs a s i n g l e compression s t a g e d r i v e n by a s i n g l e
impulse steam t u r b i n e s t a g e p a s s i n g t h e e n t i r e loop steam f low. A u x i l i a r y
c i r c u l a t i o n i s provided by e l e c t r i c a l l y d r i v e n c e n t r i f u g a l c i r c u l a t o r s
powered by s e p a r a t e and i n d i v i d u a l l y d r i v e n high-frequency a l t e r n a t o r s .
The r e a c t o r c o r e ( i l l u s t r a t e d p i c t o r i a l l y i n F i g . - 5 ) , comprised of
some 200 hexagonal f u e l and r a d i a l b l a n k e t boxes , 10 f t i n t o t a l l e n g t h and
each about 6-1/2 i n . a c r o s s f l a t s , i s s u p p o r t e d from a top-mounted s i n g l e
g r i d p l a t e t o which each box is r i g i d l y a t t a c h e d . The f u e l boxes are t h u s
clamped s o l e l y a t t h e i r c o l d ends. They are i n i t i a l l y spaced some 1 / 4 i n .
a p a r t o v e r t h e i r whole l e n g t h t o accommodate r a d i a t i o n - i n d u c e d s w e l l i n g
and d i s t o r t i o n . T h e g r i d p l a t e , e s s e n t i a l l y c o n s i s t i n g of a s o l i d l l - f t -
diam, 2-1/2-f t - thick d i s c w i t h 6 i n . h o l e s t o accommodate c i r c u l a r e x t e n s i o n s
t o t h e f u e l boxes , is i tself t o p suppor ted by a sur rounding c y l i n d e r connected
t o t h e l i n e r 0-f t h e vessel t o p p e n e t r a t i o n . The e n t i r e g r i d p l a t e i s
r e p l a c e a b l e , i f ever n e c e s s a r y . T i g h t clamping of t h e f u e l boxes t o t h e
g r i d p l a t e , as w e l l as t h e means f o r o p e r a t i n g v a r i a b l e o r i f i c e s w i t h i n
each box , is f a c i l i t a t e d by p r o v i s i o n of i n d i v i d u a l s m a l l p e n e t r a t i o n s i n
t h e t o p access p l u g above each box.
Core l o a d i n g - ( r e q u i r i n g d e p r e s s u r i z a t i o n ) i s e f f e c t e d by a n i n s e r t e d
f u e l machine, which lowers and traverses f u e l i n t h e v a c a n t s p a c e below
t h e c o r e t o a s i n g l e e x i t p o r t l e a d i n g t o a t r a n s p o r t i n g c a s k b e n e a t h
t h e vessel s t r u c t u r e .
798
C o n t r o l i s by 27 r o d s i n s e r t e d from above i n t o f u e l boxes having a n
a p p r o p r i a t e c e n t r a l s p a c e w i t h i n . Normal o p e r a t i o n o f t h e r e a c t o r ,
r e q u i r i n g a t o t a l r e a c t i v l t y swing of $ 1 7 , i n c l u d i n g a $ 3 shutdown margin
a t a l l t i m e s , i s provided by 2 1 of t h e s e rod:;, each of which is l i m i t e d f o r
s a f e t y r e a s o n s t o 85c wor th . The six a d d i t i o n a l r o d s , each of $1 .6 w o r t h ,
form a backup system c a p a b l e of independent shutdown.
P r o t e c t i o n of t h e c o r e l i n e r and d u c t s Erom neut ron i r r a d i a t i o n i s
provided by a generous t h i c k n e s s of s h i e l d i n g . Around t h e c o r e , t h i s
s h i e l d i n g t a k e s t h e form of a removable inne:c l a y e r of s teel b l o c k s ,
surrounded by a c i r c u l a r s e c t i o n of s t e e l t u b e s c o n t a i n i n g g r a p h i t e , as
shown i n F ig . 3 . Above t h e g r i d p l a t e , v e r y t h i c k s h i e l d i n g l a y e r s p r o t e c t
bo th t h e c o r e p lug above and t h e r a d i a l i n t a k e d u c t s . Cooling of t h e r a d i a l
s h i e l d i n g i s by a bypass from t h e e n t r y hel ium, which i s a r r a n g e d t o
s t i m u l a t e v i g o r o u s i n t e r n a l c i r c u l a t i o n by i n j e c t o r a c t i o n .
A t y p e of c o n c r e t e t o p c o r e a c c e s s p lug is used which, w h i l e n o t
p r e s t r e s s e d , uses t h e sur rounding g a s p r e s s u r e t o s u p p r e s s t e n s i l e stresses
under a l l c o n d i t i o n s . Thrus t l o a d s are t a k e n p r i m a r i l y by t o p compression
s t r u t s , backed up by a n independent "gun breech" l o c k a c t i n g on an appro-
p r i a t e vessel l i n e r s h e a r anchor .
P l u g s of s i m i l a r s t y l e a re used above t h e b o i l e r s , i n t h i s case
i n c o r p o r a t i n g l a r g e c e n t r a l h o l e s f o r c i r c u l a t o r removal , and smaller
s u r r o u n d i n g h o l e s t o accommodate steam p i p e p e n e t r a t i o n s . To avoid need
f o r p lug r o t a t i o n , t h e breech- lock backup h o l d is r e p l a c e d by r a d i a l
b o l t s t h a t are o p e r a b l e from t h e c e n t e r h o l e a f t e r c i r c u l a t o r removal.
Tube p lugging can b e done e x t e r n a l l y , t h e main p e n e t r a t i o n opening
only b e i n g needed f o r complete b o i l e r removal.
A major d e s i g n c r i t e r i o n a p p l i e d h e r e t o a l l p e n e t r a t i o n s is t h a t
secondary r e s t r i c t o r s are used t o l i m i t possible d e p r e s s u r i z a t i o n r a t e
i n t h e e v e n t of pr imary b a r r i e r f a i l u r e t o a v a l u e t h a t does n o t endanger
c o r e c o o l i n g , even i n t h e e v e n t of a s imul taneous loss of one c i r c u l a t o r .
799
A s shown i n F i g . 6 , a secondary containment i s employed, b u t u n l i k e
@ t h e s i t u a t i o n w i t h LMFBRs, i n e r t i n g i s n o t r e q u i r e d s i n c e t h e c o o l a n t i s
nonflammable. The containment i s s i z e d t o r e a c h 2 a t m a b s o l u t e p r e s s u r e
on l o s s of c o o l a n t , which p r e s s u r e c o n s i d e r a b l y a i d s c o o l i n g i n t h e c r i t i c a l
p e r i o d immediately f o l l o w i n g a n a c c i d e n t a l d e p r e s s u r i z a t i o n .
The steam c y c l e used (F ig . 7) i s noteworthy because of t h e u s e of
r e s u p e r h e a t e r s fo l lowing t h e blower t u r b i n e s . T h i s , i n e f f e c t , c o n f e r s
most of t h e advantages of normal r e h e a t , b u t w i t h o u t t h e need t o accommodate
low-densi ty steam i n t h e t u b e banks , and a v o i d s t h e c o s t and p r e s s u r e l o s s
p e n a l t i e s of r e h e a t l i n e s l e a d i n g t o t h e main t u r b i n e . This r e s u p e r h e a t i n g
p r o v i d e s d r y enough steam t o avoid t h e n e c e s s i t y of p r o v i d i n g a m o i s t u r e
s e p a r a t i n g t u r b i n e and g i v e s a n o v e r a l l p l a n t e f f i c i e n c y of n e a r l y 38%,
even though g a s tempera tures a re l i m i t e d t o 542°C by d e c i s i o n t:o keep
c l a d d i n g hot -spot tempera tures down t o 700°C.
CORE THERMAL AND NUCLEAR D E S I G N
Design C o n s t r a i n t s
A number of d e s i g n r e s t r a i n t s have been adopted on t h e h a s i s - .. of p r e v i o u s
s t u d i e s and i n t h e i n t e r e s t of p r o p e r l y r e p r e s e n t i n g l a t e r t y p i c a l l a r g e
p l a n t r e q u i r e m e n t s . The p r i n c i p a l i tems are g i v e n i n Table 1.
Table 1. D e s i g n C o n s t r a i n t s f o r GCFR D e m o n s t r a t i o n P l a n t
P r e s e n t Previous Design Design 1
Electr ic power o u t p u t , MW 310 330
Coolant p r e s s u r e drop r a t i o i n pr imary l o o p , AP/P 0.048 0.048
Cladding O D / I D 1 .15 1 . 1 0
Clearance between e l e m e n t s , i n . 0 .25 0.12
Maximum tempera ture (mid-clad) , "C 7 00 760
F u e l smear d e n s i t y , % t h e o r e t i c a l 80 88
Maximum rod r a t i n g (:LO% power o v e r s h o o t ) , kW/ft 13.8 1 6 . 5
800
Taking t h e s e i n o r d e r , p l a n t s i z e w a s , i n e f f e c t , d i c t a t e d by t h e
b a s i c f a c t t h a t g a s c o o l i n g is n o t t o o e f f e c t i v e f o r small c o r e s , where
h i g h n e u t r o n l e a k a g e p r e c l u d e s a l l o c a t i o n O S a r e a l l y adequate c o o l a n t
volume f r a c t i o n .
The s i z e chosen s imply r e f l e c t s a judgment of a minimum c o n s i s t e n t
w i t h r e t e n t i o n of a s u f f i c i e n t l y r e p r e s e n t a t i v e and a t t r ac t ive performance,
b o t h as an economic power producer and as a tes t r e a c t o r . P r e s s u r e drop
a l l o c a t i o n i s based on t h e l i m i t s of a s i n g l e - s t a g e c i r c u l a t o r and on t h e
l o s s of c i r c u l a t i o n c o n s i d e r a t i o n s , r a t h e r t h a n on performance opt imiza t ion-
which i n d i c a t e d some b e n e f i t i n h a r d e r blowing.
The c o o l a n t p r e s s u r e (1250 p s i ) chosen is l i k e w i s e n o t t h e r e s u l t of
"opt imiza t ion" b u t h a s been set r a t h e r by what is cons idered a prudent
increment of p r e s e n t HTGR r e q u i r e m e n t s , w i t h i n t h e l a t t e r ' s v e s s e l - t y p e
technology.
The c l a d t h i c k n e s s chosen f o r t h e f i r s t c o r e l o a d i n g s i s t a k e n s imply
b e c a u s e most LMFBR i r r a d i a t i o n e x p e r i e n c e l i e s i n t h i s area. S u b s t a n t i a l l y
t h i n n e r c l a d d i n g is b e l i e v e d a p p r o p r i a t e f o r t h e vented t y p e of f u e l r o d s
h e r e employed , and l a t e r l o a d i n g s are c o n f i d e n t l y expected t o b e n e f i t
g r e a t l y from t h i s .
Cladding tempera ture levels , as a l r e a d y mentioned, have been se t t o
s e c u r e c o n t i n u i t y w i t h t h e LMFBR f u e l program, and do n o t r e p r e s e n t i n h e r e n t
l i m i t a t i o n s of p r e s e n t l y a v a i l a b l e m a t e r i a l s .
The l a r g e r i n t e r b o x c l e a r a n c e of 114 i n . now proposed i s concerned
w i t h means f o r d e a l i n g w i t h meta l s w e l l i n g , r e f e r r e d t o i n more d e t a i l
l a t e r . An i n t e r e s t i n g p o i n t h e r e i s t h a t th: is h a s n o t very s i g n i f i c a n t l y
a f f e c t e d performance, thanks t o t h e low c o o l a n t - n u c l e a r i n t e r a c t i o n .
The reduced f u e l d e n s i t y a l lowance i s i n t r o d u c e d p r i m a r i l y as a
p o s s i b l e easement t o c o n t r o l of f u e l s w e l l i n g a t h i g h burnup.
The l i n e a r r a t i n g s (kW/ft) , b e i n g p r i m a r i l y d i c t a t e d by f u e l c o n d u c t i v i t y ,
are s e l e c t e d t o b e i n t h e r e p r e s e n t a t i v e range of LMFBR oxide f u e l
e x p e r i e n c e .
801
Design O p t i m i z a t i o n
~
The g e n e r a l approach t a k e n h e r e may b e b a s i c a l l y c h a r a c t e r i z e d by
employment of a r a d i a l power f l a t t e n i n g t e c h n i q u e which a i m s a t r e a c h i n g
t h e same c l a d d i n g hot -spot t e m p e r a t u r e i n each channel , a p p l y i n g l o c a l l y
a p p r o p r i a t e ho t -spot f a c t o r s , r a t h e r t h a n aiming s imply a t uniform mean
zone power. Thus, f o r i n s t a n c e , o u t e r zones are o p e r a t e d a t reduced
mean power, because t h e f l u x t i l t i s s t e e p t h e r e , and w e d e s i r e t o l i m i t
c o n d i t i o n s on t h e h o t t e s t p i n s i n t h e zone.
This mode of o p e r a t i o n is of c o u r s e dependent on our p r o v i s i o n of
on-load v a r i a b l e o r i f i c i n g on each f u e l box and h a s r e q u i r e d t h e develop-
ment of a n a p p r o p r i a t e d e s i g n computer code f o r i t s i n v e s t i g a t i o n .
A second c h a r a c t e r i s t i c of t h e o p t i m i z a t i o n s t u d y h a s been t h e
combinat ion of t h i s code w i t h a b o i l e r and steam c y c l e code, a l l o w i n g
s e l e c t i o n of a p p r o p r i a t e t r a d e o f f s , p a r t i c u l a r l y i n c h o i c e of r e a c t o r
e n t r y t e m p e r a t u r e . An i m p o r t a n t l e s s o n d e r i v e d has indeed been t h a t over-
a l l p l a n t performance is very s e n s i t i v e t o t h i s q u a n t i t y , p r i n c i p a l l y
on account of t h e r a t h e r s m a l l “p inch p o i n t ” tempera ture d i f f e r e n t i a l s
between hel ium and steam t h a t c a n e a s i l y b e i n c u r r e d by a r b i t r a r y c h o i c e s .
Large ly as a r e s u l t of t h e f o r e g o i n g c o n s i d e r a t i o n s , w e would conclude
t h a t t o o e a r l y ”broad-brush’’ s t u d i e s can b e very m i s l e a d i n g u n l e s s v e r y
c l o s e l y watched. Both t h e c o r e and t h e steam c y c l e must b e s t u d i e d to-
g e t h e r by one team f o r meaningful c o n c l u s i o n s .
R e s u l t s
The p r i n c i p a l r e s u l t s are g i v e n i n Table 2 , t o g e t h e r w i t h correspond-
i n g f i g u r e s r e l a t i n g t o t h e earlier p u b l i s h e d d e s i g n . Aside from t h e
imposed drop i n c l a d d i n g t e m p e r a t u r e , t h e only f i g u r e t h a t may seem t o b e
s i g n i f i c a n t l y changed is t h e c o n v e r s i o n r a t i o , which i s now 1.33. The only
s i g n i f i c a n t r e a s o n f o r t h i s :Low c o n v e r s i o n r a t i o i s t h e l i m i t e d b l a n k e t t h i c k -
n e s s employed f o r t h e s m a l l c o r e of t h e demonst ra t ion p l a n t . S e p a r a t e
c a l c u l a t i o n s have shown t h a t t h e o v e r a l l convers ion r a t i o could b e i n c r e a s e d
t o a t l eas t 1.48 by l e n g t h e n i n g t h e a x i a l b l a n k e t and adding one row of
802
r a d i a l b l a n k e t e lements . Although t h i s t h i c k e r b l a n k e t would b e t o o c o s t l y
f o r t h e demonst ra t ion p l a n t , i t would b e e a s i l y accommodated i n a much
l a r g e r p l a n t .
This same scale p e n a l t y i s a l s o e v i d e n t i n t h e f u e l r a t i n g , which,
a l though improved a l i t t l e , is s t i l l w e l l below t h e 1 MW/kg r a n g e t h a t our
p a r a l l e l s t u d i e s of l a r g e c o r e s i n d i c a t e a t t h e s a m e t empera tures .
The e s s e n t i a l p o i n t of i n t e r e s t i s t h a t w h i l e t h e very much c l o s e r
s t u d y involved i n t h e d e s i g n r e v i s i o n may seem t o have had l i t t l e e f f e c t on
o v e r a l l r e s u l t s , i t indeed r e p r e s e n t s a s u b s t a n t i a l g a i n i n t h e form of
much easement of i n i t i a l f u e l developmental requi rements and more t o l e r -
ance f o r g e n e r a l conserva t i sm.
This i s evidenced i n Tables 1 and 2 by .a r e d u c t i o n of c l a d d i n g t e m -
pera ture of some 6OoC, accompanied by an allowance for a 50% increase i n
c l a d d i n g t h i c k n e s s , a 10% r e d u c t i o n of needed f u e l d e n s i t y , and p r o v i s i o n
f o r a l a r g e i n t e r b o x gap t o d e a l w i t h m e t a l s w e l l i n g . That t h i s should b e
p o s s i b l e , w h i l e a c t u a l l y i n c r e a s i n g both p l a n t e f f i c i e n c y and f u e l r a t i n g
a l i t t l e , c e r t a i n t l y r e p r e s e n t s a welcome c h m g e from t h e u s u a l r e s u l t of
a c l o s e r i n s p e c t i o n of i n i t i a l p r o s p e c t s .
DETAIL FEATURES
Core S t r u c t u r e and Meta l Swel l ing
The p r o s p e c t s of i r r a d i a t i o n - i n d u c e d metal s w e l l i n g ( t o t h e t u n e of
i s c e r t a i n t l y of p r e s e n t g r e a t concern perhaps more t h a n 10% by volume)
t o all f a s t - b r e e d e r d e s i g n e r s . There i s f o r t u n a t e l y much easement of t h e
consequences of d i s t o r t i o n i n t h e c a s e o f gas-cooled b r e e d e r s because t h e y
do n o t s u f f e r t h e extreme premium on a c h i e v i n g compactness t h a t i s t h e
consequence of u s i n g a c o o l a n t a f f e c t i n g n u c l e a r b e h a v i o r . I n p a r t i c u l a r , much more w i d e l y spaced f u e l r o d s are used , t :here i s more l i b e r t y t o s p a c e
f u e l boxes a p a r t , and , a l s o , on account of i n h e r e n t l y lower c o r e v o l u m e t r i c
power d e n s i t y (-250 k W / l i t e r , a g a i n s t t y p i c a l l y over 500 k W / l i t e r f o r
LMFBRs), r e a c t i v i t y i s much less s e n s i t i v e t o f u e l d i sp lacement .
A
803
Fuel-box s w e l l i n g and d i s t o r t i o n , n o t c l a d s w e l l i n g , i s t h e concern.
:de a t t a c k t h e problem n o t by c o r e restrailit, which is c a p a b l e ~f conceal-
i n g c o n s i d e r a b l e p o t e n t i a l l y dangeraus s t r a i n energy s t o r a g e , b u t by al low-
lng growth f r e e l y t o t a k e p l a c e . The s ingle-ended f u e l s u p p o r t f a c i l i t a t e s
this c o n s i d e r a b l y f o r , i n a s s o c i a t i o n r&th t h e r a d i a l f l u x d i s t r i b u t i o n
employed, i t e n s u r e s a p r o g r e s s i v e r e d u c t i o n i n r e a c t i v i t y as t h e f u e l
boxes are bowed by d i f f e r e n t i a l growth.
C a l c u l a t i o n shows, i n f a c t , t h a t w i t h t h e box s p a c i n g employed, no
touching of f u e l boxes need b e involved o v e r t h e whole f u e l :Lifetime. Only
t h e o u t e r r i n g of f u e l boxes (having a h i g h f l u x t i l t ) , i n f a c t , s u f f e r
s u b s t a n t i a l (outward) movement a t t h e b a s e . The consequences of t h i s on
long-term r e a c t i v i t y l o s s are provided a g a i n s t by p r o v i s i o n of a n appro-
p r i a t e c l e a r a n c e between t h e c o r e and b l a n k e t and by adding f a c i l i t y t o
r o t a t e f u e l boxes on t h e o c c a s i o n of each (annual ) p a r t i a l r e l o a d .
C a l c u l a t i o n s which r e l a t e t o u s e of 20% cold-worked 316 s t e e l , 3 and
a l s o i n c l u d e t h e e f f e c t s of thermal expans ion , l e a d t o t h e fo l lowing r e s u l t s
f o r t h i s mode of o p e r a t i o n :
Maximum r a d i a l d i sp lacement
A t f u e l e lement lower end . . . . . . . 0.8 i n .
A t act ive c o r e bot tom f a c e . . . . . . 0 . 4 i n .
A t c o r e c e n t e r p l a n e . . . . . . . . . 0 . 1 i n .
C i r c u l a t o r s
Main c i r c u l a t i o n , as a l r e a d y remarked, i s by t h e t y p e of i n t e g r a l
series steam turboblower u n i t t h a t h a s b e e n s u c c e s s f u l l y developed f o r
t h e HTGR class of r e a c t o r s .
These machines are p a r t i c u l a r l y s u i t e d t o f a s t - r e a c t o r c o o l i n g , on
account of t h e i r compactness, which g r e a t l y f a c i l i t a t e s i n t e g r a l c o n t a i n -
ment even of very h i g h power u n i t s . Furthermore, t h e f a c t t h a t each
machine i s coupled d i r e c t l y t o i t s own power s o u r c e ( i . e . , t h e h e a t from
t h e loop which i t s e r v i c e s ) i s a n i m p o r t a n t f a c t o r i n e n s u r i n g cont inuous
c i r c u l a t i o n a v a i l a b i l i t y . This end i s f u r t h e r f a c i l i t a t e d by t h e c l o s e l y
a d j a c e n t l o c a t i o n of t h e c i r c u l a t o r t u r b i n e s t o t h e i r s o u r c e of steam 0
804
( t h e i n d i v i d u a l b o i l e r t h a t t h e y a r e cool ing: ) , which g r e a t l y reduces t h e
system area needing class I p r o t e c t i o n f o r t h e g u a r a n t e e of t h i s steam
supply
Locat ion of t h e series steam t u r b i n e i n t h e h i g h - p r e s s u r e steam
c i r c u i t , as opposed t o i t s ear l ier a p p l i c a t i o n i n t h e r e h e a t l i n e s of t h e
HTGR-type r e a c t o r s , i n t r o d u c e s i n t e r e s t i n g d i f f e r e n c e s , n o t on ly i n t h e
a p p r o p r i a t e machine d e s i g n approach b u t a l s o i n t h e mode of p l a n t c o n t r o l
c a l l e d f o r . I n t h e former area, t h e importance of p r o t e c t i n g t h e t h r u s t
b e a r i n g s from t h e h i g h l o a d s t h a t could come from p o s t u l a t e d sudden l o s s e s
of steam p r e s s u r e is c l e a r l y much r e i n f o r c e d by t h e h igh p r e s s u r e s used .
This has l e d , i n f a c t , t o a d e s i g n i n which t h e c i r c u l a t o r and t u r b i n e
d i s c s are r e s p e c t i v e l y s e l f - b a l a n c e d by t h e i r own working f l u i d s , a v o i d i n g
dependence of n e t d i s c t h r u s t on d i f f e r e n c e s between hel ium and steam
p r e s s u r e a b s o l u t e l e v e l s . This h a s been achieved by u s e of a p u r e impulse
steam t u r b i n e , having l a r g e d i s c h o l e s t o e n s u r e t h i s c o n d i t i o n , t o g e t h e r
w i t h t h e a p p l i c a t i o n of blower d i s c h a r g e p r e s s u r e t o a n a p p r o p r i a t e area
of t h e upstream f a c e of t h e c i r c u l a t o r d i s c .
C o n t r o l of blower speed is by an upstream steam t h r o t t l e , as opposed
t o u s e of a bypass valve, which i s a p p r o p r i a t e t o t h e H E R S l o c a t i o n o f
t h e t u r b i n e i n t h e r e h e a t l i n e .
C o n t r o l l i n g t h i s upstream t h r o t t l e t o keep a c o n s t a n t blower t u r b i n e
d i s c h a r g e p r e s s u r e a t a l l l o a d s h a s t h e e f f e c t of producing a hel ium
c i r c u l a t i o n a t a l l t i m e s c l o s e l y p r o p o r t i o n a l t o t h e steam demand, t h u s
p r e s e r v i n g approximate ly c o n s t a n t r e a c t o r tempera ture r ise. The main t u r b i n e
t h r o t t l e i s t h e r e b y f r e e d t o o p e r a t e independent ly of t h i s c o n s i d e r a t i o n .
Fuel-rod Venting
The u s e of c o l l e c t i v e rod v e n t i n g t o a manifold i s perhaps one of
t h e most n o v e l f e a t u r e s of our approach t o t h e GCFR d e s i g n . It is t h e r e f o r e
i m p o r t a n t t o d i s c u s s b o t h t h e m o t i v a t i o n s involved and t h e d e s i g n proposed
f o r such a system. The prime o b j e c t i v e s of rod v e n t i n g are t o r e l i e v e t h e
c l a d d i n g from s u p p o r t i n g t h e e x t e r n a l c o o l a n t p r e s s u r e e a r l y i n l i f e and t o
avoid h e r m e t i c containment of h i g h i n t e r n a l f f k s i o n - g a s p r e s s u r e s when t h e
805
e x t e r n a l p r e s s u r e is r e t u r n e d t o a t m o s p h e r i c , as d u r i n g f u e l unloading and
t r a n s p o r t and i n i n c i d e n t s i n v o l v i n g c o o l a n t d e p r e s s u r i z a t i o n . 0 Another r e a s o n f o r avoid ing a s u b s t a n t i a l p r e s s u r e d i f f e r e n t i a l a c r o s s
t h e c l a d d i n g is t h a t i t removes a major d i f f e r e n c e between t h e r e q u i r e m e n t s
of LMFBR and GCFR f u e l r o d s , l e a d i n g t o c l o s e commonality between t h e two
programs.
i n g f u l f u e l i r r a d i a t i o n s can b e conducted i n p r e s e n t l y a v a i l a b l e sodium-
cooled f a s t t e s t r e a c t o r s . Other b e n e f i t s of fue l - rod v e n t i n g a r e t h a t
(1) t h e r o d s do n o t r e q u i r e e x t e n s i o n t o p r o v i d e i n t e r n a l v o i d s p a c e ;
( 2 ) t h i n n e r c l a d d i n g a i d s b o t h c o o l i n g and neut ron a b s o r p t i o n ; and (3) a
s i m p l e f a c i l i t y f o r b u r s t - r o d d e t e c t i o n i s provided . Venting, does r e q u i r e
p r o v i s i o n s t o c o n t r o l r e l e a s e d f i s s i o n p r o d u c t s , b u t i t should b e remembered
t h a t a pr imary c i r c u i t f i s s i o n - p r o d u c t c leanup system i s r e q u i r e d anyway
t o d e a l w i t h p o s s i b l e fue l -e lement f a i l u r e and chemical contaminat ion .
The f u e l development program i s a l s o f a c i l i t a t e d , because mean-
F i g u r e 8 shows t h e v e n t i n g system f o r t h e s p e c i f i c d e s i g n contemplated.
The long plenum s p a c e needed a t t h e ends of nonvented f u e l r o d s i s r e p l a c e d
by a 3- in . c h a r c o a l - f i l l e d e x t e n s i o n forming t h e f i r s t s t a g e of t h e t r a p
sys tem, aimed a t d e l a y i n g v e r y s h o r t - l i v e d f i s s i o n p r o d u c t s . Connections
t o i n d i v i d u a l r o d s s ta r t w i t h i n t e r n a l i n t e r c o n n e c t i o n of t h e rods w i t h i n
each f u e l box, e f f e c t e d by passages w i t h i n a n upper i n t e r n a l rod-spacer
g r i d . From t h e r e , t h e e f f l u e n t p a s s e s t o a f i s s i o n - g a s c h a r c o a l t r a p l o c a t e d
i n t h e upper ( c o o l ) r e g i o n of each f u e l box. The demountable connec t ion of
t h e c l e a n s i d e of each of t h e s e t r a p s is made a t t h e c o n i c a l i n t e r f a c e
between t h e f u e l boxes and t h e bottom of t h e g r i d p l a t e , a n inf low of c i r c u i t
hel ium is added t o t h e e f f l u e n t s t r e a . m (kept below t h e ambient p r e s s u r e ,
which i n t h e sea l r e g i o n i s about t h a t of t h e c o r e o u t l e t c o o l a n t g a s ) .
The mixed hel ium and f i s s i o n - g a s stream i s t h e n l e d t o t h e top of t h e g r i d
p l a t e via v e r t i c a l d r i l l i n g s i n t h e 1 - a t t e r , each of which i s f e d from one o r
more a d j a c e n t f u e l boxes. Thus, a c t i v i t y moni tor ing f o r each element o r
s m a l l group of e lements p e r m i t s l o c a l i z i n g of rod f a i l u r e t o w i t h i n a few
boxes. The purpose o f t h e d i l u e n t , o r scavenge, hel ium a d d i t i o n is t o
e n s u r e t h a t any "breakawayff f low from t h e i n t e r n a l t r a p s (due t o ambient
p r e s s u r e f l u c t u a t i o n s ) i s swept o u t of t h e p i p e s l e a d i n g t o t h e e x t e r n a l
c leanup t r a p s r a p i d l y enough t o avoid s u b s t a n t i a l l o c a l decay and d e p o s i t .
806
F i g u r e 9 i l l u s t r a t e s t h e t r a p p i n g system e x t e r n a l t o t h e c o r e b u t
w i t h i n t h e PCRV. B a s i c a l l y , t h e e f f l u e n t from t h e in-core t r a p s (approxi-
mately 1 l i t e r l d a y of f i s s i o n gas from t h e whole c o r e ) , p l u s t h e d i l u e n t
he l ium, p a s s e s through t h e water-cooled d e l a y beds and l i q u i d - n i t r o g e n -
cooled t r a p s ( i n t h e manner used i n HTGRs) and r e t u r n s t o t h e main c i r c u i t
blower i n t a k e , where t h e s t a t i c p r e s s u r e i s well below t h a t of t h e s ea l
r e g i o n and can induce a n adequate d i l u e n t f low under a l l c o n d i t i o n s . I n
t h i s way, t h e need f o r a n independent loop c i r c u l a t o r i s e l i m i n a t e d and a
proper d i r e c t i o n of scavenge hel ium f low i s main ta ined a t a l l t i m e s .
CONCLUSION
The g e n e r a l c o n c l u s i o n of t h i s paper i s t h a t tempera tures h i g h e r t h a n
c u r r e n t l y envisaged i n sodium b r e e d e r s are f a r from a p r e r e q u i s i t e f o r
success of gas cooling and t h a t , on t h e c o n t r a r y , even w i t h l i t t l e o r no
more g a i n s i n t h i s d i r e c t i o n , p r o s p e c t s a r e most a t t r a c t i v e when f u e l - c y c l e
c o s t , c a p i t a l c o s t , a n d , above a l l , c o s t of maintenance and r e p a i r are
a l l c o n s i d e r e d . This i s n o t t o d e n i g r a t e t h e advantages of p u r s u i n g f u r t h e r tempera-
t u r e r a i s i n g - e s s e n t i a l t o t h e u l t i m a t e u s e of t h e gas t u r b i n e - b u t merely
t o p o i n t o u t t h a t g a s c o o l i n g a p p e a r s t o o f f e r a r ea l contemporary a l t e r n a t i v e
t o l i q u i d - m e t a l technology f o r b r e e d e r s , i n a .dd i t ion t o t a n t a l i z i n g f u t u r e
p r o s p e c t s .
REFERENCES
1. P. F o r t e s c u e , e t a l . , "A Developmental Gas-Cooled F a s t Reac tor P l a n t , " I n t e r n a t i o n a l Nuclear I n d u s t r i e s F a i r (BIUCLEX 6 9 ) , October 6-11, 1969, B a s i l , S w i t z e r l a n d .
2. P . F o r t e s c u e , "Gas-Cooled F a s t Breeder R.eactor Development , ' I Proc . American Power Conference, Chicago, Ill., A p r i l 2 2 - 2 4 , 1969, Vol. 31, 1969.
3 . W . K. Appleby, e t a l . , " S t a i n l e s s S t e e l Swel l ing ," J o i n t C o n t r i b u t i o n of Bat te l le Northwest Labora tory and Westinghouse Advanced Reac tors D i v i s i o n t o t h e Twenty-ninth High Temperature Fuels Committee Meet ing, December, 1969.
Table 2. Comparative L i s t i n g of Designs
P resen t Previous Design Design
Core Geometry
Volume, l i t e r s
Length-to-diameter r a t i o
Volume f r a c t i o n s
Fue l , i nc lud ing c e n t e r ho le 0.300 0.386
Cladding 0.097 0.081
Gaps and s t r u c t u r e 0.160 0.111
Coolant 0.443 0.422
Fuel rod d iamete r , cm 0.723 0.787
Number of f u e l rods 30,700 28,400
Number of f u e l elements 87 89
Number of c o n t r o l elements 31 19
Number of b l a n k e t elements 9 3 90
Core Physics
Fuel average enrichment, % f i s s i l e 18.5 14.5
Rad ia l power maximum t o average 1.248 1.120
Conversion r a t i o 1 .33 1.47
R e a c t i v i t y drop pe r r e load , $ 9.00 3.40
Performance
Reactor i n l e t temperature , O C 312 283
Reactor 6 u t l e t temperature , "C 542 598
MWt/kg f i s s i l e 0.605 0.576
Thermal e f f i c i e n c y , % 37.6 37.2
Maximum rod r a t i n g , kW/ft 12.6 15 .1
Power d e n s i t y , kW/l i ter 238 243
Thermal ou tpu t , MW 824 916
E l e c t r i c o u t p u t , MW 310 341
Fig . 1. GCFR Nuclear Steam Supply System
84' OU.
Fig. 2. Vertical Section through PCRV Fig. 3. through
FUEL SERVICE MACHINE PENETAATIO
FUEL HANDLING HlNE PLNETPIT ION
Vertical Section Reactor in Cavity
809
27 CONTROL ROD ELEMENTS 184 FUEL 8 BLANKET ELEMENTS
INNER SbIELD BLOCKS
6 SECONDARY GRID SUPPORT RODS
THERMAL SHIELD INNER THERMAL (INNER) SHIELD LINER
Fig. 4. Horizontal Section through Reactor
I ! I I
J
Fig. 5. Perspective of GCFR Core
810
S E C O N D A R Y C O N T A I N M E N T
GENERATOR
R E A C T O R COMPARTMENT
H A N D L I NG
F i g . 6. Secondary Containment
I- I . I I I I I I I I 1 1 I I L
TO MONITOR STATIONS AND HELIUM PURIF ICATION SYSTEM COOLANT
I--- I F I S S I O N PRODUCT-
I I I I I I 1 I I I I I I I I I I I I I I
I
A C T I V I T Y DETECTORS ( O N E / L I N E )
---
L I N E S
---__--- ---- PCRV BOUNDARY MA1 F’
C IRCULATOR
PLATE
STEAM GENERATOR
U - lo - L
r
THROTTLING VALVE
HEL I UM P U R I F I C A T I O N SYSTEM
PCRV BOUNDARY
1 I I I 1 I I I I I I ! I I I I I I I I
J Fig. 9. Fission-product Venting and Trapping System -
Fig. 8. Vented Fuel Element
Paper 2/114
GAS TURBINE POWER CONVERSION SYSTEMS FOR HELaIUM COOLED BREEDER REACTORS
L.A. Lys G . Ciszewski H, F r u t s c h i
V ' ABSTRACT
From t h e po in t of view of f u e l cyc le c o s t , helium cooled fast r e a c t o r s do not r e q u i r e high e f f i c i e n c i e s . Thus, t h e a t t r a c t i v e n e s s o f u s ing gas t u r b i n e s , even a t t h e moderate gas temperatures t y p i c a l o f t h i s r e a c t o r t y p e , rests on t h e a b i l i t y t o achieve a reduct ion of t h e c a p i t a l investment which is s u f f i c i e n t t o produce lower power genera t ion c o s t . Two main types of system are pos- s i b l e : a d i r e c t helium t u r b i n e system and an i n d i r e c t system us ing C02 t u r b i n e s . I n t h e pre.sent paper t h e t w o systems are descr ibed . Problems r e l a t e d t o t h e turboma- ch inery design and t o p l a n t c o n t r o l are d iscussed .
GENERAL
When cons ider ing power genera t ion system:; f o r helium cooled fast
breeder r e a c t o r s it i s important t o r e a l i z e t h a t t h i s t ype of . r eac to r
produces cons iderably more f u e l t han it consumes and t h e r e f o r e should
not simply be regarded as a power p l a n t , but a l s o as a kind of plutonium
f a c t o r y . As a consequence of t h e va lue o f t h e f i s s i l e m a t e r i a l produced,
t h e f u e l c o s t s are very low and only weakly a f f e c t e d by s t a t i o n e f f i -
c iency. Thus minimization o f power gene ra t ion c o s t may l e a d -to des igns
f e a t u r i n g smaller c a p i t a l investment even at t h e expense o f s i g n i f i c a n t -
l y lower e f f i c i e n c y .
Using metal-clad mixed PuO -UO f u e l rods wi th a maximum al lowable 0
2 2 s u r f a c e temperature ( inc lud ing hot -spots ) of 800 C , r e a c t o r o u t l e t t e m -
p e r a t u r e s o f t h e o rde r o f 650°C r e s u l t . These temperatures are q u i t e
adequate t o provide "standard" steam cond i t ions a t t h e b o i l e r o u t l e t and A
812
813
t h u s s t a t i o n e f f i c i e n c i e s i n excess of Lu % i f a reheat steam t u r h i n e
cyc le i s employed. El iminat ion of t h e r ehea t s e c t i o n of t h e b o i l e r redu-
ces t h e s t a t i o n e f f i c i e n c y by over 3 percentage p o i n t s . However, because
o f t h e f e a t u r e explained ahove, t h e r e s u l t i n g cos t savings f u l l y j u s t i f y
t h e use of t h e design with t h e lower e f f i c i e n c y .
