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14th Int. Conf. on Nuclear Reactions Mechanisms, June 15-19, 2015, Varenna, Italy Marilena Avrigeanu 1 Role of the direct mechanisms in the Role of the direct mechanisms in the deuteron-induced surrogate deuteron-induced surrogate reactions reactions Marilena Avrigeanu and Vlad Avrigeanu Marilena Avrigeanu and Vlad Avrigeanu Horia Hulubei National Institute for Physics and Nuclear Engineering (IFIN-HH), Horia Hulubei National Institute for Physics and Nuclear Engineering (IFIN-HH), Bucharest, Romania Bucharest, Romania 14th INTERNATIONAL CONFERENCE ON NUCLEAR REACTION MECHANISMS June 15-19, 2015, Varenna, Italy F4E-GRT-168.02, Tasks 5.1/8.2 PN-II-ID-PCE-3-2011-0450 Content Content 1. Introduction 1. Introduction 2 2 . Surrogate Reaction Approximations . Surrogate Reaction Approximations 3. Deuteron 3. Deuteron BU effects BU effects 4. Conclusions 4. Conclusions
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14th Int. Conf. on Nuclear Reactions Mechanisms, June 15-19, 2015, Varenna, ItalyMarilena Avrigeanu 1 Role of the direct mechanisms in the deuteron-induced.

Dec 31, 2015

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Page 1: 14th Int. Conf. on Nuclear Reactions Mechanisms, June 15-19, 2015, Varenna, ItalyMarilena Avrigeanu 1 Role of the direct mechanisms in the deuteron-induced.

14th Int. Conf. on Nuclear Reactions Mechanisms, June 15-19, 2015, Varenna, ItalyMarilena Avrigeanu 1

Role of the direct mechanisms in theRole of the direct mechanisms in thedeuteron-induced surrogate reactionsdeuteron-induced surrogate reactions

Marilena Avrigeanu and Vlad AvrigeanuMarilena Avrigeanu and Vlad Avrigeanu Horia Hulubei National Institute for Physics and Nuclear Engineering (IFIN-HH), Horia Hulubei National Institute for Physics and Nuclear Engineering (IFIN-HH),

Bucharest, RomaniaBucharest, Romania

14th INTERNATIONAL CONFERENCE ON NUCLEAR REACTION MECHANISMS

June 15-19, 2015, Varenna, Italy

F4E-GRT-168.02, Tasks 5.1/8.2PN-II-ID-PCE-3-2011-0450

ContentContent

1. Introduction1. Introduction

22. Surrogate Reaction Approximations. Surrogate Reaction Approximations

3. Deuteron 3. Deuteron BU effects BU effects

4. Conclusions4. Conclusions

Page 2: 14th Int. Conf. on Nuclear Reactions Mechanisms, June 15-19, 2015, Varenna, ItalyMarilena Avrigeanu 1 Role of the direct mechanisms in the deuteron-induced.

14th Int. Conf. on Nuclear Reactions Mechanisms, June 15-19, 2015, Varenna, ItalyMarilena Avrigeanu 2

DEUTERON Surrogate ReactionsDEUTERON Surrogate Reactions

2Marilena Avrigeanu

Page 3: 14th Int. Conf. on Nuclear Reactions Mechanisms, June 15-19, 2015, Varenna, ItalyMarilena Avrigeanu 1 Role of the direct mechanisms in the deuteron-induced.

14th Int. Conf. on Nuclear Reactions Mechanisms, June 15-19, 2015, Varenna, ItalyMarilena Avrigeanu 3

Breakup deuteron effects :Breakup deuteron effects : 231231Pa(d,3n)Pa(d,3n)230230UU reaction reaction

10 12 14 16 18 2010-1

100

101

102

103

(

mb)

Ed (MeV)

231Pa(d,3n)230U Morgenstern+ (2009) PE+CN

6 9 12 15 18 21100

101

102

103

R

BU

(Avrigeanu+, 2009)

(

mb)

Ed (MeV)

d + 231

91Pa

BREAKUP channel

10 12 14 16 18 2010-1

100

101

102

(m

b)

Ed (MeV)

231Pa(d,3n)230U

Morgenstern+ (2009) PE+CN UNCORRECTED for BU

(PE + CN)*(1-BU/R)

BF (231Pa(pbreakup,2n)230U) BF+PE+CN

Page 4: 14th Int. Conf. on Nuclear Reactions Mechanisms, June 15-19, 2015, Varenna, ItalyMarilena Avrigeanu 1 Role of the direct mechanisms in the deuteron-induced.

