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Spin-dependent electron scattering in 2D electron systems Aitor Mugarza Catalan Institute of Nanoscience and Nanotecnology (ICN2) Barcelona, Spain Nanospain, Donostia, March 9 th 2017
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Catalan Institute of Nanoscience and Nanotecnology … · Spin-dependent electron scattering in 2D electron systems Aitor Mugarza Catalan Institute of Nanoscience and Nanotecnology

Oct 06, 2018

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Page 1: Catalan Institute of Nanoscience and Nanotecnology … · Spin-dependent electron scattering in 2D electron systems Aitor Mugarza Catalan Institute of Nanoscience and Nanotecnology

Spin-dependent electron scattering in 2D electron systemsAitor Mugarza

Catalan Institute of Nanoscience and Nanotecnology (ICN2)Barcelona, Spain

Nanospain, Donostia, March 9th 2017

Page 2: Catalan Institute of Nanoscience and Nanotecnology … · Spin-dependent electron scattering in 2D electron systems Aitor Mugarza Catalan Institute of Nanoscience and Nanotecnology
Page 3: Catalan Institute of Nanoscience and Nanotecnology … · Spin-dependent electron scattering in 2D electron systems Aitor Mugarza Catalan Institute of Nanoscience and Nanotecnology
Page 4: Catalan Institute of Nanoscience and Nanotecnology … · Spin-dependent electron scattering in 2D electron systems Aitor Mugarza Catalan Institute of Nanoscience and Nanotecnology

-k s k

Spin locked to momentum

J(x) S(x)

Charge

current Spin

density

Rashba statesTopological states

Page 5: Catalan Institute of Nanoscience and Nanotecnology … · Spin-dependent electron scattering in 2D electron systems Aitor Mugarza Catalan Institute of Nanoscience and Nanotecnology

-k s k

Spin locked to momentum

J(x) S(x)

Charge

current Spin

density

Rashba statesTopological states

Page 6: Catalan Institute of Nanoscience and Nanotecnology … · Spin-dependent electron scattering in 2D electron systems Aitor Mugarza Catalan Institute of Nanoscience and Nanotecnology

-k s k

Spin locked to momentumJ(x) S(x)

Charge

current Spin

density

Page 7: Catalan Institute of Nanoscience and Nanotecnology … · Spin-dependent electron scattering in 2D electron systems Aitor Mugarza Catalan Institute of Nanoscience and Nanotecnology
Page 8: Catalan Institute of Nanoscience and Nanotecnology … · Spin-dependent electron scattering in 2D electron systems Aitor Mugarza Catalan Institute of Nanoscience and Nanotecnology

Scattering coefficients

Quantum mirage

Quantum invisibility

Heller Nature 369, 464 (1994)

Manoharan Nature 403, 512 (2000)

Fransson Nano Lett. 10, 1600 (2010).

Page 9: Catalan Institute of Nanoscience and Nanotecnology … · Spin-dependent electron scattering in 2D electron systems Aitor Mugarza Catalan Institute of Nanoscience and Nanotecnology

Vacancy island on Ag(111)

Topo

ST

S

𝑒𝑖𝑘𝑥𝑟 𝑒−𝑖𝑘𝑥

𝑡 𝑒𝑖𝑘𝑥𝑡𝑟 𝑒𝑖𝑘𝑥

𝑡𝑟𝑟 𝑒𝑖𝑘𝑥

7

6

5

4

3

2

1

4002000

V (mV)

on flat Ag(111) terraceinside triangle

dI/

dV

(a.u

)

Page 10: Catalan Institute of Nanoscience and Nanotecnology … · Spin-dependent electron scattering in 2D electron systems Aitor Mugarza Catalan Institute of Nanoscience and Nanotecnology

Quantum interference effects in a

potential well: standing waves and

discrete energy levels

Particle in a box

A. Mugarza et al. PRL 87, 3 (2001)F. Schiller et al., NJP 16, 123025 (2014)J. E. Ortega et al. PRB 87, 115425 (2013)J. E. Ortega et al., Handbook of Surface Science(Springer, coming son!)

Monoatomic steps on Ag(111)

|Y(x)|2

0 L

EF

V

Vbarrier

N=1

N=2

N=3

x

Page 11: Catalan Institute of Nanoscience and Nanotecnology … · Spin-dependent electron scattering in 2D electron systems Aitor Mugarza Catalan Institute of Nanoscience and Nanotecnology
Page 12: Catalan Institute of Nanoscience and Nanotecnology … · Spin-dependent electron scattering in 2D electron systems Aitor Mugarza Catalan Institute of Nanoscience and Nanotecnology

12nm

500ºC

12nm

550ºC

18nm

600ºC

27nm

625ºC

12nm

450ºC

Page 13: Catalan Institute of Nanoscience and Nanotecnology … · Spin-dependent electron scattering in 2D electron systems Aitor Mugarza Catalan Institute of Nanoscience and Nanotecnology

S. J. Altenburg et al., PRL 108 (2012)

D. Subramaniam et al., PRL 108 (2012)

S. K. Hämäläinen et al., PRL 107 (2011)A. Garcia-Lekue et al., PRL 112, 066802 (2014)

Page 14: Catalan Institute of Nanoscience and Nanotecnology … · Spin-dependent electron scattering in 2D electron systems Aitor Mugarza Catalan Institute of Nanoscience and Nanotecnology