With t h e above r e a c t o r o u t l e t t empera tures a f u r t h e r important reduc-
t i o n of p l an t e f f i c i ency must be accepted i f a d i r e c t cyc le helium t u r -
b ine i s s u b s t i t u t e d f o r t h e steam t u r b i n e power genera t ion system. The
r e s u l t i n g e f f i c i e n c y depends on t h e degree of hea t regenera t ion and on
assumptions concerning p res su re l o s s e s i n t h e c i r c u i t , s ink tempera ture ,
e tc . , but f o r a reasonable set o f assumptions it i s of t h e o rde r of 30 %.
Again, i n sp i t e .o f i t s lower e f f i c i e n c y , t h i s design may prove more ad-
vantageous i f it b r ings about a r educ t ion of t h e c a p i t a l investment which
i s s u f f i c i e n t t o produce lower power genera t ion c o s t s .
A helium t u r b i n e i s a s impler , and above a l l , a much smaller machine
than a steam t u r b i n e of t h e same output . The es t imated weight o f a s i n g l e -
s h a f t , eight-exhaust-flow steam t u r b i n e considered i n our design s tudy
of a 1000 MWe fast breeder p l a n t i s approximately 2500 t o n s . In t h e a l -
t e r n a t i v e d i r e c t cyc le vers ion t h e same power output is provided by t h r e e
s p l i t s h a f t helium t u r b i n e s , t h e t o t a l weight o f which amounts t o only
1 / 3 of t h e weight of t h e above steam t u r b i n e . Since t h e cos t of machines
of s i m i l a r cha rac t e r i s roughly p ropor t iona l t o t h e i r weight , one can ex-
pec t much cheaper turbomachinery i n t h e d i r e c t cyc le case.
A c e r t a i n , though no t very impor tan t , r educ t ion of t h e c o s t of hea t
exchanging equipment can a l s o be expected i n t h e case of t h e d i r e c t gas
t u r b i n e cyc le s i n c e t h e t o t a l c o s t o f t h e r egene ra to r s and coo le r s i s ex-
pected t o be smaller than t h e c o s t of t h e steam gene ra to r s and feed-water
hea te r s . Fur ther r educ t ion of t h e c a p i t a l investment r e s u l t s from t h e e l i -
mination of helium c i r c u l a t o r s and feed water pumps and poss ib ly from t h e
gene ra l s i m p l i f i c a t i o n of t h e duc t ing system. However, it is important t o
no te t h a t t h e i n t e g r a t i o n of t h e primary loop i s much more d i f f i c u l t i n
t h e case of t h e d i r e c t gas t u r b i n e c y c l e , s i n c e enc los ing t h e turbomachines
814
t o g e t h e r with t h e r e l a t e d hea t exchangers and duc t ing wi th in a p r e s t r e s s -
ed concre te r e a c t o r v e s s e l i nvo lves , i n comparison wi th t h e i n d i r e c t cyc le
des ign , a s i g n i f i c a n t i nc rease of t h e vessel . s i z e . The r e s u l t i n g cos t i n -
c r ease can be only p a r t i a l l y compensated by t h e e l imina t ion of t h e t u r -
b ine house. This drawback of t h e d i r e c t cyc le i s of course not present i n
t h e non-integrated des ign , i n which t h e turbogroups a r e arranged i n t h e
containment bu i ld ing around t h e r e a c t o r v e s s e l . However t h e choice of t h e
non-integrated design depends upon t h e p o s s i b i l i t y of s a t i s f y i n g s a f e t y
requirements i n case of dep res su r i za t ion .
It i s noteworthy t h a t i n a d i r e c t cyc le p l a n t t h e coo le r s normally
r ep resen t an important cos t i t e m , i n our des igns of t h e o rde r $ 6-8 pe r
kW. This is because s a f e t y r e q u i r e s t h a t an in te rmedia te cool ing water
c i r c u i t i s provided i n t h i s class of p l a n t i n o rde r t o prevent t h e escape
of p o t e n t i a l l y r a d i o a c t i v e gas from t h e pr imwy c i r c u i t t o t h e environ-
ment through a l e a k i n a c o o l e r . From t h e cap i ta l investment po in t o f
view t h i s means not only t h a t a d d i t i o n a l hea t exchangers must be i n s t a l l -
ed but a l s o t h a t t h e s i z e of t h e primary coo le r s must be increased s i n c e
they must be designed f o r only a f r a c t i o n of t h e temperature d i f f e r e n c e
o r i g i n a l l y a v a i l a b l e .
An in te rmedia te coo l ing c i r c u i t i s , of cour se , not needed i n t h e
case of an i n d i r e c t gas t u r b i n e cyc le b u t , on t h e o t h e r hand, hea t ex-
changers between t h e primary and secondary loop and gas c i r c u l a t o r s a r e
r equ i r ed . However, t h i s design has , i n p r i n c i p l e , a number of very a t t -
r a c t i v e f e a t u r e s . F i r s t , it al lows employment: of a more advantageous
working medium, e .g . carbon d iox ide , i n t h e secondary loop while r e t a i n -
i n g helium as r e a c t o r coolan t . Secondly, t h e i n t e g r a t i o n of t h e primary
c i r c u i t i s e a s i e r . Th i rd ly , t h e number of tur>bines can be reduced s i n c e
it is determined s o l e l y by t h e maximum f e a s i h l e s i z e of a u n i t . Since
for t h e same
ed t o be only s l i g h t l y h igher t han i n t h e case of t h e d i r e c t helium c y c l e ,
t h e economic comparison of t h e two cyc le s red.uces t o t h e comparison of
t h e c a p i t a l investments involved.
r e a c t o r o u t l e t temperature t h e p l an t e f f i c i e n c y i s expect-
- ..
81 5
DIRECT HELIUM TLJRRINE SYSTEM
The Cycle
The schematic of a t y p i c a l d i r e c t t u r b i n e cyc le for a helium cooled
fast r e a c t o r i s shown i n Fig. 1 and t h e temperature-entropy diagram i s
shown i n Fig. 2 .
0 Helium a t about 80 b a r s and 650 C i s de l ive red from t h e r e a c t o r t o
t h e h igh p res su re t u r b i n e where it i s p a r t i a l l y expanded t o provide d r i v e
power f o r t h e compressors (2-3). From here t h e helium flows t o t h e low
p res su re t u r b i n e (3-4) which d r i v e s the e lec t r ica l genera tor . Leaving
t h e t u r b i n e s t h e helium passes through t h e low p res su re s i d e of t h e re-
gene ra to r (4-5) and t h e p recoo le r ( 5 - 6 ) i n which i t s temperature i s re-
duced t o about 2 5 C . Leaving t h e precooler t h e helium passes through t h e
two compressors (6-7 and 8 - 9 ) where i t s p res su re i s r a i s e d by a f a c t o r
of approximately t h r e e . Between t h e compressors an i n t e r c o o l e r i s i n -
s t a l l e d ( 7 - 8 ) i n which t h e gas g ives up t h e compression hea t t o t h e w a -
t e r of an in te rmedia te coo l ing c i r c u i t . Before being de l ive red back t o
t h e r e a c t o r t h e helium passes through t h e high p res su re s i d e of t h e r e -
genera tor (9-1) where it i s heated by t h e exhaust hea t o f t h e t u r b i n e .
The cyc le e f f i c i e n c y i s 30 %.
0
It should be noted t h a t a l though only one loop i s shown i n t h e d i a -
gram t h e actual helium flow is subdivided i n t o a t l eas t t h r e e p a r a l l e l
loops i n o rde r t o provide t h e r equ i r ed redundancy f o r t h e case when t h e
o p e r a t i o n a l turbogroups are u t i l i z e d f o r emergency cool ing .
The Design of t h e Helium Turbogroups
Two b a s i c arrangements of helium turbogroups are p o s s i b l e : t h e s i n g l e
s h a f t and t h e double s h a f t arrangement. For a number of reasons it is
p r e f e r a b l e t o u t i l i z e a two s h a f t design i n which t h e high p res su re t u r -
b ine , t h e compressors and t h e s t a r t i n g motor are mounted on one s h a f t and
t h e low p res su re t u r b i n e and t h e e l e c t r i c a l genera tor on t h e o t h e r . This
Starting
816 /
Fig
Regenerator
Fig. 1. Flow diagram of d i r e c t F!e-turbine c y c l e
k J Entropy: - kg "C
2 . Temperature-entropy diagram of d i r e c t He-turbine cyc le
817
arrangement eases both t h e load on t h e s t a r t i n g motor dur ing s t a r t - u p and
i t s use as an emergency d r i v e should it be r equ i r ed . However, t h e main
a t t r a c t i o n of t h e double s h a f t des ign i s t h e p o s s i b i l i t y of provid ing t h e
proper speed f o r t h e compressors while main ta in ing t h e low p res su re s h a f t
at t h e speed r equ i r ed f o r t h e genera tor .
A t t h e high helium p res su res requi red i n fast breeder r e a c t o r s t h e
volume flow of t h e gas through t h e turbomachinery is very l o u , even f o r
l a r g e power u n i t s . A s a consequence, s u b s t a n t i a l l y h ighe r r o t a t i o n a l
speeds than t h e synchronous speed of t h e genera tor are necessary i n or-
der t o reduce t h e number of s t a g e s and t h e diameter of t h e u n i t and t h u s
t o reduce t h e c o s t of t h e machine. The inc rease of t h e b lade speed i s
p o s s i b l e s i n c e t h e son ic v e l o c i t y i n helium is so high t h a t t h e per iphe-
r a l speed of t h e b lades is l i m i t e d by material stresses r a t h e r t han by
Mach numbers. This l i m i t a t i o n has c l e a r l y a s t r o n g e r impact on t h e design
of t h e high p res su re t u r b i n e than on t h e des ign of t h e compressors s i n c e
t h e t u r b i n e has t o work a t a h igher temperature . However, i n t h e p l a n t s
considered he re t h e t u r b i n e i n l e t temperatures are r e l a t i v e l y l o w , of
t h e order of only 650 C , so t h a t adequate c reep s t r e n g t h s can be provid-
ed by t h e use of n i c k e l a l l o y s .
0
A 335 MWe s p l i t - s h a f t turbogroup designed according t o t h e above c r i -
t e r i a is shown i n Fig. 3 . Both s h a f t s are housed i n one cas ing . There are
only two compressors mounted on t h e high p res su re s h a f t i n o rde r t o a l low
a two bear ing support o f t h e s h a f t and t h u s t o ease t h e v i b r a t i o n pro-
blem. On t h e o t h e r hand, t r ade -o f f s t u d i e s have shown t h a t t h e employ-
ment of t h r e e compressors does not b r i n g any r ea l economic advantage. The
improved thermodynamic performance r e s u l t i n g from t h e use of an a d d i t i o n a l
i n t e r c o o l e r is o f f s e t by t h e increased complexity of t h e system.
The high p res su re and t h e low p res su re t u r b i n e s are arranged c l o s e
t o each o t h e r so t h a t t h e volume of gas between them i s very small. This
is a very important design f e a t u r e , s i n c e it a l lows t h e l o s s of genera-
t o r load i n c i d e n t t o be c o n t r o l l e d by means of a simple va lve arrange-
ment.
818
0
111 0 I 2rn
Fig . 3. 335 MWe s p l i t - s h a f t He-turbogroup
A l l t u r b i n e and compressor d i s c s a r e f e m i t i c . However, i n t h e zone o f t h e first t u r b i n e - s t a g e s , a small coo l ing helium f low i s necessary i n
o r d e r t o keep t h e d i s c r i m t empera ture below 550 C . 0
The b lades o f t h e high p res su re t u r b i n e a r e made from Nimonic 115.
This material i s expected a l s o t o meet t h e requirements wi th regard t o
co r ros ion , s i n c e t h e use o f high p u r i t y helium i s assumed. Should t h i s
no t be t h e case, a more expensive molybdenum based a l l o y , e.g. TZM, must
be used.
The b lades of t h e low p r e s s u r e t u r b i n e a r e made from a u s t e n i t i c mate-
r i a l , e.g. G18B. The b lad ings o f t h e compressors are f e r r i t i c .
Convent ional , o i l l u b r i c a t e d j o u r n a l and t h r u s t bear ings a r e used.
To prevent excess ive o i l contaminat ion o f t h e helium, l a b y r i n t h type
s e a l s with back f l u s h i n g systems are provided.
819
The e n t i r e turbogroup i s 13.4 m long and i t s l a r g e s t diameter i s
3.7 m. The mass flow rate of helium i s 625 kg/sec. Other c h a r a c t e r i s t i c s
of t h e machine are summarized i n Tab. 1.
Table 1. P r i n c i p a l C h a r a c t e r i s t i c s of a 335 MWe He-Turbogroup
I n l e t p r e s s u r e , ba r s 81.8 42.2 26.6 47.6
Out le t p r e s s u r e , b a r s 42.2 27.2 48.1 90.7
Tip d iameter , m 1.462: 2.03s 1.42 1.36
Number of s t a g e s 6 6 6 8
653 462 24 24
46 2 356 114 124
0
0
A Last s t a g e
0
An a l t e r n a t i v e arrangement of t h e shafo; is presented i n Fig. 4. This
design i s a consequence of layout s t u d i e s which have shown t h a t a cons i -
de rab le reduct ion of t h e r e a c t o r bu i ld ing dimensions can be achieved by
a r r ang ing t h e high p res su re s h a f t s of t h e turbogroups v e r t i c a l l y while
keeping t h e r e l a t i v e l y s h o r t l o w p re s su re t u r b i n e s and t h e gene ra to r s i n
a h o r i z o n t a l p o s i t i o n . These gene ra to r s w i l l most probably be l o c a t e d
ou t s ide t h e main bui ld ing . Because o f t h e r a t h e r small weight of t h e ro-
t o r s mounted on t h e high p res su re s h a f t i t s v e r t i c a l o r i e n t a t i o n should
no t pose important development problems. The a x i a l load i s cons iderably
reduced by t h e upward d i r e c t i o n of t h e r e s u l t a n t t h r u s t so t h a t a con-
ven t iona l Mi tche l l bear ing l o c a t e d a t t h e upper end of t h e machine can
be used t o support t h e s h a f t .
820
111 0 I 2m
Fig. 4. 335 MWe He-turbogroup in angular s h a f t arrangement
n
821
The des ign of t h e ind iv idua l t u r b i n e s and compressors is i d e n t i c a l
wi th t h a t p rev ious ly descr ibed . The cas ing of t h e h igh p res su re s h a f t
and t h e cas ing of t h e low p res su re s h a f t are bo l t ed t o g e t h e r by means
of a r i g i d bend so t h a t t hey , i n f ac t , r ep resen t a s i n g l e p i e c e of m a -
ch inery . An annular duct wi th in t h e bend provides t h e connection between
t h e t u r b i n e s . In o rde r t o ob ta in a uniform gas flow t h e annulus is sub-
d iv ided i n t o a number of s e c t i o n s .
The turbogroup rests on a common p e d e s t a l wi th t h e gene ra to r . It i s
l a t e r a l l y cons t ra ined but can f r e e l y move i n t h e l o n g i t u d i n a l d i r e c t i o n
r e l a t i v e t o t he 'gene ra to r i n o rde r t o compensate for thermal expansions.
In t h e v e r t i c a l d i r e c t i o n t h e turLogroup i s not r equ i r ed t o a l i g n with
any o t h e r p i ece of equipment and t h u s is not l i m i t e d i n i t s movements.
It remains s t i l l t o examine a p o s s i b l e i n t e r a c t i o n of t h e v i b r a t i o n s o f
t h e two s h a f t s but it is be l ieved t h a t t h i s w i l l no t ca l l i n ques t ion
t h e f e a s i b i l i t y o f t h e above des ign .
Operation and Control of t h e Direc t He-Cycle System
St ar t -up
For an explana t ion of t h e s t a r t - u p procedure F ig . 1 is r e f e r r e d t o
again.
With t h e a i d of a s t a r t i n g motor, t h e h igh p res su re t u r b i n e s h a f t is
brought up t o approximately 20 % of i t s nominal speed. With i n i t i a l l y
c o l d helium, under t h e system equi l ibr ium p r e s s u r e , t h e r equ i r ed e l ec t r i -
cal power i s about 4 MW p e r group. The r e a c t o r is t hen brought t o power
and t h e gas temperature g radua l ly r a i s e d . With inc reas ing i n l e t gas t e m -
pe ra tu re t o t h e t u r b i n e , t h e speed of r o t a t i o n of t h e high p res su re s h a f t
i nc reases . A t t h i s s t a g e t h e low p r e s s u r e t u r b i n e is bypassed by opening
t h e va lve TB.
0 A t a t u r b i n e i n l e t temperature of about 350-400 C t h e high p res su re
s h a f t reaches s e l f s u s t a i n i n g cond i t ions . A s t h e gas temperature r i s e s
f u r t h e r , t h e low p res su re t u r b i n e is s ta r ted-up by gradual ly c l o s i n g the
822
valve TB. Once t h e r a t e d speed of t h e low p:ressure s h a f t is reached, t h e
gene ra to r i s synchronized and connected t o -the g r i d . By c l o s i n g t h e by-
pas s valve f u r t h e r , and inc reas ing t h e r e a c t o r o u t l e t temperature t o t h e
design va lue , t h e r a t e d power i s reached.
Power Control
For par t - load ope ra t ion t h e va lve C S ( s e e Fig. 1) i s appropr i a t e ly
opened. This causes t h e mass flow ra te through t h e compressors r e l a t i v e
t o t h e m a s s flow rate through t h e high p res su re t u r b i n e , t o be increased .
A s a r e s u l t , t h e speed of r o t a t i o n of t h e high p r e s s u r e s h a f t s i n k s t o a
new equi l ibr ium va lue . This r educ t ion i n t h e speed o f r o t a t i o n improves
t h e par t - load e f f i c i e n c y because of t h e smal.ler mass flow i n t h e r e a c t o r .
The r e t u r n t o f u l l l oad cond i t ions can be quick ly achieved by c l o s i n g t h e
va lve CS.
Fig. 5 shows t h e v a r i a t i o n of e f f i c i e n c y with power. For reasons g i -
ven e a r l i e r t h e e l e c t r i c i t y gene ra t ing c o s t s of a fas t breeder r e a c t o r
under pa r t - load cond i t ions should only be weakly dependent on t h e v a r i a -
t i o n of e f f i c i e n c y . Hence the shape of t h e above curve can be considered
as being s a t i s f a c t o r i l y f la t .
Q
Fig. 5. Var i a t ion of e f f i c i e n c y with power i n d i r e c t cyc le He- t u r b i n e p l a n t
A
823
Generator-Trip Inc ident
The i n s t a n t t h e gene ra to r l o s e s i ts l o a d , t h e low p res su re s h a f t ex-
pe r i ences an a c c e l e r a t i o n . A dis turbance s i g n a l from a number of indepen-
dent impulse senders ( e .g . loss o f load r e l a y , a c c e l e r a t i o n r e g u l a t o r )
l e a d s t o an immediate opening of a series of t u r b i n e bypass va lves TB.
It i s accep tab le if t h i s occurs 0.2-0.3 secs a f te r t h e load i s lost, a
t i m e i n t e r v a l , which from p a s t experience with a i r t u r b i n e s i s known t o
be e a s i l y achievable . A t t h i s t i m e , t h e overspeed of t h e low p res su re
s h a f t has not exceeded 5 %. The t u r b i n e bypass va lves are t o be so d i -
mensioned t h a t when they are f u l l y open, t h e expansion r a t i o of t h e low
pres su re t u r b i n e is only 1.03-1.04. Because t h e mass o f gas enclosed b e t -
ween t h e high and low p res su re t u r b i n e is s m a l l , t h i s r a t i o i s reached
so quick ly t h a t t h e r e s u l t i n g a c c e l e r a t i o n t i m e can hard ly cause an over-
speed i n excess of 7-8 %.
The moment t h e bypass va lve T B opens, t h e h igh p res su re t u r b i n e i s
sub jec t ed t o p r a c t i c a l l y t h e e n t i r e p re s su re d i f f e r e n c e , so t h a t t h e high
p res su re s h a f t begins t o accelerate a l s o . To prevent t h i s , t h e va lves C S
are s imultaneously opened, t he reby s h o r t - c i r c u i t i n g t h e compressor flow
pa th .
INDIRECT C02 TURBINE SYSTEM
The Cycle
A flow diagram of an i n d i r e c t carbon d iox ide t u r b i n e cyc le i s shown
i n F ig . 6 and t h e temperature-entropy diagram is shown i n Fig. 7 . This
arrangement has been s e l e c t e d from a number of p o s s i b l e a l t e r n a t i v e s be-
cause it seems t o be t h e most appropr i a t e f o r t h e p re sen t a p p l i c a t i o n .
Helium a t 85 bars is de l ive red from t h e r e a c t o r t o a number of pa ra l -
l e l h e a t exchanger u n i t s i n which it g ives up i t s hea t t o carbon d ioxide .
C i r c u l a t o r s r e t u r n t h e helium from t h e hea t exchangers back t o t h e reac-
824
4 L 7 , w
L 3 elium Circulator v “pawer lrculator Tvbine Turbine ComPeSsr M P
- /
2 Generator
I II 4
I Intercooler
Regenerator
First Second Regenemtor Regenerator
F i g . 6 . Flow diagram of i n d i r e c t CO - t u r b i n e c y c l e 2
E Precaaler
k J Entropy : - kg “C
Temperature-entropy diagram of i n d i r e c t CO - t u r b i n e c y c l e Fig. 7 . 2
825
0 t o r . Leaving t h e hea t exchangers, CO a t 216 b a r s and about 600 C passes 2 t o t h e high pressure t u r b i n e s (2-3) i n which it - p a r t i a l l y expands t o pro-
v ide power f o r d r i v i n g t h e helium c i r c u l a t o r s . Prom he re t h e CO f lows
t o t h e main t u r b i n e i n which it expands down from 180 t o approximately
22 b a r s (3-4). The main t u r b i n e d r i v e s t h e two compressors and t h e elec-
t r i c a l gene ra to r . Leaving t h e t u r b i n e , t h e CO
t h e second (5-6) r egene ra to r s i n which it g ives up i ts hea t t o t h e high
p res su re CO Now t h e CO passes t h e precooler ( 6 - 7 ) where i t s tempera- 2 ' t u r e is reduced t o 40 C . After having passed t h e low p res su re compressor
2 (7-81, t h e t h i r d r egene ra to r (8-9) and t h e
i s d e l i v e r e d t o t h e high p res su re compressor (pump). A t t h e pump i n l e t
i t s temperature is 25 C and i t s p res su re is s l i g h t l y s u p e r c r i t i c a l . Af t e r
i t s p res su re has been approximately t r i p l e d i n t h e pump (10-11) t h e CO
flows through t h e high p res su re s i d e of t h e second and t h i r d r egene ra to r s
(11-12) and then through t h e h igh p res su re s i d e of t h e f i rs t r egene ra to r
(12-1). Its temperature is now about 240 C and it is de l ive red back t o
t h e hea t exchanger (1-2). The s p e c i a l arrangement of t h e r e g e n e r a t o r s ,
i n which t h e h igh p res su re s i d e s of t h e second and t h i r d r egene ra to r s are
i n p a r a l l e l i s necessary due t o t h e s t r o n g inc rease of s p e c i f i c hea t of
carbon d ioxide wi th p re s su re i n t h e v i c i n i t y of t h e s a t u r a t i o n l i n e . The
o v e r a l l p l a n t effic-iency is 33.6 %.
crs 2
passes t h e f i rs t (4-5) and 2
2 0
i n t e rcoo le r (9-101, t h e CO
0
2
0
The Design o f t h e CO Turbogroups 2
The choice of one or more turbogroups f o r a 1000 M W e p l a n t depends
upon t h e cyc le parameters , t h e most important being t h e cond i t ion o f t h e
gas at t h e i n l e t t o t h e compressor. This is because f o r a given speed o f
r o t a t i o n , t h e maximum pe rmis s ib l e diameter of t h e machine is determined
by t h e v e l o c i t y o f sound i n CO
flow
For a given gas density, the maximum m a s s 2 ' r a te of gas is t h u s a l s o s p e c i f i e d .
The v e l o c i t y of sound i n CO i s low, almost f o u r t i m e s lower than i n 2 helium. Increas ing t h e speed o f r o t a t i o n of t h e compressor above t h e syn-
chronous speed o f t h e gene ra to r , as is forseen with helium t u r b i n e s ,
would i n t h i s case be p o i n t l e s s . Since t h e maximum u n i t power of a turbo- 0
826
group decreases approximately wi th t h e squarle of t h e compressor r o t a t i o -
nal speed an inc rease of t h e compressor speed would i n e v i t a b l y l ead t o a
s p l i t t i n g up of t h e p l a n t i n t o s e v e r a l p a r a l l e l turbogroups, without of -
f e r i n g any p a r t i c u l a r advantage. Mainly f o r t h e s e r easons , CO turboma-
ch ines o f s i n g l e s h a f t design were chosen. 2
In Fig. 8 , a 500 M W e , 3000 rpm s i n g l e s h a f t turbogroup i s shown. The
c y c l e p re s su res given i n Tab. 2 are such that they r e q u i r e t h e employment
o f two p a r a l l e l u n i t s . In o rde r t o be a b l e t o u s e a s i n g l e 1000 M W e t u r -
bogroup, it would be necessary t o have h igher gas p r e s s u r e s , e .g . 200 b a r
a t i n l e t t o t h e main t u r b i n e and 32 ba r before t h e compressor.
The turbogroup c o n s i s t s o f t h r e e components, t h e s h a f t s of which a r e
coupled t o g e t h e r : a t u r b i n e , a low p res su re compressor and a high p res su re
compressor. Each component i s loca ted i n i t s i n d i v i d u a l housing. The de-
s ign o f t h e machine i s e n t i r e l y convent ional as t h e requirements f o r t h e
s h a f t s e a l i n g are cons iderably less s t r i n g e n t t h a n i n t h e case of t h e d i -
rect cyc le helium machine. I t i s o f i n t e r e s t t o no te t h e small s i z e of
t h e high p res su re compressor, which is i n fact a pump r a t h e r t han a gas
compressor.
Thanks t o t h e low p e r i p h e r a l v e l o c i t y of t h e r o t o r s t h e b lades a r e
only moderately s t r e s s e d , d e s p i t e t h e h igh gas dens i ty . Therefore under
t h e p r e v a i l i n g temperature cond i t ions , an a u s t e n i t i c s t e e l would comple-
t e l y f u l f i l t h e requirements o f t h e t u r b i n e blading. The compressor blad-
i n g and a l l t h e d i s c s a r e made of f e r r i t i c m3teria1, perhaps s l i g h t l y
a l loyed t o inc rease cor ros ion r e s i s t a n c e . S imi l a r ly as i n t h e case of
helium t u r b i n e s , t h e d i s c r i m temperature i n t h e r eg ion of t h e first s ta -
ges of t h e t u r b i n e i s con t ro l l ed by means of a small flow o f co ld gas .
The e n t i r e turbogroup and t h e gene ra to r m e supported on a common
s t ee l pedes t a l . The turbogroup i s free t o expand i n an a x i a l d i r e c t i o n ,
r e l a t i v e t o t h e s t a t o r of t h e gene ra to r . The o v e r a l l l eng th o f t h e turbo-
group is 20.4 m and i t s l a r g e s t diameter i s :3.2 m . The mass flow ra te of
CO i s 3500 kg/sec. Other r e l e v a n t da t a of t h e machine are given i n Tab. 2 . 2
Fig. 8. 500 M W e CO 2 -turbogroup
828
Table 2 . P r i n c i p a l C h a r a c t e r i s t i c s o f a 500 MWe CO -Turbogroup 2
~ ~
Turbine Compressor Pump
577 40 25
343 159 k0
I n l e t p r e s s u r e , b a r s 1 8 0 2 1 74
0 I n l e t t empera ture , C
Out le t t empera ture , C 0
Out le t p re s su re , b a r s 2 2 76 229
Tip d iameter , m 1.75;" 1 . 2 1 0.60
Number of s t a g e s 6 7 4
fi L a s t s t a g e
Operat ion and Cont ro l of t h e I n d i r e c t CO -Cycle System 2
S t a r t -up
The s t a r t - u p of t h e turbogroup is achieved wi th t h e a i d o f an auxi -
pump, connected i n p a r a l l e l wi th t h e high p res su re compressor l i a r y CO
(main pump). The e l e c t r i c a l l y d r iven supplementary pump has a volume flow
rate of approximately 15 % o f t h a t o f t h e main pump.
2
The s t a r t - u p is c a r r i e d out a t a system equi l ibr ium p res su re which
should be s l i g h t l y above c r i t i c a l . Once t h e a .ux i l ia ry pump i s i n opera-
t i o n , gas begins t o c i r c u l a t e through t h e e n t i r e c i r c u i t , as t h e o u t l e t
p i p e of t h e main pump is f i t t e d wi th a non-return va lve . S ince the pres-
s u r e r a t i o of t h e pump i s i n i t i a l l y very low, i t s volume f low is h igher L5 t h a n nominal, about 1 .0 m /sec wi th a power consumption of approximately
5 M W . A t t h i s stage, t h e helium c i r c u l a t o r s are s e t i n ope ra t ion wi th
t h e a i d of a u x i l i a r y e lec t r ica l motors and t h e r e a c t o r brought t o power.
A s a r e s u l t , t h e tempera ture of t h e CO
g radua l ly increased . Already a t a tempera ture of 230 C t h e s p e c i f i c vo-
lume of CO
l e a v i n g t h e hea t exchangers i s 0
2
is about 1 0 times g r e a t e r than a t t h e pump i n l e t temperature 2 A
1
I
829
0 0
@ of 2 5 C. Hence, a t t h i s temperature of 230 C a t t h e i n l e t t o t h e t u r b i n e ,
t h e volume flow r a t e w i l l be about 1 0 m /sec. Th i s volume flow r e p r e s e n t s
approximately 30 % of t h e design va lue and is s u f f i c i e n t f o r s t a r t i n g
t h e turbogroup.
3
From t h e beginning t h e c i r c u l a t o r t u r b i n e s g radua l ly t a k e over more
and more of t h e d r i v e t o t h e c i r c u l a t o r . The moment t h e speed of r o t a t i o n
of t h e main pump i s s u f f i c i e n t l y high t o produce t h e same p res su re r a t i o
as t h e a u x i l i a r y pump, it begins t o t a k e p a r t i n i nc reas ing t h e CO mass
flow, so t h a t from a c e r t a i n poin t onwards, t h e a u x i l i a r y pump can be
switched o f f . A t t h i s p o i n t , t h e s e l f - s u s t a i n i n g cond i t ions of t h e turbo-
groups are reached. A s t h e gas temperature inc reases f u r t h e r , t h e turbo-
group a t t a i n s syhchronous speed. I t i s then connected t o t h e g r i d and
brought t o f u l l power.
2
Summarising one can say t h a t t h e l a r g e inc rease i n CO volume wi th 2
temperature a t a p res su re which i s s l i g h t l y over c r i t i c a l al lows t h e
s t a r t - u p of t h e system with r e l a t i v e l y l i t t l e e l e c t r i c a l power i n p u t , as
a l a r g e p a r t o f t h e s t a r t - u p power i s provided by t h e r e a c t o r h e a t .
Power Control
The power of t h e turbogroup i s r egu la t ed by varying t h e C 0 2 mass flow.
To achieve t h i s , t h e i n l e t temperature of t h e gas t o t h e pump is r a i s e d
by t h r o t t l i n g t h e coo l ing water flow. Due t o t h e r e s u l t i n g r educ t ion i n
gas d e n s i t y , t h e pump o u t l e t p re s su re (and consequently t h e p re s su re be-
f o r e t h e t u r b i n e ) i s reduced. Since t h e p re s su re before t h e pump has t o
be kept cons t an t , a p a r t of t h e CO
c u i t , as i s t h e case wi th t h e p re s su re l e v e l ( i nven to ry ) c o n t r o l method
normally employed with c losed cyc le a i r t u r b i n e s . The mass flow ra te
through t h e t u r b i n e g e t s sma l l e r and t h e p l a n t power s i n k s correspondingly.
conten t must be removed from t h e cir- 2
It should be noted t h a t when us ing t h i s method o f r e g u l a t i o n , t h e op-
e r a t i n g po in t of t h e compressor w i l l change t o a higher p re s su re r a t i o .
To keep t h e r e s u l t i n g e f f i c i e n c y v a r i a t i o n low down t o 60 % l o a d , t h e de-
@
830
s i g n poin t of t h e compressor should be set a t 80 % r a t h e r than 1 0 0 % of
t h e nominal load .
Let us now look at t h e behaviour of t h e helium blowers under t h e
above cond i t ions . It i s d e s i r a b l e t o keep t h e gas temperatures i n t h e
r e a c t o r , at any power l e v e l , as cons t an t as p o s s i b l e . This means t h a t t h e
CO tempera ture be fo re t h e blower t u r b i n e , a l s o remains about t h e same
under pa r t - load c o n d i t i o n s and t h a t t h e r a t i o of mass flow rates of t h e
two gases s t a y s unchanged. A s a r e s u l t , on t r a n s f e r r i n g t o par t - load ope-
r a t i o n , t h e r equ i r ed helium c i r c u l a t o r pumping power becomes cons iderably
lower than t h e power f o r t h e c i r c u l a t o r t u r b i n e s a v a i l a b l e a t t h e t i m e .
In o rde r t o r e s t o r e equ i l ib r ium, t h e c i r c u l a t o r t u r b i n e is t h r o t t l e d a t
o u t l e t .
2
With changes i n t h e coo l ing water tempera ture , t h e nominal power i s
maintained by t h r o t t l i n g t h e water flow when t h e water tempera ture s i n k s
and by swi tch ing on t h e p a r a l l e l connected a u x i l i a r y pump when t h e water
temperature rises from i t s nominal va lue .
Fig. 9 shows e f f i c i e n c y as a func t ion o f l oad . Load r educ t ion below
60 % can be reached by p a r t i a l l y s h o r t - c i r c u i t i n g t h e compressor f low
pa th .
Generator-Trip Inc iden t
When t h e gene ra to r l o s e s l o a d , t h e r e s u l t i n g a c c e l e r a t i o n of t h e
turbogroup opens va lves s h o r t - c i r c u i t i n g t h e compressor and pump flow
pa ths f u l l y , so t h a t t h e CO mass flow i n t h e c i r c u i t s i n k s t o i t s i d l e
running va lue a t t h e nominal r o t a t i o n a l speed.. To avoid an over-cool ing
of t h e r e a c t o r , t h e blower t u r b i n e i s simulta.neously t h r o t t l e d , as i n
t h e case of pa r t - load ope ra t ion p rev ious ly descr ibed .
2
. . . . . . - .. . . . . . . .- - .. -
831
Fig. 9. Var ia t ion o f e f f i c i e n c y wi th power i n i n d i r e c t cyc le CO - 2 t u r b i n e p l a n t
FINAL REMARKS
A v a l i d comparison of t h e two gas t u r b i n e systems d iscussed above and
t h e determinat ion of t h e i r p o s s i b l e economic advantages r e l a t i v e t o t h e
steam t u r b i n e system i s c e r t a i n l y not a simple t a s k . Since one i s looking
he re for r e l a t i v e l y s m a l l cos t d i f f e r e n c e s , it is important t o compare
optimum designs. In commercially o r i e n t e d systems t h i s means t h a t f o r
each v a r i a n t t h a t design must be determined which minimizes t h e cos t of
energy produced. To perform t h e op t imiza t ions , r e l i a b l e c o s t information
i s o f course r equ i r ed . This in format ion , however, can be suppl ied by
component manufacturers only on t h e b a s i s o f d e t a i l e d des igns .
Along with t h e opt imiza t ion s t u d i e s it is a l s o necessary t o compare
t h e o p e r a t i o n a l c h a r a c t e r i s t i c s of t h e d i f f e r e n t systems and t o determine
t h o s e a d d i t i o n a l f e a t u r e s which must be provided i n o r d e r t o ensure f o r
each system t h e same degree of confidence wi th regard t o p l an t s a f e t y .
In fact , t h e economic impact o f t h e o p e r a t i o n a l and s a f e t y a s p e c t s may
sometimes be s u f f i c i e n t t o in f luence s u b s t a n t i a l l y t h e comparison. @
832
Optimizstion s t u d i e s o f gas-cooled breeder r e a c t o r s employing d i f f e -
r e n t power conversion systems have been performed wi th t h e he lp of a se-
r ies o f computer codes r e c e n t l y developed a t t h e Swiss Federa l I n s t i t u t e
f o r Reactor Research. Using t h e s e codes, t h e t e c h n i c a l and economic cha-
r a c t e r i s t i c s o f t h e optimum p l a n t can be determined, for a s e l e c t e d cycle, by a j o i n t op t imiza t ion of t h e nuc lea r and t h e power genera t ing p a r t s of
t h e s t a t i o n .
