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Precision spectroscopy of atomic hydrogen and the proton charge radius puzzle N. Kolachevsky MPQ MPQ
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atomic hydrogen and the proton charge radius puzzlepower1.pc.uec.ac.jp/~toru/kolachevsky/notes/H-spectroscopy.pdf · atomic hydrogen and the proton charge radius puzzle N. Kolachevsky

Jun 24, 2018

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Page 1: atomic hydrogen and the proton charge radius puzzlepower1.pc.uec.ac.jp/~toru/kolachevsky/notes/H-spectroscopy.pdf · atomic hydrogen and the proton charge radius puzzle N. Kolachevsky

Precision spectroscopy of

atomic hydrogen and the proton

charge radius puzzle

N. Kolachevsky

MPQMPQ

Page 2: atomic hydrogen and the proton charge radius puzzlepower1.pc.uec.ac.jp/~toru/kolachevsky/notes/H-spectroscopy.pdf · atomic hydrogen and the proton charge radius puzzle N. Kolachevsky

Why proton charge radius is so

important?- needed for accurate Rydberg constant

determination

R

1 2S S

Page 3: atomic hydrogen and the proton charge radius puzzlepower1.pc.uec.ac.jp/~toru/kolachevsky/notes/H-spectroscopy.pdf · atomic hydrogen and the proton charge radius puzzle N. Kolachevsky

Hydrogen atomic levels

Schrödinger :Schrödinger (atomic units):

Dirac:QED:

recoil:

nuclear size correction:

Page 4: atomic hydrogen and the proton charge radius puzzlepower1.pc.uec.ac.jp/~toru/kolachevsky/notes/H-spectroscopy.pdf · atomic hydrogen and the proton charge radius puzzle N. Kolachevsky

Fundamental constants

2 , , n e pE R F m M r

Relative uncertainties:10: 3 10 10: 4 10em M

Do not contribute

(small corrections!)

2 : 1%pr Leading uncertainty!

L1Sself-energy vacuum pol. rp

total

e p 8 383 MHz -215 MHz 1.253(50) MHz 8 172 MHz

Page 5: atomic hydrogen and the proton charge radius puzzlepower1.pc.uec.ac.jp/~toru/kolachevsky/notes/H-spectroscopy.pdf · atomic hydrogen and the proton charge radius puzzle N. Kolachevsky

Method 1: Electron scattering

e p

d

d

Measured

value

Mott cross-section:

ep

Transferred momentum

Non point-like proton:

form-factor

For small q

(0) 1F impact parameter >>

proton size

Page 6: atomic hydrogen and the proton charge radius puzzlepower1.pc.uec.ac.jp/~toru/kolachevsky/notes/H-spectroscopy.pdf · atomic hydrogen and the proton charge radius puzzle N. Kolachevsky

Form-factor and charge radius

Form-factor is the Fourier transformation of the charge distribution

Mean proton charge radius

0

0 0

/( ) , 0.8 fm

r rr e r

Since proton possesses anomalous magnetic moment :

1F

2F

“Dirac” charge form-factor

“Anomalous” magnetic form-factor

(1 )

2

p

p

p

e

m

1.79p

Page 7: atomic hydrogen and the proton charge radius puzzlepower1.pc.uec.ac.jp/~toru/kolachevsky/notes/H-spectroscopy.pdf · atomic hydrogen and the proton charge radius puzzle N. Kolachevsky

Electric and magnetic form-factors

Electric Magnetic

2

2 22

2

( )6

0

p

E

r

dG q

dqQ

Derivative at q=0

Page 8: atomic hydrogen and the proton charge radius puzzlepower1.pc.uec.ac.jp/~toru/kolachevsky/notes/H-spectroscopy.pdf · atomic hydrogen and the proton charge radius puzzle N. Kolachevsky

e-p scattering results

Page 9: atomic hydrogen and the proton charge radius puzzlepower1.pc.uec.ac.jp/~toru/kolachevsky/notes/H-spectroscopy.pdf · atomic hydrogen and the proton charge radius puzzle N. Kolachevsky

Hydrogen spectroscopy

2 , , n e prE mR F MTwo unknowns

Two equations necessary!

Page 10: atomic hydrogen and the proton charge radius puzzlepower1.pc.uec.ac.jp/~toru/kolachevsky/notes/H-spectroscopy.pdf · atomic hydrogen and the proton charge radius puzzle N. Kolachevsky

Hydrogen spectroscopy: limitations

Precision spectroscopy in H:

- ALL levels except 2S promptly decay

3 3 (4 ) 10 MHzS P P

- Natural linewidth of Rydberg states reduces, but they become

sensitive to electric fields (Stark effect)

7

DCE n

Scattered electric field at the level of 1V/m is hard to control!

