Assessing bi-directional ammonia transport using the Community Multi-Scale Air Quality (CMAQ) Model Megan L. Gore and Viney P. Aneja Department of Marine,

Assessing bi-directional ammonia transport using the Community Multi-Scale Air Quality (CMAQ) Model Megan L. Gore and Viney P. AnejaDepartment of Marine, Earth & Atmospheric SciencesNorth Carolina State UniversityRaleigh, NC, USA

Ellen J. Cooter, Robin L. Dennis, and Jonathan E. PleimU.S. Environmental Protection AgencyResearch Triangle Park, NC, USA

NC STATE UNIVERSITY8th Annual CMAS Conference, Chapel Hill, NC October 19-21, 2009

Outline NC STATE UNIVERSITYIntroduction Atmospheric Ammonia Project Overview Modeling Ammonia

Methods Data Emission Potential (gamma)

Results Emissions

Current & Future Work

Limitations

Summary & Conclusions

Atmospheric Ammonia NC STATE UNIVERSITYImpactsEcosystems: soil & water acidification, eutrophication, forest damageAtmospheric: neutralization of sulfuric and nitric acid, leading to the formation of fine particulate matter (PM2.5)TrendsNot federally regulated fertilizer sales increasing; ammonia emissions projected to increaseEnergy Independence and Security Act (EISA-RFS2)

~ 85% of total U.S. NH3 emissions are from agricultural sources ~ 35% of all agricultural NH3 emissions are from soils receiving commercial nitrogen fertilizer Source: (U.S. EPA, NEI 2002)

Project OverviewNC STATE UNIVERSITYProject DescriptionCMAQ bi-directional flux pilot study for the Eastern U.S. 2002Adjustment of current bi-directional flux module in CMAQ with the addition of a soil emission potential componentSoil emission potential calculated offline using commercial fertilizer survey dataResearch Needs AddressedDevelopment and testing of methods of providing agricultural fertilizer information into CMAQ for full CONUS implementation in 2010Clarification of possible CMAQ ammonia and overall one-atmosphere chemical budget changes with the implementation of bi-directional flux option planned for the 2011 CMAQ releaseHypothesis/ExpectationsChanges in emissions and fate for ammonia and other chemical species, particularly PM2.5, due to refinement of bi-directional flux in CMAQ

Atmospheric Ammonia Modeling NC STATE UNIVERSITYConstant Emissions InventoryUse of composite emission factors and agricultural activity to determine annual emissionsLarge uncertainty in the magnitude of emission factors; fails to account for temporal and spatial variationsProcess-Based bottom-up emission estimates; based on most detailed spatial and temporal information available about emission sources and rates limited by the quantity and spatial limitations of dataInverse-Modeled top-down emission estimates; regional and seasonal correction factors through successive model applications and comparison with observations of ambient concentration and wet depositionsusceptible to model input bias Next stepmodeling bi-directional flux

Ammonia Soil and Canopy ExchangeNC STATE UNIVERSITYSource: Cooter et al., 2009Resistance to DepositionCapacitance for re-emissionComputes emission and deposition of ammonia via a temperature dependent parameterization of canopy and soil compensation point.Canopy and underlying surfaces treated as an infinite chemical sink for atmospheric ammonia.

Methods DataNC STATE UNIVERSITYNational Nutrient Loss & Soil Carbon Database (NNLSC) crop mixes and temporal application profilesCatalog of databases and tools to aid in evaluating relationships between agricultural practices and resulting impacts on carbon, nitrogen, and phosphorus fluxes over 298 million cropland acres (79% of total U.S.)EPIC biophysical model 40-year runs based on 1997 data; outputs from 768,785 model runs are assigned a probability of occurrence based on management practices and environmental characteristicsModel inputs: nutrient management data from Cropping Practice Survey (CPS) and Area Studies (USDA-ERS), crop and management data from 1997 National Resource Inventory (NRI), soil data from Map Unit Interpretation Record, monthly climate statisticsCrops included: corn, soybeans, wheat, cotton, barley, sorghum, rice, potatoes, oats, peanuts, legume hay, and grass hay2002 Census of Agriculture total crop acres by countyMCIP meteorology for the standard 12km Eastern CMAQ domain

EPIC Fertilizer Application and Emissions NC STATE UNIVERSITY40-year average of annual commercial fertilizer application rates for nitrogen in model simulations40-year average of annual per-acre nitrogen lost to the atmosphereSource: NNLSC, 2006