It w a s t h e o r i g i n a l i n t e n t i o n of t h e au tho r s t o p re sen t t h e r e s u l t s
of t h e s e s t u d i e s at t h i s conference. However, t h e r e s u l t s obtained s o far
a r e considered not t o be s u f f i c i e n t t o permit clear conclusions t o be
drawn. More i n v e s t i g a t i o n s are s t i l l necessary and t h e au tho r s p r e f e r t o
r e s e r v e t h e i r judgement u n t i l t h e s e s t u d i e s m e completed.
n
Paper 3/139
DEVELOPMENT OF COATED PARTICLE F vEmAs-3xygDER REACTOR .-u
3 L o o
H . B a i r i o t i
J.M. Thomson
L . Aer t s
BELGONUC LEAIRE Member of t he GBR Assoc ia t ion
ABS TRACT
The paper summarizes the work c a r r i e d out i n order t o def ine a coated p a r t i c l e f u e l f o r an helium-cooled f a s t r e a c t o r .
The f i r s t type envisaged i s a modi f ica t ion of t he coa ted p a r t i c l e s developed f o r the HTR. Typica l ly , the ke rne l i s 800 microns mixed oxide, coa ted wi th PyC and S i c . i s t i c s , a mechanical design of such a p a r t i c l e has been c a r r i e d out and t h e in f luence of the in-put da t a has been cons idered . This has l e d t o a r e fe rence p a r t i c l e present ly being developed. The paper inc ludes the da t a on the f u e l ob ta ined on a l abora to ry s c a l e .
On the b a s i s of the a v a i l a b l e m a t e r i a l charac te r -
A s an a l t e r n a t i v e f o r t he S i c coa t ing , va r ious m e t a l l i c coa t ings have been considered : mechanical design cons ide ra t ions have enabled t o propose a few coa t ings des igns . The development of t hese coa t ings i s i n the i n i t i a l s t a g e of demonstrating the f e a s i b i l i t y ; pre l iminary r e s u l t s a r e included i n the paper .
Two m a i n draw-backs have appeared f r o m t hese two programs and have l e d t o t h e cons ide ra t ion of a l a r g e r s i z e p a r t i c l e (10 mm diameter) coa ted wi th a m e t a l l u r g i c a l l y s t rong coa t ing . compared . Various concepts are p resen t ly being
I NTRODUC T I ON
This paper o u t l i n e s a pre l iminary s tudy r e l a t i n g t o a poss ib l e design
f o r a coa ted p a r t i c l e f u e l f o r a gas breeder r e a c t o r cooled by helium.
833
834
Q The fo l lowing ope ra t ing cond i t ions have been adopted a s guiding-
l i n e :
- Burn-up
- Neutron f l u x
10 % fima
cm-2 ( > 0.10 M ~ V )
- Maximum gas temperature 800°C
- Power dens i ty i n the f u e l reg ion 500 - 1000 MW/m3
- Density
- Kernel diameter 0.8 - 10.0 mm
80 - 95 % TD
2 ' - Fuel ( u- Pu 1 0
A pre l iminary scanning program i s being pursued on these bas i c
da t a , wi th no at tempt t o opt imize.
DESCRIPTION OF THE COATED PARTICLE FOR A GBR
The f u e l c o n s i s t s of a mixed dioxide U-llu sphere coa ted by seve ra l
concen t r i c l a y e r s (F ig . 1).
The two s t r u c t u r a l l a y e r s a r e success ive ly : t h e bu f fe r layer and
t h e S ic o r m e t a l l i c l a y e r . A s w i l l be expla ined l a t e r , an in te rmedia te
l aye r between t h e s e two ones might be necessary and one or more p r o t e c t i v e
l a y e r s can be added.
The bu f fe r l aye r i s p re sen t ly supposed t.o be a l o w d e n s i t y PyC l aye r ;
i t performs two v i t a l func t ions :
- it p r o t e c t s a l l t h e o ther l a y e r s aga ins t f i s s i o n product r e c o i l bombard-
ment e f f e c t s ; on t h a t account , i t should be approximately 30 microns
t h i c k f o r t he envisaged d e n s i t i e s ;
- i t provides f r e e volume through i t s i n t e r n a l po ros i ty and, by i r r a d i a t i o n
induced shr inkage, permits k e r n e l swel l ing and minimizes f i s s i o n gas
pressure . The S i c or m e t a l l i c l aye r assumes two func t ions :
- i t i s the pressure v e s s e l ,
- i t a c t s a s b a r r i e r f o r s o l i d f i s s i o n product d i f f u s i o n . I
A
design :
835
MATERIALS FOR THE PRESSURE VESSEL
he f i r s t s t age , t h r e e m a t e r i a l s were consider d f o r a prel iminary
a vanadium a l l o y , chromium and s i l i c o n ca rb ide .
Physic a 1 pro p e r t i e s
The phys ica l p r o p e r t i e s which a r e of main i n t e r e s t are given i n
Table 1.
Table 1. Phys ica l p r o p e r t i e s of poss ib l e pressure v e s s e l m a t e r i a l s
Ma te r i a l v C r S i C Nb
Melting poin t "C 1,900 1,875 2,600 2,500
T r a n s i t i o n temperature "C l , O O O a 0-600
Melting poin t of the oxide "C 6 60 2,400 1,750 1,500
Dens i t y g/cm3 6 .1 7.19 3 .2 8.6
1, gooa b
_ _ ~ _ _
a
b R e c r y s t a l l i z a t i o n
Duct i le t o b r i t t l e t r a n s i t i o n .
Chromium i s undergoing the d u c t i l e t o b r i t t l e t r a n s i t i o n i n the
opera t iona l temperature range '. occurs depends mainly on t h e impur i ty con ten t , the coo l ing r a t e , t h e g r a i n
s i z e , t h e s t r a i n r a t e and the specimen p repa ra t ion technique .
The temperature a t which the t r a n s i t i o n
Vanadium, being a very o x i d i z a b l q m e t a l , has t o be a l loyed t o elements
reducing t h i s o x i d i z a b i l i t y l i k e aluminum, chromium or s i l i c o n . The compa-
t i b i l i t y of t he a l l o y wi th the oxide f u e l i s f a i r ; with ca rb ide f u e l , a 2
r e a c t i o n zone of 70-75 microns has been de tec t ed a f t e r 1000 h r s a t 800°C . Pyrocarbon has t o be d i scarded , due t o f a s t neutron dimensional
change s .
836
The s i l i c o n carb ide r e a c t s w i t h oxygen forming a v o l a t i l e compound
a t low oxygen p a r t i a l pressures ; vanadium and niobium r e s p e c t i v e l y have
the same tendency but t o a decreasing e x t e n t .
1 ~3 ,4 95 96 Mechanic a 1 proper t i e s
The main mechanical p r o p e r t i e s a r e g iven i n Table 2, f o r a tempera-
t u r e of 800°C.
Table 2 . Mechanical p r o p e r t i e s of t he c o n s t i t u t i v e m a t e r i a l s
~
P r o p e r t i e s Units V C r S i C Buffer PyC (u-PU)~, ,
6 6 6 Young's modulus p s i 19 x 10 36 x 10 52.5 x lo6 2.4 x lo6 16 x 10
s t r e n g t h p s i 10 x lo3 18 x lo3 i+6 x 10 - nd U1 t imat e t ens i 1 e
- nd Yield s t r e n g t h p s i 4.0 x 10 15.5 x lo3 46 x 10
Thermal expansion "C 9.4 x 5 . 5 ~ 1 0 - ~ 5 ,, 35 x 5 . 4 ~ 1 0 - ~ 10 x
Poisson ' s r a t i o - 0.33 0.33 0..25-0.3 0.24 0.23
The r m a 1 conduc t iv i ty W/m"C 38 46 36 75 3 .O
3
3 3
-1
The neutron f l u x enhances the thermal c reep t o an unknown e x t e n t f o r
most m a t e r i a l s cons idered . An equiva len t c r eep r a t e was t h e r e f o r e s e l e c t e d
and t h e s e n s i t i v i t y of t he va r ious des igns t o t h e c r e e p c o e f f i c i e n t was
a s ses sed . For vanadium and chromium, the fo l lowing r e l a t i o n was u t i l i z e d
a t 800°C :
-22 3.5 A = 1.62 x 10 x (T E
and f o r s i l i c o n ca rb ide ( a t t he same temperature) :
-0.65 = 4.16 x x Q x t E
837
0 where :
U = t he s t r e s s ( p s i )
t = time (second) a t t he given s t r e s s
- = f r a c t i o n a l c r eep r a t e (s-’). E
Nuclear p r o p e r t i e s
Figure 2 shows the evo lu t ion of t he macroscopic cap tu re c ros s -
s e c t i o n c as a func t ion of neutron energy f o r s e v e r a l elements (V, C r ,
T i , Fey Z r , Nb). The average neutron energy i s around 0.15 MeV f o r a
spectrum r e p r e s e n t a t i v e of an helium-cooled breeder r e a c t o r .
C
Table 3 gives the (n , a ) and ( n , p) microscopic c ros s - sec t ions , i n
m i l l i b a r n s , f o r a r e p r e s e n t a t i v e f i s s i o n spectrum. From these d a t a i t
appears t h a t vanadium would give a b e t t e r neutron economy and a b e t t e r
s t a b i l i t y under i r r a d i a t i o n than chromium.
Table 3 . Microscopic c ros s - sec t ion (mb) f o r t he ( n , a ) and (n , p> r e a c t i o n s
Element (n , a ) U “ ( n , p)
v 0.04 1 .o C r 0.34 1.76
T i 2 . 9 2.9
The macroscopic c ros s - sec t ion of capture and the dimensional change
of s i l i co r ! ca rb ide under i r r a d i a t i o n are n e g l i g i b l e .
BUFFER LAYER PROPERTIES
The bu f fe r l aye r i s assumed t o have a d e n s i t y between 1.0 and 3 1.2 g/cm . Table 2 gives the p r o p e r t i e s u t i l i z e d f o r design purposes.
838
A d e n s i f i c a t i o n occurs quick ly under i r r a d i a t i o n t o reach a c r y s t a l - 3 21 lographic va lue of 1.9 g/cm a f t e r a neut ron dose of 5 x 10 . The f u r t h e r
a n i s o t r o p i c dimensional changes a r e supposed t o be counterac ted by i r r a d i a -
t i v e c reep t h e l aye r being squeezed between the k e r n e l and t h e pressure
l a y e r .
FUEL PROPERTIES
Table 2 g ives the des ign d a t a u t i l i z e d f o r a (U-Pu)O f u e l of 80 % 2
TD, a t a temperature of 1000°C approximately.
The volumetr ic f u e l swel l ing r a t e i s assumed t o take t h r e e d i s c r e t e
va lues :
up to 2.85 % fima
2.85 t o 7.65 % fima
7.65 t o 12 .0 % fima
3.51 x lod2 % / % f i m a
1.00 x IO-' % J yo fima
5.58 x lo-' % J % f ima.
These va lues were i n t e r p o l a t e d from experimental swe l l ing curves .
The f i s s i o n gas and C O p re s su re bui ld-up a r e taken i n t o account
a s burn-up dependent.
COMPUTER CODE FOR MECHANICAL DESIGN
A COCONUT i s a computer code which permits t o c a l c u l a t e t he s t r e s s e s
and s t r a i n s i n t h e f u e l and the c o a t i n g l a y e r s and has been developed a t
BELGONUCLEAIRE s i n c e 1967 f o r the HTR Fuel Program . 7
It proceeds through success ive t ime s t e p s and has been w r i t t e n f o r
any f u e l , coa t ing m a t e r i a l , number of l a y e r s , temperature and i r r a d i a t i o n
evo lu t ion .
The s t r e s s e s and s t r a i n s i n t h e l a y e r s a r e u s u a l l y based on the f i s s i o n
gas and C O p re s su re , t he f u e l swel l ing and t h e dimensional changes induced
by t h e thermal h i s t o r y and the i r r a d i a t i o n damages. A t each time s t e p , t h e
'Coating - Computation f o r w c l e a r Technology.
8 39
s t r e s s e s and s t r a i n s a r e co r rec t ed f o r c r eep e f f e c t s induced by i r r a d i a t i o n
and temperature .
For high power dens i ty cond i t ions , t he s t r e s s e s induced by the t h e r -
m a l f l u x through the coa t ing a r e a l s o considered, through a subrout ine
t rea tment .
PRELIMINARY D E S I G N RESULTS
Temperature p r o f i l e
Consider ing a power dens i ty of 800 MW/m3 ( f u e l ) w i th 60 v / o loading
(volumetr ic propor t ion of coa ted p a r t i c l e s ) , one o b t a i n s , f o r a small
s i z e (1000 microns) coa ted p a r t i c l e , a temperature d i f f e r e n c e of 1 0 0 ° C
between t h e c e n t e r of the f u e l and the outer su r f ace of t h e pressure
v e s s e l .
It appears t h a t the h igh power dens i ty reached wi th moderate f u e l
temperatures i s one of the most important advantages of the GBR's f u e l l e d
wi th coa ted p a r t i c l e s and d i r e c t cool ing through the bed.
E f f e c t of t he bu f fe r t h i ckness on the evo lu t ion of t he t a n g e n t i a l s t r e s s e s
This i n f luence has been emphasized f o r vanadium a l l o y as pressure
v e s s e l , w i t h a ke rne l diameter of 800 m i c r o n s , a t o t a l c o a t i n g th ickness
of 100 microns and a coolan t gas a t 700 p s i .
F igure 3 shows the evo lu t ion of the t a n g e n t i a l s t r e s s e s wi th a
bu f fe r th ickness of 5 microns and a vanadium a l l o y th i ckness of 95 microns.
Up t o 0 .3 % fima t h e v e s s e l i s submit ted t o an e x t e r n a l p re s su re ,
the cool ing gas pressure being h igher t han the f i s s i o n gas and the CO
pressure .
a l l e v i a t e d a s a consequence of t h e gap c losu re between the bu f fe r and t h e
pressure v e s s e l .
pressure vessel .
g e n t i a l s t r e s s e s makes the equiva len t s t r e s s va lue pass through zero
and t h e coa t ing g e t s soon i n t ens ion . Af te r 8 % fima, the t a n g e n t i a l
A t 0.4 % fima, t he e f f e c t of t he pressure d i f f e rences i s
A t t h i s moment, t he f u e l swel l ing s tar ts a f f e c t i n g the
Around 7 % fima, t h e evo lu t ion of t h e r a d i a l and tan-
840
t Table 4 . Coating s t r a i n a t 10 % fima
7 Buffer t h i ckness
( m i c r on>
S t r a i n
(%I
Diameter i nc rease
( %>
0 1 . 7 1 . 7
1 . 6
5
20
s t r e s s b u i l d s up i n t ens ion and p r a c t i c a l l y l e v e l s of f due t o the c reep
phenomenon,
Figure 4 presen t s t h e same evo lu t ion but wi th a bu f fe r th ickness
of 20 microns and a vanadium a l l o y thickness of 80 microns. The gap
c l o s e s l a t e r (1 .3 % f ima) . A t the end of l i f e , we have p r a c t i c a l l y the
same evo lu t ion a s f o r the previous c a s e .
For no bu f fe r l aye r and 100 microns of vanadium a l l o y (F ig . 5 ) ,
t h e evo lu t ion i s p r a c t i c a l l y the same, a t t he end of l i f e , as f o r the
f i r s t case ( b u f f e r 5 microns and 95 microns vanadium a l l o y ) .
A s can be seen , t he t h r e e cases g ive a very low t e n s i l e s t r e n g t h .
It corresponds t o l e s s than 5 % of the rup tu re s t r e n g t h of vanadium and
could not by i t s e l f be a c r i t e r i o n t o s e l e c t n e i t h e r a bu f fe r nor a v e s s e l
t h i ckness . These r e s u l t s should however be i n t e r p r e t e d wi th c a r e , s ince
swel l ing phenomena might occur a t t he h igh f:Luences and inc rease the s t r e s s
l e v e l .
The s t r a i n s a t 10 % fima a r e given i n Table 4 ; they a r e p r a c t i c a l l y
unaf fec ted by t h e space p a r t i t i o n between the bu f fe r and vanadium l a y e r s .
The diameter of the coa ted p a r t i c l e s v a r i e s over t he same range a s the
mentioned s t r a i n ; it decreases i n i t i a l l y when t h e vanadium coa t ing co l l aps -
es on the d e n s i f i e d b u f f e r l a y e r and inc reases l a t e r . Although, a l l the
f u e l beds b r e a t h t o the same e x t e n t , t h e f i n a l expansion
a t the end of l i f e depends on the bu f fe r th ickness which could be s e l e c t e d
according t o d e s i r a b l e bed behaviour during i r r a d i a t i o n .
841
E f f e c t of the coa t ing m a t e r i a l a s a pressure v e s s e l
F igure 6 gives t h e stress evo lu t ion i n a chromium c o a t i n g . The
coa ted p a r t i c l e i s made of a 800 microns k e r n e l diameter , a bu f fe r
t h i ckness of 5 microns and 95 microns of chromium. The evo lu t ion i s the
same a s f o r t he vanadium case wi th t h e same dimensions ; t h i s r e s u l t s
mainly from t h e adopt ion of a same c r e e p law, The s t r e s s e s a r e h igher i n
abso lu t e va%lue because chromium Young's modulus i s higher t han vanadium
Young's modulus ; t he r e l a t i v e va lue i s however only 2 % of the rup tu re
s t r e n g t h , For what coa t ing s t r a i n and dimensional s t a b i l i t y of t he
coa t ing i s concerned the same va lues apply f o r vanadium and chromium.
The only arguments f o r a choice between the two m a t e r i a l s a r e then :
- t he i r r a d i a t i o n s t a b i l i t y ( i n favour of vanadium) ;
- t he c o m p a t i b i l i t y wi th the s u b s t r a t e and the coolan t ;
- t he thermal cyc l ing behaviour ; t h e chromium i s favoured wi th a
t h i c k bu f fe r and the vanadium wi th a t h i n o r no b u f f e r ;
- the manufacturing problems and coa t ing q u a l i t i e s ;
- a b e t t e r d e f i n i t i o n of t h e r e l a t i v e c r e e p behaviour under i r r a d i a t i o n .
F igure 7 g ives the stress evo lu t ion i n a s i l i c o n ca rb ide coa t ing .
The coa ted p a r t i c l e i s made of a 800 microns k e r n e l diameter , a bu f fe r
t h i ckness of 20 microns and 80 microns of Sic. Compared t o the vanadium
case , wi th the same dimensions, t h e s t r e s s e s evo lu t ion i s q u i t e d i f f e r e n t .
The gap c losu re occurs very l a t e (8 % f ima) , because the S i c thermal c r e e p
i s s m a l l compared t o metallic thermal c reep . When t h i s gap i s c losed , t h e
coa t ing g e t s immediately i n t e n s i o n because of t he thermal c r e e p and
Young's modulus c h a r a c t e r i s t i c of t h e m a t e r i a l . The c o a t i n g s t r a i n and
diameter v a r i a t i o n range a r e small ( 0 . 3 %). The t e n s i l e s t r e s s could be
reduced by inc reas ing the bu f fe r t h i ckness t o an e x t e n t depending on the
k e r n e l dens i ty (Table 5) ; t h i s would a l s o decrease the coa t ing s t r a i n
and s t a b i l i z e the diameter . The h ighes t heavy metal loading i s obta ined
f o r a dens i ty around 90 % TD. The u t i l i z a t i o n of S i c i s then only
dependent on :
- the i r r a d i a t i o n behaviour t o high fluence:;,
- t he compa t ib i l i t y wi th f u e l and coo lan t ,
- t he l o s s of coolan t s a f e t y requirements .
Table 5. Suggested bu f fe r th icknesses wi th S i c coa t ings
Kerne 1 dens i ty Re la t ive bu f fe r t% TD) th i ckness (th/D)
80 0.04
90 0.05
95 0.06
FEASIBILITY TESTS
Plutonium bear ing coa ted p a r t i c l e f u e l has been f a b r i c a t e d s ince
1962 by the Belgian r e sea rch team lo. Development work on coa ted p a r t i c l e
c a r r i e d out i n the frame of t h e HTR f u e l program i s a l s o providing use fu l
background .
Kerne 1
Three poss ib l e f a b r i c a t i o n techniques can be s e l e c t e d , each one
having i t s proper l i m i t s .
Powder r o u t e s
Agglomeration technique :
Kernels up t o 8000 microns have been f a b r i c a t e d but a normal s p h e r i c i t y
can be guaranteed only up t o 1200 microns. I 'ollowing the UO rou te den-
s i t i e s a s low a s 80 % TD can be achieved and by the U 0 r o u t e , as low
Spheres above 2000 m,crons can be success fu l ly manufacture1 i n t h e dens i ty
range 75-98 % TD (F ig . 10).
mechanical s t r e n g t h w i l l be the l i m i t i n g f a c t o r .
It has t o be no t i ced t h a t below 80 % TD the
Chemical p r e c i p i t a t i o n method
By s tandard techniques and an ox ida t ive c a l c i n a t i o n , d e n s i t i e s a s l o w
as 70 % TD can be achieved wi th UO the p a r t i c l e s remaining s u f f i c i e n t l y
s t rong ; t he diameter limit i s s e t a t max. 1200 microns '. same r e s u l t s can be achieved wi th mixed oxides .
2' Undoubtedly the -
A Sol-Gel technique descr ibed e a r l i e r by one of t he au thors could
a l s o be app l i ed even f o r lower d e n s i t i e s .
Ceramic coa t ings
Dimensional limits
Coat ings of PyC, S i c and Z r C fol lowing the c l a s s i c a l f l u i d i z e d bed
technique have been success fu l ly achieved on ke rne l s of 800 microns and
80 % TD. The ke rne l diameter might be increased i f the dens i ty drops below
80 % but up t o now no evidence i s a v a i l a b l e .
The d i r e c t depos i t ion of o ther carb ide coa t ings has not ye t been
i n v e s t i g a t e d . Some t r i a l s t o carbonize niobium depos i ted on PyC were not
success fu l due t o s p a l l i n g of the l a y e r s . It was concluded t h a t the carb ide
must be formed i n s i t u during coa t ing .
For high temperature coa t ing of ke rne l s of l a r g e r diameters , new
coa t ing equipments should be designed and developed.
In te rmedia te l a y e r s
For manufacturing and q u a l i t y reasons , a t r a n s i t i o n layer should be
incorpora ted between the bu f fe r and the S i c .
l a y e r s could be envisaged (F ig . 8) :
The fol lowing success ion of
844
- Porous PyC l aye r wi th a dens i ty of 1.0 g/crn3 f o r f i s s i o n product r e c o i l
and a v a i l a b i l i t y of f r e e space, a s mentioned e a r l i e r .
- A t r a n s i t i o n o r s c a l i n g layer of PyC wi th ,a dens i ty inc reas ing t o 3 1.6 g/cm or more. The t o t a l t h i ckness of t h e bu f fe r and t r a n s i t i o n
l aye r s should be 30-50 microns.
3 - A S i c l aye r wi th a dens i ty of 3.2 g/cm and a th i ckness over 30 microns.
- Sic i s known t o be uns t ab le under flowing gas wi th a low oxygen p a r t i a l
p ressure so t h a t a supplementary p r o t e c t i o n l aye r i s probably necessary.
This l aye r could be Nb, NbC o r Z r C . V o r 'GI a r e not excluded but look
l e s s promising from the compa t ib i l i t y point: of view,
Z r C seems t o be t h e most adherent and r e s i s t a n t t o thermal shocks ( t h e r -
m a l expansion c o e f f i c i e n t 6.6 x 1 0 q 6 / " C versus 5.35 x 10
Of a l l m a t e r i a l s ,
-6 /"C f o r S i c ) .
Ref rac tory metal coa t ings
The r e f r a c t o r y metal coa t ings can be con.sidered as a proper coa t ing
o r as a p r o t e c t i v e l aye r on the ceramic pressure v e s s e l . Metal coa t ing
can be depos i ted fol lowing t h r e e d i f f e r e n t techniques .
Vacuum m e t a1 l i z a t i on
The c l a s s i c a l vapor i za t ion method or t he plasma s p u t t e r i n g technique i s
developed by EURATOM-Ispra. Nearly no l i m i t a t i o n e x i s t s on the k ind of
metal and the dimensions and weight of t he p a r t i c l e , but t h e maximum i n -
d u s t r i a l l y conceivable l aye r t h i ckness i s 10 inicrons. Tes ts have been
performed on coa ted p a r t i c l e s up t o 8 microns (F ig . 9 ) .
E 1 ec t r o l y t i c depos i t i on
A t Mol, t he method has been app l i ed s u c c e s s f u l l y on f i s s i l e material
f o r Nb, W , Mo, Fe and N i lo. The method seems t o be very a t t r a c t i v e except
f o r the f a c t t h a t t he m a t e r i a l i s depos i ted a t room temperature ; the coated
p a r t i c l e s a r e then under s t r e s s a t ope ra t ing temperature, except f o r vana-
dium. Moreover, ex tens ive t e s t s a r e necessary t o prove the v a l i d i t y of the
1
a45
@ technique, f o r what t h e q u a l i t y of t h e l aye r i s concerned ( impur i ty , s t r u c -
t u r e , e t c ... ) ; t he maximum laye r t h i ckness f o r q u a l i t y reasons i s thought
t o be l e s s than 150 microns.
High temperature c l a s s i c a l vapor depos i t i on
The method a l r eady appl ied i n our l a b o r a t o r i e s on Z r , Nb, W , A 1 2 0 3 ,
A1N and Z r C i s app l i cab le t o most of t h e r e f r a c t o r y m a t e r i a l s . The
th i ckness might be l imi t ed by the tendency t o form a d e n d r i t i c s t r u c t u r e ,
but t h i s can normally be overcome. The m a t e r i a l i s u s u a l l y d u c t i l e and
adherent bu t t h e same l i m i t a t i o n s on ke rne l s i z e a s expla ined previously
(Cf r . page 9) a r e worth. Coating i n a r o t a r y furnace can however be
envisaged (F ig . 10).
Prel iminary i r r a d i a t i o n t e s t
Samples of 800 microns UO ke rne l s coa ted wi th S i c a r e i n the BR2 2 r e a c t o r i n a s t a t i c helium atmosphere a t approximately 800°C. This
sc reening t e s t w i l l be stopped a t a low f luence (0.9 x lo2' n/cm > 0.1 MeV). 2
C ONC LUS IONS
S i l i c o n ca rb ide appears p re sen t ly a s t he most favourable m a t e r i a l
f o r mechanically r e s i s t a n t l a y e r . It imposes however the presence of a
q u i t e t h i c k b u f f e r ( s t r e s s l i m i t a t i o n ) and a t r a n s i t i o n l a y e r , and the u t i -
l i z a t i o n of s m a l l ke rne l s (800 microns) . The heavy metal loading i s the re -
f o r e l i m i t e d t o 2.4 g/cm . 3
Metallic coa t ings can be designed and f a b r i c a t e d t o reach heavy metal 3 loadings over 3 . 0 g/cm , s ince no l i m i t a t i o n s e x i s t on ke rne l s i z e .
core should however be designed t o accommodate f o r a d i a m e t e r v a r i a t i o n of
t h e coa ted p a r t i c l e s dur ing l i f e up t o q u i t e l a r g e va lues (1 .7 X I .
The
846
ACKNOWLEDGEMENT
The experimental programme on coating was performed by the
CCR - Ispra (Mr. Block and Mr. Brossa), the S.C.K.-C.E.N. (Mr. Vangeel)
and by the Joint C .E.N.-BELGONUCLEAIRE The S .C .K.-C .E.N.
is also participating through the irradiations in BR2.
Plutonium Group.
The authors like finally to thank the GIlR Group (Brussels) for
fruitful discussions, and especially Mr . Vieider .
REFERENCES
1. Chromium and Chromium Alloys, DMIC R e p . 2 3 4 ( O c t . 1, 1 9 6 6 ) . - 2. J. Trouwe, Y. Kauffmann and A. Accary, L'Utilisation du Vanadium
et de ses Alliages en Energie Nuclgaire, En. Nucl., vol. 11, nr. 7, (Oct. 1969).
3. Union Carbide Metals Review, vol. 2, ni:. 1.
4 . U. Hebner, Termische und Elektrische Leitfzhigkeit von Vanadin- legierungen zwischen 20 und 650" Cy Journ. of Nucl. Mat. 32 p. 88 - 100, (1969).
- -3
5. Private communication.
6. R. W. M. D'Eye, The Development of Silj-cium Carbide Clad Fuel Pins for Advanced Gas-Cooled Reactors, Symposium on Advanced and High Temperature Gas-Cooled Reactors, Jiflich/Federal Republic of Germany, 21/25 Oct., 1968, IAEA - SM 13-1/35.
7. J. M. Thomson, Computation for Coated Particle Fuel Design, BELGONUCLEAIRE Repa. BN 6911-05, (Nov. 1.969).
8. Prof. Facchini, Private communication.
9. H. Bairiot and G. Vanhellemont, Product.ion of Th and Pu diluted Sol-Gel Particles, IAEA Panel on Sol-Gel Processes for Ceramic Nuclear Fuel, Vienna, (May 1968)
10. C. Sari and I. Lafontaine, Preparation et recouvrement de parti- cules sphgriques de Pu02 et de mixtes (U-Pu)02 , BELGONUCLEAIRE Rep. BN 6309-23, (Sept. 1963).
A
NUCLEURE
FIG. 1
VESSEL - PRESSURE VESSEL
DETAIL OF COATING LAYERS
FOR SMALL SIZE COATED PARTICLE
loop I
I
EC Crr?’
15
10
5
I’0-2 A
1 o d 1
loo 10’
848
I
"e
2 .o
1.0
0 -
- 1.0
-2.0 -
I 103 psi METALLIC COATED PARTICLE
(U-PU)O2 8001.1
BUFFER 5 P
VANADIUM 95 1.1
HELIUM GAS PRESSURE 700 psi
RUPTURE STRENGTH ( IRRADIATED) L.lO3 psi
w@ NUCWRE
I , 1 2 3 4 5 6
*le FlMA
VANADIUM COATING ( 95p )
FIG. 3 1 GAP CLOSURE BETWEEN BUFFER AND PRESSURE VESSEL
2'o i 1.0 4
METALLIC COATED PARTICLE
( U - P U ) O 2 8001.1
20 L1 BUFFER
VANADIUM 80 p
HELIUM GAS PRESSURE 700 psi RUPTURE STRENGTH I IRRADIATED 1 4.1113 psi
'I. FlMA
0
1 2 3 4 5 6
- 1.0 -
VANADIUM COATING ( 80 p )
GAP CLOSURE BETWEEN BUFFER AND PRESSURE VESSEL
-2-o !A FIG. 4
849
CHROMIUM COATING
% 0 2 .o
1.0
0
1.0
2 0
0
-lD
2D
x 103 psi
1 1 3 0 ~ ---
METALLIC COATED PARTICLE
(U-Pu 1 0 2 800 p VANADIUM 100 p
RUPTURE STRENGTH I IRRADIATED) 4.103 psi
HELIUM GAS PRESSURE 700 psi
J -- : w 3 4 5 6 7 9 10 BURN UP 1 2
'1, F IMA
VANADIUM COATING (loop
FIG. 5
x 103 psi METALLIC COATED PARTICLE
(U-FU)02 800p
BUFFER 5P
CHROMIUM 95 )r HELIUM GAS PRESSURE 700 psi
RUPTURE STRENGTH (IRRADIATED) 15.103 psi
FIG. 6
=e 20
10
0
-6
Sic COATED PARTICLE 103 x psi ( u-Pu 102 800 p'"
20 P @JP
BUFFER
sic E O R HELIUM GAS PRESSURE 700 psi
RUPTURE STRENGTH I IRRADIATED) 50.103 psi
6 7- 1 2 3 4 5
SILICON CARBIDE COATING
w 9 10 BURN UP
*I. FlMA
GAP CLOSURE BETWEEN BUFFER
AND S;C
FIG. 7
Fig. 8. SIC coatings.
851
Fig. 9. Nb protective layer on a small particle.
Fig. 10. Niobium coating on a 2 . 3 mm P ~ K - L X L ~ :
(by decomposition of NbCl >. 5
DISCUSSION
M. D a l l e Donne: I do n o t t h i n k t h a t t h e i r r a d i a t i o n per formance of
c o a t e d p a r t i c l e s i n t h e r m a l r e a c t o r s i s c o m p l e t e l y i n d i c a t e of t h e Ir
b e h a v i o r i n f a s t r e a c t o r s , due t o t h e v e r y b i g d i f f e r e n c e i n f a s t f l u e n c e ;
f o r i n s t a n c e , PYC i s o u t f o r f a s t r e a c t o r s . W e a r e a l s o l o o k i n g t o
m e t a l c o a t i n g s ( V , C r ) , b u t w e have d i f f i c u l t i e s i n making t h i c k l a y e r s
of m e t a l (100 microns o r s o ) , 5-10 microns a r e no problem; b i g g e r l a y e r s
a r e . Could you comment on t h i s ?
H. F. B a i r i o t : W e a g r e e t h a t t h e r m a l i r r a d i a t i o n s a r e n o t comple t e ly
s i g n i f i c a n t . They a r e , however, r e l e v a n t a s s c r e e n i n g tes ts t o i n v e s t i -
g a t e c o m p a t a b i l i t y , t h e r m a l s t r e s s i n g , t e n s i l e b e h a v i o u r , e t c . , i n f a i r l y
r e p r e s e n t a t i v e c o n d i t i o n s ; t h e o n l y r e a l j u s t i f i c a t i o n of t h o s e t es t s i s
budget l i m i t a t i o n . W e a r e a l s o e x p e r i e n c i n g d i f f i c u l t i e s i n t h e d e p o s i t i o n
of t h i c k l a y e r s . M u l t i l a y e r d e p o s i t s a r e r e q u e s t e d above 30 micron .
L. W . Graham: S i n c e me mast have l o w heavy me ta i d e n s i t y r e l a t i v - t,
c o n v e n t i o n a l m e t a l c l a d p i n s , what i s t h e p h i l o s o p h y of u s i n g m e t a l
c o a t i n g s ? I n your c a l c u l a t i o n s a compress ive f o r c e i s assumed on m e t a l
c o a t e d p a r t i c l e s f rom t h e p r i m a r y c i r c u i t he l ium. Would n o t t h e m e t a l be
permeable t o he l ium, so e o u a l i z i n g t h e p r e s s u r e ? I n o t i c e d t h a t i n t h e
photomicrograph you have a s e a l i n g l a y e r of r e l a t i v e l y h i g h d e n s i t y PyC on
t o p of t h e b u f f e r , p resumably t o p r e v e n t r e a c t i o n w i t h t h e k e r n e l d u r i n g
d e p o s i t i o n of t h e o u t e r c o a t i n g . Would n o t t h e c o a t i n g be d i s i n t e g r a t e d
by a f a s t n e u t r o n damage?
H . F . B a i r i o t : I n a t y p i c a l p i n t y p e GBR, t h e f u e l d e n s i t y i n t h e 3 core i s 2.2t/m . I f p r e s s u r e d r o p c o n s i d e r a t i o n s a l lowed t h e u s e of a
core made of packed c o a t e d p a r t i c l e s , t h e f u e l d e n s i t y would be 2.5t/m . I n t h e r a n g e of power d e n s i t i e s ment ioned i n the pape r , in-and o u t l e t
c o o l a n t d u c t s need t o be f o r e s e e n , t o m a i n t a i n t h e p r e s s u r e d r o p s i n
a c c e p t a b l e l i m i t s , s o t h a t t h e advan tage i s lost. A he l ium l e a k t i g h t -
n e s s i s i n d e e d assumed i n t h e c o a t i n g d e s i g n s . . The PyC t r a n s i t i o n l a y e r
i s i n d e e d u n a c c e p t a b l e . The pu rpose of s e a l i n g t h e k e r n e l s a g a i n s t r e a c t i o n
w i t h t h e S i c d u r i n g d e p o s i t i o n w i l l be f u l f i l l - e d w i t h one of t h e o t h e r
b a r r i e r s mentioned i n t h e pape r . PyC i s u t i l i z i e d a t t h i s modest s t a g e of
o u r program f o r i t i s produced r o u t i n e l y i n o u r f a c i l i t i e s .
3
853
C. B. Z i t e k : H o w a r e th.e c o a t e d p a r t i c l e s h e l d o r c o n t a i n e d i n t h e
r e a c t o r core?
H. F. B a i r i o t : The p a r t i c l e s a r e inpe rmeab le a n n u l a r t u b e s and t h e
h e l i u m p a s s e s th rough t h e c o n t a i n e r from t h e o u t s i d e t o i n s i d e , a s was
d e s c r i b e d by t h e UKAEA i n t h e l i t e r a t u r e .
G . Meijer: I have a p r i n c i p a l q u e s t i o n on t h e u n s u i t a b i l i t y of
c o a t e d p a r t i c l e s f o r g a s cool f a s t r e a c t o r s . With c o a t e d p a r t i c l e s t h e
heavy m e t a l i s much more d i l u t e d t h a n i n t h e c a s e of p e l l e t s i n a t i n , i . e .
normal c l a d f u e l . The power d e n s i t y i s v e r y h i g h i n a f a s t r e a c t o r . I
n o t i c e d t h a t you t a k e a s a d e s i g n b a s i s f o r your p a r t i c l e development a
core w i t h 800 MW/m3.
t y p e f u e l , t h e f u e l e l e m e n t s w i l l burnup v e r y r a p i d l y w i t h t h e consequence
t h a t t h e r e a c t o r w i l l have t o be s h u t down u n d e s i r a b l y o f t e n f o r r e f u e l i n g .
Can you comment on t h i s ?