Page 11: atomic hydrogen and the proton charge radius puzzlepower1.pc.uec.ac.jp/~toru/kolachevsky/notes/H-spectroscopy.pdf · atomic hydrogen and the proton charge radius puzzle N. Kolachevsky

Hydrogen spectroscopy: results

Dominating uncertainty results from spectroscopy of higher excited

states (not 2S)

Page 12: atomic hydrogen and the proton charge radius puzzlepower1.pc.uec.ac.jp/~toru/kolachevsky/notes/H-spectroscopy.pdf · atomic hydrogen and the proton charge radius puzzle N. Kolachevsky

Muonic hydrogen p

p

Hydrogen Muonic

hydrogen

Bohr radius 50 pm 0.25 pm

Lyman- 121 nm

(10 eV)

2 keV

200

em m

mc

2 23 8mc

L2Sself-energy vacuum pol. rp

total

e p 1 085 MHz -27 MHz 0.14 MHz 1 057 MHz

p 0.1 THz -45 THz 0.93 THz -49 THz

Page 13: atomic hydrogen and the proton charge radius puzzlepower1.pc.uec.ac.jp/~toru/kolachevsky/notes/H-spectroscopy.pdf · atomic hydrogen and the proton charge radius puzzle N. Kolachevsky

Spectroscopy of 2S-2P transition in p

Transition line width 10 GHzGoal – uncertainty of 1 GHz

(1999)

Page 14: atomic hydrogen and the proton charge radius puzzlepower1.pc.uec.ac.jp/~toru/kolachevsky/notes/H-spectroscopy.pdf · atomic hydrogen and the proton charge radius puzzle N. Kolachevsky

Target (H2)

Page 15: atomic hydrogen and the proton charge radius puzzlepower1.pc.uec.ac.jp/~toru/kolachevsky/notes/H-spectroscopy.pdf · atomic hydrogen and the proton charge radius puzzle N. Kolachevsky

Resonance line 2S-2P in p

Page 16: atomic hydrogen and the proton charge radius puzzlepower1.pc.uec.ac.jp/~toru/kolachevsky/notes/H-spectroscopy.pdf · atomic hydrogen and the proton charge radius puzzle N. Kolachevsky
Page 17: atomic hydrogen and the proton charge radius puzzlepower1.pc.uec.ac.jp/~toru/kolachevsky/notes/H-spectroscopy.pdf · atomic hydrogen and the proton charge radius puzzle N. Kolachevsky

Where the problem resides ?!

-Errors in QED calculations are

excluded at such level of discrepancy

“New”

physics?

Page 18: atomic hydrogen and the proton charge radius puzzlepower1.pc.uec.ac.jp/~toru/kolachevsky/notes/H-spectroscopy.pdf · atomic hydrogen and the proton charge radius puzzle N. Kolachevsky

Are

- e-p scatteing experiments

- H spectroscopy results

flawless?

Page 19: atomic hydrogen and the proton charge radius puzzlepower1.pc.uec.ac.jp/~toru/kolachevsky/notes/H-spectroscopy.pdf · atomic hydrogen and the proton charge radius puzzle N. Kolachevsky

Hydrogen spectroscopy

Page 20: atomic hydrogen and the proton charge radius puzzlepower1.pc.uec.ac.jp/~toru/kolachevsky/notes/H-spectroscopy.pdf · atomic hydrogen and the proton charge radius puzzle N. Kolachevsky

Measurements of the 1S-2S transition

Page 21: atomic hydrogen and the proton charge radius puzzlepower1.pc.uec.ac.jp/~toru/kolachevsky/notes/H-spectroscopy.pdf · atomic hydrogen and the proton charge radius puzzle N. Kolachevsky

Hydrogen

Theory

Frequency comb

Mobile fountain clock

Optical fiber link

Christian Parthey

Arthur Matveev

Janis Alnis

Axel Beyer

Nikolai Kolachevsky

Randolf Pohl

Thomas Udem

Theodor Häncsh

Tobias Wilken

Birgitta Benhardt

Ulrich Jents

Brett Altschul

Michel Abgrall

Daniele Rovera

Christophe Salomon

Philippe Laurent

Katharina Predehl

Stefan Droste

Ronald Holzwarth

Harald Schnatz

Gesine Grosche

Thomas Legero

Stefan Weyers

The Team

Page 22: atomic hydrogen and the proton charge radius puzzlepower1.pc.uec.ac.jp/~toru/kolachevsky/notes/H-spectroscopy.pdf · atomic hydrogen and the proton charge radius puzzle N. Kolachevsky