Methods Crop Mixes & Temporal ProfilesNC STATE UNIVERSITYIdentify sub-regions with relatively distinct crop mixes accounting for the majority of the fertilizer use by the magnitude of N application in each U.S. region (e.g. Southern Great Plains).Compute a median annual N application rate for each crop in the sub-region.Compute state temporal application profiles by determining the probability of an acre in that sub-region receiving a particular fertilizer application treatment (10 options, e.g. Fall, Spring and At Plant, etc.). If 1 application, application = median annual N rate; if 2 applications, assume 85/15 split.Multiply time series of daily gammas by the fraction of sub-region acres in a state. Sum across all states in sub-region. The result is a single time series for each crop in the sub-region.Multiply each weighted crop time series (# 4) by the fraction of total acres of that crop in the sub-region. Sum across all crops in sub-region. The result is a single time series of gammas for the sub-region.

Methods Calculating Emission PotentialNC STATE UNIVERSITYDimensionless Emission Potential (g)Majority of [NH4+] contributing to the soil emission potential is from Biological Nitrogen Fixation (BNF) and the application of commercial fertilizers[H+] is managed on an annual basis, but also varies on shorter time scales as a result of nitrification processesg calculated via a box model constructed from EPIC algorithms representing the nitrification processBox model inputs: physical properties of the ambient soil profile, meteorology, and crop management practices[NH4+] is the ammonium ion concentration in the soil[H+] is the hydrogen ion concentration in the soil

Results Gamma Weighting Example NC STATE UNIVERSITYCrop Mixes - Southern Great PlainsRepresentative MCIP Weather Locations

Results Gamma Weighting Example NC STATE UNIVERSITYEmission Potential, g (dimensionless) for dryland cotton. Variable meteorology across the sub-region is represented by 2 MCIP grid cells (46=solid, 50=dashed). All cotton acres in sub-region B are assumed to receive 31.5 kg/ha annual N fertilizer application. Application schedule is defined as: 0001=1 application on January 1, 1000=1 application 30 days prior to planting, 0010=1 application 30 days after planting and 0011=2 applications assumed to be 15% of annual on January 1 and 85% of annual 30 days after planting.

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Julian Date

Emission Potential (gamma)

Sub-Region B Emission Potential for Dryland Cotton

Region A 07 soil test

doy001_0100007_0100037_0100054_0100057_0100103_0100134_0100164_0100JP3_0100mnn_0100001_0101007_0101037_0101054_0101057_0101103_0101134_0101164_0101JP3_0101mnn_0101001_1000007_1000037_1000054_1000057_1000103_1000134_1000164_1000JP3_1000mnn_1000001_1100007_1100037_1100054_1100057_1100103_1100134_1100164_1100JP3_1100mnn_1100

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20.00E+000.00E+000.00E+000.00E+000.00E+000.00E+000.00E+000.00E+000.00E+000.00E+001.02E+051.02E+051.02E+051.02E+051.02E+051.02E+051.02E+051.02E+051.02E+051.02E+050.00E+000.00E+000.00E+000.00E+000.00E+000.00E+000.00E+000.00E+000.00E+000.00E+000.00E+000.00E+000.00E+000.00E+000.00E+000.00E+000.00E+000.00E+000.00E+000.00E+00

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1944.82E+045.48E+045.26E+045.24E+044.89E+044.81E+045.19E+045.45E+045.16E+045.16E+042.17E+042.50E+042.39E+042.38E+042.21E+042.17E+042.36E+042.49E+042.34E+042.34E+041.39E+041.61E+041.54E+041.53E+041.42E+041.39E+041.51E+041.60E+041.50E+041.50E+043.50E+044.00E+043.84E+043.82E+043.55E+043.50E+043.78E+043.98E+043.76E+043.76E+04

1955.33E+046.07E+045.83E+045.81E+045.41E+045.33E+045.75E+046.04E+045.71E+045.71E+042.40E+042.77E+042.65E+042.64E+042.45E+042.40E+042.61E+042.77E+042.59E+042.59E+041.55E+041.78E+041.71E+041.70E+041.57E+041.54E+041.68E+041.78E+041.67E+041.67E+043.88E+044.43E+044.25E+044.24E+043.94E+043.87E+044.19E+044.41E+044.16E+044.16E+04