I am a f r a i d t h a t w i t h t h i s d i l u t e d c o a t e d p a r t i c l e
H. F. B a i r i o t : I n any r e a c t o r , t h e a d v a n t a g e s of a h i g h power d e n s i t y
have t o be b a l a n c e d a g a i n s t t h e i n c r e a s i n g p e n a l t y f rom down t i m e f o r re-
f u e l l i n g , a s you mentioned, t h e h i g h e r age f a c t o r s , t h e i n c r e a s i n g p r e s s u r e
d rop , e t c . The power d e n s i t y u t i l i z e d f o r t h i s f u e l d e s i g n and deve lop -
ment s t u d y i s by no means o p t i m i z e d f rom t h e r e a c t o r d e s i g n p o i n t o f view.
I n f a c t , when t h e h i g h e r power d e n s i t y c a p a c i t y i s n o t u t i l i z e d , t h e
v o i d a g e f o r c o o l a n t f l o w c a n be reduced and t h e heavy m e t a l d e n s i t y i n
t h e core i n c r e a s e d .
C. Rennie : The main r e a s o n f o r l o o k i n g i n t o c o a t e d p a r t i c l e s i s t h e
p o s s i b i l i t y of r e d u c i n g t h e f a b r i c a t i o n cost w i t h t h a t t y p e of f u e l .
ABSTRACT
The p a p e r g i v e s t h e r e s u l t s of t h e l a t e s t n u c l e a r and t h e r m a l c a l c u l a t i o n s pe r fo rmed f o r a GCFR w i t h vanadium a l l o y (V-3Ti-1Si) c l a d p i n s and o x i d e and c a r b i d e f u e l . The h e l i u m t e m p e r a t u r e a t r e a c t o r o u t l e t i s s l i g h t l y above 7 0 O 0 C , i n c a s e of o x i d e f u e l , which s h o u l d g i v e a r e a s o n a b - l e p l a n t e f f i c i e n c y w i t h a d i r e c t c y c l e g a s t u r b i n e a n d / o r r e d u c e d c a p i t a l costs . The core f i s s i l e i n v e n t o r y aiid t h e d o u b l i n g t i m e a r e 2800 and 1600 k g , arid 18 and 8 y e a r s f o r o x i d e and c a r b i d e f u e l r e s p e c t i v e l y . The p rob lems connec- t e d w i t h t h e c h o i c e of t h e c l a d d i n g m a t e r i a l ( c r e e p s t r e n g t h , h i g h t e m p e r a t u r e e m b r i t t l e m e n t , s w e l l i n g , c o m p a t i b i l i t y w i t h f u e l and c o o l a n t ) a r e s h o r t l y d i s c u s s e d .
I NTRODUCT I ON
T h e r e a s o n s t h a t make g a s c o o l i n g a t t r a c t i v e f o r f a s t b r e e d e r s have been d i s c u s s e d e l s e w h e r e . 1 * 2 , 3 * 4 p 5 The main a d v a n t a g e s r e l a t i v e t o sodium-cooled b r e e d e r s a r e t h e p r o b a b l e lower c a p i t a l c o s t , e s p e - c i a l l y w i t h d i r e c t c y c l e gas t u r b i n e s , t h e e x p e c t e d h i g h e r a v a i l a b i - l i t y , e a s i e r m a i n t e n a n c e and r e p a i r ( a l t h o u g h t h e s e t w o l a s t p o i n t s a r e d i f f i c u l t t o q u a n t i f y w i t h o u t a p r o t o t y p e ) and t h e b e t t e r b r e e d i n g . F u r t h e r m o r e , when r e a l l y h i g h c o o l a n t t e m p e r a t u r e a r e a v a i l a b l e t h e h e a t s i n k f o r t h e gas t u r b i n e s c o u l d b e a i r or a h e a t i n g s y s t e m . I n - d e e d a w a t e r r e a c t o r o f 1000 Mwe h a s a w a s t e o f h e a t of a b o u t 1900 Alwth, enough t o h e a t 400,000 homes i f a v a i l a b l e a t s a y 6 O o C , which is not p r a c t i c l e w i t h water r e a c t o r s or sodium r e a c t o r s w i t h s t e a m t u r - b i n e s .
+) Work pe r fo rmed w i t h i n t h e a s s o c i a t i o n i n t h e f i e l d of f a s t r e a c t o r s be tween t h e E u r o p e a n A t o m i c Ene rgy Community and G e s e l l s c h a f t f u r Kernf o r s c h u n g m b H , K a r l s r u h e
+ + ) D e l e g a t e d by Eura tom t o t h e K a r l s r u h e F a s t B r e e d e r P r o j e c t . +++> p r e s e n t l y a t t h e Dep t .o f Nucl.Engineering,Univ.of W a s h . , S e a t t l e , W a s h . ,
USA
854
855
The d i s a d v a n t a g e s kre t h e s l i g h t l y h i g h e r p l u t o n i u m i n v e n t o r y and t h e much h i g h e r coolant p r e s s u r e w i t h t h e consequen t s a f e t y problems ( loss of c o o l a n t a c c i d e n t , and inadequacy of h e l i u m n a t u r a l c o n v e c t i o n t o remove a f t e r h e a t from t h e core) . T h e s e s a f e t y problems c a n , however , be overcome by t h e u s e o f a c o n c r e t e p r e s s u r e v e s s e l and h i g h l y re l iab- l e and r e d u n d a n t c o o l a n t c i r c u l a t o r s . On t h e o t h e r hand , GcFR's d o n o t s u f f e r f rom s a f e t y problems of sodium-cooled f a s t reactors, s u c h a s b i g p o s i t i v e v o i d c o e f f i c i e n t s and f u e l - c o o l a n t r e a c t i o n s .
W e would l i k e h e r e t o stress a g a i n , a s s a i d b e f o r e , t h a t t h e r e a r e s t i l l many open q u e s t i o n s r e g a r d i n g t h e f u e l f o r a GCFR. The main e f f o r t s h o u l d t h e r e f o r e be directed t o f u e l deve lopment and i n - p i l e tests.
VANADIUM CLADDING
I n K a r l s r u h e w e s t r i v e a s h a s been s a i d , u l t i m a t e l y , t o have he- l i u m g a s o u t l e t t e m p e r a t u r e s f rom t h e core e q u a l or g r e a t e r t h a n 70O0C, w i t h a n e y e t o g a s t u r b i n e a p p l i c a t i o n or steam t u r b i n e a p p l i - c a t i o n w i t h r a t h e r s m a l l h e a t e x c h a n g e r s . S t e e l s a r e n o t s t r o n g enough for s u c h t e m p e r a t u r e s , a l t h o u g h t h e y c o u l d be u s e d f i r s t a t lower t e m - p e r a t u r e s w i t h a s t e a m t u r b i n e , e s p e c i a l l y i f a v e n t e d f u e l c o n c e p t i s a d o p t e d .
A series of a l l o y s b a s e d on vanadium, t i t a n i u m , n iob ium, and s i l i - c o n are b e i n g d e v e l o p e d by Bohm o f t h e M a t e r i a l s L a b o r a t o r y of t h e K a r l s r u h e C e n t e r i n c o l l a b o r a t i o n w i t h t h e M e t a l l g e s e l l s c h a f t .6,7 Of t h e s e w e choose t h e one c o n t a i n i n g 96% V , 3% T i , 1% S i b e c a u s e , a f t e r 20,OOO h o u r s a t 85OoC, i t h a s p r a c t i c a l l y t h e same stresse r u p - t u r e s t r e n g t h as n iob ium-con ta in ing a l l o y s and t h e h i g h l y n e u t r o n ab- s o r b i n g e l e m e n t s have been e l i m i n a t e d (10% niobium i n t h e c l a d d i n g
would p roduce a d e c r e a s e of t h e b r e e d i n g r a t i o of 0 . 1 : 3 ) 3
O u t - o f - p i l e c r e e p tes ts per formed a t t h e K a r l s r u h e M a t e r i a l s Labora - t o r y h a v e shown t h a t t h i s alloy c a n s t a n d t h e stresses g i v e n by t h e c o o l a n t gas o u t e r p r e s s u r e , t h e g a s e o u s f i s s i o n p r o d u c t s i n n e r p r e s s u r e , and t h e p r e s s u r e g i v e n by t h e s w e l l i n g o f t h e o x i d e f u e l f o r a p e r i o d of t w o y e a r s and t e m p e r a t u r e s u p t o 85OoC, p r o v i d e d t h a t t h e o u t - o f - p i l e mechan ica l p r o p e r t i e s of t h i s a l l o y a r e n o t c o n s i d e r a b l y worsened by t h e v e r y h i g h f a s t n e u t r o n d o s e s t o which t h e f u e l e l e m e n t s of a f a s t r e a c t o r a r e s u b j e c t e d . However, t h e r e a r e i n d i c a t i o n s 7 f 8 t h a t , l i k e o t h e r vanadium a l l o y s , t h i s one t e n d s t o m a i n t a i n d u c t i l i t y when i r r a d i a t e d a t h i g h t e m p e r a t u r e s i n a f a s t f l u x , or a t l e a s t i s much less a f f e c t e d t h a n s teels or n i c k e l - b a s i s a l l o y s . I r r a d i a t i o n e x p e r i - ments carried o u t by K a r l s r u h e on d i f f e r e n t V - a l l o y s i n d i c a t e d t h a t no high-temperature-embrittlement o c c u r s f o r f a s t d o s e s ( E 3 0 . 1 MeV) up t o 1.4 x IO2' and t e m p e r a t u r e s u p t o 750°C.7 T h e s e r e s u l t s have been con- f i r m e d by r e s u l t s o b t a i n e d by ANL f o r f a s t d o s e s up t o 3 x loz2 and t h e same t e m p e r a t u r e s . Recen t r e s u l t s a t t h e K a r l s r u h e c y c l o t r o n show t h a t a h e l i u m c o n c e n t r a t i o n of 1 x a toms /me ta l a tom, e q u i v a l e n t t o a f a s t dose of a b o u t 1 x ( E b O . 1 & l e v ) , does n o t p roduce any h i g h -
temper. .? t u r.e -
856
e m b r i t t l e m e n t i n t h e V-3Ti-1Si a l l o y u p t o 900"C, a l t h o u g h o t h e r vana- dium a l l o y s e m b r i t t l e i n t h e t e m p e r a t u r e icange 850-950OC. 8
The i n f o r m a t i o n on s w e l l i n g o f vanadium and vanadium-based a l l o y s u n d e r a h i g h f a s t f l u x is s p a r e . From t h e d a t a of W i f f e n and S t i e g l e r '
22 i t is p o s s i b l e t o deduce t h a t p u r e vanadium u n d e r a d o s e of 1 .7 x 10 (E50.1 M e V ) a t 600 C shows a volume irrcreilse of 0.1% Harkness'O d i d n o t f i n d any p o r e s i n V-20 T i a f t e r a d o s e of 2 x loi2 a t 5 5 0 O C . Both t h e s e r e s u l t s t e n d t o i n d i c a t e t h a t t h e s w e l l i n g r a t e is s m a l l e r t h a n t h a t of s t a i n l e s s s teel .
0
Vanadium a l l o y s e m b r i t t l e v e r y r a p i d l y i n t h e p r e s e n c e of oxygen and n i t r o g e n . W e h a v e t h e r e f o r e l o o k e d i n t o t h e c o m p a t i b i l i t y p rob lems . The main c o n s i d e r a t i o n s a r e g i v e n be low.
Assuming t h a t t h e f u e l e l e m e n t s remain i n t h e reactor f o r t w o y e a r s , t h a t h e l i u m l e a k a g e f rom t h e core is e q u a l t o 0.1% p e r day and t h a t e v e r y t w o y e a r s t h e r e a c t o r i s e m p t i e d of h e l i u m and f i l l e d a g a i n w i t h commer- c i a l l y a v a i l a b l e h e l i u m ( c o n t a i n i n g t h e i m p u r i t i e s O 2 = 10 vpm, €I20 = 10 vpm, N2 = 25 vpm), t h e n , d u r i n g t h e i r l i f e , t h e p i n s come i n c o n t a c t w i t h 1.7 r e a c t o r f i l l i n g s , t h a t is 26 vpm of O2 and 4 3 vpm of N2. Assuming t h a t all these i m p u r i t i e s r e a c t o n l y w i t h t h e c l a d d i n g , t h e w e i g h t p e r c e n t a g e of 0 and N i m p u r i t i e s i n t h e vanadium a l l o y a t t h e end of t h e pin l i f e w i l l be 200 ppm, wh ich i s w e l l below t h e l i m i t whe re t h e s e i m p u r i t i e s s t a r t t o a f f e c t t h e vanadium a l l o y m e c h a n i c a l properties (3000-5000 ppm). I t is c l e a r t h a t t h e amount of w a t e r coming f r o m l e a k a g e s of t h e h e a t e x c h a n g e r s c o u l d b e c o n s i d e r a b l y h l g h e r t h a n t h e amount men t ioned above . We recommend t x l e r e f o r e t h e u s e of t h i s c l a d - d i n g o n l y i n c o n n e c t i o n w i t h g a s t u r b i n e cycles, or w i t h s t e a m t u r b i n e c y c l e s , where t h e s t e a m p r e s s u r e i s lower t h a n t h e h e l i u m p r e s s u r e , f o r i n s t a n c e 130 and 1 2 0 atms r e s p e c t i v e l y .
The c o m p a t i b i l i t y of' vanadium and vanadium based a l l o y s c o n t a i n i n g s m a l l q u a n t i t i e s of t i t a n i u m , i s good, r e s p e c t i v e l y , w i t h UOg and UC f o r t e m p e r a t u r e u p l i t y o f u ran ium c a r b i d e w i t h vanadium is b t ? t t e r t h a n w i t h steels1',12. The e f f e c t o f f i s s i o n p r o d u c t s is s t i l l u n c l e a r b u t w e hope t o o b t a i n i n f o r m a t i o n f r o m o u r i r r a d i a t i o n s i n FR2. Hof mann14 h a s f o u n d r e c e n t l y w i t h o u t - o f - p i l e c o m p a t i b i l i t y e x p e r i m e n t s t h a t t h e worst f i s s i o n pro- d u c t s a r e i o d i n e , s e l e n i u m , t e l l u r i u m and c:esium. The r e s u l t s of t h e s e t es t s w i t h oxide f u e l and t h e s e f i s s i o n p r o d u c t s i n c o n c e n t r a t i o n s c o r r e s p o n d i n g t o burn-up o f 50 t o 10070 a r e g i v e n in T a b l e 1.
t o 1000°C and 9 0 0 O C ; it a p p e a r s t h a t t h e c o m p a t i b i -
T a b l e 1. E x t e n t of r e a c t i o n zones. U 0 2 + J + Se + Te + cs
A l l o y 600°C/ lo00 h 800°C/ 1000 h
V - Z r 2-Cr 15 10 p m 50 p m X 8 C r N i M o V N b1613( 4988) 100 /urn 150 p m AIS1 321 SS 300 pm I n c o n e l 625 2mm
I n c o l o y 800 400 p m 2mm
a57
A l l t h e h e r e s i m u l a t e d f i s s i o n p r o d u c t s react p r e f e r a b l y w i t h chromium, w e t h i n k t h e r e f o r e t h a t t h e V-3Ti-1Si a l l o y s h o u l d be e v e n b e t t e r t h a n t h e best i n v e s t i g a t e d a l l o y (V-Zr2-Cr-15).
PERFORMANCE
T a b l e 2 shows t h e r e s u l t s of t h e t h e r m a l and n u c l e a r c a l c u l a t i o n s w i t h V-3Ti-1Si c l a d f u l p i n s .
t i o n set of K a r l s r u h e , t h e so c a l l e d MOXTOT set . Compared w i t h t h e p r e - v i o u s sets, t h i s one i s improved as f o l l o w s :
a . t h e l a t e s t e v a l u a t e d v a l u e s f o r a ( P u ) a r e i n c o r p o r a t e d ( v a l u e s of G w i n)
b . t h e c a p t u r e cross sec t ion o f U238 have been lowered (MOXON d a t a ) c . t h e cross s e c t i o n s of t h e h i g h e r Pu i s o t o p e s have been improved .
The d e t a i l s of t h i s set have been p r e s e n t e d a t t h e BNES c o n f e r e n c e i n June 1969 i n London by E . K i e f h a b e r e t a l .
F u r t h e r m o r e , t h e Pu e u i l i b r i u m c o m p o s i t i o n h a s been m o d i f i e d . I n t h e p r e v i o u s c a l c u l a t i o n s ' t h i s was assumed t o be a m i x t u r e be tween p l u t o n i u m coming from LWR's and GCFR's, w h i l e i n t h e p r e s e n t c a l c u l a t i o n t h e Pu i s o t o p i c c o m p o s i t i o n is t h e e q u i l i b r i u m c o m p o s i t i o n f rom GCFR's o n l y . T h i s d e c r e a s e t h e b r e e d i n g r a t i o f o r o x i d e f u e l by 0 . 0 4 4 , w h i l e t h e new set of cross s e c t i o n s p roduce a d e c r e a s e o f 0.143. An a d d i t i o n a l 0.015 is d u e t o t h e e l i m i n a t i o n o f t h e 0 .4% U235 i n t h e b l a n k e t s , assumed i n t h e p r e v i o u s c a l c u l a t i o n s . Thus t h e r e l a t i v e l y l o w b r e e d i n g r a t i o of 1 . 3 1 5 f o r a GCFR d o e s n o t come f rom t h e V-3Ti- lSi c l a d d i n g , which h a s a s l o w a n e u t r o n a b s o r b t i o n a s s teel , b u t f rom t h e u s e of t h i s new set o f d a t a and f rom t h e new Pu c o m p o s i t i o n .
The n u c l e a r c a l c u l a t i o n s were pe r fo rmed w i t h t h e l a t e s t cross sec-
1 4
F o r t h e o x i d e t h e h e l i u m t e m p e r a t u r e a t core o u t l e t is 72OoC, w h i l e t h e maximum h o t s p o t t e m p e r a t u r e a t c l a d midwal l is t 85OoC. F o r t h e c a r - b i d e t h i s t e m p e r a t u r e s h o u l d be a b o u t t h e same, b u t i t is n o t s u r e t h a t t h e c l a d d i n g c a n w i t h s t a n d t h e h i g h e r s w e l l i n g p r e s s u r e of t h e c a r b i d e and t h e c o n s i d e r a b l e t h e r m a l stresses across t h e c l a d w a l l . However, i f t h e vanadium a l l o y m a i n t a i n s i ts o u t - o f - p i l e d u c t i l i t y a f t e r i r r a d i a t i o n t h e s e stresses a r e r e l a t i v e l y l o w . I n t h e o x i d e c a s e t h e p r e s s u r e d r o p i n r e a c t o r h a s been c a l c u l a t e d w i t h a c o n s t a n t a r t i f i c i a l r o u g h n e s s on t h e p i n w a l l s , w h i l e i n t h e c a r b i d e c a s e t h r e e d i f f e r e n t r o u g h n e s s e s have been assumed. F o r c o n t i n o u s l y v a r i a b l e r o u g h n e s s , t h e p r e s s u r e d r o p i n t h e r e a c t o r would be 3.5 and 8.7 kg/cm , r e s p e c t i v e l y . The r o u g h n e s s d a t a a r e f rom W i l k i e l ' and D a l l e Donne and Meerwa1d.l'
The o u t - o f - p i l e i n v e n t o r i e s and t h e s y s t e m d o u b l i n g t i m e have been c a l c u l a t e d w i t h t h e a s s u m p t i o n s used i n t h e LNEA s t u d y 4 , i . e . , w i t h an o u t - o f - p i l e t i m e f o r r e p r o c e s s i n g and r e f a b r i c a t i o n of 0 . 7 5 y e a r s . The r e s u l t i n g o u t - o f - p i l e i n v e n t o r i e s a r e v e r y l a r g e , e s p e c i a l l y i n t h e c a r - b i d e c a s e , and show t h a t t h e r e is a b ig i n c e n t i v e f o r t r y i n g t o r e d u c e t h i s o u t - o f - p i l e t i m e a n d / o r i n c r e a s e t h e mean f u e l d i s c h a r g e burnup.
2
858
T a b l e 2 . Main P a r a m e t e r s of l(Xy) Mwe CXFR
Vanadium C l a d (96% V I 3% T i , 1% S i )
O x i d e C a r b i d e
C o r e volume ( l i t e r s ) 8 4 i O
F u e l volume f r a c t i o n 0 . 2 9 8
C o o l a n t volume f r a c t i o n 0 . 5 5 2
S t r u c t u r e m a t . ( 1 6 i l 3 S 3 ) volume f r a c t i o n 0 . 0 7 3
C l a d d i n g volume f r a c t i o n 0 . 0 7 7
F u e l p i n d i a m e t e r (cm) 0 . 7 4
C l a d t h i c k n e s s (mm) 0 . 4
4181
0 . 2 8 4 5
0 . 5 6 9 7
0 . 0 7 0
0 . 0 7 5 8
0.835
0 . 4 5
R e a c t o r i n l e t c o o l a n t t e m p e r a t u r e (OC) 410 3 9 0
R e a c t o r o u t l e t c o o l a n t r e m p e r a t u r e ( O C ) 7 20 :w
ilax.nom. s u r f a c e t e m p e r a t u r e ( W ) 7 5 6 767
Man . fue1 p i n l i n e a r power (W/cm) 4 4 0 1 2 7 1 . 7
C o o l a n t p r e s s u r e a t r e a c t o r i n l e t (kg /cm2) 1 0 0 120
P r e s s u r e d r o p i n r e a c t o r (kg /cm2) 4 . 8 1 0 . 2
T o t a l t h e r m a l o u t p u t ( i n c l . h e a t p roduced in b l a n k e t s ) (hhvth) 2449 2778
P l a i i t n e t e f l i c i e n c y w i t h g a s t u r b i n e C y c l e 4 0 . B'b 36%
C o r e power d e n s i t y ( k w l l i t e r ) 267 581
Pu i s o t o p i c c o m p o s i t i o n 0 .83O6 ,0143! , 0 . 0 2 1 1 ,O.O052
Maximum t o t a l n e u t r o n f l u x (n / cm2 s e c ) 0.78 x 1016 1 . 3 2 x 10l6
(EaO.1 M e V ) ( n l cm ' sec ) 0 . 4 6 x 10l6 1.06 x 10IG
( n / c m 2 ) 1 . 9 x 1 0 2 3 2 . 5 x loz3
hlnxinium f a s t n e u t r o n f l u x
Maximum f a s t d o s e ( E 7 0 . 1 hlev)
A v e r a g e core e n r i c h m e n t 1 3 . 7 5 13.2%
T o t a l f i s s i l e mass i n c o r e
A v e r a g e r a t i n g (MwthLkg ~u 239 + kg
( k g of Pu 239 + Pu 241) 2818 1586
Pu 241)) 0 . 869 1 . 7 5 2
Mean d i s c h a r g e b u r n u p (hlwd/t) 55 ,Ooo 55.000
F u e l s m e a r d e n s i t y ( S of t h e o r e t i c a l ) 8 3 % 80%
I n t e r n a l c o n v e r s i o n r a t i o =
0 . 7 6 6 n e u t r o n s c a p t u r e d in c o r e f e r t . m a t . n e u t r o n s a b s o r b e d i n c o r e f iss . m a t .
T o t a l b r e e d i n g =
0 . 7 7 6
1 . 4 7 6 n e u t r o n s c a p t u r e d in r e a c . i e r t . m a t . n e u t r o n s a b s o r b e d in r e a c . i i s s . m a t . 1'315
U r e e d i n g g a i n =
0.330 0 . 4 6 9 e x c e s s Pu a t o m s p r o d u c e d t o t a l a toms f i s s i o n e d
0 . 5 7 2 x lo-' dk dT D o p p l e r c o n s t a n t - T - (T i n OK)
T o t a l r e a c t i v i t y i n c o o l a n t ($1 0.6Y 0 . 7 6
O u t - o f - p i l e f i s s i l e i n v e n t o r y (kg ) ' 1 4 1 5 1507
0 . 7 3 1 x lo-'
S y s t e m l i n e a r d o u b l i n g t i m e ( y e a r s ) + 1 7 . 7 7 . 9
+ C a l c u l a t e d w i t h : p l a n t l o a d f a c t o r = 0.8; o u t - o f - p i l e t i m e f o r r e p r o c e s s i n g and r e f a b r i c a t i o n = 0 . 7 5 y e a r s ; r e p r o c e s s i n g Pu losses = 27..
T h e n e t p l a n t e f f i c i e n c y h a v e b e e n c a l c u l a t e d a c c o r d i n g t o t h e g a s t u r b i n e c y c l e s u g g e s t e d by Bammert." O t h e r au tho i - s16 s u g g e s t t h a t t h e opt imum e f f i c i e n c i e s wou ld b e lower, w i t h c o n s e q u e n t r e d u c t i o n i n com- p o n e n t s i z e a n d c a p i t a l costs.
T a b l e 3 shows t h e a s s u m p t i o n s made t o o b t a i n 1;he e f f i c i e n c y i n d i - c a t e d i n T a b l e 1. T h e T a b l e shows a l s o a s o l u t i o n w i t h r e d u c e d c a p i t a l costs and lower p l a n t e f f i c i e n c y ( 3 3 . 5 % ) . A t t h i s s t a g e w e a r e n o t a b l e t o s a y wh ich is t h e b e t t e r o f t h e s e s o l u t i o n s , b e c a u s e w e h a v e no d a t a on t h e c a p i t a l costs.
859
T a b l e 3. Gas t u r b i n e c y c l e d a t a
High c a p i t a l Low c a p i t a l c o s t c o s t s o l u t i o n s o l u t i o n
R e a c t o r i n l e t he l ium t e m p e r a t u r e (OC)
R e a c t o r o u t l e t he l ium t e m p e r a t u r e COC)
P r e s s u r e d r o p i n r e a c t o r
P r e s s u r e d r o p i n rest of t h e c i r c u i t
T u r b i n e i n t e r n a l e f f i c i e n c y
T u r b i n e e x p a n s i o n r a t i o
R e c u p e r a t o r temp.d i f f e r e n c e (OC)
Number of c o o l e r s and compressors
I n t e r n a l e f f i c i e n c y of compressors (LP , MP ,HP)
i n l e t (OC) Helium t e m p e r a t u r e a t compressor
P l a n t n e t e f f i c i e n c y
P l a n t n e t o u t p u t (Mwe)
410.5
720
4.8%
5.5%
90%
2.585
27
3
20
40.8%
lo00
3 4 3 . 9
706
4.5%
h 5%
9 1%
3
45
2
88%, 87%
30
33.5%
962
The he l ium t e m p e r a t u r e a t r e a c t o r o u t l e t i n t h e l o w c a p i t a l c o s t s o l u t i o n is o n l y 706OC because a r e c e n t c l a d d i n g s t a t i s t i c a l h o t s p o t a n a l y s i s based on a method developed by Amendola" h a s shown t h a t t h e mixed mean he l ium t e m p e r a t u r e a t r e a c t o r o u t l e t is 706"C. and n o t 720OC. mainly due t o t h e s t rongpower r a d i a l g r a d i e n t in t h e o u t e r m o s t f u e l s u b a s s e m b l i e s and i n t h e r a d i a l b l a n k e t . The c a l c u l a t i o n t a k e s in- t o account of t h e c o o l a n t mixing a s w e l l , which is based on e x p e r i m e n t s of Baumann and M o l l e r m .
I n t h e c a s e of t h e l o w c a p i t a l c o s t s o l u t i o n t h e amount of h e a t a v a i l a b l e f o r h e a t i n g ( w a t e r a t 60°C) would be 1450 Mwth. i . e . 1245 Gcal /h .
REFERENCES
1. M . D a l l e Donne, E . Eisemann, and K. W i r t z , Some C o n s i d e r a t i o n s on Gas Cool ing f o r F a s t B r e e d e r s , KFK 595 (1967) ; c . f . a l s o K. W i r t z , Gascool ing f o r F a s t B r e e d e r s , T h i r d FOMTOM Congress , London, 1967 p r i n t e d i n " l ) iscussion" t o t h e Conference , B r i t i s h Nuclear Forum (1967) 26.
2. M . D a l l e Donne, and K . W i r t z , Gas Cool ing f o r F a s t Breeders , T r a n s . A m . Nucl . SOC. 10 2 (1967) 649; and KFK 689 (1967) . -
3 . M . D a l l e Donne, E . Eisemann, F . Thummler, and K . Wirtz , High Tempe- r a t u r e Gas Cool ing f o r F a s t B r e e d e r s , S M 111/12, Proc . of t h e IAEA Conf. on Advanced High Temperature G a s c o o l e d R e a c t o r s , J u l i c h , Oktober 1968 and KFK 841.
4 . ENEA Working Team on F a s t R e a c t o r E v a l u a t i o n , A n Assessment Study of Gas-Cooled F a s t R e a c t o r s f o r C i v i l Power G e n e r a t i o n , W i n f r i t h , J u l y 1968.
5. Gulf General A t o m i c i3urope, Reference Design of a 1000 Mwe Gas c o o l e d F a s t R e a c t o r P l a n t , GAE 37 ( 1 9 6 8 ) ; see a l s o GA 6132; GA 6667; NUCLEX 1966, GAE paper 4/13.
6 . 11. BBhm, and h l . S c h i r r a , Z e i t s t a n d und K r i e c h v e r h a l t e n von Vanadin T i t a n und Vanadin-Ti tan-Niob-Legierungen , KFK 774 (1968) .
860
7 . H . Bohm, W . i l i e n s t , H . Hauck, and H . J . L a u e , I r r a d i a t i o n E f f e c t s on t h e Mechan ica l P r o p e r t i e s of V - a l l o y s , ASTM S p e c . Techn. P u b l . 426 (1967).
-
8. K . E h r l i c h , and H . Bohm, I r r a d i a t i o n E f f e c t s i n Vanadium Based A l l o y s , S M 120/G-4, P r o c . of t h e IAEA Conf . on R a d i a t i o n Damage in R e a c t o r M a t e r i a l s , June 1969.
9 . F . W . W i f f e n , and J . 0. S t i e g l e r , I r r a d i a t i o n Damage i n Vanadium at 6 0 0 ° C , A N S T r a n s . 1 2 , 1 , June 1969, -
10. S . D . H a r k n e s s , Vo ids i n EBR I1 C o n t r o l Rod Shroud and I r r a d i a t e d Vanadium A l l o v s . ANL 7457. Mav 1968.
11. 0. Goetzmann, and F . Thiimmler, Wechse lwirkungen von mog l i chen hltill- w e r k s t o f f e n d e s s c h n e l l e n B r i i t e r s m i t UN and U 0 2 , KFK 1081 ( 1 9 6 9 1 7
1 2 . 0. Goetzmann, and W . H e i n , V e r g l e i c h von Lang- und K u r z z e i t v e r t r a g - l i c h k e i t s u n t e r s u c h u n g e n an UN und UO,, KFK 1086 ( 1 9 7 0 ) .
13. P. IIofmanii, p a p e r t o be p r e s e n t e d a t the R e a k t o r t a g u n g 1 9 7 0 , 20-22 A p r i l 197u , D e u t s c h e s Atomforum e . V . , 13er l in
1 4 . E . K i e f h a b e r , H . K u s t e r s , J . J . S c h m i d t , H . Bachmann, B. Krieg, JL. S t e i n , D . Thiem, K . Wagner, B. Hinkelmann, and I . S i e p , E v a l u a t i o n of F a s t C r i t i c a l E x p e r i m e n t s by Use of Recen t Methods and D a t a , P r o c . of t h e BNES Conf . on The P h y s i c s of F a s t R e a c t o r O p e r a t i o n and D e s i g n , London, J u n e 196'3.
15. I). W i l k i e , F o r c e d C o n v e c t i o n Heat T r a n s f e r from S u r f a c e s Roughened by T r a n s v e r s e R i b s , AICHE Proc. 3 I n t . Heat T r a n s f e r C o n f . , V o l . I , 1966.
16. M. D a l l e Donne, and E . Meerwald, Heat T r a n s f e r f r o m S u r f a c e s Roughened by Thread-Type R i b s a t Ifigh T e m p e r a t u r e ( t o be p u b l i s h e d ) .
17. K . Bammert, and W . T w a r d z i a k , K e r n k r a f t w e r k e m i t H e l i u m t u r b i n e n f u r grol3e L e i s t u n g e n , A tomkernene rg ie , 1 2 , 9/ 10, 1967. -
18. L. A . L y s , R . B rog l i , and W . H e l b l i n g , P a r a m e t e r i c S t u d i e s of Gas cooled F a s t R e a c t o r s w i t h C l o s e d c y c l e Gas T u r b i n e s , A t o m k e r n e n e r g i e , 1 4 . 2 . 1969.
19. A . Amendola, Advanced S t a t i s t i c a l H o t S p o t A n a l y s i s , KFK 1134 (1970)
20. W . Saumann, and R . Moller, E x p e r i m e n t e l l e Un te r suchung d e r hi ihl- m i t t e l q u e r v e r m i s c h u n g i n V i e l s t a b b i i n d e l n , K F K 807 (1969). -
861
DISCUSSION
R. A. U. Huddle: When you d i d t h e c a l c u l a t i o n s concerning the
embr i t t l ement of vanadium and i t s a l l o y s by oxygen and n i t r o g e n d i d you
assume t h a t t h e i m p u r i t i e s r e a c t e d homogeniously w i t h a l l the vanadium i n
the core , or d i d you t ake i n t o c o n s i d e r a t i o n t h e temperature e f fec t on t h e
r e a c t i v i t y - - p a r t i c u l a r l y the effect of peak random channel temperature and
h o t s p o t s .
M. Da l l e Donne: W e d i d t r y t o t ake i n t o account t he temperature d i f f e r e n c e s i n c a l c u l a t i n g t h e d i s t r i b u t i o n of oxygen and n i t r o g e n i n the
vanadium a l l o y c ladding . The c a l c u l a t i o n i s ve ry d i f f i c u l t because i t
depends on the dynamics of t h e va r ious r e a c t o r s involved, on the h e l i u m
v e l o c i t y , and on t h e d i s t r i b u t i o n and d i f f u s i o n of t h e i m p u r i t i e s i n
helium. W e f ee l , however, t h a t t he d i s t r i b u t i o n of t h e i m p u r i t i e s i n
t h e c l add ing should be f a i r l y even, because even a t t h e minimum c l a d
temperature (about 45OOC.) t h e i m p u r i t i e s r e a c t wi th t h e c ladding
extremely quick ly . Furthermore, the va lue c a l c u l a t e d w i t h t h e assumption
of uniform d i s t r i b u t i o n (200 PPM) i s much below the dangerous l e v e l
(3000-5000 ppm).
D. D. Tytga t : What i s t h e accep tab le water i n l eakage r a t e from
the exchangers for the 96 percent V , 3 percent T i , 1 percent S i a l l o y
corrosion rate?
M. D a l l e Donne: W e d i d c a l c u l a t e t h i s in leakage r a t e . Th i s r a t e ,
however, should be very , v e r y low and w e t h i n k t h a t i t i s ve ry d i f f i c u l t
and/or ve ry expensive t o make exchanges capable of guarantee ing such
ex t remely low water in leakage r a t e s .
P. U. F i sche r : Concerning the c a p i t a l c o s t in format ion presented
by Lsy, I would l i k e t o po in t ou t t h a t h i s work i s based on d e t a i l e d
des ign work and has had t h e b e n e f i t of a l o t of i n d u s t r i a l i npu t i nc lud ing
component c o s t s .
K. Wirtz: I r e f e r t o my c o n t r i b u t i o n t o y e s t e r d a y ' s panel . This
paper p o i n t s t o t h e second gene ra t ion of GCFBR. I t shows t h a t w i t h metal
c l a d p i n s t he use of t he helium t u r b i n e becomes f e a s a b l e . The use of
c a r b i d e f u e l would remove a drawback of GCFBR; namely, t h e h igh f i s s i le
inventory . The work mainly i s t o demonstrate t h e p r a c t i c a l i t y of
862
of advanced c ladding meta ls and t o j u s t i f y t h e i r development. Presumably
t h e immediate p r a c t i c a l goa l wi th r e s p e c t t o t h e GCFVR i tself should be
con t inua t ions of pro to type development for a p p l i c a t i o n t o t h e f i r s t genera-
t i o n r e a c t o r s of t h e GGA Type.
L. A . Lys: S ince I wias r e f e r r e d t o i n t h e paper, I would l i k e t o
comment on t h e d i f f e r e n c e between t h e c y c l e des igns which a r e normally
proposed i n t h e l i t e r a t u r e and t h e des igns proposed by t h e Swiss Federa l
z n s t i t u t e f o r Reactor Research. To exp la in t h i s I would l i k e t o r e f e r t o
t h e f i g u r e below. The f i g u r e i s based on a ho t spo t temperature of 800OC.
which i s 5 O O C . lower than t h e temperature used i n t h e paper. One can see
t h a t even wi th tlris lower temperature an e f f i c i e n c y of 40-41 percent can
be obta ined . However, compared wi th t h e optimum design a t 30-31 percent
e f f i c i e n c y an i n c r e a s e of power gene ra t ion c o s t of t h e o r d e r of 0.35-0.50
m i l l s pe r kwh r e s u l t s . This i n c r e a s e i s p r i m a r i l y t h e consequence of
h ighe r c a p i t a l c o s t s r e l a t e d t o t h e inc reased s ize of t h e hea t exchanger
equipment which i s necessary t o o b t a i n t h e h ighe r e f f i c i e n c y .