14th Int. Conf. on Nuclear Reactions Mechanisms, June 15-19, 2015, Varenna, ItalyMarilena Avrigeanu 4

SURROGATE REACTIONS: SURROGATE REACTIONS: STRONG EFFECTS OF THE DEUTERON BREAKUPSTRONG EFFECTS OF THE DEUTERON BREAKUP

test of d-surrogate

232Th(d,p)

Page 5: 14th Int. Conf. on Nuclear Reactions Mechanisms, June 15-19, 2015, Varenna, ItalyMarilena Avrigeanu 1 Role of the direct mechanisms in the deuteron-induced.

14th Int. Conf. on Nuclear Reactions Mechanisms, June 15-19, 2015, Varenna, ItalyMarilena Avrigeanu 5

SURROGATE REACTIONS: SURROGATE REACTIONS: STRONG EFFECTS OF THE DEUTERON BREAKUP STRONG EFFECTS OF THE DEUTERON BREAKUP

5

desired reaction: 232Th(n,ɤ)233Th surrogate reaction: 232Th(d,pɤ)233Th

Eex : [4.786 - 5.782] MeVEp : [9.672 - 8.676] MeV; θp :[ 124o -138o]

inelastic breakup enhancement

232Th(nBU,ɤ)233Th

Ed=12 MeV; = 14.458 MeV

10 12 14

102

103

Ed (MeV)

m

b

d + 232

90Th

Reaction - Han (2006)

BU - Avrigeanu+ (2009)

R

232Th(d,p)

20 40 60 800.1

0.2

0.3

0.4

0.50.60.70.8

Ed (MeV)

p B

U/

R

proton breakup ratio: d +232Th

Kleinfeller+ (1981) Wu+ (1979) Avrigeanu+ (2009))

Page 6: 14th Int. Conf. on Nuclear Reactions Mechanisms, June 15-19, 2015, Varenna, ItalyMarilena Avrigeanu 1 Role of the direct mechanisms in the deuteron-induced.

14th Int. Conf. on Nuclear Reactions Mechanisms, June 15-19, 2015, Varenna, ItalyMarilena Avrigeanu 6

SURROGATE REACTIONS: SURROGATE REACTIONS: STRONG EFFECTS OF THE DEUTERON BREAKUP STRONG EFFECTS OF THE DEUTERON BREAKUP

desired reaction: 232Th(n,ɤ)233Th surrogate reaction: 232Th(d,pɤ)233Th

E* : [4.786 - 5.782] MeVEp : [9.672 - 8.676] MeV; θp :[ 124o -138o]

233Th*: BU inelastic enh.BU inelastic enh. 232Th(nbreakup,ɤ) DRDR (strippingstripping) 232Th(d,p) CNCN 232Th(d,p)

NOT CONSIDERED : LARGENOT CONSIDERED : LARGE leakage of leakage of d fluxd flux flux through flux through BU BU beforebefore CN CN fformormaationtion

CN mechanismCN mechanism,, too restrictive frame for d-surrogated-surrogate

EXCEPTEXCEPT the SSurrogate RRatio Method, where the effects of BUBU & DR& DR are diminished

Page 7: 14th Int. Conf. on Nuclear Reactions Mechanisms, June 15-19, 2015, Varenna, ItalyMarilena Avrigeanu 1 Role of the direct mechanisms in the deuteron-induced.

14th Int. Conf. on Nuclear Reactions Mechanisms, June 15-19, 2015, Varenna, ItalyMarilena Avrigeanu 7

BreakupBreakup Cross Sections Parametrizations Cross Sections ParametrizationsKalbach (2003)Kalbach (2003)

Kalbach (2010)Kalbach (2010)

Avrigeanu+ (2009)Avrigeanu+ (2009)

0.2

0.4

0.6

58Ni Kalbach (2003) Avrigeanu+ (2009) Kalbach (2010)

0.2

0.4

0.6

119Sn

20 40 60 80

0.2

0.4

0.6

Ed (MeV)

181Ta

20 40 60 80

0.2

0.4

0.6

Ed (MeV)

232Th

cadru 9

0.2

0.4

0.6

90Zr

0.1

0.2

0.3

0.4

p B

U/ R

eact

ion

27Al

Pampus+ (1978) Wu+ (1979) Matsuoka+ (1980) Kleinfeller+ (1981)

0.2

0.4

0.6

93Nb

0.2

0.4

0.6

62Ni

BUP_comp_new

20 40 60 80

0.2

0.4

0.6

Ed (MeV)

208Pb

Fusion. Eng. Design, 84, 418 (2009)

Phys. Rev. C 89, 0446613 (2014)

www.tunl.duke.edu/publications/tunlprogress/2003/

www-nds.iaea.org/fendl3/vardocs.html.