1965.61E+046.39E+046.14E+046.11E+045.69E+045.61E+046.05E+046.36E+046.01E+046.01E+042.53E+042.92E+042.79E+042.78E+042.58E+042.53E+042.75E+042.91E+042.73E+042.73E+041.63E+041.88E+041.80E+041.79E+041.66E+041.63E+041.77E+041.87E+041.76E+041.76E+044.08E+044.67E+044.48E+044.46E+044.15E+044.08E+044.41E+044.65E+044.38E+044.38E+04

1974.43E+045.04E+044.84E+044.83E+044.49E+044.43E+044.78E+045.02E+044.74E+044.74E+042.00E+042.31E+042.21E+042.20E+042.04E+042.00E+042.18E+042.30E+042.16E+042.16E+041.29E+041.49E+041.42E+041.42E+041.31E+041.29E+041.40E+041.48E+041.39E+041.39E+043.22E+043.69E+043.54E+043.53E+043.27E+043.22E+043.49E+043.67E+043.46E+043.46E+04

1984.27E+044.86E+044.67E+044.65E+044.33E+044.26E+044.60E+044.84E+044.57E+044.57E+041.93E+042.23E+042.13E+042.12E+041.97E+041.93E+042.10E+042.22E+042.08E+042.08E+041.24E+041.44E+041.37E+041.37E+041.26E+041.24E+041.35E+041.43E+041.34E+041.34E+043.11E+043.56E+043.41E+043.40E+043.16E+043.11E+043.36E+043.54E+043.34E+043.34E+04

1993.88E+044.43E+044.25E+044.23E+043.94E+043.88E+044.19E+044.41E+044.16E+044.16E+041.76E+042.03E+041.94E+041.93E+041.79E+041.76E+041.91E+042.03E+041.90E+041.90E+041.13E+041.31E+041.25E+041.25E+041.15E+041.13E+041.23E+041.31E+041.22E+041.22E+042.83E+043.24E+043.11E+043.10E+042.87E+042.83E+043.06E+043.23E+043.04E+043.04E+04

2003.46E+043.95E+043.79E+043.77E+043.51E+043.46E+043.73E+043.93E+043.71E+043.71E+041.57E+041.81E+041.73E+041.72E+041.60E+041.57E+041.71E+041.81E+041.69E+041.69E+041.01E+041.17E+041.12E+041.11E+041.03E+041.01E+041.10E+041.16E+041.09E+041.09E+042.52E+042.89E+042.77E+042.76E+042.56E+042.52E+042.73E+042.88E+042.71E+042.71E+04

2013.94E+044.49E+044.31E+044.30E+044.00E+043.93E+044.25E+044.47E+044.22E+044.22E+041.79E+042.06E+041.97E+041.96E+041.82E+041.79E+041.95E+042.06E+041.93E+041.93E+041.15E+041.33E+041.27E+041.27E+041.17E+041.15E+041.25E+041.33E+041.25E+041.25E+042.87E+043.29E+043.16E+043.14E+042.92E+042.87E+043.11E+043.28E+043.09E+043.09E+04

2024.53E+045.17E+044.96E+044.95E+044.60E+044.53E+044.89E+045.15E+044.86E+044.86E+042.06E+042.38E+042.27E+042.26E+042.10E+042.06E+042.24E+042.38E+042.22E+042.22E+041.33E+041.54E+041.47E+041.46E+041.35E+041.33E+041.45E+041.53E+041.44E+041.44E+043.31E+043.79E+043.64E+043.62E+043.36E+043.31E+043.58E+043.78E+043.56E+043.56E+04

2034.17E+044.76E+044.57E+044.55E+044.23E+044.16E+044.50E+044.74E+044.47E+044.47E+041.90E+042.19E+042.09E+042.08E+041.93E+041.90E+042.07E+042.19E+042.05E+042.05E+041.23E+041.42E+041.35E+041.35E+041.25E+041.22E+041.33E+041.41E+041.32E+041.32E+043.04E+043.49E+043.35E+043.33E+043.09E+043.04E+043.30E+043.48E+043.27E+043.27E+04

2043.44E+043.93E+043.77E+043.76E+043.49E+043.44E+043.71E+043.91E+043.69E+043.69E+041.57E+041.81E+041.73E+041.72E+041.60E+041.57E+041.71E+041.81E+041.69E+041.69E+041.01E+041.17E+041.12E+041.11E+041.03E+041.01E+041.10E+041.17E+041.09E+041.09E+042.51E+042.88E+