Plant Eff iciency:percent
863
M. Da l l e Donne: As I s a i d t h e paper, w e cannot say from our da t a
which of t h e two gas t u r b i n e c y c l e s i s p r e f e r a b l e , because w e have no
information on the c a p i t a l c o s t s . I would agree w i t h M r . Lys t h a t due t o
t h e ve ry smal l f u e l c y c l e c o s t s t y p i c a l of a f a s t b reeder , e s p e c i a l l y i n
t he c a s e of smal l plutonium i n v e n t o r i e s , the economic optimum i s the
d i r e c t i o n of low c a p i t a l c o s t s . What i s impor tan t , a s f a r a s w e a r e con-
cerned, i s the f a c t t h a t even w i t h t h e reduced p l a n t e f f i c i e n c y (33/5%)
given by t h e gas t u r b i n e c y c l e proposed by M r . Lys, w e a r e a b l e t o g e t
from the same c o r e almost the same n e t e l e c t r i c a l ou tpu t . T h i s i s due t o
t he f a c t i n t h e lower e f f i c i e n c y c y c l e the d i f f e r e n c e between t h e helium
temperature a t co re o u t l e t and a t c o r e i n l e t i s cons ide rab ly h igher , which
Metals and Ceramics Division G Oak Ridge National Laboratory Oak Ridge, Tennessee 37830
ABSTRACT
A cooperative design study and iriradiation t e s t program i s being car r ied out by ORNL and GGA t o provide a metal-clad ceramic f u e l p in for the GCBR. The design study indicated t h a t i f t he problems associated with the high overpressure on the f u e l pins from t h e 85-atm helium coolant can be over- come, much of t he f u e l and cladding technology developed on the LMFBR program would be applicable 1;o GCBR f u e l pin design. Both sealed and manifold-vented f u e l piin concepts were con- sidered. The manifolded design has been chosen as the reference GCBR design due t o i t s projected performance and economic poten t ia l .
culminated with a successful t e s t of fuel-cladding-interacting- type pins . Hastelloy X o r type 316 s t a in l e s s stee:L and operated with 700°C cladding temperatures t o 60,000 Ibd/tonne burnup. serious fuel-cladding mechanical o r chemical in te rac t ions were observed i n these p ins . describing mechanical s t a b i l i t y and fuel-cladding chemical in te rac t ions as a function of cladding temperature and cool- ant overpressure a r e a l so presented.
progress and performing sa t i s fac tor i ly . , Fuel pins of t h i s
The thermal flux i r r ad ia t ion t e s t i n g of sealed f u e l pins
The (U,12% Pu)O;! f u e l pins were .clad with e i the r
No
Data developed i n e a r l i e r t e s t s
A thermal f lux t e s t of the manifolded p in design i s i n
type a re being fabricated fo r fast flu: t e s t i n g t o begin i n FY 197 1.
*Work done under sponsorship of U.S. A1;omic Energy Commission by
?Gulf General Atomic . OWL and by GGA under Contract AT(O4-3)-167, Project Agreement 23.
8 64
865
INTRODUCTION
A design study and i r r ad ia t ion t e s t program i s being conducted
cooperatively by G u l f General Atomic (GGA) and Oak Ridge National Laboratory (ORNL) t o develop f u e l elements f o r the Gas-Cooled Fast
Breeder Reactor (GCBR).
a t GGA and the i r r ad ia t ion t e s t ing has been implemented a t ORNL.
t he course of t h e design study, it became apparent that t he only basic difference i n t h e service condition between a gas-cooled and a l iquid- metal-cooled breeder reactor i s t h e r e l a t i v e l y high pressure of t h e helium coolant i n the gas-cooled system. t h e gas-cooled concept t o a t t a i n higher cladding temperatures; but they a r e not essent ia1, l as t h e reference design i s based on a 700°C peak cladding temperature, including a31 hot spot fac tors . as the peak cladding temperatures given f o r LMFBR power reactors .
The design work has been performed pr imari ly
In
There i s some incentive i n
This i s t h e same
FUEL PIN CONCEPTS
Several f u e l p in concepts t h a t might withstand the approximately
85-atm pressure of t he helium coolant have been evaluated. i n t e re s t ing of these a re l i s t e d i n Table 1 along w i t h t h e major l imita- t ions and advantages of each. The free-standing and t h e fuel-cladding-
in te rac t ing (FCI) concept a r e both based upon a sealed f u e l pin. a r e very similar, w i t h the only s igni f icant difference being tha t f o r t h e FCI design the cladding w a l l thickness i s minimized t o the point t h a t slow, uniform creep collapse of t he cladding can occur under t h e
i n i t i a l operating conditions. re lease of f i s s i o n gases from the f u e l and minimal support from t h e
f u e l a r e r e l i e d upon t o prevent complete col lapse of t he cladding.
high thermal s t r e s ses which are developed i n t h e heavy cladding on the
free-standing p in and t h e breeding gain pena l t ies associated with
neutron losses t o t h e cladding provide t h e incentive t o go from the free-standing t o the FCI concept.
collapse of t he cladding must be prevented, and a carefu l design e f f o r t i s required.
The most
They
An in t e rna l pressure buildup by t h e
The
In t h e FCI concept, premature creep
Table 1. Major Charac te r i s t ics , Limitations, and Advantages of Gas-Cooled Fast Breeder Reactor Fuel Rod Concepts
~ ~~
Concept Charac te r i s t ics Problems or Limitations Advantages - Free -standing Thick cladding o r prepressurized Breeding penal t ies associated Relat ively simple
de s ign with strong t h i c k cladding cans Sealed can
Pressure d i f f e r e n t i a l decreasing High thermal s t r e s s e s i n
Prepressurization may be with b urnup thick-wall cladding
required
P) Fuel-cladding- Long-term creep col lapse of Creep collapse of cladding i n Economically
i n t e r a c t i n g (FCI) cladding e a r l y l i f e i s undesirable a t t r a c t i v e sealed 0-3 Q,
pin Sealed can Pressure d i f f e r e n t i a l decreasing
Subject t o cycling fa t igue Prepressurization may be mn,ri w i t h burnup b =-I bU
Manifolded -vented Pre s sure equalizing Achieving to le rab le leak r a t e LMFBR s i m i l a r i t y a t coupling
system i n fuel element
Vented e x t e r n a l t o core Manifolded t o common connector Re l i a b i l i t y of manifolding p o t e n t i a l
Higher performance
Potent ia l ly addi t i ona 1 plant systems costs
867
The manifolded or vented-to-plenum concept reduces or eliminates t h e overpressure on t h e cladding by balancing t h e pressures i n t e r n a l
and ex te rna l t o the f u e l cladding through a manifolding system.
provides a f u e l p i n very similar t o an LMFBR p i n and permits t h e use
of much of t h e f u e l and cladding da ta developed on t h a t program. I n addi t ion , t h i s design approach eliminates t h e danger of a sudden, l a r g e
r e l ease of f i s s i o n gases i n t o t h e primary coolant system during operation.
The economic p o t e n t i a l f o r t he manifolded concept includes both
This
l o w f u e l cyc le cos t and a poss ib l e ne t decrease i n t h e c a p i t a l cos t of
t h e GCBR p l a n t . These lower cos t estimates a r e based upon t h e p o t e n t i a l
f o r minimizing t h e cladding thickness, reducing t h e f u e l p i n and o v e r a l l
core length by reducing t h e f i s s i o n gas plenum, and optimizing t h e operating pressures and temperatures. The cos t of manifolding, f i s s i o n
product vent connections, and f i s s i o n product monitoring s t a t i o n s must
be added; but t hese a r e more than compensated f o r by t h e cost decreases. Evaluation of t h e problems associated with these various designs
and an ana lys i s of t h e e f f o r t required t o overcome these problems have r e s u l t e d i n t h e se l ec t ion of t h e manifolded-vented f u e l p i n concept f o r t h e reference design f o r t h e GCBR. The FCI concept has been adopted as t h e backup design.
IRRADIATION TESTJYG
The in- reac tor evaluation of t hese concepts has been ca r r i ed out over t h e l as t four years i n t h e Oak Ridge Research Reactor (ORR) pool-
s ide f a c i l i t y . * J 3 The ea r ly t e s t s employed U02 f u e l , whereas t h e l as t
seven p ins have contained (U, 12% Pu)02. The t e s t p re sen t ly in- reac tor
contains t h e f i r s t f u e l p i n of t h e manifolded type. All of these t e s t s
a r e conducted i n NaK-filled i r r a d i a t i o n capsules ( see Fig. 1) t h a t provided an ex te rna l pressure of 1000 p s i a on t h e t e s t p ins and thermo-
couple monitoring of -c ladding temperatures. The next t e s t s i n t h i s program w i l l involve seven f u e l p ins p re sen t ly being fabr ica ted f o r
fast-flux t e s t i n g i n t h e EBR-11.
868
ORNL-DWG 68-11396R
rARGON FLUX MONITOR 7 HASTELLOY X
lNaK LEVEL
I 'GA-4:5 U02 IN HASTELLOY X \GA-46 (U-Pu)O*
(0.354-in.OD) IN HASTELLOY X (0.354-in. OD)
Zr-2 THERMAL DA IH
LINNER CAPSULE STAINLESS STEEL
(f5/8-in. OD)
I- 22.5 in,- d Capsule 03 - P7.
Fig. 1. Typical GCBR ORR I r rad ia t ion Test Design.
Sealed Pin Tests
The designs employing sealed f u e l pins, both free-standing and FCI types, have been evaluated i n 8 capsules incorporating 16 separate
f u e l rods. Early r e s u l t s from these were reported previously.4 All
of these t e s t s a r e l i s t e d i n Table 2 along with t h e most important
fabr ica t ion and t e s t information.
60,000 Mwd/tonne.
temperatures from 560 t o 840°C.
Burnups have ranged from 3,400 t o
Heat ra t ings ranged from. 7 t o 22 kw/ft and cladding
The p r inc ipa l var iables i n these t e s t s were the r e l a t i v e cladding w a l l s t rength as affected by the w a l l thickness, wal l temperature, and
cladding material , and the pressure d i f f e r e n t i a l across the cladding
w a l l . This pressure d i f f e r e n t i a l was varied by changing the i n i t i a l i n t e r n a l pressure (prepressurizat ion) and t h e i n t e r n a l volume provided
f o r the accumulation of released f i s s ion gases.
i n t e r e s t from these t e s t s concern the dimensional s t a b i l i t y of t he f u e l
p in and the fuel-cladding chemical in te rac t ions .
The major r e su l t s of
Dimensional S t a b i l i t y
The t e s t conditions have been varied t o cover the f u l l range of
cladding s t a b i l i t y from instantaneous collapse of the cladding onto
the f u e l through a f u l l y free-standing cladding. No mechanical
I
Table 2. Summary of Gas-Cooled Fas t Breeder Reactor I r r a d i a t i o n Tests
Specimens collapsed; negllgibla ha1 support of cladding
Good condition; collapse in region of th in cladding; negligible Puel support of cladding
Slight creep deformation
Good collapse s t ab i l i t y
Some cladding deformation under t h e m - couple used t o mni tor temperature
Good collapse s t ab l l i t y
Good collapse s t ab i l i t y
Collapsed into 0-1 shaps; r i e g ~ i b l s
Cladding failed under theruncoupla band; negligible fuel support of cladding. localized couapse and failure
16,000 Mwd/tonnc
GA-16 which experienced wry localized collapse and failed.
fuel support of cladding
Irradiation discontinued a t
FissiOn-pKduct le& detected in pin
Fuel pin specimens all in excellent condition; no significant Qfo ra t ion observed
Fissionqroduct emission a t top of iucl pin and top of fission-prcduct t rap will be mnitored; i n s tnmnted pin and trap; pin external pressure - 950 psi , in te rna l - 1000 psi under n o m 1 operating conditions
a A l l fuel c o l m s appmxjaately 3 in. long.
bSmar density was leas than or equal to 85s of theoretical.
dSpecial purpose sodium bonded design, dropped from program. ePrepressurlzed rod.
fTemperature swing on this rod from 560 t o 660°C during each reactor cycle.
Gas-bonded sealed-can design, except for rod GA-20, which is manifolded with a fuel colunn 9.3 in. long.
CRLkt, EM-.
870
ra tche t t ing of f u e l p e l l e t s with the cladding has been observed. dimensional s t a b i l i t y of t he f u e l pins varied with the cladding thick- ness and temperatures, as would be expected and as i l l u s t r a t e d i n Fig. 2. Here we see the f i n a l cross-sectional shape of an or ig ina l ly cyl indri- c a l f u e l p in a f t e r i r r ad ia t ion under the indicated conditions. Where t h e i n i t i a l pressure d i f f e r e n t i a l across the cladding was high, t he
cladding w a l l was thin, and the cladding temperature was a l so high, as i n t h e f i r s t case, very severe and qui te unsat isfactory collapse of the f u e l p in occurred. operated with a high pressure d i f f e r e n t i a l and a r e l a t i v e l y high cladding
temperature, but with a thicker cladding which was more s tab le and col-
lapse occurred more slowly. 16,000 Mwd/tonne burnup before developing a dimple, and a t t h a t location, a crack i n the cladding. When we went t o lower cladding temperatures
and s l i g h t l y th icker cladding we found a more s t ab le condition, and i n f ac t , t h i s pa r t i cu la r p in ( t h e t h i r d one on the f igure) survived t o the
design goal of 60,000 Mwd/tonne burnup.
t h e diameter change of l e s s than 1% was qui te acceptable. p in i n the same i r r ad ia t ion t e s t i s shown as the fourth cross section. This p in w a s prepressurized t o lower t h e i n i t t a l a on the cladding
and showed no deformation whatsoever a t 60,000 Mwd/tonne.
The
The second cross sect ion i s from a p in t h a t a l so
This par t icu lar t e s t survived t o
S l igh t ova l i ty developed, but A similar
Chemical Interact ions
The chemical in te rac t ions between fuel, f i s s i o n products, and
cladding a re generally present but not severe below 75OoC, although they increase i n sever i ty a t higher temperatures. t r a t e d the general trend of the react ion between f u e l and cladding as a function of cladding temperature fo r Hastelloy X cladding on (U, Pu) O2
fueled GCBR pins . A t a cladding ins ide temperature of about 700°C up
t o 60,000 Mwd/tonne burnup there i s a react ion layer about 2 t o 3 mils
thick; but it i s a uniform react ion layer, and there i s no measurable
thinning of t he cladding.
d i t ion .
developed i n the cladding, and these a re a source of concern.
In Fig. 3 we have i l l u s -
- This i s considered t o be a sa t i s f ac to ry con-
A t 750°C and 16,000 Mwd/tonne burnup, subsurface voids have
A t the
Q
A
871
1 - 5 1 3 5 0
950 500 800 950
7 50
IN IT IAL AP.psi
700 700 CLAD 1, 'C 800
15 19.5 15 9 CLAD THICKNESS, mils
CLAD O.O..in. 0.345 0.345 0.373 0.353
Fig . 2. Has te l loy X Clad (U,Pu)02 GCBR Fuel Pins with Varying Degrees of S t a b i l i t y .
TEMP, "C
B.U. Mwd/T
700
60,000
7 50
16,000
810
5,000
8 50
5,000
Fig. 3 . Chemical In t e rac t ion Between Hastel loy X Cladding and ( U , P U ) O ~ i n GCBR Fuel Pins .
872
higher temperatures t h e extent of t h e r eac t ion increases, more voids a r e observed even deeper i n the cladding, sometimes in te rgranular cracks
a r e observed, and cladding thinning becomes measurable. This i s con- s idered an undesirable condition.
I n Fig. 4 we see a comparison of t h e type 316 s t a i n l e s s s t e e l
cladding and Hastelloy X cladding compat ib i l i ty with the mixed oxide
f u e l .
a t the fuel-cladding in t e r f ace , but it represents t h e extent of our compatibil i ty experience with type 316 s t a i n l e s s s t e e l t o da te . This
comparison may ind ica t e t h a t Hastelloy X i s s l i g h t l y super ior t o t h e s t a i n l e s s s t e e l . On t h e o ther hand, type 3l6 s t a i n l e s s s t e e l has shown
s a t i s f a c t o r y compat ib i l i ty with t h e mixed oxide f u e l a t temperatures up
t o 700°C i n work a t General E l e c t r i c Company on t h e LMFBR program.
This i s a l imi ted comparison a t somewhat d i f f e ren t temperatures
Fig. 4 . Comparison of Fuel Cladding In t e rac t ions i n Fuel Rods GA-17 and -18, Capsule P8.
We have examined by e l ec t ron microprobe ana lys i s t h e r eac t ion l aye r on a Hastelloy X c lad rod which operated a t :7000C t o 60,000 Mwd/tonne
burnup.
n i cke l and chromium through t h e r eac t ion zone i s q u i t e similar t o t h a t
observed i n t h e sur face l aye r on s t a i n l e s s s t e e l oxidized i n moist a i r a t 800°C.
As shown i n Fig. 5, we found t h a t t h e d i s t r i b u t i o n of i ron ,
The low poin t on each curve represents background l e v e l
873
Fig. 5 . Strip-Chart Recordings of Microprobe X-Ray Scans Across Fuel-Cladding Interface.
( t he re i s no plutonium i n the cladding).
products i n the react ion zone or obtained absolute values f o r the con-
centrat ion of the const i tuents . We hope t h a t ref ined analyses of t h i s
type w i l l lead t o a be t t e r understanding of t h e reactions tha t a r e
taking place and, perhaps, t o means for control l ing o r minimizing these
fuel-cladding interact ions.
We have not looked fo r f i s s i o n
a74
Summary
The sealed fuel-cladding-interacting concept appears t o be qui te This con- viable a t low and intermediate temperatures (below 750°C).
cept has performed successfully i n the l a t e s t t e s t i n t h i s se r ies with
t h e mixed oxide f u e l and both Hastelloy X and type 316 s t a in l e s s s t e e l
cladding. However, some of t h e e a r l i e r t e s t pins (pa r t i cu la r ly one operating a t 750°C and another a t 835°C) f a i l e d during tes t ing .
of these ear ly r e s u l t s and because of i t s higher temperature po ten t i a l
and s imi l a r i t y with the W B R technology, t h e manifolded-vented concept
has been chosen as the reference f o r the GCBR and t h e fuel-cladding-
in te rac t ing concept relegated t o backup s t a tus .
Because
Manifolded Pin Test
The f i r s t i r r ad ia t ion t e s t of an instrumented (U,Pu)O2 fueled
manifolded f u e l p in was s t a r t e d i n t h e ORR i n March 1970 toward a burhup
goal of grea te r than 50,000 Mwd/tonne a t a l inear heat generation r a t e
of 16 kw/ft.
sure external t o t h e f u e l cladding i s 1000 : p s i , while t he i n t e r n a l
pressure i s 25 p s i higher. The design of tine f u e l p in and capsule i s shown i n Fig. 6. The f u e l p in i s a shortened version of a GCBR mani-
folded f u e l p in with a 10-in. f u e l column, TJO2 blanket p e l l e t s a t t he
ends of t h e f u e l column, and an in t e rna l charcoal t r ap . The charcoal
t r a p would be located on the i n l e t coolant end of a f u e l p in and i s therefore maintained a t 300°C t o simulate the GCBR coolant i n l e t temper-
a tures .
used t o co l l ec t samples of t he f i s s i o n gases t h a t ge t out of t he f u e l
and blanket region, i n t o and through t h e charcoal t rap . permit t he maintenance of a dynamic balance between the coolant over-
pressure and t h e f u e l p i n in t e rna l pressure. There a re thermocouples along the length of the f u e l p in and i n the charcoal t r ap region.
The cladding outer surface temperature i s 700°C; t h e pres-
The gas l i nes running in to t h e top and bottom of t h e t r ap a re
These a l so
A preliminary analysis of t h e r e s u l t s too date from t h i s capsule
indicates very sa t i s f ac to ry performance of t,he f i s s i o n product t r ap .
Measurements under s teady-state operating conditions show t h a t t he short-l ived gaseous f i s s i o n products decay i n the t r ap and a r e not
A
r
875
GAS LINES
HEATER
GAS LINE
THERMOCOUPLES I + (TYPICAL ) -
.- 2 THERMAL DAM-
CHARCOAL TRAP
THERMOCOUPLES
AI203 INSULATOR U02BLANKET
U02 (ENR) PELLETS
(U-12% Pu) O,.,, FUEL
316 STAINLESS STEEL CLADDING
a
UOz(ENR) PELLETS
U02 BLANKET INSULATOR
B NaK-
PRIMARY AND
CONTAINMENT+
i
Fig. 6. I r r a d i a t i o n Manifolded Fuel Pin;
Capsule Capsule
Containing 04- P9.
Table 3 . I n i t i a l GCBR Em-IT I r r a d i a t i o n Tests
Cladding Temperature
( " C >
Burnup (Mwd/t onne)
700 25,000 700 50,000 700 100,000
600
650
750
800
50,000
50,000
50,000
50,000
876
re leased i n s ign i f icant quant i ty from the f u e l pin. A s was expected,
t h e very long-lived gases a r e not s ign i f i can t ly affected by the t rap .
Future measurements of t r ap performance w i l l include both steady-state
and pressure t rans ien t conditions.
Fast Flux Tests
We a re present ly constructing a s e t of eight GCBR f u e l pins t o be
i r r ad ia t ed i n EBR-11.
t h a t there w i l l be a low pressure d i f f e r e n t i a l across the cladding and
a la rge f i s s ion gas plenum and charcoal t r a p a r e included t o prevent
t he buildup of high f u e l p in i n t e r n a l pressilres.
t ions f o r t h e t e s t pins a r e outlined i n Tab:Le 3.
operated a t cladding temperatures between 600 and 800°C. The 600°C
temperature i n these tests w i l l provide a common point for comparison
of r e s u l t s with those from the LMFBR program
a cladding outside diameter temperature of ?OO"C w i l l permit a d i r e c t comparison with the manifolded f u e l p in i n our current thermal reactor
t e s t .
neutrons/cm2 at the maximum design burnup of: 100,000 Mwd/tonne.
cladding fluences, although only one-third to one-fourth of those
a t t a ined a t f u l l burnup i n a GCBR, w i l l produce s igni f icant fast neutron
damage t o the cladding and should answer some of t h e questions about t he
influence of t h i s damage on the performance of GCBR f u e l pins . pos t i r rad ia t ion analysis of charcoal fissiora. product t raps included i n
these pins will provide information on the a -b i l i t y of hot charcoal t o
remove condensable f i s s i o n products and t o d.elay short-l ived gaseous
products i n t h e fast f lux environment. Additional small, sealed con-
t a ine r s of charcoal are included t o study the e f f ec t s of t h e environ-
ment on charcoal sorption propert ies .
These w i l l simulate the manifolded design i n
The operating condi-
The pins w i l l be
Three of these pins with
The pins w i l l a t t a i n cladding fast f:Luences up t o 6 X lo2*
These
The
Our cooperative program w i t h GGA has shown t h a t a fuel-cladding in te rac t ing p in concept i s very promising; however, it requires t e s t ing
A
877
@ i n a f a s t - f l u reactor i n order t o examine the e f f ec t of f a s t neutron
damage on t h e cladding and how t h a t would influence the design of a f u e l
p i n which r e l i e s on uniform, controlled creep collapse of t h e cladding t o maintain f u e l p in in tegr i ty . The reference manifolded concept, which
has grea te r po ten t ia l , i s current ly under t e s t and appears t o be performing sat i s f a c t o r i l y .
We would l i k e t o g ra t e fu l ly acknowledge t h e numerous contributions
of others, both a t ORNL and GGA, which have contributed t o the e f f o r t reported here. In par t icu lar , J. R. Sil tanen and R. J. Campana of GGA
contributed strongly t o the design e f fo r t , and A. W. Longest and
J. A. Conlin of ORNL provided t h e i r r ad ia t ion capsule design and operat ion.
REFERENCES
1. P. Fortescue and W. I. Thompson, "GCFR Demonstration Plant Design," t h i s publication.
2 . D. B. Trauger, Some Major Fuel I r rad ia t ion Test F a c i l i t i e s of the Oak Ridge National Laboratory, ORI!&-3574 (Apri l 1964).
4. E. L. Long, Jr., F.'R. McQuilkin, D. R. Cuneo, J. R. Lindgren, and J. N. Sil tanen, " I r rad ia t ion Testing 'of Fuel Rods Containing UO;! and (U,Pu)O2 fo r GCFR," pp. 179-184 i n Ceramic Nuclear Fuels ( Inter- nat ional Symposium, May 3-8, 1969, Washington, D. C. Sponsored by t h e Nuclear Division of t h e American Ceramic Societyj ed. by 0. L. Kruger and A. I. Kaznoff, American Ceramic Society, Columbus, Ohio, 1969.
DISCUSSION
K. Wirtz: I t h i n k one has t o c o n g r a t u l a t e ORNL f o r these r e s u l t s .
I would l i k e t o make the fo l lowing comment. The temperatures i n d i c a t e d i n
your paper would n o t a l low a d i r e c t helium t u r b i n e cyc le . For a secondary
steam c y c l e lower temperatures would be s u f f i c i e n t . May I a sk whether
Oak Ridge has i n mind t o look a l s o t o advanced a l l o y s of any type t h a t
would al low h ighe r gas o u t l e t temperatures .
R. B. F i t t s : W e a r e examining t h e maximum tempera ture p o t e n t i a l s
f o r t h e s t a i n l e s s steel c l add ing m a t e r i a l s i n o r d e r t o a l low f o r t h e
recognized u n c e r t a i n t i e s i n des ign maximum c ladding temperature r equ i r e -
ment and i n o rde r t o cover t h e temperature reg ion above t h a t i n d i c a t e d
i n t h e p re sen t LMFBR program. W e a r e consid.ering the higher temperature
a l l o y s , such a s the Has te l loy X and o t h e r s , however, our p re sen t program
does n o t i nc lude f i r m p l ans t o e v a l u a t e these.
D. B. Trauger: W e t end t o be somewhat c o n s e r a t i v e a t ORNL. In
deference t o p o s s i b l e h o t s p o t s i n t h e core , i t seems d e s i r a b l e t o
e s t a b l i s h upper l i m i t s f o r f u e l performance. T h i s i s an important reason
f o r t he tests a t t empera tures above 700OC.
D. D. Tytga t : In t he EBR-I1 i r r a d i a t i o n , what w i l l be t h e r a t i o
between the f a s t f l u x i n t h e test r e a c t o r and tk one i n t h e 30 MWe
r e a c t o r a s desc r ibed by D r . Fo r t e scue? A r e ORNL and/or GGA doing some
work on t h e coated p a r t i c l e f u e l element des ign a s desc r ibed by M r . B a i r i o t .
R. B. F i t t s : A s I s a i d i n the t e x t , the f a s t f l u x w i l l be less
than t h a t expected f o r the r e fe rence GCBR. This is, of course, a l i m i t a -
t i o n encountered i n a l l c u r r e n t f a s t f l u x tests, however, the EBR-I1 f l u x
may a c t u a l l y provide a h ighe r damage r a t e due t o a different neutron
energy spectrum (See Reference 3 of paper) and i t w i l l probably provide
more than 1/3 of the r e f e r e n c e f a s t neut ron damage t o the c ladding .
Designs o t h e r than t h e meta l c l a d f u e l p in a r e n o t r e c e i v i n g our s e r i o u s
cons ide ra t ion a t ORNL a t t h i s t i m e .
Paper 6,409 A
J . A. Larr imore </ 0 J J . M. Waage
7
5 ’ ABSTRACT
The s t a t u s of t h e j o i n t East C e n t r a l Nuclear Group- Gulf General Atomic program on s a f e t y a s p e c t s of t h e Gas- Cooled F a s t Reac tor (GCFR), as p a r t of t h e o v e r a l l GCFR U t i l i t y Program, i s p r e s e n t e d . I n t r i n s i c and d e s i g n s a f e t y f e a t u r e s of t h e GCFR, s t u d i e s of a n t i c i p a t e d o p e r a t i o n a l o c c u r r e n c e s , s t u d i e s of des ign-bas is a c c i d e n t s , and con- ta inment s t u d i e s are reviewed. The c l o s e r e l a t i o n s h i p of GCFR technology t o HTGR technology is d i s c u s s e d , and t h e d i f f e r e n c e s between GCFR and LMFBR s a f e t y c o n s i d e r a t i o n s are p o i n t e d o u t .
INTRODUCTION
For t h e p a s t two y e a r s a program sponsored j o i n t l y by t h e East
C e n t r a l Nuclear Group and Gulf Genera l Atomic h a s been d i r e c t e d toward
t h e s a f e t y - r e l a t e d a s p e c t s of t h e Gas-Cooled F a s t Reac tor (GCFR) as p a r t
of t h e o v e r a l l GCFR U t i l i t y Program, whose p r o g r e s s i s r e p o r t e d i n a n o t h e r
paper’ i n t h i s s e s s i o n .
namely :
1.
The s a f e t y program h a s f o u r broad o b j e c t i v e s ,
E s t a b l i s h i n g s a f e t y c r i t e r i a f o r t h e d e s i g n of t h e GCFR and
i t s engineered s a f e t y f e a t u r e s .
2. Developing t h e d e s i g n b a s e s and f u n c t i o n a l requi rements f o r
p l a n t p r o t e c t i v e and engineered s a f e t y systems.
3 . Developing a n a l y t i c a l t e c h n i q u e s t o p r e d i c t t h e t r a n s i e n t
r e s p o n s e of t h e r e a c t o r t o v a r i o u s f a u l t c o n d i t i o n s .
Performing s a f e t y a n a l y s e s of t h e GCFR demonst ra t ion p l a n t
b e i n g des igned under t h e GCFR U t i l i t y Program.
4 .
T h i s p a p e r p r e s e n t s t h e s t a t u s of t h a t program.
879
aao
During t h e f i r s t y e a r , work w a s accomplished i n areas (1) and ( 3 ) ,
above. I n t h e second y e a r , t h e GCFR U t i l i t y Program h a s focused on t h e
d e s i g n of a demons t r a t ion p l a n t
changed from p r e l i m i n a r y s t u d i e s and methods development i n t o s a f e t y a n a l -
y s e s of t h e d e m o n s t r a t i o n p l a n t d e s i g n . Continued emphasis h a s been g iven
t o development of s a f e t y c r i t e r i a and t o t h e j - r i n c o r p o r a t i o n i n t h e demon-
s t r a t i o n p l a n t d e s i g n .
1 and t h e s a f e t y program h a s p r o g r e s s i v e l y
SAFETY FEATURES OF THE: GCFR
There are obv ious s a f e t y advan tages i n t h e u s e of t h e i n e r t gaseous
c o o l a n t , hel ium. E l i m i n a t i o n of p o s s i b l e change-of-phase problems and
c l a d d i n g - c o o l a n t reac t ions s i g n i f i c a n t l y ease t h e problems of e n g i n e e r i n g
f o r o v e r a l l system s a f e t y .
Impor t an t i n t r i n s i c s a f e t y f e a t u r e s of t h e GCFR are t h e n e g a t i v e ex-
p a n s i o n and Doppler r e a c t i v i t y t e m p e r a t u r e c o e f f i c i e n t s . These o v e r r i d e
t h e s m a l l p o s i t i v e c o o l a n t t e m p e r a t u r e c o e f f i c i e n t , r e s u l t i n g from dec reased
g a s d e n s i t y , d u r i n g a l l a n t i c i p a t e d o p e r a t i o n a l and a c c i d e n t s i t u a t i o n s .
The r e a c t o r h a s , t h e r e f o r e , a n e t n e g a t i v e po'der c o e f f i c i e n t .
The t o t a l r e a c t i v i t y worth of t h e p r e s s u - r i z e d he l ium i n a GCFR i s
s m a l l ; f o r t h e d e m o n s t r a t i o n p l a n t , i t i s c a l c u l a t e d t o b e about $ 0 . 3 8 .
T h e r e f o r e , f a i l u r e of t h e h e l i u m p r e s s u r e con ta inmen t , c a u s i n g r e d u c t i o n
i n he l ium d e n s i t y th roughou t t h e c o r e , canno t have a s e r i o u s r e a c t i v i t y
e f f e c t . L o c a l i z e d c o o l a n t v o i d i n g i s , o f cou:cse, n o t p o s s i b l e .
The r e a c t i v i t y e f f e c t of steam e n t r y i n t o t h e c o r e h a s been i n v e s t i -
g a t e d and found t o b e n e g a t i v e i n t h e d e m o n s t r a t i o n p l a n t f o r c o n c e n t r a t i o n s
up t o 3.4 l b / f t , c o r r e s p o n d i n g t o comple t e replacement of he l ium by s a t u -
r a t e d steam a t t h e p r e s s u r e vessel r e l i e f v a l v e s e t t i n g , which r e p r e s e n t s
a c o n s e r v a t i v e upper l i m i t . The n e g a t i v e e f f e c t i s due t o t h e r e sonance
a b s o r p t i o n by f i s s i o n p r o d u c t s . I n t h e i n i t i a l c o r e p r i o r t o a t t a i n m e n t
o f f i s s i o n - p r o d u c t e q u i l i b r i u m , t h e e f f e c t i s a l s o n e g a t i v e due t o i n c r e a s e d
3
881
worth o f t h e shim c o n t r o l r o d s , which are i n t h e c o r e d u r i n g t h a t per iod .
@ T h i s means t h a t steam g e n e r a t o r l e a k a g e o r f a i l u r e s w i l l n o t c a u s e reac-
t i v i t y a d d i t i o n s .
Perhaps t h e most impor tan t d e s i g n s a f e t y f e a t u r e of t h e GCFR is t h e
e n c l o s u r e of t h e e n t i r e pr imary c o o l a n t system i n t h e p r e s t r e s s e d c o n c r e t e
r e a c t o r v e s s e l (PCRV), t h e r e b y e l i m i n a t i n g pr imary c o o l a n t d u c t s . Because
of t h e c o n s e r v a t i v e d e s i g n b a s e s , t h e h i g h l y redundant p r e s t r e s s i n g system,
and t h e p r e d i c t a b l e , n o n c a t a s t r o p h i c f a i l u r e modes, PCRVs are c o n s i d e r e d
by many t o have a s i g n i f i c a n t s a f e t y advantage over s t e e l v e s s e l s . 2 A s
d e s i g n , c o n s t r u c t i o n , and o p e r a t i o n a l e x p e r i e n c e w i t h PCRVs accumulates
b o t h i n t h i s cotmtry and i n Europe, wider unders tanding and acceptance of
PCRVs can b e expec ted .
I n t h i s connec t ion , t h e c l o s e r e l a t i o n s h i p of GCFR technology t o t h e
High Temperature Gas-Cooled Reac tor (HTGR) technology i s worth emphasizing,
e s p e c i a l l y r e g a r d i n g t h e PCRV and t h e pr imary c o o l a n t system. The GCFR
development w i l l b e n e f i t i n many areas from HTGR e x p e r i e n c e , n o t on ly w i t h
r e s p e c t t o d e s i g n , c o n s t r u c t i o n , and o p e r a t i o n b u t a l s o w i t h r e s p e c t t o
s a f e t y and l i c e n s i n g exper ience . I n HTGR e x p e r i e n c e i n t h e U.S. t o d a t e ,
nonmechanis t ic g r o s s f a i l u r e of a PCRV p e n e t r a t i o n c l o s u r e i s p o s t u l a t e d
as a d e s i g n b a s i s f o r engineered s a f e t y f e a t u r e s , analogous t o t h e non-
m e c h a n i s t i c p i p e r u p t u r e used f o r t h e same purpose i n water r e a c t o r s .
( G r o s s f a i l u r e of t h e PCRV i t s e l f is n o t assumed c r e d i b l e . ) It must b e
expec ted t h a t a similar d e s i g n - b a s i s a c c i d e n t w i l l b e p o s t u l a t e d f o r t h e
GCFR, because t h e pr imary c o o l a n t system and PCRV d e s i g n are e s s e n t i a l l y
s imilar t o t h o s e i n t h e HTGR. It s h o u l d b e k e p t i n mind t h a t g r o s s PCRV
p e n e t r a t i o n f a i l u r e s are only p o s t u l a t e d e v e n t s and t h a t i n h e r e n t l y r e l i a b l e
p r e s s u r e containment i s provided by t h e PCRV.
A d e s i g n s a f e t y f e a t u r e s p e c i f i c t o t h e GCFR i s t h e d i rec t u s e of t h e
steam g e n e r a t e d t o p r o v i d e t h e hel ium c i r c u l a t i o n power, through series
d r i v e n t u r b o - c i r c u l a t o r s . The c o u p l i n g of t h e h e a t dump and t h e c i r c u -
l a t o r i n each loop increases t h e r e l i a b i l i t y of each c o o l i n g l o o p , and t h u s
a l s o t h e r e l i a b i l i t y of c o r e c o o l i n g . The GCFR t u r b o - c i r c u l a t o r s are
s i m i l a r i n concept and i n many d e t a i l s t o t h e HTGR t u r b o - c i r c u l a t o r s .
882
Another impor tan t d e s i g n f e a t u r e of t h e GCFR i s t h e p h y s i c a l separa-
t i o n of f u e l e lements t o accommodate fuel-element i r r a d i a t i o n s w e l l i n g and
bowing due t o g r a d i e n t s i n t h a t s w e l l i n g .
reducing mechanical i n t e r f e r e n c e between fue.L elements and by reducing t h e
r e a c t i v i t y swing d u r i n g a n i r r a d i a t i o n cyc le . .
T h i s i n c r e a s e s s a f e t y by g r e a t l y
The u s e of p r e s s u r e - e q u a l i z e d f u e l r o d s a l s o h a s impor tan t e f f e c t s on
a number of s a f e t y areas. Most impor tan t i s t h e e l i m i n a t i o n of f u e l f a i l -
u r e modes due t o c l a d d i n g c o l l a p s e from h i g h e x t e r n a l p r e s s u r e ( a t s t a r t
of i r r a d i a t i o n ) o r due t o c l a d d i n g deformat ion o r r u p t u r e from i n t e r n a l
f i s s i o n gas p r e s s u r e ( l a t e r d u r i n g i r r a d i a t i o n ) .
