1 Closing the Carbon Cycle: Fuels from Air, Phoenix, 29/9-2016 Theis L. Skafte (1,2), P. Blennow (1), J. Hjelm (2), and C. Graves (2) Carbon formation during conversion of CO 2 to synthetic fuels by means of electrolysis (1) Haldor Topsoe A/S, Haldor Topsøes Allé 1, 2800 Kgs. Lyngby, Denmark (2) Department of Energy Conversion and Storage, Technical University of Denmark, Risø campus, Frederiksborgvej 399, 4000 Roskilde, Denmark
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Closing the Carbon Cycle: Fuels from Air, Phoenix, 29/9-2016
Theis L. Skafte (1,2), P. Blennow (1), J. Hjelm (2), and C. Graves (2)
Carbon formation during conversion of CO2 to synthetic fuels by means of electrolysis
References:[1] Graves, C., Ebbesen, S. D., & Mogensen, M., Co-electrolysis of CO2 and H2O in solid oxide cells: Performance and durability, Solid StateIonics, 192(1), 398-403, (2011).
[2] Rostrup-nielsen, J. R., 50 years in catalysis, Lessons learned, Catalysis Today, 272, 2–5, (2016).
[3] Skafte, T. L., Graves, C., Blennow, P., & Hjelm, J., Carbon Deposition during CO2 Electrolysis in Ni-Based Solid-Oxide-Cell Electrodes, ECSTransactions, 68, 3429–3437, (2015).
[4] Irvine, J. T. S., Neagu, D., Verbraeken, M. C., Chatzichristodoulou, C., Graves, C., & Mogensen, M. B., Evolution of the electrochemicalinterface in high-temperature fuel cells and electrolysers, Nature Energy, 1(1), 15014 (2016).
[5] J. R. Rostrup-Nielsen, Sulfur-passivated nickel catalysts for carbon-free steam reforming of methane, J. Catal., 85, 31–43, (1984).
[5] Skafte, T. L., Sudireddy, B. R., Blennow, P., & Graves, C., Carbon and Redox Tolerant Infiltrated Oxide Fuel-Electrodes for Solid OxideC6lls, ECS Transactions, 72(7), 201–214, (2016).
[7] Graves, C., Martinez, L., & Sudireddy, B. R., High Performance Nano-Ceria Electrodes for Solid Oxide Cells, ECS Transactions, 72(7), 183–192 (2016).
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Topsoe Stack Platform (TSP-1)75 cells combined with interconnects, spacers and sealings in one stack
• Internal fuel manifold
• External air manifold
• Cell group voltage probing
• Compression free handling (cold)
• Robustness and leak tightness QA test in SOFC mode