A. Garcia-Lekue et al., PRL 112, 066802 (2014)

Page 15: Catalan Institute of Nanoscience and Nanotecnology … · Spin-dependent electron scattering in 2D electron systems Aitor Mugarza Catalan Institute of Nanoscience and Nanotecnology

A. Garcia-Lekue et al., PRL 112, 066802 (2014)

Page 16: Catalan Institute of Nanoscience and Nanotecnology … · Spin-dependent electron scattering in 2D electron systems Aitor Mugarza Catalan Institute of Nanoscience and Nanotecnology

A. Garcia-Lekue et al., PRL 112, 066802 (2014)

Page 17: Catalan Institute of Nanoscience and Nanotecnology … · Spin-dependent electron scattering in 2D electron systems Aitor Mugarza Catalan Institute of Nanoscience and Nanotecnology
Page 18: Catalan Institute of Nanoscience and Nanotecnology … · Spin-dependent electron scattering in 2D electron systems Aitor Mugarza Catalan Institute of Nanoscience and Nanotecnology

G

GG

Page 19: Catalan Institute of Nanoscience and Nanotecnology … · Spin-dependent electron scattering in 2D electron systems Aitor Mugarza Catalan Institute of Nanoscience and Nanotecnology

G

Page 20: Catalan Institute of Nanoscience and Nanotecnology … · Spin-dependent electron scattering in 2D electron systems Aitor Mugarza Catalan Institute of Nanoscience and Nanotecnology

𝑠𝑝 − SS

𝑑 − SR

Page 21: Catalan Institute of Nanoscience and Nanotecnology … · Spin-dependent electron scattering in 2D electron systems Aitor Mugarza Catalan Institute of Nanoscience and Nanotecnology
Page 22: Catalan Institute of Nanoscience and Nanotecnology … · Spin-dependent electron scattering in 2D electron systems Aitor Mugarza Catalan Institute of Nanoscience and Nanotecnology

Ag(111)

Bi (1/3 ML)

BiAg2

top view

side view

Band structure

Page 23: Catalan Institute of Nanoscience and Nanotecnology … · Spin-dependent electron scattering in 2D electron systems Aitor Mugarza Catalan Institute of Nanoscience and Nanotecnology
Page 24: Catalan Institute of Nanoscience and Nanotecnology … · Spin-dependent electron scattering in 2D electron systems Aitor Mugarza Catalan Institute of Nanoscience and Nanotecnology

Only intraband transitions!

FFT q(E) vs Theory

𝑞 = 𝑘𝑖 − 𝑘𝑓

Page 25: Catalan Institute of Nanoscience and Nanotecnology … · Spin-dependent electron scattering in 2D electron systems Aitor Mugarza Catalan Institute of Nanoscience and Nanotecnology

pz px py

Δ𝐉 = Δ𝐋 +1

2Δ𝐒 = 0

𝑝𝑦, ↓ 𝐋 ⋅ 𝐒 𝑝𝑥 , ↑ ≠ 0

Page 26: Catalan Institute of Nanoscience and Nanotecnology … · Spin-dependent electron scattering in 2D electron systems Aitor Mugarza Catalan Institute of Nanoscience and Nanotecnology

Different intensity

Page 27: Catalan Institute of Nanoscience and Nanotecnology … · Spin-dependent electron scattering in 2D electron systems Aitor Mugarza Catalan Institute of Nanoscience and Nanotecnology
Page 28: Catalan Institute of Nanoscience and Nanotecnology … · Spin-dependent electron scattering in 2D electron systems Aitor Mugarza Catalan Institute of Nanoscience and Nanotecnology

L. Bürgi et al., Phys. Rev. Lett. 81, 5370 (1998).

Page 29: Catalan Institute of Nanoscience and Nanotecnology … · Spin-dependent electron scattering in 2D electron systems Aitor Mugarza Catalan Institute of Nanoscience and Nanotecnology

rl rr jl/p jr/p

A-step 0.70±0.30 0.21±0.07 -0.83±0.02 -0.95±0.02

B-step 0.40±0.18 0.36±0.15 -0.56±0.02 -0.51±0.02

strong resonator weak resonator

N=2

N=2

Page 30: Catalan Institute of Nanoscience and Nanotecnology … · Spin-dependent electron scattering in 2D electron systems Aitor Mugarza Catalan Institute of Nanoscience and Nanotecnology

The Curved Surface Approach

d

Tunable

h, e-

Sample center

[hkl]

step parallel

[h’k’l’]

miscut range

º

c-X(hkl)

Curved surfaces allows to tune and achieve atomic scale control overphysical-chemical processes related to atomic steps

Page 31: Catalan Institute of Nanoscience and Nanotecnology … · Spin-dependent electron scattering in 2D electron systems Aitor Mugarza Catalan Institute of Nanoscience and Nanotecnology

Scattering analysis framework: 1D Kronig-Penney model

d b

ytyr

yi

U0

2

*

2

01

2*

2

2

12

Em

bUtg

dmE

1D Kronig-Penney model

J. Lobo-Checa et al., unpublished

B-typeA-type

Page 32: Catalan Institute of Nanoscience and Nanotecnology … · Spin-dependent electron scattering in 2D electron systems Aitor Mugarza Catalan Institute of Nanoscience and Nanotecnology
Page 33: Catalan Institute of Nanoscience and Nanotecnology … · Spin-dependent electron scattering in 2D electron systems Aitor Mugarza Catalan Institute of Nanoscience and Nanotecnology

New scattering mechanism in spin-orbitronic materials

Controlled by chemical composition of steps

Lateral spin-filtering

Efficiency depends on edge structure