STUDIES OF ANTICIPATED OPERATIONAL OCCURRENCES
A s p a r t of t h e development of o v e r a l l p l a n t s a f e t y and r e l i a b i l i t y
c r i t e r i a , p l a n t f a u l t c o n d i t i o n s have been c l a s s i f i e d a c c o r d i n g t o accept -
a b l e s a f e t y consequences and a c c e p t a b l e f requency-of-occurrence, a l s o tak-
i n g i n t o account p l a n t a v a i l a b i l i t y . T h i s h a s r e s u l t e d i n i d e n t i f i c a t i o n
of t h o s e o p e r a t i o n a l o c c u r r e n c e s expec ted moderately f r e q u e n t l y o r i n f r e -
q u e n t l y t h a t w i l l b e ana lyzed t o e s t a b l i s h t h e d e s i g n b a s e s f o r t h e p l a n t
c o n t r o l system and t h e p l a n t p r o t e c t i v e system.
Assessment of a c c e p t a b l e sys tem responses t o t h e s e o p e r a t i o n a l t r a n -
s i e n t s r e q u i r e s a n u n d e r s t a n d i n g of fue l -e lement damage t h r e s h o l d s . I n
t h e GCFR, f u e l - c l a d d i n g damage i s more l i m i t i n g t h a n f u e l m e l t i n g i n most
cases. Although c l a d d i n g hot -spot t e m p e r a t u r e s are l i m i t e d i n t h e GCFR
d e m o n s t r a t i o n p l a n t t o below 700°C (1300°F) i n normal o p e r a t i o n t o a s s u r e
s a t i s f a c t o r y long-term performance, c o n s i d e r a b l y h i g h e r c l a d d i n g tempera-
t u r e s are a c c e p t a b l e f o r b r i e f o p e r a t i o n a l t r a n s i e n t s . A s mentioned i n
t h e p r e v i o u s s e c t i o n , t h e i n e r t gaseous c o o l a n t and t h e p r e s s u r e - e q u a l i z e d
f u e l rod e l i m i n a t e s f u e l f a i l u r e modes d u e t o c ladding-coolant chemical
r e a c t i o n s o r t o deformat ion from e i t h e r i n t e r n a l o r e x t e r n a l p r e s s u r e .
Under a c c i d e n t c o n d i t i o n s , c l a d d i n g tempera tures c l o s e t o t h e m e l t i n g
p o i n t i n t h e h o t t e s t f u e l rods may w e l l b e a c c e p t a b l e .
Analyses c a r r i e d o u t t o d a t e i n t h i s a r e a of t h e s a f e t y program have
i n c l u d e d r e a c t o r p l a n t c o n t r o l and s t a b i l i t y s t u d i e s . The i n i t i a l s t u d i e s n
833
w e r e d i r e c t e d toward e s t a b l i s h i n g t h e k i n e t i c response of t h e GCFR c o r e .
@ These i n c l u d e d p r e l i m i n a r y t r a n s i e n t a n a l y s e s f o r b o t h s t a r t u p ana at-
power c o n d i t i o n s and a c o r e s t a b i l i t y a n a l y s i s i n which t h e e f f e c t s of
u n c e r c a i n t i e s i n t h e r e a c t i v i t y c o e f f i c i e n t s w e r e a s s e s s e d and found t o b e
minor. A n o n l i n e a r sys tems a n a l y s i s model, GAFTRN, u s i n g d i g i t a l - a n a l o g
s i m u l a t i o n t e c h n i q u e s i s p r e s e n t l y under development. T h i s computer code
i n c l u d e s models f o r t h e c o r e , b l a n k e t , and s h i e l d s , i n c l u d i n g h e a t t r a n s f e r
and k i n e t i c s w i t h r e a c t i v i t y feedbacks ; models f o r t h e main c o o l i n g l o o p s ,
i n c l u d i n g t h e steam g e n e r a t o r and t u r b o - c i r c u l a t o r ; and models f o r t h e
p l a n t c o n t r o l and p r o t e c t i v e systems. The code w i l l b e expanded t o t rea t
p a r a l l e l c o o l i n g loops . GAFTRN w i l l b e t h e p r i n c i p a l t o o l used f o r s tudy-
i n g a n t i c i p a t e d o p e r a t i o n a l o c c u r r e n c e s and w i l l b e used t o e s t a b l i s h
d e t a i l e d f u n c t i o n a l requi rements f o r t h e GCFR demonst ra t ion p l a n t c o n t r o l
and p r o t e c t i o n systems.
One p o t e n t i a l o p e r a t i o n a l o c c u r r e n c e i s t h e f a i l u r e of a steam gener-
a t o r t u b e , r e s u l t i n g i n t h e i n g r e s s of steam i n t o t h e pr imary c i r c u i t . T h i s
i s n o t a p o t e n t i a l l y dangerous event because , as mentioned ea r l i e r , t h e re-
a c t i v i t y e f f e c t w i l l b e n e g a t i v e . The p r i n c i p a l r a p i d e f f e c t w i l l b e an
i n c r e a s e i n p r e s s u r e i n s i d e t h e PCRV. D e t e c t i o n and loop i s o l a t i o n mea-
s u r e s are under s t u d y t o avoid PCRV p r e s s u r e r e l i e f v a l v e opening and t o
l i m i t t h e amount of water l e a k a g e i n t o t h e PCRV i n o r d e r t o reduce p l a n t
l o s s of a v a i l a b i l i t y i n case of s team t u b e leakage .
L o c a l damage, o r i g i n a t i n g i n a s i n g l e rod o r f u e l e lement from l o c a l
c o o l a n t f low r e d u c t i o n , must a l s o b e c o n s i d e r e d an i n f r e q u e n t b u t p o s s i b l e
o c c u r r e n c e , d e s p i t e d e s i g n p r o v i s i o n s a g a i n s t fue l -e lement f low b lockage .
The p r i n c i p a l concern i s t h e l i m i t i n g of p r o p a g a t i o n of l o c a l damage t o
a d j a c e n t e lements .
ena i n t h e GCFR, l o c a l damage can o n l y b e propagated by f u e l m e l t i n g ,
which would c a u s e channel b lockage and consequent r e d u c t i o n i n c o o l i n g
i n ne ighbor ing rods o r c a u s e o v e r h e a t i n g i n a d j a c e n t r o d s by c o n t a c t w i t h
molten material. The t i m e scale f o r p r o p a g a t i o n i s determined by t h e t i m e
t o reach m e l t i n g i n f u e l r o d s w i t h p a r t i a l l y reduced c o o l i n g and t h e t i m e
f o r p e n e t r a t i o n of h o t f u e l through one fuel-element w a l l t o an a d j a c e n t
one. S t u d i e s have been made u s i n g c o n s e r v a t i v e assumptions concern ing h e a t
With no p o t e n t i a l c o o l a n t phase-change-related phenom-
~ ~
884
t r a n s f e r and f u e l movement and t h e s e s u g g e s t t h a t l o c a l f a i l u r e p r o p a g a t i o n
i n a GCFR c o r e p r o g r e s s e s r e l a t i v e l y s lowly and t h a t t i m e s of t e n s of sec-
onds are a v a i l a b l e f o r d e t e c t i o n and r e a c t o r shutdown t o l i m i t damage t o
a c c e p t a b l e amounts. T h i s means t h a t s i g n a l s such as main c o o l a n t loop
a c t i v i t y may w e l l b e a d e q u a t e f o r r a p i d f u e l - f a i l u r e d e t e c t i o n ; t h e s u i t -
a b i l i t y of such d e t e c t i o n means i s c u r r e n t l y under a c t i v e s t u d y .
STUDIES OF DESIGN BASIS ACCIDENTS
A s mentioned ear l ier , t h e major d e s i g n - b a s i s a c c i d e n t f o r t h e GCFR
has been p o s t u l a t e d as t h e r a p i d d e p r e s s u r i z a t i o n of t h e pr imary system
due t o a nonmechanis t ic f a i l u r e of a PCRV p e n e t r a t i o n pr imary c l o s u r e w i t h
t h e r e a c t o r i n i t i a l l y a t ful l -power c o n d i t i o n s . T h i s a c c i d e n t i s b e i n g
used t o e s t a b l i s h t h e d e s i g n b a s e s f o r t h e p r i n c i p a l engineered s a f e t y
f e a t u r e s i n t h e p l a n t : PCRV p e n e t r a t i o n f low r e s t r i c t i o n means, emergency
c o r e c o o l i n g sys tems, and r e a c t o r containment b u i l d i n g and containment
c leanup sys tems. The a b i l i t y of t h e s e systems t o cope a d e q u a t e l y w i t h t h i s
p o s t u l a t e d a c c i d e n t w i l l a s s u r e t h a t ample margin e x i s t s i n coping w i t h
more r ea l i s t i c a c c i d e n t s , such as slow primary system d e p r e s s u r i z a t i o n .
Fol lowing HTGR p r a c t i c e , f low r e s t r i c t i o n means are des igned i n t o each
l a r g e p e n e t r a t i o n , s t r u c t u r a l l y independent oE t h e pr imary c l o s u r e , t o con-
t r o l t h e maximum ra t e of d e p r e s s u r i z a t i o n i n t o t h e secondary containment .
Core c o o l i n g d u r i n g and a f t e r such a n accideni: w i l l b e provided by c o n t i n -
ued o p e r a t i o n of t h e main c o o l i n g loops . Main-cooling-loop r e l i a b i l i t y
i n t h i s s i t u a t i o n i s i n c r e a s e d by h a v i n g t h e motive power f o r each h e l i i m
c i r c u l a t o r provided d i r e c t l y by steam produced from t h e r e a c t o r h e a t i n i t s
own loop. A u x i l i a r y c o o l i n g l o o p s , which are used f o r normal long-term
shutdown c o o l i n g , w i l l p r o v i d e a n i n d e p e n d e n t , redundant backup t o t h e
main c o o l i n g l o o p s . The redundancy and c a p a c i t i e s of t h e main and t h e aux-
i l i a r y c o o l a n t systems are s u f f i c i e n t t o a s s u r e adequate c o r e c o o l i n g cap-
a b i l i t y f o r t h e d e s i g n - b a s i s d e p r e s s u r i z a t i o n a c c i d e n t , c o n s i d e r i n g reason-
a b l e c o n c u r r e n t f a i l u r e s .
I n h e r e n t s t r u c t u r a l c h a r a c t e r i s t i c s of t h e PCRV, t o g e t h e r w i t h i n c l u -
s i o n of f low r e s t r i c t i o n means, a s s u r e t h a t d u r i n g d e p r e s s u r i z a t i o n t h e A
normal c o o l a n t f low p a t h s w i l l n o t b e i n t e r r u p t e d and t h a t no s i z a b l e
mechanical f o r c e s w i l l b e induced on PCRV i n t e r n a l s . C o n t r o l of c o r e
t e m p e r a t u r e s d u r i n g a d e p r e s s u r i z a t i o n a c c i d e n t r e q u i r e s o n l y b a l a n c i n g
d e c r e a s i n g c o o l a n t f low w i t h d e c r e a s i n g r e a c t o r r e s i d u a l power, a l l o w i n g
f o r degraded h e a t t r a n s f e r due t o reduced c o o l a n t d e n s i t y .
h e a t - t r a n s f e r phenomena d u r i n g t h e a c c i d e n t are r e a d i l y p r e d i c t a b l e and
can b e ana lyzed w i t h l i t t l e u n c e r t a i n t y , i n c o n t r a s t t o s i t u a t i o n s i n which
c o o l a n t change of phase o c c u r s .
@
F l u i d f low and
To a l l o w d e f i n i t i v e a n a l y s i s of d e p r e s s u r i z a t i o n a c c i d e n t s i n t h e GCFR,
a d i g i t a l t r a n s i e n t a n a l y s i s code, LOCTRN, i s b e i n g developed and i s cur-
r e n t l y b e i n g t e s t e d . LOCTRN r e p r e s e n t s t h e r e a c t o r as a multivolume sys-
t e m w i t h p a r a l l e l f low p a t h s d e p i c t i n g t h e pr imary c o o l a n t loops . The code
treats d e p r e s s u r i z a t i o n i n t o t h e secondary containment due t o a l e a k from
any volume, p r e d i c t i n g t h e c o o l a n t d i s c h a r g e ra te , p r e s s u r e s , and f lows i n
each s e c t i o n of t h e r e a c t o r , and t h e t r a n s i e n t r e s p o n s e of t h e c o r e , steam
g e n e r a t o r s , and c i r c u l a t o r s a t each t i m e s t e p .
c o o l i n g loops w i l l a l s o b e handled by t h e code.
The a c t i o n of a u x i l i a r y
To a i d i n t h e e s t a b l i s h m e n t of t e n t a t i v e s p e c i f i c a t i o n s f o r emergency
c o r e c o o l i n g systems f o r t h e GCFR demonst ra t ion p l a n t p r i o r t o complet ion
of LOCTRN, s i m p l i f i e d p a r a m e t r i c s t u d i e s of c o r e t e m p e r a t u r e s d u r i n g de-
p r e s s u r i z a t i o n a c c i d e n t s have been made u s i n g d i g i t a l h e a t - t r a n s f e r codes.
P a r t i a l l o s s of blower c a p a c i t y d u r i n g t h e a c c i d e n t h a s been cons idered .
The e f f e c t s of d e p r e s s u r i z a t i o n ra te , scram d e l a y t i m e , and secondary con-
ta inment b a c k p r e s s u r e have been i n v e s t i g a t e d . S i m i l a r s t u d i e s r e c e n t l y made
f o r a lOOO-MW(e) GCFR p l a n t by ORNL u s i n g a n a l o g computing methods are re-
p o r t e d i n a n o t h e r paper a t t h i s meet ing. 3
Maximum c l a d d i n g tempera tures d u r i n g a d e p r e s s u r i z a t i o n a c c i d e n t are
p l o t t e d i n F ig . 1. The c o n d i t i o n s are: 30-sec e x p o n e n t i a l d e p r e s s u r i z a -
t i o n down t o 2 a t m p r e s s u r e ; scram e f f e c t e d 3 sec a f t e r s ta r t of depressur -
i z a t i o n ; cont inued c o o l i n g by a l l main loops w i t h c i r c u l a t o r s m a i n t a i n i n g
c o n s t a n t speed, c o n s t a n t c o o l a n t i n l e t t empera ture t o t h e r e a c t o r .
The c l a d d i n g tempera ture h i s t o r i e s a f t e r scram e x h i b i t a c h a r a c t e r i s t i c
i n i t i a l o v e r c o o l i n g phase , d u r i n g which t h e h e a t removal from t h e c l a d d i n g
886
exceeds t h e t r a n s f e r of s t o r e d and decay h e a t from t h e f u e l t o t h e clad-
d ing , fol lowed by t r a n s i t i o n t o a q u a s i - s t a t i c e q u i l i b r i u m between decay
h e a t p r o d u c t i o n and c o o l a n t h e a t removal. During e s t a b l i s h m e n t of t h i s
second phase, c l a d d i n g tempera tures reach t h e i r h i g h e s t v a l u e s a f t e r
s e v e r a l hundred seconds .
From t h e curves i t can b e s e e n t h a t t h e t r a n s i e n t h e a t removal cap-
a b i l i t y of t h e main c o o l i n g loops i s such t h a t c l a d d i n g tempera ture rises
are a c c e p t a b l e . R e s u l t s f o r p a r t i a l l o s s of c i r c u l a t i o n c a p a b i l i t y cases
a l s o i n d i c a t e a c c e p t a b l e c l a d d i n g tempera ture rises, even down t o a l o s s
of two of t h e t h r e e main blowers . However, i n such a s i t u a t i o n , t h e aux-
i l i a r y loops would t a k e o v e r c o r e c o o l i n g w e l l b e f o r e c l a d d i n g tempera tures
r i s e f a r above normal.
The 30-sec t i m e c o n s t a n t , used i n t h e a c c i d e n t shown, i s the p r e s e n t
d e s i g n g o a l f o r t h e most r a p i d d e p r e s s u r i z a t i o n rate. Ear l ie r s t u d i e s in-
d i c a t e d t h a t t h i s i s r e a d i l y a t t a i n a b l e i n lOOO-MW(e) systems. I n t h e
demonst ra t ion p l a n t , i t may r e q u i r e smaller b u t s t i l l f e a s i b l e f low re-
s t r i c t i o n areas. S t u d i e s f o r a range of d e p r e s s u r i z a t i o n t i m e c o n s t a n t s
have shown t h a t t h e peak c l a d d i n g t e m p e r a t u r e s , o c c u r r i n g a f t e r s e v e r a l
hundred seconds when d e p r e s s u r i z a t i o n i s complete , are n o t v e r y s e n s i t i v e
t o t h i s v a l u e ; e . g . , t h e maximum c l a d d i n g tempera ture f o r t h e case shown
would b e about 40°F h i g h e r f o r a 20-sec, inst:ead of a 30-sec, d e p r e s s u r -
i z a t i o n t i m e c o n s t a n t .
A more s i g n i f i c a n t parameter a f f e c t i n g t :emperatures i n t h e depressur -
i z e d c o n d i t i o n i s t h e containment b a c k p r e s s u r e . D e p r e s s u r i z a t i o n of t h e
pr imary he l ium c o o l a n t i n t o t h e secondary Containment w i l l r e s u l t i n a
f i n a l o v e r p r e s s u r e i n any case, t h e amount depending on containment volume
and pr imary he l ium i n v e n t o r y . S i n c e g r e a t e r b a c k p r e s s u r e h a s a s i g n i f i c a n t
b e n e f i c i a l e f f e c t on emergency c o r e c o o l i n g d u r i n g t h e q u a s i - e q u i l i b r i u m
phase i n which peak c l a d d i n g t e m p e r a t u r e s o c c u r , t h e r e i s i n c e n t i v e b o t h
on s a f e t y and economic grounds t o keep containment volume l o w . C l e a r l y ,
a t r a d e - o f f s t u d y between emergency c o o l i n g equipment and procedures on
t h e one hand and h a n d l i n g and maintenance w i t h i n t h e containment on t h e
o t h e r i s r e q u i r e d t o e s t a b l i s h t h e optimum containment s i z e . S t u d i e s t o
887
d a t e i n d i c a t e t h a t a t l eas t 1 a t m o v e r p r e s s u r e can b e provided w i t h a n
a c c e p t a b l e s i z e d containment .
H i s t o r i c a l l y , a n o t h e r c lass of a c c i d e n t s h a s been hypothes ized f o r
f a s t r e a c t o r s i n v o l v i n g c o r e meltdown and p o s s i b l y subsequent compaction
i n t o a more reactive c o n f i g u r a t i o n fo l lowed by e x p l o s i v e d isassembly .
T h i s class of a c c i d e n t s h a s been extended t o c o n s i d e r s e v e r e r e a c t i v i t y
a c c i d e n t s r e s u l t i n g i n e x p l o s i v e d isassembly i n t h o s e r e a c t o r s i n which
c r e d t b l e o r a t least p h y s i c a l l y p o s s i b l e mechanisms f o r such r e a c t i v i t y
i n s e r t i o n s e x i s t . Using gas c o o l i n g i n h e r e n t l y e l i m i n a t e s t h e r e a c t i v i t y
i n s e r t i o n mechanism due t o c o o l a n t v o i d i n g . T h i s , coupled w i t h t h e pro-
v i s i o n of h i g h l y r e l i a b l e emergency c o r e c o o l i n g i n t h e GCFR, i n o u r
o p i n i o n , a l l o w s e l i m i n a t i o n of g r o s s c o r e meltdown o r e x p l o s i v e d i s -
assembly a c c i d e n t s as a d e s i g n b a s i s f o r t h e GCFR, as h a s been done f o r
thermal r e a c t o r systems. N e v e r t h e l e s s , because of a n t i c i p a t e d concern
over such a c c i d e n t s , w e have i n c l u d e d i n o u r program t h e development of
c a p a b i l i t y t o a n a l y z e them. R e s u l t s of GCFR tes t cases u s i n g a modi f ied
v e r s i o n of t h e MARS code f o r disassembly c a l c u l a t i o n s y i e l d v a l u e s s imi l a r
t o t h o s e f o r LMFBR sys tems. The v e r y c o n s e r v a t i v e d e s i g n of PCRVs f o r
s t a t i c l o a d i n g i n h e r e n t l y p r o v i d e s a l a r g e dynamic energy a b s o r p t i o n cap-
a b i l i t y . P r e l i m i n a r y e v a l u a t i o n s have shown t h a t t h e r e l a t i v e l y low p r e s -
s u r e s a s s o c i a t e d w i t h c o r e d isassembly r e s u l t i n dynamic l o a d i n g of t h e
PCRV w e l l w i t h i n i t s d e s i g n c a p a b i l i t y .
CONTAINMENT STUDIES
E f f o r t i s a l s o b e i n g g i v e n t o d e f i n i t i o n of d e s i g n b a s e s f o r c o n t a i n -
ment. The d e p r e s s u r i z a t i o n a c c i d e n t h a s been used as i n p u t f o r de te rmining
t h e p r e s s u r e and t e m p e r a t u r e h i s t o r y i n t h e conta inment , u s i n g t h e CONTEMPT
code4 modi f ied f o r t h e GCFR. The energy c o n t e n t of t h e hel ium i s l o w s o
t h a t on ly s m a l l p r e s s u r e o v e r s h o o t s above t h e d e s i r e d f i n a l o v e r p r e s s u r e
occur .
of c o n c u r r e n t steam g e n e r a t o r r u p t u r e h a s been c o n s i d e r e d ; a margin of a
few pounds p e r s q u a r e i n c h seems adequate .
a b l y n o t b e r e q u i r e d .
To e v a l u a t e t h e margin f o r containment d e s i g n p r e s s u r e , t h e e f f e c t
Containment c o o l i n g w i l l prob-
These c o n d i t i o n s g i v e c o n s i d e r a b l e f l e x i b i l i t y i n
@ containment d e s i g n f o r t h e GCFR.
888
F i s s i o n - p r o d u c t release r e s u l t i n g from t h e des ign-bas is d e p r e s s u r i z a -
Few c l a d d i n g f a i l u r e s w i l l occur , t i o n a c c i d e n t i s expec ted t o b e s m a l l .
and t h e o p e r a t i o n of t h e p r e s s u r e - e q u a l i z a t i o n system w i l l ac t t o l i m i t
release from f a i l e d r o d s .
REFERENCES
1. P. F o r t e s c u e and W. I. Thompson, "The GCFR Demonstrat ion P l a n t Design," ORNL Gas-Cooled Reac tor I n f o r m a t i o n Meeting, Oak Ridge , Tennessee, A p r i l 27-29, 1970.
2. C . P. Tan, "A Review of t h e Technology of P r e s t r e s s e d - C o n c r e t e Reactor P r e s s u r e Vessels," Nuclear S a f e t y , 11, I., 25-33, Jan.-Feb. 1970. -
3 . C . S. Walker, "Safe ty and A f t e r h e a t Removal S t u d i e s of t h e Gas-Cooled F a s t Reac tor , " ORNL Gas-Cooled Reac tor I n f o r m a t i o n Meeting, Oak Ridge, Tennessee, A p r i l 27-29, 1970; see a l s o , I I . G . O'Brien, 0. W. Burke, "Loss-of-Cooling Accidents and C o r e Coolclown R a t e s i n a Gas-Cooled F a s t Reac tor , " USAEC, Report ORNL-TM-2783, Oak Ridge N a t i o n a l Labora tory , December 1, 1969.
4 . L. C . R ichardson , e t a l . , "CONTEMPT--A Computer Program f o r P r e d i c t i n g t h e Containment Pressure-Temperature Response t o a Loss-of-Coolant Accident , " USAEC, Report IDO-17220, P h i l l i p s Petroleum Company, June 1967.
h
," 1800 v
W cz I- =I 1600 a
2 1400
cz W
W I-
0 z 1200 - 0 0 a
5 1000
2 800 X
2 A T M B A C K P R E S S U R E ; A L L BLOWERS O P E R A T I N G ; 3 0 - S E C D E P R E S S U R I Z A T I O N T I M E C O N S T A N T
D E S I G N I t C L A D D I N
h
0
v
900 2 + a
800 5 a
w E
700 t- U z
600 a
400 2 E
600 0 40 80 120 I60 200 240 280 320 360 400
T I M E ( S E C ) I
I
Fig . 1. Cladding Temperatures d u r i n g D e p r e s s u r i z a t i o n Accident i n t h e GCFR Demonstrat ion P l a n t .
Q 889
DISCUS S I ON
M. D a l l e Donne: I would l i k e t o know how you e n s u r e t h e w a t e r
f l o o d i n g of t h e s team t u r b i n e s which d r i v e t h e g a s b lowers does n o t
o c c u r .
J. A . Lar r imore : One i m p o r t a n t f u n c t i o n of t h e p l a n t c o n t r o l system
i s t o e n s u r e t h e p r o p e r b a l a n c e between f e e d w a t e r and he l ium f l o w s t o
each s team g e n e r a t o r d u r i n g s t e a d y s t a t e and t r a n s i e n t c o n d i t i o n s . A s
mentioned i n Pape r 1/119, t h i s c a n be performed b y a c o n t r o l v a l v e
between t h e s team g e n e r a t o r and t h e c i r c u l a t o r . The c o n t r o l and
t r a n s i e n t s t u d i e s referred t o i n t h e pape r w i l l be u s e d t o d e f i n e t h e
r e q u i r e d c o n t r o l system c h a r a c t e r i s t i c s .
W. K. Ergen: Is t h e gas-cooled f a s t r e a c t o r s u s c e p t i b l e t o compac-
t i o n and r e a c t i v i t y i n c r e a s e connec ted w i t h such compact ion?
J. A. La r r imore : The f u e l e l e m e n t s a r e s e p a r a t e d t o a l l o w space
f o r s t r u c t u r a l m a t e r i a l s w e l l i n g and bowing. Such a s e p a r a t i o n i s
a c c e p t a b l e o n l y i f c r e d i b l e c o r e compact ions would r e s u l t i n a c c e p t a b l e
r e a c t i v i t y i n s e r t i o n s . The most s e v e r e p o t e n t i t a l c o r e compaction
mechanism i d e n t i f i e d t o d a t e i s seismic induced motion. T h i s i s b e i n g
s t u d i e d e x t e n s i v e l y , c o n s i d e r i n g t h e dynamic r e sponse of s o i l , founda-
t i o n , con ta inmen t b u i l d i n g , PCRV and s u p p o r t , c o r e s u p p o r t , and f u e l
e l e m e n t s t o seismic l o a d i n g s . C u r r e n t r e s u l t s i n d i c a t e t h a t a c c e p t a b l y
s m a l l r e a c t i v i t y i n s e r t i o n s would r e s u l t even c o n s i d e r i n g wors t c o h e r e n t
f u e l e l emen t movement p a t t e r n s .
/
R . Cyhan: Have you c o n s i d e r e d a backup shutdown system f o r t h e
c o n t r o l r o d s ?
J. A. Lar r imore : I n t h e c u r r e n t d e s i g n , t h e 27 c o n t r o l r o d s a r e
d i v i d e d i n t o 2 1 sh im-con t ro l rods , e a c h hav ing '$0 .85 worth, and 6 s h u t -
down r o d s , e a c h hav ing $1.60 worth. The numbers of r o d s and w o r t h s a r e
chosen so t h a t t h e r e a c t o r can be shutdown by e i t h e r set s e p a r a t e l y , a l low-
i n g f o r an i n o p e r a t i v e rod. An a d e q u a t e shutdown c a p a b i l i t y i s p rov ided
by t h e s e two sets and an a d d i t i o n a l backup shutdown system i s n o t con-
@ s i d e r e d t o be n e c e s s a r y .
Paper 7/110
S A F E T Y AND A F T E R H E A T REMOVAL STUDIES O F T H E GAS-COOLED FAST REACTOR
2 $a C . S . W a l k e r
O a k R idge Na t iona l L a b o r a t o r y
ABSTRACT
T h e t e m p e r a t u r e v a r i a t i o n s in t h e f u e l a n d c ladding following loss of h e a t r e m o v a l capab i l i t y , m o d e l s t o r e p r e s e n t c o r e m e l t i n g a n d m o v e m e n t , a n d t h e cool ing r e q u i r e d to con ta in a m o l t e n c o r e have been s t u d i e d . m a i n coo lan t l oops , a n d two a u x i l i a r y c o o h n t loops w a s t aken as the p lan t m o d e l . ding t e m p e r a t u r e to 1 8 0 0 ° F a f t e r a d e p r e s s u r i z a t i o n to 15 p s i a on a 3 0 - s e c t i m e c o n s t a n t w a s found t o be a l m o s t 1% of t h e d e s i g n v a l u e . Mel t ing of t h e c ladding would begin within (3 f e w s e c o n d s if t h e coolan t w e r e lo s t t o 0 . 1 % of the d e s i g n v a l u e o n a 1 - s e c t i m e c o n s t a n t . me l t ing and c o m p a c t i o n would t a k e s eve ra l m i n u t e s , and c o m p a c t i o n would not o c c u r if f u e l f e l l f r o m the c o r e v o l u m e . It a p p e a r s f e a s i b l e t o con ta in t h e m o l t e n c o r e on t h e v e s s e l l i n e r a b o v e the bo t tom h e a d of t h e r e a c t o r v e s s e l if t he v e s s e l l i n e r cool ing is i n c r e a s e d t o a t o t a l w a t e r f low of 25, 000 g p m . having v e r y low p robab i l i t y of o c c u r r e n c e , but shou ld be of va lue in s e l e c t i n g t h e d e s i g n - b a s i s a c c i d e n t s .
A 1000 M w ( e ) G C F R having a mul t i cav i ty v e s s e l , six
T h e m i n i m u m mass f low t o l i m i t t h e m a x i m u m fue l c l a d -
F u e l
T h e a c c i d e n t s lexamined a r e l imi t ing c a s e s
INTRODUCTION
T h e g e n e r a l o b j e c t i v e s of t h e O R N L s a f e t y s t u d i e s a r e to
d e t e r m i n e t h e r e q u i r e m e n t s of t he p r o t e c t i v e a c t i o n s and p lan t
f e a t u r e s n e c e s s a r y t o i n s u r e t h a t c r e d i b l e a c c i d e n t s wi l l h a v e a c c e p t -
a b l e c o n s e q u e n c e s .
i n t e r e s t i n t h e s e s t u d i e s a r e t h o s e c o n c e r n e d with t h e e f f ec t s of
a loss of coo lan t p r e s s u r e o r a l o s s of cool.ant f l ow.
of h igh p o w e r d e n s i t y a n d low h e a t capac i ty- would be expec ted to
p r o d u c e a r a p i d t e m p e r a t u r e r i s e of t h e fue l following a n y d r a s t i c
a n d s u d d e n r e d u c t i o n in h e a t r e m o v a l c a p a b i l i t y .
T h e s a f e t y q u e s t i o n s in the G C F R concep t of
A combina t ion
T h e s t u d i e s to be d e s c r i b e d inc luded a n e x a m i n a t i o n of t h e
t e m p e r a t u r e v a r i a t i o n of t h e fue l e l e m e n t s fol lowing l o s s - o f - p r e s s u r e
and l o s s - o f - f l o w a c c i d e n t s t o g e t h e r with a Ideter ininat ion of t h e
890
891
@ e m e r g e n c y cool ing n e c e s s a r y t o cope wi th t h e s e a c c i d e n t s , a n e x a m i -
na t ion of p o s s i b l e m o d e l s t o s t u d y c o r e m e l t i n g and m o v e m e n t , a n d
a n e x a m i n a t i o n of t h e cool ing r e q u i r e d t o con ta in a m o l t e n c o r e .
In a n e f f o r t to r e p r e s e n t c u r r e n t t r e n d s in G C F R d e s i g n s , t h e
r e f e r e n c e w a s t aken to be a c o m p o s i t e of s e v e r a l d e s i g n s by Gulf
G e n e r a l A t o m i c .
b i l i ty s t u d y ; h o w e v e r , m a n y of t h e d e t a i l s a r e not s ign i f i can t i n e x a m -
ining t r e n d s i n a c c i d e n t b e h a v i o r .
of a lOOO-Mw(e) p lan t d e s c r i b e d in t h e A l t e r n a t e Coolant T a s k F o r c e
eva lua t ion s t u d y , WASH- 1089, w a s u s e d in t h e s e s t u d i e s .
A r e a s o n a b l y c o n s i s t e n t d e s i g n is needed f o r a f e a s i -
T h e d e r a t e d c o r e d e s i g n ( G C F R - 4 D )
1
LOSS O F COOLING ACCIDENTS AND COOLDOWN RATES
S e v e r a l l o s s -of - coolan t p r e s s u r e and l o s s -of - flow a c c i d e n t s
and v a r i o u s m e t h o d s f o r coping with t h e r e s u l t i n g c i r c u m s t a n c e s h a v e
been e x a m i n e d with a n ana log c o m p u t e r .
d e r a t e d c o r e d e s i g n w a s s i m u l a t e d by a r e p r e s e n t a t i v e fue l c h a n n e l
having t h e h i g h e s t power d e n s i t y expec ted in n o r m a l o p e r a t i o n with
the c o r r e s p o n d i n g t e m p e r a t u r e p r o f i l e of t h i s channe l , as ob ta ined
f r o m R e f . 1 .
o r l u m p s , wi th a point m o d e l f o r t h e n u c l e a r k i n e t i c s .
g e n e r a t o r b e h a v i o r w a s not inc luded e x c e p t t h a t t h e c o r e in le t t e m p - e r a t u r e w a s d e c r e a s e d f r o m 592 to 3 0 0 ° F i n the f i r s t 60 s e c a f t e r
r e a c t o r s c r a m t o r e p r e s e n t t h e p r o b a b l e t e m p e r a t u r e c h a n g e . T h e
mass f low w a s c o m p u t e d as a func t ion of c i r c u l a t o r s p e e d , a v e r a g e
coolan t p r e s s u r e , a n d c o r e in l e t t e m p e r a t u r e .
2 T h e p e r f o r m a n c e of t h e
T h e fue l c h a n n e l w a s b r o k e n into t h r e e axial r e g i o n s ,
T h e s t e a m
It w a s a s s u m e d t h a t t h e lOOO-Mw(e) G C F R would h a v e a m u l t i -
cav i ty v e s s e l , six m a i n coo lan t loops ( c i r c u l a t o r s a n d steam g e n e r a t o r s ) ,
and two a u x i l i a r y ( o r e m e r g e n c y ) coo lan t loops s i m i l a r t u t h e c u r r e n t
d e s i g n s f o r t h e 330-Mw(e) d e m o n s t r a t i o n p l a n t . 3
Dep res s u r i z a t ion A c c i d e n t s
A n exponen t i a l p r e s s u r e d e c a y to 1 5 p s i a f r o m t h e o r i g i n a l
va lue of 1 2 5 0 p s i a o n a t i m e c o n s t a n t of 30 s e c w a s c o n s i d e r e d as
892
being typical of the m o r e rap id l o s s - o f - p r e s s u r e acc idents .
of p r e s s u r e l o s s is representa t ive of that of a 3 6 , 3 0 0 f t
a 90 in .
s igna l .
the c o r e w a s overcooled init ially, with the cladding t e m p e r a t u r e
decreas ing f r o m 1200 " F to approximate ly 4 5 0 ° F and then increas ing
gradual ly t o approximately 1 0 6 6 ° F in t h e fuel channels having the
highest expected power densi ty .
This r a t e 3 volume having
2 hole . A r e a c t o r s c r a m w a s init iated by a flux-minus-flow
If al l the m a i n c i r c u l a t o r s remained in operat ion a t full speed ,
A d e p r e s s u r i z a t i o n accident accompanied with p a r t i a l loss of
the c i r c u l a t o r s w a s examined by assuming that s o m e of the c i r c u l a t o r s
began a coastdown at the s t a r t of the d e p r e s s u r i z a t i o n and the r e m a i n d e r
continued to r u n at full s p e e d .
c r i t e r i o n of l imiting the peak in the cladding t e m p e r a t u r e to 1800"F , it would be necessa ry f o r the ci rculators that remained in operat ion
a f t e r d e p r e s s u r i z a t i o n t o provide a mass flow of a l m o s t 1% of the full
p r e s s u r e des ign value, as shown in F i g . 1 . This flow capabili ty is
approximately 5070 of that of all six m a i n c i r c u l a t o r s operat ing at t h e i r
design speed , consider ing the 8 0 : l p r e s s u r e reduct ion and the reduced
c i r c u l a t o r inlet t e m p e r a t u r e .
of t h r e e m a i n c i r c u l a t o r s , but it does exceed the capabili ty of two
main c i r c u l a t o r s o r the two auxi l ia ry c i r c u l a t o r s provided f o r e m e r -
gency cooling i f all the m a i n c i r c u l a t o r s should fa i l .
Based on ari a r b i t r a r y cladding fa i lure
Such a flow capabili ty is l e s s than that
Addition of s e c o n d a r y containment that would hold the equi l ibr ium
p r e s s u r e to 30 psia would improve the mas:; flow capabili ty of the
c i r c u l a t o r s so that only one auxi l ia ry circul.ator would be needed to cc.01
the c o r e , and t h e r e b y redundancy would be p r e s e r v e d in e m e r g e n c y
cooling. C u r r e n t G C F R design proposa ls include p r e s s u r e - s u s t a i n i n g
secondary containment buildings that give a n equi l ibr ium p r e s s u r e of
30 psia after a d e p r e s s u r i z a t i o n acc ident .
values of equi l ibr ium p r e s s u r e indicate a d i r e c t trade-off between the
equi l ibr ium p r e s s u r e and the c i r c u l a t o r capac i ty . It a p p e a r s that a n
investigation of the economics of this t r a d e - off would be worthwhile.