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14th Int. Conf. on Nuclear Reactions Mechanisms, June 15-19, 2015, Varenna, ItalyMarilena Avrigeanu 8

Importance of Deuteron Breakup mechanismImportance of Deuteron Breakup mechanism

5 10 15 20

10

100

1000

5 10 15 20

10

100

1000

d + 231

91Pa

R

BU (Avrigeanu+, 2009)

BU (Kalbach, 2003)

(

mb)

d + 27

13Al

5 10 15 20

Ed (MeV)

d + 181

79Ta

d + 63

29Cu

d + 119

50Sn

d + 93

41Nb

Warning for d-surrogates

Warning for d-surrogates

BU-Dominance !!!

BU-Dominance !!!

Page 9: 14th Int. Conf. on Nuclear Reactions Mechanisms, June 15-19, 2015, Varenna, ItalyMarilena Avrigeanu 1 Role of the direct mechanisms in the deuteron-induced.

14th Int. Conf. on Nuclear Reactions Mechanisms, June 15-19, 2015, Varenna, ItalyMarilena Avrigeanu 9

232Th(d,p)233Th STRIPPING REACTIONS: 232Th(d,p)233Th STRIPPING REACTIONS: IMPORTANT CONTRIBUTIONIMPORTANT CONTRIBUTION

Page 10: 14th Int. Conf. on Nuclear Reactions Mechanisms, June 15-19, 2015, Varenna, ItalyMarilena Avrigeanu 1 Role of the direct mechanisms in the deuteron-induced.

14th Int. Conf. on Nuclear Reactions Mechanisms, June 15-19, 2015, Varenna, ItalyMarilena Avrigeanu 10

CONCLUSIONSCONCLUSIONS

PE & EVAPORATIONPE & EVAPORATION cross sections corrected for

initial flux leakage towards DIRECT INTERACTIONSDIRECT INTERACTIONS

DIRECT INTERACTIONSDIRECT INTERACTIONS (DI) effects to dd interactions

BREAKUPBREAKUP: DOMINANTDOMINANT for heavy targets at Ed~VC

BREAKUP ENHANCEMENTBREAKUP ENHANCEMENT of activation c.s. STRIPPING & PICK-UPSTRIPPING & PICK-UP maxima Ed~ 8-10 MeV

Nuclear Reactions studies based on Nuclear Reactions studies based on

deuteron induced reactions deuteron induced reactions should consider should consider

BREAKUP & STRIPPING / PICK-UP EFFECTSBREAKUP & STRIPPING / PICK-UP EFFECTS

Thank you!Thank you!

DEUTERON SURROGATE DEUTERON SURROGATE RATIORATIO METHOD METHOD IS THE SOLUTION

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14th Int. Conf. on Nuclear Reactions Mechanisms, June 15-19, 2015, Varenna, ItalyMarilena Avrigeanu 1111Marilena AvrigeanuMarilena Avrigeanu

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14th Int. Conf. on Nuclear Reactions Mechanisms, June 15-19, 2015, Varenna, ITALY

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14th Int. Conf. on Nuclear Reactions Mechanisms, June 15-19, 2015, Varenna, ItalyMarilena Avrigeanu 1212Marilena AvrigeanuMarilena Avrigeanu

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14th Int. Conf. on Nuclear Reactions Mechanisms, June 15-19, 2015, Varenna, ITALY

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14th Int. Conf. on Nuclear Reactions Mechanisms, June 15-19, 2015, Varenna, ItalyMarilena Avrigeanu 13

d

Surrogate reactions methodSurrogate reactions method

δ = d + D

CNCNExcited nucleusExcited nucleus

CNCN

= a + A

= c + C

DR:DR:

n

pBU+DR+CNBU+DR+CN

IF:

EXCEPT: 1=2, CN1≠ CN2 (ESR)1=2, CN1= CN2, 1 ≠ 2 (ISR)

= c + C