Prof. T.W. Hänsch’s

group

The BossHydrogen 1S-2S

Frequency Comb & Menlo Systems

Page 23: atomic hydrogen and the proton charge radius puzzlepower1.pc.uec.ac.jp/~toru/kolachevsky/notes/H-spectroscopy.pdf · atomic hydrogen and the proton charge radius puzzle N. Kolachevsky

The team

2009-A. Beyer,

Ph.D.

J. Alnis

Post. Doc.

A. Matveev

Post. Doc.

K. Khabarova

Post. Doc.

C. Partey

Ph. D.

Th. Udem

T.W. Hänsch

me

Page 24: atomic hydrogen and the proton charge radius puzzlepower1.pc.uec.ac.jp/~toru/kolachevsky/notes/H-spectroscopy.pdf · atomic hydrogen and the proton charge radius puzzle N. Kolachevsky
Page 25: atomic hydrogen and the proton charge radius puzzlepower1.pc.uec.ac.jp/~toru/kolachevsky/notes/H-spectroscopy.pdf · atomic hydrogen and the proton charge radius puzzle N. Kolachevsky

N. Kolachevsky et al., Opt. Lett. 36, 4299 (2011)

Page 26: atomic hydrogen and the proton charge radius puzzlepower1.pc.uec.ac.jp/~toru/kolachevsky/notes/H-spectroscopy.pdf · atomic hydrogen and the proton charge radius puzzle N. Kolachevsky

1.5 cm÷ 3

Standard ECDL

25 cm

EOM

Long cavity ECDL

972 nm diode laser with a 20 cm long external resonator and intra-cavity EOM

Beat note diode - dye laser

Master oscillator

2exp rmsη φ

64

eff IRη η8-photon process =>

at 972 nm

-25 -20 -15 -10 -5 0 5 10 15 20 25

0

1000

2000

3000

Frequency detuning, kHz

Long cavity diode laser

Dye laser

Co

un

t ra

te,

co

un

ts/s

Page 27: atomic hydrogen and the proton charge radius puzzlepower1.pc.uec.ac.jp/~toru/kolachevsky/notes/H-spectroscopy.pdf · atomic hydrogen and the proton charge radius puzzle N. Kolachevsky

FP1-FP2 Allan deviation

0,01 0,1 1 10 100 1000 10000

1E-15

1E-14

1s Gate time, 5.5 Hours of measurement

10 ms Gate time, 350 s of measurement

gate time, s

Alla

n d

evia

tion

Thermal noise limit

Page 28: atomic hydrogen and the proton charge radius puzzlepower1.pc.uec.ac.jp/~toru/kolachevsky/notes/H-spectroscopy.pdf · atomic hydrogen and the proton charge radius puzzle N. Kolachevsky

Fiber

Laser

I()

Hydrogen maser

Stabilized

op

tical fiber

FP5

Distributionamplifier

Wenzel Chain 4 5 5

Wenzel Chain 4 5 5

PLL

PLL

I()

temperature stabilized

1GHz

1GHz

Comb-comb comparison setup

250 MHzsystem

100 MHzsystem

1542 nm

Page 29: atomic hydrogen and the proton charge radius puzzlepower1.pc.uec.ac.jp/~toru/kolachevsky/notes/H-spectroscopy.pdf · atomic hydrogen and the proton charge radius puzzle N. Kolachevsky

17107200/2 THzmHz

Comb-comb comparison: result

Page 30: atomic hydrogen and the proton charge radius puzzlepower1.pc.uec.ac.jp/~toru/kolachevsky/notes/H-spectroscopy.pdf · atomic hydrogen and the proton charge radius puzzle N. Kolachevsky