4 Examinat ion of higher
893
Limiting L o s s of Flow C a s e s
T h e c i r c u l a t o r s in the c u r r e n t GCFR designs have v e r y l i t t le
iner t ia , and they can coas t down in speed rapidly a f t e r a l o s s of motive
power to produce a l o s s of mass flow m o r e rapidly than a d e p r e s s u r i -
zat ion. A loss of flow w a s r e p r e s e n t e d by a n exponential decay having
a t i m e constant of 1 s e c .
c i r c u l a t o r speed s igna l .
it i s difficult to envision events f o r a well-designed s y s t e m that could
lead t o rapid l o s s of motive power to a l l the c i r c u l a t o r s . However , in
a n effor t to examine l imiting c a s e s , t h e mot ive power w a s a s s u m e d to
be instantaneously removed f r o m different n u m b e r s of c i r c u l a t o r s , with
the remain ing c i r c u l a t o r s operat ing at full s p e e d .
a l s o r e p r e s e n t the coastdown of all the c i r c u l a t o r s to a m i n i m u m flow
produced by auxi l ia ry water tu rb ines o r pony m o t o r s dr iving t h e m a i n
c i r c u l a t o r s . A s shown in F i g . 2 , the m a x i m u m value of the cladding
t e m p e r a t u r e could be held below the a r b i t r a r y fa i lure point of 1 8 0 0 ° F
with a m i n i m u m uninterrupted flow capabili ty of approximate ly 17’70 of
that produced by all six c i r c u l a t o r s . T h i s i s l e s s than the capaci ty of
one of the m a i n o r auxi l ia ry c i r c u l a t o r s .
a f t e r s e v e r a l seconds during the 1 - s e c c a s e is the r e s u l t of a d e c r e a s e
in the t e m p e r a t u r e of t h e gas re turning to the c i r c u l a t o r s f r o m the
s t e a m g e n e r a t o r s .
A r e a c t o r s c r a m w a s init iated by a f lux-minus-
With the c i r c u l a t o r s dr iven by s t e a m turb ines ,
This s i tuat ion could
T h e i n c r e a s e in m a s s flow
If motive power w e r e instantaneously removed f r o m all t h e m a i n
c i r c u l a t o r s , one auxi l ia ry c i r c u l a t o r would have to be s t a r t e d within a n
i m p r a c t i c a l t i m e m a r g i n of 1 . 5 s e c a f t e r the scram t o keep the a r b i t r a r y
fa i lure c r i t e r i a ‘from being exceeded.
the coastdown would have t h e advantage of g r e a t l y reducing the r e q u i r e -
m e n t s placed on the e m e r g e n c y c o r e cooling s y s t e m s .
in the c a s e of uninterrupted minimum flow, increas ing the t i m e constant
f o r the coastdown f r o m 1 to 5 s e c ( a l s o shown in F i g . 2 ) allowed the
minimum flow capabili ty to be reduced f r o m 1 7 t o 1% (1 .52% mass flow),
which could be readi ly achieved with auxi l ia ry d r i v e m o t o r s f o r the m a i n
c i r c u l a t o r s .
constant to 10 s e c reduces the peak to 1 3 4 2 ° F f o r 1% flow capabi l i ty .
Increas ing the t i m e dura t ion of
F o r ins tance ,
F i g u r e 2 a l s o shows that a f u r t h e r lengthening of the t i m e
894
F i g u r e 3 shows how the i n c r e a s e in the t i m e constant to 5 s e c would
a l s o allow the m a x i m u m t i m e in te rva l f o r initiation of s t a r t u p of one of
the auxi l ia ry c i r c u l a t o r s to be as long as 30 s e c , a n in te rva l that is
comparable to the s t a r t u p t i m e s f o r e m e r g e n c y c o r e cooling s y s t e m s
in l ight-water-cooled pawer r e a c t o r s .
t i m e constant f o r the coastdown to 10 s e c vJould allow the t i m e m a r g i n
f o r s ta r t ing up auxi l ia ry c i r c u l a t o r s to be extended to 100 s e c .
A f u r t h e r lengthening of the
Cooldown Following a Reac tor S c r a m
A n o r m a l r e a c t o r s c r a m with the coolant m a s s flow held constant
produced cooldown r a t e s that might be rapid enough to cause concern
for t h e r m a l cycling of the c o r e and s t e a m g e n e r a t o r .
e r a t u r e at the c o r e outlet dropped f r o m 1082 to 6 5 0 ° F in 17 s e c , as
shown in F i g . 4 .
F i g . 4, o r purposefu l coastdowns of all the c i r c u l a t o r s a f t e r a s c r a m
might be used to limit the cooldown rate to a reasonable va lue .
ab le r a t e s of t e m p e r a t u r e change f o r i t e m s such as the fuel and cladding,
p r i m a r y loop ducting, and s t e a m g e n e r a t o r components need to be
es tab l i shed . A coolant flow reduct ion on a t i m e constant s o m e w h e r e
between 5 and 10 s e c would probably give a s y s t e m cooldown r a t e of 1
to 3 ' F / s e c , which approaches the limit f o r one type of s t e a m g e n e r a t o r .
T h e coolant t e m p -
A r a m p reduct ion i n c i r c u l a t o r s p e e d , as shown in
Accept-
5
MODELS FOR CORE MELTING AND MOVEMENT
The t e m p e r a t u r e var ia t ion as a function of t i m e throughout the
c o r e following a l o s s of cooling abi l i ty h a s been examined by m e a n s of
the CHEMLOC p r o g r a m . 'This p r o g r a m f r o m the Code C e n t e r a t the
Argonne National Labora tory w a s adapted to the IBM 360/75 computer
f o r the n e c e s s a r y calculat ions. The pr0gra.m had been or iginal ly p r e -
pared f o r studying the melt ing of water-cooled c o r e s a f t e r a loss-of-
coolant accident , and modifications w e r e m.ade to account f o r he l ium
r a t h e r than water ( o r s t e a m ) as a coolant, its well as to p e r m i t m o r e
r e a l i s t i c t e m p e r a t u r e prof i les .
6
895
In t h e s e calculat ions, the coolant mass flow w a s a t tenuated
exponentially on a 1 - s e c t i m e constant down to a n asymptot ic value of
0 .1% of n o r m a l . (This lower limit w a s chosen to prevent instabi l i t ies
that a p p e a r e d in the CHEMLOC p r o g r a m at z e r o f low.) At the instant
attenuation began, all f i ss ion power production w a s a s s u m e d to be
t e r m i n a t e d , and the only s o u r c e of power w a s taken to be that f r o m
the decay of f i ss ion products f r o m a n end-of-l ife c o r e .
divided into eight r a d i a l zones , numbered 1 through 8 f r o m inner to
o u t e r , e a c h containing a n equal vo lume.
subdivided into 13 axial zones .
t i m e r e q u i r e d a f t e r the init iation of the l o s s of mass flow & r the hot tes t
fucl cladding to r e a c h var ious t e m p e r a t u r e s in each r a d i a l zone .
a zone achieved a t e m p e r a t u r e of 5000"F, the f rac t ion of fuel that
mel ted w a s taken to be proport ional to che amount of hea t f u r t h e r
deposited in that zone .
the t i m e in te rva ls a f t e r the beginning of the l o s s of flow f o r half the
f u e l in each zone to mel t a r e shown in F i g . 6 .
The c o r e w a s
Each r a d i a l zone w a s f u r t h e r
F i g u r e 5 contains a n indication of t h e
After
Under the a s s u m p t i o n that the fuel did not move,
Melting w a s found to begin n e a r the c e n t e r of the axial length of
the fuel r o d s .
mol ten m a t e r i a l f e l l to the bottom of the c o r e and col lected on the
boundary of the c o r e and lower blanket without leakage.
rods remained inser ted without mel t ing . T h e molten m a t e r i a l w a s
added to the sol id m a t e r i a l a l r e a d y t h e r e in o r d e r to obtain the amount
of the c o r e that had reached full compact ion. T h e unmelted fuel pel le ts
above the mel ted zone w e r e a s s u m e d to fall t o t h e l o w e r in te r face of the
mel ted zone, where they would be supported by the j a m m e d sol ids below.
A r a d i a l zone would then cons is t of a compacted region at the bottom,
a region of unmelted jumbled fuel above it, and then a void extending
to the top.
to physical rea l i ty .
of the DOT computer code.
when approximately 7770 of the fuel w a s in t h e compacted region of
mel ted and unmelted m a t e r i a l , and 23% w a s in the jumbled region
In one model of the ana lys i s , it w a s a s s u m e d that the
T h e cont ro l
No a t tempt has been m a d e to r e l a t e th i s sequence of events
Reactivity calculat ions w e r e p e r f o r m e d by m e a n s
This m o d e l w a s found to become c r i t i c a l
896
above t h e compacted region.
r e q u i r e s e v e r a l m i n u t e s .
The approach to this condition would
Another m o d e l being examined is based on the assumpt ion that
melting of the fuel cladding allows the unrrielted fuel pel le ts to fa l l to
the boundary of the c o r e and lower blanket .
indicate that th i s collection of f u e l f r o m a jumbled c o r e could go c r i t i c a l ,
resul t ing i n rapid melt ing of this col lect ion.
mel ted fuel would r a i s e the react ivi ty a t a higher r a t e .
a p p e a r s to give the upper boundary to the energ; r e l e a s e f r o m cr i t ical i ty
caused by c o r e compact ion.
P r e l i m i n a r y calculations
F u r t h e r compaction of the
This model
P r e v i o u s models f o r calculating the reac t iv i ty excurs ion f r o m
the melting and compact ion in s m a l l fast r e a c t o r s have a s s u m e d that
l a r g e portions of the c o r e compacted in a gravi ty fa l l .
d e s c r i b e d above r e p r e s e n t a n a t tempt to es tab l i sh m o r e r e a l i s t i c
descr ip t ions of c o r e compact ion to d e t e r m i n e the m a x i m u m hypothetical
nuc lear e x c u r s i o n .
for es t imat ing the l imiting reac t iv i ty r a t e s f r o m compact ion of the c o r e
in o r d e r to es tab l i sh a n upper limit on the energy r e l e a s e . In a n ac tua l
meltdown, s o m e of the molten fuel, as well as s o m e of the unmelted
pel le ts , would probably fall f r o m the c o r e reg ion and cri t icali ty might
never be r e a c h e d .
8 J The models
T h e s e models w e r e developed to provide the bas i s
CONTAINING A N D COOLING THE MOLTEN CORE
T h e fuel, cladding, blankets , and c o r e in te rna l s t r u c t u r a l
m e m b e r s w e r e a s s u m e d to fa l l onto the bottom t h e r m a l shield 10 s e c
a f t e r r e a c t o r shutdown a t the s t a r t of the acc ident .
r a t e in the fuel and blanket a t any t i m e w a s a s s u m e d to be that f r o m
decay heat only.
m e l t in about 30 m i n .
c o r e and axial blankets w e r e to s e t t l e to th'e bottom of the mol ten
m a t e r i a l in a u n i f o r m layer without vaporizat ion, a s l a b about 5 i n .
thick with a n ini t ia l in te rna l heat-generat ion r a t e of 49 Mw(t) o r
approximately 10 B t u / h r * f t would f o r m . The v e s s e l l iner and
T h e hea t -genera t ion
In th i s s i tuat ion, the bottom t h e r m a l shield would
If the heavy oxide arid f i ss ion products f r o m the
6 3
subsequent ly the concre te would be subjected to molten U 0 2 at 5 0 0 0 ° F .
Since the n o r m a l v e s s e l l iner cooling water flow r a t e is not adequate to
remove the heat , the molten fuel would penet ra te the bottom head of the
r e a c t o r v e s s e l . If the concre te w e r e to spa11 off and float in the mol ten
U 0 2 , the 12-ft bottom head could be pene t ra ted in about 37 m i n . On the
o ther hand, if the fuel w e r e supported until the concre te mel ted , it
would r e q u i r e about 5 h r f o r the fuel to pene t ra te the head .
It a p p e a r s feas ib le to contain the mol ten fuel inside the v e s s e l
l iner i f the v e s s e l l iner cooling is i n c r e a s e d .
the cold s u r f a c e and provide a n insulating l a y e r that would limit the
heat flux into the v e s s e l l i n e r .
cooling on the f loor and lower s idewall of the v e s s e l l iner to r e m o v e
heat f r o m the f r o z e n U 0 2 l a y e r and main ta in the integri ty of the v e s s e l
l i n e r . T h e heat flux is approximately 750, 000 B t u / h r * f t . The heat
radiated f r o m the top of the mol ten pool would m e l t all the t h e r m a l
s h i e l d s .
v e s s e l l iner above t h e mol ten pool to remove the heat deposi ted by r a d i -
a t ion and convection. A to ta l water flow of approximate ly 25, 0 0 0 gpm
under the v e s s e l f loor and up the s idewalls f o r 15 f t would remove the
heat being genera ted with a 5 0 ° F r i s e in the water t e m p e r a t u r e . The
requi red flow would be equivalent to a shee t of water 2 in . thick flowing
a t a velocity of 10 f t / s e c with a path length of approximate ly 25 f t .
T h e fuel would f r e e z e on
It would be n e c e s s a r y to provide adequate
2
The cooling water flow would a l s o have to be i n c r e a s e d on the
A method f o r increas ing the s u r f a c e a r e a for cooling the mol ten
fuel would be to subdivide the v e s s e l f loor into deep, n a r r o w p a s s a g e s
with cooling w a t e r in tubes inside the par t i t ion w a l l s to f r e e z e the fuel
as the molten m a t e r i a l fell into the v e s s e l cavi ty . This approach would
minimize t h e meltdown of the t h e r m a l sh ie lds and reduce the heat input
to the upper p a r t of the v e s s e l .
cause s t r u c t u r a l complicat ions and probably be m o r e cost ly than i n c r e a s
ing the cooling water flow on the f loor and lower s idewalls of the v e s s e l
l i n e r .
However, th i s a r r a n g e m e n t would
89R
C ONC LUS IO NS Q
1.
2.
3 .
4.
5 .
6 .
rp I ..e a c c i d e n t s e x a m i n e d a r e h ighly un l ike ly , but w e r e thought
t o b e a p p r o p r i a t e l y s e v e r e .
t h o s e t h a t m a y be even tua l ly c o n s i d e r e d as. d e s i g n - b a s i s a c c i d e n t s .
Obv ious ly , t h e d e s i g n - b a s i s a c c i d e n t s m u s t be s e l e c t e d b e f o r e t h e a c t u a l
func t iona l r e q u i r e m e n t s c a n b e e s t a b l i s h e d f o r t h e e m e r g e n c y cool ing
sys tems.
e s t a b l i s h e d .
T h e y m a y o r m a y not be r e p r e s e n t a t i v e of
F a i l u r e c r i t e r i a f o r t h e f u e l and c ladding need t o be
T h e s t u d i e s h a v e b e e n i n s t r u c t i v e , a n d e v e n t h e s e p r e l i m i n a r y
r e s u l t s shou ld be he lp fu l i n eva lua t ing t h e (concept of t h e G C F R .
to c o p e wi th t h e l imi t ing c a s e s of the a c c i d e n t s e x a m i n e d a r e wi th in t h e
realm of e n g i n e e r i n g d e s i g n .
of e a c h a c c i d e n t e x a m i n e d shou ld place even less d e m a n d s on the d e s i g n .
S y s t e m s
S y s t e m s t o cope wi th m o r e r e a l i s t i c m o d e l s
R E F E R E N C E S
U . S . A t o m i c E n e r g y C o m m i s s i o n , An. E v a l u a t i o n of G a s - C o o l e d Fast R e a c t o r s , USAEC R e p o r t WASH-1089 ( A p r i l 1969) .
H . G . O ' B r i e n a n d 0. W. B u r k e . L o s s - o f - C o o l i n e Acc iden t s a n d 0
C o r e Cooldown R a t e s i n a G a s - C o o m F a s t R e a c t o r , O R N L - T M - 2 7 8 3 ( D e c e m b e r 1 , 1 9 6 9 ) .
P . F o r t e s c u e a n d W . I . T h o m p s o n , G C F R D e m o n s t r a t i o n P l a n t D e s i g n , P a p e r No . 119, S e s s i o n VII, O a k R idge Na t iona l L a b o r a - t o r y G a s - C o o l e d R e a c t o r I n f o r m a t i o n Mee t ing , A p r i l 27 -May 1 , 1970, t o a p p e a r in C o n f e r e n c e P r o c e e d i n g s , USAEC R e p o r t C O N F - 7 0 0 . 4 0 1 .
J . M . W a a g e a n d J . A . L a r r i m o r e , Sa.fety S tud ie s f o r t he G a s - Cooled Fast R e a c t o r , P a p e r No . 109, S e s s i o n N o . VII, O a k Ridge Nat io na 1 Lab0 r ato r y G as - C oo le d R e a c t o r I n f o r m a t i o n Mee t ing , A p r i l 27 -May 1, 1970, t o a p p e a r i n C o n f e r e n c e P r o c e e d i n g s , USAEC R e p o r t C O N F - 7 0 0 . 4 0 1 .
G a s - C o o l e d F a s t R e a c t o r P r o j e c t Staff (GGA), p e r s o n a l c o m m u n i - c a t i o n t o U . B . T r a u g e r , R . s . C a r l s m i t h , J . P . S a n d e r s , a n d C . S . W a l k e r ( O R N L ) , M a y 1969 .
J . C . H e s s o n , 3 . L . A n d e r s o n , a n d R . 0. Iv ins , CHEMLOC-11: A C o m p u t e r P r o g r a m D e s c r i b i n g t h e C o r e Heat ing and Cladding- Steam R e a c t i o n f o r a W a t e r - c o o l e d P o w e r R e a c t o r Fol lowing a Loss of Coo lan t , USAEC R e p o r t ANL-7361 ( A p r i l 1968) .
A
899
F. R . Mynatt , A U s e r s Manual. for DOT - A T w o Dimensional D i s c r e t e Ordinates T r a n s p o r t Code with Anisotropic Sca t te r ing , USAEC Repor t K-1694, Oak Ridge Gaseous Diffusion Plan t ( t o be publ ished) .
Argonne National Labora tory , A G e n e r a l Survey of the P r o c e e d - ings of the Conference on Safety, F u e l s , and C o r e Design in L a r g e Fast P o w e r R e a c t o r s , U S A E C Repor t ANL-7120 (October 14-15, 1965).
T . 3 . Thompson and J . G . Becker ley , The Technology of Nuclear Reac tor Safety, Chap. 1 0 , V o l . 1, T h e M . I . T . P r e s s , 1964.
900
3000
W [L
" 3 2000
1000
I-
0 -
w n 3 t- LL w a I w +
a
-___ 5-sec TIME CONSTANT --_ -
10- sec TIME CONSTANT
1-sec TIME CONSTANT
0 100 200 300 400 500 TIME (sec)
F i g . 1 . D e p r e s s u r i z a t i o n with M i n i m u m Coolant F l o w to P r e v e n t Cladding F a i l u r e .
100
50
0
F i g . 2 . E x a m p l e s of Loss of Coolant F low a t F u l l Coolant P r e s s u r e .
901
ORNL-DWG 69-42460
I
IO0
cn 2 50 I I- z J 0
a
8 0
p - I000 D Q J V
a
0
TIME (sec)
F i g . 3 . Loss of F low a t F u l l P r e s s u r e o n a 5-sec T i m e - C o n s t a n t with S t a r t u p of One A u x i l i a r y B l o w e r .
100
50 E 0
71-- -r--
---LA--
CONSTANT FLOW
I - FLOW RAMPDOWN
ORNL-DWG 69- 4 246t
100 120 20 40 60 80 TIME (sec )
F i g . 4. Cooldown Fol lowing a R e a c t o r S c r a m .
902
70
2 .o
h
0 a, ln Y
I-
W 0 0 0 Q LL 0 I-
1.5
-
1.0
2 cn [r W I- LL 0.5 a W 2 I- -
O
300
1 2 3 4 5 6 7 8 R A D I A L RING NUMBER
210
--180-
10 240
70 300
F i g . 5 . T i m e for H o t t e s t C lddd ing to R e a c h V a r i o u s T e m pe r a t u r e s F o 110 wing Loss of C o o l i n g .
903
DISCUSSION
D. B. T r a u g e r : A s t h e p a p e r s and t h e d i s c u s s i o n of t h i s s e s s i o n
i n d i c a t e , t h e i m p o r t a n t problems f o r t h e GCFBR a r e s u b j e c t t o r a t h e r
s t r a i g h t f o r w a r d e n g i n e e r i n g a n a l y s i s and t e s t i n g . I t s h o u l d be p o s s i b l e
t h r o u g h a modest e f f o r t t o u n d e r s t a n d t h e s e problems. With s u c h r e s u l t s
a t hand and t1.e r e a c e s s m e n t of t h e i n d i c a t e d economic a d v a n t a g e s , i t t h e n
would be p o s s i b l e t o e f f e c t i v e l y e v a l u a t e t h e c o n c e p t . A t t h a t t i m e a
d e c i s i o n s h o u l d be made t h a t t h e GCFBR i s e i t h e r i m p r a c t i c a l and s h o u l d be
d ropped or i s a t t r a c t i v e and s h o u l d be pu r sued . The i m p o r t a n t p o i n t i s
t h a t t h e c o n c e p t c a n be e v a l u a t e d b y r a t h e r s t r a i g h t f o r w a r d methods and
a modest e f f o r t . S i n c e t h i s i s p o s s i b l e w i t h o u t much effor t i t s h o u l d be
done .
904
DISCUSS ION
W. F. Hzussermann
ASPECTS OF GAS-COOLED FAST REACTOR DEVELOPMXNT AT ENEA
In J a n u a r y 1968 t h e ENE-4 committee of Exper t s on Co-operat ion i n t h e
Reac tor F i e l d , known a s t h e Top Level Group m e t t o examine what scope
t h e r e was f o r c o - o p e r a t i o n between LTEA Member C o u n t r i e s t o deve lop and
e x p o l i t advanced power reac-cors . The Top Level Group concluded t h a t any
j o i n t e f f o r t would b e s t be d i r e c t e d towards promoting t h e c o n s t r u c t i o n
of heavy w a t e r power r e a c t o r s and e x t e n d i n g t h e scope of t h e development
of f a s t r e a c t o r s .
Up t o t h a t t i m e , a n enormous amount of FR work i n Europe had concen-
t r a t e d on sodium c o o l i n g , whereas t h e p o t e n t i a l of o t h e r c o o l a n t s had been
t r e a t e d o n l y b r i e f l y . I t was dec ided t h a t , because a l a r g e amount of
proving remained t o be done b e f o r e sodium c o u l d be confirmed a s a good
s o l u t i o n t o t h e problem of c o o l i n g a f a s t r e a c t o r , i t was d e s i r a b l e a t
l e a s t t o a s e s s t h e p o s s i b i l i t i e s of u s i n g s team and g a s a s a l t e r n a t i v e
c o o l a n t s .
The c o s t of such a s s e s s m e n t s would p r e v e n t Western European c o u n t r i e s
from embarking on s e p a r a t e n a t i o n a l programmes, e s p e c i a l l y s i n c e i t would
create c o m p e t i t i o n f o r money a l r e a d y b e i n g s p e n t on sodium c o o l i n g . Thus
t h e i n v e s t i g a t i o n of a l t e r n a t i v e c o o l a n t s f o r f a s t r e a c t o r s appeared v e r y
s u i t a b l e f o r i n t e r n a t i o n a l co-opera t ion where governmental a s w e l l a s
i n d u s t r i a l i n t e r e s t would be involved .
A s a f i r s t s t e p , t w o s p e c i a l i s t teams were set up by ENEA t o e v a l u a t e
t h e m e r i t s of s team and g a s c o o l i n g r e l a t i v e t o sodium. The t e c h n i c a l
b a s i s f o r t h e s t u d i e s was c o n t r i b u t e d from n a t i o n a l s t u d i e s done i n Belgium,
Germany, Sweden, S w i t z e r l a n d and t h e United Kingdom. I n a d d i t i o n , t h e
p r e l i m i n a r y c o n c l u s i o n s of a s i m i l a r exercise done by t h e USAEC i n c o l l a b -
o r a t i o n w i t h American i n d u s t r y were made a v a i l a b l e . I n d u s t r i a l f i r m s were
encouraged t o p a r t i c i p a t e i n t h e work of t h e two s p e c i a l i s t teams and
i n d u s t r y ' s formal a s s o c i a t i o n was a s s u r e d through Foratom.
905
I t soon became c l e a r t h a t f u e l s h o u l d be g i v e n p r i o r i t y f o r deve lop -
ment f o r b o t h g a s and steam c o o l e d f a s t r e a c t o r s . The members of t h e s e
e x p e r t teams a l s o ag reed t h a t t h e r e was a need f o r a l a r g e f u e l tes t
f a c i l i t y which might a l s o be conce ived a s a p r o t o t y p e power s t a t i o n . A
number of f u e l - c l a d d i n g o p t i o n s w e r e s t u d i e d , i n c l u d i n g v a r i o u s n i c k e l -
based a l l o y s f o r t h e SCR p r e p r e s s u r i z e d t o w i t h s t a n d t h e f o r c e of t h e
c o o l a n t p r e s s u r e , and a l s o " s t r o n g c l a d " and "weak c l a d " ( v e n t e d ) f u e l s
f o r t h e GCR a l t h o u g h f o r t h i s r e a c t o r p a r t i c u l a r i n t e r e s t i s be ing shown
i n f u e l d e s i g n s u s i n g c o a t e d p a r t i c l e s w i t h a s i l i c o n e c a r b i d e o u t e r
l a y e r , a s deve loped by t h e Dragon P r o j e c t f o r t h e HTR.
To s t r e a m l i n e a c o - o p e r a t i v e development programme, some r e d u c t i o n
was o b v i o u s l y n e c e s s a r y i n t h e o p t i o n s a v a i l a b l e . One s t e p i n t h i s
d i r e c t i o n was t h e s t o p p i n g of work on s team c o o l i n g f o r f a s t r e a c t o r s ,
f i r s t i n t h e U.S.A. and more r e c e n t l y i n Germany, and development of t h i s
v a r i a n t i s u n l i k e l y t o be t a k e n any f u r t h e r w i t h i n t h e framework of ENEA.
S t i l l , t o e s t a b l i s h a sound b a s i s f o r f u t u r e d e c i s i o n s on gas -coo led f a s t
r e a c t o r s , t h e e x p e r t s e s t i m a t e d t h a t a c o n s i d e r a b l e body of e x p e r i m e n t a l
r e s u l t s was needed i n s u p p o r t of t h r e e f u e l c o n c e p t s ; s t r o n g c l a d , v e n t e d ,
and c o a t e d p a r t i c l e and on two t y p e s of c o o l a n t ; CO and hel ium. 2
The a c t u a l development of gas-cooled f a s t r e a c t o r f u e l s would cer-
t a i n l y be done i n n a t i o n a l l a b o r a t o r i e s unde r government s p o n s o r s h i p where
t h e n e c e s s a r y e x p e n s i v e f a c i l i t i e s a l r e a d y e x i s t . W e feel t h a t i f a
c l o s e d i n t e r g o v e r n m e n t a l group of f u e l t e s t i n g were formed, under t h e
a u s p i c e s of ENEA, i t c o u l d n o t o n l y c o - o r d i n a t e t h e s e n a t i o n a l programmes,
b u t a l s o r e q f o r c e t h e p r i v a t e i n d u s t r i a l e f f o r t s now drawing up t h e
t e c h n i c a l j u s t i f i c a t i o n f o r a f u l l - s c a l e gas -coo led f a s t r e a c t o r i n s t a l l a -
t i o n . -
An a t t e m p t was made by ENEA i n S p r i n g 1969 t o d e v i s e a v o l u n t a r y
d i s t r i b u t i o n of t h e e s s e n t i a l development work amongst t h e i n d u s t r i a l and
governmental e s t a b l i s h m e n t s of i n t e r e s t e d c o u n t r i e s . U n f o r t u n a t e l y , i t
was n o t p o s s i b l e t o o b t a i n agreement upon an immediate j o i n t programme,
because t h e r e were l a r g e d i f f e r e n c e s of o p i n i o n a s t o t h e j u s t i f i c a t i o n s
f o r f o l l o w i n g up t h e p o t e n t i a l of c o o l a n t s a l t e r n a t i v e t o sodium.
~~~~ ~~ ~
906
F o r example, one body of o p i n i o n h e l d -chat t h e r e was n o t a s t r o n g
enough r e a s o n f o r d i v e r t i n g some of t h e e f f o r t which i s a t p r e s e n t dep loy-
ed on sodium r e a c t o r deve lopment ; and t h a t work on an a l t e r n a t i v e c o o l a n t
was a d m i s s i b l e o n l y a s a s u p p o r t i n g measure t o i n s u r e a g a i n s t un fo reseen
d i f f i c u l t i e s i n t h e a p p l i c a t i o n of sodium t e c h n o l o g y on a l a r g e s c a l e .
Thus t h i s g r o u p b e l i e v e d t h a t i t was a d v i s a b l e t o c o n c e n t r a t e f o r y e a r s
y e t on sodium c o o l i n g b e f o r e d e v o t i n g much f i n a n c i a l and s c i e n t i f i c e f f o r t
t o d e v e l o p i n g a l t e r n a t i v e c o o l a n t s .
On t h e o t h e r hand, an e q u a l l y s t r o n g body of o p i n i o n h e l d t h a t t h e
ENEA e v a l u a t i o n had r e v e a l e d s u f f i c i e n t p o t e n t i a l a d v a n t a g e s t o j u s t i f y
t h e development of an a l t e r n a t i v e c o o l a n t irk i t s own r i g h t , i r r e s p e c t i v e
of t h e s u c c e s s o r problems of sodium. T h i s s c h o o l of though t b e l i e v e d
t h a t t h e g a s c o o l i n g concep t had ample scope f o r s h a r i n g i n t h e f u t u r e
f a s t r e a c t o r market w i t h sodium and t h a t t h e r e was m e r i t i n m a i n t a i n i n g
t h e p r i n c i p l e o f c h o i c e which h a s e v o l v e d i n t h e t h e r m a l r e a c t o r marke t .
S u c c e s s f u l commercial development of t h e t h e r m a l HTGCR and c o a t e d
p a r t i c l e f u e l s i s c l e a r l y i m p o r t a n t for t h e f u t u r e of g a s c o o l i n g f o r
f a s t r e a c t o r s , and hence t h e n e x t t w o y e a r s a r e l i k e l y t o be c r u c i a l i n
t h i s r e s p e c t . W e hope t h a t w i t h i n t h i s t ime s c a l e , i t w i l l be p o s s i b l e
t o o r g a n i z e a v i a b l e i n t e r n a t i o n a l p r o j e c t f o r t h e development of g a s
c o o l i n g f o r f a s t r e a c t o r s .
A s an i n i t i a l s t e p , a Working Group on Gas-Cooled F a s t R e a c t o r s h a s
been set up by ENEA t o exchange i n f o r m a t i o n and t o f o r m u l a t e more p r e c i s e
p l a n s f o r f u t u r e work. E leven European c o u n t r i e s , t h e U.S.A., and Japan,
a s w e l l a s Euratom and Foratom p a r t i c i p a t e i n t h i s Working Group which
m e t i n May and i n December 1969 and p u b l i s h e d a S t a t u s Repor t on Gas-
Cooled F a s t R e a c t o r Development i n November 1969. T h i s Group w i l l make
recommendations a t i t s n e x t mee t ing i n Autumn 1970 a s t o t h e c o - o r d i n a t i o n
of f u t u r e work i n Europe on t h e b a s i s of deve lopments i n Member c o u n t r i e s
d u r i n g t h e f i r s t h a l f of 1970.
907
FAST BREEDER REACTORS NOT LMFBR OR GCFR - BUT FBR
Compton A . Rennie*
Systems a n a l y s i s s t u d i e s c a r r i e d o u t i n var ious coun t r i e s a l l show
t h a t t h e r e i s a c o s t i ncen t ive t o in t roduce f a s t r e a c t o r s i n t o t h e nuc lear
and f u e l cyc le c o s t s and t h e p red ic t ed performance.
i ngs and t h e t i m e a t which t h e s e f a s t r e a c t o r s a r e introduced will of
course depend on the c o s t s and performance which can a c t u a l l y be achieved.
The a c t u a l cos t sav-
It must a l s o be remembered t h a t when t h e s e fas t r e a c t o r s a r e ready t o
be introduced they w i l l have t o compete wi th t h e advanced conver te r reac-
t o r s a v a i l a b l e a t that t ime and un le s s t hey have s u f f i c i e n t l y good c o s t s
and performance t h e i r i n t roduc t ion w i l l be delayed.
t o r s must be introduced because of l i m i t a t i o n s i n uranium supp l i e s b u t i n
o r d e r t o o b t a i n t h e maximum cos t b e n e f i t , it i s necessary t o have a good
f a s t r e a c t o r a v a i l a b l e as e a r l y as poss ib l e .
Eventual ly fast reac-
These same systems a n a l y s i s s t u d i e s show t h a t w i t h t h e e s t ima tes now
a v a i l a b l e f o r c a p i t a l and f u e l cyc le c o s t s o f r e a c t o r s , which w i l l no t be
b u i l t i n quan t i ty u n t i l t h e 1980's a t t h e e a r l i e s t , i t i s not p o s s i b l e t o make a c l e a r - c u t choice between t h e sodium cooled fast r e a c t o r (LMFBR) and t h e helium cooled fast r e a c t o r (GCFR) as t h e l i m i t s o f unce r t a in ty would a l t e r t h e preference f r o m one t o the o the r .
It i s important t o have a good f a s t r e a c t o r a v a i l a b l e a t t h a t time as
t h e cos t b e n e f i t t o t h e nuc lea r power indus t ry could be seve ra l b i l l i o n d o l l a r s a t p re sen t day p r i c e s . Large ly f o r h i s t o r i c a l reasons t h e cu r ren t
emphasis i s on t h e LMFBR type and t h e r e i s a real danger t h a t no t enough
e f f o r t w i l l be put i n t o t h e GCFR type t o enable a proper comparison t o be
made so t h a t t h e customer can be i n a p o s i t i o n t o choose t h e b e t t e r type
for h i s own use. *
COMPTON A . RENNIE w a s Chief Executive of t h e OECD High Temperature Reactor P ro jec t , t h e DRAGON P ro jec t , from 1959 t o 1968, and i s now a p r i - v a t e consu l t an t . r e a c t o r work be ing c a r r i e d o u t by G u l f General Atomic i n San Diego and by t h e Gas-cooled Breeder Reactor Assoc ia t ion i n Brusse ls , and worked on s o d i m cooled f a s t r e a c t o r s i n t h e UKAEA during t h e pe r iod 1950 t o 1957.
He has r e c e n t l y been a s s o c i a t e d wi th t h e gas cooled f a s t
908
HISTORICAL BA CKGROUnlD A
Over t e n yea r s ago when f a s t r e a c t o r programmes were adopted i n France,
Germany, t h e UK, t h e US and t h e USSR, t h e r e was no t e c h n i c a l l y acceptab le
a l t e r n a t i v e t o t h e sodium cooled fas t r e a c t o r . Each of t hese coun t r i e s has
an LMFBR programme and because of t h e d e s i r e t o in t roduce fas t r e a c t o r s i n
t h e 1980's t h e r e i s a l a r g e programme i n each country, a l b e i t wi th consid-
e r a b l e d u p l i c a t i o n of e f f o r t . The dec i s ion t o embark on a new coolant
technology, sodium cool ing, was taken more than t e n yea r s ago not because
i t looked an easy t e c h n i c a l problem b u t because it seemed t o be t h e only
way t o in t roduce fas t r e a c t o r s . In f a c t some of t h e e a r l i e r p r a c t i c a l
experiences were discouraging bu t t h e work w a s pushed ahead because of t he
incen t ive , and t h e money and e f f o r t a l l o c a t e d t o it have been s t e a d i l y in-
creased as t h e t e c h n i c a l problems have proved d i f f i c u l t t o so lve .
About t e n yea r s ago two s i g n i f i c a n t developments took p l ace . One was t h e ex tens ion of work on a new r e a c t o r coolant technology, helium cooling,
which i s now being app l i ed t o t h e High Temperature Gas-cooled Reactor (HTGR),
and t h e o t h e r w a s t h e acceptance of a new p res su re v e s s e l technology, t he
p r e s t r e s s e d concre te r e a c t o r ves se l , which permi ts h igher ope ra t ing pres-
s u r e s and l i m i t s dep res su r i za t ion ra tes of t h e pr imary gas c i r c u i t as com-
pared t o l a r g e s t e e l p re s su re v e s s e l s . These two developments have now been
brought t o g e t h e r t o produce t h e HTGR programmes now under way i n Europe and
t h e USA. The f i r s t l a r g e commercial HTGR power s t a t i o n s a r e l i k e l y t o be
ordered wi th in a yea r o r so and w i l l provide it p r a c t i c a l confirmation of
helium r e a c t o r technology. There a r e a l r e a d y carbon d ioxide cooled power
r e a c t o r s w i th p r e s t r e s s e d concre te p re s su re v e s s e l s ope ra t ing i n Europe and
t h e r e w i l l soon be a helium cooled power demonstration HTGR r e a c t o r opera t -
i n g i n t h e US.
