Aerosols Chemistry Clouds and Radiation
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8/16/2019 Aerosols Chemistry Clouds and Radiation
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Frontiers in Climate and Earth System Modeling: Advancing the Science
May 20, 2013
Geophysical Fluid Dynamics Laboratory
Speakers: Yi Ming and Chris Golaz
Moderator: Leo Donner
Using Models and Observations to
Understand
Climate Processes: Aerosols,
Chemistry, Clouds and Radiation
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•
Key to reducing model biases and uncertainties; Affirmed by the 2012 National Research Council
(NRC) Report on Advancing Climate Modeling and the
2010 NOAA Next-generation Strategic Plan (NGSP).
•
Relevant to NOAA’s climate adaptation andmitigation goal;
• Striving for a healthy balance between resolution and
complexity;
•
New opportunities created by “marrying” more
advanced physics and chemistry with finer spatial
resolutions.
8/16/2019 Aerosols Chemistry Clouds and Radiation
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Overarching theme: Understanding the complexroles of short-lived species and clouds in
influencing climate and air quality.
1. Atmospheric Composition
• High resolution modeling of aerosol emissions and transport
[Paul Ginoux];
• Influence of inter-continental transport and stratospheric
intrusion on the western U.S. air quality [Meiyun Lin]
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2. Radiation and climate forcing• Parameterization of water vapor continuum [David Paynter];
• Validation of modeled surface radiative flux [Stuart
Freidenreich];
•
Surface radiative flux trends (global dimming) [Geeta Persad];• Active participation in the Atmospheric Chemistry and Climate
Model Intercomparsion Project (ACCMIP) [Vaishali Naik and
Larry Horowitz];
3. Climate response• Aerosol effects on South Asian monsoon [Massimo Bollasina];
• Non-local aerosol effects on the Atlantic Meridional Overturning
Circulation (AMOC) [Dan Schwarzkopf];
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4. Cloud Processes• Large-scale clouds and aerosol-cloud interactions [Chris
Golaz];
• Deep cumulus and satellite/process-level observations [Leo
Donner];
• Shallow cumulus and climate sensitivity [Ming Zhao].
Outline of this talk
1. Yi Ming: overview, and the first three research fields(atmospheric composition, radiation and climate response);
2. Chris Golaz: cloud processes, and future research directions.
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0E=H=?=A"F >G:A IFG@?: "=> F"=> G:?
Accidents US I-60 near
Tulsa (Oct 19, 2012)
Credit: P. Ginoux
Dust Optical Depth and emission from
agriculture (Oct 18, 2012)
Nudged 50-km AM3 with land use dust sources (Ginoux et al., 2012)
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Sunphotometer @ CRT
Emission (mg/m2/day) by land use type
A O D ( 5 5 0
n m
)
date
ObsModel
0
20
40
60
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Southern California (May 23)
GFDL AM3
1 2 0
Lidar (CalNex)
O 3 S
M o
d e l 8 - h r S u r f a c e
O 3
( p p b )
Observed 8-hr Surface O3 (ppb)
Air qualitystandard
Stratospheric O3
(~50%)
A l t i t u d e ( k m
a . s . l .
)
Flight Track
O3 [ppb]
Lin et al. (2012) Credit: M. Lin
Apr. 12-16
Total O3 (100%)
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.GBP"<? :9EBAN"R? B">;"HR? K..,L MGS AB?=>
Credit: G. Persad
Global Energy
Balance Archive
(GEBA) stations
used in Norris
and Wild (2009)
The GFDL AM3/CM3 model has the best representation of the
dimming trends among all CMIP5 model (Allen et al., 2012).
Obs.
AM2.1
AM3
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.GBP"<? :9EBAN"R? B">;"HR? MGS K..,L AB?=> K%L
C l e a
r - s k y s u r f a c e
s o
l a r r a
d i a t i o n
( W / m 2 ) Surface:
-12 W/m2
AM3
Ext.
Int. Mixing More Less Aerosol
+More absorption
More dimming
Less absorption
Less dimming
AM2.1 AM3
A b s or p t i on ( W
/ m2 )
-10
-6
-2
2
6
10
Absorption:8 W/m2
TOA
Surface
Cooling
Atmosphere
Warming
Similartrends
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Linear trends ofaverage JJAS rainfall
over central-northern
Indian (mm day-1)GG
All forcing
CRUAERO
Credit: M. Bollasina
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Climatology GG
All forcingAERO
ALL_FAERO
WMGGO3Climatology
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*?BE:EF ;@I"<A E= @E=:EE= E=:?A
CRU
Obs.