The Hydrogen spectrometer1S-2S spectrometer

Page 31: atomic hydrogen and the proton charge radius puzzlepower1.pc.uec.ac.jp/~toru/kolachevsky/notes/H-spectroscopy.pdf · atomic hydrogen and the proton charge radius puzzle N. Kolachevsky
Page 32: atomic hydrogen and the proton charge radius puzzlepower1.pc.uec.ac.jp/~toru/kolachevsky/notes/H-spectroscopy.pdf · atomic hydrogen and the proton charge radius puzzle N. Kolachevsky
Page 33: atomic hydrogen and the proton charge radius puzzlepower1.pc.uec.ac.jp/~toru/kolachevsky/notes/H-spectroscopy.pdf · atomic hydrogen and the proton charge radius puzzle N. Kolachevsky
Page 34: atomic hydrogen and the proton charge radius puzzlepower1.pc.uec.ac.jp/~toru/kolachevsky/notes/H-spectroscopy.pdf · atomic hydrogen and the proton charge radius puzzle N. Kolachevsky
Page 35: atomic hydrogen and the proton charge radius puzzlepower1.pc.uec.ac.jp/~toru/kolachevsky/notes/H-spectroscopy.pdf · atomic hydrogen and the proton charge radius puzzle N. Kolachevsky
Page 36: atomic hydrogen and the proton charge radius puzzlepower1.pc.uec.ac.jp/~toru/kolachevsky/notes/H-spectroscopy.pdf · atomic hydrogen and the proton charge radius puzzle N. Kolachevsky
Page 37: atomic hydrogen and the proton charge radius puzzlepower1.pc.uec.ac.jp/~toru/kolachevsky/notes/H-spectroscopy.pdf · atomic hydrogen and the proton charge radius puzzle N. Kolachevsky
Page 38: atomic hydrogen and the proton charge radius puzzlepower1.pc.uec.ac.jp/~toru/kolachevsky/notes/H-spectroscopy.pdf · atomic hydrogen and the proton charge radius puzzle N. Kolachevsky
Page 39: atomic hydrogen and the proton charge radius puzzlepower1.pc.uec.ac.jp/~toru/kolachevsky/notes/H-spectroscopy.pdf · atomic hydrogen and the proton charge radius puzzle N. Kolachevsky
Page 40: atomic hydrogen and the proton charge radius puzzlepower1.pc.uec.ac.jp/~toru/kolachevsky/notes/H-spectroscopy.pdf · atomic hydrogen and the proton charge radius puzzle N. Kolachevsky
Page 41: atomic hydrogen and the proton charge radius puzzlepower1.pc.uec.ac.jp/~toru/kolachevsky/notes/H-spectroscopy.pdf · atomic hydrogen and the proton charge radius puzzle N. Kolachevsky
Page 42: atomic hydrogen and the proton charge radius puzzlepower1.pc.uec.ac.jp/~toru/kolachevsky/notes/H-spectroscopy.pdf · atomic hydrogen and the proton charge radius puzzle N. Kolachevsky

C.G. Parthey et al., PRL 107, 203001 (2011)

Page 43: atomic hydrogen and the proton charge radius puzzlepower1.pc.uec.ac.jp/~toru/kolachevsky/notes/H-spectroscopy.pdf · atomic hydrogen and the proton charge radius puzzle N. Kolachevsky

C.G. Parthey et al., PRL 107, 203001 (2011)

Page 44: atomic hydrogen and the proton charge radius puzzlepower1.pc.uec.ac.jp/~toru/kolachevsky/notes/H-spectroscopy.pdf · atomic hydrogen and the proton charge radius puzzle N. Kolachevsky

C.G. Parthey et al., PRL 107, 203001 (2011)

Page 45: atomic hydrogen and the proton charge radius puzzlepower1.pc.uec.ac.jp/~toru/kolachevsky/notes/H-spectroscopy.pdf · atomic hydrogen and the proton charge radius puzzle N. Kolachevsky
Page 46: atomic hydrogen and the proton charge radius puzzlepower1.pc.uec.ac.jp/~toru/kolachevsky/notes/H-spectroscopy.pdf · atomic hydrogen and the proton charge radius puzzle N. Kolachevsky
Page 47: atomic hydrogen and the proton charge radius puzzlepower1.pc.uec.ac.jp/~toru/kolachevsky/notes/H-spectroscopy.pdf · atomic hydrogen and the proton charge radius puzzle N. Kolachevsky
Page 48: atomic hydrogen and the proton charge radius puzzlepower1.pc.uec.ac.jp/~toru/kolachevsky/notes/H-spectroscopy.pdf · atomic hydrogen and the proton charge radius puzzle N. Kolachevsky
Page 49: atomic hydrogen and the proton charge radius puzzlepower1.pc.uec.ac.jp/~toru/kolachevsky/notes/H-spectroscopy.pdf · atomic hydrogen and the proton charge radius puzzle N. Kolachevsky