Another change which has taken p l ace dur ing t h e l a s t t e n yea r s i s a
gradual i nc rease i n t h e s i z e of power p l an t s , now about 1000 MWe and l i k e l y
t o go t o 2000 MWe u n i t s , and t h e s e l a r g e u n i t s i z e s favour t h e nuc lea r per-
formance c h a r a c t e r i s t i c s of GCFRs. The c u r r e n t GCFR programmes a r e exten-
s ions of t he HTGR r e a c t o r technology wi th a d i - f f e ren t f u e l concept. I n f a c t
t h e c u r r e n t f u e l concept f o r t h e GCFR i s based on t h e LMFBR p in type f u e l
9 09
and t h e cu r ren t designs a r e based on making t h e f u e l ope ra t ing condi t ions
as similar as poss ib le , us ing an i n d i r e c t steam cycle power p l a n t . Another
f u e l concept based on e x i s t i n g HTGR f u e l technology i s a l s o being worked on b u t t h i s coated p a r t i c l e f u e l concept i s c u r r e n t l y seen as a longe r term
and poss ib ly cheaper a l t e r n a t i v e t o t h e p i n type f u e l , w i t h t h e p o t e n t i a l
o f be ing a b l e t o be used wi th d i r e c t cyc le helium gas t u r b i n e power p l a n t s .
The use of helium cool ing i n a p r e s t r e s s e d concre te r e a c t o r v e s s e l
enables a t e c h n i c a l performance t o be achieved which i s comparable t o o r
even b e t t e r than t h a t f o r sodium r e a c t o r s wi th similar f u e l , bear ing i n
mind t h a t bo th s t u d i e s a r e s t i l l paper s t u d i e s . This equivalence w a s not
known t e n yea r s ' o r more ago and it i s an i n t e r e s t i n g specu la t ion as t o
whether t h e r e would have been so many LMFBR programmes i n ex i s t ence today
if it had been known, o r whether t h e r e might now be some LMFBR and some
GCFR programmes, o r even a l l GCFR programmes. The middle a l t e r n a t i v e would
anyway be t h e most s a t i s f a c t o r y as it i s very d e s i r a b l e t o have competi t ion
between fas t r e a c t o r types as we l l as competi t ion between d i f f e r e n t manu-
f a c t u r e r s of t h e same type .
PRESENT STATUS
There a r e c u r r e n t l y major r e sea rch and development programmes on sodium
cooled f a s t r e a c t o r s i n France, Germany, I t a l y , Japan, t h e UK, t h e US and
t h e USSR and t h e t o t a l annual expendi ture i s probably over 200 m i l l i o n d o l l a r s . T h i s expendi ture has been going on a t a smal le r l e v e l for s e v e r a l
yea r s and i s l i k e l y t o cont inue a t t h e same gene ra l l e v e l f o r t h e next t e n
yea r s . Probably about 1000 m i l l i o n d o l l a r s has been spent on sodium cooled
r e a c t o r technology and f u e l development up t o now and it i s l i k e l y that some
2000 m i l l i o n d o l l a r s w i l l have been spent over t h e next t e n yea r s .
Severa l demonstration LMFBR power p l a n t s a r e planned i n t h e 200 t o
500 MWe range t o be o p e r a t i o n a l i n t h e 1970's: one by t h e UK i n '72, one
by France i n '73, one by Germany-Benelux i n '75, one i n t h e US i n '76 and
another one i n '78, one i n Japan about '78 and two i n t h e USSR, one i n '71 and one i n '75. I n a d d i t i o n a similar number of smaller power p l a n t s o r
t e s t f a c i l i t i e s have been b u i l t o r a r e planned.
f a c t
910
There a r e GCFR programmes i n the US a i d i n Europe supported by manu-
Lrers, by u t i l i t i e s , and by government l a b o r a t o r i e b u t t n e t o t a l annual
expendi ture d i r e c t l y a t t r i b u t a b l e t o t h i s Mark i s probably l e s s than t e n
m i l l i o n d o l l a r s . This f i g u r e i s however r a t h e r misleading as the GCFR
r e l i e s heav i ly on t h e HTGR programmes f o r helium coolant technology and on
t h e LMFRR programmes f o r f u e l element technology.
how much money i s con t r ibu ted i n d i r e c t l y i n t h i s way, and it i s not r e a l l y
necessary t o spec i fy it as t h e s e programmes a l r eady e x i s t .
s ea rch and development work needed t o be a b l e t o b u i l d GCFR power demonstra-
t i o n p l a n t s has been es t imated as about 250 m i l l i o n d o l l a r s over t h e next
t e n yea r s , t h a t i s between 10 and 15 percent of t h a t planned f o r LMFIBRs.
It i s d i f f i c u l t t o say
The e x t r a re-
In t h e US, s t u d i e s on helium cooled fast , r e a c t o r s have been i n progress
f o r a number of years , mainly by GGA and a group of 42 u t i l i t i e s ( r ep resen t - ing toge the r 25% of t h e gene ra t ing capac i ty i n t h e U S ) w i th support from
t h e AEC. A proposed des ign f o r a 300 MWe GCF'R power demonstrat ion p l a n t
has been prepared and i s now be ing considered by the i n d u s t r y and u t i l i t i e s .
This scheme fol lows t h e e a r l i e r work on l a r g e r 1000 MWe power p l a n t s which
e s t a b l i s h e d t h e f e a s i b i l i t y and economic prospec ts of such p l a n t s .
I n Europe t h e r e have been va r ious n a t i o n a l s t u d i e s on gas cooled fas t
r e a c t o r s inc luding those by Belgo-Nucleaire i n Belgium, by ASM-Atom i n
Sweden, by EIR WLirenlingen i n Switzer land, by t h e AEA i n t h e UK and by
KFK Karlsruhe i n West Germany. In a d d i t i o n t h e r e i s a s tudy due f o r com-
p l e t i o n l a t e r i n 1970, sponsored by t h e West German Minis t ry for S c i e n t i f i c
Research, i n which KFA J'Lilich, KFK Karlsruhe, BBK, GHH and Siemens a r e
p a r t i c i p a t i n g , t o a s s e s s t h e p o t e n t i a l of t h e gas cooled f a s t r e a c t o r .
F i n a l l y t h e Gas-cooled Breeder Reactor Assoc ia t ion w a s se t up i n Brusse ls
i n October 1969 f o r an i n i t i a l per iod of two yea r s by eleven i n d u s t r i a l
groups, u t i l i t i e s and government o r g a n i z a t i o n j t o i n v e s t i g a t e the techni -
c a l and economic prospec ts of helium cooled f a s t r e a c t o r s w i th i n d i r e c t
steam cycle power p lan ts .*
f o r a power demonstrat ion p l a n t of around 300 W e .
This s tudy i s a l s o l i k e l y t o l e a d t o a proposal
* The members of t h e GBR Assoc ia t ion c u r r e n t l y a r e : Belgo-Nucleaire
and CEN Mol from Belgium, GAAA and SOCIA from France, Neratoom from t h e Netherlands, ASEA-Atom from Sweden, BBST from Switzer land, T N E and C E B from UK and BBK and GHH from West Germany.
911
TECHNICAL BACKGROUND
Fas t r e a c t o r s a r e a d i f f i c u l t t e c h n i c a l problem, no ma t t e r what coolant
i s used, as it i s e s s e n t i a l t o g e t a high breeding ga in and a low system
inventory of f i s s i o n m a t e r i a l t o o b t a i n an adequate doubling t ime.
sodium cooled f a s t r e a c t o r s t h e r e i s an i n e v i t a b l e l o s s of breeding gain
compared wi th t h a t f o r helium cooled f a s t r e a c t o r s because of t he neutron
moderation and abso rp t ion i n t h e sodium coolant . This can be o f f s e t by
aiming f o r a high r a t i n g and low inventory because of t h e good hea t t r a n s -
f e r p r o p e r t i e s of sodium but t h e need t o minimize t h e amount of sodium i n
t h e core means t h a t small c learances between f u e l p i n s a r e then i n e v i t a b l e ,
and t h i s complicates t h e core design because of poss ib l e coolan t r e a c t i v i t y
e f f e c t s . With sodium cool ing, because of p o s s i b l e chemical r e a c t i o n s and
induced r a d i o a c t i v i t y , it seems e s s e n t i a l t o have an in te rmedia te sodium
c i r c u i t between t h e primary sodium c i r c u i t and steam c i r c u i t . These prob-
lems have l e d t o a major e f f o r t be ing mounted on sodium technology a p a r t
from t h e major e f f o r t devoted t o r e sea rch and development on f u e l f o r t h e s e
r e a c t o r s .
In t h e
In a helium cooled r e a c t o r t h e breeding ga in i s h igher and t h e f u e l
r a t i n g i s lower than i n a sodium cooled r e a c t o r b u t t h e doubling time i s
about t h e same o r even s l i g h t l y l e s s . The small magnitude of any coolan t
r e a c t i v i t y e f f e c t s and hence t h e wider spacing allowed and needed between f u e l p ins eases t h e core design problems cons iderably . However, high abso-
lute helium p res su res a r e needed i n t h e primary c i r c u i t t o ob ta in adequate
hea t t r a n s f e r and hea t t r a n s p o r t r a t e s and t h e r e a l problem i s t o maintain
adequate helium flow rates i n t h e primary c i r c u i t a t a l l t imes inc luding p o s s i b l e dep res su r i za t ion i n c i d e n t s .
A l t h o u g h t h e above remarks on sodium cool ing and helium cool ing a r e
very b r i e f they do b r i n g out t h e fundamental d i f f e r e n c e s between the two
types of cool ing. With helium cool ing t h e e s s e n t i a l problem i s t o conta in
a high p res su re helium c i r c u i t and t o c i r c u l a t e t h e helium i n t h a t c i r c u i t
a t a l l t imes. This i s e s s e n t i a l l y an engineer ing problem which i s v i r t u a l l y
independent of t h e r eac to r , except t h a t t he r e a c t o r determines t h e combina-
t i o n of dep res su r i za t ion r a t e s and coolant flow r a t e s which i s a l lowable .
912
With sodium cool ing t h e r e i s much more i n t e r a c t i o n between t h e design of
t h e core and t h e r e s t of t h e c i r c u i t because of t h e r e a c t i v i t y e f f e c t s of
t h e sodium coolant , and t h e need t o avoid o r c o n t r o l r e a c t i v i t y t r a n s i e n t s
a r i s i n g from phase changes i n coolan t or dimensional changes i n t h e f u e l
assembly . With both coolants , f u e l needs t o be developed but , provided vented
f u e l i s used wi th helium cool ing, t h e b a s i c problems a r e e s s e n t i a l l y t h e
same and t h e ope ra t ing l i m i t s can a l s o be t h e same f o r p i n type f u e l . It
may be poss ib l e wi th helium cool ing t o use coated p a r t i c l e type f u e l which
may be cheaper t o f a b r i c a t e b u t t h i s i s a f u t u r e development and any r e a l -
i s t i c comparison made a t t h e p re sen t time between sodium and helium cool ing
must assume p i n type f u e l w i t h e s s e n t i a l l y t h e same ope ra t ing condi t ions .
It i s perhaps worth no t ing here t h a t t h e d i f f i c u l t y i s n o t t o design
a f a s t r e a c t o r , as t h i s can be done e a s i l y by d e r a t i n g t h e core s u f f i c i e n t l y ,
, b u t t o design a s a f e f a s t r e a c t o r w i t h adequzte performance and acceptab le
c o s t . The engineer ing and safety arguments s.re c l o s e l y l inked t o g e t h e r i n
each type of r e a c t o r , and it i s not p o s s i b l e t o quan t i fy i n abso lu t e terms
t h e r e l a t i v e d i f f i c u l t i e s of LMFBRs and G C F R s b u t t h e r e i s no reason t o
suppose that t h e design problems cannot be sc,lved i n e i t h e r case.
However, it would seem on t h e f ace of i t t h a t t h e GCFR problem i s more
amenable t o s o l u t i o n as it involves e s s e n t i a l l y ma t t e r s which are n o t i n t i -
mately connected wi th t h e core design and which a r e capable of proving out-
s i d e a r e a c t o r due t o t h e l a c k of p o s i t i v e r e a c t i v i t y e f f e c t s from t h e coolant
i t s e l f . The l a r g e r c l ea rances i n t h e f u e l p i n assembly i n t h e GCFR mean t h a t
i r r a d i a t i o n phenomena such as swel l ing o r bowing have l e s s e f f e c t on t h e
cool ing c a p a b i l i t y . In o t h e r words t h e GCFR problems seem t o be more s t r a i g h t -
forward engineer ing ones wi th f a r l e s s interdependence on t h e d e t a i l e d f u e l
element design than i n t h e LMFBR case, and involve a coolant technology which
i s more r e a d i l y a v a i l a b l e and needs l e s s r e sea rch and development e f f o r t .
PROPOSALS
Large commitments on sodium technology and LMFBRs were made because a t the time t h i s work s t a r t e d it seemed t h a t t h i s was t h e only rou te poss ib l e
t o in t roduce fas t r e a c t o r s . This work i s being c a r r i e d ou t a l l over t h e
913
@ world and cons iderable progress has been made i n f u e l development and
sodium technology. Helium coolant technology w a s developed f o r advanced
thermal r e a c t o r s and i s be ing app l i ed f i r s t t o t h e high temperature gas
cooled r e a c t o r . This experience w i l l be d i r e c t l y app l i cab le t o t h e GCFR
and t h e only r e a l ex tens ion needed i s t o h igher ope ra t ing p res su res . The
i n i t i a l f u e l concept f o r t h e GCFR r e l i e s almost e n t i r e l y on t h e sodium
cooled r e a c t o r work. The GCFR i s t h e r e f o r e not an e n t i r e l y new r e a c t o r
concept b u t a combination of thermal r e a c t o r helium technology and sodium
f a s t r e a c t o r f u e l technology.
A t p resent t h e r e i s undoubtedly cons iderable d u p l i c a t i o n o f e f f o r t i n
t h e s e v e r a l n a t i o n a l LMFBR programmes and i f t h e r e were some r a t i o n a l i z a -
t i o n of t h e var ious proposed n a t i o n a l programmes it would be q u i t e poss ib l e
t o save enough t o put t h e r equ i r ed r e sea rch and development e f f o r t on t h e
GCFR, some 10 t o 15% of t h e t o t a l proposed e f f o r t on f a s t r e a c t o r s . This
would make economic sense f o r everyone as it would ensure product ion of
t h e information necessary t o enable bo th systems t o be judged on t h e i r
mer i t s , r a t h e r than pre juding t h e r e s u l t by no t ob ta in ing t h e requi red
information on t h e a l t e r n a t i v e system.
I n t e r n a t i o n a l cooperat ion would seem t o be p a r t i c u l a r y appropr i a t e
f o r t h e GCFR as by h i s t o r i c a l acc iden t and by new t e c h n i c a l developments
t h i s concept a r r i v e d on t h e scene much l a t e r than t h e LMFBR bu t neverthe- l e s s on t h e basis of p re sen t s t u d i e s looks equally o r even more promising
and i s a r e a l compet i tor t o t h e LMFBR. A s t h e bulk of t h e r e sea rch and
development work f o r each concept i s t h a t needed f o r t h e f u e l and as t h i s
i s common t o each concept it i s no t as b i g a change as it looks a t f i r s t
s i g h t t o inc lude t h e GCFR i n fast r e a c t o r programmes.
A s w i th t h e LMFBR one of t h e v i t a l s t ages i s t o b u i l d one o r more
power demonstration r e a c t o r s t o e s t a b l i s h t h a t t h e p red ic t ed c o s t s are
r e a l i s t i c and t h a t t he p red ic t ed performance can be a t t a i n e d .
it i s poss ib l e t o envisage not i nc reas ing t h e number of power demonstra-
t i o n fast r e a c t o r s a l r e a d y proposed but to make one o r two of them helium
cooled r e a c t o r s i n s t ead of sodium cooled r e a c t o r s .
Here aga in
914
Because of t h e l a r g e amount of government money a l r eady inves ted i n @ seven n a t i o n a l sodium cooled f a s t r e a c t o r programmes and because of t h e
smal le r amount of money inves ted by industriy t h e r e a r e undoubtedly com-
merc ia l problems t o be reso lved t o minimize dup l i ca t ion of e f f o r t and make
money a v a i l a b l e f o r helium cooled f a s t r e a c t o r s . However, t h e r e i s a n
i ncen t ive t o do t h i s because of t h e l a r g e amounts of money involved and
because of t h e need t o o b t a i n information on competi t ive systems.
Some pre l iminary meetings were held i n P a r i s i n 1968 under t h e auspices
o f t h e European Nuclear Energy Agency (ENEA)* t o d i scuss poss ib l e i n t e r -
n a t i o n a l cooperat ion on gas cooled fas t r e a c t o r s b u t no f i r m proposals
emerged a l though a working group i s s t i l l i n ex i s t ence and meets once or
twice a yea r t o review t h e p o s i t i o n . In a d d i t i o n t h e r e a r e more f requent
meetings of s p e c i a l i s t s working i n t h i s f i e l d . There has been a d e f i n i t e change i n t h e s i t u a t i o n s i n c e 1968 and t h e helium cooled f a s t r e a c t o r now
proposed needs l e s s r e sea rch and development; work and t h i s i s mainly en-
g inee r ing as t h e b a s i c f u e l concept i? now more o r l e s s t h e same as t h a t
f o r t h e LMFBR.
Since t h e r e a r e now groups both i n Europe and t h e USA a c t i v e l y en-
gaged i n helium cooled f a s t r e a c t o r work it would seem appropr i a t e t o con-
s i d e r having f u r t h e r meetings under t h e auspices of ENFA ( i n which bo th
Japan and t h e USA a r e represented as w e l l a s t h e Ruropean c o u n t r i e s ) wi th
t h e o b j e c t of coord ina t ing the remaining r e sea rch and development work on
the GCFR and d i scuss ing t h e p o s s i b i l i t y of cons t ruc t ing one o r even two
power demonstration p l a n t s . Such d i scuss ions would need t o t ake i n t o
account t he commercial r e a l i t i e s of t h e p re sen t s i t u a t i o n b u t t h i s should
n o t c r e a t e insuperable d i f f i c u l t i e s . It would be t o everyone 's advantage
t o have a f a s t b reeder r e a c t o r programme r a t h e r than an LMFBR programme
o r a GCFR programme. -)c
E?JEA sponsored t h e success fu l OECD High Temperature Reactor P ro jec t , t h e DRAGON P ro jec t , i n which twelve European coun t r i e s p a r t i c i p a t e d . The DRAGON P r o j e c t s t a r t e d i n 1959 and i s s t i l l i n ex i s t ence , t h e t o t a l budget up t o 1910 being about 75 m i l l i o n d o l l a r s .
A
Q
915
SWARY
1.
2 .
3 .
4 .
5 .
6 .
0
There i s a need f o r f a s t r e a c t o r s i n t h e i980's provided they can
corr,pete economically w i t h t h e advanced conve r t e r r e a c t o r s a v a i l a b l e
a t that , t ime.
f a s t r e a c t o r s u n t i l l a t e r when r i s i n g uranium p r i c e s w i l l make
them competi t ive.
I f t hey cannot compete then t h e r e i s no need f o r
The major e f f o r t on f a s t r e a c t o r s a l l over t h e world i s concentrated
on sodium cooling, because a t t h e t ime most of t h e s e programmes
were s t a r t e d over t e n yea r s ago it w a s t h e t e c h n i c a l l y appropr i a t e
choice.
The development of helium cooled r e a c t o r technology f o r HTGRs and
t h e use of p r e s t r e s s e d concre te r e a c t o r v e s s e l s f o r gas cooled
r e a c t o r s means t h a t helium cooled f a s t r e a c t o r s a r e now t e c h n i c a l l y
f e a s i b l e and must be considered as competi tors t o sodium cooled f a s t
r e a c t o r s .
Assuming t h e use of t h e same b a s i c p in type f u e l f o r each type of
f a s t r eac to r , then t h e helium cooled r e a c t o r i s e s s e n t i a l l y a problem
o f t h e c o r r e c t design of t h e high p res su re primary c i r c u i t w i th l i t t l e
interdependence on t h e d e t a i l e d core design, w h i l s t t h e sodium cooled
r e a c t o r des ign depends much more on t h e d e t a i l e d design and behaviour
of the core and in t roduces a more d i f f i c u l t coolan t technology.
Because o f t h e l a r g e amount of money and e f f o r t a l r e a d y inves ted i n sodium cooled fas t r e a c t o r s it i s d i f f i c u l t t o launch a programme
f o r another type of fast r e a c t o r on a n a t i o n a l b a s i s even though t h e
e x t r a money and e f f o r t needed i s r e l a t i v e l y modest. However, t h e r e
i s a s t rong case f o r having a p a r a l l e l helium cooled f a s t r e a c t o r
programme, on an i n t e r n a t i o n a l basis i f n o t on a n a t i o n a l b a s i s .
There would then be a fast b reede r r e a c t o r programme r a t h e r t han an
LMFBR o r a GCFR programme.
There a r e a l r eady s t u d i e s on helium cooled f a s t r e a c t o r s a v a i l a b l e
i n t h e US and t h e r e a r e now s t u d i e s under way i n Europe.
s t u d i e s seem t o confirm t h a t t h e r e a r e no major f e a s i b i l i t y ques t ions
These
916
remaining, so t h a t a j o i n t e f f o r t on an i n t e r n a t i o n a l b a s i s could
be considered. Such a j o i n t e f f o r t cou.Ld l e a d t o the cons t ruc t ion
of a helium cooled power demonstrat ion r eac to r e i t h e r i n Europe o r
i n the US ( o r even two r e a c t o r s ) on a t ime s c a l e comparable t o t h a t
f o r sodium cooled power demonstrat ion p:Lants.
The money f o r such a j o i n t internationa:L programme could be found
e i t h e r as a moderate a d d i t i o n a l investment i n fast r e a c t o r technology
or by d i v e r t i n g a modest f r a c t i o n of t h e money c u r r e n t l y planned t o
be spent on sodium cooled f a s t r eac to r s . . The incen t ive f o r doing
t h i s i s t o make it more c e r t a i n t h a t t h e r e a r e competi t ive f a s t
r e a c t o r s a v a i l a b l e f o r commercial e x p l o i t a t i o n i n t h e 1980's and
t h a t t h e u t i l i t i e s can e x e r c i s e t h e i r normal opt ions of choice as t o which r e a c t o r s t hey p r e f e r t o buy.
It i s suggested t h a t discussions should t ake p l ace soon on t h e
d e s i r a b i l i t y of mounting an internatiom.i . l programme t o develop
and prove helium cooled fast r e a c t o r s SCI t h a t t hey can be compared
w i t h sodium cooled f a s t r e a c t o r s on a similar b a s i s bo th by i n d u s t r y
and by u t i l i t i e s . It i s suggested furtbermore t h a t such d i scuss ions
could we l l t ake p l ace under t h e sponsorship of t h e European Nuclear
Energy Agency, which has a l r e a d y taken some i n i t i a t i v e i n t h i s f i e l d .
7 .
8.
8 917
CLOSING REMARKS
D. B. Trauger, General Chairman, ORNL
If we compare the task of developing the Gas-Cooled Reactor concept t o that of climbing a mountain, we now perhaps have come full-around t o
the s ide where we s t a r t e d , bu t a t a higher leve l . t e red t h e helium-cooled reac tor f i e l d with a ser ious e f f o r t , they f i r s t
looked a t the reac tor c i r c u i t . The questions were: Could the c i r c u i t be designed f o r the high temperatures and f o r hot, d ry helium a t low
l e v e l s of impuri t ies? Could helium be contained? How would the equip- ment operate?
When each group en-
Early experiments were reassuring and intensive programs were mounted f o r the s a d 1 reactors - Dragon, Peach Bottom, and AVR. the reac tor projects were under way, it w a s necessary t o f u e l them adequately. The HTGR is r e a l l y successful, as Dr. MacPherson said a t
the outse t of t h i s meeting, because of the coated p a r t i c l e .
Once
Five years ago a t Brussels, coated p a r t i c l e f u e l s which would sus-
m b r i c a t i o n problems By the time of the J ' a i c h meeting i n
t a i n high temperatures and burnups were reported. and costs were foremost concerns. 1968, these problems had been solved and fas t neutron damage was just becoming i d e n t i f i e d as an important problem. It was a t h r e a t t o p a r t i c l e integrity and, m o r e importantly, to f u e l element structures, particularly
for bonding.
This week we have heard many papers and discussions on HTGR fue l . It seems safe t o say that coated p a r t i c l e f u e l and the f u e l element s t r u c t u r e s are now well i n hand. W e understand the basic performance reasonably w e l l .
be f inished, i s the task of f inding ultimate l i m i t s f o r service. includes pushing t h e technology t o reduce costs, t o develop thorium recycle methods, and t o extend it f o r d i r e c t cycle appl icat ion.
What may be confusing t o the observer and remains t o
This
Thus, f o r the HTGR, we are a t a point where small reactors have worked well, f u e l i s developed, and la rge plant designs have been pro- duced w i t h prestressed concrete pressure vessels . Fort St . Vrain con-
s t r u c t i o n experience ind ica tes t h a t the path may be correct .
918
Now, i n coming around t h e mountain, w e fo r tuna te ly have climbed t o @ t h e new l e v e l , one from which t h e v i s t a of E L f e r t i l e p l a i n f o r commercial app l i ca t ion seems t o be c l e a r l y v i s i b l e .
The road s t i l l leads upward, however, and I think w e are back t o the
point, where more e f f o r t m u s t be put on the c i r c u i t . This i s obvious f o r t he commercial designs where equipment must be highly r e l i a b l e . t h e advanced t a sks t o be achieved requi re b e t t e r mater ia l s , new devices
and equipment, perhaps even new mater ia l s . t h e way i n times past on Magnox cans and coacted p a r t i c l e s . I note t h a t
he now works on the behavior of n a t e r i a l s a t higher temperatures than
those present ly needed. i n t h e papers today.
However,
Roy Huddle helped t o point
This may bear watch.ing and has been emphasized
It has been brought out i n these four days t h a t there i s substant ia l
incent ive t o develop the d i r e c t cycle and p a r t i c u l a r l y the Gas-Cooled Fhst Etreeder. ment of long-range energy needs.
The GCBR may be v i t a l l y important t o an optimum fu l f i l l -
It a l s o points t o f u r t h e r i n t e r n a t i o n a l cooperation such as t h a t
suggested by M r . Rennie and as t h a t exhibited here t h i s week. I thrill
as g r e a t l y t o t h i s exemplification o f what ci2n be done through the coop-
e r a t i o n of people from many places as t o the progress i n Gas-Cooled Reactor technology. We m u s t do a l l t h a t i s poss ib le t o f u r t h e r both causes. There seems t o be a unique opportunity f o r us t o provide some
l i g h t i n troubled times.
Thank you one and a l l - good evening.
J
Pages 919-930 excluded
931
PARTIC I PAT ING ORGAN I ZATI ON S
BELGIUM
Centre d' Etude de 1' Energie Nucleaire (CEN)
European Atomic Energy Community (EURATOM)
Gas-Cooled Breeder Reactor Association (GCBRA)
Societe Belge Pour 1' Industrie Nucleaire, S. A. (Belgonucleaire) I 1 I
BRAZIL
Central Eletrica de Furnas S.A.,
Comissao Nacional de Energia Nuclear
(FURNAS)
(CNEN-C)
CANADA
Atomic Energy of Canada, Ltd. (AECL)
FRANCE
Commissariat a 1' Energie Atmoique (CEA)
European Nuclear Energy Agency (ENEA)
GERMANY
Arbeitsgemeinschaft Versuchsreaktor GmbH (AVR)
Brown, Boveri & Cie., AG (BBC)
Brown Boveri/Krupp Reaktorbau GmbH (BBK)
Bundesanstalt fGr MaterialprGfung (BFM)
Gesellschaft fir Kernforschung mbH (GfK)
! Gutehoffnungshstte Sterkrade AG (GHH) , I
Kernforschungsanlage JGlich GmbH (KFA)
Ke rnf orschungszen t rum Karl sruhe (KFK)
Nuklear Chemie und Metallurgie GmbH (NUKEM) 0
932
ITALY
AGIP N u c l e a i r e , S . P.A. (AGIP)
C e n t r o Commune R i c e r c h e N u c l e a r i I s p r a (CCR-ISPRA)
European A t o m i c Energy Community (EURATOM)
NETFE RLANDS
TNO-Project Team Nuc lea r E n g i n e e r i n g
SW I TZERLAN D
Brown, Bover i & C i e . (BBC)
Brown, B o v e r i - S u l z e r Turbomachinery, L td . (€ET)
E i d g e n g s s i s c h e s I n s t i t u t fiir R e a k t o r f o r s c h u n g (EIR)
S o c i e t e G e n e r a l e d e 1' I n d u s t r i e C o n s u l t i n g E n g i n e e r s (SGI) I t I 1
UNITED KINGDOM
A t o m i c Ene rgy Resea rch E s t a b l i s h m e n t - Harwe l l (UKAEA)
C e n t r a l E lec t r i c G e n e r a t i n g Board (CEGB)
OECD High Tempera ture R e a c t o r P r o j e c t (Dragon P r o j e c t )
P r i v a t e C o n s u l t a n t - Compton A . Rennie
The Nuc lea r Power Group, L td . (TNPG)
Uni t ed Kingdom A t o m i c Energy A u t h o r i t y - R e a c t o r Group ( R i s l e y )
UNITED STATES OF M R I C A
American Nuclear Soc ie ty (ANS)
Argonne National Laboratory ( ANL,)
A t l a n t i c R ich f i e ld Handford
B a t t e l l e Memorial I n s t i t u t e , P a c i f i c Northwe5,t Laboratory (BMI-PNL)
Bechtel Corporation
933
@ Black and Veatch Consulting Engineers
Brush Beryllium
Clemson University
Commonwealth Edison Company
Consumers Power Company
Ebasco Services, Inc . Eugene Water & E l e c t r i c Board
Gas Turbine Magazine
General E l e c t r i c Company (GE)
Great Lakes Carbon Corporation
Gulf General Atomic (GGA)
North Carolina S t a t e University
Northeast U t i l i t i e s Services Company
Nuclear U t i l i t y Services Corporation (NUS)
Oak Ridge National Laboratory (ORNL)
Oklahoma G a s and E l e c t r i c Company
Pac i f i c Power and Light Company
Philadelphia E l e c t r i c Company (PE)
Poco Graphite, Inc.
Power Engineering Magazine
Public Service Company of Colorado (PSC)
Public Service Company of Oklahoma
Puget Sound Power and Light Company
S. M. S t o l l e r Corporation
Tennessee Valley Authority (TVA)
Texas E l e c t r i c Service Company Union Carbide Corporation
934
Union E l e c t r i c Company
United Nuclear Corporation
United S t a t e s Atomic Energy Commission (USPJE)
United S t a t e s Department of I n t e r i o r
Universi ty of I l l i n o i s (Univ. of 111.)
Westinghouse Corporation
935
AUTHOR INDEX
Aerts, L., 547, 833
Ashworth, F. P. O . , 192, 293, 385,
Baier, J., 598, 607, 608
B a i r i o t , H . , 547, 585, 649, 671,
Barthold, W. P., 193
Bell , W. E . , 361
B u r , M., 649 . Eauer, M . , 671
B u s t , E . , 214
Bender, M. , 32, 111, 140, 288, 431
Benzler, H . , 432
Blanco, R. E. , 386, 646 Bohm, E., 231
Bohnenstingl, J., 621
Brodda, B. G . , 621
386, 752
692, 708, 833, 852, 853
Bugl, J., 473, 586, 788
Callahan, J. P., 403, 431 Carlsmith, R. S., 723, 725
Chamberlain, A. , 194
Chapman, B. G. , 3, 32, 112, 193,
Ciszewski, G. , 812
Coenegracht, O. , 621
Cohen, P., 58
Conlin, J. A., 456
782, 783
Connery, L. J., 228
Coobs, J. H. , 456, 597 c o r n , J. M., 403 Cuneo, D. R. , 864
Culler, F. L., 160
Cyhan, I t . , 791, 889
Dahlbere:, R. C . , 58, 694, 708, 709, 723
Dalle Donne, M . , 140, 179, 289, 472, (;45, 786, 852, 854, 861, 863, M39
Daub, J8 , , 726
deNordwal1, J., 384, 385, 386
Ehlers, K. , 180, 586
Eisemarui, E., 854
Ergen, I d . K., 889
Ferguson, D. E., 647 Fischer , E . , 621
Fischer , P. U.) 546, 724, 753, 784, 861
F i t t s , 11. B., 864, 878
Flowers, R. H . , 311, 359, 360, 384
Formann, E. , 384
Fortesciie, P., 781, 795 Fraas, A. P., 32, 267
Frutsch:i, H . , 812
Furber, B. N. , 113, 140, 141, 179,
Gaube, I L , 518
Ghi lardot t i , G. , 649, 671
2 50
i
Goodjohn, A. J., 195, 212, 214, 785, ’786
Goeddel, W. V., 439, 455 Graham, L* W e , 192, 472, 494, 517,
608, ‘789, 852
Grazian:i, G . , 649, 671, 726
Gutmann, H., 492, 546, 693, 726,
Hackstein, K . , 585, 586, 610, 617,
Hantke, H. J. , 34 Harder, H . , 180, 192, 193, 194
Hart , J. D . , 194, 386, 617
Haubert, P., 649, 671
Haussermann, W. F., 904 Helms, R. E. , 213
Hewette 11, D. M . , 456, 607 Hintermann, K. O . , 288
Hodzic, A . , 214
Hoinkis, E . , 58, 385
Huddle, R. A . U . , 33, 140, 268,
752, 753
618
288, 545, 617, 692, 7013, 788, 861
i n der Schmitten, W . , 598
Ivens, G., 39, 66, 67, 194, 267 Jaeger, T. A . , 112, 192, 213, 359,
Journet, J . , 726
Kaiser, G., 621
Kaplan, S. I., 89, 228, 359, 517
Kemper, J. S., 32, 58, 89
Kirchner, H. , 621
Knufer, H . , 8
Krsmer, H. , 145, 160, 194, 455,
Lane, J. A . , 767, 786
Larrimore, J. A . , 879, 889
Laser, M., 621
Liebmann, B. G., 586, 597, 617 Lindgren, J. R., 864
Litzow, W . , 621
431
617, 692, 708, 724, 780
. .-
936
Lotts , A. L., 645 Lowthian, C . S., 113
Luby, C. S * , 439 u s , L. A., 193, 229, 812, 862
Macrlabb, W. V. , 710
MacPherson, H. G. , 517
Malherbe, J., 726
Martin, W. R . , 193
Marx, K. W . , 214
Meijer, G., 89, 111, 140, 212,
Merrett , D. J . , 518, 545, 546,
Merz, E. R . , 621, 644, 645, 646 Morgan, M. T. , 361, 517
Nephew, E. A . , 34 Nei l l , F. H. , 267, 385
Norman, J. H. , 360 Oehme, H. , 161, 228, 229, 231
Pahler, R., 788
Patterson, D. , 213
Paul, S. L., 387 Pederson, J., 726
Rennie, C . A . , 853, 907
Rickard, C. L., 768, 783, 784, 785,
Riedel, H. J., 621
Rinaldini , C., 649, 671, 726
Robertson, J. A., 493, 617
Robbins, J. M., 456 Scarborough, J. C., 492, 710, 723,
Schnobrich, W. C . , 387
Schober, H. , 726
Schoning, J., 161, 179
228, 455, 853
693, 752
789, 791
725
Lockett, G. E., 111, 268, 288, 289,
Long, E. L., Jr., 864
289, 290 Schroder, E., 180 Scot t , J. L e , 456, 472, 473, 492,
607, 617
937
Senn, R. L., 456 Sisman, o., 361
Skinner , R. A., 547 Smith, E., 474, 492, 493, 546 Sozen, M. A., 387 Steward, K. P., 60, 89 Stewar t , H. B., 90, 545, 723 Stiirmer, W . , 214 Te rps t r a , J., 432
Th ie l e , D . , 621 Thompson, W. I., 795 Thomson, J. M . , 833 Thorn, J. E., 223, 2 3 , 49 Trauger, D. B., 111, 384, 431, 878,
903, 917 Turner, R. F., 617 Twardziok, W . , 214, 229, 230, 231, 250, 289, 290
Tytga t , D., 89, 212, 359, 432, 473, 607, 708, 787, 861 , 878
Vangeel , J. , 547 Vanslager, F. E., 361, 384, 385,
38 6 Vaughn, R. D . , 179, 455, 773, 783,
789, 790 Vaughen, V. C. A., 644 von d e r Decken, C. B., 251, 267,
Waage, J. M . , 879 Walger, P., 598 Walker, C . S. , 890
Weinberg, A. M . , 644 Weiskopf, H. , 231
Wellhouser, H. N . , 93, 111, 112
Weltevreden, P., 58 Wenzel, U., 621
Whitman, G. D . , 112, 402, 403 Wiemer, H. , 621
386, 472
Winkler, E. O., 439 Wirtz , K. , 455, 608, 777, 789,
Witte, H., 621
Zanan tmi , C., 649, 671 , 692, 693,
Zimmer, E . , 621
Zi tek , C. B., 517, 645, 709, 783,
Z u m w a l t , L. R. , 267, 360, 385,
790, 854, 861 , 878
72 5
784, 786, 853
644
ERRATA FOR REPORT CONF-700401 ,
The co r rec t ions l i s t e d below should be made i n t h e subjec t r e p o r t . be s u b s t i t u t e d for t h e one included i n t h e o r i g i n a l copy.
I n addi t ion , enclosed i s a rev ised au thor index t o
Page 315, Table 1, inventory of '34Caesium should be 4.4 x lo6.
Page 345, f i f t h l i n e f r o m t o p of page should read: "With only 150°C d i f f e rence between A and B . . . . . ' I