May June
•
Aerosols tend to
increase rainfall
in May and June,
whilesuppressing it in
JAS;
•
An earlier
monsoon onset;
•
Consistent withobservations.
JAS (July-Aug-Sep)
AERO
Linear trends of precipitation [mm day-1 50 yr -1]
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*?BE:EF ;@I"<A E= @E=:EE= E=:?A K%L
warm &moist air
warm &moist air
May
June
Aerosols
Higher
SLP
LowerSLP
Surface
wind
Precipitation
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Sensitivity and forcing are key
climate properties. At
equilibrium:
!" " # $
$ "#$%&'()$* forcing: radiative"#$%&'()$* forcing: radiative
perturbation (GHGs, aerosols,clouds, land-use,!)
# sensitivity: temperaturesensitivity: temperature
response per unit of forcing.
! Clouds impact both.
Forster et al. (2013); Kiehl (2007).
Anti-correlation between sensitivity
and forcing among models that
reproduce observed warming.
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Zhao (2013 , J. Climate, submitted)
Red: tropical average
Blue: global average
Credit: M. Zhao
"
Increased climate sensitivityin HiRAM (and AM3)
compared to AM2.
" Sensitivity highly correlated
with cloud feedback (change
in cloud radiative effect).
Cloud feedback
! impacted by details of
convective parameterization,
! linked to convective
precipitation efficiency.
S e n
s i t i v i t y
Cloud feedback parameter AM2
0 c48 HiRAM
1-4 perturbed cumulus mixing
5-8 perturbed cumulus microphysics
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ModelsCM3: official GFDL CMIP5
model.
CM3w,c: configurations
with alternate but plausible
parameter choices.
NOAA NCDC 0.59 ºC
NASA GISS 0.53 ºC
HadCRUT3 0.56 ºC
CM3w 0.57 ºC
CM3 0.22 ºC
CM3c -0.01 ºC
Net warming
Golaz et al. (2013, GRL)Credit: C. Golaz
Observations
Models
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Evaluation of CFMIP1 and CFMIP2 modelsKlein et al. (2013, JGR)
g2: AM2(GAMDT, 2004,
J. Climate)
G3: AM3(Donner et al.,
2011, J. Climate)
AM3/CM3 results are being widely analyzed (53 citations to date).GFDL CFMIP credit: L. Donner, C. Seman, L. Horowitz, B. Hurlin
Shortwave relevant cloud properties Longwave relevant cloud properties
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• Long-standing stratocumulus biases
are reduced in AM3-CLUBB.
• Overall performance slightly lags AM3.
Credit: H. Guo
CLUBB* (NOAA/NSF Climate Process Team)Short-wave cloud forcing error [W m-2]
S t r a t o c u m u l u s b i a s e s
*Cloud Layers Unified by Bi-Normals
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! Full liquid water path response to aerosols could
potentially decrease magnitude of indirect effect.
Droplet concentration (cm-3)
CLUBB
Guo et al. (GRL, 2011)
L i q u i d w a t e r p a t h
( g m -
2 )
Credit: H. Guo
CLUBB* (NOAA/NSF Climate Process Team)Indirect effect for different stratocumulus cases
Droplet concentration (cm-3) L i q u i d w a t e r p a t h
( g m -
2 )
Ackerman et al. (Nature, 2004)
Large eddy simulations
*Cloud Layers Unified by Bi-Normals
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Improved understanding and new modeling capabilities:• Aerosol-ice cloud interactions (e.g., black carbon as ice nuclei);
• Double-moment aerosol/cloud microphysics;
• Aerosols (e.g., black carbon and dust) on snow;
•
Aerosol-vegetation-biogeochemistry coupling (e.g., dust andwild fires);
• Chemistry-climate interactions (e.g., methane lifetime);
• Improvement of radiative transfer parameterization (e.g., water
continuum);
• More unified and physically sound cloud and convective
parameterizations (e.g., CLUBB coupled with double-moment
cloud microphysics).
8/16/2019 Aerosols Chemistry Clouds and Radiation
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,?F?R"=<? AE A9? 7-**\: 7].8 CE"F:
•
Our process-oriented research generates1) mechanistic understanding of existing
model biases and uncertainties,
2) new modeling capabilities that enhance the
realism of regional climate and Earth
System simulation.
•
Both aspects are crucial for developing the
next-generation GFDL Earth System Model, anessential tool for advancing NOAA’s climate
adaptation and mitigation goal.
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