Uncertainly in the 1S-2S transition

cannot solve the proton charge

radius puzzle

Page 50: atomic hydrogen and the proton charge radius puzzlepower1.pc.uec.ac.jp/~toru/kolachevsky/notes/H-spectroscopy.pdf · atomic hydrogen and the proton charge radius puzzle N. Kolachevsky

It is desirable to measure

independently other transitions in H

with higher accuracy

We already use a laser to excite 2S-4P

(486 nm) transition in a cold atomic

beam of H

Page 51: atomic hydrogen and the proton charge radius puzzlepower1.pc.uec.ac.jp/~toru/kolachevsky/notes/H-spectroscopy.pdf · atomic hydrogen and the proton charge radius puzzle N. Kolachevsky

2S-4P transition measurements (Yale’95)

Page 52: atomic hydrogen and the proton charge radius puzzlepower1.pc.uec.ac.jp/~toru/kolachevsky/notes/H-spectroscopy.pdf · atomic hydrogen and the proton charge radius puzzle N. Kolachevsky

2S-4P spectroscopy at MPQ

Cold beam of metastable atoms

(4 K)

Optically populated only one

hyperfine sublevel 2S (F=0)

Velocity selective detection,

typical velocities down to 100

m/s

Frequency measurement is

reliable

Page 53: atomic hydrogen and the proton charge radius puzzlepower1.pc.uec.ac.jp/~toru/kolachevsky/notes/H-spectroscopy.pdf · atomic hydrogen and the proton charge radius puzzle N. Kolachevsky

Natural line width of

the 4P level

13 MHz

Page 54: atomic hydrogen and the proton charge radius puzzlepower1.pc.uec.ac.jp/~toru/kolachevsky/notes/H-spectroscopy.pdf · atomic hydrogen and the proton charge radius puzzle N. Kolachevsky

2S-4P experimental setup

H(2S)

486 nm

Page 55: atomic hydrogen and the proton charge radius puzzlepower1.pc.uec.ac.jp/~toru/kolachevsky/notes/H-spectroscopy.pdf · atomic hydrogen and the proton charge radius puzzle N. Kolachevsky

Antiparallel BeamsActive fiber-based retroreflector:

Page 56: atomic hydrogen and the proton charge radius puzzlepower1.pc.uec.ac.jp/~toru/kolachevsky/notes/H-spectroscopy.pdf · atomic hydrogen and the proton charge radius puzzle N. Kolachevsky

Inside the chamber

Page 57: atomic hydrogen and the proton charge radius puzzlepower1.pc.uec.ac.jp/~toru/kolachevsky/notes/H-spectroscopy.pdf · atomic hydrogen and the proton charge radius puzzle N. Kolachevsky

Gaussian beam

Assembly of spherical lenses

Aspherical lens

4 mm

Page 58: atomic hydrogen and the proton charge radius puzzlepower1.pc.uec.ac.jp/~toru/kolachevsky/notes/H-spectroscopy.pdf · atomic hydrogen and the proton charge radius puzzle N. Kolachevsky

Data evaluation

Page 59: atomic hydrogen and the proton charge radius puzzlepower1.pc.uec.ac.jp/~toru/kolachevsky/notes/H-spectroscopy.pdf · atomic hydrogen and the proton charge radius puzzle N. Kolachevsky

Data scattering (polarization dependent?)

Page 60: atomic hydrogen and the proton charge radius puzzlepower1.pc.uec.ac.jp/~toru/kolachevsky/notes/H-spectroscopy.pdf · atomic hydrogen and the proton charge radius puzzle N. Kolachevsky

Cross damping: coherent and incoherent parts

incoherent

coherent

Page 61: atomic hydrogen and the proton charge radius puzzlepower1.pc.uec.ac.jp/~toru/kolachevsky/notes/H-spectroscopy.pdf · atomic hydrogen and the proton charge radius puzzle N. Kolachevsky

Cross damping problem in the 2S-4P experiment

P1/2

P3/2

Analysis of systematic

effects is

still in progress

Simple rule: if one wants to split the line by the factor

of N, the perturbing line should be further away as N

Page 62: atomic hydrogen and the proton charge radius puzzlepower1.pc.uec.ac.jp/~toru/kolachevsky/notes/H-spectroscopy.pdf · atomic hydrogen and the proton charge radius puzzle N. Kolachevsky

Thank you for attention!

MPQ